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1.
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2.
The atmospheric concentration of peroxyacetylnitrate (PAN) was measured during a cruise of the R.S. Polarstern from Bremerhaven (Germany) to Rio Grande do Sul (Brazil) in September/ October 1988. The measurements were made in-situ by a combination of electron capture gaschromatography with a cryogenic preconcentration step. The theoretical lower limit of detection (3) was 0.4 ppt. The mixing ratios of PAN varied by more than three orders of magnitude from 2000 ppt in the English Channel to less than 0.4 ppt south of the Azores (38° N). South of 35° N, PAN levels were below the detection limit, except at 30–31° S off the eastern coast of South America. Here, PAN mixing ratios of 10 to 100 ppt were detected in continentally influenced air masses. Detectable levels of PAN were mostly observed in air masses of continental or high northern origin. Changes in the wind directions were usually associated with substantial changes in the PAN mixing ratios.  相似文献   

3.
Springtime measurements of NOx, ozone, PAN,J(NO2), and other compounds were made near Ny-Ålesund,Svalbard (78°54N, 11°53E), in 1994 and Poker Flat,Alaska (65°08N, 147°29W), in 1995. At Svalbard medianmixing ratios for PAN and NOx of 237 and 23.7 pptv,respectively, were observed. The median mixing ratios at Poker Flat for PANand NOx were 79.5 and 85.9 pptv, respectively. These data areused to estimate thermal PAN decomposition using several differentapproaches. At Svalbard PAN decomposition was very small, while at PokerFlat up to 30 pptv/h PAN decomposed. At both sites the NOx/PANratio increased with temperature between –10 and 20°C implyingthat PAN decomposition is an important NOx source. In-situozone production was calculated from the measured NO, NO2,O3, J(NO2), and temperature data, using thesteady state assumption Median ozone production was 605 pptv/h at PokerFlat, and one order of magnitude smaller at Svalbard during the daytime.Only at Poker Flat could a direct influence on the diurnal ozone cycle beobserved from in-situ production. These results imply that PAN decompositionis a major source of NOx in the high latitude troposphere, andthat this contributes to the observed spring maximum in surface ozone.  相似文献   

4.
Measurement of ocean temperature and salinity via microwave radiometry   总被引：4，自引：0，他引：4  
Sea-surface temperature with an accuracy of 1 °C and salinity with an accuracy of 1 were measured with a 1.43 and 2.65 GHz radiometer system after correcting for the influence of cosmic radiation, intervening atmosphere, sea-surface roughness, and antenna beamwidth. The radiometers are a third-generation system using null-balancing and feed-back noise injection. Flight measurements from aircraft over bay regions and coastal areas of the Atlantic resulted in contour maps with spatial resolution of 0.5 km.  相似文献   

5.
Temperature above the surface layer   总被引：1，自引：0，他引：1  
Three published data sets of upper-air global temperatures, two from radiosondes and one from satellites, are examined and compared for the lower stratosphere and troposphere.The global lower stratosphere exhibits a downward trend for the past 16+ years of -0.53 °C (-0.33 °C per decade). Since the 1960's (using radiosondes before 1979 which are subject to known and unknown inhomogeneities) it is likely that there has been a downward trend of about the same magnitude. Significant issues of the stratospheric radiosonde data are: (1) that the long-term time series is biased toward spurious cooling; and (2) the earliest years of Angell display unrealistic variability. Inhomogeneities in satellite data due to orbit drifting and instrument calibration are examined.The tropospheric temperature has shown a downward trend of -0.11 °C since 1979 (-0.07 °C per decade). Beginning in earlier years, (relying only on radiosonde data before 1979) the estimated warming trend since the late 1950's is +0.07 to +0.11 °C per decade.Tropospheric and surface temperature anomalies are compared. There is concern that the disproportionate representation of extratropical continents, with their high temperature variance, may bias any long term global surface trend toward a maximum-possible value than would be calculated had all regions (including those with much lower responsiveness) been monitored.  相似文献   

6.
In June 1991 the EFEDA-field experiment (ECHIVAL Field Experiment in a Desertification-Threatened Area) was carried out in the Spanish province Castilla-La Mancha, to improve the understanding of the interactions between the soil, the vegetation and the atmosphere.Here results of energy balance studies at the Barrax site are given, one of the three intensively studied experimental sites within Castilla-La Mancha. This area is characterized by a large fraction of irrigated fields (40%) while the remaining 60% was fallow land at the end of June 1991. The energy balances over these two characteristic land-use classes totally differ. While for the irrigated fields the evapotranspiration is dominant, for the non-irrigated fields the sensible and the soil heat fluxes dominate and the latent heat flux is nearly negligible.In order to achieve areally averaged turbulent fluxes, surface, SODAR and aircraft data have been used. Comparing the surface fluxes from all three facilities, it can be found that:The sensible heat flux estimation from SODAR (w-method) gives reliable results when a calibration of w is done with another independent system (e.g. aircraft).Aircraft measurements in conjunction with energy budget methods yield surface fluxes of sensible heat, which are about 20% lower than the areally averaged values calculated by the surface measurements. The areally averaged latent heat fluxes from aircraft and surface measurements agree better than the sensible heat fluxes.  相似文献   

7.
Quantitative infrared measurements of ethane (C2H6) in the upper troposphere and lower stratosphere are reported. The results have been obtained from the analysis of absorption features of the 9 band at 12.2 m, which have been identified in high-resolution ballon-borne and aircraft solar absorption spectra. The ballon-borne spectral data were recorded at sunset with the 0.02 cm-1 resolution University of Denver interferometer system from a float altitude of 33.5 km near Alamogordo, New Mexico, on 23 March 1981. The aircraft spectra were recorded at sunset in July 1978 with a 0.06 cm-1 resolution interferometer aboard a jet aircraft at 12 km altitude, near 35°N, 96°W. The balloon analysis indicates the C2H6 mixing ratio decreased from 3.5 ppbv near 8.8 km to 0.91 ppbv near 12.1 km. The results are consistent with the colum value obtained from the aircraft data.  相似文献   

8.
Summary Two techniques for deriving horizontal and vertical air motions using vertically scanning airborne Doppler radar data are presented and discussed. These techniques make use of the scanning ability of the NOAA P-3 tail-mounted radar antenna to view a region of space from at least two vantage points during a straight-line flight track. The scanning methodology is termed the Fore/Aft Scanning Technique or FAST because the antenna is alternately scanning forward and then aft of the flight track. The major advantages of FAST over flying two quasi-orthogonal flight tracks with the antenna scanning normal to the flight track are that the data are collected in roughly half the time and the aircraft does not have to execute a right-angle turn. However, accuracy of the resulting wind field is compromised slightly because the beam intersection angle is reduced from 90° to about 50°. The reduction of area covered because of large drift angles is also discussed.A three-dimensional wind field can be constructed using the dual-Doppler equations from FAST data using the two radial velocity estimates and vertical integration of the continuity equation with a boundary condition of no vertical motion at cloud top and the Earth's surface. To keep errors in the calculated winds acceptably small, the elevation angles are typically restricted to ±45° from the horizontal to minimize contamination of the horizontal wind by terminal fallspeeds.A different, and perhaps more believable vertical velocity, can be derived using a second technique that utilizes two (or more) airborne Doppler radar equipped aircraft each using FAST to observe the echo-top vertical velocity at common point (e.g., two aircraft flying parallel flight, paths, or by using an L-shaped flight track with a single aircraft). This technique results in 4 (or more) radial velocity estimates at each point (hence is called the quad-Doppler technique). Horizontal winds can be derived using either an overdetermined three-equation solution or an overdetermined dual-Doppler solution, whichever is more accurate. For the calculation of vertical velocity a new approach is proposed that utilizes the overdetermined triple-Doppler solution for vertical particle motion near cloud top, minus an estimate of terminal fallspeeds, as a top boundary condition for the downward vertical divergence integration to derive vertical air velocity elsewhere in the domain. In addition, this approach allows measurements at steep elevation angles allowing for more depth of coverage for a given range.To show the utility of the method, analyses of data collected using FAST are compared to conventional dual-Doppler-derived wind fields constructed from data collected simultaneously by S-band ground-based Doppler radars. An example of the quad-Doppler technique is also presented from the recently completed Tropical Oceans/Global Atmospheres Coupled Ocean/Atmosphere Response Experiment (TOGA/COARE). Comparisons of quad-Doppler vertical velocity are made with in-situ derived vertical air motions collected by the NASA DC-8 to judge the quality of the approach.With 9 Figures  相似文献   

9.
In the first two weeks of May 1981, the research jet of the German Aerospace Research Establishment (DFVLR) was charted to fly a meridional section between 5° and 82°N. A scanning filter photometer, developed at the Max Planck Institut für Aeronomie to measure column content values of atmospheric ozone and nitrogen dioxide, using ultra violet and visible absorption techniques, constituted part of the experimental payload for this campaign that was called SIMOC. The vertical NO2 column content above the aircraft, flying at approximately 10 km, was found to decrease rapidly from 6.9×1015 molecules cm-2 to 2.5×1015 molecules cm-2 around 50°N and then to increase again north of 75°N. A sharp rise in the NO2 content was observed south of the subtropical jet but this could possibly be due to the increased depth of the troposphere above the aircraft in these regions.  相似文献   

10.
This is a report on the calibration tests and the determination of the response characteristics of a thrust anemometer designed to measure the three-dimensional instantaneous wind vector. Static tests determined the instrument calibration constants and checked the linearity of the system. Dynamic tests performed in a wind tunnel established that the V 2 drag law applies to the sensing system. The wind-tunnel tests also determined the range of angles for which the anemometer was capable of resolving the vector wind. Finally, the amplitude and phase frequency response characteristics were measured. It was found that knowledge of the latter was important in studying turbulence spectra and cross spectra. Some preliminary results from a recent field program are presented which document the need for correcting the amplitude and phase responses.  相似文献   

11.
A detector for the chemiluminescent measurement of NO in background air is described. A large reduction of interferences is achieved by using a stabilized ozone generator which allows operation of the instrument at lower O3 concentrations. Purification and humidification of the O3 stream further reduces interferences and shortens the instrumental clean-up time, which is important for aircraft missions. From a series of laboratory tests and from measurements performed aboard an aircraft it is demonstrated that the remaining interferences are acceptable for measurements in the undisturbed troposphere. In particular, no remnant NO signal is observed in clean air at night. During flight, a detection limit (2) of 20 ppt is achieved for a 1 min integration time.  相似文献   

12.
An instrument is described which is capable of making Eulerian measurements of microscale fluctuations in the static pressure when it is placed within the turbulent flow of the lower atmospheric boundary layer. The sampling ports are located on an accurately shaped streamlined circular disc; dynamic pressure changes at these ports, due to the flow fluctuations, are small when compared to the static pressure changes. Wind tunnel tests and anin situ test show that the instrument can sample the amplitudes and phases of fluctuations in the static pressure to better than ± 20% and to about ± 5 °, respectively.  相似文献   

13.
A calibration equation and some results of the field performance of an infrared instrument, which is designed to measure simultaneous fluctuations of atmospheric carbon dioxide and water vapor, are described. Field observations show that the instrument is suitable for simultaneous measurement of turbulent fluxes of carbon dioxide and water vapor in conjunction with a sonic anemometer. Measured values of carbon dioxide and water vapor fluxes show diurnal variations characterized by crop activity with respect to assimilation, respiration and evapotranspiration. Carbon dioxide is transferred downward during the daytime and upward at night, while latent heat and sensible heat are transferred in the opposite sense. The non-dimensional gradient of carbon dioxide is expressed in the following form under weak unstable conditions: c = (1 – 16 v )-1/2. Here, v is the Monin-Obukhov stability parameter including the humidity effect. This relation was originally proposed for temperature and humidity. Thus, the results indicate that the turbulent mechanisms of carbon dioxide fluctuations are similar to those of other scalar entities. This is strongly supported by the high correlation coefficient found between fluctuations of carbon dioxide and temperature or humidity in the air layer over crop fields.  相似文献   

14.
Summary A one dimensional analytical model of katabatic wind over the Antarctica has been developed. This parametric model is derived from the bulk two-layer model of Ball including the surface friction and taking into account the Earth's rotation and the geostrophic wind in the upper layer.This model is validated using the data set (70 soundings) collected during IAGO experiment at D47 (67°24S, 138°43E, altitude 1 564m), 110 km inland from the coast of Adélie Land.The parameteric model is then introduced into a GCM which is a spectral global version of the operational numerical weather prediction model used by the French weather service. The most significant effect of the parameterization is a 50 m increase of the geopotential height over the South Pole. The surface temperature at the South Pole increases (2°C) reducing the pole-midlatitude thermal gradient. The westerly circulation at 50° S is slowed down (4m/s at 850 hPa), and the surface pressure at the South Pole increases (4hPa). These results, consistent with an increase of katabatic winds, would however be improved by a better coupling between the parameterization and the GCM boundary layer.With 8 Figures  相似文献   

15.
A three-component sonic anemometer/thermometer system has been developed. It employs single switched transducer pairs and the inverse timed pulse method to yield an absolute calibration. Microprocessor control and use of newly developed transducers give a very small parts cost. The path length of the instrument can be varied from 10 to 15 cm; output is available in digital or analog form. Temperature sensing, via a 5 Μm tungsten resistance element, is integrated into the digital system. Wind tunnel and field results have confirmed the success of the prototype and a set of operational instruments has been constructed.  相似文献   

16.
A series of nearly daily ozone vertical profiles obtained at station T-3 on Fletcher's Ice Island (85°N, 90°W) during the period January-March 1971 shows several significant ozone intrusions into the troposphere. These intrusions are not only associated with enhanced ozone amounts in the stratosphere but also require tropopause folding events to transport ozone into the troposphere. These folds in the Arctic tropopause appear to be capable of contributing significantly to the ozone budget of the Arctic troposphere during the late winter and spring seasons. The importance of tropopause folding for bringing ozone into the troposphere seen in the daily ozone profiles confirms the results found in the Arctic Gas and Aerosol Sampling Program aircraft flights.  相似文献   

17.
Summary The objective of this study is to describe spatial and temporal patterns of sea-surface temperature (SST) variability in the Atlantic and Indian Oceans. The analysis domain extends from 40°S to 25°N and 50°W to 80°E, hence the tropical and most of the South Atlantic and central and western Indian Oceans. The investigation, covering the years 1948 to 1979, utilizes the COADS marine data set. Empirical orthogonal functions and spectral analysis are used to analyze SST fields.A major finding of this investigation is that SSTs vary coherently throughout most of the analysis domain. The greatest coherence is evident from 10°N to 30°S in the Atlantic and from 20°N to 35°S in the western Indian Ocean. Spectral analysis of regional time series shows that throughout this region the time scale of 5–6 years is the dominant one in the fluctuations; this is also the case for the Southern Oscillation and for equatorial rainfall. SST variations are roughly in-phase within each ocean and the two oceans are roughly in-phase with each other, i.e., the lags which exist are much smaller than the dominant time scale of the fluctuations. The SST anomalies appear to propagate eastward from NE Brazil; the eastern Atlantic lags the western by two to six months and the Indian Ocean lags the western Atlantic by four to eight months.With 15 Figures  相似文献   

18.
This paper presents a new reconstruction of the mean annual temperature obtained from a high altitude pollen sequence in equatorial Africa (3°28S, 29°34E, 2240 m). It has been achieved with an extended modern African reference data set by adding spectra from 228 new sites and using another selection for pollen taxa. The purpose of this paper is to test how the obtained temperature value depends upon the availability of modern analogues. The results are in good agreement with those previously published, reinforcing the validity of the method. The mean standard error is reduced by 0.3°C. The mean temperature for the Holocene appears + 1.4°C warmer than the present and the last glacial maximum (25-18 kyrs BP) cooling is better specified at – 3 ± 1.9° C, a conservative value, more consistent with reconstructed sea surface temperature in the equatorial ocean.Contribution to Clima Locarno - Past and Present Climate Dynamics; Conference September 1990, Swiss Academy of Sciences — National Climate Program  相似文献   

19.
Daily and zonal (latitudinal belt) averages of heat and momentum fluxes were computed using bulk aerodynamic formulae, from the meteorological parameters measured onboard M. S. Thuleland during the sixth Indian scientific expedition to Antarctica (26th November, 1986 to 22nd March, 1987). Both estimates showed significant variations, the momentum flux showing the largest variation. The maximum values of sensible and latent heat fluxes were observed over the 30°–40° S and 10°–20° S zones during the southern summer and fall respectively while the minimum values of latent heat flux were observed in the 60°–70° S zone for both seasons. The sensible heat flux minimum was observed in the 50°°60° S and 60°–70° S zones for summer and fall, respectively. Higher momentum flux values over the 40°–50° S zone in summer shifted to the 50°–60° S zone during fall.  相似文献   

20.
Summary The seasonal and diurnal variations in the vertical component of the atmospheric electric field, air temperature, relative humidity and horizontal wind speed were studied using the surface data for the two periods (1936–40) and (1962–66) recorded at the tropical urban station, Colaba, Bombay (18°51N, 72°49E, 11 m ASL), located on the west coast of India.The atmospheric electric field during the latter period (1962–66) is significantly higher (up to 42.3%) than the earlier period (1936–40). This has been attributed to the enhanced particulate concentrations in the atmosphere. The increase noticed in the atmospheric electric field is a maximum during winter and minimum during the monsoon. The atmospheric electric field exhibited a marked semi-diurnal oscillation with peaks at 0900 LST and 2200 LST during winter, premonsoon and post-monsoon seasons of both the periods. During the monsoon season the double oscillation is not marked.The variations noticed in the surface air temperature and the relative humidity are in agreement with those observed in the atmospheric electric field. The horizontal wind speed showed a decrease which has been attributed to the surface roughness resulting from urbanization.With 7 Figures  相似文献   

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