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1.
乌梁素海和岱海沉积磷形态分布的差异性研究 总被引：3，自引：0，他引：3
湖泊沉积物中磷的含量及形态分布等地球化学信息可以用来反演湖泊流域的古环境及污染历史。本文以乌梁素海和岱海两个不同类型的湖泊为研究对象,对两个湖泊沉积柱芯中磷形态分布的差异性进行了研究。结果表明,乌梁素海和岱海沉积柱芯中沉积磷的主导形态均为ACa P、De P和 Or P,但乌梁素海表层沉积物和沉积柱芯中Al P和 ACa P的含量水平明显高于岱海,而Ex P、De P和 Or P的含量水平明显低于岱海。两个湖泊沉积磷形态分布的差异性能较好地揭示出湖泊流域的地理环境、化学风化程度以及湖泊富营养化类型的差异性,沉积柱芯中ACa P含量及其分布特征能很好的指示湖泊自身发展过程中的富营养化水平,而De P含量及其分布特征则能较好的揭示出整个湖泊流域的古环境古气候信息。 相似文献
2.
东海陆架泥质区沉积地球化学比较研究 总被引：38，自引：4，他引：34
利用东海陆架泥质沉积区和周围砂质沉积区的表层沉积物元素含量和海水悬浮沉积物总量分析资料,对泥质区的沉积地球化学进行了比较研究。结果表明东海不同泥质区的沉积地球化学过程很不相同。浙江近岸泥质区沉积物元素以Fe、Mn、Zn的含量高,Na、Sr、Al、Ca的含量低为特征,其地球化学特征与长江沉积物非常一致。近岸泥质区的沉积物基本来源于长江输入海的沉积物,在台湾暖流的作用下沉积在浙江沿岸。远岸济州岛西南泥质区沉积物以Na、Sr的高含量,较高的Al、Ca含量和低的Fe、Mn、Zn含量为特征,其地球化学特征与黄河源沉积物有好的相关性,但有一定的混合源性质,该泥质区的沉积物主要来源于黄河源的细颗粒沉积物,由黄海沿岸流搬运到该区并沉积下来。沉积物在搬运沉积过程中,元素粒度分异作用明显。东海陆架泥质区沉积地球化学过程的控制性影响因子是东海环流系统和物源,其中台湾暖流对东海陆架远岸和近岸泥质区的沉积地球化学分区具有关键作用。 相似文献
3.
晚第四纪湖泊沉积物盐类与碎屑矿物反相关关系的沉积学解释 总被引：1，自引：0，他引：1
湖泊沉积物中矿物组合是古气候环境研究的敏感性指标之一, 充分认识湖泊沉积物中各类矿物组合类型、沉积过程, 对正确解释矿物学指标有重要意义. 我国晚第四纪湖泊沉积记录中, 盐类矿物与碎屑矿物含量普遍存在反相关关系, 影响了矿物组合作为气候指标的解释和应用. 从地球科学的角度正确理解这种关系, 可以为湖泊动力学以及古气候环境定量研究提供重要的科学依据. 选择甘肃民勤盆地石羊河下游终端湖猪野泽不同位置5个全新世剖面, 在明确湖泊沉积物来源、搬运方式和沉积动力机制的基础上, 研究了以碳酸盐矿物为主的盐类矿物含量与粒度指标之间的关系. 结果表明:猪野泽各剖面砂层富含的中砂、细砂沉积物主要是来自于巴丹吉林沙漠和腾格里沙漠的风成砂; 水动力作用主导了湖相沉积层200 μm以下沉积物的沉积, 风力作用对20~70 μm粉砂组分沉积也有所贡献. 同时, 猪野泽湖相沉积层中高含量的碳酸盐主要来自于流水搬运, 湖相沉积层位200 μm以下的粉砂和极细砂是碳酸盐的主要富集区. 综上所述, 干旱区湖泊沉积物中盐类矿物含量与其沉积过程密切相关, 盐类矿物在全球变化研究中的应用要建立在充分研究其沉积动力机制的基础上. 相似文献
4.
文章以柴达木盆地西部尕斯库勒盐湖沉积物为研究对象,通过对钻孔沉积物和地表沉积物中铀和钍含量的研究,探讨了盐湖沉积物中铀和钍的地球化学特征。分析表明,钻孔沉积物中铀和钍之间存在明显的正相关关系。在横向上,随地表取样点逐渐远离湖表卤水,沉积物中铀和钍的含量先增高后又急剧降低,且受补给水铀含量影响大;在纵向上,同一个晶间卤水层或者碎屑物沉积层内铀含量垂直分异明显,铀含量随深度增加而递增。就沉积物中铀和钍的赋存形式而言,2/3的铀被黏土质点吸附,1/3的铀夹杂在盐类矿物中;而90%以上的钍被黏土质点吸附,10%以下的钍夹杂在盐类矿物中。干盐滩中毛细蒸发和淋滤等化学沉积分异作用造成盐湖沉积中心的沉积物铀含量相对较高。 相似文献
5.
地震液化脉是地震作用引起的软沉积变形的重要构造之一,前人对脉体形态学和动力学做了大量的研究工作,但对其成因的微观地球化学行为研究较少。笔者采取开化裴岭脚剖面2期地震事件沉积的3套地震液化脉层样品21块,分别对其脉体和含脉体围岩做了微量元素分析。结果显示,液化脉中Cs、Ba、Th、Zr、Hf、Cr、Rb、Nb等反映陆源性质元素明显高于含脉体围岩,而Sr、Y、Ni反映海相沉积特征元素则表现为含脉体围岩高于脉体。通过对V、Mo富集度和微量元素特征参数Sr/Ba、Th/U等的综合研究,发现液化脉体表现为氧化环境,含脉体围岩为还原环境,且脉体和围岩均具有淡水作用特点。研究认为,早寒武世大陈岭期白云质灰岩沉积过程中有蚀源区陆源碎屑物的补入;在地震突发振动力作用下,富含水的软沉积层液化泄水,因化学沉积物和碎屑沉积物性质的差异,塑性碳酸盐沉积物随水部分流失,使得单位体积内碳酸盐沉积含量低于围岩,导致脉体中更富陆源物质;地震事件沉积层属潮上带,特别是地震液化泄水后期至成岩期,含地震液化脉沉积层曾暴露地表,受后期陆源物的再补给及大气降水淋滤蚀变作用影响,表现为古气候和古盐度异常,为浙西大陈岭组浅水沉积提供了地球化学的证据。 相似文献
6.
7.
对太湖不同污染状况和生态系统状况的湖区沉积物中磷的地球化学形态及其分布进行了研究。结果发现,沉积物的理化性质和磷的化学形态一般都在表层下深5～15cm发生明显的转折;草型湖区、藻型湖区、开阔湖面的大湖区沉积物的理化性质、间隙水中的磷浓度及沉积物中磷的形态存在较大的差异。东太湖沉积物间隙水磷浓度和交换态磷含量都显著低于其他湖区;风浪扰动相对剧烈的开阔湖面湖区沉积物中磷的沉积规律也不同于梅梁湾藻型湖区和东太湖草型湖区。研究表明,浅水湖泊中水生生物状况、风浪扰动状况对沉积物中磷的地球化学行为有至关重要的影响。 相似文献
8.
通过对南极布兰斯菲尔德海峡26个站位表层沉积物的地球化学组成的因子分析和相关分析,探讨了影响表层沉积物地球化学特征的主要因素。揭示了控制沉积物特征的地球化学作用。结果表明,岛（陆）架－－岛坡区表层沉积物地球化学特征较复杂,受到多种因素的影响,最主要的是受沉积区离岸远近和水深大小等因素控制的钙质生物、硅质生物和陆源碎屑的沉积作用,其次为中酸性火山碎屑沉积作用与基性火山碎屑的沉积作用;海槽－－陆坡区有层沉积物地球化学特征主要由硅质碎屑沉积和粘土质陆源、火山碎屑在时空旧的交替沉积所控制,宇宙源沉积、自生沉积、碱性火山碎屑沉积、热液作用等的影响较小。 相似文献
9.
冲绳海槽北部现代沉积物地球化学研究 总被引：5，自引：0，他引：5
本文对冲绳海槽北部现代海底表层沉积物的沉积物地球化学特征进行了系统的分析，探讨了分别代表陆源，火山源和生物源沉积物的地球化学指标。结果表明，ＳｉＯ２主要富集于东海外陆架与陆架坡折带，基本上反映了陆源碎屑沉积或东海陆架外缘的残留砂沉积；Ａｌ２Ｏ３和Ｎａ２Ｏ的含量分布与玻屑砂或火山玻璃的含量有关；ＣａＯ或ＣａＣＯ３代表了生物沉积组份的多寡。 相似文献
10.
用137Cs计年法确定湖泊沉积物沉积速率研究进展 总被引：15，自引：0，他引：15
137Cs计年法利用137Cs固有的理化和沉降特性,在湖泊沉积物的137Cs垂直分布与大气137Cs沉降间确立对应关系,找出有异常137Cs含量的沉积层作为时标,但需注意137Cs从水体表面至湖底的时间和粘粒含量对各层137Cs含量的影响,并用其它方法校验时标的可靠性。再求取不同时标层间的年均沉积厚度,或因克服了压实效应而更能反映真实沉积速率的年均沉积通量,且结合GIS等手段进一步估算湖泊各区域的沉积总量;还可延伸研究湖泊内源污染负荷及相关环境演变和湖泊演化。但是,沉积柱样的分割厚度取多少才能既满足计年精度要求又不使工作量过大,137Cs的大气沉降时间与进入沉积物时间还与泥沙的陆地迁移时间有关,沉积物中究竟是否发生137Cs下渗及其机理等都还是此法应用中有待解决的问题。 相似文献
11.
The levels and depth distributions of As, Cd, Cu, Zn, Pb, Hg, Fe and Mn in two sediment cores DY2 and DY4 collected from the ＂Cattle Pond＂ of Dongdao Island, South China Sea, were determined and analyzed with the main objective to identify the sources of these elements and evaluate the corresponding sedimentological and geochemical processes. Lithological characters and sedimentary parameters such as LOI950℃, CaO, LOI550℃ and TOC indicate that the depth of 96 cm and 87 cm are the critical points for DY2 and DY4 cores, respectively. As, Cd, Cu, Zn, Hg and P are remarkably enriched in the ornithogenic sediments above the critical depth points; their concentration-versus-depth profiles are similar to those of TOC and LOI550℃; the ratios of As, Cd, Cu, Zn, Hg over Ca are significantly correlated with P/Ca. Statistical and comparative analyses of these elements＇ levels in the ornithogenic sediments of DY2 and DY4 strongly suggest that seabird droppings are the main source of these elements. Additionally, for the upper sediment layers of DY2 and DY4 cores, Fe oxide sorption mechanism, like organic matter, may also play an important role in the abundances of heavy metals. Heavy metal Pb has geochemical characteristics distinctly different from those of As, Cd, Cu, Zn, Hg and P, and its isotope composition indicates an origin of anthropogenic emissions from the surrounding countries. These geochemical characteristics in the orinithogenic sediments of Xisha Islands are compared with the studies in the remote Antarctic and Arctic regions. 相似文献
12.
Sr/Ca,Mg/Ca:珊瑚岛鸟粪沉积的物源指示计* 总被引：1，自引：0，他引：1
文章尝试用Sr/Ca,Mg/Ca比值作物源指示计,区分了珊瑚岛屿受到海鸟粪影响的湖泊沉积物中鸟粪、珊瑚砂、植物这几种主要的环境介质对沉积物的相对贡献,据此恢复1800年来西沙群岛东岛海鸟数量变化和植被演化的历史。结果表明,东岛海鸟数量的变化历史可划分为潜伏期、增长期、稳定期和衰退期4个阶段,历史时期东岛海鸟生态系统的建立和发展与岛屿植被的演变有着密切的联系。研究获得的方法和初步结论为进一步开展西沙岛屿海鸟数量变化、植被演化的广泛对比并探讨与气候变化、人类活动的相互联系提供了基础。 相似文献
13.
Heavy Metal Distributions and Source Tracing in the Lacustrine Sediments of Dongdao Island, South China Sea 总被引：1，自引：0，他引：1
The levels and depth distributions of As,Cd,Cu,Zn,Pb,Hg,Fe and Mn in two sediment cores DY2 and DY4 collected from the"Cattle Pond"of Dongdao Island,South China Sea,were determined and analyzed with the main objective to identify the sources of these elements and evaluate the corresponding sedimentological and geochemical processes.Lithological characters and sedimentary parameters such as LOI_(950℃),CaO,LOI_(550℃) and TOC indicate that the depth of 96 cm and 87 cm are the critical points for DY2 and DY4 cores,respectively.As,Cd,Cu,Zn,Hg and P are remarkably enriched in the ornithogenic sediments above the critical depth points;their concentration-versus-depth profiles are similar to those of TOC and LOIssooc;the ratios of As,Cd,Cu, Zn,Hg over Ca are significantly correlated with P/Ca.Statistical and comparative analyses of these elements' levels in the ornithogenic sediments of DY2 and DY4 strongly suggest that seabird droppings are the main source of these elements.Additionally,for the upper sediment layers of DY2 and DY4 cores,Fe oxide sorption mechanism,like organic matter,may also play an important role in the abundances of heavy metals.Heavy metal Pb has geochemical characteristics distinctly different from those of As,Cd,Cu,Zn,Hg and P,and its isotope composition indicates an origin of anthropogenic emissions from the surrounding countries.These geochemical characteristics in the orinithogenic sediments of Xisha Islands are compared with the studies in the remote Antarctic and Arctic regions. 相似文献
14.
利用在长江口崇明岛北支北四滧港（SY）、北堡港（BBG）以及新卫村（XW）潮滩获取的表层沉积物,测试总有机碳（TOC）、总氮（TN）及总硫（TS）含量,分析有机地球化学元素在潮滩微相的分布规律及影响因素,试图建立TOC/TN、TS/TOC等潮滩微相识别指标。研究结果显示,影响长江口潮滩TN、TS微相分布的重要因素为有机质含量及类型。在淤涨型潮滩,TOC/TN在高潮滩一般大于10,在中潮滩明显降至10以下;中潮滩植被带TS/TOC最高,平均值达0.063,其次为高潮滩互花米草带和中潮滩光滩（分别为0.055和0.054）,高潮滩芦苇带最低;TS-TOC一元线性回归斜率在高潮滩芦苇带呈现为显著低值,自高潮滩米草带向光滩,逐渐增大。在侵蚀型潮滩,TOC/TN从高潮滩到低潮滩均大于10,而且中、低潮滩的比值大于高潮滩,潮下带骤降至小于10;TS/TOC自陆向海逐渐增大,TS-TOC一元回归斜率高潮滩最低,中潮滩最高。另外,侵蚀型潮滩各微相的TS-TOC一元线性回归斜率均明显低于淤涨型潮滩。上述研究结果表明,长江口沉积物的TOC/TN和TS/TOC及TS-TOC一元线性回归斜率与潮滩沉积微相之间存在一定的关系,具有应用于全新世钻孔识别潮滩沉积物微相的潜力。 相似文献
15.
Organic carbon isotopes in sediments have been frequently used to identify the source of organic matter.Here we present a study of organic δ~(13)C on two sediment profiles influenced by guano from Guangjin and Jinqing islands in the Xisha Archipelago,South China Sea.Organic matter from ornithogenic coral sand sediments has two main sources,guano pellets and plant residues,and their organic δ~(13)C(δ~(13)C_(OM)) are significantly different.Organic carbon δ~(13)C_(guano) is much higher thanδ~(13)C_(plants),and δ~(13)C_(OM)of bulk samples is intermediate.Based on a two-end-member mixing model,the proportions of guano-and plant-derived organic matter in the bulk samples were reconstructed quantitatively.The results showed that seabirds began to inhabit the islands around approximately1200-1400 AD,and that guano pellets have been an important source of soil organic matter since then.With the accumulation of guano-derived nutrients,plants began to develop prosperously on the islands in the last 200 years,which is reflected by the significant increase of plant-derived organic matter in the upper sediment layer.However,guano-derived organic matter decreased greatly in recent decades,indicating a rapid decrease in seabird population.Our results show that organic δ~(13)C can be effectively used to quantitatively determine different source contributions of OM to bulk ornithogenic coral sand sediments. 相似文献
16.
Vertical distribution patterns of organic geochemical constituents and the enzymes aminopeptidase and β-glucosidase provide
insights about the nature and reactivity of sediment organic matter in the sandy sediments of two shallow “South Texas” estuaries.
Sediment total organic carbon (TOC) δ13C values indicated that the organic matter (OM) was derived more from a mixture of seagrass and phytoplankton than from terrigenous
OM. Down-core amounts of TOC and total nitrogen (TN) were <0.2% of dry weight, respectively. Enzyme activities were highest
near surface and ranged from 25 to 1 μM/h for aminopeptidase as compared to 5 to 0.2 μM/h for glucosidase. In Aransas Bay,
aminopeptidase activity correlated with sediment TN content (r
s = 0.30) and β-glucosidase with TOC content (r
s = 0.27). In Copano Bay, aminopeptidase correlated with TOC, TN, and carbohydrate content (r
s = 0.89, 0.90, and 0.83, respectively). Variations of glucosidase activity also related positively to TOC, TN, and total carbohydrate
content (r
s = 0.68, 0.77, and 0.48, respectively). Overall, enzyme activities in these low OM, sandy sediments resembled those for other
benthic marine environments. 相似文献
17.
鹤庆钻孔沉积物总有机碳、氮含量测定的前处理方法及其环境意义 总被引：2，自引：0，他引：2
湖泊沉积物中的总有机碳含量(TOC)、总有机氮含量(TN)和碳氮比值(C/N)已被广泛应用于第四纪湖泊古环境研究中。对湖泊沉积物样品进行TOC和TN测定前, 首先要有效去除沉积物中的无机碳酸盐, 同时较好地保留有机质组分, 才能使实验结果较准确地反映古气候环境的变化。选取鹤庆钻孔不同深度的不同岩性样品, 分别进行粒度、盐酸浓度、洗除残留酸方法等对去除碳酸盐和总有机碳测定结果影响的前处理条件实验, 根据测得的TOC、TN和C/N, 结合总无机碳酸盐含量(TIC), 确定了鹤庆钻孔沉积物有机碳含量测定的前处理方法:室温条件下, 将磨得足够细(无需过筛处理)的样品与足量浓度为2mol/L盐酸充分反应24小时, 期间超声震荡3次, 采用离心加速沉淀的方法清洗酸处理样品至中性, 烘干, 研磨均匀上机测定。结果显示, 该流程可有效去除沉积物中的无机碳酸盐, 测得的TOC、TN数值具有很好的稳定性和可重复性。在此基础上测定了鹤庆钻孔沉积物样品的TOC、C/N和TIC, 它们间存在很好的正相关关系, 指示了西南季风强度的变化。 相似文献
18.
Xiangchao Chen Muhua Feng Fan Ke Jizheng Pan Fan Fan Yarui Wang Wenchao Li 《Aquatic Geochemistry》2018,24(1):55-77
The source, quantity and quality of sedimentary organic matter (SOM) were investigated in the surface sediments of Lake Fuxian, a deep oligotrophic lacustrine system in China. Granulometry, biochemical organic composition, bulk organic proxies and their stable isotopes were determined in the surface sediments (0–4 cm). The values of δ13C, δ15N and atomic ratio of total organic carbon to total nitrogen (TOC/TN) indicated that the sediments in the large partial lake were influenced by autochthonous organic matter. The concentrations of TOC, protein (PRT) and total hydrolysable amino acids may be mainly modulated by phytodetritus sinking from euphotic zones since they correlated significantly with chlorins. Otherwise, the lack of correlation between chlorins concentrations and carbohydrate (CHO) and lipid (LIP) indicated that the latter may have an additional terrestrial source. The highest sediment quantity was found in the deepest station NC owing to its fine sediment. Stations near northwestern shore accumulated more SOM than other littoral stations, which was in accordance with sewage discharge strength. Degradation quality indices, such as chlorin index, degradation index, PRT/CHO, and LIP/CHO, were in general agreement in showing the degraded status of SOM in Lake Fuxian. No clear spatial patterns were found in sediment degradation quality, which may be influenced by bottom oxygen concentration in the deep stations. 相似文献
19.
苏北潮滩湿地不同生态带碳、氮、磷分布特征* 总被引：1，自引：0，他引：1
通过对比苏北潮滩湿地不同生态带的表层以及柱状沉积物中总有机碳、总氮、总磷和有机磷含量,并结合不同植被不同植株部位中碳、氮、磷的含量变化,分析了潮滩沉积物中碳、氮、磷的垂向和水平分布特征与规律,探讨了不同生态带以及潮滩植被对碳、氮、磷等生源要素的富集作用。对比分析结果表明:苏北潮滩湿地各生态带对不同的测量指标有着不同的富集作用,互花米草滩的总有机碳、总氮和有机磷含量要远大于其他几个生态带,光滩沉积物中总磷的含量最高; 粒度效应是控制互花米草前缘地带以及互花米草滩沉积物中有机碳和氮分布的一个重要因素,盐蒿和芦苇滩中有机碳和氮的分布更多的是受粒度之外的其他因素影响; 不同生态带表层沉积物中的C/N比值分布,大致可反映其有机物来源的差异,而不同生态带中柱状沉积物中的C/N比值相对接近,很难根据C/N比值大小来对不同生态带中的有机物来源进行判断,这可能是埋藏在柱状沉积物中的有机物更多的受到了早期成岩作用造成的。植被对潮滩湿地中碳、氮、磷的分布有着重要影响,3种物质在互花米草、盐蒿和芦苇中的含量差别不是很大,因此潮滩植被对沉积物中上述3种物质的贡献差别主要是由不同植被的生物量和其所处环境的沉积动力差异造成的。 相似文献
20.
Saburo Sakai Masaru Nakaya Yoshikazu Sampei David L. Dettman Katsumi Takayasu 《Environmental Earth Sciences》2013,68(7):1999-2006
The relationship among H2S, total organic carbon (TOC), total sulfur (TS) and total nitrogen contents of surface sediments (0–1 cm) was examined to quantify the relationship between H2S concentrations and TOC content at the sediment water interface in a coastal brackish lake, Nakaumi, southwest Japan. In this lake, bottom water becomes anoxic during summer due to a strong halocline. Lake water has ample dissolved SO4 2? and the surface sediments are rich in planktic organic matter (C/N 7–9), which is highly reactive in terms of sulfate reduction. In this setting the amount of TOC should be a critical factor regulating the activity of sulfate reduction and H2S production. In portions of the lake where sediment TOC content is less than 3.5 %, H2S was very low or absent in both bottom and pore waters. However, in areas with TOC >3.5 %, H2S was correlated with TOC content (pore water H2S (ppm) = 13.9 × TOC (%) ? 52.1, correlation coefficient: 0.72). H2S was also present in areas with sediment TS above 1.2 % (present as iron sulfide), which suggests that iron sulfide formation is tied to the amount of TOC. Based on this relationship, H2S production has progressively increased after the initiation of land reclamation projects in Lake Nakaumi, as the area of sapropel sediments has significantly increased. This TOC–H2S relationship at sediment–water interface might be used to infer H2S production in brackish–lagoonal systems similar to Lake Nakaumi, with readily available SO4 2? and reactive organic matter. 相似文献