Can channel banks be the dominant source of fine sediment in a UK river?: an example using 137Cs to interpret sediment yield and sediment source          下载免费PDF全文

Simon Pulley  Ian Foster 《地球表面变化过程与地形》2017,42(4):624-634

Cultivated fields have been shown to be the dominant sources of sediment in almost all investigated UK catchments, typically contributing 85 to 95% of sediment inputs. As a result, most catchment management strategies are directed towards mitigating these sediment inputs. However, in many regions of the UK such as the Nene basin there is a paucity of sediment provenance data. This study used the caesium‐137 (¹³⁷Cs) inventories of lake and floodplain cores as well as the ¹³⁷Cs activities of present day sediment to determine sediment provenance. Sediment yields were also reconstructed in a small lake catchment. Low ¹³⁷Cs inventories were present in the lake and floodplain cores in comparison to the reference inventory and inventories in cores from other UK catchments. Caesium‐137 activities in the present day sediments were low; falling close to those found in the channel bank catchment samples. It was estimated that 60 to 100% of the sediment in the Nene originated from channel banks. Pre‐1963 sediment yields were approximately 11.2 t km^?2 yr^?1 and post‐1963 was approximately 11.9 t km^?2 yr^?1. The lack of increased sediment yield post‐1963 and low sediment yield is unusual for a UK catchment (where a yield of 28 to 51 t km^?2 yr^?1 is typical for a lowland agricultural catchment), but is explained by the low predicted contribution of sediment from agricultural topsoils. The high channel bank contribution is likely caused by the river being starved of sediment from topsoils, increasing its capacity to entrain bank material. The good agreement between the results derived using cores and recently transported sediments, highlight the reliability of ¹³⁷Cs when tracing sediment sources. However, care should be taken to assess the potential impacts of sediment particle size, sediment focusing in lakes and the possible remobilization of ¹³⁷Cs from sedimentary deposits. Copyright © 2016 John Wiley & Sons, Ltd.  相似文献   

Gamma emitting fission products in surface sediments of the Ravenglass estuary     

S.R Aston  D.A Stanners 《Marine pollution bulletin》1982,13(4):135-138

The occurrence of some fission products from the Sellafield (formerly Windscale) nuclear fuel reprocessing facility has been determined for surface sediments from forty locations in the Ravenglass estuary, North-west England. The influence of the silt-sized fraction in the sediments on the geographic distribution of ¹³⁷Cs is clearly important, and to a lesser extent also influences the distributions of ¹⁰⁶Ru, ${}^{134}\text{Cs}\text{+}{}^{95}\text{Zr}\text{Nb}$ and ¹⁴⁴Ce. The data are compared with recently published results reported by the Ministry of Agriculture, Fisheries and Food for a monitoring site in this estuary.  相似文献   

Selected trace metals (As,Cd and Hg) distribution and contamination in the coastal wetland sediment of the northern Beibu Gulf,South China Sea     

Huayang Gan  Jinqin Lin  Kai Liang  Zhen Xia 《Marine pollution bulletin》2013,66(1-2):252-258

Contamination with As, Cd and Hg, their spatial and temporal distribution are reported from the coastal wetland sediments of the northern Beibu Gulf, South China Sea. The content of As, Cd, Hg and TOC in surface sediments is 8.1 ± 5.8 μg g^?1, 0.08 ± 0.14 μg g^?1, 0.034 ± 0.028 μg g^?1 and 0.45 ± 0.39%, respectively. The mean sedimentation rates are 0.93–1.37 cm year^?1 during 1920s to 2008 determined by ²¹⁰Pb and ¹³⁷Cs dating in three cores. The vertical profiles of As, Cd and Hg content in the cores retrieved from Qin and Nanliu River estuaries show increasing trends during 1985–2008 due to anthropogenic impact caused by local economic development. Locally the surface sediments have potential ecological risk of As to benthos according to the NOAA sediment quality guidelines.  相似文献   

The impact of typhoons on sediment connectivity: lessons learnt from contaminated coastal catchments of the Fukushima Prefecture (Japan)   总被引：1，自引：0，他引：1       下载免费PDF全文

Caroline Chartin  Olivier Evrard  J. Patrick Laceby  Yuichi Onda  Catherine Ottlé  Irène Lefèvre  Olivier Cerdan 《地球表面变化过程与地形》2017,42(2):306-317

Sediment connectivity characterizes the physical transfer of sediment through different geomorphic compartments in catchments due to sediment detachment, transport and deposition. Quantifying and modelling sediment connectivity is therefore a key prerequisite to improving our understanding of the dispersion of particle‐borne contaminants, especially in catchments exposed to highly erosive climates. The objective of this study is to provide novel insights into typhoon impacts on sediment connectivity from hillslopes to rivers. The dispersion of particle‐bound caesium‐137 (¹³⁷Cs) was investigated in two coastal catchments draining the main contamination plume from the Fukushima Daiichi Nuclear Power Plant accident. Five sampling campaigns were carried out from November 2011 to November 2015, after each typhoon season. The spatial and temporal evolution of ¹³⁷Cs contamination was investigated through the calculation of ¹³⁷Cs enrichment ratios in sediment relative to nearby soils. Rainfall erosivity (EI₃₀) associated with the main typhoons that occurred prior to each sampling campaign were computed, mapped, and finally used to improve a topographic‐based index of connectivity. From 2011 to 2015, mean contamination levels in Mano and Niida catchments decreased from 11.9 kBq kg^?1 to 3.3 kBq kg^?1 and from 34.1 kBq kg^?1 to 8.0 kBq kg^?1, respectively. Regional mean EI₃₀ ranged from 262 MJ mm ha^?1 h^?1 for typhoon Jelawat (in 2012) to 1695 MJ mm ha^?1 h^?1 for typhoon Roke (in 2011). Typhoons Roke (2011) and Etau (2015) showed the highest connectivity from contaminated sources to the rivers, and induced a significant export of sediment to the ocean. In 2013 a slight increase in ¹³⁷Cs levels in river sediments occurred, likely resulting from initial decontamination works and the occurrence of two consecutive typhoons. Importantly, this research provides new insights into the connectivity of the main sources of sediments contaminated with radiocaesium in Fukushima Prefecture and their temporal evolution, which will help with ongoing decontamination efforts. Copyright © 2016 John Wiley & Sons, Ltd.  相似文献   

Radioactivity in sediments of the Great Lakes: Post-depositional redistribution by deposit-feeding organisms     

J.A. Robbins  J.R. Krezoski  S.C. Mozley 《Earth and Planetary Science Letters》1977,36(2):325-333

At two locations in southern Lake Huron (U.S.A.), twelve 35.5-cm diameter cores of fine-grained sediments were taken for comparison of the vertical distributions of²¹⁰Pb and falllout¹³⁷Cs with the distributions of benthic macroinvertebrates, mainly oligochaete worms (Tubificidae) and the amphipod,Pontoporeia affinis. Locations were selected on the basis of²¹⁰Pb distributions measured a year earlier which indicated contrasting depths of mixing of surface sediments. At one location the activity of²¹⁰Pb is uniform down to about 6 cm and 95% of total invertebrates occur within this zone; at the other location the zone of constant activity is only 3 cm deep but 90% of the invertebrates occur within it. Comparison of published tubificid defecation rates with sediment accumulation rates based on²¹⁰Pb shows that oligochaetes alone can account for mixing in one case while the effects of amphipods may be required in the case of shallower mixing. If mixing is represented as a diffusional process, eddy diffusion coefficients are at least 5.8 and 3.3 cm² yr^?1 at respective locations. In comparison with bioturbation, molecular diffusion is of minor importance in the post-depositional mobility of¹³⁷Cs. The necessity for introducing a diffusion coefficient varying continuously with depth is indicated by characteristics of the distribution of¹³⁷Cs. Biological reworking of near-surface sediments is an important process affecting radioactivity and chemical profiles in profundal deposits of this and probably other Great Lakes.  相似文献   

Floodplain sedimentation rates in an alpine watershed determined by radionuclide techniques     

Frederick M. Soster  Gerald Matisoff  Peter J. Whiting  William Fornes  Michael Ketterer  Scott Szechenyi 《地球表面变化过程与地形》2007,32(13):2038-2051

Vertical profiles of the activities of ¹³⁷Cs and ²¹⁰Pb were measured on floodplain sediment cores and upland soil cores along the Soda Butte Creek and the Yellowstone River to determine floodplain sedimentation rates. The position of mine tailings from a 1950 impoundment failure was used as a stratigraphic marker to estimate the sedimentation rates and to make comparisons with rates provided by radionuclide‐based methods. Mass accumulation (sedimentation) rates calculated from the position of the mine tailings ranged from 0·00 to 0·17 g cm^?2 yr^?1 and were in good agreement with sedimentation rates calculated from the inventories of ¹³⁷Cs and ²¹⁰Pb. Sedimentation rates calculated from the position of the ¹³⁷Cs peak generally overestimated the sedimentation rates, probably because of increased downward migration of ¹³⁷Cs caused by the low pH of water moving through the mine tailings or the high permeability of floodplain sediments relative to upland reference soils. This study demonstrates that the ¹³⁷Cs and ²¹⁰Pb inventory methods for determining sedimentation rates can be applied to an alpine floodplain where sedimentation events are episodic and where orographic effects on precipitation generate strong downstream gradients in the delivery of atmospheric radionuclides. Copyright © 2007 John Wiley & Sons, Ltd.  相似文献   

Distribution and content of different artifical radio nuclides in the water of the North Sea during the years 1977 to 1981 (complemented with some results from 1982 to 1984)     

Dr. Hans Kautsky 《Ocean Dynamics》1985,38(5):193-224

Summary The measured concentrations of¹³⁷Cs in the water of the North Sea gained during the years 1977 to 1982 largely confirm the results found in the preceding years (Fig. 1). After a distinct maximum in 1978 — brought about by a particularly strong influx during 1977 — the total quantity of¹³⁷Cs present in the North Sea has reced, to around half of these peak values by the year 1982 (Table 1).On the way from the Sellafield Works near the Irish Sea as far as into the North Sea, a strong shift of the¹³⁷Cs:⁹⁰Sr ratio in favour of the⁹⁰Sr can be observed.By following the temporal course of that ratio at different measurement points, a transport time can be deduced of around 3 years between the Sellafield Works and the Pentland Firth; a further year would be needed to reach into the southeastern North Sea.The ratio Cs:Sr furthermore permits, in the southeastern North Sea, a good distinction between the watermasses comming from the north into the North Sea with respect to those that come through the Channel from the South. These masses practically flow side by side until about the entrance to the Skagerrak.The vertical distribution of the¹³⁷Cs shows, as is to be expected, seasonally conditioned differences. However, effects also occur, which — on the basis of the data available to date — do not yet permit a clear explanation.The⁹⁰Sr, as well as the^239+240Pu, present in the North Sea show an analogous distribution scheme compared with that of the¹³⁷Cs. Their concentrations lie far below that of the¹³⁷Cs (⁹⁰Sr 17.5%;^239+240Pu 0.03%).Tritium, on the other hand — with essentially higher concentrations — shows a completely different distribution, because it is principly introduced via the freshwater flowing in from the land.

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Verteilung und Gehalt verschiedener künstlicher Radionuklide im Wasser der Nordsee in den Jahren 1977 bis 1981 (ergänzt durch einige Ergebnisse von 1982 bis 1984)

Zusammenfassung Die in den Jahren 1977 bis 1982 gewonnenen Meßdaten der Aktivitätskonzentrationen von¹³⁷Cs im Wasser der Nordsee bestätigen weitgehend die in den vorhergehenden Jahren gefundenen Ergebnisse (Fig. 1) Nach einem deutlichen Maximum im Jahre 1978 — hervorgerufen durch eine besonders starke Zufuhr im Jahre 1977 —ist die in der Nordsee insgesamt vorhandene Menge an¹³⁷Cs bis zum Jahre 1982 wieder auf rund die Hälfte zurückgegangen (Tab. 1).Auf dem Weg von den Sellafield Works an der Irischen See bis in die Nordsee ist eine starke Verschiebung des¹³⁷Cs:⁹⁰Sr Verhältnisses zugunsten des⁹⁰Sr zu beobachten.Aus dem zeitlichen Verlauf dieses Verhältnisses an verschiedenen Meßpunkten ergeben sich Transportzeiten zwischen den Sellafield Works und dem Pentland Firth von rund 3 Jahren; bis in die südöstliche Nordsee wird ein weiteres Jahr benötigt.Das Verhältnis Cs:Sr erlaubt außerdem in der südöstlichen Nordsee eine gute Unterscheidung der aus der Nordsee bzw. durch den Kanal von Süden kommenden Wassermassen, die praktisch nebeneinander her bis etwa zum Beginn des Skagerraks fließen.Die Vertikalverteilung des¹³⁷Cs zeigt, wie zu erwarten ist, jahreszeitlich bedingte Unterschiede. Es treten aber auch Effekte auf, die sich anhand der bisher vorliegenden Daten noch nicht eindeutig erklären lassen.Das in der Nordsee vorhandene⁹⁰Sr sowie das^239+240Pu zeigen ein analoges Verteilungsschema verglichen mit dem des¹³⁷Cs. Ihre Konzentrationen liegen weit unter der des¹³⁷Cs (⁹⁰Sr 17,5%,^239+240Pu 0,03%).Das Tritium zeigt bei wesentlich höheren Konzentrationen dagegen eine völlig andere Verteilung, da seine Hauptzufuhr im wesentlichen über das von Land her zufließende Süßwasser erfolgt.

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Distribution et teneur de differents radionucleides artificiels, dans les eaux de la Mer du Nord entre les années 1977 et 1981 (completes par quelques résultats de 1982 à 1984)

Résumé Les mesures de concentration du Césium 137 dans les eaux de la Mer du Nord, acquises entre les années 1977 et 1982, confirment largement les résultats obtenus au cours des années précédentes. Après un net maximum en 1978 — occassionné par un apport particulièrement fort en 1977 — la quantité totale de Césium 137 présent en Mer du Nord a régressé,jusqu'en 1982, aux alentours de la moitié de ces valeurs maximales.Il a pu être observé une modification importante du rapport Césium 137/Strontium 90, en faveur du Strontium 90, sur le trajet de Sellafield Works prés de la Mer d'Irlande jusqu'à la Mer du Nord.En suivant l'évolution temporelle de la valuer de ce rapport en différents points de mesure, on peut en déduire une durée de transport d'environ 3 ans entre Sellafield Works et Pentland Firth; une année supplémentaire est ensuite nécessaire pour pénétrer en Mer du Nord Sud-orientale.En Mer du Nord Sud-orientale, le rapport Césium/Strontium permet en outre d'effectuer une nette distinction entre les masses d'eau pénétrant respectivement par le Nord dans la Mer du Nord et celles pénétrant par le Sud et venant de la Manche. Ces masses d'eau s'écoulent pratiquement côte à côte jusqu'à l'entrée du Skagerrak.Comme l'on pouvait s'y attendre, la distribution verticale du Césium est différente suivant les saisons. Cependant il apparaît également des effects qui, sur la base des données disponibles à ce jour, ne s'expliquent pas encore clairement.Le Strontium 90 aussi bien que le Plutonium 239+240 présent dans la Mer du Nord, montrent une distribution comparable, analogue à celle du Césium 137. Leurs concentrations sont bien inférieures à celle du Césium 137 (Strontium 90 17,5%; Plutonium 239+240 0,03%).Le tritium d'autre part, — avec des concentrations significativement plus fortes —montre une distribution complètement différente, due principalement au fait qu'il est introduit par l'intermédiaire de l'écoulement d'eau douce provenant de la terre.

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Plutonium,radiocesium and radiocobalt in sediments of the Hudson River estuary     

C.R. Olsen  H.J. Simpson  R.M. Trier 《Earth and Planetary Science Letters》1981,55(3):377-392

Anthropogenic radionuclides have reached the Hudson estuary as global fallout from nuclear weapons testing and through local releases from commercial nuclear reactors. Significant activities of²³⁸Pu and^239,240Pu (fallout-derived),¹³⁴Cs and⁶⁰Co (reactor-released), and¹³⁷Cs (derived from both sources), have accumulated in the sediments throughout the estuary, with the primary zone of accumulation near the downstream end of the system in New York harbor. The estuary appears to have trapped nearly all of the^239,240Pu delivered as fallout, and consequently, ocean dumping of dredged harbor sediment is currently the primary means for the net transport of these nuclides to coastal waters. In contrast, only 10–30% of the¹³⁷Cs,¹³⁴Cs and⁶⁰Co delivered to the estuary have been retained on the fine particles which accumulate at a rapid rate in the harbor.The primary factors which have governed the distribution of anthropogenic radionuclides in Hudson sediments are: (1) spread of fine particles labeled with both fallout and reactor nuclides throughout the axis of the estuary, (2) differences in timing of the peak fallout years (1962–1964) and years of maximum reactor releases (1971–1972), (3) large variations in sediment accumulation rates, ranging from a few millimeters per year or less to many tens of centimeters per year, (4) appreciable desorption of¹³⁷Cs and¹³⁴Cs from particles at higher salinities, and (5) possible enhanced desorption of⁶⁰Co at higher salinities (relative to¹³⁴Cs and¹³⁷Cs) which may be associated with the release of reduced manganese from the harbor sediments.  相似文献   

Landscape‐scale controls on the spatial distribution of caesium 137: A study based on an airborne geophysical survey across Northern Ireland     

B. G. Rawlins  C. Scheib  D. Beamish  R. Webster  A. N. Tyler  M. E. Young 《地球表面变化过程与地形》2011,36(2):158-169

The spatial distribution of ¹³⁷Cs across the landscape and the processes controlling its redistribution are of interest because (i) ¹³⁷Cs has been widely used to quantify the movement of soil and sediments and (ii) substantial fallout of ¹³⁷Cs after the Chernobyl accident has led to contamination of foodstuffs in some places. A high‐resolution airborne geophysical radiometric survey of Northern Ireland has provided an opportunity to study the distribution and possible redistribution of ¹³⁷Cs. The ¹³⁷Cs activity (recorded at 1·2 million points) is distributed in a series of bands oriented approximately 160° and 115° clockwise from north. Geostatistical analysis of the data shows a strong, short‐range structure (correlation ranges between 0·6 and 8 km) in ¹³⁷Cs activity across the vast majority of the region; the spatial distribution shows association with a published, coarse‐scale depositional pattern of ¹³⁷Cs from Chernobyl. Two indices of land form derived from a digital elevation model, namely compound topographic index and the length–slope factor of the Revised Universal Soil Loss Equation, account for only 3% of the variance in ¹³⁷Cs activity. In contrast, soil type and land cover in combination (including their interaction) account for 20% of the variance. In areas that received moderate fallout from Chernobyl, soil type alone accounts for a substantial proportion of the spatially correlated ¹³⁷Cs activity. We attribute this to each soil type having a fairly uniform radiocaesium interception potential that differs from those of other soil types and that this potential controls the vertical migration of ¹³⁷Cs. Over the granitic Mourne Mountains there is a strong spatial cross‐correlation between ¹³⁷Cs activity and airborne estimates of soil potassium, suggesting that the latter provides a measure of the soil's radiocaesium interception potential; this is probably dominated by the quantity of the mineral illite. Copyright © 2010 John Wiley & Sons, Ltd. and British Geological Survey  相似文献   

¹³⁷Cs湖泊沉积年代学方法应用的局限——以Crawford湖为例   总被引：17，自引：5，他引：12  

项亮 《湖泊科学》1995,7(4):307-313

＾１３７Ｃｓ湖泊沉积年代学方法是测定现代湖泊沉积物沉积年代和沉积速率的重要同位素年代学方法之一。对加拿大Ｃｒａｗｆｏｒｄ湖采集的沉积孔柱内＾１３７Ｃｓ垂直分布的研究发现,该方法给出时的标有明显偏差。比较＾２１０Ｐｂ和纹层等年代方法的结果,其１９６３年时标蓄积峰值所在位置明显移向表层,而作为１９５４年时标的该核素出现蓄积的层位则远早于该年沉积物蓄积层位。研究还表明,孔柱中较高的间隙水含量、缺少足以吸  相似文献   

Effect of deposit feeders on migration of¹³⁷Cs in lake sediments     

John A. Robbins  Peter L. McCall  J. Berton Fisher  John R. Krezoski 《Earth and Planetary Science Letters》1979,42(2):277-287

Illite clay particles with adsorbed¹³⁷Cs were added as a submillimeter layer to the surface of silt-clay sediments contained in rectangular Plexiglas cells stored in a temperature-regulated aquarium, in order to trace the effect of the oligochaete, Tubifex tubifex, and the amphipod, Pontoporeia hoyi, on mass redistribution near the sediment-water interface. A well-collimated NaI gamma detector scanned each sediment column (～10 cm deep) at daily or weekly intervals for six months, depicting the time evolution of radioactivity with and without added benthos. In a cell with tubificids (～5 × 10⁴ m^?2), which feed below 3 cm and defecate on surface sediments, the labeled layer was buried at a rate of 0.052 ± 0.007 cm/day (20°C). When labeled particles entered the feeding zone,¹³⁷Cs reappeared in surface sediments creating a bimodal activity profile. In time, the activity tended toward a uniform distribution over the upper 6 cm, decreasing exponentially below to undetectable levels by 9 cm. In a cell with amphipods (～1.6 × 10⁴ m^?2) uniform activity developed rapidly (～17 days) down to a well-defined depth (1.5 cm). The mixing of sediments by Pontoporeia is described by a simple quantitative model of eddy diffusive mixing of sediment solids. The value of the diffusion coefficient, 4.4 cm²/yr (7°C) was computed from a least squares fit of theoretical to observed profile broadening over time. In a cell without benthos, small but measurable migration of¹³⁷Cs indicated an effective molecular diffusion coefficient of 0.02 cm²/yr.  相似文献   

Assessment of sediment yield in a small karst catchment by using ¹³⁷Cs tracer technique     

Dong-chun YAN  Xin-bao ZHANG  An-bang WEN  Xiu-bin HE  Yi LONG 《国际泥沙研究》2012,27(4):547-554

There is very thin soil layer in karst rocky desertification areas in Southwest China,sediment deposition and sediment yield in the karst area affects the development of vegetation greatly.In the present study,the ¹³⁷Cs technique was used to assess the rate of sediment deposition and sediment yield in a small karst catchment.The ¹³⁷Cs inventory within the depression varied between 800 m^-2 and 2,200 Bq m^-2,with the mean value of 1,500.1 Bq m^-2.The ¹³⁷Cs reference inventory at a nearby reference site was 805.9 Bq m^-2.It could be inferred to that sediment deposition had occurred in the catchment.The mean depth of sediments deposition in the depression was 6 cm and the deposition rate was approximately 0.13 cm yr^-1.The analysis of the topographic characteristics of the catchment revealed that the sediment deposition occurred mainly at the lower part of the small catchment.Although,there was a sinkhole in the depression,little sediment had drained out with runoff through the sinkhole,because the local people built ridges around the sinkholes for storing water.According to this,sediment yield rate in the small catchment was estimated to be approximately 19.25 to 27.5 t km^-2 yr^-1,and the extremely low sediment yield was maybe the main obstacle to vegetation restoration in karst rocky desertification areas.  相似文献   

Geochronological reconstruction of Cs transport from the Coruh river to the SE Black Sea: comparative assessment of radionuclide retention in the mountainous catchment area     

S. B. Gulin  G. G. Polikarpov  J. -M. Martin 《Continental Shelf Research》2003,23(17-19):1811

The deposition record of ¹³⁷Cs was traced in the SE Black Sea sediments adjacent to the Coruh river mouth in comparison with the earlier studied chronology of ¹³⁷Cs deposition in front of the Danube delta (NW Black Sea). In both cases, the ¹³⁷Cs profiles showed two subsurface peaks attributable to maximum fallout of ‘bomb’ and Chernobyl radionuclides. The Coruh profile revealed a larger contribution of ‘bomb’ ¹³⁷Cs in comparison with the Chernobyl input, suggesting different coverage of NW and SE Black Sea regions with the Chernobyl fallout. The ¹³⁷Cs-derived dating showed that maximum deposition of particulate bound ¹³⁷Cs in sediments adjacent to the Coruh river mouth was delayed for 14 yr relative to date of Chernobyl accident, reflecting a buffer effect of the watershed soils. This transit time is 3 times longer than in the Danube catchment area, indicating a difference in retention processes in these mountainous (Coruh) and lowland (Danube) river basins. The ¹³⁷Cs profile in Coruh sediments showed penetration of ¹³⁷Cs to much greater depth than would be expected from ¹³⁷Cs fallout chronology, suggesting the sediment mixing rate of 1.3 cm² yr⁻¹. This value was used to evaluate deposition chronology of ¹³⁷Cs, applying the model developed for pulse fallout case. Comparing the measured and modelled data has allowed differentiation of the flood-induced discharge of the ¹³⁷Cs-containing suspended matter and the slower transit of eroded soil particles from the contaminated catchment areas. The obtained results may be used for the prediction of period when the pollutants, deposited over the river basins, can reach the Black Sea.  相似文献   

Dating of sediments from Lake Zurich (Switzerland) with210Pb and137Cs     

H. N. Erten  H. R. von Gunten  E. Rössler  M. Sturm 《Aquatic Sciences - Research Across Boundaries》1985,47(1):5-11

²¹⁰Pb- and¹³⁷Cs-measurements, and varve counting have been used to date sediment cores from Lake Zurich (Switzerland). Two cores from different water depths were dated with²¹⁰Pb/²¹⁰Po and revealed sediment accumulation rates of (0.055±0.015) g·cm^?2·y^?1 and (0.09±0.03) g·cm^?2·y^?1, respectively. A comparable rate of (0.07±0.01) g·cm^?2·y^?1 has been obtained from¹³⁷Cs measurements. These rates were confirmed by annual layer (varve)-counts which lead to rates of 0.07 g·cm^?2·y^?1. Constant²¹⁰Pb activities were observed in the top 6 cm of the sediment cores. This constancy is generally explained in the literature by mixing processes caused by bioturbation and by distortion during coring operations of the uppermost water-rich fluffy sediments. However the distinct¹³⁷Cs-maxima and the regular and undisturbed varve lamination of the top sediment observed in the cores of Lake Zurich contradict this assumption. In addition, measurements of⁷Be at the water/sediment interaces proved complete sediment core recovery and mechanically undisturbed sediments. Remobilization processes are assumed to cause the observed constant²¹⁰Pb activities. Remobilization may also be the reason for an incomplete²¹⁰Pb inventory in the sediments which contain only about 50% of the fallout from atmosphere. The results of the²¹⁰Pb dating should therefore be considered with some care. If existent, varve counting represents the easiest and most reliable means for dating lake sediments.  相似文献   

Accumulation,solid partitioning and remobilisation of 99Tc in subtidal and intertidal sediments in the Irish Sea     

Paul Finegan  Luis León Vintró  Peter I. Mitchell  Dominique Boust  Aurélien Gouzy  Peter J. Kershaw  Julie A. Lucey 《Continental Shelf Research》2009,29(16):1995-2010

Recent studies have shown that accumulation of ⁹⁹Tc in seabed sediments labelled by authorised radioactive liquid discharges into the NE Irish Sea from the Sellafield reprocessing complex is greater than previously thought. In this paper, new data on ⁹⁹Tc concentration profiles in subtidal and intertidal sediments from the eastern and western Irish Sea are provided with a view to elucidating the processes responsible for the incorporation and retention of ⁹⁹Tc in the seabed. The data show that substantial amounts of ⁹⁹Tc have accumulated in the fine-grained subtidal sediments off the Cumbrian coast, particularly after increased releases from Sellafield following the commissioning of the Enhanced Actinide Removal Plant (EARP) in 1994. In all the cores taken in this area, ⁹⁹Tc has been found to be present to depths in excess of 30 cm. Analysis of ¹³⁷Cs and ²⁴¹Am profiles, together with other supporting geochemical data, show a high degree of homogenisation of the sediments down to these depths as a result of physical and biological processes, and confirm that incorporation of ⁹⁹Tc into the sediment compartment is actually the result of mixing and reworking, rather than active sediment accumulation. In contrast, active deposition of material transported from this mixed pool of sediment appears to be the dominant mechanism controlling ⁹⁹Tc profiles in intertidal areas close to the Sellafield discharge outfall.Data obtained from the analysis of subtidal sediment cores from the western Irish Sea mud basin suggest that similar mixing processes to those occurring in the subtidal sediments of the eastern Irish Sea are also active in this area. Time-series data on ⁹⁹Tc concentrations in surficial sediments from this basin, gathered in the period 1988–2004, inclusive, show a clear increase in concentrations, by a factor of ～2, between samples collected pre-EARP and post-EARP. The constancy of ⁹⁹Tc concentrations in surface sediments throughout the 1980s and the early-1990s suggests that little redissolution and export of ⁹⁹Tc occurred over this extended period. A similar observation applies to the post-EARP period, when concentrations remained relatively constant despite the reported steady decrease in ⁹⁹Tc concentrations in the overlying waters.This apparent lack of remobilisation is consistent with data from sequential extraction analyses, which indicate that the bulk of the ⁹⁹Tc is strongly bound to non-labile geochemical phases, with only a small proportion associated with exchangeable and acido-soluble phases. Further, these analyses show that ⁹⁹Tc is not associated with oxygen-sensitive and highly-reactive acid-volatile sulphides (AVS) to any significant extent.  相似文献   

Establishing a high-resolution surface sediment chronology with multiple dating methods – Testing 137Cs determination with Nurmijärvi clastic-biogenic varves     

《Quaternary Geochronology》2017

The uppermost 50 cm of sediments from the 23 m deep lacustrine basin of Nurmijärvi, a lake in south-central Finland, are composed of the clastic-biogenic type of varves. We use multiple dating methods to render a sediment chronology that is as precise and accurate as possible for future paleoenvironmental research on this high-fidelity sedimentary archive. The 250-year-long varve chronology contains a chronological error of ±2%, as estimated based on repeated varve counts. The varve-based chronology was verified with the vertical distribution of ¹³⁷Cs by comparing variations in the paleomagnetic relative declination of the surface sediments with instrumental observations and a calculated representation of declination features in Finland. A comparison of the sediment cesium content using two gamma counters, different sediment pretreatments, and normalization of the ¹³⁷Cs concentration with masses and accumulation rates of different sediment components revealed that the AD 1986 fallout peak from the Chernobyl accident is the dominant feature in the studied sediments, regardless of the sample pretreatment or normalizing procedure. The vertical distribution of the AD 1986 peak in sediments with clastic-biogenic varves is fairly narrow, thus providing an accurate age-depth marker for the recent deposits. However, the Nurmijärvi section also reveals a ca. 10-year-long period of catchment-to-basin ¹³⁷Cs mobilization and redeposition after the AD 1986 fallout, as well as significant downwards diffusion of the Chernobyl-derived cesium in the sediment. This study highlights the ways in which the quality of surface sediment chronology needs to be considered and secured prior to comparisons between paleoproxy records and instrumental observations.  相似文献   

Quantitative assessment of dissolved radiotracers in the English Channel: Sources, average impact of la Hague reprocessing plant and conservative behaviour (1983, 1986, 1988, 1994)     

P. Bailly du Bois  P. Guguniat 《Continental Shelf Research》1999,19(15-16)

Knowledge of long-term movements of water-masses in the English Channel has been substantially improved using hydrodynamic modelling coupled with radio-tracers studies; nevertheless, the precision of results so obtained is still largely dependent on measurement precision. New tools are now available to make more accurate determinations of radio-tracer distribution: (1) Repositioning of station locations at the same tide reference-time, giving a homogeneous spatial data set, coupled with the possibility of interpolating and quantifying the amounts of dissolved radioactivity flowing through the English Channel; (2) the first measurements of tritium (³H) in seawater on a large scale in the English Channel demonstrate that this fully conservative radionuclide is a clearly identifiable marker of industrial releases; (3) recent campaigns carried out during the FLUXMANCHE II CCE (1994) programme show the general distribution of dissolved radionuclides ¹³⁷Cs, ¹³⁴Cs, ⁶⁰Co, ¹²⁵Sb, ¹⁰⁶Ru and ³H in the English Channel and the Irish Sea; and (4) the re-utilisation of data from previous campaigns (1983, 1986, 1988) provides indications, at any given location in the English Channel, about the average dilution and distribution of releases derived from the La Hague reprocessing plant. Excesses and losses of radionuclides are now quantified with respect to known source terms; estimates of losses are provided for non-conservative radionuclides, while an excess of ¹³⁷Cs was observed in the English Channel during the period 1983–1994. This excess, which has the same order of magnitude as the quantities released from La Hague plant in the English Channel, could be explained by about 1% of the Sellafield reprocessing plant releases entering the Channel. These results confirm and give a more detailed picture of the previously known distribution of water masses in the English Channel. They lead to clear information about transit times and dilution at this scale, and provide directly comparable data for the validation of hydrodynamic models.  相似文献   

Elevated sedimentation in lake records linked to agricultural activities in the Ishikari River floodplain,northern Japan     

Young Sang Ahn  Futoshi Nakamura  Toshikazu Kizuka  Yugo Nakamura 《地球表面变化过程与地形》2009,34(12):1650-1660

The purpose of this study was to examine the historical change in sedimentation rates in lakes that have been impacted by river regulation and agricultural activities in the Ishikari River floodplain. We dated sediment cores using caesium‐137 (¹³⁷Cs) dating and tephrochronology, and we estimated sediment sources from ¹³⁷Cs concentrations in the topsoil of representative land covers. We found that, between 1739 and 1963, the distance between the lake and the main river channel and whether or not the lake was connected to the river affected the sedimentation rates. After 1963, agricultural drainage systems were established in the Ishikari River floodplain. The average sedimentation rate before and after the construction of drainage ditches varied between 1–66 and 87–301 mg cm^–2 a^–1, respectively. The increase in the sedimentation rate after 1963 was caused by the construction of a number of drainage networks, as well as extensive cultivation activity and/or fragmentation of the swamp buffers surrounding the lakes. The ¹³⁷Cs activities at the surfaces of the lake as well as the catchment‐derived ¹³⁷Cs contributions and ¹³⁷Cs inventory in the lake profiles were used to examine the sediment influx from the various drainage areas after the establishment of the drainage system. Our results indicate that the majority of the lake sediments were derived from cultivated areas, and therefore the catchment‐derived ¹³⁷Cs contribution in the lakes was strongly correlated with the sedimentation rate. The ¹³⁷Cs inventory across all of the lake profiles was also significantly greater than the atmospheric fallout. We identified a negative correlation between the ¹³⁷Cs lake profile inventory and the sedimentation rate. This is because the sediment originating from the drainage areas contained low ¹³⁷Cs concentrations, which diluted the overall concentration of ¹³⁷Cs in the lake sediment. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

The application of caesium‐137 measurements to investigate floodplain deposition in a large semi‐arid catchment in Queensland,Australia: a low‐fallout environment     

Kathryn J. Amos  Jacky C. Croke  Heiko Timmers  Philip N. Owens  Celia Thompson 《地球表面变化过程与地形》2009,34(4):515-529

Floodplains comprise geomorphologically important sources and sinks for sediments and associated pollutants, yet the sedimentology of large dryland floodplains is not well understood. Processes occurring on such floodplains are often difficult to observe, and techniques used to investigate smaller perennial floodplains are often not practical in these environments. This study assesses the utility of ¹³⁷Cs inventory and depth‐profile techniques for determining relative amounts of floodplain sedimentation in the Fitzroy River, northeastern Australia; a 143 000 km² semi‐arid river system. Caesium‐137 inventories were calculated for floodplain and reference location bulk soil cores collected from four sites. Depth profiles of ¹³⁷Cs concentration from each floodplain site and a reference location were recorded. The areal density of ¹³⁷Cs at reference locations ranged from 13 to 978 Bq m^–2 (0–1367 Bq m^–2 at the 95% confidence interval), and the mean value ± 2 (standard error of the mean) was 436 ± 264 Bq m^–2, similar to published data from other Southern Hemisphere locations. Floodplain inventories ranged from 68 to 1142 Bq m^–2 (0–1692 Bq m^–2 at the 95% confidence interval), essentially falling within the range of reference inventory values, thus preventing calculation of erosion or deposition. Depth‐profiles of ¹³⁷Cs concentration indicate erosion at one site and over 66 cm of deposition at another since 1954. Analysis of ^239+240Pu concentrations in a depositional core substantiated the interpretation made from ¹³⁷Cs data, and depict a more tightly constrained peak in concentration. Average annual deposition rates range from 0 to 15 mm. The similarity between floodplain and reference bulk inventories does not necessarily indicate a lack of erosion or deposition, due to low ¹³⁷Cs fallout in the region and associated high measurement uncertainties, and a likely influence of gully and bank eroded sediments with no or limited adsorbed ¹³⁷Cs. In this low‐fallout environment, detailed depth‐profile data are necessary for investigating sedimentation using ¹³⁷Cs. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

The Fate of Chernobyl137Cs in Lake Lugano     

J. Dominik  D. Span 《Aquatic Sciences - Research Across Boundaries》1992,54(3-4):238-254

A rapid removal of Chernobyl¹³⁷Cs from a number of large lakes has been previously reported. Our measurements of¹³⁷Cs in water, sediments and pore water in the mono- and meromictic basins of Lake Lugano (Lago di Lugano) reveal generally slower half-removal times of 1.2 and 6.7 yrs, respectively. In the seasonally anoxic southern basin, this is most probably related to an intensive recycling of¹³⁷Cs between water and sediments. In the permanently stratified northern basin the removal rate is much slower due to an important inventory build up in the deep anoxic part of the basin.  相似文献