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1.
We used sediment chronology data from fourteen published studies of lake cores across much of North America and Scandinavia in order to make a large scale comparison of the different dating techniques. The uncertainty of210Pb derived dates was determined using common sediment event markers: the stable Pb rise, the137Cs rise, and theAmbrosia pollen rise. For all data combined, the 95% confidence intervals for the stable Pb rise and theAmbrosia rise, were approximately 30 years. These 95% confidence intervals are slightly higher than those derived by First-Order Error analysis performed by others on210Pb derived dates. When comparing the concordance of two210Pb models (CRS and CIC) against markers of known history, we found that the CRS model dates (constant rate of supply) had consistently better agreement than the CIC model dates (constant initial concentration). Major discrepancies between137Cs and210Pb were common, but were consistently more severe in sediments of soft water lakes pointing to an inability of sediments with low mineral content to immobilize Cs.This is the ninth of a series of papers to be published by this journal following the 20 th anniversary of the first application of210Pb dating of lake sediments, Dr. P. G. Appleby is guest editing this series.  相似文献   

2.
Low-background gamma counting: applications for210Pb dating of sediments   总被引：1，自引：0，他引：1  
Sediment cores from three lakes were dated with210Pb using a constant rate of supply (CRS) model. We used low-background gamma counting to measure naturally occurring levels of210Pb,226Ra, and137Cs in sediment samples because sample preparation is simple and non-destructive,226Ra activity provides a direct measure of supported210Pb activity for each sample analyzed, and137Cs activity may provide an independent age marker for the 1962–1963 peak in atmospheric fallout of this radionuclide. In one core supported210Pb activity was estimated equally well from226Ra activity of each sampling interval or from the mean total210Pb activity of constant activity samples at depth. Supported210Pb activity was constant with depth in this core. In a short freeze core, determining226Ra activity of every sample proved advantageous in estimating supported210Pb activity because supported210Pb activity could be estimated from210Pb measurements only at the deepest sampling interval. Supported210Pb activity estimated from226Ra activity also yielded more precise estimates of highly variable sedimentation rates. In the third core226Ra activity exceeded210Pb activity at the top of the core and varied 20 fold with depth. This high input of226Ra in disequilibrium with210Pb is attributed to recent erosion of radium-bearing materials in the drainage basin. These data invalidate the assumption that supported210Pb activity is constant in sediment cores and can be estimated from the mean total210Pb activity at depths where210Pb activity is constant. We recommend using gamma counting or another independent assay of226Ra to validate the assumption of constant supported210Pb activity in sediment cores if there is reason to expect that226Ra activity varies with depth.This is the fourth of a series of papers to be published by this journal following the 20 th anniversary of the first application of210Pb dating of lake sediments. Dr. P.G. Appleby is guest editing this series.  相似文献   

3.
210Pb and 137Cs dating methods in lakes: A retrospective study   总被引：1，自引：0，他引：1  
210Pb has been used for more than two decades to provide the geochronology of annually deposited sediments and to construct pollution histories. Evidence from some lakes suggests that this radionuclide may be adequately mobile to compromise dating reliability. This study provides one test of that possibility by comparing recent measurements of 210Pb and trace metals to ones carried out more than 20 yrs in the past. 137Cs dating is used to confirm sediment accumulation rates in the recent cores. In the three Connecticut, USA, lakes studied, sediment accumulation rates changed abruptly to higher values between 40-50 yrs ago (increasing by factors of 2.2, 2.9, and 3.0). In all three lakes, rates calculated from 210Pb distributions both above and below this horizon agreed, within measurement uncertainty, in recent and older cores. Furthermore, when the older data were corrected for 20 yrs of burial, the changes in slope in 210Pb distributions occurred at the same depth in each pair of cores. The depth of sharp peaks in concentrations of trace metals also matched. In general, this evidence supports the idea that sediments in these lakes have simply been buried, without significant diagenetic remobilization of 210Pb and trace metals . Nevertheless, some important differences were also observed. For two of the three lakes, there was a significant difference in average sediment accumulation rate during the past 33 yrs as calculated from 137Cs and 210Pb in the recent cores. Most potential causes for this difference can be ruled out, and it appears that one of the two nuclides is remobilized compared to the other. There were also significant differences in the total inventories of both 210Pb and trace metals (both up to 2 ×) between recent and older cores in some cases. This may be due to dissimilar sediment focusing, since it is not known for certain whether the new cores were collected at exactly the same sites as in the past.  相似文献   

4.
A large seabird colony of northern fulmars (Fulmarus glacialis) at Cape Vera on Devon Island in the Canadian high Arctic has been shown to act as an effective biological pump, transporting large quantities of marine-derived nutrients and contaminants to the ponds beneath their nesting sites. Previous research has shown that seabirds also have the potential to elevate radionuclide concentrations in their immediate surroundings. Here, we assess the influence of the Cape Vera seabird colony on the 210Pb budgets of six affected ponds and one control site, and discuss potential implications with respect to 210Pb dating methodologies. In general, fluxes of 210Pb at Cape Vera were similar to, or less than, those measured at other Arctic locations not influenced by seabirds. Plots of unsupported 210Pb activity versus depth showed a number of non-monotonic features in all sediment cores, necessitating the use of the constant-rate-of-supply (CRS) model to derive age-depth profiles. We conclude that seabird activity has not dramatically increased the 210Pb flux to the ponds at Cape Vera. Overall, the low flux of excess 210Pb made accurate dating problematic for some of the study cores, necessitating the use of independent dating markers (e.g., 137Cs and PCB concentrations) to verify the reliability of the chronologies.  相似文献   

5.
A combination of tephrochronology and 14C, 210Pb, and 137Cs measurements provides a robust chronology for sedimentation in Upper Klamath Lake during the last 45 000 years. Mixing of surficial sediments and possible mobility of the radio-isotopes limit the usefulness of the 137Cs and 210Pb data, but 210Pb profiles provide reasonable average sediment accumulation rates for the last 100–150 years. Radiocarbon ages near the top of the core are somewhat erratic and are too old, probably as a result of detrital organic carbon, which may have become a more common component in recent times as surrounding marshes were drained. Below the tops of the cores, radiocarbon ages in the center of the basin appear to be about 400 years too old, while those on the margin appear to be accurate, based on comparisons with tephra layers of known age.Taken together, the data can be combined into reasonable age models for each site. Sediments have accumulated at site K1, near the center of the basin, about 2 times faster than at site CM2, on the margin of the lake. The rates are about 0.10 and 0.05 cm/yr, respectively. The chronological data also indicate that accumulation rates were slower during the early to middle Holocene than during the late Holocene, consistent with increasing wetness in the late Holocene.  相似文献   

6.
We present a historical overview of applications of210Pb dating in Switzerland with a special emphasis on the work performed at the University of Bern. It is demonstrated that the average specific activity of210Pb in the lower atmosphere is very constant and does not show seasonal variations. We then concentrate on new results from Lobsigensee, a very small lake, and on published and new data from Lake Zurich. Several210Pb profiles from these lakes show obvious disturbances and a disagreement of the resulting sedimentation rate when compared to that for the 23 years defined by137Cs peaks of 1986 (Chernobyl) and 1963 (bomb fallout).A mean sedimentation rate of about 0.14 g cm–2 y–1 is found in the oxic and suboxic center part of Lake Zurich. In the oxic locations, the210Pb flux to the sediments was close to the atmospheric input of about 1/60 Bq cm–2 y–1. In other parts of the lake a significant deficit in the inventory of210Pb was found in the sediments. This could be due to a chemical redissolution of210Pb together with Mn under reducing conditions. In contrast, in the suboxic part of the lake (135 m depth) the flux of210Pb was about twice the atmospheric input. This excess is not caused by allochthonous contributions and is tentatively explained by the transport of sediment material resulting from small slides at the very steep lake shores or more probably by reprecipitation of210Pb together with Mn when the conditions in the lake water become locally and seasonally more oxidizing. Dissolved210Pb may migrate from locations with reducing conditions and reprecipitate under more oxic conditions. Indeed, a correlation of Mn and210Pb in sediments of Lake Zurich was found.This is the first of a series of papers to be published by this journal following the 20th anniversary of the first application of210Pb dating of lake sediments. Dr P. G. Appleby is guest editing this series.  相似文献   

7.
Post-depositional mobility of137Cs,239+240Pu and210Pb was assessed in six small lake basins by comparing sedimentary nuclide profiles with their known fallout history. Laminae couplets, when present, were determined to be varves because the137Cs and239+240Pu 1963 fallout peaks are present in laminae couplets corresponding to years 1962–1964. There is no evidence of mobility of210Pb, because 1) mass accumulation rates based on210Pb agree with those based on137Cs and239+240Pu peak depths and with those based on varve counts, and 2)210Pb ages agree with varve ages. Significant mobility of137Cs is evident from the penetration of137Cs to depths 15–20 cm deeper than239+240Pu. Deep penetration of137Cs in spite of a sharp gradient below the peak is interpreted by a numerical model to suggest that137Cs is present in two distinct forms in these sediments, 67–82% as an immobile form and 18–33% reversibly adsorbed with a K d of approximately 5000. The profiles can be interpreted equally well assuming a small portionof the total137Cs was present as an extremely mobile phase (K d 5000) in the months to years following peak fallout, slowly becoming more strongly adsorbed. High NH 4 + concentrations in porewaters may enhance diffusion of the mobile form of137Cs, but not of the immobile form of137Cs that defines the sharp gradient. Mobility of137Cs is likely also enhanced by the low clay content and the high porosity of these sediments. Thus the first detection of137Cs in the sediments cannot automatically be assumed to correspond to a date of 1952 (initial testing of thermonuclear weapons), although the depth of the peak can be assumed to correspond to 1963 (the year of maximum fallout from testing of thermonuclear weapons).239+240Pu is a more reliable sediment chronometer than137Cs because it is significantly less mobile.This is the sixth of a series of papers to be published by this journal following the 20 th anniversary of the first application of210Pb dating of lake sediments. Dr P.G. Appleby is guest editing this series.  相似文献   

8.
We present 137Cs profiles for three low lying coastal lagoons in Southwest England that show a decline in activity with sediment depth. 137Cs inventories are lower than expected by comparison with local reference inventories despite the fact that sampling was undertaken in the deep-water zone of each lake where sediment and 137Cs focusing would be expected. At all three locations, lake sediment 7Be and unsupported 210Pb (210Pbun) inventories are not significantly lower than the local reference inventory. 137Cs inventories in the study cores range from 38 to 95% of local reference inventories. The standing water level and mud: water interface at two sites are below maximum tide level and, at all three sites, salinity increases significantly in the water columns between low and high tide and in the pore waters of the underlying sediments. We suggest that the difference in hydrostatic pressure between sea level and standing water levels in the lagoons forces salt water up through the sediment column and that monovalent cations (especially Na+ and K+) replace 137Cs on exchange sites leading to the upward migration and loss of 137Cs. Rising sea levels may therefore contribute to remobilisation and release of 137Cs to the aquatic environment from the sediments of coastal lagoons.  相似文献   

9.
Application of210Pb in soils   总被引：2，自引：0，他引：2  
The spectroscopic measurement of soil samples is described.210Pb data from a soil survey in western-Europe are briefly reviewed. The average210Pb flux from the atmosphere, as determined from210Pb exc soil inventories, is 90 Bq m–2a–1. A simple one-dimensional box-chain model is described. The model simulates the vertical, post depositional transport of natural and fall-out radionuclides in the soil. Simulation of measured210Pb exc ,134Cs,137Cs, and241Am soil profiles shows that mixing (bioturbation) is a very efficient transport mechanism. Lead seems to be strongly fixed to organic and clay particles. It is transported by the displacement of the organic and clay carrier substances. The mean residence time of lead, caesium, plutonium and americium in organic rich forest soils is in the order of 250–1000 years. An applicability study in investigate the use of210Pb in erosion problems showed erosion rates from 60–180 g m–2a–1 on organic rich forest and meadow sites with 10°–25° slopes.This is the eighth of a series of papers to be published by this journal following the 20 th anniversary of the first application of210Pb dating of lake sediments. Dr P. G. Appleby is guest editing this series.  相似文献   

10.
Seven cores were collected from different sediment zones of tidal flats at Xinyanggang in north Jiangsu province in August 2007. Sediment grain-size distribution and radioisotopes of 137Cs and 210Pb analysis were carried out for these cores. Sediment rates of the cores and radioisotopes distribution in surface sediment in different zones of the tidal flat were calculated from the 137Cs and 210Pb activities in sediments cores. The results indicated that each tidal zone had experienced different evolution phases, hydrological dynamics in the tidal flats made the grain-size of the surface sediment change gradually. 137Cs and 210Pb activities on the superficial layer of the cores varied spatially and the reason was discussed. On tidal flats, the fluctuation of 137Cs and 210Pb activities in the cores reflected the special sedimentary characteristics. Vegetation affects the grain-size distribution and the vertical profiles of 137Cs and 210Pb in the upper depths. 137Cs and 210Pb chronology got the comparable average sediment rates on the tidal flat. The characteristics of 137Cs and 210Pb in the cores reflected various depositional dynamical environments in different tidal zones and gave information on the different evolvement phases of the tidal zones. Based on the information of grain-size distribution, texture of the cores, sediment rates and topography, the evolution lines of the tidal flat were reconstructed.  相似文献   

11.
210Pb geochronologies should be validated with independent tracers such as 137Cs. In the cases with constant 210Pb activity in the topmost sediments, the presence of a distinct 137Cs peak within the 210Pb plateau has been used as a definitive demonstration of acceleration (increase in the sedimentation rate in recent years) versus fast mixing. Nevertheless, some limitations can be identified in the use of semiquantitative arguments, and a global understanding of the whole 137Cs activity profile is then required. Particularly, the incomplete mixing within the top sediment zone (described through the Incomplete Mixing Zone model) can explain quantitatively and simultaneously the 137Cs peak and the flattening in the 210Pb activity profile. This is demonstrated using selected examples from literature data. Thus, measured constant 210Pb activities in the top 6 cm of a sediment core from Lake Zürich. Nevertheless, they found 7Be only in the uppermost layer, the distinct 137Cs maximum at 6 cm depth, and undisturbed varves. The fast mixing seemed then opposed to common sense. The constant rate of supply model shows acceleration and it adequately matches the position of the 1963 137Cs peak. Nevertheless it fails to explain the whole 137Cs profile when handling time series of 137Cs atmospheric deposition. Finally, it is shown how the incomplete mixing of the activity (through the pore water) over a certain mass depth at the top sediment, with a finite value of the mixing coefficient, can quantitatively explain the whole activity versus mass depth profiles of 137Cs and 210Pb, and the presence of 7Be only in the uppermost sediment layer. A further validation of these ideas is presented from other literature data.  相似文献   

12.
Traditional techniques used to assemble information on rates of erosion and soil redistribution possess many important limitations. As a result, the use of environmental radionuclides, and more particularly 137Cs measurements, has attracted increasing attention in recent years as a means of obtaining spatially distributed information on rates of erosion and deposition. The application of the 137Cs approach is, however, hampered in some areas of the world where 137Cs inventories are low and the low concentrations of 137Cs found in soils and sediments cause problems for laboratory analysis. These problems will increase as time progresses due to the radioactive decay of the existing inventory, most of which was deposited as fallout ca. 40 years ago. This contribution explores the potential for using another fallout radionuclide, namely unsupported 210Pb, as an alternative to 137Cs, in the small (63 km2) Upper Kaleya catchment in southern Zambia where 137Cs inventories are already very low. The approach employed with unsupported 210Pb is similar to that used for 137Cs, although the essentially constant fallout of unsupported 210Pb through time means that the resulting estimates of erosion and soil redistribution rates reflect a longer period of time (ca. 100 years rather than ca. 40 years). The estimates of erosion and deposition rates derived from the unsupported 210Pb measurements are used to construct typical sediment budgets for the three main land-use types in the Upper Kaleya catchment, namely, commercial cultivation, communal cultivation and bush grazing. The results obtained from the unsupported 210Pb are compared with equivalent results based on 137Cs measurements provided by a previous investigation undertaken in the study catchment. The two sets of results are highly consistent. The study reported confirms the viability of using unsupported 210Pb as an alternative to 137Cs in this environment and demonstrates that conjunctive use of both radionuclides can provide additional information on the erosional history of a study area.  相似文献   

13.
There is an important volume of published information on Lac Dufault (Québec) which describes the history of metal inputs over 70 years and the changes that occurred in the lake as a result of this contamination. We used this abundant source of chronological markers to test the hypothesis that lake sediments can provide true historical records of trace metal loading from metal mining. Sediment cores were obtained from the deepest zone of the lake (19 m). The sediments were dated using 210Pb and 137Cs and they were analyzed for total elemental concentrations (Ca, Cd, Cu, Fe, P, Pb, S, Zn). Metal profiles in the sediment core preserved the distinct signatures of different mine exploitations documented in the lake watershed. In particular, the core recorded: the beginning of industrialization in 1926; increasing sedimentation rates associated with perturbations in the lake watershed; the maximum of sediment [Cu] and the contemporary exploitation of ore bodies rich in Cu; the maximum of sediment [Fe] and the contemporary production of pyrite by a mining operation; the low sediment [Cu] and [Zn] in the 1950s and the low contemporary production of these metals by mining operations; the maximum of sediment [Cd] and the contemporary production of Cd by a subsequent mining operation. Anomalies in the distribution of 214Pb activities in sediments reflected the intensity of acid mine drainage (AMD). There is good evidence that the lake resisted acidification from this AMD for the last thirty years. Overall, our results support the thesis that profiles of sedimentary Cd, Cu, Zn, Pb and Fe levels reflect the past history of metal input to Lac Dufault.  相似文献   

14.
The world fallout of caesium-137 (137Cs) associated with nuclear weapons testing during the 1950s and 1960s has provided a valuable man-made tracer for studies of soil erosion and sediment delivery. But relatively few researchers have used it to estimate wind erosion. In this paper, the137Cs technique is introduced into the study of wind erosion and its modern processes in the Qinghai-Tibet Plateau. Two137Cs reference inventories of 982·11 and 2376·04 Bq m−2was established preliminarily, which distribute in the south and mid-north parts of the study area respectively. By analysing the patterns of137Cs depth profiles from sampling sites, the aeolian processes of erosion and deposition along nearly 40 years has been revealed, i.e. the shrub coppice dunes(S1) and semi-fixed dunefields (S3) had experienced the alternation of erosion and deposition, while the grasslands (S4, S6 and S7) and dry farmlands (S5) suffered erosion only. By using the137Cs model, the average wind erosion rates for shrub coppice dune (S1), semi-fixed dunefields (S3), dry farmlands (S5) and grasslands (S4, S6 and S7) were estimated to be 84·14, 69·43, 30·68 and 21·84 tha−1a−1respectively, and for the whole Plateau, averaging 47·59 ha−1a−1which can be regarded as the medium erosion standard. These results derived from137Cs for the first time have significant implications for the further research of wind erosion and desertification control in the Qinghai-Tibet Plateau.  相似文献   

15.
Although lake sediment archives are widely used for reconstructing historical records of atmospherically delivered pollutants, the quantitative relationship between fallout levels and their record in the sediments is complex and not well known. The original input signal from the atmosphere can be significantly distorted by mediating transport processes in the catchment, through the water column and within the sediments themselves. Since these processes also affect the fallout radionuclide 210Pb commonly used to date sediments, a better understanding of their impact is also important to improving the accuracy and reliability of sediment dating. Blelham Tarn has been the subject of a number of palaeolimnological investigations using radiometric dating techniques since the early 1970s. More recently it was the site of a major study carried out within the EU Transuranics project concerning the long-term fate of fallout radionuclides in catchment/lake systems. This paper reviews the radiometric data from this study and uses the results to determine mass balances for fallout 210Pb, 137Cs and 239+240Pu in Blelham Tarn, and their spatial distribution over the bed of the lake. Atmospheric fluxes were determined by measuring concentrations in rainwater and cumulative inventories in soil cores from non-eroding sites. Sediment records in a grid of 16 cores were used to determine the spatial distribution over the bed of the lake, and net inputs from the catchment. Mass balance calculations indicate that c. 47% of 210Pb in the sediments derives from erosive inputs from the catchment. For 239+240Pu the figure rises to 61%. Reduced amounts of 137Cs in the sediments are attributed to greater losses of this radionuclide from the water column via the outflow due to its greater solubility. Inputs of radionuclides from the catchment are concentrated near one of the major input streams. Away from this part of the lake the sediment record is dominated by direct atmospheric fallout, though the detailed pattern is influenced by sediment focussing. A one parameter catchment/lake transport model is developed that incorporates the assumption that transport rates will decline with time as fallout on the catchment diffuses into the soil and becomes less available for removal. Values of the transport parameter were calculated for 210Pb and 239+240Pu and found to be comparable. The results suggest that it will take c. 11000 years to remove 50% of 239+240Pu from the catchment to the lake.  相似文献   

16.
Over the past 150 years, major land use changes have occurred in the Stemple Creek Watershed in northern California that have caused erosion to move soils from the upland to the flood plain, stream channels, and the bay. The purpose of this study is to document the recent (1954 to present) sediment deposition patterns in the flood plain area adjacent to Stemple Creek using the 137Cesium technique. Sediment deposition ranged from 0.26 to 1.84 cm year−1 for the period from 1964 to 2002 with an average of 0.85±0.41 cm year−1. Sediment deposition rates were higher for the 1954 to 1964 period with a range of 0.31–3.50 cm year−1 and an average of 1.29±1.04 cm year−1. These data indicate that sediment deposition in the flood plain has decreased since the middle 1950s, probably related to reduction in row crop agriculture and an increase in pasturelands. This study shows that the flood plains in the Stemple Creek Watershed are a significant sink for the soils being eroded from the upland area. Given the significance of the flood plain for trapping eroded materials before they reach the stream channels or the bay, efforts need to be made to manage these flood plain areas to insure that they do not change and become a source rather than a sink for eroded materials as improved management practices on the upland areas reduce sediment input to the flood plain.  相似文献   

17.
Pb-210 dating of two metal-polluted organic sedimentcores obtained near a former pyrometallurgical zinc smelter in Lommel, Belgiumhave been used to reconstruct atmospheric lead deposition rates during the20th century. Independent knowledge concerning historical pollutionevents and 137Cs fall-out profiles has allowed a criticalevaluation of the CRS, CIC and CF-CS models for the 210Pb ageinterpretation. Resulting ages for the three models suggest that, in this case,the CIC model gives the most accurate interpretation of historical pollutionevents and atmospheric lead fall-out. The 210Pbwater-sediment flux was estimated at 141–1158Bq·m–2·yr–1 for one site and62–106 Bq·m–2·yr–1 at theother site, during the last century. The large difference illustrates thatsediment focusing was important on a small spatial scale (10 m).The direction of focusing correlates with the predominant wind direction.Maximum atmospheric lead deposition rates were found to be 1.63 ± 0.59g·m–2·yr–1 around 1968 AD,which is 2 orders of magnitude larger than the Belgian average in 1980 AD, and5 orders larger than Holocene atmospheric lead deposition.  相似文献   

18.
Short core stratigraphy of total N, P, Zn, Hg and diatoms were investigated in the varved sediment of Lake Heinälampi, a small 8 m deep pond in East Finland. The sediment has recently changed from organic mud to minerogenic silt. The presence of varved sediment offers independent control for 210Pb and 137Cs dates and these are in good agreement: the sediment quality initially changed around the year 1930 due to increaed field erosion, and the inflow of mineral matter was further increased by ditching of paludified forests in 1980.Diatom analysis reveals that eutrophication has occurred before and concurrent with the sedimentary change. The causes of eutrophication and the increased levels of Zn and Hg are discussed.  相似文献   

19.
The Portil lagoon is a natural freshwater reservoir located at the southwest of Spain, near the coast. In its surroundings an important tourist complex has been developed since the earlier 1970s. This has resulted in increased loads of nutrients, specially during summer months. In order to evaluate the impact from humans on the lagoon caused by anthropogenic activities, we have determined vertical profiles of excess 210Pb and 137Cs in a sediment core taken from its bottom. Vertical profile of excess 210Pb seems to indicate that the sediment core was affected by large-scale mixing processes. Nevertheless this possibility was ruled out based on the shape of the 137Cs vertical distribution after modelling the 137Cs profile considering large-scale mixing. The chronology developed from 210Pb and 137Cs has allowed us to calculate the temporal evolution of the mass sedimentation rate during the last century. This mass sedimentation rate increased in 1973: from 0.08(2) g cm-2 a-1 in the period 1900-1973 to 0.17(5) g cm-2 a-1 in the period 1973-1995. This increase could be related to land-movements in the drainage area and to permitted sewage inputs into the lagoon, both with its origin in the growing/running of the surrounding tourist complex.  相似文献   

20.
A sedimentary record of human disturbance from Lake Miragoane,Haiti   总被引：1，自引：0，他引：1  
Lake Miragoane, Haiti is one of the largest, natural freshwater lakes in the Caribbean (A=7.06 km2, zmax=41.0 m, conductivity = 350 S cm–1). Lake waters are dominated by calcium and bicarbonate ions. The lake was thermally stratified, and oxygen profiles were clinograde during summer visits in 1983 and 1985. A 72-cm mud-water interface core was taken near the center of the lake and dated with 210Pb. The local 210Pb fallout rate is low (0.09 pCi cm–2 yr–1), about 20% of the global average. Bulk sedimentation rates ranged from 0.008 to 0.030 g cm–2 yr–1 during the past 130 years (0–8 cm depth). Sediment geochemistry and pollen have been analyzed in the topmost 58 cm of the section. Tentative ages were assigned to the core by extrapolation of 210Pb dates. According to this preliminary chronology, the bottom part of the core (58–30 cm) records pre-Columbian sedimentation (1000–500 B.P.) and contains pollen evidence of intact, dry and mesic forest. Pre-Columbian deposits are rich in organic matter (x = 30%) and relatively poor in carbonates (x = 15% as CO2). The top 30 cm of the core preserve the record since European contact (500 B.P. to present). Pollen data reveal two episodes of deforestation following European arrival. Consequent soil erosion is documented by a decrease in organic matter content (x = 15%) and an increase in carbonates (x = 27% as CO2). Surficial sediments reflect the widespread deforestation and soil loss that characterize the watershed today.  相似文献   

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