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1.
Abstract— Concentrations of the trace elements Mg, Al, Ca, Ti, V, Fe, Sr, Y, Zr, Ba and Ce were determined by ion microprobe mass spectrometry in 60 individual silicon carbide (SiC) grains (in addition, Nb and Nd were determined in 20 of them), from separate KJH (size range 3.4–5.9 μm) of the Murchison carbonaceous meteorite, whose C-, N- and Si-isotopic compositions have been measured before (Hoppe et al., 1994) and provide evidence that these grains are of stellar origin. The selected SiC grains represent all previously recognized subgroups: mainstream (20 < 12C/13C < 120; 200 < 14N/15N; Si isotopes on slope 1.34 line), grains A (12C/13C < 3.5), grains B (3.5 < 12C/13C < 10), grains X (15N excesses, large 28Si excesses) and grains Y (150 < 12C/13C < 260; Si isotopes on slope 0.35 line). Data on these grains are compared with measurements on fine-grained SiC fractions. Trace-element patterns reflect both the condensation behavior of individual elements and the source composition of the stellar atmospheres. A detailed discussion of the condensation of trace elements in SiC from C-rich stellar atmospheres is given in a companion paper by Lodders and Fegley (1995). Elements such as Mg, Al, Ca, Fe and Sr are depleted because their compounds are more volatile than SiC. Elements whose compounds are believed to be more refractory than SiC can also be depleted due to condensation and removal prior to SiC condensation. Among the refractory elements, however, the heavy elements from Y to Ce (and Nd) are systematically enriched relative to Ti and V, indicating enrichments by up to a factor of 14 of the s-process elements relative to elements lighter than Fe. Such enrichments are expected if N-type carbon stars (thermally pulsing AGB stars) are the main source of circumstellar SiC grains. Large grains are less enriched than small grains, possibly because they are from different AGB stars. The trace-element patterns of subgroups such as groups A and B and grains X can at least qualitatively be understood if grains A and B come from J-type carbon stars (known to be lacking in s-process enhancements shown by N-type carbon stars) or carbon stars that had not experienced much dredge-up of He-shell material and if grains X come from supernovae. However, a remaining puzzle is how stars become carbon stars without much accompanying dredge-up of s-process elements.  相似文献   

2.
Abstract— Carbon stars are an important source of presolar TiC, SiC, and graphite grains found in meteorites. The elemental abundances in the stellar sources of the SiC grains are inferred by using condensation calculations. These elemental abundances, together with C isotopic compositions, are used to identify possible groups of carbon stars that may have contributed SiC grains to the presolar dust cloud. The most likely parent stars of meteoritic SiC mainstream grains are N-type carbon stars and evolved subgiant CH stars. Both have s-process element abundances higher than solar and 10 < 12C/13C < 100 ratios. The J stars and giant CH stars, with solar and greater than solar abundances of s-process elements, respectively, are good candidate parents for the ‘A’ and ‘B’ SiC grains with low 12C/13C ratios. A special subgroup of CH giant stars with very large 12C/13C ratios could have parented the ‘Y’ SiC grains with 12C/13C ratios > 100. The carbon star population (e.g., N, R, J, CH groups) needed to provide the observed SiC grains is compared to the current population of carbon stars. This comparison suggests that low-metallicity CH stars may have been more abundant in the past (>4.5 Ga ago) than at present. This suggestion is also supported by condensation-chemistry modeling of the trace element patterns in the SiC grains that shows that subsolar Fe abundances may be required in the stellar sources for many SiC grains. The results of this study suggest that presolar SiC grains in meteorites can provide information about carbon stars during galactic evolution.  相似文献   

3.
In this paper the results of an experimental investigation of the spectra of submicrometersized silicon carbide grains are presented. The grains manufactured from two types of commercial -SiC were prepared according to the Jena IR spectroscopy program for particulates of cosmic importance. From the spectral records mass absorption coefficients have been derived. These data have been used to make a comparison of the laboratory spectra with the well-known 11.5 m emission band observed in the spectra of carbon stars, which is probably due to a transition in circumstellar SiC grains. For this aim, a simple model of an optically thin circumstellar envelope containing SiC grains has been calculated. The theoretical profile of the 11.5 m band derived by means of this model and based on the experimental mass absorption coefficients of SiC grains shows a striking similarity with the observed profile in the spectrum of the carbon star Y CVn. The total amount of SiC dust in the envelope of this star has been estimated at about 1024 g.  相似文献   

4.
Abstract— We have investigated the 7.5–13.5 μm spectra of 30 definite or candidate carbon stars. We discuss the discrepancies between properties of SiC grains found in meteorites and the spectral properties of dust emitting in red giant winds, where most of the meteoritic grains are believed to have formed. We have investigated the nature of carbon star SiC and its relationship to meteoritic SiC dust, by using a X2-minimisation routine to fit the observed SiC features with laboratory optical constants that have been published for a variety of SiC samples. All but one of the observed astronomical SiC features are best fitted by α-SiC grains. All but one of the sources with 8–13 μm colour temperatures >1200 K (corresponding to mass-loss rates at the bottom end of the range) are best fitted by α-SiC in pure emission; whereas, all but one of the sources with 8–13 μm colour temperatures <1200 K (corresponding to higher mass-loss rates) are best fitted using self-absorbed α-SiC emission. The four sources whose SiC features are in net absorption (and which have the lowest 8–13 μm colour temperatures and, therefore, presumably the highest mass-loss rates) are also well fitted by self-absorbed α-SiC emission but with higher optical depths. Given that β-SiC is the form most commonly found in meteorites, we have searched for evidence of β-SiC in the circumstellar shells of all these stars. However, our observations provide no unequivocal evidence for the presence of β-SiC around these stars. Other discrepancies between meteoritic SiC grains and astronomical spectra are discussed. The self-absorption that we find in the observed SiC emission features has not previously been taken into account in radiative transfer modeling and so the amount of SiC present in the outflows may have been underestimated in the past.  相似文献   

5.
The influence of temperature changes in circumstellar silicate-like envelopes upon the polarization effects is investigated. It is shown that under the assumption that ΔT g>50° and conductivity of silicate grains is indirectly proportional toT g this mechanism can be responsible for the observed dependence of intensity vs polarization in some late-type stars, e.g. V CVn. The same effects can be produced by dirty ices and graphite grains. It is suggested that irradiation by electrons and/or protons can affect the circumstellar envelopes in a similar way, especially those of early-type stars, and irradiation by neutrons can exert an influence on the envelopes of supernovae.  相似文献   

6.
We studied 14 presolar SiC mainstream grains for C‐, Si‐, and S‐isotopic compositions and S elemental abundances. Ten grains have low levels of S contamination and CI chondrite‐normalized S/Si ratios between 2 × 10?5 and 2 × 10?4. All grains have S‐isotopic compositions compatible within 2σ of solar values. Their mean S isotope composition deviates from solar by at most a few percent, and is consistent with values observed for the carbon star IRC+10216, believed to be a representative source star of the grains, and the interstellar medium. The isotopic data are also consistent with stellar model predictions of low‐mass asymptotic giant branch (AGB) stars. In a δ33S versus δ34S plot the data fit along a line with a slope of 1.8 ± 0.7, suggesting imprints from galactic chemical evolution. The observed S abundances are lower than expected from equilibrium condensation of CaS in solid solution with SiC under pressure and temperature conditions inferred from the abundances of more refractory elements in SiC. Calcium to S abundance ratios are generally above unity, contrary to expectations for stoichiometric CaS solution in the grains, possibly due to condensation of CaC2 into SiC. We observed a correlation between Mg and S abundances suggesting solid solution of MgS in SiC. The low abundances of S in mainstream grains support the view that the significantly higher abundances of excess 32S found in some Type AB SiC grains are the result of in situ decay of radioactive 32Si from born‐again AGB stars that condensed into AB grains.  相似文献   

7.
We have investigated the chemistry of phosphorus-bearing compounds in the circumstellar envelopes of both oxygen-rich and carbon-rich evolved stars. In accordance with thermodynamic calculations of photospheric chemistry, we have assumed that the dominant forms of phosphorus in the inner circumstellar envelope (CSE) are PS and HCP in each case. In the C-rich case, we can reproduce the observed CP abundance reasonably well if it is the photodaughter of HCP. In the O-rich case we find, for the same amount of P available in PS, that large abundances of atomic P are available for reaction but that a low abundance of PO can be produced. We have not extensively explored the effect of additional neutral processes since our results are partly compromised by the fact that neither HCP nor PS is detected in the three CSEs where searches have been made; our models predict column densities in excess of the published upper limits. Sensitive searches for these molecules at higher frequencies are required before their presence in circumstellar envelopes can definitely be ruled out. Dust condensation may incorporate all the available P into refractory grains and so we suggest that searches for P-bearing molecules may have the greatest opportunity for success in more evolved objects, such as protoplanetary nebulae, where P has been released from grains through the action of strong shock waves.  相似文献   

8.
We present broad-band photometry in the optical, near-infrared and submillimetre, and mid-infrared spectrophotometry of a selection of carbon stars with optically thin envelopes. Most of the observations were carried out simultaneously.   Beside the emission feature at 11.3 μ m due to silicon carbide grains in the circumstellar environment, many of our mid-infrared spectra show an emission feature at 8.6 μ m. All the observed spectral energy distributions exhibit a very large far-infrared flux excess. Both these features are indeed common to many carbon stars surrounded by optically thin envelopes.   We have modelled the observed spectral energy distributions by means of a full radiative transfer treatment, paying particular attention to the features quoted above. The peak at 8.6 μ m is usually ascribed to the presence of hydrogenated amorphous carbon grains. We find also that the feature at 8.6 μ m might be reproduced by assuming that the stars have a circumstellar environment formed of both carbon- and oxygen-rich dust grains, although this is in contrast with what one should expect in a carbon-rich environment. The far-infrared flux excess is usually explained by the presence of a cool detached dust shell. Following this hypothesis, our models suggest a time-scale for the modulation of the mass-loss rate of the order of some 103 yr.  相似文献   

9.
Within the framework of classical nucleation theory we have shown that Mg2SiO4 grains (radii of nearly 0.1 μm) which are likely candidates as condensation products in circumstellar shells around late-type stars must condense at about 750 K to remain amorphous. If the condensation temperature is about 1000 K the newly formed grains must be rather small to rest in the amorphous state during cooling. Submicron sized MgSiO3grains are entire stable against crystallization for Tcond ≤ 1000 K.  相似文献   

10.
Abstract– We have analyzed eleven presolar SiC grains from the Murchison meteorite using time‐of‐flight secondary ion mass spectrometry. The Si isotopic compositions of the grains indicate that they are probably of an AGB star origin. The average abundances of Mg, Fe, Ca, Al, Ti, and V are strongly influenced by their condensation behavior into SiC in circumstellar environments. Depth profiles of Li, B, Mg, Al, K, Ca, Ti, V, Cr, and Fe in the SiC grains show that trace elements are not always homogenously distributed. In approximately half of the SiC grains studied here, the trace element distributions can be explained by condensation processes around the grains’ parent stars. These grains appear to have experienced only minimal processing before their arrival in the presolar molecular cloud, possibly due to short residence times in the interstellar medium. The remaining SiC grains contained elevated abundances of several elements within their outer 200 nm, which is attributed to the implantation of energetic ions accelerated by shockwaves in the interstellar medium. These grains may have spent a longer period of time in this region, hence increasing the probability of them passing through a shockfront. Distinct groups of presolar SiC grains whose residence times in the interstellar medium differ are consistent with previous findings based on noble gas studies, although some grains may also have been shielded from secondary alteration by protective outer mantles.  相似文献   

11.
We have investigated the optical properties of the carbon dust grains in the envelopes around carbon-rich asymptotic giant branch stars, paying close attention to the infrared observations of the stars and the laboratory-measured optical data of the candidate dust grain materials. We have compared the radiative transfer model results with the observed spectral energy distributions of the stars including IRAS Point Source Catalog and IRAS Low Resolution Spectrograph data. We have deduced an opacity function of amorphous carbon dust grains from model fitting with infrared carbon stars. From the opacity function, we have derived the optical constants of the AMC grains. The optical constants satisfy the Kramers–Kronig relation and produce the opacity function that fits the observations of infrared carbon stars better than previous works in the wide wavelength range 1–1000 μm. We have used simple mixtures of the AMC and silicon carbide grains for modelling. We have compared the contributions that AMC and SiC grains make to the opacity for the cases of simple mixtures of them and spherical core–mantle type grains consisting of a SiC core and an AMC mantle .  相似文献   

12.
We have measured polarization of the 1.1 mm and 0.8 mm continuum emission for 3 pre-T Tauri stars and 2 T Tauri stars. Positive detections were made for NGC 1333 IRAS 4 and IRAS 16293-2422, while L1551 IRS 5 and HL Tau were only marginally detected. For GG Tau we measured a 2 upper limit of 3%. The polarization is interpreted in terms of thermal emission by magnetically aligned dust grains in circumstellar disks or envelopes. We have found a definite geometrical relation between the polarization and other circumstellar structure.  相似文献   

13.
Summary Cosmic dust grains play an important role for the thermal, dynamical, and chemical structure of the interstellar medium. This is especially true for the star formation process and the late stages of stellar evolution. Dust grains determine the spectral appearance of protostars, very young stellar objects with disk-like structures as well as of evolved stars with circumstellar envelopes.In this review, we will demonstrate that solid particles in interstellar space are both agent and subject of galactic evolution. We will especially discuss the different dust populations in circumstellar envelopes, the diffuse interstellar medium, and the molecular clouds with strong emphasis on the evolutionary aspects and the metamorphosis of these populations.  相似文献   

14.
We discuss our JHKLM photometry for nine carbon Mira stars, eighteen carbon semiregular variables, and two oxygen Mira stars. For fourteen carbon stars, we present and analyze their infrared light and color curves. For all of the observed objects, we have estimated the optical depths of the circumstellar dust envelopes, the angular diameters of the stars, and their temperatures.  相似文献   

15.
The presence of heated circumstellar dust around WC type Wolf-Rayet stars requires the episodic or persistent condensation of carbon grains in their stellar winds. In order to survive in the stars' strong ultraviolet radiation fields, the grains must be located at least 100AU from the stellar surfaces. The densities in isotropic winds at such large distances are too low to allow grain growth and anisotropies such as clumps, disks or wind-collision wakes in colliding-wind binary systems are required to provide grain nurseries. Observational evidence for such features in grain-forming W-R stars is examined.  相似文献   

16.
The circumstellar envelopes of carbon-rich AGB stars show a chemical complexity that is exemplified by the prototypical object IRC +10216, in which about 60 different molecules have been detected to date. Most of these species are carbon chains of the type C n H, C n H2, C n N, HC n N. We present the detection of new species (CH2CHCN, CH2CN, H2CS, CH3CCH and C3O) achieved thanks to the systematic observation of the full 3 mm window with the IRAM 30m telescope plus some ARO 12m observations. All these species, known to exist in the interstellar medium, are detected for the first time in a circumstellar envelope around an AGB star. These five molecules are most likely formed in the outer expanding envelope rather than in the stellar photosphere. A pure gas phase chemical model of the circumstellar envelope is reasonably successful in explaining the derived abundances, and additionally allows to elucidate the chemical formation routes and to predict the spatial distribution of the detected species.  相似文献   

17.
We report on the isotopic, chemical, and structural properties of four O‐rich presolar grains identified in situ in the Adelaide ungrouped C2, LaPaZ Icefield (LAP) 031117 CO3.0, and Dominion Range (DOM) 08006 CO3.0 chondrites. All four grains have oxygen‐isotopic compositions consistent with origins in the circumstellar envelopes (CSE) of low‐mass O‐rich stars evolved along the red‐giant and asymptotic‐giant branch (RGB, AGB, respectively) of stellar evolution. Transmission electron microscope (TEM) analyses, enabled by focused‐ion‐beam scanning electron microscope extraction, show that the grain from Adelaide is a single‐crystal Mg‐Al spinel, and comparison with equilibrium thermodynamic predictions constrains its condensation to 1500 K assuming a total pressure ≤10?3 atm in its host CSE. In comparison, TEM analysis of two grains identified in the LAP 031117 chondrite exhibits different microstructures. Grain LAP‐81 is composed of olivine containing a Ca‐rich and a Ca‐poor domain, both of which show distinct orientations, suggesting changing thermodynamic conditions in the host CSE that cannot be precisely constrained. LAP‐104 contains a polycrystalline assemblage of ferromagnesian silicates similar to previous reports of nanocrystalline presolar Fe‐rich silicates that formed under nonequilibrium conditions. Lastly, TEM shows that the grain extracted from DOM 08006 is a polycrystalline assemblage of Cr‐bearing spinel. The grains occur in different orientations, likely reflecting mechanical assembly in their host CSE. The O‐isotopic and Cr‐rich compositions appear to point toward nonequilibrium condensation. The spinel is surrounded by an isotopically solar pyroxene lacking long‐range atomic order and could have served as a nucleation site for its condensation in the interstellar medium or the inner solar protoplanetary disk.  相似文献   

18.
Abstract— We have determined the recoil losses from silicon carbide (SiC) grain‐size fractions of spallation Ne produced by irradiation with 1.6 GeV protons. During the irradiation, the SiC grains were dispersed in paraffin wax in order to avoid reimplantation into neighboring grains. Analysis for spallogenic 21Ne of grain‐size separates in the size range 0.3 to 6 μm and comparison with the 22Na activity of the SiC + paraffin mixture indicates an effective recoil range of 2–3 μm with no apparent effect from acid treatments, which are routinely used in the isolation of meteoritic SiC grains. Our results indicate that the majority of presolar SiC grains in primitive meteorites, which are micrometer‐sized, will have lost essentially all spallogenic Ne produced by cosmic‐ray interaction in the interstellar medium. This argues against the validity of previously published presolar ages of Murchison SiC (～10 to ～130 Ma, increasing with grain size; Lewis et al., 1994), where recoil losses had been based on calculated recoil energies. It is argued that the observed variations in meteoritic SiC grain‐size fractions of 21Ne/22Ne ratios are more likely due to the effects of nucleosynthesis in the He‐burning shell of the parent AGB stars which imposes new boundary conditions on nuclear parameters and stellar models. It is suggested that spallation‐Xe produced on the abundant Ba and REE in presolar SiC, rather than spallogenic Ne, may be a promising approach to the presolar age problem. There is a hint in the currently available Xe data (Lewis et al., 1994) that the large (>1 μm) grains may be younger than the smaller (<1 μm) grains. The retention of spallogenic 21Ne produced by the bombardment of SiC grains of different grain sizes with 1.6 GeV protons, avoiding reimplantation into neighboring grains by dispersing the SiC grains in paraffin wax, has been derived from a comparison of mass spectrometrically determined 21Ne, retained in the grains, with the 22Na activity of the grains‐plus‐paraffin mixture. Compared to estimates of retention used in previous attempts to determine presolar ages for SiC (Tang and Anders, 1988b; Lewis et al., 1990, 1994), the results indicate significantly lower values. They do, however, agree with retention as expected from previous measurements of recoil ranges in similar systems (Nyquist et al., 1973; Steinberg and Winsberg, 1974). The prime reason for the discrepancy must lie in the energy of the recoiling nuclei entering in the calculation of retention by Tang and Anders (1988b), which is based on considerations by Ray and Völk (1983). Based on the results, it appears questionable that spallation contributes significantly to the observed variations of 21Ne/22Ne ratios among various SiC grain‐size separates (Lewis et al., 1994). We rather suggest that the variations, just as it has been observed for Kr and Ba already (Lewis et al., 1994; Prombo et al., 1993), have a nucleosynthetic origin. Confirmation needs input of improved nuclear data and stellar models into new network calculations of the nucleosynthesis in AGB stars of elements in the Ne region. Finally we argue that, to determine presolar system irradiation effects, spallation Xe is more favorable than is Ne, primarily because of smaller recoil losses for Xe. Although preliminary estimates hint at the possibility that the larger (>1 μm) grains are younger than the smaller (<1 μm) ones, the major uncertainty for a quantitative evaluation lies in the exact composition of the Xe‐N component thought to originate from the envelope of the SiC grains' parent stars.  相似文献   

19.
We present new mid-IR images of AGB and post-AGB circumstellar envelopes (CSEs) obtained with the 10–20 μm imaging camera CAMIRAS mounted at the TIRGO infrared telescope (Gornergrat, Switzerland). Diffraction limited images of the sources are obtained, and extended emission for the brightest sources is detected for several arcseconds. Simple radiative transfer modelling is necessary to fit the observed data and derive the physical and chemical state of the envelope. This kind of analysis is an important test for dust formation theories, because it gives indications of dust properties along their condensation path through the envelope. This revised version was published online in September 2006 with corrections to the Cover Date.  相似文献   

20.
We report the development of a novel method to nondestructively identify presolar silicon carbide (SiC) grains with high initial 26Al/27Al ratios (>0.01) and extreme 13C‐enrichments (12C/13C ≤ 10) by backscattered electron‐energy dispersive X‐ray (EDX) and micro‐Raman analyses. Our survey of a large number of presolar SiC demonstrates that (1) ~80% of core‐collapse supernova and putative nova SiC can be identified by quantitative EDX and Raman analyses with >70% confidence; (2) ~90% of presolar SiC are predominantly 3C‐SiC, as indicated by their Raman transverse optical (TO) peak position and width; (3) presolar 3C‐SiC with 12C/13C ≤ 10 show lower Raman TO phonon frequencies compared to mainstream 3C‐SiC. The downward shifted phonon frequencies of the 13C‐enriched SiC with concomitant peak broadening are a natural consequence of isotope substitution. 13C‐enriched SiC can therefore be identified by micro‐Raman analysis; (4) larger shifts in the Raman TO peak position and width indicate deviations from the ideal 3C structure, including rare polytypes. Coordinated transmission electron microscopy analysis of one X and one mainstream SiC grain found them to be of 6H and 15R polytypes, respectively; (5) our correlated Raman and NanoSIMS study of mainstream SiC shows that high nitrogen content is a dominant factor in causing mainstream SiC Raman peak broadening without significant peak shifts; and (6) we found that the SiC condensation conditions in different stellar sites are astonishingly similar, except for X grains, which often condensed more rapidly and at higher atmospheric densities and temperatures, resulting in a higher fraction of grains with much downward shifted and broadened Raman TO peaks.  相似文献   

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