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本文选取多个臭氧总量观测站点,采用"三重制约法"分别对下列3组仪器观测臭氧总量数据进行统计分析,解算出不同观测资料的误差标准差,进而对比研究各种仪器的精度特征:1)1996~2003年期间地基WOUDC(World Ozone and Ultraviolet Radiation Data Centre)观测网络仪器(包括Brewer、Dobson和Filter臭氧测量仪)与星载TOMS(Total Ozone Mapping Spectrometer)和GOME(The Global Ozone Monitoring Experiment)仪器;2)2004~2013年期间WOUDC与星载OMI(ozone monitoring instrument)和SCIAMACHY(scanning imaging absorption spectrometer for atmospheric chartography)仪器;3)2004~2013年期间地基SAOZ(Système D’Analyse par Observations Zénithales)与星载OMI和SCIAMACHY仪器。结果表明,1996~2003年期间TOMS V8和GOME观测精度相当,分别为7.6±2.8 DU/46(其中,7.6±2.8 DU为所分析站点观测资料的平均精度及其标准差,46为站点数目)和7.6±1.5 DU/46。TOMS V8观测精度优于TOMS V7(8.5±3.0 DU/46),验证了前者对后者有所改进。2004~2013年期间OMI和SCIAMACHY在WOUDC地基站点观测精度接近,分别为6.6±1.4 DU/21和6.0±1.6 DU/21。SAOZ地基仪器精度为8.4±3.6 DU/8。对于3类WOUDC地基仪器,Brewer站点观测资料的平均精度最优(7.9±3.3 DU/12),Dobson次之(8.7±2.3 DU/19),Filter最差(14.7±4.0 DU/15)。相比于卫星,3种地面仪器观测平均精度较差(10.5±4.3 DU/46),这主要是由于Filter精度较差引起。中国境内的瓦里关(Brewer)、香河(Dobson)和昆明(Dobson)3个地基站点仪器观测精度均较优,分别为7.8 DU、6.7 DU和6.6 DU。尽管不同站点之间存在一定差异,但整体来说,地基与卫星仪器在中国境内3个站点观测臭氧总量吻合较好。 相似文献
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北大西洋臭氧极小值和北太平洋极大值及其相互关系 总被引：2，自引：0，他引：2
利用1979～2002年TOMS卫星观测资料,采用臭氧总量纬向偏差和区域强迫的分析方法,研究北大西洋东北部大气臭氧低值与北太平洋西北部臭氧高值的季节变化过程和相互关系.研究表明,(1)北大西洋东北部存在一个大气臭氧极小值,年平均臭氧总量比纬向平均值低20 DU以上,冬季低50 DU以上; 北太平洋西北部存在一个大气臭氧极大值,年平均臭氧总量比纬向平均值高35 DU以上,冬季高70 DU以上.(2)上述两个地区大气臭氧的季节变化具有很强的区域特征,区域大气动力学输送和化学过程对上述两个地区大气臭氧季节变化的强迫分别为50.3%和42.6%.(3)上述两个地区大气臭氧纬向偏差的季节变化间存在很好的反相关,相关系数达到-0.98,说明其臭氧区域强迫之间存在良好的关系. 相似文献
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60～70oS臭氧总量的QBO和ENSO信号 总被引：2，自引：0，他引：2
本文利用Ｎｉｍｂｕｓ－７上搭载的臭氧总量观测光谱仪（ＴＯＭＳ）得到的６０～７０ｏＳ纬圈中臭氧总量资料,分析研究了该地区臭氧总量准两年振荡（ＱＢＯ）和ＥＮＳＯ信号的纬向分布,指出在该纬圈臭氧总量的长期变化中包含着的ＱＢＯ和ＥＮＳＯ信号。同时,本文还分析研究了沿纬圈分布的大气臭氧总量季节变化和长期变化趋势,指出在该纬圈各个季节中臭氧总量呈下降趋势,以６０～１００ｏＷ十月份的下降最大,达到－９．３ＤＵ／ａ。研究同时表明：臭氧总量季节变化、长期变化趋势、以及ＱＢＯ信号的纬向分布都在西南极上空出现异常。本文对此进行了讨论,认为这是西南极海陆分布调整大气环流及大气波动造成对臭氧总量分布和变化的影响 相似文献
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1990～2002年北京地区大气臭氧垂直分布Umkehr观测反演研究 总被引：4，自引：0，他引：4
基于标准Umkehr反演算法, 利用北京地区Dobson仪器逆转观测资料, 反演计算出臭氧垂直分布.在反演过程中加入气溶胶订正因子, 使反演结果更加合理.利用臭氧垂直分布反演结果, 研究1990～2002年北京地区臭氧垂直分布特征和变化情况.结果表明在1992年秋季和1993年春季期间, 在10.3～23.5 km范围内臭氧浓度有较大幅度降低, 造成了这个期间月平均臭氧总量的明显偏低; 1990年到2002年期间, 臭氧总量的变化呈现出缓慢下降趋势, 但不同高度臭氧含量的变化趋势有所不同. 相似文献
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火山气溶胶对北京地区臭氧总量变化趋势的影响 总被引：4，自引：3，他引：1
分析了1979～1995年北京地区臭氧总量的变化趋势、1980～1994年整层气溶胶光学厚度和1981～1985、1990～1994年平流层气溶胶光学厚度。分析依据的数据资料来自Dobson仪器所观测的臭氧总量资料和太阳辐射表提供的气溶胶光学厚度资料。结果表明,1979～1995年期间北京地区臭氧总量年变化率为-0.269%,1982～1985、1991～1994年间臭氧总量年变化率分别高达-0.954%和-1.439%。这说明厄尔奇琼火山和皮纳图博火山爆发对臭氧总量减少可能起到重要作用。 相似文献
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对我国河北香河、云南昆明、青海瓦里关及黑龙江龙凤山地基观测臭氧总量与不同时期、不同卫星反演的产品差别特点进行比较,评估地基和卫星观测臭氧总量数据的质量信息以及近30年来我国不同区域臭氧总量的变化趋势特征。结果表明:4个站点的地基与卫星观测臭氧总量的绝对和相对差别分别为-5~10 DU和-5%~4%;日平均相对差别基本上呈现随机分布特征。TOMS算法反演的卫星臭氧总量与地基差别总体上要优于与DOAS算法反演的同期产品。地基与卫星臭氧总量差别呈明显的区域特点,可能反映了卫星反演计算中所需的臭氧、温度垂直分布等初始条件的纬度分布差异对卫星产品精度的影响。在过去30年,4个站点的臭氧总量在经历1993年前的显著降低后于1995—1996年逐渐回升,而瓦里关站在2001年前后的回升更为明显。 相似文献
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利用1979—2018年太阳后向散射紫外辐射计SBUV(/2)星下点臭氧遥感资料,结合ERA-Interim和MERRA-2大气温度再分析资料,考察青藏高原区域内拉萨和共和两地春季臭氧和大气温度变化趋势的差异性。结果表明拉萨和共和两个地区的臭氧和大气温度逆转趋势均发生于1999年。对比2008年以来青藏高原整体臭氧总量变化速率（4.5 DU/(10 a)),拉萨臭氧总量变化更快,为5.9 DU/(10 a),共和相对较慢,仅为3.7 DU/(10 a);同时,1999年以来拉萨和共和春季下平流层（100~30 hPa）大气温度分别以0.5~1.4℃/(10 a)和0.01~0.9℃/(10 a)速率增加,上对流层(250~175 hPa)大气温度分别以0.2~1.5℃/(10 a)和0.2~1.2℃/(10 a)速率降低。与2008年以来高原整体大气温度变化相比较,均慢于高原下平流层（125~70 hPa) 1~2℃/(10 a)的增温速率,快于高原上对流层（225~175 hPa）0.4~1.1℃/(10 a)的降温速率。两地臭氧与大气温度的相关系数和回归系数计算结果表明,拉萨和共和两个地区1999年以来春季臭氧恢复速率的不同是导致两地同期下平流层-上对流层温度逆转速率差异的重要因子之一。 相似文献
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根据Dobson和TOMS资料分析北京和昆明大气臭氧总量变化特征 总被引：11，自引：0，他引：11
用约２０年 Ｄｏｂｓｏｎ和ＴＯＭＳ资料来分析北京（３９.９３°Ｎ，１１６.４０°Ｅ）和昆明 （２５.０２°Ｎ，１０２．６８°）两地大气臭氧总量的变化特征，结果表明：（１）在１９７９－２０００年间北京大气臭氧长期变化趋势是－０．６４２ ＤＵ／年，而昆明在１９８０－２０００年间的趋势是－０.００９ ＤＵ／年；（２）北京和昆明两地大气臭氧都有很强的季节内变化（尤其冬季更强），与季节性变化强度相当；（３）在北京和昆明，由记录较短的大气臭氧资料分析得到的长期变化趋势，与较长记录得到的结果有显著差异；（４）在北京（中纬度）和昆明（低纬度）大气臭氧都有显著的准两年振荡信号；（５）两个站点大气臭氧的年际变化主要由长期趋势项和准两年振荡信号组成；（６）Ｄｏｂｓｏｎ仪测量得到的臭氧总量与ＴＯＭＳ资料非常一致。 相似文献
11.
M. Van Roozendael P. Peeters H. K. Roscoe H. De Backer A. E. Jones L. Bartlett G. Vaughan F. Goutail J.-P. Pommereau E. Kyro C. Wahlstrom G. Braathen P. C. Simon 《Journal of Atmospheric Chemistry》1998,29(1):55-83
Comparisons of total column ozone measurements from Dobson, Brewer and SAOZ instruments are presented for the period 1990 to 1995 at seven stations covering the mid- and the high northern latitudes, as well as the Antarctic region. The main purpose of these comparisons is to assess, by reference to the well established Dobson network, the accuracy of the zenith-sky visible spectroscopy for the measurement of total ozone. The strengths and present limitations of this latter technique are investigated. As a general result, the different instruments are found to agree within a few percent at all stations, the best agreement being obtained at mid-latitudes. On average, for the mid-latitudes, SAOZ O3 measurements are approximately 2% higher than Dobson ones, with a scatter of about 5%. At higher latitudes, both scatter and systematic deviation tend to increase. In all cases, the relative differences between SAOZ and Dobson or Brewer column ozone are characterised by a significant seasonal signal, the amplitude of which increases from about 2.5% at mid-latitude to a maximum of 7.5% at Faraday, Antarctica. Although it introduces a significant contribution to the seasonality at high latitude, the temperature sensitivity of the O3 absorption coefficients of the Dobson and Brewer instruments is shown to be too small to account for the observed SAOZ/Dobson differences. Except for Faraday, these differences can however be largely reduced if SAOZ AMFs are calculated with realistic climatological profiles of ozone, pressure and temperature. Other sources of uncertainties that might affect the comparison are investigated. Evidence is found that the differences in the air masses sampled by the SAOZ and the other instruments contribute significantly to the scatter, and the impact of the tropospheric clouds on SAOZ measurements is displayed. 相似文献
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Tomi Karppinen Alberto Redondas Rosa D. García Kaisa Lakkala C. T. McElroy Esko Kyrö 《大气与海洋》2015,53(1):66-73
AbstractSpectrometers are designed to isolate particular wavebands and suppress light from wavelengths outside the band of interest. However, a small amount of undesired light will always enter the detector, not through the designed optical path, but through random scattering from the instrument optical components, housing, and dust particles. Every spectrophotometer has stray light coming from outside the nominal measurement waveband. For Dobson spectrophotometers and single monochromator Brewer spectrophotometers, which are basic instruments in the World Meteorological Organization (WMO) ozone and ultraviolet (UV) monitoring network, the error introduced by stray light is substantial when the ozone slant path becomes very large because of high solar zenith angles and a thick ozone layer. These are common conditions during Arctic spring. To study the issue, a long ozone slant path Intercomparison/Calibration campaign for Nordic Brewers and Dobsons was held at Sodankylä 8–24 March 2011 and a follow-up campaign to extend calibrations to shorter ozone slant paths took place at Izaña observatory, Tenerife, between 28 October and 18 November 2011. These campaigns were part of the Committee on Earth Observation Satellites (CEOS) Intercalibration of Ground-based Spectrometers and Lidars project funded by the European Space Agency (ESA), intended to permit the homogenization of ozone data from the European ozone ground-truthing network. During the active intercomparison periods, measurements were taken only when good conditions for sun or moon observations existed. Laboratory measurements using calibration lamps and helium-cadmium (HeCd) lasers were an essential part of both campaigns. The campaigns produced a high-quality database of total ozone and UV measurements and an accurate, up-to-date calibration and characterization of participating Brewers and Dobsons against the European standard instruments from the Regional Dobson Calibration Centre-Europe (RDCC-E) and the Regional Brewer Calibration Centre-Europe (RBCC-E). In the present work we focus on single monochromator Brewers and present a physics-based method to compensate for the stray-light effects in ozone retrieval using laboratory characterizations and radiative transfer modelling. The method was tested with independent data from the campaign. 相似文献
13.
Formation of the Summertime Ozone Valley over the Tibetan Plateau: The Asian Summer Monsoon and Air Column Variations 总被引：3，自引：0，他引：3
The summertime ozone valley over the Tibetan Plateau is formed by two influences,the Asian summer monsoon(ASM) and air column variations.Total ozone over the Tibetan Plateau in summer was ～33 Dobson units(DU) lower than zonal mean values over the ocean at the same latitudes during the study period 2005-2009.Satellite observations of ozone profiles show that ozone concentrations over the ASM region have lower values in the upper troposphere and lower stratosphere(UTLS) than over the non-ASM region.This is caused by frequent convective transport of low-ozone air from the lower troposphere to the UTLS region combined with trapping by the South Asian High.This offset contributes to a ～20-DU deficit in the ozone column over the ASM region.In addition,along the same latitude,total ozone changes identically with variations of the terrain height,showing a high correlation with terrain heights over the ASM region,which includes both the Tibetan and Iranian plateaus.This is confirmed by the fact that the Tibetan and Iranian plateaus have very similar vertical distributions of ozone in the UTLS,but they have different terrain heights and different total-column ozone levels.These two factors(lower UTLS ozone and higher terrain height) imply 40 DU in the lower-ozone column,but the Tibetan Plateau ozone column is only ～33 DU lower than that over the non-ASM region.This fact suggests that the lower troposphere has higher ozone concentrations over the ASM region than elsewhere at the same latitude,contributing ～7 DU of total ozone,which is consistent with ozonesonde and satellite observations. 相似文献
14.
《大气与海洋》2013,51(4):325-338
Abstract A portable ground‐based instrument has been constructed for the automated measurement of vertical column abundances of a number of gases pertinent to stratospheric ozone chemistry. The instrumentation is described in this paper and results are presented from the first set of field measurements, made during the Middle Atmosphere Nitrogen TRend Assessment (MANTRA) 1998 field campaign at Vanscoy, Saskatchewan, Canada. Zenith‐sky spectra in the near ultraviolet and visible wavelength regions were recorded for a period of seven days, prior to and following the launch of the MANTRA balloon on 24 August 1998. The spectra were then analysed using the differential optical absorption spectroscopy (DOAS) technique in conjunction with a radiative transfer model to determine vertical column amounts of ozone and NO2. Ozone measurements compared favourably with concurrent observations by ozonesondes, a Brewer spectrophotometer, and satellite instruments. Vertical NO2 columns were in broad agreement with those determined by the Global Ozone Monitoring Experiment (GOME) satellite instrument. 相似文献
15.
Abstract This work presents the climatology of the sulphur dioxide column over Thessaloniki derived from three years of observation with the Brewer spectrophotometer. The SO2 column averages 2.5 m atm‐cm and the shielding of UV‐B by SO2 is investigated and compared with the changes in shielding resulting from an anticipated ozone reduction. Columnar and surface SO2 concentrations over Thessaloniki appear to be typical of those in major industrial‐urban regions of the world. It is concluded that, for urban regions, predictions of changes in UV‐B as a result of man's activities must consider projections of changes in the SO2 column as well as ozone. 相似文献
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利用SAGE Ⅱ和HALOE臭氧垂直分布资料和TOMS臭氧总量资料, 研究我国北方(45°~55°N和35°~45°N范围), 东部(105°~135°E) 和西部(75°~105°E) 大气臭氧总量和垂直分布特征和差异。结果表明:我国北方东部冬季、春季和秋季臭氧总量明显大于西部, 主要表现在平流层臭氧极大值附近及其以下高度臭氧含量东部比西部明显偏大, 这种差异在冬、春季尤为明显; 随着纬度的降低, 冬季和秋季臭氧总量东、西部差异减小, 但春季臭氧总量东、西部差异没有明显改变; 夏季, 在45°~55°N范围, 东、西部臭氧分布没有明显差异, 但在35°~45°N范围, 臭氧分布东、西部差异较明显, 臭氧总量东、西部差异达到20.6 DU, 16 km以下臭氧柱总量东、西部差异达到12.8 DU。该文还对导致我国东、西部臭氧分布差异的原因进行了分析。 相似文献
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AbstractThe influence of variations in atmospheric temperature and ozone profiles on the total ozone column (TOC) derived from a Brewer MKII spectrophotometer operating in Thessaloniki, Greece, is investigated using three different sets of ozone absorption cross-sections. The standard Brewer total ozone retrieval algorithm uses the Bass and Paur (1985) cross-sections without accounting for the temperature dependence of the ozone cross-sections which produces a seasonally dependent bias in the measured TOC. The magnitude of this temperature effect depends on the altitude where the bulk of the ozone absorption occurs. Radiosonde measurements for the period 2000 to 2010 combined with climatological ozone profiles were used to calculate the effective temperature of ozone absorption and investigate its effect on the retrieved ozone column. Three different ozone absorption cross-section spectra convolved with the instrument's slit function were used: those of Bass and Paur (hereafter BP), currently used in the standard Brewer retrieval algorithm; those of Brion, Daumont, and Malicet (Malicet et al., 1985; hereafter BDM); and the recently published set by Serdyuchenko et al. (2013 hereafter S13). The temperature dependence of the differential ozone absorption coefficient ranges between 0.09 and 0.13% per degree Celsius for BP, between ?0.11 and ?0.06% per degree Celsius for BDM, and between 0.018 to 0.022% per degree Celsius for S13, resulting in a seasonal bias in the derived TOC of up to 2%, 1.8%, and 0.4%, respectively. The temperature sensitivity of the differential ozone absorption coefficient for the Brewer spectrophotometer at Thessaloniki for the BP and BDM cross-sections is found to be within the range reported for other Brewer instruments in earlier studies, whereas the seasonal bias in TOC is minimized when using the new S13 cross-sections because of their small temperature dependence. 相似文献