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1.
Stratigraphical investigations, geomorphological mapping, and diatom, plant macrofossil and pollen analyses were undertaken in and around two lakes in central Ireland to establish correlations between changes in lake conditions and catchment vegetation throughout the Holocene. Similar investigations of an adjacent mire reveal early Holocene changes in lake level and area. The palaeoecological data show high correlations related to variations in lake depth and area, catchment vegetation type, organic inputs and trophic status. Catchment‐scale deforestation is gradual and occurs through the Bronze and the Iron Ages, and the construction of a crannog in the early Medieval period (seventh century AD ) appears to be associated with a widespread increase in deforestation and mixed agriculture in the catchment. Both pollen and plant macrofossils suggest that one of the crannogs was used for crop storage in addition to domestic and any other activities. In the early to middle Holocene similarities in the proxy‐data appear to be climatically driven through changing lake levels and areal extent whereas the later Holocene record is clearly dominated by anthropogenic changes within the catchment and the construction of crannogs in the lakes. The advantages of combining multi‐proxy indicators of lake hydroecology with the vegetation record are illustrated. Copyright © 2005 John Wiley & Sons, Ltd.  相似文献   

2.

Equilibrium-kinetic modeling allows investigating metal behavior in the water–rock-organic matter system with time to evaluate anthropogenic effects on the environment. In the article, the interactions of stagnant mine drainage water of the flooded mine “Arsenic” with ore and gangue minerals were simulated using different organic matter incorporation approaches. If the model is closed to humic substances (no additional organic matter input), most fulvic acids are bound in the Fe fulvate complex. While under the removal of Fe fulvate from the model, the Cu fulvate becomes prevalent, the contribution of the fulvate complexes with Zn, Mg, and Ca also increases. This scenario simulates the organo-mineral complexes behavior well and allows identifying the sequence of metal binding to organic ligands as follows Fe?>?Cu?>?Zn?>?Mg?>?Ca. The second scenario imitates the constant input of organic matter to the model (open system regarding humic substances). The dissolved metal concentrations in the model solution are extremely high in comparison to the mine drainage water. This scenario demonstrates that excessive input of organic matter leads to the accumulation of the metals in a dissolved form and blocks the secondary mineral formation despite the faster dissolution of the primary minerals under a more acidic pH than in the first scenario. However, despite the differences between the model solution and the mine drainage water, this scenario is useful to address specific issues associated with changes in natural and anthropogenic conditions. Both scenarios show the importance of organic matter incorporation to the equilibrium-kinetic models.

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3.
Pollen‐ and related proxy‐based studies of human–environment interactions during the Norse and later periods within Greenland have primarily involved the investigation of peat, lake and soil deposits, all of which have taphonomic and sampling problems. Many small ponds exist, but they seem to have been relatively ignored in investigations of palaeoecologically based environmental history. To evaluate their usefulness for studies of ecologically related cultural history, especially where sites are in intimate association with the archaeology, a pond in the Norse Eastern Settlement has been examined to investigate three principal questions: (i) Does such a site contain a useful record of environmental history? (ii) Does it offer a record of sufficient resolution and sensitivity for the study of anthropogenic landscape impacts? (iii) Are there any apparent drawbacks to these sequences? Using data obtained from palynological, diatom, sedimentological and radiocarbon analyses, it is concluded that environmental data for each proxy – aside from 14C dating – are clearly capable of being explained in a reasonably straightforward and compatible manner and fulfil the hopes for the sampling medium. Copyright © 2011 John Wiley & Sons, Ltd.  相似文献   

4.
The organic fraction in soils has a significant influence on heavy metal transport. In this study, the organic carbon content was measured by dry oxidation procedure from 21 Xuzhou urban roadside soils to assess the relationships between the concentrations of heavy metals (Pb, Cu, Zn, and Cr) and the amount of organic carbon. The anthropogenic heavy metals (e.g. Pb, Cu, Zn) were strongly correlated with organic carbon (denoted by Corg−c) extracted by dry oxidation while natural heavy metal (e.g. Cr) showed no correlation to the Corg−c. The anthropogenic heavy metals were also strongly correlated with the amount of the total carbon. These results show that the anthropogenic heavy metals are mainly enriched in the organic matter in the Xuzhou urban roadside soils.  相似文献   

5.
Sea level fluctuation is common in the stratigraphical record and is partly explained by periodic polar glaciation. Such fluctuation in the absence of polar glaciation, during the warm periods of Earth's history, is poorly understood and currently under discussion. Here, I reconsider the palaeo-environmental information extracted from the variation in the carbon-isotope record and explain the phenomenon by coupling the levels of marine and fresh-water reservoirs through long-term wet and arid climate modes. The arido-eustasy model produces a standard anti-covariation pattern of marine organic and carbonate carbon-isotope records, which may appear throughout the geochemical record of the last 200 Myr. Under the model, orbitally forced periods of extremely wet climate result in environmental crisis, sea level falls, and carbon cycle perturbations, during which negative excursions in the marine organic carbon-isotope record of sediments containing matter from terrestrial vegetation should be understood as a proxy reporting periods of high precipitation rather than changes in the global carbon reservoir. I propose that the early Toarcian oceanic anoxic event is an example of arido-eustasy.  相似文献   

6.
Holocene temperature fluctuations in the northern Tibetan Plateau   总被引：4，自引：0，他引：4  
Arid Central Asia (ACA) lies on a major climatic boundary between the mid-latitude westerlies and the northwestern limit of the Asian summer monsoon, yet only a few high-quality reconstructions exist for its climate history. Here we calibrate a new organic geochemical proxy for lake temperature, and present a 45-yr-resolution temperature record from Hurleg Lake at the eastern margin of the ACA in the northern Tibetan Plateau. Combination with other proxy data from the same samples reveals a distinct warm–dry climate association throughout the record, which contrasts with the warm–wet association found in the Asian monsoon region. This indicates that the climatic boundary between the westerly and the monsoon regimes has remained roughly in the same place throughout the Holocene, at least near our study site. Six millennial-scale cold events are found within the past 9000 yr, which approximately coincide with previously documented events of northern high-latitude cooling and tropical drought. This suggests a connection between the North Atlantic and tropical monsoon climate systems, via the westerly circulation. Finally, we also observe an increase in regional climate variability after the mid-Holocene, which we relate to changes in vegetation (forest) cover in the monsoon region through a land-surface albedo feedback.  相似文献   

7.
Shelf sediments from near the mouth of the Mississippi River were collected and analyzed to examine whether records of the consequences of anthropogenic nutrient loading are preserved. Cores representing approximately 100 yr of accumulation have increasing concentrations of organic matter over this period, indicating increased accumulation of organic carbon, rapid early diagenesis, or a combination of these processes. Stable carbon isotopes and organic tracers show that virtually all of this increase is of marine origin. Evidence from two cores near the river mouth, one within the region of chronic seasonal hypoxia and one nearby but outside the hypoxic region, indicate that changes consistent with increased productivity began by approximately the mid-1950s when the inorganic carbon in benthic forams rapidly became isotopically lighter at both stations. Beginning in the mid-1960s, the accumulation of organic matter, organic δ13C, and δ15N all show large changes in a direction consistent with increased productivity. This last period coincides with a doubling of the load of nutrients from the Mississippi River, which levelled off in the mid-1980s. These data support the hypothesis that anthropogenic nutrient loading has had a significant impact on the Louisiana shelf.  相似文献   

8.
The impact of increasing urbanization on the quality of a river system has been investigated by examining the current concentration of trace metals in the Chattahoochee River south of Atlanta, GA, and comparing these to previously published historical sediment data from reservoirs along the river. The lack of historical data for dissolved metal concentrations prior to 1980 requires an approach using these historic metal data from sediment cores. Core data are combined with current suspended load and dissolved metal data to “backcast” dissolved metal concentrations in the metro-Atlanta portion of the Chattahoochee River. The data suggest that the per capita input of dissolved trace metals have actually decreased since the 1920s, but anthropogenic inputs of metal are still a substantial water quality issue.  相似文献   

9.
We tested the response of lacustrine testate amoebae (thecamoebians) to climate and environmental changes for the Lateglacial–Holocene transition. The palaeoenvironmental history of the study site (Lake Lautrey, Jura Mountains, eastern France) was previously established based on high‐resolution multi‐proxy studies of the same core. The present study is characterised by a high taxonomic resolution (54 taxa), inclusion of small species (down to 25 µm) and high total counts (>500 individuals per sample on average). Changes in the composition of testate amoeba assemblages (dominant species and assemblage structure), as well as in the accumulation rate (tests cm?2 a?1), corresponded to major climatic phases (i.e. Oldest Dryas, Bølling–Allerød Interstadial, Younger Dryas, Preboreal) as well as changes in organic matter inputs. Furthermore, decreases in the accumulation rate characterised minor short‐lived cooling events, such as Older Dryas event or Gerzensee oscillation. However, the Preboreal oscillation, which was well registered by other proxies at Lake Lautrey, could not be recognised in the testate amoeba record. This work demonstrates that lacustrine testate amoebae can be used for palaeoclimatic and palaeoecological reconstructions. Nevertheless, a better understanding of the relation between climate, organic matter and lacustrine testate amoebae requires further high‐resolution studies based on multi‐proxy approaches and the development of appropriate modern analogues. Copyright © 2010 John Wiley & Sons, Ltd.  相似文献   

10.
Many small estuaries are influenced by flow restrictions resulting from transportation rights-of-way and other causes. The biogeochemical functioning and history of such systems can be evaluated through study of their sediments. Ten long and six short cores were collected from the length of Jordan Cove, Connecticut, a Long Island Sound subestuary, and analyzed for stratigraphy, radionuclides (14C, 210Pb, 226Ra, 137Cs, and 60Co), and metals (Ag, Cd, Cu, Pb, Zn, Fe, and Al). For at least 3,800 yr, rising sea level has gradually inundated Jordan Cove, filling it with mud similar to that currently being deposited there. Long-term sediment accumulation in the cove averaged close to 0.1 cm yr−1 over the last three millennia. Recent sediment accumulation rates decrease inland from 0.84 cm yr−1 to 0.40 cm yr−1, and are slightly faster than relative sea-level rise at this site (0.3 cm yr−1). Similarity of depth distributions of trace metals was used to confirm relative sediment accumulation rates. 60Co and Ag are derived from sources outside the cove and its watershed, presumably the Millstone nuclear power plant and regional contaminated sediments, respectively. The combined data suggest that Long Island Sound is an important source of sediment to the cove; a minor part of total sediment is supplied from the local watershed. Trace metal levels are strongly correlated with Fe but not with either organic matter or Al. Sediment quality has declined in the cove over the past 60 yr, but only slightly. Cu, Pb, and Zn data correlate strongly with Fe but not with either organic matter or aluminum. Ratios of Ag to Fe and to trace metals suggest that Ag in the cove is derived almost entirely from Long Island Sound. This result supports the notion that Fenormalized Ag can serve as a better tracer of some kinds of contamination than more common and abundant metals, like Cu, Pb, and Zn. *** DIRECT SUPPORT *** A01BY085 00008  相似文献   

11.
Ma, L., Wu, J., Yu, H., Zeng, H. & Abuduwaili, J. 2011: The Medieval Warm Period and the Little Ice Age from a sediment record of Lake Ebinur, northwest China. Boreas, Vol. 40, pp. 518–524. 10.1111/j.1502‐3885.2010.00200.x. ISSN 0300‐9483. Lake Ebinur, Xinjiang, northwest China, is a closed‐basin, shallow lake that responds rapidly to changes in the ratio of precipitation to evaporation (P/E). A sediment record spanning the last 1500 years was obtained from the lake. We used δ18O and δ13C in bulk carbonate, and δ13C of organic matter in the lake sediments to infer environmental changes in the Ebinur region during the Medieval Warm Period (MWP) and the Little Ice Age (LIA). Decreased δ18O values of carbonate largely reflect an enhanced P/E ratio within the basin and a higher lake level. Bulk carbonates with higher δ13C values are deposited during periods when lake‐water pH is high, while lower δ13C values reflect a lower pH in the water column. δ13C in organic matter is associated with the amount of precipitation. The results indicate that the Ebinur region experienced a dry MWP and a wet LIA, although the MWP and LIA were warm and cold periods, respectively, as expected. Furthermore, the MWP and LIA were hydrologically complex and cannot be characterized as uniformly wet or dry. Peak wet periods are recorded in the sediment core around AD 1000, 1400 and 1700, and a dry event also occurred in the period of temperature change within the LIA (cold to warm around AD 1500). A comparison of the Lake Ebinur data with proxy records for the strength of the Siberian High and climate proxy indicators suggests that precipitation in the Ebinur region was a consequence, in part, of an enhanced Siberian High during the LIA.  相似文献   

12.
Sediment cores were collected from the Neuse and Pamlico River estuaries, North Carolina, at seven different sites, and the data show strong anthropogenic influence on water quality. The sediments from these cores were dated using210Pb,137Cs,14C, and pollen horizon techniques. Specific parameters investigated include bulk density, sedimentation rates, diatom assemblage changes, nutrient and trace metal flux, and vegetation changes as recorded in the pollen record. The greatest increases in sedimentation, nutrient and metal flux and changes in diatom assemblages have occurred in the past 50–60 yr in the Pamlico and Neuse. Diatom diversity has decreased and small planktonic forms have become dominant over time, most likely due to eutrophication and increased turbidity and sedimentation. Major changes occur before phytoplankton surveys and monitoring were initiated. Overall trends are similar to those found in Chesapeake Bay, although the time frame of major changes is more recent. Dominant small planktonic diatom species differ between Chesapeake Bay and the Neuse and Pamlico. Variance in paleoecological indicators between these mid-Atlantic estuaries may be due to geomorphology and land use history.  相似文献   

13.
Marine Isotope Stage 11 has been proposed as an analogue for the present interglacial interval; yet, terrestrial climate records from both this region and time interval are rare. The sediments deposited at Lake El'gygytgyn (67°30′N, 172°5′E) in Far East Russia contain a 3·56 Ma record of climate variability. This study presents a high‐resolution record of sediment colour change from Marine Isotope Stage 8 to 12 (ca 275 to 475 ka) and demonstrates the link between lake catchment processes and climate variability. The hue colour parameter, calculated from data collected via colour reflectance spectroscopy in the visible spectrum (380 to 720 nm), exhibits correspondence with global climate records. Determining the source of sediment colour changes was achieved through detailed mineralogical and sedimentological methods, and linked to colour changes through a series of colour sensitivity tests. Mineralogical data, measured by X‐ray diffraction, reveal fluctuations in concentrations of clay minerals corresponding to colour changes. Further analyses of the clay mineral assemblages show no change in relative clay mineral abundances, yet demonstrate a lake catchment dominated by physical weathering processes. Using measured mineral abundances, reconstructions of sediment colour based on colour reflectance mineral standards link mineral and clay mineral content to overall sediment colour. Colour sensitivity tests demonstrate the ability of iron oxide minerals to stain sediments red. Additionally, colour sensitivity to organic matter content was tested, suggesting that organic content drives variability in the red portion of the spectrum and darkens the overall colour signal. Sediment colour is then ultimately linked to physical weathering of bedrock minerals, with small amounts of chemical weathering producing iron oxides during wet intervals. Fluctuations in the sediment colour reveal a high‐resolution record of wet/dry cycles, and provide new information about wet periods for the Russian Arctic region not yet understood from other lake proxy records.  相似文献   

14.
Increased offshore development in the Alaskan Arctic has stimulated interest in assessing potential impacts to the environment before the onset of any adverse effects. Concentrations of trace metals in sediments are used in this paper to provide one sensitive indicator of anthropogenic inputs from offshore activity over the past several decades. Sediments in coastal waters of the western Beaufort Sea are patchy with respect to sediment granulometry, organic carbon content, and concentrations of trace metals. However, results for surface sediments and age-dated cores show that nearly all samples contain natural concentrations of Ag, Ba, Be, Co, Cr, Cu, Hg, Ni, Pb, Sb, Tl, V and Zn, with metal/Al ratios that have been constant for many decades. Metal concentrations for incoming river-suspended matter compare well with sediment metal values and, along with vertical distributions in sediments, show no discernible diagenetic impacts that distort the sedimentary record for metals, except for Mn, As and possibly Cd. Slightly elevated concentrations of Ba, Hg, Ag, Sb and Zn were observed in a total of eight instances or in only 0.7% of the 1,222 data points for metals in surface sediments.  相似文献   

15.
A sea ice record for Barrow Strait in the Canadian Arctic Archipelago (CAA) is presented for the interval 10.0–0.4 cal. kyr BP. This Holocene record is based primarily on the occurrence of a sea ice biomarker chemical, IP25, isolated from a marine sediment core obtained from Barrow Strait in 2005. A core chronology is based on 14C AMS dating of mollusc shells obtained from ten horizons within the core. The primary IP25 data are compared with complementary proxy data obtained from analysis of other organic biomarkers, stable isotope composition of bulk organic matter, benthic foraminifera, particle size distributions and ratios of inorganic elements. The combined proxy data show that the palaeo-sea ice record can be grouped according to four intervals, and these can be contextualised further with respect to the Holocene Thermal Maximum (HTM). Spring sea ice occurrence was lowest during the early–mid Holocene (10.0–6.0 cal. kyr BP) and this was followed by a second phase (6.0–4.0 cal. kyr BP) where spring sea ice occurrence showed a small increase. Between 4.0 and 3.0 cal. kyr BP, spring sea ice occurrence increased abruptly to above the median and we associate this interval with the termination of the HTM. Elevated spring sea ice occurrences continued from 3.0 to 0.4 cal. kyr BP, although they were more variable on shorter timescales. Within this fourth interval, we also provide evidence for slightly lower and subsequently higher spring sea ice occurrence during the Mediaeval Warm Period and the Little Ice Age respectively. Comparisons are made between our proxy data with those obtained from other palaeo-climate and sea ice studies for the CAA.  相似文献   

16.
《Quaternary Science Reviews》2004,23(3-4):261-281
The organic carbon content of marine sediments is commonly used as a proxy for export production. However, in continental margin sediments a large fraction of the organic matter may be of terrestrial origin, and it is necessary to correct the total organic carbon data accordingly. Radiocarbon dating of bulk organic carbon, organic geochemistry and isotope data (δ13C and δ15N) are used here to characterize the type of organic matter present in Core JT96-09 collected at a water depth of 920 m on the slope off Western Canada. The quantities of marine and terrestrial organic carbon are then estimated using the δ13C data. The 16 kyr record obtained from Core JT96-09 suggests that accumulation of total organic carbon was highest during the late glacial and deglacial, but geochemical data indicate that as much as 70% of this carbon is terrestrial in origin. When the palaeo-record is corrected for this terrigenous input it is observed that accumulation of marine organic matter, and presumably marine export production, increased at the end of the last glacial contemporaneous with the Bølling, and that it peaked during the Allerød. Data from other palaeoproductivity proxies (i.e., bio-barium, opal and alkenones) also indicate relatively high productivity during the deglacial. These results indicate a return to modern upwelling conditions and high marine export production at ∼14.3 calendar kyr BP and a period of enhanced upwelling, relative to the present, during the Allerød.  相似文献   

17.
Mineral soil horizons (Ae, Bhf1, Bhf2, Bf, BC and C) were carefully collected from two podzolic soil profiles in the Lake Clair watershed (Québec) in order to assess anthropogenic trace metal accumulation. Petrographic and selective analyses were performed to establish the soil mineralogy and properties. Furthermore, a complete sequential extraction procedure has been applied to help understanding the complex chemical speciation of Pb in forest soils. Chemical speciation of Pb showed a strong vertical gradient: 85% of this metal is mainly partitioned in refractory minerals in the C-horizon whereas in the upper Bhf1 and Ae-horizons, less than 50% of Pb is associated with this fraction. In the Ae-horizon, for example, 35%, 30% and 12% of total Pb, respectively, is associated with the exchangeable, labile organic matter and amorphous Fe-Mn oxides fractions. The distribution of Pb and Cr in the studied forest soils mainly reflects progressive contamination of the watershed by anthropogenic atmospheric sources. The anthropogenic source is indicated by elevated Cr and Pb concentrations in the topsoil (Bhf and Ae) horizons and by strong negative correlation between 206Pb/207Pb ratios and total Pb concentrations. According to these isotopic values, penetration of anthropogenic Pb does not exceed 10 cm in both soil profiles. Below this depth, both Pb concentrations and isotopic ratios remain nearly constant and similar to values observed in pre-anthropogenic sediments from Lake Clair. These values are interpreted as the natural geochemical backgrounds of the watershed. Based on that behaviour, calculated anthropogenic Pb net inputs amounted to between 1.24 and 1.8 g/m2.  相似文献   

18.
The temporal resolution of marine proxy data is limited by analytically required sample size. We present in-situ reflectance spectroscopy techniques (usually applied in remote sensing) to analyse the organic fraction of marine and terrestrial sediment. From absorption band depths, photosynthesis pigment variations are derived for sediments from the upwelling region off Peru, where productivity is related to the annual variability of El Niño strength. Quantitative estimations of diagenetic photosynthesis pigments derived from absorption band analysis in reflectance spectra are highly correlated to organic carbon content. The ratio of pigment fractions is related to chlorine concentration and reflects organic matter preservation and deep-water ventilation changes. The import of terrigenous mineroclastics (TM) by local rivers is semi-quantitatively documented in the spectrum continuum. TM is inversely varying with organic matter preservation and chlorine concentration.  相似文献   

19.
Geochemical, mineralogical and biological indicators preserved in sediments are widely used to reconstruct past climate change, but proxies differ in the degree to which their utility as climate indicators has been validated via laboratory experiments, modern spatial calibrations, or down‐core comparisons with instrumental climate data. Multi‐proxy studies provide another means of evaluating interpretations of proxies. This paper presents a multi‐proxy assessment comparing 19 sub‐centennially resolved late Holocene proxy records, covering the period 300–1900 AD, from seven Icelandic marine and lacustrine core sites. We employ simple statistical comparisons between proxy reconstructions to evaluate their correlations over time and, ultimately, their utility as proxies for regional climate. Proxies examined include oxygen isotopic composition of benthic and planktonic foraminifera, abundance of the sea‐ice biomarker IP25, allochthonous quartz in marine sediments (a proxy for drift ice around Iceland), marine carbonate abundance, total organic carbon concentration, chironomid assemblages, lacustrine biogenic silica and carbon/nitrogen ratios in lake sediments. Most of the examined proxy records, including temperature and sea‐ice proxies, correlate strongly with each other over multi‐centennial timescales, and thus do appear to record changes in regional climate. Copyright © 2011 John Wiley & Sons, Ltd.  相似文献   

20.
Mudflats and associated mangroves are most important ecosystems of tropical coastal regions. Mangroves play a very important role in maintaining the environmental balance; thus in addition to mangrove reforestation and restoration, afforestation has also been practiced. We studied distribution of sediment components (sand, silt, clay) organic carbon (OC), heavy metals (Fe, Mn, Cu, Zn, Cr and Co) and pH in six cores collected from one of the largest mudflats of Mandovi estuary, west coast of India. The temporal distribution patterns of these proxies suggested that past changes in tidal energy conditions, fresh water inflow and anthropogenic activities over the last few decades, together helped in development of a middle tidal flat in this estuary. In cores collected from the mangroves, trapping and deposition of finer particles and organic matter were enhanced by a complex aerial mangrove root system in recent years. Mangroves were, therefore, suggested to enhance the buildup of mudflats in Mandovi estuary. Cores collected from mudflats also exhibited higher deposition of finer particles and organic matter (except MF2) in recent years, suggesting maturity and greater stability of the entire mudflat in recent years. Middle tidal flats (mudflats) of Mandovi estuary may, therefore, prove to be suitable substrates for mangrove proliferation in the near future. Finer sediments deposited mainly from mining activities in recent years exhibited lower pH and higher metal content. Organisms dwelling in these recently deposited sediments are, therefore, at higher risk of bioaccumulation and metal toxicity.  相似文献   

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