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1.
The rates of production of21Ne and22Ne in spallation reactions, both due to solar as well as galactic cosmic rays, in some major meteoritic minerals, e.g. olivines, feldspars and pyroxenes, are calculated using their energy spectra and excitation functions. The production profiles of21Ne and22Ne due to galactic cosmic rays, and the22Ne/21Ne ratio depend upon the size of the meteoroid. The22Ne/21Ne ratio is very sensitive to the abundance of sodium and consequently its depth profile is distinctly different in feldspars, the ratio increasing with depth rather than decreasing as in pyroxenes and olivines. In the near-surface regions, up to a depth of 2cm, production due to solar flare protons dominates, giving rise to a steep gradient in isotopic production as well as in the22Ne/21Ne ratio. Composite production profiles are given and compared with measurements in some meteorites.  相似文献   

2.
Recent results on cosmic ray interactions in lunar samples and meteorites resulting in production of stable and radionuclides, particle tracks and thermoluminescence are reviewed. A critical examination of26A1 depth profiles in lunar rocks and soil cores, together with particle track data, enables us to determine the long term average fluxes of energetic solar protons (>10 MeV) which can be represented by (J s,R o)=(125, 125). The lunar rock data indicate that this flux has remained constant for 5×105 to 2×106 years. Production rates of stable and radionuclides produced by galactic cosmic rays is given as a function of size and depth of the meteoroid. Radionuclide (53Mn,28Al) depth profiles in meteorite cores, whose preatmospheric depths are deduced from track density profiles are used to develop a general procedure for calculating isotope production rates as a function of meteoroid size. Based on the track density and22Ne/21Ne production rates, a criterion is developed to identify meteorites with multiple exposure history.22Ne/21Ne ratio <1·06 is usually indicative of deep shielded exposure. An examination of the available data suggests that the frequency of meteorites with multiple exposure history is high, at least 15% for LL, 27% for L and 31% for H chondrites. The epi-thermal and the thermal neutron density profiles in different meteorites are deduced from60Co and track density data in Dhajala, Kirin and Allende chondrites. The data show that the production profile depends sensitively on the size and the chemical composition of the meteoroid. Cosmic ray-induced thermoluminescence in meteorites of known preatmospheric sizes has been measured which indicates that its production profile is nearly flat and insensitive to the size of the meteoroid. Some new possibilities in studying cosmic ray implanted radionuclides in meteorites and lunar samples using resonance ionisation spectroscopy are discussed.  相似文献   

3.
Galactic cosmic rays and solar protons ionize the present terrestrial atmosphere,and the air showers are simulated by well-tested Monte-Carlo simulations,such as PHITS code.We use the latest version of PHITS to evaluate the possible ionization of protoplanetary disks by galactic cosmic rays(GCRs),solar protons,and by supernova remnants.The attenuation length of GCR ionization is updated as 118 g cm~(-2),which is approximately 20% larger than the popular value.Hard and soft possible spectra of solar protons give comparable and 20% smaller attenuation lengths compared with those from standard GCR spectra,respectively,while the attenuation length is approximately 10% larger for supernova remnants.Further,all of the attenuation lengths become 10% larger in the compound gas of cosmic abundance,e.g.128 g cm~(-2) for GCRs,which can affect the minimum estimate of the size of dead zones in protoplanetary disks when the incident flux is unusually high.  相似文献   

4.
Study of several cosmic ray effects, such as VH track density, spallogenic26Al and53Mn activity,21Ne and22Ne/21Ne ratio, made in the same sample or in cores taken from different meteorites can identify parameters related to the exposure history of meteorites and cosmic ray flux variations. Meteorites with single or multiple exposure can be distinguished from a track production rate —22Ne/21Ne correlation diagram and cosmic ray flux variations over 106–107 years can be deduced from a three-isotope correlation diagram of26Al,53Mn and21Ne. Isotopic data based on chondrites with simple, one-stage exposure are consistent with the same average galactic cosmic ray intensity over the past 2 million years as that during the past 107 years.  相似文献   

5.
The radionuclide10Be (half-life = 1.5my), produced naturally in the Earth’s atmosphere by nuclear interactions of cosmic rays, was sought in ocean sediments in the late fifties, considering its potential usefulness as a radiotracer for dating sediments.10Be was discovered independently by two groups, one in India and the other in the USA, and used only for dating marine sediments and manganese nodules until the seventies. Subsequently, as a result of a technical advance resulting in the improvement in the sensitivity of measurement of10Be by about a factor of 106, there was a global rush to measure this nuclide in most materials participating in the physical, chemical and biological processes in the dynamic geosphere. This paper outlines the reasons for this “isotope rush”, and the lessons learned from these studies. I also present my personal views of the special attractive features of this nuclide on the one hand, and on the other, the pitfalls or the wrong message this nuclide could convey!  相似文献   

6.
Cosmogenic radionuclides with distinctive half-lives from chondritic falls were used as natural detectors of galactic cosmic rays (GCR). A unique series of uniform data was obtained for variations in the integral gradients of GCR with a rigidity of R > 0.5 GV in 1955–2000 on heliocentric distances of 1.5–3.3 AU and heliographic latitudes between 23° S and 16° N. Correlation analysis was performed for the variations in GCR gradients and variations in solar activity (number of sunspots, SS, and intensity of the green coronal line, GCL), the intensity of the interplanetary magnetic field (IMF), and the inclination of the heliospheric current sheet (HCS). Distribution and variations of GCR were analyzed in 11-year solar cycles and during a change in 22-year magnetic cycles. The detected dependencies of GCR gradients on the intensity of IMF and HCS inclination provided insight into the differences in the processes of structural transformation of IMF during changes between various phases of solar and magnetic cycles. The investigated relationships lead to the conclusion that a change of secular solar cycles occurred during solar cycle 20; moreover, there is probably still an increase in the 600-year solar cycle, which can be among the major reasons for the observed global warming.  相似文献   

7.
Measurements of15N/14N in dissolved molecular nitrogen (N2), nitrate (NO 3 ) and nitrous oxide (N2O) and18O/16O in N2O [expressed as δ15N and δ18O, relative to atmospheric N2 and oxygen (O2), respectively] have been made in water column at several locations in the Arabian Sea, a region with one of the thickest and most intense O2 minima observed in the open ocean. Microbially-mediated reduction of NO 3 to N2 (denitrification) in the oxygen minimum zone (OMZ) appears to greatly affect the natural isotopic abundances. The δ15N of NO 3 increases from 6‰ in deep waters (2500 m) to 15‰ within the core of the denitrifying layer (250–350 m); the δ15N of N2 concurrently decreases from 0.6‰ to 0.20‰ Values of the isotopic fractionation factor (ε) during denitrification estimated using simple advection-reaction and diffusion-reaction models are 22‰ and 25‰, respectively. A strong decrease in δ15N of NO 3 is observed from ∼ 200m (> 11‰) to 80m (∼ 6‰); this is attributed to the input of isotopically light nitrogen through nitrogen fixation. Isotopic analysis of N2O reveals extremely large enrichments of both15N and18O within the OMZ, presumably due to the preferential reduction of lighter N2O to N2. However, isotopically light N2O is observed to accumulate in high concentrations above the OMZ indicating that the N2O emitted to the atmosphere from this region cannot be very heavy. The isotope data from the intense upwelling zone off the southwest coast of India, where some of the highest concentrations of N2O ever found at the sea surface are observed, show moderate depletion of15N, but slight enrichment of18O relative to air. These results suggest that the ocean-atmosphere exchange cannot counter inputs of heavier isotopes (particularly18O) associated with the stratospheric back flux, as proposed by previous workers. This calls for additional sources and/or sinks of N2O in the atmosphere. Also, the N2O isotope data cannot be explained by production through either nitrification or denitrification, suggesting a possible coupling between the two processes as an important mechanism of N2O production.  相似文献   

8.
An increase in the cosmogenic beryllium-10 content of the Orca basin sediments due to the flooding of the Gulf of Mexico (GM) by meltwaters during the late Wisconsin interglacial is reported. A strong negative correlation (γ =-0.99) betweenδ 18 O (in the range o f-1.5‰ to +0.5‰) and10Be/Al ratio is seen. During intense flooding reflected by a decrease in δ18O by ∼ 2‰, this correlation may not hold as some of the sediments with low10Be/Al ratio and deposited on the shelf and slope regions of the GM during the earlier glacial period would also be washed into the basin. The deposited sediment would then be a mixture with a10Be/Al ratio lower than expected from the correlation  相似文献   

9.
Five chondrites with short cosmic ray exposure ages (< 3Myr) have been analyzed for 53Mn (t1.2 = 3.7Myr), 26Al(t1.2 = 0.72Myr) and the stable isotopes of He, Ar, and in particular, Ne. In addition, rare gases were determined for five other short-lived chondrites from the same aliquots which had previously been used for 26Al and 53Mn determinations by the Cologne Laboratory. Improved curves of growth were constructed for 26Al and 53Mn to deduce the respective saturation values 26Al0 and 53Mn0 and to obtain 21Ne production rates (21P).26Al and 53Mn saturation values deduced from short-lived chondrites alone agree within 20%, with those deduced from all chondrites. Values of 21p based on 53Mn and 26Al are 0.30 ± 0.03 and 0.46 ± 0.05, respectively, in H chondrites. Possible causes for the difference include half-life errors, data selection and a recent (?2.5Myr) increase in the cosmic ray intensity.  相似文献   

10.
The Sulagiri meteorite fell in India on 12 September 2008,LL6 chondrite class is the largest among all the Indian meteorites.Isotopic compositions of noble gases(He,Ne,Ar,Kr and Xe) and nitrogen in the Sulagiri meteorite and cosmic ray exposure history are discussed.Low cosmogenic(~(22)Ne/~(21)Ne)_c ratio is consistent with irradiation in a large body.Cosmogenic noble gases indicate that Sulagiri has a 4πcosmic-ray exposure(CRE) age of 27.9 ± 3.4 Ma and is a member of the peak of CRE age distribution of IX chondrites.Radiogenic ~4He and ~(40)Ar concentrations in Sulagiri yields the radiogenic ages as 2.29 and4.56 Ca,indicating the loss of He from the meteorite.Xenon and krypton are mixture of Q and spallogenic components.  相似文献   

11.
Cosmic ray exposure ages of Rumuruti chondrites from North Africa   总被引:1,自引:0,他引:1  
We analyzed noble gases and determined 3He, 21Ne, and 38Ar cosmic ray exposure ages (CREAs) of Rumuruti chondrites from North West Africa (NWA) to rule on potential pairings and/or source pairings of North Africa R chondrite samples. The 21Ne exposure ages range between 10 and 74 Ma, with NWA 2897 and 1668 having the highest known exposure ages among R chondrites. We also include other R chondrites from North Africa (Schultz et al., 2005) and, based on their noble gas characteristics and their 21Ne CREAs, propose pairings of the following samples: NWA 2198, 5069, 755, 4615, 845, 851, 978, 1471, and possibly DaG 013 belonging to one fall with a CREA of ∼10 Ma, and NWA 753, 4360, 4419, 5606, 1472, 1476, 1477, 1478, and 1566 representing one fall with a CREA of ∼14 Ma. NWA 2821, 2503, 2289, 3364, 3146, 4619, 4392, 3098, and 2446 seem to belong to one single fall with a CREA of ∼20 Ma, and NWA 2897 and 1668 seem to be paired and show a common CREA of ∼66 Ma. Overall, all R chondrite samples from North Africa analyzed for noble gases so far represent ∼16 individual falls. Comparing falls from North Africa to literature CREAs of R chondrites worldwide, it seems possible that a significant number of all R chondrite falls studied for noble gases were ejected from the R chondrite parent body during one large collisional event between 15 and 25 Ma ago. However, the database is still too small to draw definitive conclusions. The large portion of brecciated R chondrites in collections suggests severe impact brecciation of the R chondrite parent body.  相似文献   

12.
Abundances of cosmic ray-produced noble gases and 26Al, including some new measurements, have been compiled for some 23 stone meteorites with exposure ages of < 3 × 106 yr. Concentrations of cosmogenic He, Ne, and Ar in these meteorites have been corrected for differences in target element abundances by normalization to L-chondrite chemistry. Combined noble gas measurements in depth samples of the Keyes and St. Séverin chondrites are utilized to derive equations for normalizing the production rates of cosmogenic 3He, 21Ne, and 38Ar in chondrites to an adopted ‘average’ shielding: 22Ne21Ne = 1.114. The measured unsaturated 26Al concentrations and the calculated equilibrium 26Al for these meteorites are combined to estimate exposure ages. These exposure ages are statistically compared with chemistry- and shielding-corrected concentrations of cosmogenic He, Ne, and Ar to derive absolute production rates for these nuclides. For L-chondrites, at ‘average’ shielding, these production rates (in 10?8 cm3/g 106 yr) are: 3He = 2.45,21Ne = 0.47, and 38Ar = 0.069, which are ~ 25% higher than production rates used in the past. From these production rates and relative chemical correction factors, production rates for other classes of stone meteorites are derived.  相似文献   

13.
A series of yearly data on the concentration of radioactive carbon 14C in tree rings measured at the Tbilisi State University in 1983–1986 and covering the time interval 1600–1940 is statistically analyzed. We find evidence for a 22-year cyclicity in the intensity of Galactic cosmic rays (GCRs) during the Maunder minimum of the solar activity (1645–1715), testifying that the solar dynamo mechanism continued to operate during this epoch. Variations of Δ14C on timescales of tens and hundreds of years correlate well with the corresponding variations of the GCR intensity and solar activity, making radiocarbon a reliable source of information on long-timescale variations of solar activity in the past. Short-timescale (<30 years) fluctuations of Δ14C may be appreciably distorted by time variations not associated directly with solar activity; probable origins of this distortion are discussed.  相似文献   

14.
《Applied Geochemistry》1998,13(4):441-449
Noble gas elemental and isotopic compositions have been measured as well as the abundance of C and its isotopic ratios in 11 glasses from submarine pillow basalts collected from the Mariana Trough. The 3He/4He ratios of 8.22 and 8.51 Ratm of samples dredged from the central Mariana Trough (∼18°N) agree well with that of the Mid-Ocean Ridge Basalt (MORB) glasses (8.4±0.3 Ratm), whereas a mean ratio of 8.06±0.35 Ratm in samples from the northern Mariana Trough (∼20°N) is slightly lower than those of MORB. One sample shows apparent excess of 20Ne and 21Ne relative to atmospheric Ne, suggesting incorporation of solar-type Ne in the magma source. There is a positive correlation between 3He/4He and 40Ar/36Ar ratios, which may be explained by mixing between MORB-type and atmospheric noble gases. Excess 129Xe is observed in the sample which also shows 20Ne and 21Ne excesses. Observed δ13C values of ∼20°N samples vary from −3.76‰ to −2.80‰, and appear higher than those of MORB, and the corresponding CO2/3He ratios are higher than those of MARA samples at ∼18°N, suggesting C contribution from the subducted slab.  相似文献   

15.
Abundances and isotopic compositions of He, Ne, Ar, and Xe have been measured in eight recently fallen chondrites. Ratios of concentrations of cosmic ray-produced 3He, 21Ne, 22Ne and 38Ar indicate that all eight samples experienced less than average cosmic ray shielding. 3He and 21Ne exposure ages were calculated using shielding corrected chondritic production rates and the measured 22Ne21Ne. Exposure ages calculated from 22Na22Ne and 26Al21Ne ratios and constant relative production rates show a bias between the two ages due to variations in 22Na26Al. Arguments are presented that this bias is due to irradiation hardness differences, and therefore the use of constant values for both the 22Na22Ne and 26Al21Ne production ratios is not permitted. Dwaleni, Swaziland, was found to be an unusual gas-rich chondrite with high concentrations of solar-derived He and Ne and planetary-type Xe.  相似文献   

16.
Cosmic ray produced 10Be (half-life = 1.36 × 106 yr), 26Al (7.05 × 105 yr), and 36Cl (3.01 × 105 yr) were measured in a depth profile of 19 carefully-ground samples from the glass-coated lunar surface rock 64455. The solar cosmic ray (SCR) produced 26Al and 36Cl in this rock are present in high concentrations, which in combination with the low observed erosion rate, <0.5 mm/Myr, provide well defined depth profiles characterizing the SCR component of the cosmic rays. In conjunction with new experimentally determined excitation functions, the 36Cl concentrations suggest a softer solar-proton spectral shape than that derived from most previous measurements. The fact that no SCR-produced 10Be activity could be detected in 64455 is in good agreement with observations in 68815 and also indicates a softer SCR spectrum. Comparison of observed SCR profiles in 64455 with theoretical calculations indicates that the average solar-proton spectrum over the past 2 Myr (based on 26Al) has an exponential rigidity parameter (R0) of about 90 MV with a proton flux (J) of 73 protons/cm2/s·4π above 10 MeV. Over the last ∼0.5 Myr (based on 36Cl) R0 is about 70 MV with a flux of ∼196 protons/cm2/s·4π above 10 MeV. These SCR fluxes are consistent with most previous work.  相似文献   

17.
Noble gas analyses of the Ni-Fe of 9 L, 5 H and 2 LL chondrites quantitatively support previous suggestions of radiogenic 4He recoil and 3He deficits. Furthermore, noble gases in the Ni-Fe show evidence for in situ produced radiogenic 4He and in some cases for recoil loss of 38Ar and gain of 21Ne.The ratio of spallogenic 21Ne and 38Ar in the metal phase is found to correlate strongly with 3He/21Ne and 22Ne/21Ne in bulk samples of these chondrites. This is proof of the dependence of these ratios on the irradiation hardness experienced by the meteoroid in space. ‘Hardness indices’ n = 1.9–2.2 are found, indicating that on the average the stone meteoroids from which the samples came were smaller in mass than iron meteoroids. The spallogenic 21Ne/38Ar ratio in metallic Ni-Fe can be used with the semi-empirical production model deduced from the Grant iron meteorite to calibrate spallogenic 3He/21Ne and 4Ne/21Ne in bulk samples of L, LL and H chondrites for meteoroid size and sample location allowing the estimation of minimal meteoroid masses. 3He and 21Ne production rates calculated from previously determined 36Ar/38Ar exposure ages for four L chondrites indicate that they are probably not single-valued functions of the 3He/21Ne ratio. The ratio of 3He in bulk samples to 38Ar in metal samples of the same meteorite is constant (= 20 ± 3) whereas the ratio of 21Ne in the bulk to 38Ar in the metal varies by as much as a factor of two in correlation with 3He/21Ne.  相似文献   

18.
An integrated study of the cosmic ray exposure history of the San Juan Capistrano meteorite was carried out using measurements of rare gas isotopic abundances, particle track densities and radioisotope concentrations. Spallation systematics determined for Kr isotopes in lunar samples are shown to be valid also for the San Juan Capistrano and St. Severin meteorites, thus allowing us to determine a reliable 81Kr/83Kr production ratio as needed for applying the 81Kr-Kr dating method. The 81Kr-Kr age of SJC is 28.7 ± 2.0 Myr, about 35% longer than ages determined by spallation He or Ne. The minimum observed track production rate (2.6 × 105 tracks/cm2 · Myr) sets a minimum of 8 cm for the preatmospheric radius of an assumed spherical body. Track density gradients and the low 60Co activity (<2.9 dpm/g Co) both set an upper limit of 10 cm to the radius. Track results show that ablation losses have averaged 6cm. The relative spallation yields of 78Kr and 83Kr, and the ratios 3He/21Ne and 22Ne/21Ne are all compatible with a hard irradiation as would be experienced by a sample depth of about 6 cm in a body of 8–10 cm. The low activities of 54Mn, 22Na and 26Al are also consistent with these irradiation conditions.  相似文献   

19.
The cosmic ray exposure (CRE) ages of aubrites are among the longest of stone meteorites. New aubrites have been recovered in Antarctica, and these meteorites permit a substantial extension of the database on CRE ages, compositional characteristics, and regolith histories. We report He, Ne, and Ar isotopic abundances of nine aubrites and discuss the compositional data, the CRE ages, and regolith histories of this class of achondrites. A Ne three-isotope correlation reveals a solar-type ratio of 20Ne/22Ne = 12.1, which is distinct from the present solar wind composition and lower than most ratios observed on the lunar surface. For some aubrites, the cosmic ray-produced noble gas abundances include components produced on the surface of the parent object. The Kr isotopic systematics reveal significant neutron-capture-produced excesses in four aubrites, which is consistent with Sm and Gd isotopic anomalies previously documented in some aubrites. The nominal CRE ages confirm a non-uniform distribution of exposure times, but the evidence for a CRE age cluster appears doubtful. Six meteorites are regolith breccias with solar-type noble gases, and the observed neutron effects indicate a regolith history. ALH aubrites, which were recovered from the same location and are considered to represent a multiple fall, yield differing nominal CRE ages and, if paired, document distinct precompaction histories.  相似文献   

20.
Cosmic ray produced isotopes in terrestrial systems   总被引:2,自引:0,他引:2  
Continuing improvements in the sensitivity of measurement of cosmic ray produced isotopes in environmental samples have progressively broadened the scope of their applications to characterise and quantify a wide variety of processes in earth and planetary sciences. In this article, I will concentrate on the new developments in the field of nuclear geophysics, based on isotopic changes produced by cosmic rays in the terrestrial systems. This field, which is best described as cosmic ray geophysics, caught roots with the discovery of cosmogenic14C on the Earth by Willard Libby in 1948, and grew rapidly at first, but slowed down during the ’60s and ’70s. In the ’80s, there was arenaissance in cosmic ray produced isotope studies, thanks mainly to the developments of the accelerator mass spectrometry technique capable of measuring minute amounts of radioactivity in terrestrial samples. This technological advance has considerably enhanced the applications of cosmic ray produced isotopes and today we find them being used to address diverse problems in earth and planetary sciences I discuss the present scope of the field of cosmic ray geophysics with an emphasis ongeomorphology. I must stress here that this is the decade in which this field, which has been studied passionately by geographers, geomorphologists and geochemists for more than five decades, has at its service nuclear methods to introduce numeric time controls in the range of centuries to millions of years.  相似文献   

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