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1.
A three-step sequential extraction procedure with Milli-Q, CaCl2 and H3PO4 was applied for extraction of arsenic species in lichen transplants and airborne particulate matter (fine and coarse fractions). The samples used in this work were collected in 1994–1995 near coal-fired power plants. Both transplant lichens and airborne particulate matter were submitted to the same environment simultaneously. Arsenic species identification and quantification was performed by HPLC–UV–HG–AFS. Inorganic forms of arsenic (arsenite and arsenate) were present in significant amounts in most of the samples. Only in lichens also organic forms of arsenic (monomethyl arsonic acid and dimethyl arsinic acid) were identified which may indicate biotransformation of inorganic arsenic.  相似文献   

2.
Spatial distribution and trends in mean and absolute maximum and minimum temperatures and in the diurnal temperature range were analysed at 47 stations in the eastern Baltic region (Lithuania, Latvia and Estonia) during 1951–2010. Dependence of the studied variables on geographical factors (latitude, the Baltic Sea, land elevation) is discussed. Statistically significant increasing trends in maximum and minimum temperatures were detected for March, April, July, August and annual values. At the majority of stations, the increase was detected also in February and May in case of maximum temperature and in January and May in case of minimum temperature. Warming was slightly higher in the northern part of the study area, i.e. in Estonia. Trends in the diurnal temperature range differ seasonally. The highest increasing trend revealed in April and, at some stations, also in May, July and August. Negative and mostly insignificant changes have occurred in January, February, March and June. The annual temperature range has not changed.  相似文献   

3.
A series of measurements of ice-nucleating particles (INPs) were performed at two sites in Beijing. At the Beijing Meteorological Service (BMS) site, which was an urban site, no INPs were found to be active above–15°C. However, at the Yanjiaping (YJP) site, which was a rural site, the concentration of INPs active at temperatures above–15°C was found to be as high as 1.73 g–1. Two parameterizations were constructed by respectively fitting the data obtained at BMS site and YJP site. The two parameterizations, as well as another parameterization from the literature, were implemented into a parcel model to investigate the effect of INPs active above–15°C on phase partitioning in mixed-phase clouds. At a vertical velocity of 0.01 m s–1, which is typical for stratiform clouds associated with frontal systems, the INPs active above–15°C nucleate ice crystals at low levels. The growth of these ice crystals remarkably reduces both the maximum liquid water mixing ratio and the altitude where the maximum liquid water mixing ratio is reached. When the vertical velocity of the parcel is increased to 0.1 m s–1 or an even higher value, the evolution of liquid water mixing ratio is not controlled by the INPs active above–15°C but those active below–15°C.  相似文献   

4.
Summary We analysed long-term temperature trends based on 12 homogenised series of monthly temperature data in Switzerland at elevations between 316 m.a.s.l. and 2490 m.a.s.l for the 20th century (1901–2000) and for the last thirty years (1975–2004). Comparisons were made between these two periods, with changes standardised to decadal trends. Our results show mean decadal trends of +0.135 °C during the 20th century and +0.57 °C based on the last three decades only. These trends are more than twice as high as the averaged temperature trends in the Northern Hemisphere. Most stations behave quite similarly, indicating that the increasing trends are linked to large-scale rather than local processes. Seasonal analyses show that the greatest temperature increase in the 1975–2004 period occurred during spring and summer whereas they were particularly weak in spring during the 20th century. Recent temperature increases are as much related to increases in maximum temperatures as to increases in minimum temperature, a trend that was not apparent in the 1901–2000 period. The different seasonal warming rates may have important consequences for vegetation, natural disasters, human health, and energy consumption, amongst others. The strong increase in summer temperatures helps to explain the accelerated glacier retreat in the Alps since 1980. Authors’ addresses: Martine Rebetez, WSL Swiss Federal Research Institute, 1015 Lausanne, Switzerland; Michael Reinhard, Laboratory of Ecological Systems (ECOS), EPFL Swiss Federal Institute of Technology, 1015 Lausanne, Switzerland.  相似文献   

5.
The observed meridional overturning circulation (MOC) and meridional heat transport (MHT) estimated from the Rapid Climate Change/Meridional Circulation and Heat Flux Array (RAPID/MOCHA) at 26.5°N are used to evaluate the volume and heat transport in the eddy-resolving model LASG/IAP Climate system Ocean Model (LICOM). The authors find that the Florida Current transport and upper mid-ocean transport of the model are underestimated against the observations. The simulated variability of MOC and MHT show a high correlation with the observations, exceeding 0.6. Both the simu-lated and observed MOC and MHT show a significant seasonal variability. According to the power spectrum analysis, LICOM can represent the mesoscale eddy characteristic of the MOC similar to the observation. The model shows a high correlation of 0.58 for the internal upper mid-ocean transport (MO) and a density difference between the western and eastern boundaries, as noted in previous studies.  相似文献   

6.
The threat of climate change is emerging at a time of rapid growth for many economies in sub-Saharan Africa (SSA). Dominant narratives comprising ambitious development plans are common and often based around sectors with strong inter-dependencies that are highly exposed to climate variability. Using document analysis and key informant interviews, this article examines how climate change is addressed in policy, how it is being mainstreamed into water, energy and agriculture sector policies and the extent to which cross-sectoral linkages enable coordinated action. These questions are addressed through a case study of Tanzania, highlighting broader lessons for other developing countries, particularly those in SSA facing similar challenges. The article finds that, while the agriculture and water sectors are increasingly integrating climate change into policies and plans in Tanzania, practical coordination on adaptation remains relatively superficial. Publication of the Tanzania National Adaptation Plan of Action (NAPA) in 2007 marked a step change in the integration of climate change in sectoral policies and plans; however, it may have reinforced a sectoral approach to climate change. Examining the policies for coherence highlights overlaps and complementarities which lend themselves to a coordinated approach. Institutional constraints (particularly structures and resources) restrict opportunities for inter-sectoral action and thus collaboration is confined to ad hoc projects with mixed success to date. The results highlight the need for institutional frameworks that recognize and address these constraints to enable development goals to be pursued in a more sustainable and climate-resilient manner.

KEY POLICY INSIGHTS

  • The NAPA has been successful at encouraging climate change mainstreaming into sectoral policies in Tanzania; however, the cross-sectoral collaboration crucial to implementing adaptation strategies remains limited due to institutional challenges such as power imbalances, budget constraints and an ingrained sectoral approach.

  • Collaboration between nexus sectors in Tanzania is largely through ad hoc projects with limited progress on establishing deeper connections to enable collaboration as a process. Regular cross-sectoral planning meetings and consistent annual budgets could provide a platform to enhance cross-sectoral coordination.

  • Plans to develop hydropower and agriculture are prevalent across sub-Saharan Africa. Insights from Tanzania highlight the importance of institutional and policy frameworks that enable cross-sectoral coordination.

  相似文献   

7.
The United Nations Environment Programme (UNEP) performed field surveys at 15 sites in Bosnia–Herzegovina where depleted uranium (DU) ammunition was used by the North Atlantic Treaty Organization (NATO) during the Balkans conflict (1994–1995). During the field missions, the Italian Environmental Protection Agency (APAT) evaluated airborne contamination due to DU dusts or aerosol particles, generated at the time of the conflict by the impact of DU ammunition on hard targets, using lichens and tree barks as biomonitors. Each sample was analyzed by alpha-spectrometry for DU determination. The 234U/238U activity concentration ratios were used to distinguish natural from anthropogenic uranium. This paper reports the data obtained by the UNEP investigation, including (non-radioactive) metal and other element concentrations in lichen and tree bark samples measured by instrumental neutron activation analysis (INAA). The results indicated: (i) lichens and tree barks are sensitive bio-accumulators of past airborne contamination by depleted uranium dusts; (ii) 8 years after the conflict, environmental DU contamination is still present at some of the target sites; and (iii) the highest concentrations of most non-radioactive elements were found at sites used for ammunition destruction.  相似文献   

8.
北极极涡是一个存在于极区对流层中上层和平流层的大尺度气旋性环流系统,是极区大气运动的主要特征。赤道平流层风场的准两年振荡,可以对行星波的传播进行调制,从而对北极极涡的强度产生影响。为了定量描述,赤道平流层风场的准两年振荡对北极极涡的影响,我们对表征北极极涡强度的55–65°N纬度带平流层纬向风进行了分析,提取出了北极极涡中的准两年振荡信号,并发现了该信号的纬向不均一性,120–180°E为高值区,25–45°E为低值区。  相似文献   

9.
On the basis of the analysis of atmospheric carbon dioxide concentration variations and the annual mean air temperature at Syowa Station, Antarctica in the period of 1984-1988, the following results are easily obtained:(1) The annual mean values of the atmospheric carbon dioxide concentration are gradually increased and equal to 342.59, 343.80, 345.15, 346.83 and 348.82 ppmv for 1984, 1985, 1986, 1987 and 1988, respectively. Its annual increase rates are 1.21, 1.35, 1.68 and 1.99 ppmv/yr. For 1984-1985, 1985-1986, 1986-1987 and 1987-1988, respectively and are raised year by year.The seasonal variations are observed and the maximum concentration is in spring and the minimum one is in late-summer or early-autumn.(2)The increasing tendency of the concentration of the atmospheric carbon dioxide is consistent with that of the a.ir temperature.  相似文献   

10.
Daily and monthly total precipitation of 155 synoptic stations with relatively regular distribution over Iran, covering the 1990–2014 period, were used to investigate the spatial pattern of precipitation seasonality and regimes over Iran, using a set of precipitation seasonality indices. The results suggest a strong agreement between the indices computed at monthly time scale. The result also shows a latitudinal decreasing gradient from the lower index values in the north to the highest values in the south of Iran, suggesting a strong negative relationship between the latitude and the indices. A weak but statistically significant association was also found between the indices and the longitude, showing a gradual west-east contrast between the mountainous western Iran and the central-eastern lowlands and deserts of the country. The spatial patterns of the indices well agree in revealing different precipitation regimes in Iran, in spite of the observed discrepancies in their areal extent of the regions identified. All the indices characterized northern Iran by a precipitation regime having a moderate seasonality, while the mountainous areas of the western and northern Iran are featured by a marked precipitation regime possessing a longer dry season. However, the most seasonal precipitation regime with the longest dry period describes the southern country and some spot areas of the central-eastern Iran. The spatial distribution of the seasonal precipitation regimes and the month and season of maximum precipitation amounts across Iran was also identified, suggesting that from the 24 possible precipitation regimes over the globe, eight were found in Iran, from which a precipitation regime with the highest precipitation amount in winter, followed by autumn, spring, and summer characterized most parts of the country. January and JFM were also found as the month and season of maximum precipitation in a majority of stations distributed over Iran, respectively. The precipitation concentration index (DPCI) computed using daily precipitation data ranges between 0.56 and 0.76 across the country; nonetheless, the values between 0.64 and 0.70 characterized a majority of stations distributed over most parts of Iran. Contrarily to the indices computed at monthly time scale, the DPCI does not show a clear latitudinal pattern over the country. The Mann–Kendal trend test and the Sen slope estimator were applied to the computed indices relative to 16 stations with the longest and complete precipitation records during 1951–2014 time period. The indices time series showed no significant trend in the majority of the stations, indicating that the precipitation regimes of the studied stations did not change over 1951–2014 period.  相似文献   

11.
The trend significance and the residual variability of integral atmospheric characteristics in the atmospheric action centers in the Asian-Pacific region in summer in 1950-1979 and 1980-2012 are computed. Basic differences are revealed between trends in circulation and residual variability in the atmo spheric action centers in the surface pressure field and in the field of geopotential H 500 for these time periods. Increase in significant trends for the whole period and decrease in residual variability were found in the area of the Asian low in 1980-2012. A significant trend was observed in June and September in the area of the Hawaiian high. The summer Far Eastern low has intensified in recent years. The Okhotsk high strengthened in May and weakened in June, August, and September in the 2000s.  相似文献   

12.
Recent trends in seasonal cycles in China are analyzed, based on a homogenized dataset of daily temperatures at 541 stations during the period 1960–2008. Several indices are defined for describing the key features of a seasonal cycle, including local winter/summer (LW/LS) periods and local spring/autumn phase (LSP/LAP). The Ensemble Empirical Mode Decomposition method is applied to determine the indices for each year. The LW period was found to have shortened by 2–6 d (10 yr)-1, mainly due to an earlier end to winter conditions, with the LW mean temperature having increased by 0.2°C–0.4°C (10 yr)?1, over almost all of China. Records of the most severe climate extremes changed less than more typical winter conditions did. The LS period was found to have lengthened by 2–4 d (10 yr)?1, due to progressively earlier onsets and delayed end dates of the locally defined hot period. The LS mean temperature increased by 0.1°C–0.2°C (10 yr)-1 in most of China, except for a region in southern China centered on the mid-lower reaches of the Yangtze River. In contrast to the winter cases, the warming trend in summer was more prominent in the most extreme records than in those of more typical summer conditions. The LSP was found to have advanced significantly by about 2 d (10 yr)-1 in most of China. Changes in the autumn phase were less prominent. Relatively rapid changes happened in the 1980s for most of the regional mean indices dealing with winter and in the 1990s for those dealing with summer.  相似文献   

13.
The diurnal temperature range(DTR) has decreased dramatically in recent decades, but it is not yet obvious whether the extreme values of DTR have also reduced. Based on the daily maximum and minimum temperature data of 653 stations in China, a set of monthly indices of warm extremes, cold extremes, and DTR extremes in summer(June, July, August) and winter(December, January, February) were studied for spatial and temporal features during the period 1971–2013. Results show that the incidence of warm extremes has been increasing in most parts of China, while the opposite trend was found in the cold extremes for summer and winter months. Both increasing and decreasing trends of monthly DTR extremes were identified in China for both seasons. For high DTR extremes, decreasing trends were identified in northern China for both seasons, but increasing trends were found only in southern China in summer, while in winter, they were found in central China. Monthly low DTR extreme indices demonstrated consistent positive trends in summer and winter, while significant increases(P 0.05) were identified for only a few stations.  相似文献   

14.
水汽输送的变化对于降水的变化有重要贡献。基于优选的13个CIV1IP5模式发现:RCP4.5和RCP8.5排放情景下,1.5°C和2.0°C增暖时东亚夏季水汽输送均加强,且2.0°C增暖时模式间一致性更好;水汽含量的增加对东亚南部和北部水汽输送的加强均有贡献,东亚南部水汽输送的加强也与低层环流的加强相联系。0.5°C额外增暖(1.5°C和2.0°C增暖间比较)时,两种排放情景下水汽输送的变化在我国南海与东北地区存在差异,使得两个地区降水变化存在差异;水汽输送的变化与低层环流的变化关系密切,且模式间一致性相对低。  相似文献   

15.
Validation of ECMWF and NCEP–NCAR Reanalysis Data in Antarctica   总被引：3，自引：0，他引：3  
The European Center for Medium-Range Weather Forecast (ECMWF) Re-Analysis (ERA-40) and the National Centers for Environmental Prediction-National Center for Atmospheric Research (NCEP-NCAR) ECMWF (ERA-40) and NCEP-NCAR reanalysis data were compared with Antarctic station observations, including surface-layer and upper-layer atmospheric observations, on intraseasonal and interannual timescales. At the interannual timescale, atmospheric pressure at different height levels in the ERA-40 data are in better agre...  相似文献   

16.
As "the third pole", the Tibetan Plateau (TP) is sensitive to climate forcing and has experienced rapid warming in recent decades. This study analyzes annual and seasonal near-surface air temperature changes on the TP in response to transient and stabilized 2.0°C/1.5°C global warming targets based on simulations of the Community Earth System Model (CESM). Elevation-dependent warming (EDW) with faster warming at higher elevations is predicted. A surface energy budget analysis is adopted to uncover the mechanisms responsible for the temperature changes. Our results indicate a clear amplified warming on the TP with positive EDW in 2.0°C/1.5°C warmer futures, especially in the cold season. Mean TP warming relative to the reference period (1961–90) is dominated by an enhanced downward longwave radiation flux, while the variations in surface albedo shape the detailed pattern of EDW. For the same global warming level, the temperature changes under transient scenarios are ~0.2°C higher than those under stabilized scenarios, and the characteristics of EDW are broadly similar for both scenarios. These differences can be primarily attributed to the combined effects of differential downward longwave radiation, cloud radiative forcing, and surface sensible and latent heat fluxes. These findings contribute to a more detailed understanding of regional climate on the TP in response to the long-term climate goals of the Paris Agreement and highlight the differences between transient and stabilized warming scenarios.  相似文献   

17.
Climate sensitivity is an important index that measures the relationship between the increase in greenhouse gases and the magnitude of global warming. Uncertainties in climate change projection and climate modeling are mostly related to the climate sensitivity. The climate sensitivities of coupled climate models determine the magnitudes of the projected global warming. In this paper, the authors thoroughly review the literature on climate sensitivity, and discuss issues related to climate feedback processes and the methods used in estimating the equilibrium climate sensitivity and transient climate response (TCR), including the TCR to cumulative CO2 emissions. After presenting a summary of the sources that affect the uncertainty of climate sensitivity, the impact of climate sensitivity on climate change projection is discussed by addressing the uncertainties in 2°C warming. Challenges that call for further investigation in the research community, in particular the Chinese community, are discussed.  相似文献   

18.
Trends and periodicity analyses can provide information on climate variability inherent in a particular variable. In this study, trend tests and spectral analysis are used to examine the existence of trends and cycles in temperature series (1901–2000) of Nigeria. Periods 1901–1929 and 1942–1980 exhibited cooling trends while 1930–1941 and 1981–2000 showed warming trends. The warmest years in Nigeria were 1941, 1935, 1931 and 1987. The coldest years were 1929, 1975, 1925 and 1974. Whereas no significant trends were detected for 1901–1930 period, the standard period 1931–1960 was marked by significant cooling while 1961–1990 was marked with significant warming. Annual temperature has risen by 0.03?°C/decade during the last century. The overall warming was mostly confined to the south of 12°N especially during April and June. Changes in minimum temperature are higher than that of maximum temperature. The quasi-biennial oscillation was found in annual data for all the six zones with periods of about 2–4?years. Nigeria landscape is under strong North Atlantic Oscillation influence in dry season and under ENSO influence during wet season. Annual temperature series was also found to exhibit significant negative correlation with SOI.  相似文献   

19.
China has been experiencing widespread air pollution due to rapid industrialization and urbanization in recent decades.The two major concerns of ambient air quality in China are particulate matter(PM) and tropospheric ozone(O_3). With the implementation of air pollution prevention and control actions in the last five years, the PM pollution in China has been substantially reduced. In contrast, under the conditions of the urban air pollution complex, the elevated O_3 levels in city clusters of eastern China, especially in warm seasons, have drawn increasing attention. Emissions of air pollutants and their precursors not only contribute to regional air quality, but also alter climate. Climate change in turn can change chemical processes, long-range transport, and local meteorology that influence air pollution. Compared to PM, less is known about O_3 pollution and its climate effects over China. Here, we present a review of the main findings from the literature over the period 2011–18 with regard to the characteristics of O_3 concentrations in China and the mechanisms that drive its interannual to decadal variations, aiming to identify robust conclusions that may guide decision-making for emissions control and to highlight critical knowledge gaps. We also review regional and global modeling studies that have investigated the impacts of tropospheric O_3 on climate, as well as the projections of future tropospheric O_3 owing to climate and/or emission changes.  相似文献   

20.
From joint wavelet analysis of long-wavelength baroclinic Rossby waves and SST anomalies in the 5–10?yr band in the North and tropical Atlantic, and Reduced Rainfall Height (RRH) in Western Europe and Eastern North America, some key mechanisms involved in the interannual rainfall variability are highlighted. Systematic work has been undertaken to highlight the resonance of long planetary waves in the tropical oceans. Quasi-stationary Waves (QSWs) are produced resulting from the combination of gravitational forces and trade wind stress or ENSO events to compensate for energy lost in the resonator and, above all, to produce a strong modulated output current at the open end, contributing to the western boundary currents. Gravitational forces are resulting from the topography of the surface of the ocean at the antinodes, the dimension of the basin and the wavelength of planetary waves involved in the resonance being of the same order of magnitude. Remote resonances occur at critical latitudes, nearly 40°N and 40°S, forming QSWs the role of which is crucial in the functioning of sub-tropical gyres. In the North Atlantic subtropical gyre, an 8-yr period QSW appears to have a decisive role in the interannual rainfall variability. The pattern of SST anomalies depends on buoyancy of the advected layer associated with this QSW, which is controlled by the amplitude and the phase of long-period sub-harmonics. Rainfall oscillation in Western Europe has occurred for some decades and extended as the dipole formed by SST anomalies on both antinodes became unbalanced, due to the emergence of the advected layer further north. Since then cyclonic or anticyclonic conditions are prevailing at midlatitudes, depending on the polarity. Strengthening of RRH anomalies in Eastern North America is attributed to the buoyancy of the advected layer that re-circulates along the sub-tropical gyre, which evidences the excitation of long-period sub-harmonics, too. Frequency of exceptional events increased in areas heavily exposed to RRH anomalies, subject to oceanic influences even during extreme events, as this occurs in the north of France. Changes in rainfall patterns is attributed to global warming, i.e. the resonance of long-period sub-harmonics associated with solar magnetic cycles whose amplitude has increased drastically at the end of the second millennium, not including the possible contribution of greenhouse gas emissions whose impact on climate is non-resonant.  相似文献   

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