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1.
A stochastic optimization model based on an adaptive feedback correction process and surrogate model uncertainty was proposed and applied for remediation strategy design at a dense non-aqueous phase liquids (DNAPL)-contaminated groundwater site. One hundred initial training samples were obtained using the Latin hypercube sampling method. A surrogate model of a multiphase flow simulation model was constructed based on these samples employing the self-adaptive particle swarm optimization kriging (SAPSOKRG) method. An optimization model was built, using the SAPSOKRG surrogate model as a constraint. Then, an adaptive feedback correction process was designed and applied to iteratively update the training samples, surrogate model, and optimization model. Results showed that the training samples, the surrogate model, and the optimization model were effectively ameliorated. However, the surrogate model is an approximation of the simulation model, and some degree of uncertainty exists even though the surrogate model was ameliorated. Therefore, residuals between the surrogate model and the simulation model were calculated, and an uncertainty analysis was conducted. Based on the uncertainty analysis results, a stochastic optimization model was constructed and solved to obtain optimal remediation strategies at different confidence levels (60, 70, 80, 90, 95%) and under different remediation objectives (average DNAPL removal rate ≥?70,?≥?75,?≥?80,?≥?85,?≥?90%). The optimization results demonstrated that the higher the confidence level and remediation objective, the more expensive was remediation. Therefore, decision makers can weigh remediation costs, confidence levels, and remediation objectives to make an informed choice. This also allows decision makers to determine the reliability of a selected strategy and provides a new tool for DNAPL-contaminated groundwater remediation design.  相似文献   

2.
This paper investigates numerical optimization of dense nonaqueous phase liquid (DNAPL) site remediation design considering effects of prediction and measurement uncertainty. Results are presented for a hypothetical problem involving remediation using thermal source reduction (TSR) and bioremediation with electron donor (ED) injection. Pump-and-treat is utilized as a backup measure if compliance criteria are not met. Remediation system design variables are optimized to minimize expected net present value (ENPV) cost. Adaptive criteria are assumed for real-time control of TSR and ED duration. Source zone dissolved concentration data enabled more reliable and lower cost operation of TSR than soil concentration data, but using both soil and dissolved data improved results sufficiently to more than offset the additional cost. Decisions to terminate remediation and monitoring or to initiate pump-and-treat are complicated by measurement noise. Simultaneous optimization of monitoring frequency, averaging period, and lookback periods to confirm decisions, in addition to remediation design variables, reduced ENPV cost. Results indicate that remediation design under conditions of uncertainty is affected by subtle interactions and tradeoffs between design variables, compliance rules, site characteristics, and uncertainty in model predictions and monitoring data. Optimized designs yielded cost savings of up to approximately 50% compared with a nonoptimized design based on common engineering practices. Significant improvements in accuracy and reductions in cost were achieved by recalibrating the model to data collected during remediation and re-optimizing design variables. Repeating this process periodically is advisable to minimize total costs and maximize reliability.  相似文献   

3.
We examine the effect of uncertainty due to limited information on the remediation design of a contaminated aquifer using the pump and treat method. The hydraulic conductivity and contaminant concentration distributions for a fictitious contaminated aquifer are generated assuming a limited number of sampling locations. Stochastic optimization with multiple realizations is used to account for aquifer uncertainty. The optimization process involves a genetic algorithm (GA). As the number of realizations increases, a greater extraction rate and more wells are needed. There was a total cost increase, but the optimal remediation designs became more reliable. Stochastic optimization analysis also determines the locations for extraction wells, the variation in extraction rates as a function of the change of well locations, and the reliability of the optimal designs. The number of realizations (stack number) that caused the design factors to converge could be determined. Effective stochastic optimization may be achieved by reducing computational resources. An increase in the variability of the conductivity distribution requires more extraction wells. Information about potential extraction wells can be used to prevent failure of the remediation task.  相似文献   

4.
Dense nonaqueous phase liquid (DNAPL) source areas containing chlorinated volatile organic compounds (cVOCs) such as trichloroethene (TCE) and perchloroethene (PCE) often give rise to significant dissolved plumes in groundwater, leading to the closure of downgradient water supply wells and creating vapor intrusion issues in buildings located above the plume. Hydraulic containment via pump‐and‐treat has often been implemented to limit migration but must continue indefinitely. Removal of the DNAPL source area by means such as in situ thermal remediation (ISTR) offers the potential to diminish or end the need for hydraulic containment if the associated dissolved plume attenuates sufficiently following source removal. A question often raised is whether this occurs or whether the back diffusion of contaminants from secondary sources such as low‐permeability lenses in the dissolved plume precludes it. The authors conducted DNAPL source removal using ISTR at dozens of sites. This paper presents a compilation of cases—10 separate DNAPL source areas at five project sites—where data indicate that the implementation of a thorough ISTR in a DNAPL source area can result in the attenuation of the associated dissolved plume, such that in several cases, long‐standing pump‐and‐treat systems could be turned off. Our findings contrast with recent assertions that aggressive source remediation may not be justifiable because dissolved plume concentrations will not decline sufficiently. We show that the application of ISTR can result in the thorough removal of the DNAPL source, effective diminution of dissolved plume groundwater concentrations, and achievement of drinking water standards.  相似文献   

5.
Air sparging was evaluated for remediation of tetrachloroethylene (PCE) present as dense nonaqueous phase liquid (DNAPL) in aquifers. A two-dimensional laboratory tank with a transparent front wall allowed for visual observation of DNAPL mobilization. A DNAPL zone 50 cm high was created, with a PCE pool accumulating on an aquitard. Detailed process control and analysis yielded accurate mass balances and insight into the mass-transfer limitations during air sparging. Initial PCE recovery rates were high, corresponding to fast removal of residual DNAPL within the zone influenced directly by air channels. The vadose zone DNAPL was removed within a few days, and the recovery in the extracted soil vapors decreased to low values. Increasing the sparge rate and pulsing the air injection led to improved mass recovery, as the pulsing induced water circulation and increased the DNAPL dissolution rate. Dissolved PCE concentrations both within and outside the zone of air channels were affected by the pulsing. Inside the sparge zone, aqueous concentrations decreased rapidly, matching the declining effluent PCE flux. Outside the sparge zone, PCE concentrations increased because highly contaminated water was pushed away from the air injection point. This overall circulation of water may lead to limited spreading of the contaminant, but accelerated the time-weighted average mass removal by 40% to 600%, depending on the aggressiveness of the pulsing. For field applications, pulsing with a daily or diurnal cycling time may increase the average mass removal rate, thus reducing the treatment time and saving in the order of 40% to 80% of the energy cost used to run the blowers. However, air sparging will always fail to remove DNAPL pools located below the sparge point because the air will rise upward from the top of a screen, unless very localized geological layers force the air to migrate horizontally. Unrecognized presence of DNAPL at chlorinated solvent sites residual and pools could potentially hamper success of air sparging cleanups, since the presence of small DNAPL pools, ganglia or droplets can greatly extend the treatment time.  相似文献   

6.
The comparison between two series of optimal remediation designs using deterministic and stochastic approaches showed a number of converging features. Limited sampling measurements in a supposed contaminated aquifer formed the hydraulic conductivity field and the initial concentration distribution used in the optimization process. The deterministic and stochastic approaches employed a single simulation–optimization method and a multiple realization approach, respectively. For both approaches, the optimization model made use of a genetic algorithm. In the deterministic approach, the total cost, extraction rate, and the number of wells used increase when the design must satisfy the intensified concentration constraint. Growing the stack size in the stochastic approach also brings about same effects. In particular, the change in the selection frequency of the used extraction wells, with increasing stack size, for the stochastic approach can indicate the locations of required additional wells in the deterministic approach due to the intensified constraints. These converging features between the two approaches reveal that a deterministic optimization approach with controlled constraints is achievable enough to design reliable remediation strategies, and the results of a stochastic optimization approach are readily available to real contaminated sites.  相似文献   

7.
Chang LC  Hsiao CT 《Ground water》2002,40(5):481-490
In time-varying ground water remediation, the lack of an optimal control algorithm to simultaneously consider fixed costs and time-varying operating costs makes it nearly impossible to obtain an optimal solution. This study presents a novel algorithm that integrates a genetic algorithm (GA) and constrained differential dynamic programming (CDDP) to solve this time-varying ground water remediation problem. A GA can easily incorporate the fixed costs associated with the installation of wells. However, using a GA to solve for time-varying policies would dramatically increase the computational resources required. Therefore, the CDDP is used to handle the subproblems associated with time-varying operating costs. A hypothetical case study that incorporates fixed and time-varying operating costs is presented to demonstrate the effectiveness of the proposed algorithm. Simulation results indicate that the fixed costs can significantly influence the number and locations of wells, and a notable total cost savings can be realized by applying the novel algorithm herein.  相似文献   

8.
DNAPL to LNAPL Transitions During Horizontal Cosolvent Flooding   总被引：1，自引：0，他引：1  
Cosolvent flooding is a technology with the potential to remove nonaqueous phase liquid (NAPL) sources from the subsurface. It can be used to initiate separate phase mobilization, which allows removal of NAPL within very few pore volumes. Mobilization may result in a sinking DNAPL bank during horizontal flooding of NAPLs denser than water. Reversal of phase density difference between aqueous and DNAPL phases could potentially avoid this downward migration of mobilized DNAPLs. We achieved phase density difference reversal and made DNAPLs float using two components in the cosolvent flooding solution. A low-density cosolvent partitions preferentially into the DNAPL and swells it, which causes a reduction in density of the DNAPL and reversal of the density difference between the NAPL and aqueous phases. A highdensity additive that remains in the aqueous phase allows the cosolvent flooding solution overall to have a density greater than that of water and permits control of the flooding instability. This study focused on tert-butanol as the swelling cosolvent and tetrachloroethylene as the contaminant. In batch tests with sucrose and glycerol as dense additives, phase density difference reversal occurred. To investigate the applicability of phase density difference reversal as a remediation technology, horizontal column and sandbox experiments were performed. These experiments demonstrated the occurrence of phase density difference reversal and effective remediation in horizontal cosolvent floods.  相似文献   

9.
The objective of in situ thermal treatment is typically to reduce the contaminant mass or average soil concentration below a specified value. Evaluation of whether the objective has been met is usually made by averaging soil concentrations from a limited number of soil samples. Results from several field sites indicate large performance uncertainty using this approach, even when the number of samples is large. We propose a method to estimate average soil concentration by fitting a log normal probability model to thermal mass recovery data. A statistical approach is presented for making termination decisions from mass recovery data, soil sample data, or both for an entire treatment volume or for subregions that explicitly considers estimation uncertainty which is coupled to a stochastic optimization algorithm to identify monitoring strategies to meet objectives with minimum expected cost. Early termination of heating in regions that reach cleanup targets sooner enables operating costs to be reduced while ensuring a high likelihood of meeting remediation objectives. Results for an example problem demonstrate that significant performance improvement and cost reductions can be achieved using this approach.  相似文献   

10.
We aim to determine the effects of agricultural factors input per hectare on wheat production, and to optimize the allocation of wheat production factors under three scenarios and in different operating modes. Data were collected from 204 farming households using a face-to-face questionnaire. The sampled farms were selected through a stratified random sampling technique. We find fertilizer cost, irrigation cost and machinery cost all positively and significantly affect the per-unit-area wheat production, indicating the labor cost is not the major driving factor on wheat yield increment. Multi-object optimization model is used to allocate the production factors per hectare. We find under the Business as usual (BAU) scenario, the irrigation cost per-hectare wheat production after optimization in 2014 grows at a rate of 24.31% and accounts for 14.9% of total input. Under the Cooperate Environmental Sustainability (CES) scenario, the fertilizer and pesticide costs after optimization drop significantly by 42.83% and 21.41%, respectively. Under the Rapid Benefit Growth (RBG) scenario, the irrigation cost after optimization increase by 2.56% and the fertilizer cost increases by 4.69% compared with the surveyed data. Comparison of optimized data among three operating modes shows that the labor costs at household farm and cooperative farm both increase significantly. Cooperative farms are more successful in production factor use efficiency and economic performance. In conclusion, wheat production at different operating modes could be improved so as to constitute more efficient and economic use of production factors.  相似文献   

11.
The design and the management of pump-and-treat (PAT) remediation systems for contaminated aquifers under uncertain hydrogeological settings and parameters often involve decisions that trade off cost optimality against reliability. Both design objectives can be improved by planning site characterization programs that reduce subsurface parameter uncertainty. However, the cost for subsurface investigation often weighs heavily upon the budget of the remedial action and must thus be taken into account in the trade-off analysis. In this paper, we develop a stochastic data-worth framework with the purpose of estimating the economic opportunity of subsurface investigation programs. Since the spatial distribution of hydraulic conductivity is most often the major source of uncertainty, we focus on the direct sampling of hydraulic conductivity at prescribed locations of the aquifer. The data worth of hydraulic conductivity measurements is estimated from the reduction of the overall management cost ensuing from the reduction in parameter uncertainty obtained from sampling. The overall cost is estimated as the expected value of the cost of installing and operating the PAT system plus penalties incurred due to violations of cleanup goals and constraints. The crucial point of the data-worth framework is represented by the so-called pre-posterior analysis. Here, the tradeoff between decreasing overall costs and increasing site-investigation budgets is assessed to determine a management strategy proposed on the basis of the information available at the start of remediation. The goal of the pre-posterior analysis is to indicate whether the proposed management strategy should be implemented as is, or re-designed on the basis of additional data collected with a particular site-investigation program. The study indicates that the value of information is ultimately related to the estimates of cleanup target violations and decision makers’ degree of risk-aversion.  相似文献   

12.
The influence of aquifer property correlation on multiphase fluid migration, entrapment and recovery was explored by incorporating correlated and uncorrelated porosity, permeability, and capillary pressure-saturation (Pc-Sat) parameter fields in a cross-sectional numerical multiphase flow model. Comparison of two-dimensional entrapped organic saturation distributions for a simulated tetrachloroethylene (PCE) spill in ensembles of aquifer realizations suggests that the degree of spatial correlation in Pc-Sat parameters exerts a controlling influence on dense nonaqueous phase liquid (DNAPL) spreading and redistribution in saturated aquifers. The predicted evolution of DNAPL source zones and resultant remediation efficiency under surfactant enhanced aquifer remediation (SEAR) also appear to be strongly influenced by the spatial correlation of aquifer parameters and multiphase flow constitutive relationships. Results for a limited number of realizations selected from each ensemble showed that removal of 60% to 99% of entrapped PCE could reduce dissolved contaminant concentration and mass flux by approximately two orders of magnitude under natural gradient conditions. Aqueous phase contaminant mass flux did not vary uniformly as a function of % DNAPL removed, however, and notable differences in behavior were observed for models incorporating correlated versus uncorrelated Pc-Sat and permeability fields. Although these results must be confirmed through analysis of additional realizations, it is likely that similar or larger differences between correlated and uncorrelated system behavior will be observed in aquifers with greater spatially variability than that of the nonuniform, homogeneous sand aquifer studied here. Funding for this research was provided by the United States Environmental Protection Agency, Great Lakes and Mid-Atlantic Center for Hazardous Substance Research under Grant No. R-825540, the Michigan Department of Environmental Quality under Contract No. Y80011, and the Strategic Environmental Research and Development Program under Project No. CU-1293. The content of this publication does not necessarily represent the views of these agencies and has not been subject to agency review.  相似文献   

13.
Dense nonaqueous phase liquids (DNAPLs) are immiscible fluids with a specific gravity greater than, water. When present, DNAPLs present a serious and long-term source of continued ground water and soil contamination (Pankow and Cherry 1996). Accurate characterization and delineation of DNAPL in the subsurface is critical for evaluating restoration potential and for remedy design at a site. However, obtaining accurate and definitive direct evidence of DNAPL is difficult. A field study was recently performed comparing several approaches to DNAPL characterization at a site where anecdotal and limited direct evidence of DNAPL exists. The techniques evaluated included a three-dimensional high-resolution seismic survey, field screening of soil cores with a flame ionization detector (FID)/organic vapor analyzer (OVA), hydrophobic (Sudan IV) dye-impregnated reactive FLUTe® (Flexible Liner Underground Technologies) liner material in combination with Rotasonic drill cores, centrifuged soil with Sudan IV dye, ultraviolet light (UV) fluorescence, a Geoprobe® Membrane Interface Probe (MIP®), and phase equilibrium partitioning evaluations based on laboratory analysis of soil samples. Sonic drilling provided reliable continuous cores from which minor soil structures could be evaluated and screened with an OVA, The screening provided reliable preliminary data for identifying likely DNAPL zones and for selecting samples for further analyses. The FLUTe liner material provided the primary direct evidence of the presence of DNAPL and reliable information on the thickness and nature of its occurrence (i.e., pooled or ganglia). The MIP system provided good information regarding the subsurface lithology and rapid identification and delineation of probable DNAPL areas. The three-dimensional seismic survey was of minimal benefit to this study, and the centrifuging of samples with Sudan IV dye and the use of UV fluorescence provided no benefit. Results of phase equilibrium partitioning concentration calculations for soil samples (to infer the presence of DNAPL) were in good agreement with the site screening data. Additionally, screening data compared well with previous ground water data and supported using 1% of the pure phase solubility limit of Freon 113 (2 mg/L) as an initial means to define the DNAPL study area. Based on the results of this study, the preferred approach for identifying and delineating DNAPL in the subsurface is to initially evaluate ground water data and define an area where dissolved concentrations of the target analyte(s) approach 1% of the pure phase solubility limit. Within this study area, the MIP device is used to more specifically identify areas and lithologic zones where DNAPL may have accumulated. Core samples (either Rotasonic or Geoprobe) are then collected from zones where MIP readings are indicative of the presence of DNAPL. Soil samples from the free-product portions of the core(s) are then submitted to a laboratory for positive analyte identification. Soil analyses are then combined with site-specific geotechnical information (i.e., fraction organic carbon, soil bulk density, and porosity) and equilibrium partitioning algorithms used to estimate concentrations of organic contaminants in soil samples that would be indicative of free product. Used in combination, the soil analysis and the MIP records appear to provide accurate DNAPL identification and delineation.  相似文献   

14.
Traditional single-objective programs cannot deal with the tradeoffs between the decision makers who represent different perspectives and have inconsistent decision goals. Multi-objective ones can hardly represent a complex dominant-subordinate relationship between the leader and the follower. This study presents a new bilevel programming model with considering leader–follower-related health-risk and economic goals for optimal groundwater remediation management. The bilevel model is formulated by integrating health-risk assessment and environmental standards (the leader or the environmental concern) and remediation cost (the follower or the economic concern) into a general framework. In addition, stochastic uncertainty in health risk assessment is considered into the decision-making process. The developed bilevel model is then applied to a petroleum-contaminated aquifer in Canada. Results indicate that the performance of bilevel programming can not only meet the low remediation cost as the expectation from the follower but also simultaneously conform to the low contamination level as the expectation from the leader. Furthermore, comparative analyses show that the bilevel model with two-level concerns has the advantage of maximizing the interests and satisfaction degrees of decision makers, which can avoid the extreme results generated from the single-level models.  相似文献   

15.
The recovery of coal tar or creosote, which are dense nonaqueous phase liquids (DNAPLs), from the subsurface has been used as a means of site remediation at several former manufactured-gas plant sites and wood-treating facilities. Surface-active components in these complex DNAPL can have acid/base and surfactant characteristics that can significantly affect the wettability in these systems, with a reversal to DNAPL wetting at low pHs. These changes in wettability as a function of pH were employed to evaluate their significance on waterflooding efficiency in one-dimensional soil columns. The use of pH as a means of controlling wettability resulted in identical density and viscosity properties between the water-and DNAPL-wet conditions. At some of the higher pHs, the interracial tension changed as well as the wettability. Maintaining a constant dimensionless capillary number was used to minimize the effect of this variable. DNAPL saturations remaining in the DNAPL-wet systems after waterflooding ranged from 38% to 47%. Significantly lower final DNAPL saturations were achieved for water-wetting systems (15% to 30%).  相似文献   

16.
The spontaneous expansion and mobilization of discontinuous gas above dense non-aqueous-phase liquid (DNAPL) pools can affect the aqueous-phase concentrations of the DNAPL constituents above the pool. The results of an intermediate-scale, two-dimensional flow cell experiment showed that the discontinuous gas flow produced by spontaneous expansion, driven by the partitioning of 1,1,1-TCA from the surface of a DNAPL pool, resulted in detectable aqueous-phase concentrations of 1,1,1-TCA well above the pool surface. In comparison to a conventional model for DNAPL pool dissolution in the absence of a discontinuous gas phase, these concentrations were greater than expected, and were present at greater than expected elevations. Additionally, this study showed that the discontinuous gas flow produced transient behavior in the aqueous-phase concentrations, where the elevated concentrations occurred as short-term, pulse-like events. These results suggest that the spontaneous expansion and mobilization of discontinuous gas in DNAPL source zones could lead to the misdiagnosis of source zone architecture using aqueous concentration data, and that the transient nature of the elevated concentrations could further complicate the difficult task of source zone characterization.  相似文献   

17.
A systematic hydrogeologic site characterization has been completed in a fractured rock flow system, with the objective of identifying contaminant migration and fate pathways from a historical release of 1,1,1-trichloroethane (TCA). The study integrated hydrogeologic analysis techniques such as borehole geophysical logging, pumping test analysis, and hydrochemical facies analysis to study the impact of a dense nonaqueous phase liquid (DNAPL) in a sparsely fractured crystalline bedrock. The assessment methodology can be divided into two parts: (1) characterization of the source area, where DNAPL is acting as a residual source of TCA, and (2) characterization of the downgradient plume. Reduction in DNAPL mass in the source area has resulted in significant and sustained reductions in downgradient concentrations, suggesting that remediation of fractured crystalline bedrock contaminated with DNAPL is possible and not "technically infeasible."  相似文献   

18.
Naturally occurring radon in ground water can potentially be used as an in situ partitioning tracer to characterize dense nonaqueous phase liquid (DNAPL) saturations. The static method involves comparing radon concentrations in water samples from DNAPL-contaminated and noncontaminated portions of an aquifer, while the push-pull method involves the injection (push) and extraction (pull) of a radon-free test solution from a single well. In the presence of DNAPL, radon concentrations during the pull phase are retarded, with retardation manifested in greater dispersion of radon concentrations relative to a conservative tracer. The utility of these methods was investigated in the laboratory using a physical aquifer model (PAM). Static and push-pull tests were performed before and after contamination of the PAM sediment pack with trichloroethene (TCE), and after alcohol cosolvent flushing and pump-and-treat remediation. Numerical simulations were used to estimate the retardation factor for radon in push-pull tests. Radon partitioning was observed in static and push-pull tests conducted after TCE contamination. Calculated TCE saturations ranged up to 1.4% (static test) and 14.1% (push-pull test). Post-remediation tests showed decreases in TCE saturations. The results show that radon is sensitive to changes in DNAPL saturation in space and time. However, the methods are sensitive to DNAPL saturation heterogeneity, test location, sample size, and test design. The influence of these factors on test results, as well as the apparent overestimation of the retardation factor in push-pull tests, warrant further investigation.  相似文献   

19.
This study applies implicit stochastic optimization (ISO) to develop monthly operating rules for a reservoir located in Northeast Brazil. The proposed model differs from typical ISO applications as it uses the forecast of the mean inflow for a future horizon instead of the current-month inflow. Initially, a hundred different 100-year monthly inflow scenarios are synthetically generated and employed as input to a deterministic operation optimization model in order to build a database of optimal operating data. Later, such database is used to fit monthly reservoir rule curves by means of nonlinear regression analysis. Finally, the established rule curves are validated by operating the system under 100 new inflow ensembles. The performance of the proposed technique is compared with those provided by the standard reservoir operating policy (SOP), stochastic dynamic programming (SDP) and perfect-forecast deterministic optimization (PFDO). Different forecasting horizons are tested. For all of them, the results indicate the feasibility of using ISO in view of its lower vulnerability in contrast to the SOP as well as the proximity of its operations with those by PFDO. The results also reveal that there is an optimal choice for the forecasting horizon. The comparison between ISO and SDP shows small differences between both, justifying the adoption of ISO for its simplified mathematics as opposed to SDP.  相似文献   

20.
Contamination from the use of chlorinated solvents, often classified as dense nonaqueous phase liquids (DNAPLs) when in an undissolved state, represents an environmental challenge with global implications. Mass-transfer limitations due to rate-limited dissolution can lead to long-term aquifer persistence for even small volumetric fractions. The identification of DNAPL source zones located beneath the water table is critical to ultimately achieve site remediation and aquifer restoration. This paper provides a comparison of the advantages and disadvantages of many of the methods being used for detecting and delineating DNAPL contaminant source zones. The objective is to determine which options are best to pursue based on site characteristics, method performance, and method costs. DNAPL characterization methods are grouped into approaches, which include site preparation, characterization, and data-processing activities necessary to design an effective remediation system. We compare the different approaches based on the level of chemical and hydrogeologic resolution, and the need for additional data requirements. Our findings can be used to assist with selection of appropriate site remediation management options.  相似文献   

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