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Vishwas B. Khodse Narayan B. Bhosle V. V. Gopalkrishna 《Journal of Earth System Science》2009,118(2):147-156
Suspended particulate matter (SPM) of surface seawaters was collected during December 2003 to October 2004 at 10 stations
in the Bay of Bengal, and analyzed for particulate organic carbon (POC), total particulate nitrogen (TPN), total particulate
carbohydrate (TPCHO) and total particulate uronic acids (TPURA). The concentrations of POC, TPCHO and TPURA varied from 4.80
to 29.12, 0.85 to 4.24, 0.09 to 0.91 μM C, respectively. The TPCHO-C and TPURA-C accounted for 6.6–32.5% and 0.87–3.65% of
POC. The trends observed for the distribution of these compounds were generally similar to those recorded for the distribution
of chlorophyll a (Chl a). The C/N ratios varied from 3.2 to 22.3 with most of the values being < 10. This suggests that the organic matter was mostly
derived from phytoplankton and bacteria. Relatively low C/N ratios and high TPCHO yield imply that freshly derived organic
matter was present during SWM and FIM. Our data suggest that the quality and quantity of organic matter varied spatially and
seasonally. 相似文献
3.
P. V. Bhaskar Evonne Cardozo Asha Giriyan Anita Garg Narayan B. Bhosle 《Estuaries and Coasts》2000,23(5):722-734
Data on hydrography, nutrients, suspended particles, and sedimented particles were collected at weekly intervals from November to May during 1995 to 1997 at a station in the coastal waters of Dona Paula Bay, India. Suspended and sedimented particles were analyzed for total suspended matter (SPM), total sedimented particulate matter (TPM), particulate organic carbon (POC), particulate organic nitrogen (PON), chlorophylla (chla), and diatom abundance. Variations in hydrography and nutrients influenced the quantity and composition of sedimented particles. The TPM, POC, PON, and chla fluxes showed small-scale seasonal variations and were higher in the summer (February to May) than in the winter (November to January). Resuspension of carbon accounted for approximately 25% of the gross POC and was highest in April 1997 (45%). The mean net POC flux was 197±90 mg C m−2 d−1 and accounts for 4.6% of the TPM. The average C∶N (w∶w) ratio of the sedimented material was 13.2±6.6. The POC:chla ratio was relatively higher in the sedimented material as compared to the suspended material. The particulate carbon reaching the bottom sediment was 39% of the primary production. The low organic carbon concentration (approximately 0.1% of dry sediment) in the sediments implies that about 98% of the sedimented carbon was either consumed at the sedimentwater interface or resuspended/advected before it was finally buried into the sediments. 相似文献
4.
Particulate organic carbon (POC) was measured for 77 water samples collected over a 3000 m water column along 88° E in the
central Bay of Bengal. The POC values varied from 80 to 895 μg per litre at the surface and 171 to 261 μg per litre at 2000
m. The POC decreased with increasing water depth at all the stations. Deep water concentrations of POC were higher than those
reported from other oceanic waters. Distribution of POC was not influenced by water masses. The POC was not significantly
correlated with chlorophylla. 相似文献
5.
A conceptual isotopic/geochemical model is presented to explain the variation of major, trace and rare earth element (REE)
geochemistry and Sr isotope systematics in suspended particulate matter (SPM) as a function of particle/colloid size. This
conceptual model is an extension of a previous investigation of the origin of SPM in the Murray-Darling River system (MDRS)
that utilised Sr isotope systematics to examine aspects of SPM (particle/colloid) origin, structure and mineralogy. The geochemical
processes that give rise to the often coherent trends in major, trace and REE geochemistry and Sr isotopic signature as a
function of particulate (<1 μm) and colloidal (>1 μm) size in the MDRS have been identified using an enhanced SPM size fractionation
technique as a basis to not only obtain a broad range of particle/colloid size ranges, but also to provide sufficient material
for subsequent geochemical and isotopic analysis. The conceptual isotopic/geochemical model proposed here contains three major
components: (i) the differential weathering of micas and alkali (K-) feldspars to form the majority of the particulate (<1
μm) fractions (high 87Sr/86Sr ratio), which have a geochemical and Sr isotopic signature that closely resembles precursor
mineralogies, (ii) the differential weathering of Na, Ca-feldspars (plagioclase) which decompose to form clay minerals in
the colloidal (>1 μm) fractions (low 87Sr/86Sr ratio), with a range of geochemical signatures related to the relative proportions
of inorganic and organic constituents, and (iii) the presence of natural organic matter as coatings on the particulate (<1
μm) and colloidal (>1 μm) matter and possibly as organo-colloids which exert an increasing influence in particular on bulk
colloid geochemistry with decreasing colloid size. This conceptual isotopic/geochemical model also accounts for the distinct
variation in major, trace and REE geochemistry and Sr isotopic systematics between the particulate (<1 μm) and colloidal (>1
μm) fractions, the variation being primarily a function of the distinctly different precursor mineralogies of the SPM fractions
and geochemical fractionation during the weathering and transport. Additionally, this model explains a systematic fractionation
of REE apparent within colloidal (>1 μm) fractions. Statisitcal (hierachical cluster) analysis of two particulate and three
colloidal fractions from 23 samples from the MDRS is used as a basis to investigate geochemical and mineralogical associations
within the particulate and colloidal size fractions and to provide additional supporting evidence for the conceptual isotopic/geochemical
model.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
6.
Biochemical composition of surface sediment samples from off major and minor rivers along the east coast of India revealed that spatial distribution of sediment organic carbon (SOC) composition was mainly governed by differential characteristics of discharged water and associated biogeochemical processes in the water column. The northwest (NW) region of coastal Bay of Bengal was influenced by discharges from Ganges river while peninsular (monsoonal) rivers influenced the southwest (SW) region. The NW region characterized by low nutrients suspended particulate matter (SPM), high phytoplankton biomass in the water column and high SOC while contrasting to that observed in the SW region. The isotopic ratios of SOC (?22 ‰) in the NW region were close to that of organic matter derived from phytoplankton (?23 ‰) suggesting in situ production is the major source whereas terrigeneous source contributed significantly in the SW region (?19.6 ‰). Though low in situ biological production in the SW region, relatively higher total carbohydrates (TCHO) were found than in the NW and insignificant difference of total and free amino acid concentrations between NW and SW were resulted from faster removal of organic matter to the sediment in association with SPM in the SW region. Higher proteins concentrations than total amino acids indicate that nitrogenous organic matter is preserved in the former form. The protein to TCHO ratio was lower in the SW suggesting significant contribution of aged and non-living organic matter in this region. 相似文献
7.
珠江中下游颗粒有机质的碳氮℃稳定同位素、氨基酸和木质素组成及其地球化学意义 总被引：2，自引：0，他引：2
从东江到珠江口采集了悬浮颗粒物,通过测定总有机质的元素（TOC、TN）、同位素（δ13C、δ15N）组成以及生物标志物（氨基酸、木质素）等地球化学性质,来揭示颗粒有机质的来源和组成。结果表明,浮游生物（13%-52%）和土壤（45%-77%）是珠江颗粒有机质的主要来源,植物（0%-11%）对颗粒物的贡献较小。颗粒有机质含有高比例的氨基酸碳（TAAC）,说明浮游生物对颗粒物的重要性。氨基酸的降解指数（DI）在-0.51到0.79之间,说明这些水生来源有机质的降解程度比较小。木质素的降解参数（Ad/Al、3,5-BD/V）较大,表明珠江颗粒有机碳的陆源来源主要是土壤。在颗粒物中检测到了少量的二氨基庚二酸（Dapa）,说明细菌对颗粒有机碳也有所贡献。不同环境中颗粒物的木质素组成主要与颗粒物丰度和粒径有关：（1）相对于河流,水库颗粒物中的木质素含量显著偏低,降解程度更高;（2）相对于中游,下游颗粒物丰度较高,木质素含量较高。 相似文献
8.
《Geochimica et cosmochimica acta》1987,51(9):2579-2586
The St. Lawrence River discharges a substantial volume of water (405 km3/a) containing suspended (SPM; 3.42 × 106t) and dissolved (68.0 × 106t) materials to the Gulf of St. Lawrence. The total load contains organic carbon in paniculate (POC; 3–14% of SPM), and dissolved (DOC; 3.76 ± 0.63 mg/l) form. The concentration of POC (and particulate organic nitrogen) is positively correlated with discharge (increased during the spring flood and the fall enhancement of flow), but concentration of DOC is not so simply related to discharge. In consequence, the total organic carbon (POC + DOC) load is relatively invariant, and increased annually by only 2–3% despite a progressive increase of 8% in discharge over the years of this study. Seasonal differences in the composition of the particulate organic matter (POM) are interpreted as reflecting dominant contributions from within-river production in summer and from terrestrial sources in spring and fall. In years when the annual discharge was greater than average, a higher proportion of the POM was terrigenous. The organic matter in surface sediments of the estuary to which the river discharges is predominantly of terrestrial provenance. 相似文献
9.
We measured dissolved and particulate organic carbon (DOC and POC) in samples collected along 13 transects of the salinity gradient of Chesapeake Bay. Riverine DOC and POC end-members averaged 232±19 μM and 151±53 μM, respectively, and coastal DOC and POC end-members averaged 172±19 μM and 43±6 μM, respectively. Within the chlorophyll maximum, POC accumulated to concentrations 50–150 μM above those expected from conservative mixing and it was significantly correlated with chlorophylla, indicating phytoplankton origin. POC accumulated primarily in bottom waters in spring, and primarily in surface waters in summer. Net DOC accumulation (60–120 μM) was observed within and downstream of the chlorophyll maximum, primarily during spring and summer in both surface and bottom waters, and it also appeared to be derived from phytoplankton. In the turbidity maximum, there were also net decreases in chlorophylla (?3 μg l?1 to ?22 μg l?1) and POC concentrations (?2 μM to ?89 μM) and transient DOC increases (9–88 μM), primarily in summer. These occurred as freshwater plankton blooms mixed with turbid, low salinity seawater, and we attribute the observed POC and DOC changes to lysis and sedimentation of freshwater plankton. DOC accumulation in both regions of Chesapeake Bay was estimated to be greater than atmospheric or terrestrial organic carbon inputs and was equivalent to ≈10% of estuarine primary production. 相似文献
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Stable carbon isotope (δ13C) analysis was used in the Peridido Estuary, Florida U.S. to determine the predominant carbon source that supports the bacterial assemblage. Stable carbon isotope values were measured in the suspended particulate matter (SPM), dissolved organic and inorganic matter, and bacteria. Stable nitrogen isotope (δ15N) ratios were measured in SPM and nitrate to assist in understanding carbon cycling through the estuary. Analyses were conducted on samples from riverine, coastal, and anthropogenic sources and compared with samples from the bay. Stable isotope ratio analysis was coupled with estimates of mixing of riverine and coastal waters into the bay. Preliminary observation of the °13C data indicates that terrestrial organic matter is the primary carbon source that is assimilated by bacteria in the ecosystem. Stable isotope data from carbon and nitrogen pools in combination with analysis of estuarine current velocities indicates that primary production is an important factor in the carbon cycle. This study demonstrates the importance of stable isotope analysis of multiple carbon and nitrogen pols to assess sources and cycling of organic matter. 相似文献
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As a kind of marine organic matter with important geochemical characteristics, amino sugars can effectively reflect the source, diagenetic state and mineralization process of organic matter by their concentration and composition in marine environment. This article systematically concluded the research progresses of amino sugars from the aspects of their source, composition and distribution characteristics in marine environment, and the role as a biomarker indicating source and diagenetic state of marine organic matter. The result showed that the macromolecular morphology, the oxygen and nutrient level and the sedimentary environment could affect the reactivity of amino sugars. The higher ratios of glucosamine to galactosamine (GlcN/GalN) and the Total Hydrolysable Amino Acids to Total Hydrolysable Amino Sugars (THAA/THAS) can reflect the fresh planktonic organic matter source and the lower ratios can reflect the conversion from planktonic to bacterial organic matter. The carbon and nitrogen normalized yield of total hydrolysable amino sugars, however, could give contradictory results depending on the relative contribution of the source and degradation degree of organic matter. Muramic acid is suitable to estimate the contribution of relatively fresh bacteria organic matter to particulate and sediment organic matter, but it is not suitable for applying in the dissolved organic matter because of its very low concentration leading from its rapid recycle. It is critical to enhance the research on the contribution of different microorganisms to amino sugars and differentiate the influence of organic matter source and degradation on amino sugars in marine environment. The research on the conversion and fate of amino sugars in marine environment is also needed. 相似文献
14.
Carbon isotope ratio analysis of particulate, planktonic, and sedimentary organic carbon and dissolved inorganic carbon has been used to study the sources and sinks of the organic carbon in the St. Lawrence Estuary and Gulf of St. Lawrence, Canada. Particulate organic carbon (POC) isotope ratios in the upper St. Lawrence Estuary are uniform and indistinguishable from those of POC in the St. Lawrence River and of planktonic organic carbon in both areas. The abundance of freshwater diatoms in the upper Estuary suggests that upper Estuary POC is predominantly “fresh” organic matter of riverborne origin. Upper Estuary POC is isotopically different from POC in the lower St. Lawrence Estuary and Gaspé regions, but is not different from POC from the surface waters of the open Gulf of St. Lawrence. The isotopic composition of planktonic organic carbon mirrors that of the POC, indicating that the POC in the lower Estuary and Gulf is also “fresh” organic matter. Since the lower Estuary POC forms an isotopic barrier between the upper Estuary POC and the Gulf of St. Lawrence POC, there appears to be little mixing of POC between these three reservoirs. Therefore POC in the lower Estuary and Gulf is most likely both produced and deposited (or degraded) in situ.An examination of carbon isotope ratio differences between the planktonic and dissolved inorganic carbon reservoirs shows that this difference varies significantly and somewhat unpredictably between sectors of the study area. Interpretation of environmental carbon isotope data on the basis of an assumed, constant fractionation factor may be subject to large errors. Direct measurement of both reservoirs is obviously preferable. 相似文献
15.
In order to investigate how monsoons influence biogeochemical fluxes in the ocean, twelve time-series sediment traps were
deployed at six locations in the northern Indian Ocean. In this paper we present particle flux data collected during May 1986
to November 1991 and November 1987 to November 1992 in the Arabian Sea and Bay of Bengal respectively. Particle fluxes were
high during both the SW and NE monsoons in the Arabian Sea as well as in the Bay of Bengal. The mechanisms of particle production
and transport, however, differ in both the regions.
In the Arabian Sea, average annual fluxes are over 50gm-2y-1 in the western Arabian Sea and less than 27gm-2 y-1 in the central part. Biogenic matter is dominant at sites located near upwelling centers, and is less degraded during peak
flux periods. High particle fluxes in the offshore areas of the Arabian Sea are caused by injection of nutrients into the
euphotic zone due to wind-induced mixed layer deepening. In the Bay of Bengal, average annual fluxes are highest in the central
Bay of Bengal (over
50gm-2y-1) and are least in the southern part of the Bay (37gm-2y-1). Particle flux patterns coincide with freshwater discharge patterns of the Ganges-Brahmaputra river system. Opal/carbonate
and organic carbon/carbonate carbon ratios increase during the SW monsoon due to variations in salinity and productivity patterns
in the surface waters as a result of increased freshwater and nutrient input from rivers.
Comparison of S years data show that fluxes of biogenic and lithogenic particulate matter are higher in the Bay of Bengal
even though the Arabian Sea is considered to be more productive. Our results indicate that in the northern Indian Ocean interannual
variability in organic carbon flux is directly related to the strength and intensity of the SW monsoon while its transfer
from the upper layers to the deep sea is partly controlled by input of lithogenic matter from adjacent continents. 相似文献
16.
John H. Trefry Simone Metz Terry A. Nelsen Robert P. Trocine Brian J. Eadie 《Estuaries and Coasts》1994,17(4):839-849
This study was designed to determine the amount of particulate organic carbon (POC) introduced to the Gulf of Mexico by the Mississippi River and assess the influence of POC inputs on the development of hypoxia and burial of organic carbon on the Louisiana continental shelf. Samples of suspended sediment and supporting hydrographic data were collected from the river and >50 sites on the adjacent shelf. Suspended particles collected in the river averaged 1.8±0.3% organic carbon. Because of this uniformity, POC values (in μmol l?1) correlated well with concentrations of total suspended matter. Net transport of total organic carbon by the Mississippi-Atchafalaya River system averaged 0.48×1012 moles y?1 with 66% of the total organic carbon carried as POC. Concentrations of POC decreased from as high as 600 μmol l?1 in the river to <0.8 μmol l?1 in offshore waters. In contrast, the organic carbon fraction of the suspended matter increased from <2% of the total mass in the river to >35% along the shelf at ≥10 km from the river mouth. River flow was a dominant factor in controlling particle and POC distributions; however, time-series data showed that tides and weather fronts can influence particle movement and POC concentrations. Values for apparent oxygen utilization (AOU) increased from ～60 μmol l?1 to >200 μmol l?1 along the shelf on approach to the region of chronic hypoxia. Short-term increases in AOU were related to transport of more particle-rich waters. Sediments buried on the shelf contained less organic carbon than incoming river particles. Orgamic carbon and δ13C values for shelf sediments indicated 3 that large amounts of both terrigenous and marine organic carbon are being decomposed in shelf waters and sediments to fuel observed hypoxia. 相似文献
17.
Reactive dissolved Hg (HgR), non-reactive dissolved Hg (HgNR), particulate Hg (HgP), dissolved organic C (DOC), particulate organic C (POC), salinity and other interpretative parameters were determined in water samples collected in the North Channel and in adjacent areas of the Tagus estuary (Portugal). Higher concentrations of both dissolved and particulate Hg in the North Channel indicate a pollution source and raise the possibility of Hg escaping to adjacent areas by tidal action. This transport was confirmed by the increase of HgR with salinity and HgNR with DOC, along a longitudinal axis paralleling the North Channel. Apparently, Hg leaving this channel is progressively complexed by inorganic and organic ligands. Near the mouth of the estuary, values decreased reflecting dilution with seawater. Moreover the HgP:POC ratio also increased seaward, suggesting mixing with Hg enriched particles that escaped the North Channel, or incorporation of dissolved Hg species in river-derived particles. These results suggest that the pathway of anthropogenic Hg in contaminated waters may be identified by their enrichment in organic matter, both in the dissolved and particulate fraction. 相似文献
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对南海表层沉积物与沉降颗粒物有机碳的δ13C进行了对比研究,从古环境再造方面探讨了陆源和海源对南海表层沉积物的贡献。南海表层沉积物有机碳的δ13C比沉降颗粒物中有机碳的δ13C偏重表明,Suess效应对南海现代过程的影响不可忽视,两者的δ13C差值反映了Suess效应对南海现代过程的影响程度。利用两者的δ13C差值,对现代陆源和海源有机碳的δ13C进行修正后,计算得到,在南海陆架周围表层沉积物的有机碳中,陆源的比例为48%,海源的比例为52%;在远离陆架的表层沉积物的有机碳中,陆源的比例为14%,海源的比例为86%。 相似文献
19.
In the Antarctic zone, integrated studies of particulate matter in surface waters and the snow-ice cover were carried out
by means of geochemical (the concentrations of particulate matter, Corg, hydrocarbons, lipids, and chlorophyll a) and optical techniques. Correlations between the treated compounds were found. A regression equation was created that enabled
us to evaluate immediately the amount of particulate matter using the parameter of light attenuation by seawater. New data
were obtained for the processes of accumulation of particulate matter and organic compounds under ice formation. 相似文献
20.
Temporal changes in benthic foraminiferal morpho-groups were suggested as an effective proxy to reconstruct past monsoon intensity from the Arabian Sea. Here, in order to test the applicability of temporal variation in morpho-groups to reconstruct past monsoon intensity from the Bay of Bengal, we have documented recent benthic foraminiferal distribution from the continental shelf region of the northwestern Bay of Bengal. Based on the external morphology, benthic foraminifera were categorized into rounded symmetrical (RSBF) and angular asymmetrical benthic foraminifera (AABF). Additionally, a few other dominant groups were also identified based on test composition (agglutinated, calcareous) and abundance (Asterorotalids and Nonions). The relative abundance of each group was compared with the ambient physico-chemical conditions, including dissolved oxygen, organic matter, salinity and temperature. We report that the RSBF are abundant in comparatively warm and well oxygenated waters of low salinity, suggesting a preference for high energy environment, whereas AABF dominate relatively cold, hypersaline deeper waters with low dissolved oxygen, indicating a low energy environment. The agglutinated foraminifera, Asterorotalids and Nonions dominate shallow water, low salinity regions, whereas the calcareous benthic foraminiferal abundance increases away from the riverine influx regions. Food availability, as estimated from organic carbon abundance in sediments, has comparatively less influence on faunal distribution in the northwestern Bay of Bengal, as compared to dissolved oxygen, temperature and salinity. We conclude that the factors associated with freshwater influx affect the distribution of benthic foraminiferal morpho-groups in the northwestern Bay of Bengal and thus it can be used to reconstruct past monsoon intensity from the Bay of Bengal. 相似文献