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1.
In order to study energy and water cycles in the Huaihe River Basin, micrometeorological measurements were carried out in Shouxian County, Anhui Province, during HUBEX/IOP (May to August 1998 and June to July 1999). The employed techniques included Bowen Ratio-Energy Balance (BREB) and Eddy Covariance (EC) methods. In this paper, the basic characteristics of the energy balance components in the district are analyzed. Furthermore, the results are compared with those from other regions of China.The main results are as follows: (1) There was a consistency between the available energy (Rn-G) and the sum of sensible (H) and latent (E) heat fluxes measured by the EC method (H+E)ec, but Ebr was slightly larger (about 10%) than Eec; (2) Most of the net radiation (Rn) was used to evaporate water from the surface. During HUBEX/IOP in 1998 and 1999, the mean daily amounts of Rn were 13.89 MJ m-2 d-1 and 11.83 MJ m-2 d-1, and the mean Bowen Ratios (β) were 0.14 (over ruderal) and 0.06 (over paddy) respectively; (3) The diurnal variation characteristic of β was larger and unsteady at sunrise and sunset, and smaller and steady during the rest of the daytime. Local advection appeared in the afternoon over paddy areas in 1999; (4) In comparison with the results from other regions of China, the nean β was the lowest (0.06) over paddy areas in the Huaihe River Basin and the highest (0.57) during June-August 1998 in Inner Mongolia grassland. The Bowen Ratio β is mainly related to the soil humidity.  相似文献   

2.
The characteristics of net radiation (Rn)(0.3--10 μm) in Lhasa and Haibei in the Tibetan Plateau were analyzed based on long-term in-situ measurements of surface radiation data. The monthly average of daily Rn reached a minimum during the winter period followed by an increase until May and then a decline until January. This variation is consistent with solar activity. The annual mean daily total Rn values were 0.92 MJ m-2 d-1 and 0.66 MJ m-2d-1 in Lhasa and Haibei, respectively. A relationship between Rn and broadband solar radiation (Rs) was demonstrated by a good linear correlation at the two sites. Rn can be an accurate estimate from Rs. The estimated Rn values were similar to the observed values, and the relative deviations between the estimates and measurements of Rn were 2.8% and 3.8% in Lhasa and Haibei, respectively. The application of the Rn estimating model to other locations showed that it could provide acceptable estimated Rn values from the Rs data. Furthermore, we analyzed the influence of clouds on Rn by different clear index (Ks), defined as the ratio of Rs to the extraterrestrial solar irradiance on a horizontal surface. The results indicate that more accurate results are associated with increased cloudy conditions. The influence of the albedo was also considered, but its inclusion in the model resulted in only a slight improvement. Because surface albedo is not usually measured, an expression based solely on global solar radiation could be of more extensive use.  相似文献   

3.
The soil C balance is determined by the difference between inputs (e.g., plant litter, organic amendments, depositional C) and outputs (e.g., soil respiration, dissolved organic C leaching, and eroded C). There is a need to improve our understanding of whether soil erosion is a sink or a source of atmospheric CO2. The objective of this paper is to discover the long-term influence of soil erosion on the C cycle of managed watersheds near Coshocton, OH. We hypothesize that the amount of eroded C that is deposited in or out of a watershed compares in magnitude to the soil C changes induced via microbial respiration. We applied the erosion productivity impact calculator (EPIC) model to evaluate the role of erosion–deposition processes on the C balance of three small watersheds (∼1 ha). Experimental records from the USDA North Appalachian Experimental Watershed facility north of Coshocton, OH were used in the study. Soils are predominantly silt loam and have developed from loess-like deposits over residual bedrock. Management practices in the three watersheds have changed over time. Currently, watershed 118 (W118) is under a corn (Zea mays L.)–soybean (Glycine max [L.] Merr.) no till rotation, W128 is under conventional till continuous corn, and W188 is under no till continuous corn. Simulations of a comprehensive set of ecosystem processes including plant growth, runoff, and water erosion were used to quantify sediment C yields. A simulated sediment C yield of 43 ± 22 kg C ha−1 year−1 compared favorably against the observed 31 ± 12 kg C ha−1 year−1 in W118. EPIC overestimated the soil C stock in the top 30-cm soil depth in W118 by 21% of the measured value (36.8 Mg C ha−1). Simulations of soil C stocks in the other two watersheds (42.3 Mg C ha−1 in W128 and 50.4 Mg C ha−1 in W188) were off by <1 Mg C ha−1. Simulated eroded C re-deposited inside (30–212 kg C ha−1 year−1) or outside (73–179 kg C ha−1 year−1) watershed boundaries compared in magnitude to a simulated soil C sequestration rate of 225 kg C ha−1 year−1 and to literature values. An analysis of net ecosystem carbon balance revealed that the watershed currently under a plow till system (W128) was a source of C to the atmosphere while the watersheds currently under a no till system (W118 and W188) behaved as C sinks of atmospheric CO2. Our results demonstrate a clear need for documenting and modeling the proportion of eroded soil C that is transported outside watershed boundaries and the proportion that evolves as CO2 to the atmosphere.  相似文献   

4.
The chemical composition, as well as the sources contributing to rainwater chemistry have been determined at Skukuza, in the Kruger National Park, South Africa. Major inorganic and organic ions were determined in 93 rainwater samples collected using an automated wet-only sampler from July 1999 to June 2002. The results indicate that the rain is acidic and the averaged precipitation pH was 4.72. This acidity results from a mixture of mineral acids (82%, of which 50% is H2SO4) and organic acids (18%). Most of the H2SO4 component can be attributed to the emissions of sulphur dioxide from the industrial region on the Highveld. The wet deposition of S and N is 5.9 kgS⋅ha−1⋅yr−1 and 2.8 kgN⋅ha−1⋅yr−1, respectively. The N deposition was mainly in the form of NH4 +. Terrigenous, sea salt component, nitrogenous and anthropogenic pollutants have been identified as potential sources of chemical components in rainwater. The results are compared to observations from other African regions.  相似文献   

5.
Increased precipitation during the vegetation periods was observed in and further predicted for Inner Mongolia. The changes in the associated soil moisture may affect the biosphere-atmosphere exchange of greenhouse gases. Therefore, we set up an irrigation experiment with one watered （W） and one unwatered plot （UW） at a winter-grazed Leymus chinensis-steppe site in the Xilin River catchment, Inner Mongolia. UW only received the natural precipitation of 2005 （129 mm）, whereas W was additionally watered after the precipitation data of 1998 （in total 427 mm）. In the 3-hour resolution, we determined nitrous oxide （N20）, methane （CH4） and carbon dioxide （CO2） fluxes at both plots between May and September 2005, using a fully automated, chamber-based measuring system. N20 fluxes in the steppe were very low, with mean emissions （±s.e.） of 0.9-4-0.5 and 0.7-4-0.5 μg N m^-2 h^-1 at W and UW, respectively. The steppe soil always served as a CH4 sink, with mean fluxes of -24.1-4-3.9 and -31.1-4- 5.3 μg C m^-2 h^-1 at W and UW. Nighttime mean CO2 emissions were 82.6±8.7 and 26.3±1.7 mg C m^-2 h^-1 at W and UW, respectively, coinciding with an almost doubled aboveground plant biomass at W. Our results indicate that the ecosystem CO2 respiration responded sensitively to increased water input during the vegetation period, whereas the effects on CH4 and N2O fluxes were weak, most likely due to the high evapotranspiration and the lack of substrate for N2O producing processes. Based on our results, we hypothesize that with the gradual increase of summertime precipitation in Inner Mongolia, ecosystem CO2 respiration will be enhanced and CH4 uptake by the steppe soils will be lightly inhibited.  相似文献   

6.
常煜  樊斌  张小东 《气象科学》2018,38(2):229-236
利用1991—2015年夏季(6—8月)内蒙古地区111个国家气象站小时降水量资料,对内蒙古不同气候区(极干旱、干旱、半干旱、半湿润和湿润)短时强降水(1 h降水量≥20 mm)进行检验分析,采用累积概率方法定义内蒙古夏季不同气候区短时强降水。检验结果表明:内蒙古地区年平均降水量和小时降水量极值自西部极干旱区向东部半湿润、湿润区递增,高值区位于大兴安岭东部,次高值区位于阴山山脉以南。内蒙古极干旱区小时降水量极值低于20 mm,半湿润区和湿润区小时降水量极值高于50 mm,个别站点甚至达到100 mm以上。但在半湿润区和湿润区东部小时降水量超过20 mm年平均发生仅为1次,其余地区均1次。在内蒙古极干旱区、干旱区、半干旱区、半湿润区和湿润区小时降水量分别达到6.1、9.8、12.5、15.2和14.3 mm·h~(-1)属于极端降水事件,小时降水量≥20 mm不宜作为内蒙古短时强降水定义。综合上述研究,结合内蒙古地区地形、地貌等因素,将内蒙古极干旱区和干旱区短时强降水定义为5 mm·h~(-1),半干旱区、半湿润区和湿润区短时强降水定义为10 mm·h~(-1)。  相似文献   

7.
The results of one year’s monitoring in Srednja Bijambarska Cave (Bosnia and Herzegovina) are presented and discussed. Temporal variations of the carbon dioxide (CO2) concentration are controlled by the switching between two ventilation regimes driven by outside temperature changes. A regression model with a simple perfectly mixed volume applied to a cave sector (“Music hall”) resulted in an estimate of ventilation rates between 0.02 h−1 and 0.54 h−1. Carbon dioxide input per plan surface unit is estimated by the model at around 50 × 10−6 mh−1 during the winter season and up to more than 1000 × 10−6 mh−1 during the first temperature falls at the end of summer (0.62 μmoles m−2 s−1 and 12.40 μmoles m−2 s−1 for normal conditions respectively). These values have been found to be related to the cave ventilation rate and dependent on the availability of CO2 in the surrounding environment. For airflow close to zero the values of CO2 input per plan surface have a range in the order of magnitude of a few units × 10−6 mh−1. Based on two experiments, the anthropogenic contribution from cave visitors has been calculated, at between 0.35 lCO2 min−1 person−1 and 0.45 lCO2min−1person−1.  相似文献   

8.
The dynamics of terrestrial ecosystems depends on interactions between carbon, nutrient and hydrological cycles. Terrestrial ecosystems retain carbon in live biomass (aboveground and belowground), decomposing organic matter, and soil. Carbon is exchanged naturally between these systems and the atmosphere through photosynthesis, respiration, decomposition, and combustion. Human activities change carbon stock in these pools and exchanges between them and the atmosphere through land-use, land-use change, and forestry.In the present study we estimated the wood (stem) biomass, growing stock (GS) and carbon stock of Indian forests for 1984 and 1994. The forest area, wood biomass, GS, and carbon stock were 63.86 Mha, 4327.99 Mm3, 2398.19 Mt and 1085.06 Mt respectively in 1984 and with the reduction in forest area, 63.34 Mha, in 1994, wood biomass (2395.12 Mt) and carbon stock (1083.69 Mt) also reduced subsequently. The Conifers, of temperate region, stocked maximum carbon in their woods, 28.88 to 65.21 t C ha−1, followed by Mangrove forests, 28.24 t C ha−1, Dipterocarp forests, 28.00 t C ha−1, and Shorea robusta forests, 24.07 t C ha−1. Boswellia serrata, with 0.22 Mha forest area, stocked only 3.91 t C ha−1. To have an idea of rate of carbon loss the negative changes (loss of forest area) in forest area occurred during 1984–1994 (10yrs) and 1991–1994 (4yrs) were also estimated. In India, land-use changes and fuelwood requirements are the main cause of negative change. Total 24.75 Mt C was lost during 1984–1994 and 21.35 Mt C during 1991–94 at a rate of 2.48 Mt C yr−1 and 5.35 Mt C yr−1 respectively. While in other parts of India negative change is due to multiple reasons like fuelwood, extraction of non-wood forest products (NWFPs), illicit felling etc., but in the northeastern region of the country shifting cultivation is the only reason for deforestation. Decrease in forest area due to shifting cultivation accounts for 23.0% of the total deforestation in India, with an annual loss of 0.93 Mt C yr−1.  相似文献   

9.
A three-step methodology to assess the carbon sequestration and the environmental impact of afforestation projects in the framework of the Flexible Mechanisms of the Kyoto Protocol (Joint Implementation and Clean Development Mechanism) was developed and tested using a dataset collected from the Jonkershoek forest plantation, Western Cape, South Africa, which was established with Pinus radiata in former native fynbos vegetation and indigenous forest. The impact of a change in land use was evaluated for a multifunctional, a production and a non-conversion scenario. First, the carbon balance was modelled with GORCAM and was expressed as (1) C sequestration in tC ha−1 year−1 in soil, litter, and living biomass according to the rules of the first commitment period of the Kyoto Protocol, and (2) CO2 emission reductions in tC ha−1 year−1, which includes carbon sequestered in the above-mentioned pools and additionally in wood products, as well as emission reductions due to fossil fuel substitution. To estimate forest growth, three data sources were used: (1) inventory data, (2) growth simulation with a process-based model, and (3) yield tables. Second, the effects of land use change were assessed for different project scenarios using a method related to Life Cycle Assessment (LCA). The method uses 17 quantitative indicators to describe the impact of project activities on water, soil, vegetation cover and biodiversity. Indicator scores were calculated by comparing indicator values with reference values, estimated for the climax vegetation. The climax vegetation is the site-specific ecosystem phase with the highest exergy content and the highest exergy flow dissipation capacity. Third, the land use impact per functional unit of 1 tC sequestered was calculated by combining the results of step 1 and step 2. The average baselines to obtain carbon additionality are 476 tC ha−1 for indigenous forest and 32 tC ha−1 for fynbos. Results show that the influence of the growth assessment method on the magnitude of C sequestration and hence on the environmental impact per functional unit is large. When growth rate is assessed with the mechanistic model and with the yield table, it is overestimated in the early years and underestimated in the long term. The main conclusion of the scenario analysis is that the production forest scenario causes higher impacts per functional unit than the multifunctional scenario, but with the latter being less efficient in avoiding CO2 emissions. The proposed method to assess impacts on diverse components of the ecosystem is able to estimate the general tendency of the adverse and positive effects of each scenario. However, some indicators, more specifically about biodiversity and water balance, could be improved or reinterpreted in light of specific local data about threat to biodiversity and water status.  相似文献   

10.
Based on data obtained during the Hualhe River Basin Experiment （HUBEX） in 1999, this study intends to detect the quantitative discrepancies in the momentum （τ0）, sensible heat （H0） and latent heat （E0） fluxes among six sets of similarity functions with the aerodynamic method. It also aims to clarify the applicability of the functions under stable conditions. The relative discrepancy was studied with the normalized transfer coefficients for τ0, H0 and E0, namely CD, CH and CQ, respectively. Except for one set of functions that adopted a rather small von Kármán＇s constant （0.365）, the relative discrepancy in τ0 among the other functions was less than 10%, while that in H0（E0） sometimes reached 25% when the bulk Richardson number （R/B） was less than 0.07. The absolute discrepancy in the fluxes was studied with statistical computations. Among the six sets of functions, the discrepancy in τ0, H0 and E0 sometimes reached 0.03 kg m^-1 s^-2, 4 W m^-2 and 10 W m^-2, respectively, and the discrepancy in the energy balance ratio sometimes exceeded 0.1. Furthermore, when RiB exceeded the critical value （Ric） for a specific set of functions, no fluxes could be derived with the functions. It is therefore suggested that RiB be compared with Ric before computing the fluxes if RiB is less than Ric. Finally, two sets of nonlinear similarity functions are recommended, due to their unlimited applicability in terms of RiB.  相似文献   

11.
Summary This paper characterizes Mesoscale Convective Systems (MCSs) during 2001 over Iberia and the Balearic Islands and their meteorological settings. Enhanced infrared Meteosat imagery has been used to detect their occurrence over the Western Mediterranean region between June and December 2001 according to satellite-defined criteria based on the MCS physical characteristics. Twelve MCSs have been identified. The results show that the occurrence of 2001 MCSs is limited to the August–October period, with September being the most active period. They tend to develop during the late afternoon or early night, with preferred eastern Iberian coast locations and eastward migrations. A cloud shield area of 50.000 km2 is rarely exceeded. When our results are compared with previous studies, it is possible to assert that though 2001 MCS activity was moderate, the convective season was substantially less prolonged than usual, with shorter MCS life cycles and higher average speeds. The average MCS precipitation rate was 3.3 mm·h−1 but a wide range of values varying from scarce precipitation to intense events of 130 mm·24 h−1 (6 September) were collected. The results suggest that, during 2001, MCS rainfall was the principal source of precipitation in the Mediterranean region during the convective season, but its impact varied according to the location. Synoptic analysis based on NCEP/NCAR reanalysis show that several common precursors could be identified over the Western Mediterranean Sea when the 2001 MCSs occurred: a low-level tongue of moist air and precipitable water (PW) exceeding 25 mm through the southern portion of the Western Mediterranean area, low-level zonal warm advection over 2 °C·24 h−1 towards eastern Iberia, a modest 1000–850 hPa equivalent potential temperature (θe) difference over 20 °C located close to the eastern Iberian coast, a mid level trough (sometimes a cut-off low) over Northern Africa or Southern Spain and high levels geostrophic vorticity advection exceeding 12·10−10 s−2 over eastern Iberia and Northern Africa. Finally, the results suggest that synoptic, orographic and a warm-air advection were the most relevant forcing mechanisms during 2001.  相似文献   

12.
Janicot and Sultan (Geophys Res Lett 28(3):523–526, 2001) and Sultan et al. (J Clim 16(21):3389–3406, 2003) showed evidence of an intraseasonal signal of Sahelian rainfall corresponding to wet and dry sequences of the West African Monsoon. Using NCEP/NCAR reanalysis, NOAA outgoing longwave radiation (OLR) and observed daily rainfall over West Africa from 1968 to 1990, this paper investigates the variability of 3 to 5-day African Easterly Waves (AEWs), convection and their relationship with rainfall in these wet and dry sequences. The mean daily value rainfall during wet sequences is twice the mean value during dry sequences but the number of dry or wet sequences per year is not correlated with the annual rainfall. Wet sequences account for 39% of the annual accumulated rainfall while dry sequences account for 22%. The number of 3 to 5-day AEWs increases during wet years in wet sequences and the activity tends to be larger during wet years in both wet and dry sequences. These AEWs explain 40% of the accumulated rainfall during wet sequences whereas they contribute to 26% of the accumulated rainfall observed during dry sequences. Generally, they contribute to the increase of rainfall during these sequences. Mean convection is stronger and there are twice as many low OLR days (<225W/m2) during wet than dry sequences. The mean rainfall for days with high convective activity (convective days) is also twice as great during wet sequences. Rainfall that occurs during days without low OLR (weak convection with warm cloud tops or isolated deep convection) contributes to 69% of the total rainfall during dry sequences and 45% during wet sequences. A composite study was performed from day D 0−10 to day D 0+10 in each sequence. Wet (dry) sequences of the African monsoon start with a decrease (slight increase) of the negative meridional Ertel Potential Vorticity (PV) gradient at 700 hPa, associated with an increase (decrease) of the spectral density of AEWs. During the wet sequence, the African Easterly Jet (AEJ), detected by 700 hPa zonal wind, decreases and moves northward, whereas the Tropical Easterly Jet (TEJ), detected at 200 hPa, increases and shifts southward. Convective activity increases from D 0−6 to D 0−3 and remains high for 4 days in wet sequences. The daily rainfall increases (decreases) between D 0−6 and D 0 and returns to the mean value at D 0+4 for wet (dry) sequences.  相似文献   

13.
Previous measurements of urban energy balances generally have been limited to densely built, central city sites and older suburban locations with mature tree canopies that are higher than the height of the buildings. In contrast, few data are available for the extensive, open vegetated types typical of low-density residential areas that have been newly converted from rural land use. We made direct measurements of surface energy fluxes using the eddy-covariance technique at Greenwood, a recently developed exurban neighbourhood near Kansas City, Missouri, USA, during an intensive field campaign in August 2004. Energy partitioning was dominated by the latent heat flux under both cloudy and near clear-sky conditions. The mean daytime Bowen ratio (β) values were 0.46, 0.48, and 0.47 respectively for the cloudy, near clear-sky and all-sky conditions. Net radiation (R n ) increased rapidly from dawn (−34 and −58W m−2) during the night to reach a maximum (423 and 630W m−2) after midday for cloudy and near clear-sky conditions respectively. Mean daytime values were 253 and 370W m−2, respectively for the cloudy and near clear-sky conditions, while mean daily values were 114 for cloudy and 171W m−2 for near clear-sky conditions, respectively. Midday surface albedo values were 0.25 and 0.24 for the cloudy and near clear-sky conditions, respectively. The site exhibited an angular dependence on the solar elevation angle, in contrast to previous observations over urban and suburban areas, but similar to vegetated surfaces. The latent heat flux (Q E ), sensible heat flux (Q H ), and the residual heat storage ΔQ s terms accounted for between 46–58%, 21–23%, and 18–31% of R n , respectively, for all-sky conditions and time averages. The observed albedo, R n , and Q E values are higher than the values that have been reported for suburban areas with high summer evapotranspiration rates in North America. These results suggest that the rapidly growing residential areas at the exurban fringe of large metropolitan areas have a surface energy balance that is more similar to the rural areas from which they were developed than it is to the older suburbs and city centres that make up the urban fabric to which they are being joined.  相似文献   

14.
Information related to rainfall erosivity in the Andes is scarce. This study was carried out to determine the characteristics of rainfall events at the La Encañada watershed, northern Peru, using daily rainfall data from the 1995 to 2000 period that included all the El Niño and Southern Oscillation (ENSO) phases. Three weather stations were installed within the study area, at the top, middle and bottom of the watershed. We analysed the total amount, duration, intensity, kinetic energy and probability of return of rainfall events. In general, 80% of the rainfall events at watershed level had an average rainfall intensity lower than 2.5 mm h?1 and only 4% had an average intensity larger than 7.5 mm h?1. Rainfall erosivity registered at the bottom of the watershed was slightly higher than in the rest of the area. The highest intensities were observed during an El Niño year whereas a La Niña year was characterized by the highest amount of total rainfall compared to the other ENSO phases and by the low intensity rain events. Simulations using the WEPP model estimated higher sediment yield and runoff for the bottom of the watershed during a La Niña year versus El Niño or Neutral years. Even when the analysed rainfall data was too limited to conclude erosion and runoff during any ENSO phase, the simulated results showed us the trend of the behaviour of rainfall erosivity under the ENSO phases at different locations.  相似文献   

15.
Using a single drop experiment, the uptake of NO3 radicals on aqueous solutions of the dye Alizarin Red S and NaCl was measured at 293 K. Uptake coefficients in the range (1.7–3.1) ⋅ 10− 3 were measured on Alizarin Red S solutions. The uptake coefficients measured on NaCl solutions were in the range of (1.1–2.0) ⋅ 10−3 depending on the salt concentration. Both experiments lead to a consistent result for the mass accommodation coefficient of αNO3 = (4.2− 1.7+2.2)⋅ 10−3. The product H(Dl kCl−II)0.5 for the NO3 radical was determined to be (1.9 ± 0.2) M atm− 1 cm s−0.5 M−0.5 s−0.5 by fitting the uptake data for the NaCl solutions to the so-called resistance model. The yield of the chemical NO3 radical source was characterized using UV-VIS and FT-IR spectroscopy. The amount of gas-phase NO3 radicals measured at elevated humidities was less than expected. Instead, a rise of the gas-phase HNO3 concentration was found indicating a conversion of gas-phase NO3 radicals to gas-phase HNO3 on the moist reactor walls.  相似文献   

16.
Aerosol and rain samples were collected between 48°N and 55°S during the KH-08-2 and MR08-06 cruises conducted over the North and South Pacific Ocean in 2008 and 2009, to estimate dry and wet deposition fluxes of atmospheric inorganic nitrogen (N). Inorganic N in aerosols was composed of ~68% NH4+ and ~32% NO3– (median values for all data), with ~81% and ~45% of each species being present on fine mode aerosol, respectively. Concentrations of NH4+ and NO3− in rainwater ranged from 1.7–55 μmol L−1 and 0.16–18 μmol L−1, respectively, accounting for ~87% by NH4+ and ~13% by NO3− of total inorganic N (median values for all data). A significant correlation (r = 0.74, p < 0.05, n = 10) between NH4+ and methanesulfonic acid (MSA) was found in rainwater samples collected over the South Pacific, whereas no significant correlations were found between NH4+ and MSA in rainwater collected over the subarctic (r = 0.42, p > 0.1, n = 6) and subtropical (r = 0.33, p > 0.5, n = 6) western North Pacific, suggesting that emissions of ammonia (NH3) by marine biological activity from the ocean could become a significant source of NH4+ over the South Pacific. While NO3− was the dominant inorganic N species in dry deposition, inorganic N supplied to surface waters by wet deposition was predominantly by NH4+ (42–99% of the wet deposition fluxes for total inorganic N). We estimated mean total (dry + wet) deposition fluxes of atmospheric total inorganic N in the Pacific Ocean to be 32–64 μmol m−2 d−1, with 66–99% of this by wet deposition, indicating that wet deposition plays a more important role in the supply of atmospheric inorganic N than dry deposition.  相似文献   

17.
A study of the oxidation mechanism of N-methyl pyrrolidinone (C5H9NO, NMP) initiated by hydroxyl radicals was made at EUPHORE at atmospheric pressure (1000 ± 10) mbar of air and ambient temperature (T = 300 ± 5 K). The main products were N-methyl succinimide (NMS) (52 ± 4)% and N-formyl pyrrolidinone (FP) (23 ± 9)%. The relative rate technique was used to determine the rate constants of OH with NMP, NMS and FP, the measured values were (in units of cm3 molecule − 1 s− 1): kNMP = (2.2 ± 0.4) × 10− 11, kNMS = (1.4 ± 0.3) × 10− 12 and kFP = (6 ± 1) × 10− 12. The results are presented and discussed in terms of the atmospheric impact.  相似文献   

18.
This study utilized the MM5 mesoscale model to simulate the landfalling process of Typhoon Talim. The simulated typhoon track, weather patterns, and rainfall process are consistent with the observation. Using the simulation results, the relation of the second type thermal helicity (H 2) to rainfall caused by the landfalling typhoon Talim was analyzed. The results show that H 2 could well indicate the heavy inland rainfall but it did not perform as well as the helicity in predicting rainfall during the beginning stage of the typhoon landfall. In particular, H 2 was highly correlated with rainfall of Talim at 1-h lead time. For 1–5-h lead time, it also had a higher correlation with rainfall than the helicity did, and thus showing a better potential in forecasting rainfall intensification. Further analyses have shown that when Talim was in the beginning stage of landfall, 1) the 850–200-hPa vertical wind shear around the Talim center was quite small (about 5 m s−1); 2) the highest rainfall was to the right of the Talim track and in the area with a 300-km radius around the Talim center, exhibiting no obvious relation to low-level temperature advection, low-level air convergence, and upper-level divergence; 3) the low-level relative vorticity reflected the rainfall change quite well, which was the main reason why helicity had a better performance than H 2 in this period. However, after Talim moved inland further, 1) it weakened gradually and was increasingly affected by the northern trough; 2) the vertical wind shear was enhanced as well; 3) the left side of the down vertical wind shear lay in the Lushan and Dabieshan mountain area, which could have contributed to triggering a secondary vertical circulation, helping to produce the heavy rainfall over there; hence, H 2 showed a better capacity to reflect the rainfall change during this stage.  相似文献   

19.
Summary  Net ecosystem CO2 exchange was measured over a mountain birch forest in northern Finland throughout the growing season. The maximal net CO2 uptake rate of about − 0.5 mg(CO2) m−2 s−1 was observed at the end of July. The highest nocturnal respiration rates in early August were 0.2 mg(CO2) m−2 s−1. The daily CO2 balances during the time of maximal photosynthesis were about −15 g(CO2) m−2 d−1. The mountain birch forest acted as a net sink of CO2 from 30 June to 28 August. During that period the net CO2 balance was −448 g(CO2)m−2. The interannual representativeness of the observed balances was studied using a simplified daily balance model, with daily mean global radiation and air temperature as the input parameters. The year-to-year variation in the phenological development was parameterised as a function of the cumulative effective temperature sum. The daily balance model was used for estimating the variability in the seasonal CO2 balances due to the timing of spring and meteorological factors. The sink term of CO2 in 1996 was lower than the 15-year mean, mainly due to the relatively late emergence of the leaves. Received October 11, 1999 Revised April 25, 2000  相似文献   

20.
1998年夏季HUBEX/GAME期间热量和水汽收支(英)   总被引：4，自引：0，他引：4  
By using the high-resolution GAME reanalysis data, the heat and moisture budgets during the period of HUBEX/GAME in the summer of 1998 are calculated for exploring the thermodynamic features of Meiyu over the Changjiang-Huaihe (CH) valley. During the CH Meiyu period, an intensive vertically-integrated heat source and moisture sink are predominant over the heavy rainfall area of the CH valley, accompanied by strong upward motion at 500 hPa. The heat and moisture budgets show that the main diabatic heating component is condensation latent heat released by rainfall. As residual terms, the evaporation and sensible heating are relatively small. Based on the vertical distribution of the heat source and moisture sink, the nature of the rainfall is mixed, in which the convective rainfall is dominant with a considerable percentage of continuous stratiform rainfall. There are similar time evolutions of the main physical parameters(〈Q1〉,〈Q2〉,and vertical motion ω at 500 hPa).The time variations of〈Q1〉and〈Q2〉are in phase with those of -ω500, and have their main peaks within the CH Meiyu period. This shows the influence of the heat source on the dynamic structure of the atmosphere. The wavelet analyses of those time series display similar multiple timescale characteristics. During the CH Meiyu period, both the synoptic scale(～6 days) and mesoscale (～2 days and ～12 hours) increase obviously and cause heavy rainfall as well as the appearances of the maxima of the main physical parameters. Among them, the mesoscale systems are the main factors.  相似文献   

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