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1.
Extensive research on the sources and sinks of greenhouse gases, carbon cycle modeling, and the characterization of atmospheric aerosols has been carried out in China during the last 10 years or so. This paper presents the major achievements in the fields of emissions of greenhouse gases from agricultural lands,carbon cycle modeling, the characterization of Asian mineral dust, source identification of the precursors of the tropospheric ozone, and observations of the concentrations of atmospheric organic compounds.Special, more detailed information on the emissions of methane from rice fields and the physical and chemical characteristics of mineral aerosols are Dresented.  相似文献   

2.
Extensive research on the sources and sinks of greenhouse gases, carbon cycle modeling, and the characterization of atmospheric aerosols has been carried out in China during the last 10 years or so. This paper presents the major achievements in the fields of emissions of greenhouse gases from agricultural lands, carbon cycle modeling, the characterization of Asian mineral dust, source identification of the precursors of the tropospheric ozone, and observations of the concentrations of atmospheric organic compounds. Special, more detailed Information on the emissions of methane from rice fields and the physical and chemical characteristics of mineral aerosols are presented.  相似文献   

3.
This study estimates direct radiative forcing by tropospheric ozone and all aerosols between the years 1850 and 2000, using the new IPCC AR5 （the Intergovernmental Panel on Climate Change Fifth Assessment Report） emissions inventories and a fully coupled chemistry-aerosol general circulation model. As compared to the previous Global Emissions Inventory Activity （GEIA） data, that have been commonly used for forcing estimates since 1990, the IPCC AR5 emissions inventories report lower anthropogenic emissions of organic carbon and black carbon aerosols and higher sulfur and NOx emissions. The simulated global and annual mean burdens of sulfate, nitrate, black carbon （BC）, primary organic aerosol （POA）, secondary organic aerosol （SOA）, and ozone were 0.79, 0.35, 0.05, 0.49, 0.34, and 269 Tg, respectively, in the year 1850, and 1.90, 0.90, 0.11, 0.71, 0.32, and 377 Tg, respectively, in the year 2000. The estimated annual mean top of the atmosphere （TOA） direct radiative forcing of all anthropogenic aerosols based on the AR5 emissions inventories is -0.60 W m^-2 on a global mean basis from 1850 to 2000. However, this is -2.40 W m-2 when forcing values are averaged over eastern China （18-45°N and 95-125°E）. The value for tropospheric ozone is 0.17 W m^-1 on a global mean basis and 0.24 W m^-2 over eastern China. Forcing values indicate that the climatic effect of aerosols over eastern China is much more significant than the globally averaged effect.  相似文献   

4.
The authors present spatial and temporal characteristics of anthropogenic sulfate and carbonaceous aerosols over East Asia using a 3-D coupled regional climate-chemistry-aerosol model, and compare the simulation with the limited aerosol observations over the region. The aerosol module consists of SO2, SO4^2-, hydrophobic and hydrophilic black carbon （BC） and organic carbon compounds （OC）, including emission, advections, dry and wet deposition, and chemical production and conversion. The simulated patterns of SO2 are closely tied to its emission rate, with sharp gradients between the highly polluted regions and more rural areas. Chemical conversion （especially in the aqueous phase） and dry deposition remove 60% and 30% of the total SO2 emission, respectively. The SO4^2- shows less horizontal gradient and seasonality than SO2, with wet deposition （60%） and export （27%） being two major sinks. Carbonaceous aerosols are spatially smoother than sulfur species. The aging process transforms more than 80% of hydrophobic BC and OC to hydrophilic components, which are removed by wet deposition （60%） and export （30%）. The simulated spatial and seasonal SO4^2-, BC and OC aerosol concentrations and total aerosol optical depth are generally consistent with the observations in rural areas over East Asia, with lower bias in simulated OC aerosols, likely due to the underestimation of anthropogenic OC emissions and missing treatment of secondary organic carbon. The results suggest that our model is a useful tool for characterizing the anthropogenic aerosol cycle and for assessing its potential climatic and environmental effects in future studies.  相似文献   

5.
Using the global chemistry and transport model MOZART,the simulated distributions of tropospheric hydroxyl free radicals(OH) over China and its sensitivities to global emissions of carbon monoxide(CO),nitrogen oxide(NO x),and methane(CH 4) were investigated in this study.Due to various distributions of OH sources and sinks,the concentrations of tropospheric OH in east China are much greater than in west China.The contribution of NO + perhydroxyl radical(HO 2) reaction to OH production in east China is more pronounced than that in west China,and because of the higher reaction activity of non-methane volatile organic compounds(NMVOCs),the contributions to OH loss by NMVOCs exceed those of CO and take the dominant position in summer.The results of the sensitivity runs show a significant increase of tropospheric OH in east China from 1990 to 2000,and the trend continues.The positive effect of double emissions of NO x on OH is partly offset by the contrary effect of increased CO and CH 4 emissions:the double emissions of NO x will cause an increase of OH of 18.1%-30.1%,while the increases of CO and CH 4 will cause a decrease of OH of 12.2%-20.8% and 0.3%-3.0%,respectively.In turn,the lifetimes of CH 4,CO,and NO x will increase by 0.3%-3.1% with regard to double emissions of CH 4,13.9%-26.3% to double emissions of CO and decrease by 15.3%-23.2% to double emissions of NO x.  相似文献   

6.
In this paper, the RIEMS 2.0 model is used to simulate the distribution of sulfate, black carbon, and organic carbon aerosols over China (16.2°-44.1°N, 93.4°-132.4°E) in 1998. The climate effects of these three anthropogenic aerosols are also simulated. The results are summarized as follows: (1) The regional average column burdens of sulfate, BC, OC, and SOC were 5.9, 0.24, 2.4, and 0.49 mg m-2, with maxima of 33.9, 1.48, 7.3, and 1.1 mg m-2, respectively. The column burden and surface concentration of seco...  相似文献   

7.
The International Centre for Theoretical Physics(ICTP,Italy) Regional Climate Model version 3.0(RegCM3) is used to simulate spatio-temporal distribution characteristics and radiative forcing(RF) of organic carbon(OC) aerosols in and around China.The preliminary simulation results show that OC aerosols are mostly concentrated in the area to the south of Yellow River and east of Tibetan Plateau.There is a decreasing trend of column burden of OC aerosols from south to north in China.The maximum value of column burden of OC aerosols is above 3 mg/m2 and located in the central and southern China,southeastern Tibet,and southwestern China’s Yunnan,Guizhou,Sichuan provinces.The simulation on the seasonal variation shows that the maximum value of column burden of OC aerosols appears in winter and the secondary value is in spring and the minimum in summer.The RF of OC aerosols which varies seasonally is negative at the top of the atmosphere(TOA) and surface.The spatio-temporal characteristics of the RF of OC aerosols are basically consistent with that of IPCC,implying the high accuracy of the parameterization scheme for OC aerosols in RegCM3.  相似文献   

8.
The direct climatic effect of aerosols for the 1980-2000 period over East Asia was numerically investigated by a regional scale coupled climate-chemistry/aerosol model,which includes major anthropogenic aerosols(sulfate,black carbon,and organic carbon) and natural aerosols(soil dust and sea salt) .Anthropogenic emissions used in model simulation are from a global emission inventory prepared for the Intergovernmental Panel on Climate Change Fifth Assessment Report(IPCC AR5) ,whereas natural aerosols are calculated online in the model.The simulated 20-year average direct solar radiative effect due to aerosols at the surface was estimated to be in a range of-9--33 W m-2 over most areas of China,with maxima over the Gobi desert of West China,and-12 W m-2 to-24 W m-2 over the Sichuan Basin,the middle and lower reaches of the Yellow River and the Yangtze River.Aerosols caused surface cooling in most areas of East Asia,with maxima of-0.8-C to-1.6-C over the deserts of West China,the Sichuan Basin,portions of central China,and the middle reaches of the Yangtze River. Aerosols induced a precipitation decrease over almost the entire East China,with maxima of-90 mm/year to-150 mm/year over the Sichuan Basin,the middle reaches of the Yangtze River and the lower reaches of the Yellow River.Interdecadal variation of the climate response to the aerosol direct radiative effect is evident,indicating larger decrease in surface air temperature and stronger perturbation to precipitation in the 1990s than that in the 1980s,which could be due to the interdecadal variation of anthropogenic emissions.  相似文献   

9.
A numerical study of tropospheric ozone in the springtime in East Asia   总被引：11，自引：0，他引：11  
The Models-3 Community Multi-scale Air Quality modeling system (CMAQ)coupled with the Regional Atmospheric Modeling System (RAMS)is applied to East Asia to study the transport and photochemical transformation of tropospheric ozone in March 1998．The calculated mixing ratios of ozone and carbon monoxide are compared with ground 1evel observations at three remote sites in Japan and it is found that the model reproduces the observed features very well．Examination of several high episodes of ozone and carbon monoxide indicates that these elevated levels are found in association with continental outflow,demonstrating the critical role of the rapid transport of carbon monoxide and other ozone precursors from the continental boundary layer．In comparison with available ozonesonde data,it is found that the model-calculated ozone concentrations are generally in good agreement with the measurements,and the stratospheric contribution to surface ozone mixing ratios is quite limited．  相似文献   

10.
RegCM4.3, a high-resolution regional climate model, which includes five kinds of aerosols(dust, sea salt,sulfate, black carbon and organic carbon), is employed to simulate the East Asian summer monsoon(EASM) from 1995 to 2010 and the simulation data are used to study the possible impact of natural and anthropogenic aerosols on EASM.The results show that the regional climate model can well simulate the EASM and the spatial and temporal distribution of aerosols. The EASM index is reduced by about 5% by the natural and anthropogenic aerosols and the monsoon onset time is also delayed by about a pentad except for Southeast China. The aerosols heat the middle atmosphere through absorbing solar radiation and the air column expands in Southeast China and its offshore areas. As a result, the geopotential height decreases and a cyclonic circulation anomaly is generated in the lower atmosphere. Northerly wind located in the west of cyclonic circulation weakens the low-level southerly wind in the EASM region. Negative surface radiative forcing due to aerosols causes downward motion and an indirect meridional circulation is formed with the low-level northerly wind and high-level southerly wind anomaly in the north of 25° N in the monsoon area, which weakens the vertical circulation of EASM. The summer precipitation of the monsoon region is significantly reduced,especially in North and Southwest China where the value of moisture flux divergence increases.  相似文献   

11.
The authors used a high-resolution regional climate model(RegCM3) coupled with a chemistry/aerosol module to simulate East Asian climate in 2006 and to test the climatic impacts of aerosols on regionalscale climate.The direct radiative forcing and climatic effects of aerosols(dust,sulfate,black carbon,and organic carbon) were discussed.The results indicated that aerosols generally produced negative radiative forcing at the top-of-the-atmosphere(TOA) over most areas of East Asia.The radiative forcing induced by aerosols exhibited significant seasonal and regional variations,with the strongest forcing occurring in summer.The aerosol feedbacks on surface air temperature and precipitation were clear.Surface cooling dominated features over the East Asian continental areas,which varied in the approximate range of-0.5 to-2°C with the maximum up to-3-C in summer over the deserts of West China.The aerosols induced complicated variations of precipitation.Except in summer,the rainfall generally varied in the range of-1 to 1 mm d-1 over most areas of China.  相似文献   

12.
Ozone is well documented as the air pollutant most damaging to agricultural crops and other plants. It is reported that tropospheric O3 concentration increases rapidly in recent 20 years. Evaluating and predicting impacts of ozone concentration changes on crops are drawing great attention in the scientific community. In China, main study method about this filed is controlled experiments, for example, Open Top Chambers. But numerical simulation study about impacts of ozone on crops with crop model was developed slowly, what is more, the study about combined impacts of ozone and carbon dioxide has not been reported. The improved agroecosystem model is presented to evaluate simultaneously impacts of tropospheric O3 and CO2 concentration changes on crops in the paper by integrating algorithms about impacts of ozone on photosynthesis with an existing agroecosystem biogeochemical model (named as DNDC). The main physiological processes of crop growth (phenology, leaf area index, photosynthesis, respiration, assimilated allocation and so on) in the former DNDC are kept. The algorithms about impacts of ozone on photosynthesis and winter wheat leaf are added in the modified DNDC model in order to reveal impacts of ozone and carbon dioxide on growth, development, and yield formation of winter wheat by coupling the simulation about impacts of carbon dioxide on photosynthesis of winter wheat which exists in the former DNDC. In the paper, firstly assimilate allocation algorithms and some genetic parameters (such as daily thermal time of every development stage) were modified in order that DNDC can be applicable in North China. Secondly impacts of ozone on crops were simulated with two different methods- one was impacts of ozone on light use efficiency, and the other was direct effects of ozone on leaves photosynthesis. The latter simulated results are closer to experiment measurements through comparing their simulating results. At last the method of direct impacts of ozone on leaf growth is adopted and the coefficients about impacts of ozone on leaf growth and death are ascertained. Effects of climate changes, increasing ozone, and carbon dioxide concentration on agroecosystem are tried to be simulated numerically in the study which is considered to be advanced and credible.  相似文献   

13.
In this study, a regional air quality model system (RAQMS) was applied to investigate the spatial distributions and seasonal variations of atmospheric aerosols in 2006 over East Asia. Model validations demonstrated that RAQMS was able to reproduce the evolution processes of aerosol components reasonably well. Ground-level PM10 (particles with aerodynamic diameter ≤10 μm) concentrations were highest in spring and lowest in summer and were characterized by three maximum centers: the Taklimakan Desert (～1000 μg m-3), the Gobi Desert (～400 μg m-3), and the Huabei Plain (～300 μm-3) of China. Vertically, high PM10 concentrations ranging from 100 μg m-3 to 250 μg m-3 occurred from the surface to an altitude of 6000 m at 30o--45oN in spring. In winter, the vertical gradient was so large that most aerosols were restricted in the boundary layer. Both sulfate and ammonium reached their highest concentrations in autumn, while nitrate reached its maximum level in winter. Black carbon and organic carbon aerosol concentrations reached maximums in winter. Soil dust were strongest in spring, whereas sea salt exerted the strongest influence on the coastal regions of eastern China in summer. The estimated burden of anthropogenic aerosols was largest in winter (1621 Gg) and smallest in summer (1040 Gg). The sulfate burden accounted for ～42% of the total anthropogenic aerosol burden. The dust burden was about twice the anthropogenic aerosol burden, implying the potentially important impacts of the natural aerosols on air quality and climate over East Asia.  相似文献   

14.
The physical and chemical characteristics of the aerosol samples were studied.The samples were collected on the 3 platforms (at levels 8 m,100 m and 320 m respectively) of IAP (Institute of Atmospheric Physics,Chinese Academy of Sciences) observation tower during the periods from January 1 to 16 and from February 20 to March 2,2001.The concentrations of TSP (total suspended particles),chemical components and size distribution for aerosols were calculated.The effects of the meteorological conditions on the aerosol concentrations and its distributions werestudied.The main aerosol sources from which the aerosols in the samples collected came were investigated.The conclusion was drawn preliminarily as follows.The TSP concentrations decreased with height.Over 70% of the aerosol mass were distributed in the fine particle group (d<2.1μm).The top 20 aerosol elements with high concentration are listed from high to low according to their concentrations,and they are S,Fe,Ca,K,A1,Na,Mg,Zn,Cl,Ba,P,Ti,Pb,Mn,As,Cu,V,Br,Cr,and Sb.The aerosol element concentrations decreased with height,too.The mass of volatile elements was mainly distributed in the fine particle group.The ion mass was distributed in the same way as the element mass.From the point of view of contribution to the air aerosols,both anthropogenic and natural sources are important for Beijing.  相似文献   

15.
A regional climate model is employed to simulate the aerosols(dust,sulfate,black carbon,and organic carbon) and their direct effect on the climate over China.The emphasis is on the direct radiative forcing due to the change in mixing state of aerosols.The results show that direct radiative forcing is significantly different between externally and internally mixed aerosols.At the top of the atmosphere(TOA),the radiative forcing of externally mixed aerosols is larger than that of internally mixed ones,especially in the Tarim desert region where the difference is about 0.7 W m 2.At the surface,however,the situation becomes opposite,especially in the Sichuan basin where the difference is about-1.4 W m 2.Nonetheless,either externally or internally mixed aerosols in China can result in a significant cooling effect,except for the warming in South China in winter and the slight warming in North China in February.The cooling effect induced by externally mixed aerosols is weaker than that induced by internally mixed aerosols,and this is more obvious in spring and winter than in summer and autumn.In spring and summer,the inhibiting effect of externally mixed aerosols on precipitation is less than that of internally mixed aerosols,whereas in autumn and winter the difference is not obvious.  相似文献   

16.
Temporal-spatial variations in tropospheric ozone concentrations over East Asia in the period from 1 January 2000 to 31 December 2004 were simulated by using the Models-3 Community Multi-scale Air Quality (CMAQ) modeling system with meteorological fields calculated by the Regional Atmospheric Modeling System (RAMS). The simulated concentrations of ozone and carbon monoxide were compared with ground level observations at two remote sites, Ryori (39.03°N, 141.82°E) and Yonagunijima (24.47°N, 123.02°E). The co...  相似文献   

17.
Urban air pollution in Pakistan is a serious challenge and it causes significant damage to human health and ecosystems. This paper presents a modelling study using the Weather Research and Forecasting Model coupled with Chemistry(WRF-Chem) to simulate the spatial distributions and temporal variations of aerosol concentrations over Pakistan, focusing on contributions of domestic emission sectors(transport, industry, residential, and energy) to mass concentrations of sulfate(SO2–4), nitrate(NO–3), ammonium(NH+4), black carbon(BC), and organic carbon(OC) during the months of January, April, July, and October in 2010. Sensitivity studies indicate that, averaged over January, April, July, and October of 2010, energy and industry sectors have the largest contributions to SO2–4 concentrations, each of which contributes about 10%?20% to SO2– 4over the polluted eastern Pakistan. The contributions from residential and transport sectors to NO–3 concentrations reach 40%?50% in central Pakistan. The residential sector has the highest contribution of 50%–80% to BC and OC loading in northeastern and southern Pakistan. Examination of sector contributions to aerosol levels in Lahore, the most polluted city in Pakistan, suggests that reductions in emissions in the residential sector should be an efficient measure for improving particulate matter air quality in this region.  相似文献   

18.
Min WEI 《大气科学进展》2005,22(6):798-806
The Asian summer monsoon is an important part of the climate system. Investigating the response of the Asian summer monsoon to changing concentrations of greenhouse gases and aerosols will be meaningful to understand and predict climate variability and climate change not only in Asia but also globally. In order to diagnose the impacts of future anthropogenic emissions on monsoon climates, a coupled general circulation model of the atmosphere and the ocean has been used at the Max-Planck-Institute for Meteorology. In addition to carbon dioxide, the major well mixed greenhouse gases such as methane, nitrous oxide, several chlorofluorocarbons, and CFC substitute gases are prescribed as a function of time. The sulfur cycle is simulated interactively, and both the direct aerosol effect and the indirect cloud albedo effect are considered. Furthermore, changes in tropospheric ozone have been pre-calculated with a chemical transport model and prescribed as a function of time and space in the climate simulations. Concentrations of greenhouse gases and anthropogenic emissions of sulfur dioxide are prescribed according to observations （1860-1990） and projected into the future （1990-2100） according to the Scenarios A2 and B2 in Special Report on Emissions Scenarios （SRES, Nakcenovic et al., 2000） developed by the Intergovernmental Panel on Climate Change （IPCC）. It is found that the Indian summer monsoon is enhanced in the scenarios in terms of both mean precipitation and interannual variability. An increase in precipitation is simulated for northern China but a decrease for the southern part. Furthermore, the simulated future increase in monsoon variability seems to be linked to enhanced ENSO variability towards the end of the scenario integrations.  相似文献   

19.
Understanding the responses of mean and extreme precipitation to climate change is of great importance.Previous studies have mainly focused on the responses to prescribed sea surface warming or warming due to increases of CO2.This study uses a cloud-resolving model under the idealization of radiative-convective equilibrium to examine the responses of mean and extreme precipitation to a variety of climate forcings,including changes in prescribed sea surface temperature,CO2,solar insolation,surface albedo,stratospheric volcanic aerosols,and several tropospheric aerosols.The different responses of mean precipitation are understood by examining the changes in the surface energy budget.It is found that the cancellation between shortwave scattering and longwave radiation leads to a small dependence of the mean precipitation response on forcings.The responses of extreme precipitation are decomposed into three components(thermodynamic,dynamic,and precipitation efficiency).The thermodynamic components for all climate forcings are similar.The dynamic components and the precipitation-efficiency components,which have large spreads among the cases,are negatively correlated,leading to a small dependence of the extreme precipitation response on the forcings.  相似文献   

20.
The regional climate model (RegCM3) and a tropospheric atmosphere chemistry model (TACM) were coupled, thus a regional climate chemistry modeling system (RegCCMS) was constructed, which was applied to investigate the spatial distribution of anthropogenic nitrate aerosols, indirect radiative forcing, as well as its climatic effect over China. TACM includes the thermodynamic equilibrium model ISORROPIA and a condensed gas-phase chemistry model. Investigations show that the concentration of nitrate aerosols is relatively high over North and East China with a maximum of 29 μg m-3 in January and 8 μg m-3 in July. Due to the influence of air temperature on thermodynamic equilibrium, wet scavenging of precipitation and the monsoon climate, there are obvious seasonal differences in nitrate concentrations. The average indirect radiative forcing at the tropopause due to nitrate aerosols is -1.63 W m-2 in January and -2.65 W m-2 in July, respectively. In some areas, indirect radiative forcing reaches $-$10 W m-2. Sensitivity tests show that nitrate aerosols make the surface air temperature drop and the precipitation reduce on the national level. The mean changes in surface air temperature and precipitation are -0.13 K and -0.01 mm d-1 in January and -0.09 K and -0.11 mm d-1 in July, respectively, showing significant differences in different regions.  相似文献   

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