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1.
Summary Erythemal ultraviolet (UV) doses reaching the earths surface depend in a complex manner on the amount of total ozone, cloud cover, cloud type and the structure of the cloud field. A statistical model was developed allowing the reconstruction of UV from measured total ozone and a cloud modification factor (CMF) for the GAW site Hohenpeissenberg, Germany (48°N, 11°E). CMF is derived from solar global radiation G, normalized against a Rayleigh scattering atmosphere. By this way the complex influence of the cloud field is accounted for by introduction of a measured parameter, exposed also to this complex field. The statistical relations are derived from the period 1990–1998 where UV measurements and relevant meteorological parameters are available. With these relations daily UV doses could be reconstructed back to 1968. Tests show that the model works remarkably well even for time scales of a minute except for situations with high albedo. The comparison of measured and calculated UV irradiances shows that the model explains 97% of the variance for solar elevations above 18° on average over the period 1968–2001. The reconstruction back to 1968 indicates that maximum UV irradiances (clear days) have increased due to long-term ozone decline. Clouds show seasonally depending long-term changes, especially an increase of cirrus. Consequently the UV doses have increased less or even decreased in some months in comparison to the changes expected from the ozone decline alone. In May to August total cloud frequency and cloud cover have decreased. Therefore, the average UV doses have increased much more than can be explained by the ozone decline alone. It is also shown that the optical thickness of cirrus clouds has increased since 1953. The higher frequency of cirrus is caused in part by more frequent contrails. Besides that an observed long-term rise and cooling of the tropopause favors an easier cirrus formation. However, whether climate change and an intensification of the water cycle is responsible for the cirrus trends has not been investigated in detail. 相似文献
2.
Total ozone variations in the tropical belt: An application for quality of ground based measurements
Summary The study of the regime of ozone variations in the huge tropical belt (25° S to 25° N), which are, in general, very small and zonally nearly symmetric, permits to establish a statistical model for estimating the ozone deviations using Total Ozone Mapping Spectrometer (TOMS) data. The equatorial stratospheric winds at 25 and 50hPa and the solar flux at 10.7 cm are used as major predictors and the linear trend was also estimated. The 10m/sec stratospheric wind change is related to1.2% ozone change at the equator, to practically no change in the 8–15° belts and up to 1.4% change with opposite phase over the tropics in spring but nearly zero change in fall. The solar cycle related amplitude is about 1.4% per 100 units of 10.7 cm solar flux. The ozone trends are negative: not significant over the equator and about –2% per decade (significant at 95% level) over the tropics. The latter could have been enforced by the 2 to 4% lower ozone values during 1991–1993, part of which might be related to the effects of the Mt. Pinatubo eruption, but might also be due to the strong QBO. The estimated deviations are verified versus reliable observations and the very good agreement permits applying the model for quantitative quality control of the reported ozone data from previous years. The standard deviation of the difference between observed ozone deviations and those estimated from the model is only 0.9–1.6% for yearly mean, that means instruments used for total ozone observations in the tropical belt should have systematic error of less than 1%. Cases when the discrepancies between the model and reported observations at a given station exceed 2–3% for time interval of 2 or more years should be verified.With 17 Figures 相似文献
3.
The total ozone content in the atmosphere was determined from the multichannel photometer observations of direct solar radiation made in the urban environment at Pune (18° 32 N, 73° 51E, 559 m ASL) and Sinhagad hill station (18° 22N, 73° 45E, 1305 m ASL) during March 1980-February 1982. The total ozone content of the atmosphere was computed making use of the differential absorption of solar radiation due to ozone at 0.4 and 0.6 m wavelengths in the Chappuis band. The values of the ozone data obtained from the photometer observations at Pune and Sinhagad were compared with the corresponding ozone data obtained from the Dobson spectrophotometer located at Pune. Values of ozone obtained by the photometric method were found to be smaller by 8–18% than the Dobson values when Vigroux's absorption coefficients were used. Similarly, when the absorption coefficients of Inn and Tanaka (1953) were used, the ozone values obtained by the photometric method were smaller by 4–14% than the Dobson values. The ozone values at the hill station obtained from the photometric method were in better agreement (5%) with the Dobson values. 相似文献
4.
北京地区太阳紫外辐射的观测与分析研究 总被引：10，自引：2，他引：10
利用北京地区太阳辐射和其它常规气象观测资料，得到了到达地面的太阳紫外辐射的计算公式，并将计算值与观测值进行了比较，两者吻合得比较好。最后给出了北京地区地面太阳紫外总辐射的变化趋势，计算结果表明，地面太阳紫外总辐射对大气浑浊度的变化比对大气臭氧总量的变化敏感得多。 相似文献
5.
J. W. Krzyścin 《Theoretical and Applied Climatology》1994,49(1):1-7
Summary Composite time series combining the results of total ozone measurements taken at Dobson stations located within the latitude band 30°N–60°N, in Europe, and North America, have been examined in order to detect any trends. Various regression trend models were used to identify any trend variations over the regions during the period 1970–1990. The results of fitting the models to the data imply that the model which assumes a linear trend provides precise information about the long-term ozone trends (trends during the period 1970–1990). The study identifies short-term summer trends in the 1980s that are evidently more strongly negative than trends that occur in the 1970s (the differences are statistically significant at the 2 level). The year-round loss (in all analyzed regions) and the winter loss in total ozone (the belt 30°N–60°N) N. America, during the 1980s are about 2–3 times higher than the losses during the 1970s (the differences are statistically significant at the 1 level).With 1 Figure 相似文献
6.
Eddy-correlation measurements of the vertical fluxes of ozone, carbon dioxide, fine particles with diameter near 0.1 m, and particulate sulfur, as well as of momentum, heat and water vapor, have been taken above a tall leafless deciduous forest in wintertime. During the experimental period of one week, ozone deposition velocities varied from about 0.1 cm s–1 at night to more than 0.4 cm s-1 during the daytime, with the largest variations associated primarily with changes in solar irradiation. Most of the ozone removal took place in the upper canopy. Carbon dioxide fluxes were directed upward due to respiration and exhibited a strong dependence on air temperature and solar heating. The fluxes were approximately zero at air temperatures less than 5 °C and approached 0.8 mg m–2 s–1 when temperatures exceeded 15 °C during the daytime. Fine-particle deposition rates were large at times, with deposition velocities near 0.8 cm s–1 when turbulence levels were high, but fluxes directed upward were found above the canopy when the surface beneath was covered with snow. Diffusional processes seemed to dominate fine-particle transfer across quasilaminar layers and subsequent deposition to the upper canopy. Deposition velocities for particulate sulfur were highly variable and averaged to a value small in magnitude as compared to similar measurements taken previously over a pine forest in summer. 相似文献
7.
Rumen D. Bojkov 《Meteorology and Atmospheric Physics》1988,38(3):117-130
Summary All total ozone observations ever made in the Northern polar region, including some from the 1930's, have been corrected and the basic climatology presented. The long-term ozone changes were considered in relation to the stratospheric temperatures. For each deviation from the monthly normal of the 100 hPa temperature by 1°C, there was found to be a corresponding 5–6 m atm-cm change in the monthly ozone deviation. A distinction between the ozone regimes over the Scandinavian, Canadian and East Siberian sectors of the polar region was noted. The strong appearance of the QBO (Quasi Biennial Oscillation) in the interannual ozone fluctuations was obvious. It is demonstrated that for the past three decades the total ozone experienced a few periods with positive and a few periods with negative deviations. In view of this, trends in ozone must obviously be based on greater than 10 years of data. During 1964–86, the weighted trend over the polar stations was (–0.9±0.4)% per decade. There have been, however, three periods (1958–64, 1968–76 and 1979–86), coinciding with the declining phase of the 11 year sunspot cycle, during which the ozone at all polar stations has been declining by about 0.5% per year (or less if the QBO component is filtered out). Some of the differences with Antarctic ozone are mentioned and the dominant role of the stratospheric circulation for the ozone variations is discussed. In general the Arctic ozone observations show no evidence of a major ozone decline similar to that over Antarctica.With 9 Figures 相似文献
8.
Sinnhuber B.-M. Müller R. Langer J. Bovensmann H. Eyring V. Klein U. Trentmann J. Burrows J. P. Künzi K. F. 《Journal of Atmospheric Chemistry》1999,34(3):281-290
In this study measurements of mid-stratospheric Arctic ozone are compared with model simulations. The measurements obtained at Spitsbergen (79°N, 12°E) by ground based millimeter-wave radiometry exhibit large day to day variabilities as well as periods with low ozone. To interpret these measurements, calculations were made using the new photochemical box-trajectory model BRAPHO, with air parcel trajectories calculated from analyzed wind fields. Using a relatively simple approach, the model reproduces the observed ozone variability well, including inter-annual variations. The explanation for the observed ozone behavior is that at these altitudes ozone is determined by what we call dynamically controlled photochemistry. This means that the photochemical evolution of the ozone volume mixing ratio is mainly controlled by the atmospheric dynamics, in particular the solar zenith angle the air parcel has experienced. 相似文献
9.
采用1979—2013年6—8月欧洲中期数值预报中心ERA-Interim逐月再分析资料和2004—2010年6—8月美国国家大气和海洋管理局太阳光谱辐照度资料,利用北京气候中心大气辐射模式,计算了北半球平流层夏季臭氧加热率(Ozone Heating Rate,OHR)和净加热率(Net Heating Rate,NHR),分析了太阳准11 a变化中太阳活动强年与弱年纬向平均OHR(NHR)的差异,并讨论了差异形成的原因。结果表明:太阳活动强年比弱年的紫外辐射明显要强,导致OHR、NHR整层增强,且随高度增加而增加;臭氧浓度在平流层下层较小,在平流层上层较大,该变化导致OHR、NHR有类似的变化型,且稍向高处偏移;OHR、NHR在平流层上层的变化,由紫外辐射和臭氧共同作用,其他地区均为臭氧起主要作用。 相似文献
10.
Ozone measurements, performed since 1987, at the Swedish TOR/EUROTRACstation Åreskutan (lat. 63.4° N, long. 13.1° E, 1250 m abovesea level) are analyzed. The annual average ozone concentration at the sitehas increased by about 0.4 ppbv (1%) per year during the period1987–1994. The corresponding trends for individual months show adecrease during April–September and an increase during the rest of theyear. The ozone budget at Åreskutan has been investigated using backtrajectories of the air parcels, and the cosmogenic radionuclide7Be as a tracer of stratospheric air. From a simple diagnosticmodel, it is estimated that the contribution of stratospheric ozone to theconcentrations measured at Åreskutan is 5 ppbv (or 14% of themeasured values) on average, reaching a maximum of 23 ppbv (50%),during the episodes of direct stratospheric influence. In spring, thestratospheric contribution to ozone budget at Åreskutan is at itsmaximum, and approximately equal to the net photochemical ozone productionin the air mass affecting the site, whereas in winter, it is compensated byozone chemical sink during the transport of air masses from pollutedEuropean regions, to Scandinavia. 相似文献
11.
H. D. Behr 《Journal of Atmospheric Chemistry》1992,15(3-4):299-314
A three-week continuous record from 21 September to 5 October 1988 of solar and terrestrial downward and upward radiation flux densities (1 data set per minute) obtained during the Atlantic Ocean cruise of the R/V Polarstern (ANT VII/1) along 30° W between 30° N and 30° S is evaluated. As the cruise crossed both subtropics and tropics of the Atlantic Ocean, characteristic daily cycles and meridional distributions of the radiation components and atmospheric turbidity were obtained. Special attention is given to the ultraviolet component of global radiation. The influence of cloudiness on the radiation quantities is discussed. As the knowledge of the spatial and temporal distribution of solar and longwave atmospheric radiation at the sea surface is important for numerous meteorological, oceanographic, and physico-chemical investigations, this data set is compared with other measurements of the cruise. This work is the continuation of the measurements made during the cruise ANT V/5 of R/V Polarstern along 30° W between 40° S and 40° N in March/April 1987. 相似文献
12.
Klaus Wege 《Journal of Atmospheric Chemistry》1991,12(4):381-390
On 1 February 1989, -83.5°C was recorded in 27.8 hPa over Hohenpeißenberg, the lowest temperature in the 22-year series. This was measured together with a very low total ozone amount of 266 DU. This may be compared with nearly twice this amount on 27 February 1989. The situation was very unusual: following an extremely cold winter in the Arctic stratosphere, the stratospheric cold pole was located over southern Scandinavia on 1 February in a very southerly position. The analyzed temperatures of -92 °C in 30 hPa were also unusual. Even though the low ozone amounts over Hohenpeißenberg were probably dynamically caused, an additional very small ozone decrease due to heterogeneous reactions in altitudes from 23–28 km, where the temperatures lie below -80 °C, cannot be ruled out. Extinction measurements by the orbitting SAGE II instrument indeed show polar stratospheric clouds over Europe near 50° N during the period 31 January–2 February. Also, polar stratospheric clouds were previously observed over Kiruna at similarly low temperatures and signs of a corresponding small ozone decrease were noted there. 相似文献
13.
Measurements of NOx,y were made at Alert, Nunavut, Canada (82.5° N, 62.3° W) during surface layer ozone depletion events. In spring 1998, depletion events were rare and occurred under variable actinic flux, ice fog, and snowfall conditions. NOy changed by less than 10% between normal, partially depleted, and nearly completely depleted ozone air masses. The observation of a diurnal variation in NOx under continuous sunlight supports a source from the snowpack but with rapid conversion to nitrogen reservoirs that are primarily deposited to the surface or airborne ice crystals. It was unclear whether NOx was reduced or enhanced in different stages of the ozone depletion chemistry because of variations in solar and ambient conditions. Because ozone was depleted from 15–20 ppbv to less than 1 ppbv in just over a day in one event it is apparent that the surface source of NOx did not grossly inhibit the removal of ozone. In another case ozone was shown to be destroyed to less than the 0.5 ppbv detection limit of the instrument. However, simple model calculations show that the rate of depletion of ozone and its final steady-state abundance depend sensitively on the strength of the surface source of NOx due to competition from ozone production involving NOx and peroxy radicals. The behavior of the NO/NO2 ratio was qualitatively consistent with enhanced BrO during the period of active ozone destruction. The model is also used to emphasize that the diurnal partitioning of BrOx during ozone depletion events is sensitive to even sub ppbv variations in O3. 相似文献
14.
Summary Statistical techniques have been developed to homogenise a broken series of clear-sky solar UV-B radiation, measured by a Robertson Berger (RB) meter over the period 1981–90 at Invercargill, New Zealand, and to analyse the series for long term trend. Statistical modelling of the quasi-linear UV-B/ozone relationship evident in the departures of daily clear-sky UV-B data and coincident satellite ozone data from their respective mean references has been used to provide a self-consistent de-seasonalised data set of UV-B and ozone departures, and to bridge a major gap in calibration that separates the data set into two periods, 1981–86 and 1988–90. The choice of UV-B reference is important to the quality of the results and particular attention was given to the methodology for defining it. Four alternative objective adjustment procedures for calibrating the 1988–90 period against the 1981–86 period were examined. Because our interest lies primarily in the higher values of summer, a UV-B-weighted procedure was chosen. The modelling and homogenisation techniques developed may have application in related analysis problems. Analysis of the data for the independent 1981–86 period showed large trends in ozone and UV-B, but this was mostly due to a period of very low ozone values during 1985. Over the whole period, 1981–90, the ozone trend was –4.7%/decade. The corresponding UV-B trend was +5.8%/decade, but this result is not independent of the corresponding ozone trend because the homogenisation procedure imposes the assumption of the derived UV-B/ozone relationship on the 1988–90 UV-B data. However, the evidence suggests there is little reason to doubt that solar UV-B radiation has increased at the site by about +6% per decade.With 10 Figures 相似文献
15.
16.
Dr. R. D. Bojkov D. S. Balis C. S. Zerefos 《Meteorology and Atmospheric Physics》1998,69(1-2):119-135
Summary The total ozone decline during the past twenty years, especially strong during the winter-spring season poleward from 50° N, is well established with known average trends of 5–7% per decade. This study presents a number of additional characteristics such as ozone-mass deficiency (O3MD) from the pre- 1976 base average, and areal extent with negative deviations greater than2 and3. Gridded satellite data combined with ground-based total ozone maps, permit calculations of daily and regional ozone deficiencies from the anthropogenically undisturbed average ozone levels of the 1960s and early 1970s. Then the quantity of the O3MD and the changes in surface area, with deficiencies larger than-10 and-15% are integrated for the 1 January to 15 April period for each of the last 20 years, and compared. In addition, the polar vortex extent during the last 10 years is determined using the PV at 475°K. The quantity of the O3MD within the sunlit part of the vortex is shown to contribute from15 to 35% of the overall ozone deficiency within the-10% contours over the area 35–90°N. The ozone deficiency, integrated for the first 105 days of each year, has increased dramatically from 2,800Mt in the early 1980s to7,800Mt in the 1990s, exceeded 12,000Mt in the winter-springs of 1993 and 1995. The latter quantity is comparable with the average O3MD over the same Southern latitudes in the last ten austral springs. During the 1990s over the 35–90° latitudes the average ozone deficiency in the Southern hemisphere belt is less than over the Northern hemisphere belt by40%. It is known that the main ozone decline is observed in the lower stratosphere and the ozone loss over the Arctic is very sensitive to decreasing stratospheric temperatures; negative 50hPa monthly anomalies greater than 4°C have occurred during 7 of the springs in the last decade, thus possibly facilitating doubling the area with negative ozone deviations greater than-10% in the 1990s to5,000.106km2 and nearly tripling the O3MD as stated above. The changes in total eddy heat fluxes as a proxy indicator of the long wave perturbations are positively correlated with the ozone deficiency in the 45–75°N. The strong anticorrelation between the ozone deficiency in the region>55° N. versus the 35–50° N belt is discussed in relation to possible transport of air masses with low ozone from the sub-tropics, which in some years are the dominant reason for the observed ozone deficiency.With 11 Figures 相似文献
17.
AbstractThe solar backscattered ultraviolet (SBUV/SBUV-2) merged ozone datasets, version 8.6, including column ozone and ozone profiles for the 1979–2012 period are examined for the 35°N–60°N zonal belt in the northern hemisphere mid-latitudes and four sub-regions: central Europe, continental Europe, North America, and East Asia. The residual long-term patterns for total ozone and ozone profiles are extracted by smoothing the time series of differences between the original and the modelled ozone time series. Modelled ozone is obtained using the standard trend model accounting for ozone variability due to changes in stratospheric halogens and various dynamical factors commonly used in previous ozone trend analyses. Since about 2005 spring and summer total ozone in the troposphere and lower stratosphere has decreased in some regions (central and continental Europe, North America, and the 35°N–60°N zonal belt) compared with modelled ozone. The negative departure from modelled ozone in 2010 is approximately 2–3% of the overall 1979–2012 monthly mean level. It seems that this decrease is a result of yet unknown dynamical processes rather than to chemical destruction because the differences have a longitudinal structure, and total ozone in the upper stratosphere still follows changes in stratospheric halogen loading. 相似文献
18.
19.
晴空或少云状况下紫外辐射强度及指数预报模式 总被引：4，自引：0，他引：4
在大气辐射传输理论的基础上，利用中分辨率大气辐射传输系统，应用可测得的实际大气物理参数，建立睛空或少云天气状况下石家庄市紫外波段（280-400nm)辐射强度及指数预报模式，考虑了臭氧的两个吸收带。晴空条件下的散射主要考虑了分子和气溶胶的多次散射，少云时还考虑了云对紫外辐射的影响。其中多次散射的计算采用子离散坐标法。且对由于臭氧实时资料的短缺造成的误差进行了系统订正，并将订正结果与实况资料进行了对比。结果表明，由模式客观预报紫外辐射强度是可行的。 相似文献
20.
Joonsuk Lee Won Jun Choi Deok Rae Kim Seung-Yeon Kim Chang-Keun Song Jun Suk Hong Youdeog Hong Sukjo Lee 《Asia-Pacific Journal of Atmospheric Sciences》2013,49(3):271-278
Surface erythemal UV radiation is mainly affected by total column ozone, aerosols, clouds, and solar zenith angle. The effect of ozone on the surface UV radiation has been explored many times in the previous studies due to the decrease of ozone layer. In this study, we calculated the effect of aerosols on the surface UV radiation as well as that of ozone using data acquired from Ozone Monitoring Instrument (OMI). First, ozone, aerosol optical depth (AOD), and surface erythemal UVB radiation measured from satellite are compared with those from ground measurements. The results showed that the comparison for ozone was good with r 2 of 0.92. For aerosol, there was difference between satellite measurements and surface measurements due to the insufficient information on aerosol in the retrieval algorithm. The r 2 for surface erythemal UV radiation was high (～0.94) but satellite measurements showed about 30% larger values than surface measurements on average by not considering the effect of absorbing aerosols in the retrieval process from satellite measurements. Radiative amplification factor (RAF) is used to access the effect of ozone and aerosol quantitatively. RAF for ozone was 0.97～1.49 with solar zenith angle. To evaluate the effect of aerosol on the surface UV radiation, only clear-sky pixel data were used and solar zenith angle and total column amount of ozone were fixed. Also, RAF for aerosol was assessed according to the single scattering albedo (SSA) of aerosols. The results showed that RAF for aerosol with smaller SSA (< 0.90) was larger than that for with larger SSA (> 0.90). The RAF for aerosol was 0.09～0.22 for the given conditions which was relatively small compared to that for ozone. However, considering the fact that aerosol optical depth can change largely in time and space while the total column amount of ozone does not change very much, it needs to include the effect of aerosol to predict the variations of surface UV radiation more correctly. 相似文献