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1.
The results of measurements of the CO content in the atmospheric thickness by the method of solar molecular-absorption spectroscopy are presented. Over 87 months of observations, the annual mean CO content decreased by ～19% at a mean rate of changes equal to ?(0.14 ± 0.02) atm cm per year. Maxima and minima of seasonal variations most often fall on February and September, respectively. The mean overall amplitude of changes in the CO content during the annual cycle is about 50% of the mean value. The Fourier analysis revealed variations in the CO composition with periods from 3 to 84 months. A simple statistical model satisfactorily describes time changes in the CO content in the atmospheric thickness. The results of measurements of the CO content in the atmospheric thickness are compared with the data of CO measurements in samples of surface air at stations of the Global Atmospheric Watch.  相似文献   

2.
Data on the volume concentration of carbon oxide (CO) in surface-air samples taken in European Russia, which were obtained using the Fourier transform spectroscopy method, are given. Over 16 years of measurements, this concentration decreased by 28%. These measured concentrations of CO are separated into its regional natural background and anthropogenic components. Seasonal variations in the concentration of CO are separated from its background concentration. Their extreme intra-annual values and mean amplitudes are determined. An empirical model of time variations in the concentration of CO is proposed. The atmospheric concentration of the CO anthropogenic component decreased by ~61 ppb over the measurement period.  相似文献   

3.
We describe the specific features of the summer 2010 emergency conditions in the European part of the Russian Federation, when an anomalous heat wave (the monthly mean temperatures in the summer months were 5–9°C higher than those for 2002–2009) and prolonged blocking anticyclones led to large wildfires. We analyze their causes and consequences. The features of the satellite system for operational fire monitoring (constructed at the Aerospace Scientific Center) and examples of its application in summer 2010 are presented. On the basis of the results of processing of satellite images of low (250–1000 m), medium (∼30–50 m), and high (∼6 m) resolutions, we found that the total area covered by fire from March to November of 2010 amounted to approximately 10.9 million hectares for the entire territory of the country and and 2.2 million hectares for its European part. Daily histograms of areas covered by fire in the summer months of 2010 were constructed. On the basis of these data and empirical models, we estimate the daily emissions of carbon monoxide (CO) from wildfires in the summer months of 2010 for the European part of Russia and Moscow oblast. On some days in August 2010, these emissions reached 15000–27000 t for the European part of Russia and 3000–7500 t for Moscow oblast. On the basis of analysis of data from the AIRS spectrometer (Aqua satellite), we derived the spatial distribution of CO concentrations at heights of 2 to 10 km above the territory of the Eastern and Central Europe. Moscow was shown to have been most severely affected by smoke from wildfires occurring on August 6–9, 2010, when the concentrations of harmful gases (CO2, CO, CH4, and O3) and aerosols in the air significantly exceeded both the daily and the one-hour maximum allowable concentrations.  相似文献   

4.
The results of measuring the methane content in the entire atmospheric thickness over the St. Petersburg region are given for 1991–2007. It is shown that, within this period, the mean annual cycle of the total methane content is characterized by its maximum values in December–January and its minimum values in June–August when the annual-cycle amplitude amounts to ∼3.6%. In this case, the annual variations in the total methane content may differ significantly from the mean annual cycle obtained in some years. A statistically significant linear trend of the total CH4 content has not been revealed for 1991–2007. The obtained values of the linear-trend index have opposite signs in the winter and summer months (positive for January 0.6 ± 0.2%/year and February 0.4 ± 0.2%/year and negative for July 0.3 ± 0.2%/year and August 0.2 ± 0.1%/year). This fact suggests the tendency for an increase in the amplitude of the annual cycle of the total CH4 content. The results of a spectral analysis of a series of data on the total CH4 content show that, for 1991–2007, the following harmonics are pronounced with a confidence of 95%: 12 months (annual harmonic), 32 months (quasi-biennial oscillations), and 55 months (4.5 years), which are also pronounced in the series of meteorological parameters and total ozone content.  相似文献   

5.
The results of measurements of surface ozone in central European Russia in 2004–2010 are presented. The variation coefficient for hourly, monthly, and annual mean ozone concentrations is 78, 26, and 12%, respectively. The measurements established a link between increased (>60 μg/m3) and minimum (<12 μg/m3) hourly mean ozone concentrations with the existence of a temperature inversion in the lower 300-m atmospheric layer. Sixty-seven percent of the total number of increased hourly mean ozone concentrations over the 2004–2010 period took place in 2010. A maximum hourly mean ozone concentration of 218.5 μg/m3 was recorded at 17:00 on August 1, 2010. The annual mean ozone concentration in a climatically significant range of hourly mean concentrations from 12 to 60 μg/m3 increased by 45% in a linear approximation over the period of record. The spectral analysis of monthly mean concentrations of surface ozone identified composite oscillations with periods from 3 to 60 months. To approximate the temporal dynamics of ozone, a statistical model was used. This model satisfactorily describes the experimental monthly and annual mean concentrations.  相似文献   

6.
Time-series measurements of dissolved inorganic carbon (DIC) and nutrient concentrations were conducted in the northwestern North Pacific from October 2002 to August 2004. Assuming that data obtained in different years represented time-series seasonal data for a single year, vertical distributions of DIC and nutrients showed large seasonal variabilities in the surface layer (∼100 m). Seasonal variabilities in normalized DIC (nDIC) and nitrate concentrations at the sea surface were estimated to be 81–113 μmol kg−1 and 12.7–15.7 μmol kg−1, respectively, in the Western Subarctic Gyre. The variability in nutrients between May and July was generally at least double that in other seasons. In the Western Subarctic Gyre, estimations based on statistical analyses revealed that seasonal new production was 39–61 gC m−2 and tended to be higher in the southwestern regions or coastal regions. The seasonal new productions in the northwestern North Pacific were two or more times higher than in the North Pacific subtropical gyre and the northeastern North Pacific. It is likely that this difference is due to spatial variations in the concentrations of trace metals and the species of phytoplankton present. In addition, from estimations of surface pCO2 it was verified that the Western Subarctic Gyre is a source of atmospheric CO2 between February and May and a sink for CO2 between July and October.  相似文献   

7.
The shell chemistry of Isognomon ephippium from three Kenyan sites (Tudor, Gazi and Mida) has been investigated to determine whether these bivalves record environmental parameters. The Mg, Sr, Ba and Mn distributions in the calcite shell layer were determined by using laser ablation-inductively coupled plasma-mass spectrometry (LA-ICP-MS). In addition, whole-shell analyses were made to evaluate inter-site differences. While some variability is observed for mean Mg concentrations, the mean Sr concentrations were similar for the three sites. The decreasing mean Ba and Mn concentrations, following the order Tudor > Gazi > Mida, are related to distinct regimes of freshwater and nutrient supply. The Mg profiles, determined by LA-ICP-MS, displayed a close to regular sinusoidal pattern, depending on specimen and sample site. For the Tudor shells, an arbitrary fitting of the Mg profiles to sea-surface temperature (SST) variations emphasised the good relationship between these two parameters and allowed for the calculation of mean annual growth rates. In most of the shells, Sr partly co-varied with Mg and Ba, highlighting the complexity of Sr incorporation. The Ba and Mn profiles of the Tudor shells displayed several sharp maxima. With a time scale deduced from the Mg–SST relationship, the Ba and Mn maxima of the Tudor shells closely followed periods of maximal rainfall associated with the southeast monsoon. These Ba and Mn maxima were tentatively associated with algal bloom events known to succeed these periods of high rainfall. The less clearly marked seasonality of the Ba and Mn maxima for the Gazi and Mida specimens is thought to result from weaker seasonal variations in nutrient supply and reduced nutrients inputs. This study highlights the potential of I. ephippium as a recorder of spatio-temporal environmental variations in tropical coastal ecosystems.  相似文献   

8.
We study the seasonal and interannual variations of the field of sea-surface temperature (SST) in the Southwest Atlantic on the basis of the analysis of three data arrays, namely, the Levitus-Boyer-1994 hydrological array, the WOD-98 actual database, and the data of satellite measurements of SST. We perform the comparative analysis of the amplitude-phase characteristics of the annual course of the SST field and discuss the distinctive features of its seasonal and interannual variations. It is shown that the results obtained by using different data arrays are in good agreement. The values of the coefficient of linear correlation are equal to 0.7–0.9. It is discovered that the maximum seasonal variations of SST are observed in the zone of confluence of the Falkland and Brasil Currents in the vicinities of the South Subtropical and Antarctic Polar fronts. The minimum seasonal variations are recorded in the Antarctic region and in the Weddell Sea. The satellite data demonstrate that the level of interannual variability is high in the zones of climatic fronts. __________ Translated from Morskoi Gidrofizicheskii Zhurnal, No. 5, pp. 62–76, September–October, 2006.  相似文献   

9.
The emissions from fires in the boreal zone of northern Eurasia significantly contribute to the global emissions of greenhouse gases, their precursors, and aerosols. These emissions are an important component of the global carbon balance, and they significantly affect both seasonal and long-term variations in the chemical composition and radiation properties of the atmosphere on both regional and global scales. The atmospheric emissions of carbon monoxide (CO) from biomass burning have systematically been estimated for the entire territory of northern Eurasia over the period of 2000–2008 on the basis of satellite (MODIS MCD45A1) data on burned vegetation and the Seiler-Crutzen emission model with consideration for both regional and seasonal features. On the whole, for Russia, the annual emissions of CO from biomass burning ranged from 10.6 to 88.2 Mt/y over the indicated period. Depending on fire activity, the atmospheric emissions of CO from natural fires and agricultural work may yield from 25 to 200% of the total technogenic emissions according to the EDGAR-2000 model. In this case, the dominant contribution is made by boreal forest fires (8–57 Mt/y), whose portion amounts to 63–76% of the total emissions from biomass burning. This relatively short observational series does not allow one to reliably estimate long-term variations; however, on the whole, a stable increase in burned areas has been observed in forest, steppe, and agricultural regions over the last decade. Our analysis suggests significant spatial and seasonal variations in the large-scale fields of fire emissions, which are determined by the physical, geographic, and climatic features of individual regions. The calculated fields of emissions can be used in transport-chemical models, studies of the regional transport and quality of air, and climate models.  相似文献   

10.
本文基于SWAN(Simulating Waves Nearshore)模式研究了2001～2016年石岛海浪有效波高的季节和年际变化特征,评估了不同区域风场对其贡献,并探讨了其与ENSO的关系。结果表明,石岛有效波高受黄海季风系统的影响呈现显著的季节变化:12月份最大, 6月份最小, 1%大波有效波高季节变化不显著。石岛有效波高年际变化信号显著,其与风速年际变化之间的关系存在季节性差异:石岛有效波高和石岛、黄海区域平均风速不同月份的年际异常分别在7、10月份相关性较高,而石岛1%大波有效波高和石岛、黄海区域平均1%大风风速不同月份的年际异常则在8月份左右相关性最高。不同区域风场对石岛有效波高场的影响也呈现了季节性差异:夏季,黄海南部区域风场对石岛海浪的贡献较大,而石岛风场的贡献较小;冬季,石岛风场的贡献较大。ENSO(El Ni?o-Southern Oscillation)事件会对石岛有效波高的年际变化产生一定的影响,但影响比较小。本研究旨在对石岛海浪在季节和年际尺度上的变化特征以及风场等影响因素进行研究,对该海域海浪场进行了详细的认识,对了解该海域海浪有重要意义。  相似文献   

11.
We study the regularities of annual variations in the concentration of oxygen and the degree of saturation of waters in the Sevastopol Bay with oxygen in 1998–2009. The three-dimensional specific features of seasonal variations in the distribution of oxygen in waters of the Sevastopol Bay are revealed. Two periods can be separated in the annual course of the content of oxygen in the surface layers of waters in all parts of the bay: the period of supersaturation in March–September and the period of undersaturation in October–February. In the bottom layer of waters in all parts of the bay, we observe the undersaturation of waters with oxygen for the whole year.  相似文献   

12.
The results of measuring the total contents of carbon monoxide and methane via the method of solar-absorption spectroscopy are presented. The measurements were performed at the Molodezhnaya Station in 1977–1978, at the Mirny Observatory from 1982 to 1992, and at the Novolazarevskaya Station from 2003 to 2006. The character of seasonal variations in the contents of these gases in the Antarctic atmosphere is described and compared to the intra-annual variation of their surface concentrations measured at the Syowa Station (Japan). Synchronous intra-annual variations in the contents of carbon monoxide in the atmospheric column and in its surface concentrations are observed, while the spring maximum content of methane is observed three months after the maximum of its surface concentration. Synchronous seasonal variations in the total content of methane and ozone are observed, which makes it possible to suggest that the Antarctic circumpolar vortex has a significant influence on the characteristics of the vertical distribution of methane during Antarctic spring. Quantitative estimates of the parameters of multiyear variations in the contents of CO and CH4 are given. The content of methane was increasing (although with different rates) during the entire observation period 1977–2006. The content of CO was observed to increase until 1992 and to decrease during 2003–2006.  相似文献   

13.
Statistical characteristics of variations in surface-layer concentrations of methane, non-methane and aromatic hydrocarbons, carbon dioxide, and formaldehyde are compared with the characteristics of variations in the concentration of carbon monoxide in the air basin of Moscow. Differences in the annual cycle of concentrations of methane, carbon dioxide, non-methane hydrocarbons, and carbon monoxide are determined. It is found that the maximum concentration of carbon monoxide at most sites with an elevated surface-air pollution level and over the city as a whole tends to occur in the summer season. The seasonal variability of the diurnal mean cycle of methane, carbon dioxide, and non-methane and aromatic hydrocarbons is analyzed.  相似文献   

14.
We present measurement data from February 1998 to January 2014 obtained by Fourier spectroscopy for bulk methane concentrations in surface air samples. We have excluded the results of individual measurements of high methane concentrations arising at a temperature inversion and during fires to separate the monthly mean concentrations into the regional natural background concentration of methane and its anthropogenic addition. A seasonal concentration has been separated from the background concentration. Spectral analysis reveals a large number of composite oscillations of variations in the background methane concentra- tion with periods of 3 to 126 months. A model with the use of empirical parameters of these oscillations describes the temporal changes in the methane concentration with an error of less than 3%. The anthropogenic addition of CH4 in the atmosphere is largely of a random character. Over 16 years of observations, its increase was ~23.7 ppb, which has resulted in an increase in the total CH4 concentration by the same amount.  相似文献   

15.
The analysis is performed on the basis of comparison of the hydrological characteristics of prestrait regions of the Sea of Marmara. It is shown that, in summer, the Black-Sea waters are weakly mixed with the Mediterranean waters and the levels of salinity in the prestrait regions differ by 0.6–0.9‰. In winter, the indicated difference increases and the level of salinity near the entrance of Dardanelles reaches 29‰ and exceeds the level observed near the entrance of Bosporus by 5.5‰. In the analyzed regions, we observe local temperature maxima and minima near the interface of two water masses. This is explained by the presence of strong seasonal variations of temperature for the Black-Sea waters and their absence for the Mediterranean waters. The physical mechanisms responsible for the seasonal variations of the intensity of transformations of the Black-Sea waters are discussed. __________ Translated from Morskoi Gidrofizicheskii Zhurnal, No. 2, pp. 49–55, March–April, 2007.  相似文献   

16.
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17.
The results of continuous minute measurements of the surface concentrations of ozone, nitric oxide, nitrogen dioxide, carbon monoxide, and sulfur dioxide during the 2002–2004 period at the environmental station of the Oboukhov Institute of Atmospheric Physics, Russian Academy of Sciences (IAP), and the Faculty of Geography, Moscow State University (MSU), are discussed. It is shown that the conditions of Moscow’s southwestern region remote from large local pollution sources reflect the general regularities of the variability of trace gases in an urban atmosphere. This is manifested in the mean annual value of the ratio NO/NO2 (a little less than 1), decreased daylight values of O3, increased values of the rest of the trace gases as compared to the background region, and the presence of a secondary nocturnal maximum in the diurnal cycle of O3. The features of the annual and diurnal cycles of the concentrations of the substances under analysis are discussed. In the diurnal cycle of the primary products of combustion (NO and CO), an excess of the morning maximum (over the evening one) is observed during both warm and transition periods and higher values of the night maximum (as compared to the daylight one) are noted for summer. The temperature stratification properties determined from the MSU long-term acoustic sounding data serve as a possible cause for both of the effects revealed. The annual cycle of the concentration of surface ozone is characterized by the highest values for spring and summer. The annual cycles of NO, NO2, CO, and SO2 do not demonstrate any obvious seasonal regularities. A significant seasonal variation of the ratio NO/NO2, which is associated with the oxidizing properties of the urban atmosphere, is revealed. The record high concentrations of trace gases in the atmosphere over Moscow are given, and the meteorological conditions for their accumulation are discussed.  相似文献   

18.
Contributions of climatically significant natural and anthropogenic emission sources in northern Eurasia to seasonal carbon monoxide (CO) variations observed at the Zotino Tall Tower Observatory (ZOTTO) in Central Siberia in 2007–2011 have quantitatively been estimated using the GEOS-Chem chemical transport model. It is shown that the formation of a stable continental pollution plume from sources in Western Europe, European Russia and southern Siberia during winter plays an important role in the regional balance of surface CO and allows one to explain 55–80% of the amplitude of the CO annual cycle observed at the ZOTTO station (~70–90 ppbv). During the warm period, the effect of the anthropogenic factor is weakly pronounced, and the background concentration of CO is regulated, first and foremost, by the oxidation of biogenic volatile organic compounds and fire activity in the region.  相似文献   

19.
The values and seasonal variations of the primary production and chlorophyll a content were investigated in the Russian sector of the Southeastern Baltic in 2003–2007. The annual average values of the primary production and chlorophyll content for this area were 231 gC m−2 year−1 and 2.9 mg/m3, respectively; i.e., they corresponded to the mesotrophic level according to the trophic classification. The spatial distribution of the primary production and the chlorophyll concentrations in the different seasons and the annual average increased values exhibited at the northern coast of the Sambian Peninsula and the Curonian Spit were determined. In these areas, the values of the primary production and the chlorophyll concentrations corresponded to the eutrophic level.  相似文献   

20.
 The oxidation and reduction that occur during early diagenesis of sediments has been studied in the interstitial waters of a rapidly accumulating sedimentary sequence from the Mediterranean margin of Spain. A series of reactions that are mediated by progressively lower free energy derived from oxidation of organic matter is evident in the sedimentary sequence. Iron and manganese are rapidly reduced. Phosphate and alkalinity maxima at a subbottom depth of 15 m indicate maximal organic matter degradation. Methane first appears at ∼20 m subbottom after sulfate is depleted, and its concentrations quickly climb. Received: 27 October 1997 / Revision received: 4 March 1998  相似文献   

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