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1.
High sensitivity observations were performed at 1.2- and 3-mm wavelengths with the IRAM 30-m telescope (Spain) between April 1996 and December 1999 to investigate the nitrile composition of Titan's stratosphere. A part of our dataset consists of high resolution spectra of HC14N taken at 88.6 GHz as well as spectra of HC15N recorded at 258.16 GHz. From a thorough analysis of both lines and with the help of appropriate radiative transfer calculations we show that the isotopic ratio 15N/14N is strongly enhanced compared to the terrestrial value. We propose that the range 3.9-4.5 should be considered as a basis for the enrichment factor. Five individual lines of HC3N were measured at 39-kHz resolution using a frequency-switched technique. Several CH3CN features were recorded at 78-kHz resolution in two transitions around 147.6 and 220.7 GHz. The high spectral resolution and the good signal-to-noise ratio affecting the spectra permit us to retrieve disk-averaged vertical profiles for HCN up to 450 km and for HC3N and CH3CN up to 500 km. Comparison of our inferred vertical profiles with relevant results of presently published photochemical models is presented. We show that the profiles of HCN and HC3N predicted by various authors below 450-km altitude appear inconsistent with our new observations. We find that the three distributions present very different gradients of abundance below 200-km altitude down to the condensation levels around 80 km. In the upper stratosphere HC3N and CH3CN have approximately the same mixing ratio of about 4×10−8 at 450 km, at least one order of magnitude lower than that of HCN. In the same time, another nitrile HC5N has been searched for by observing four transitions located between 109 and 221 GHz. As no spectral features could be detected after several hours of integration time, we propose an upper limit for the mixing ratio equal to 4×10−10 assuming a uniform distribution of this compound in the lower stratosphere.  相似文献   

2.
Detections and upper limits to the continuum emission (1 ≤ λ ≤6 cm) and spectral line emission (OH, CO, CS, HCN, HCO+, CN, CH3CN, CH3C2H, NH3, H2O, HC3N, CH3CH2CN) are reported from radio observations of Comets 1983d and 1983e. Comparison is made with observations of CN at optical wavelengths. These results may be useful in planning future cometary observations.  相似文献   

3.
Using synthetic spectra derived from an updated model atmosphere together with a continuum model that includes contributions from haze, cloud and ground, we have re-analyzed the recently published (Geballe et al., 2003, Astrophys. J. 583, L39-L42) high-resolution 3 μm spectrum of Titan which contains newly-detected bands of HCN (in emission) and C2H2 and CH3D (in absorption), in addition to previously detected bands of CH4. In the 3.10-3.54 μm interval the analysis yields strong evidence for the existence of a cloud deck or optically thick haze layer at about the 10 mbar (∼ 100 km) level. The haze must extend well above this altitude in order to mask the strong CH4 lines at 3.20-3.50 μm. These cloud and haze components must be transparent at 2.87-2.92 μm, where analysis of the CH3D spectrum demonstrates that Titan's surface is glimpsed through a second cloud deck at about the 100 mbar (∼ 50 km) level. Through a combination of areal distribution and optical depth this cloud deck has an effective transmittance of ∼ 20%. The spectral shape of Titan's continuum indicates that the higher altitude cloud and haze particles responsible for suppressing the CH4 absorptions have a largely organic make-up. The rotational temperature of the HCN ranges from 140 to 180 K, indicating that the HCN emission occurs over a wide range of altitudes. This emission, remodeled using an improved collisional deactivation rate, implies mesospheric mixing ratio curves that are consistent with previously predictions. The stratospheric and mesospheric C2H2 mixing ratios are ∼10−5, considerably less than previous model predictions (Yung et al., 1984), but approximately consistent with recent observational results. Upper limits to mixing ratios of HC3N and C4H2 are derived from non-detections of those species near 3.0 μm.  相似文献   

4.
The apparition of Comet C/1996 B2 (Hyakutake) offered an unexpected and rare opportunity to probe the inner atmosphere of a comet with high spatial resolution and to investigate with unprecedented sensitivity its chemical composition. We present observations of over 30 submillimeter transitions of HCN, H13CN, HNC, HNCO, CO, CH3OH, and H2CO in Comet Hyakutake carried out between 1996 March 18 and April 9 at the Caltech Submillimeter Observatory. Detections of the H13CN (4–3) and HNCO (160,16–150,15) transitions represent the first observations of these species in a comet. In addition, several other transitions, including HCN (8–7), CO (4–3), and CO (6–5) are detected for the first time in a comet as is the hyperfine structure of the HCN (4–3) line. The observed intensities of the HCN (4–3) hyperfine components indicate a line center optical depth of 0.9 ± 0.2 on March 22.5 UT. The HCN/HNC abundance ratio in Comet Hyakutake at a heliocentric distance of 1 AU is similar to that measured in the Orion extended ridge— a warm, quiescent molecular cloud. The HCN/H13CN abundance ratio implied by our observations is 34 ± 12, similar to that measured in giant molecular clouds in the galactic disk but significantly lower than the Solar System12C/13C ratio. The low HCN/H13CN abundance ratio may be in part due to contamination by an SO2line blended with the H13CN (4–3) line. In addition, chemical models suggest that the HCN/H13CN ratio can be affected by fractionation during the collapse phase of the protosolar nebula; hence a low HCN/H13CN ratio observed in a comet is not inconsistent with the solar system12C/13C isotopic ratio. The abundance of HNCO relative to water derived from our observations is (7 ± 3) × 10−4. The HCN/HNCO abundance ratio is similar to that measured in the core of Sagittarius B2 molecular cloud. Although a photo-dissociative channel of HNCO leads to CO, the CO produced by HNCO is a negligible component of cometary atmospheres. Production rates of HCN, CO, H2CO, and CH3OH are presented. Inferred molecular abundances relative to water are typical of those measured in comets at 1 AU from the Sun. The exception is CO, for which we derive a large relative abundance of 30%. The evolution of the HCN production rate between March 20 and March 30 suggests that the increased activity of the comet was the cause of the fragmentation of the nucleus. The time evolution of the H2CO emission suggests production of this species from dust grains.  相似文献   

5.
Mid- and far-infrared spectra from the Composite InfraRed Spectrometer (CIRS) have been used to determine volume mixing ratios of nitriles in Titan's atmosphere. HCN, HC3N, C2H2, and temperature were derived from 2.5 cm−1 spectral resolution mid-IR mapping sequences taken during three flybys, which provide almost complete global coverage of Titan for latitudes south of 60° N. Three 0.5 cm−1 spectral resolution far-IR observations were used to retrieve C2N2 and act as a check on the mid-IR results for HCN. Contribution functions peak at around 0.5-5 mbar for temperature and 0.1-10 mbar for the chemical species, well into the stratosphere. The retrieved mixing ratios of HCN, HC3N, and C2N2 show a marked increase in abundance towards the north, whereas C2H2 remains relatively constant. Variations with longitude were much smaller and are consistent with high zonal wind speeds. For 90°-20° S the retrieved HCN abundance is fairly constant with a volume mixing ratio of around 1 × 10−7 at 3 mbar. More northerly latitudes indicate a steady increase, reaching around 4 × 10−7 at 60° N, where the data coverage stops. This variation is consistent with previous measurements and suggests subsidence over the northern (winter) pole at approximately 2 × 10−4 m s−1. HC3N displays a very sharp increase towards the north pole, where it has a mixing ratio of around 4 × 10−8 at 60° N at the 0.1-mbar level. The difference in gradient for the HCN and HC3N latitude variations can be explained by HC3N's much shorter photochemical lifetime, which prevents it from mixing with air at lower latitude. It is also consistent with a polar vortex which inhibits mixing of volatile rich air inside the vortex with that at lower latitudes. Only one observation was far enough north to detect significant amounts of C2N2, giving a value of around 9 × 10−10 at 50° N at the 3-mbar level.  相似文献   

6.
Sang J. Kim  John Caldwell 《Icarus》1982,52(3):473-482
The 8.6-μm emission feature of Titan's infrared spectrum was analyzed using the Voyager temperature-pressure profile. Although both C3H8 and CH3D have bands at that wavelength, we show that CH3D dominates the observed emission on Titan. We derived a CH3D/CH4 mixing ratio using this band and the strong CH4 band at 7.7 μm. The corresponding D/H ratio is 4.2?1.5+2 × 10?4, neglecting deuterium fractionation with other molecules. The main uncertainty in this value comes from the continuum emission characteristics. The D/H ratio is apparently significantly enhanced on Titan with respect to published values for Saturn.  相似文献   

7.
Lis  D. C.  Mehringer  D. M.  Benford  D.  Gardner  M.  Phillips  T. G.  Bockelée-Morvan  D.  Biver  N.  Colom  P.  Crovisier  J.  Despois  D.  Rauer  H. 《Earth, Moon, and Planets》1997,78(1-3):13-20
We present millimeter-wave observations of HNCO, HC3N, SO, NH2CHO, H13CN, and H3O+ in comet C/1995 O1 (Hale-Bopp)obtained in February–April, 1997 with the Caltech Submillimeter Observatory (CSO). HNCO, first detected at the CSO in comet C/1996B2 (Hyakutake), is securely confirmed in comet Hale-Bopp via observations of three rotational transitions. The derived abundance with respect to H2O is (4-13) × 10-4. HC3N, SO, and NH2CHO are detected for the first time in a comet. The fractional abundance of HC3N based on observations of three rotational lines is (1.9 ± 0.2) × 10-4. Four transitions of SO are detected and the derived fractional abundance, (2-8) ×10-3, is higher than the upper limits derived from UV observations of previous comets. Observations of NH2CHO imply a fractional abundance of (1-8) × 10-4. H3O is detected for the first time from the ground. The H13CN (3-2)transition is also detected and the derived HCN/H13CN abundance ratio is 90 ± 15, consistent with the terrestrial12C/13C ratio. In addition, a number of other molecular species are detected, including HNC, OCS, HCO+, CO+, and CN(the last two are first detections in a comet at radio wavelengths). This revised version was published online in July 2006 with corrections to the Cover Date.  相似文献   

8.
R.K. Khanna 《Icarus》2005,178(1):165-170
Infrared spectra of crystalline HC3N and C2H2 were investigated at several temperatures between 15 and 150 K. The characteristics of the 505 and 753 cm−1 bands of HC3N are in complete agreement with the emission spectral data on Titan obtained by the Voyager IRIS instrument, thus confirming the identification of crystalline HC3N on Titan. A composite spectrum in the 720-800 cm−1 region, with contributions from HC3N and C2H2 in crystalline phases, reproduces the Voyager emission data in that region, thus providing a suggestion for the identification of crystalline C2H2 on Titan.  相似文献   

9.
The abundances of PH3, CH3D, and GeH4 are derived from the 2100- to 2250-cm?1 region of the Voyager 1 IRIS spectra. No evidence is seen for large-scale variations of the phosphine abundance over Jovian latitudes between ?30 and +30°. In the atmospheric regions corresponding to 170–200°K, the derived PH3/H2 value is (4.5 ± 1.5) × 10?7 or 0.75 ± 0.25 times the solar value. This result, compared with other PH3 determinations at 10 μm, suggests than the PH3/H2 ratio on Jupiter decreases with atmospheric pressure. In the 200–250°K region, we derive, within a factor of 2, CH3D/H2 and GeH4/H2 ratios of 2.0 × 10?7 and 1.0 × 10?9, respectively. Assuming a C/H value of 1.0 × 10?3, as derived from Voyager, our CH3D/H2 ratio implies a D/H ratio of 1.8 × 10?5, in reasonable agreement with the interstellar medium value.  相似文献   

10.
Mid-infrared limb spectra in the range 600-1400 cm−1 taken with the Composite InfraRed Spectrometer (CIRS) on-board the Cassini spacecraft were used to determine vertical profiles of HCN, HC3N, C2H2, and temperature in Titan's atmosphere. Both high (0.5 cm−1) and low (13.5 cm−1) spectral resolution data were used. The 0.5 cm−1 data gave profiles at four latitudes and the 13.5 cm−1 data gave almost complete latitudinal coverage of the atmosphere. Both datasets were found to be consistent with each other. High temperatures in the upper stratosphere and mesosphere were observed at Titan's northern winter pole and were attributed to adiabatic heating in the subsiding branch of a meridional circulation cell. On the other hand, the lower stratosphere was much colder in the north than at the equator, which can be explained by the lack of solar radiation and increased IR emission from volatile enriched air. HC3N had a vertical profile consistent with previous ground based observations at southern and equatorial latitudes, but was massively enriched near the north pole. This can also be explained in terms of subsidence at the winter pole. A boundary observed at 60° N between enriched and un-enriched air is consistent with a confining polar vortex at 60° N and HC3N's short lifetime. In the far north, layers were observed in the HC3N profile that were reminiscent of haze layers observed by Cassini's imaging cameras. HCN was also enriched over the north pole, which gives further evidence for subsidence. However, the atmospheric cross section obtained from 13.5 cm−1 data indicated a HCN enriched layer at 200-250 km, extending into the southern hemisphere. This could be interpreted as advection of polar enriched air towards the south by a meridional circulation cell. This is observed for HCN but not for HC3N due to HCN's longer photochemical lifetime. C2H2 appears to have a uniform abundance with altitude and is not significantly enriched in the north. This is consistent with observations from previous CIRS analysis that show increased abundances of nitriles and hydrocarbons but not C2H2 towards the north pole.  相似文献   

11.
M.H. Moore  R.L. Hudson 《Icarus》2003,161(2):486-500
Infrared spectra and radiation chemical behavior of N2-dominated ices relevant to the surfaces of Triton and Pluto are presented. This is the first systematic IR study of proton-irradiated N2-rich ices containing CH4 and CO. Experiments at 12 K show that HCN, HNC, and diazomethane (CH2N2) form in the solid phase, along with several radicals. NH3 is also identified in irradiated N2 + CH4 and N2 + CH4 + CO. We show that HCN and HNC are made in irradiated binary ice mixtures having initial N2/CH4 ratios from 100 to 4, and in three-component mixtures have an initial N2/(CH4 + CO) ratio of 50. HCN and HNC are not detected in N2-dominated ices when CH4 is replaced with C2H6, C2H2, or CH3OH.The intrinsic band strengths of HCN and HNC are measured and used to calculate G(HCN) and G(HNC) in irradiated N2 + CH4 and N2 + CH4 + CO ices. In addition, the HNC/HCN ratio is calculated to be ∼1 in both icy mixtures. These radiolysis results reveal, for the first time, solid-phase synthesis of both HCN and HNC in N2-rich ices containing CH4.We examine the evolution of spectral features due to acid-base reactions (acids such as HCN, HNC, and HNCO and a base, NH3) triggered by warming irradiated ices from 12 K to 30-35 K. We identify anions (OCN−, CN−, and N3−) in ices warmed to 35 K. These ions are expected to form and survive on the surfaces of Triton and Pluto. Our results have astrobiological implications since many of these products (HCN, HNC, HNCO, NH3, NH4OCN, and NH4CN) are involved in the syntheses of biomolecules such as amino acids and polypeptides.  相似文献   

12.
The reaction of CN? with cyanoacetylene (HC3N), has been studied as a function of the HC3N pressure in a quadrupole tandem mass spectrometer. The mass spectra revealed the fast depletion of the CN? parent ion and formation of larger anions of rapidly growing size. Most of the ions observed were found to belong to two series of products: (HC3N)x·C2p+1N? and (HC3N)x·C2pN? resulting from the sequential additions of HC3N molecules and loss of HCN or HCCN molecules. The mechanism and energetics of the first two reaction steps are briefly discussed. The laboratory data are compared with those from the Cassini CAPS-ELS spectrometer. It is believed that the reactions observed could account for the growth of anions in Titan’s ionosphere.  相似文献   

13.
Bockelée-Morvan  D.  Wink  J.  Despois  D.  Colom  P.  Biver  N.  Crovisier  J.  Gautier  D.  Gérard  E.  Lellouch  E.  Moreno  R.  Paubert  G.  Rauer  H.  Davies  J. K.  Dent  W. R. F. 《Earth, Moon, and Planets》1997,78(1-3):67-67
Spectroscopic observations of comet Hale-Boppwere undertaken near perihelion at millimetre wavelengths with the Institut de Radioastronomie Millimétrique (IRAM) telescopes at Plateau de Bure (France)and Pico Veleta (Spain). They resulted in the first detections of HCOOH,SO2, NH2CHO and HCOOCH3 in a comet. HDO was detected through its312–221 line at 225.897 GHz,complementing the observation of the 101–000 line at 464.925 GHz at the James Clerk Maxwell Telescope (Meier et al., 1998,Science 279, 842).Several unidentified lines are present in the spectra. Observations of HC3N, HNCO, OCS, SO, CN, CO+, HCO+, in addition to more ‘classical’species CO, HCN, HNC, CH3CN, CH3OH, H2CO, CS and H2S (Biveret al., this issue) permit us to make out an extensive inventory of the composition of the coma of comet Hale-Bopp at its perihelion. It presents strong analogies with gas-phase abundances measured in interstellar hot cores and bipolar flows, which are believed to reflect the composition of interstellar grains. This revised version was published online in July 2006 with corrections to the Cover Date.  相似文献   

14.
An investigation of the capabilities and science goals of a submillimeter-wave heterodyne sounder onboard a Titan orbiter is presented. Based on a model of Titan’s submillimeter spectrum, and including realistic instrumental performances, we show that passive limb observations of Titan’s submillimeter radiation would bring novel and unique information on the dynamical and chemical state of Titan’s atmosphere, particularly in the so far poorly probed 500-900 km region. The 300-360, 540-660 and 1080-1280 GHz spectral ranges appear especially promising, and could be explored with an instrument equipped with a tunable local oscillator system. Vertical temperature profiles can be determined up to ∼1200 km using rotational lines of CH4, CO, and HCN. Winds can be measured over the 200-1200 km altitude range with an accuracy of 3-5 m/s from Doppler shift measurements of any strong optically thin line. Numerous molecular species are accessible, including H2O, NH3, CH3C2H, CH2NH, and several nitriles (HC3N, HC5N, CH3CN, and C2H3CN). Many of them are expected to be detectable in a large fraction of the atmosphere and in some cases at all levels, providing an observational link between stratospheric and thermospheric chemistry. Isotopic variants of some of these species can also be measured, providing new measurements of H, C, N, and O isotopic ratios. Mapping of the thermal, wind, and composition fields, best achieved from a polar orbit and with an articulated antenna, would provide a new view of the couplings between chemistry and dynamics over an extended altitude range of Titan’s atmosphere. Additional science goals at Saturn and Enceladus are briefly discussed.  相似文献   

15.
R.L. Hudson  M.H. Moore 《Icarus》2004,172(2):466-478
Motivated by detections of nitriles in Titan's atmosphere, cometary comae, and the interstellar medium, we report laboratory investigations of the low-temperature chemistry of acetonitrile, propionitrile, acrylonitrile, cyanoacetylene, and cyanogen (CH3CN, CH3CH2CN, CH2CHCN, HCCCN, and NCCN, respectively). A few experiments were also done on isobutyronitrile and trimethylacetonitrile ((CH3)2CHCN and (CH3)3CCN, respectively). Trends were sought, and found, in the photo- and radiation chemical products of these molecules at 12-25 K. In the absence of water, all of these molecules isomerized to isonitriles, and CH3CN, CH3CH2CN, and (CH3)2CHCN also formed ketenimines. In the presence of H2O, no isonitriles were detected but rather the cyanate ion (OCN−) was seen in all cases. Although isonitriles, ketenimines, and OCN− were the main focus of our work, we also describe cases of hydrogen loss, to make smaller nitriles, and hydrogen addition (reduction), to make larger nitriles. HCN formation also was seen in most experiments. The results are presented in terms of nitrile ice chemistry on Titan, in cometary ice, and in the interstellar medium. Possible connections to prebiotic chemistry are briefly discussed.  相似文献   

16.
A study has been made using a variable temperature flowing afterglow Langmuir probe technique (VT-FALP) to determine the equilibrium temperature dependencies of the dissociative electron-ion recombination of the protonated cyanide ions (RCNH+, where R=H, CH3 and C2H5) and their symmetrical proton-bound dimers (RCNH+NCR). The power law temperature dependencies of the recombination coefficients, αe, over the temperature range 180 to 600 K for the protonated ions are αe(T)(cm3 s−1)=3.5±0.5×10−7 (300/T)1.38 for HCNH+, αe(T)=3.4±0.5×10−7 (300/T)1.03 for CH3CNH+, and αe(T)=4.6±0.7×10−7 (300/T)0.81 for CH3CH2CNH+. The equivalent values for the proton-bound dimers are αe(T)(cm3 s−1)=2.4±0.4×10−6(300/T)0.5 for (HCN)2H+ to αe(T)=2.8±0.4×10−6(300/T)0.5 for (CH3CN)2H+, and αe(T)=2.3±0.3×10−6(300/T)0.5 for (CH3CH2CN)2H+. The relevance of these data to molecular synthesis in the interstellar medium and the Titan ionosphere are discussed.  相似文献   

17.
The origin of CN radicals in comets is not completely understood so far. We present a study of CN and HCN production rates and CN Haser scale lengths showing that: (1) at heliocentric distances larger than 3 AU, CN radicals could be entirely produced by HCN photolysis; (2) closer to the Sun, for a fraction of comets CN production rates are higher than HCN ones whereas (3) in the others, CN distribution cannot be explained by the HCN photolysis although CN and HCN production rates seem to be similar. Thus, when the comets are closer than 3 AU to the Sun, an additional process to the HCN photolysis seems to be required to explain the CN density in some comets.The photolysis of HC3N or C2N2 could explain the CN origin. But the HC3N production rate is probably too low to reproduce CN density profile, even if uncertainties on its photolysis leave the place for all possible conclusions. The presence of C2N2 in comets is a reliable hypothesis to explain the CN origin; thus, its detection is a challenging issue. Since C2N2 is very difficult to detect from ground-based observations, only in situ measurements or space observations could determine the contribution of this compound in the CN origin.Another hypothesis is a direct production of CN radicals by the photo- or thermal degradation of complex refractory organic compounds present on cometary grains. This process could explain the spatial profile of CN inside jets and the discrepancy noted in the isotopic ratio 14N/15N between CN and HCN. Laboratory studies of the thermal and UV-induced degradation of solid nitrogenated compounds are required to model and validate this hypothesis.  相似文献   

18.
Millimeter wavelength emission from the “parent” molecules HCN, CO, and CH3CN, the latter in both its ground and ν8 = 1 excited vibrational states, was sought from Comet Bradfield (1978c) during March 1978 after comet perihelion, when the heliocentric distance was between 0.45 and 0.55 AU. No lines were detected, and upper limits on the molecular column densities (averaged over the antenna beam) and production rates, Q are estimated. The upper limits on Q for HCN, CH3CN (ν8 = 0), and CH3CN (ν8 = 1) are less than the production rates inferred from the millimeter-wave detection of these species in Comet Kohoutek (1973f). The CO upper limit on Q is comparable to that inferred from a detection of Comet West (1975n) in the rocket uv. It seems likely that the total gas production rate of Comet Bradfield (1978c) was relatively low.  相似文献   

19.
The paper is concerned with the study of the star-forming regions S231–S235 in radio lines of molecules of the interstellar medium—carbon monoxide (CO), ammonia (NH3), cyanoacetylene (HC3N), in maser lines—methanol (CH3OH) and water vapor (H2O). The regions S231–S235 belong to the giant molecular cloudG174+2.5. The goal of this paper is to search for new sources of emission toward molecular clumps and to estimate their physical parameters from CO and NH3 molecular lines. We obtained new detections ofNH3 andHC3Nlines in the sources WB89673 and WB89 668 which indicates the presence of high-density gas. From the CO line, we derived sizes, column densities, and masses of molecular clumps. From the NH3 line, we derived gas kinetic temperatures and number densities in molecular clumps. We determined that kinetic temperatures and number densities of molecular gas are within the limits 16–30 K and 2.8–7.2 × 103 cm?3 respectively. The shock-tracing line of CH3OH molecule at a frequency of 36.2 GHz was detected in WB89 673 for the first time.  相似文献   

20.
Molecular line emission is a useful tool for probing the highly obscured inner kpc of starburst galaxies and buried AGNs. Molecular line ratios serve as diagnostic tools of the physical conditions of the gas—but also of its chemical properties. Both provide important clues to the type and evolutionary stage of the nuclear activity. While CO emission remains the main tracer for molecular distribution and dynamics, molecules such as HCN, HNC, HCO+, CN and HC3N are useful for probing the properties of the denser (n≳104 cm−3), star-forming gas. Here I discuss current views on how line emission from these species can be interpreted in luminous galaxies. HNC, HCO+ and CN are all species that can be associated both with photon dominated regions (PDRs) in starbursts—as well as X-ray dominated regions (XDRs) associated with AGN activity. HC3N line emission may identify galaxies where the starburst is in the early stage of its evolution.  相似文献   

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