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1.
The results of measurements of the total content of carbon monoxide in an atmospheric column over Moscow and the Zvenigorod Scientific Station (ZSS) are given for the period 1993–2005. The simultaneous measurements of the regional background contents of carbon monoxide over a rural area (ZSS) and over Moscow made it possible to isolate an urban portion of the CO content. The total content of CO over the city varies significantly from day to day from values close to the background value to values that are 2.5–3 times greater than the background value. The number of days with such a CO content is 5% of the total number of measurement days. Such a CO content is most often observed during the cold seasons. During the warm seasons, in most of the cases, slight excesses of the CO background value are observed in the urban atmosphere. Variations in the CO content are determined mainly by wind-velocity variations and temperature inversions. In 2002, the high CO concentrations were due to forest and peatbog fires. On some days, over the ZSS, the concentrations of CO were high as never before. Over this period (12 years), the CO content in the surface air layer over the city did not increase.  相似文献   

2.
Carbon monoxide (CO) total columns over European Russia (ER) and western Siberia (WS) have been analyzed using MOPITT (V5, TIR/NIR, L3) IR-radiometer data obtained in 2000–2014. High CO contents are revealed over large urban and industrial agglomerations and over regions of oil-and-gas production. A stable local CO maximum is observed over the Moscow agglomeration. Statistical characteristics of CO total columns observed in the atmosphere over ER and WS in 2000–2014 are presented. An analysis of long-term changes in CO content reveals nonlinear changes in the CO total column over northern Eurasia in 2000–2014. Results of a comparative analysis of annual variations in atmospheric CO contents over ER and WS are given. Based on Fourier analysis, empirical models of annual variations in total CO contents over ER and WS are proposed. Relations between regional CO contents and fire characteristics and between spatial CO distributions and features of large-scale atmospheric dynamics under conditions of weather and climate anomalies in the summers of 2010 in ER and 2012 in WS are analyzed. Data on total CO contents measured with a MOPITT satellite radiometer and a ground-based spectrometer operating at the Zvenigorod Scientific Station of the Obukhov Institute of Atmospheric Physics are compared.  相似文献   

3.
The climatic trends and basic features of seasonal variations in and anomalies of the concentration of methane in the atmospheric surface layer are considered on the basis of the current notion of the processes that form the global field of methane in the Earth’s atmosphere. Measurement data on the surface concentration of methane, which were obtained in Moscow and at a number of observation stations in Europe and Siberia in the fall-winter period of the first decade of the 21st century, have been analyzed. It is shown that, in the anomalously warm winter months of 2006/2007, the concentration of methane in the atmosphere over Moscow was higher than in the previous and following years. The excess concentration of methane amounted to 10% in March 2007, which is higher than the mean range of seasonal variations in the monthly mean concentration of surface methane. A comparison between the data obtained in Moscow and the data obtained at three stations of the NOAA global monitoring network and at three Russian Hydrometeorological Research Center stations shows the high spatial variability of the methane concentration in the atmosphere over northern Eurasia. The complex and multifactor processes that determine the content of methane in the atmospheric surface layer result in noticeable spatial and interannual deviations from the mean seasonal cycle of its concentration, which can manifest themselves on both regional and global scales. It is possible that the resumed increase in the content of methane in the Earth’s atmosphere recorded in 2007 (after its relative stabilization in the early 2000s) at the global monitoring network was also caused, to some extent, by the anomalously warm winter of 2006–2007 in northern Europe and western Siberia.  相似文献   

4.
Contributions of climatically significant natural and anthropogenic emission sources in northern Eurasia to seasonal carbon monoxide (CO) variations observed at the Zotino Tall Tower Observatory (ZOTTO) in Central Siberia in 2007–2011 have quantitatively been estimated using the GEOS-Chem chemical transport model. It is shown that the formation of a stable continental pollution plume from sources in Western Europe, European Russia and southern Siberia during winter plays an important role in the regional balance of surface CO and allows one to explain 55–80% of the amplitude of the CO annual cycle observed at the ZOTTO station (~70–90 ppbv). During the warm period, the effect of the anthropogenic factor is weakly pronounced, and the background concentration of CO is regulated, first and foremost, by the oxidation of biogenic volatile organic compounds and fire activity in the region.  相似文献   

5.
A model based on that of Kishi et al. (2001) has been extended to 15 compartments including silicon and carbon cycles. This model was applied to Station A7 off Hokkaido, Japan, in the Northwestern Pacific. The model successfully simulated the observations of: 1. a spring bloom of diatoms; 2. large seasonal variations of nitrate and silicate concentrations in the surface water; and 3. large inter-annual variations in chlorophyll-a. It also reproduced the observed features of the seasonal variations of carbon dioxide partial pressure (pCO2)—a peak in pCO2 in winter resulting from deep winter convection, a rapid decrease in pCO2 as a result of the spring bloom, and an almost constant pCO2 from summer through fall (when the effect of increasing temperature cancels the effect of biological production). A comparison of cases with and without silicate limitation shows that including silicate limitation in the model results in: 1. decreased production by diatoms during summer; and 2. a transition in the dominant phytoplankton species, from diatoms to other species that do not take up silicate. Both of these phenomena are observed at Station A7, and our results support the hypothesis that they are caused by silicate limitation of diatom growth. This revised version was published online in July 2006 with corrections to the Cover Date.  相似文献   

6.
Sea surface height anomalies observed by satellites in 1992–2010 are combined with monthly climatologies of temperature and salinity to estimate circulation in the southern Bering Sea. The estimated surface and deep currents are consistent with independent velocity observations by surface drifters and Argo floats parked at 1,000?m. Analysis reveals 1–3-Sv interannual transport variations of the major currents with typical intra-annual variability of 3–7?Sv. On the seasonal scale, the Alaskan Stream transport is well correlated with the Kamchatka (0.81), Near Strait (0.53) and the Bering Slope (0.37) currents. Lagged correlations reveal a gradual increase of the time the lags between the transports of the Alaskan Stream, the Bering Slope Current and the Kamchatka Current, supporting the concept that the Bering Sea basin is ventilated by the waters carried by the Alaskan Stream south of the Aleutian Arc and by the flow through the Near Strait. Correlations of the Bering Sea currents with the Bering Strait transport are dominated by the seasonal cycle. On the interannual time scale, significant negative correlations are diagnosed between the Near Strait transport and the Bering Slope and Alaskan Stream currents. Substantial correlations are also diagnosed between the eddy kinetic energy and Pacific Decadal Oscillation.  相似文献   

7.
The results of the carbon monoxide total content measurements over Moscow and Zvenigorod for 2005–2008 are compared with the same data sets for Moscow 1986–2005 and Beijing, 1992–2007. Two identical medium resolution diffraction spectrometers (resolution 0.2 cm?1) with solar tracking system were used. The CO total content measured simultaneously over the city and over Zvenigorod Scientific Station (ZSS) of the Obukhov Institute of Atmospheric Physics, Russian Academy of Sciences (60 km west from Moscow). This method allows to isolate an urban part of CO content. The acoustic locator SODAR LATAN-3 measurements permitted us to study the influence of the carbon monoxide ventilation conditions upon level of pollution. Correlation coefficients between the urban part of CO content and average wind speed for cold and warm seasons were obtained. The data sets analysis showed a preeminent effect of the wind within boundary layer (up to 300 m) over the CO ventilation. The urban part of the CO content hasn’t increased in spite of more than quintuple increase of the motor-vehicles number in Moscow. An increase of the rural CO total column for the 1970–1985 has transformed into its virtually stable amount in between of 1986 to 2000, changed then to a decrease for 2001–2008. We noted the 2008 as “the year of the CO total column minimum” over the past decade. The effect of urban CO sources influence on the CO total column in rural area is small, i.e. on a level of 3% of the total number of measurements. The number of extremal daily values for Moscow is estimated as 5%, and 20% for Beijing.  相似文献   

8.
连云港近海海域水质的季节和年际变化   总被引：2，自引：0，他引：2  
根据1992～2005年连云港近海海域水质监测资料,对该海域水质的季节变化和年际变化进行研究.结果表明,近海水质有明显的季节变化特征,其中盐度从春、夏季到秋季缓慢降低,冬季升高;溶解无机氮(DIN)与盐度恰恰相反,夏秋季最高且监测的超标率高.溶解氧季节性非常明显,依次为冬季>春季>秋季>夏季.总体上春冬季水质好于夏秋季.年际变化显示,1992～2005年pH和盐度均有降低趋势,尤其是2003年以后降幅更加明显;DO和COD年际变化相对平稳但季节变化幅度较大;2000年12月后油类浓度明显降低且年际变化平稳;近几年DIN有明显增加趋势,无机氮已成为该海域主要污染物.  相似文献   

9.
Based on observations of carbon monoxide (CO) concentrations at three Mosekomonitoring stations, we have analyzed the weekly cycle of CO in the surface air of Moscow in 2004–2007. At all stations the minimum long-term mean daily CO values are observed on Sunday. The weekly cycle of CO more clearly manifests itself at the center of Moscow and becomes less clear closer to the outskirts. We have analyzed the reproducibility of the weekly cycle of CO from one year to another, the seasonal dependence, its specific features at different times of day, and the changes in the diurnal cycle of CO during the week. The factors responsible for specific features of the evolution of surface CO concentrations at different observation stations have been analyzed. The empirical probability density functions of CO concentrations on weekdays and at week- end are presented. The regularity of the occurrence of the weekend effect in CO has been investigated and the possible reasons for breaks in weekly cycles have been analyzed. The Kruskal-Wallis test was used to study the statistical significance of intraweek differences in surface CO contents.  相似文献   

10.
Statistical characteristics of variations in surface-layer concentrations of methane, non-methane and aromatic hydrocarbons, carbon dioxide, and formaldehyde are compared with the characteristics of variations in the concentration of carbon monoxide in the air basin of Moscow. Differences in the annual cycle of concentrations of methane, carbon dioxide, non-methane hydrocarbons, and carbon monoxide are determined. It is found that the maximum concentration of carbon monoxide at most sites with an elevated surface-air pollution level and over the city as a whole tends to occur in the summer season. The seasonal variability of the diurnal mean cycle of methane, carbon dioxide, and non-methane and aromatic hydrocarbons is analyzed.  相似文献   

11.
Spatial variations in the distribution and fluxes of dissolved oxygen and sulfide in bottom sediments of Omega and Sevastopol bays have been studied. The results of analysis reveal that the distribution of dissolved oxygen and sulfide in pore water depends mostly on seasonal variations in the oxygen concentration in bottom water, grain size, the organic carbon content in bottom sediments, and, additionally for Sevastopol Bay, the iron content. The oxygen flux at the bottom of Sevastopol Bay is 20 times larger in winter–spring compared to that of Omega Bay. Anaerobic conditions in Sevastopol Bay sediments are observed much closer to the surface, with their subsequent development in bottom water.  相似文献   

12.
We study the seasonal and interannual variations of the field of sea-surface temperature (SST) in the Southwest Atlantic on the basis of the analysis of three data arrays, namely, the Levitus-Boyer-1994 hydrological array, the WOD-98 actual database, and the data of satellite measurements of SST. We perform the comparative analysis of the amplitude-phase characteristics of the annual course of the SST field and discuss the distinctive features of its seasonal and interannual variations. It is shown that the results obtained by using different data arrays are in good agreement. The values of the coefficient of linear correlation are equal to 0.7–0.9. It is discovered that the maximum seasonal variations of SST are observed in the zone of confluence of the Falkland and Brasil Currents in the vicinities of the South Subtropical and Antarctic Polar fronts. The minimum seasonal variations are recorded in the Antarctic region and in the Weddell Sea. The satellite data demonstrate that the level of interannual variability is high in the zones of climatic fronts. __________ Translated from Morskoi Gidrofizicheskii Zhurnal, No. 5, pp. 62–76, September–October, 2006.  相似文献   

13.
The principal statistical regularities typical of the behaviors of the CH4, CO, and CO2 concentrations in the atmospheric surface layer over the continental Russian territory are revealed from the measurements performed in 1997–2004 along the Trans-Siberian Railroad from Moscow to Khabarovsk with a mobile laboratory. The data obtained under the conditions of the atmosphere free of anthropogenic pollutants are analyzed. For near-background conditions, the typical continental methane, carbon monoxide, and carbon dioxide concentrations and characteristic features of their large-scale spatial distributions and daily variations, including those caused by surface inversions, are determined. Variations in the concentrations of these trace gases over industrial regions are analyzed. Our results are compared to the data obtained at background stations of the world network of atmospheric monitoring and to the data of a numerical simulation.  相似文献   

14.
Phytoplankton fluorescence, temperature and salinity were measured from December through February using in situ instruments deployed at two locations in the southern Ross Sea, Antarctica during the austral summers of three consecutive years (2003–2004, 2004–2005, and 2005–2006) to assess the short-term, seasonal and interannual variations in phytoplankton biomass and oceanographic conditions. The seasonal climatologies of physical forcing variables were also determined from satellite measurements, and the data from the two sites compared to the 2000–2009 mean. In situ fluorometers were deployed at three depths at 77°S, 172.7°E and 77.5°S, 180°. Significant differences between the two sites were consistently observed, confirming the anticipated high level of spatial and temporal heterogeneity. Chlorophyll fluorescence was maximal in late December, and generally decreased rapidly to modest levels in January and February. However, during 1 year (2003–2004) a secondary bloom was found, with summer maxima being similar to those observed during spring. Fluorescence displayed a strong diel cycle, with strong quenching during periods of maximum irradiance. The magnitude of this reduction was large (the minimum average fluorescence was 25% of the daily mean) and decreased with depth. Fluorescence varied interannually, with the absolute levels and temporal patterns being different among years. The two sites had different temperature/salinity properties as measured at 24 m, and both variables changed with time. During 2004–2005 we were able to continuously measure the photosynthetic quantum efficiency of PSII (Fv/Fm) at 11 m, which revealed a minimum in December, and an increase in January, whereas the absolute fluorescence (Fo) decreased simultaneously. We suggest that this reflected a mixing event, whereby available irradiance increased, allowing a short period of growth in a more favorable optical environment. While substantial variations from the mean physical forcing were observed, the linkage of these physical variations with fluorescence was not always clear. Short-term (over 24-h) changes in fluorescence occurred, and were likely related to advective events. Wind events altered fluorescence in the surface layer, and these redistributed phytoplankton in the surface. The variability in chlorophyll fluorescence and physical forcing over a variety of scales in the Ross Sea provides insights into temporal–spatial coupling of phytoplankton.  相似文献   

15.
Specimens of the hydrothermal mussel Bathymodiolus azoricus collected in Menez Gwen hydrothermal vent field (NE Atlantic) during 2002–2003 were examined for feeding patterns variations through three seasons. The fatty acid profile and lipid classes of the mussels were studied, together with the MODIS/AQUA-derived near-surface chlorophyll a to test the hypothesis that surface productivity might be related to the feeding patterns of this species. The lipid levels showed pronounced seasonal fluctuations with the highest values occurring in January and August. Seasonal variations in lipid classes and fatty acid composition of neutral and polar lipids in the mussels are presented. Differences in the fatty acid profile of lipid classes in different seasons suggest that the higher energy requirements in summer and winter were supplied by bacterial biomarkers ω7 MUFA (monounsaturated fatty acids), whereas ω6 PUFA (polyunsaturated fatty acids) and NMI (non-methylene-interrupted) fatty acids predominated during the spring. The MODIS/AQUA data show marked seasonal variability and an anomalous peak during January of 2003, although this cannot be directly linked to lipid composition variation.  相似文献   

16.
分别于2006年8月,12月和2007年4月,10月采集胶州湾及周边海域大气和海水样品,对氧化亚氮(N2O)和甲烷(CH4)浓度进行了测定,并设置1个连续站进行24 h连续观测.结果表明:大气中N2O春、夏、秋、冬的平均浓度(体积分数)分别为(3.17±0.03)×10-7,(3.24±0.15)×10-7,(3.19±0.02)×10-7和(3.08±0.25)×10-7;大气中CH4春、夏、秋、冬的平均浓度(体积分数)分别为(1.89±0.04)×10-6,(1.79±0.04)×10-6,(2.09±0.21)×10-6和(2.01±0.09)×10-6.胶州湾表、底层海水中N2O和CH4的浓度和饱和度表现出明显的季节变化,其中N2O浓度和饱和度冬季最高,春、秋季次之,夏季最低;CH4浓度和饱和度夏季最高,冬季最低.利用Liss and Merlivat(1986)公式和Wanninkhof(1992)公式估算出胶州湾海域N2O的年平均海-气交换通量分别为(11.16±14.15)和(22.42±27.56)μmol m-2·d-1;CH4分别为(7.75±6.19)和(17.76±14.84)μmol m-2·d-1.胶州湾大部分海域表层海水中N2O和CH4呈过饱和状态,是大气中N2O和CH4的净源.  相似文献   

17.
根据“908”ST04区块调查的夏、冬、春、秋季四个航次和“908”补充调查的8月航次资料对长江口及邻近海区表层水体溶解氧及其饱和度进行了探讨.研究表明东海北部表层水体在夏季和春季以浮游植物光合作用为主要控制过程,特别是7、8月份长江口外、杭州湾外及浙江近海存在大范围的强光合作用区;秋季以有机质氧化分解过程为主,表层溶...  相似文献   

18.
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19.
We investigated sources of inter-annual variability in larval supply to crab and sea urchin populations at Bodega Head and Point Reyes in northern California. During the spring and summer upwelling seasons of the years 1992 through 1997 we monitored the weekly settlement rates of nine species of crabs and two species of sea urchins. As observed in previous studies, daily values of alongshore windstress, temperature and salinity provided evidence for the poleward flow of relatively warm, low salinity water from south of Point Reyes, an apparent retention zone, during upwelling relaxation events. In years dominated by these events (1992, 1993, 1995 and 1996) we observed that alongshore windstress, temperature and salinity were coherent and temperature was significantly correlated with cancrid crab settlement. During these years the magnitude of cancrid crab settlement and the fraction of cancrid crabs relative to other crab species settling were high. Over four years of concurrent sampling there was consistently greater cancrid crab settlement at the Point Reyes site, within the retention zone, than at Bodega Head. Settlement of non-cancrid crabs (porcellanids, grapsids, pagurids and majids) was not as closely linked to intra-annual patterns of upwelling and relaxation, possibly due to the shorter seasonal availability of larvae allowing for the influence of fewer relaxation events. Settlement of this group among years was positively correlated with environmental indicators of strong seasonal upwelling; high salinity, Bakun upwelling index and low temperature. Sea urchin settlement events were observed in June and July of 1992, 1994 and 1997 during warming periods when salinity and temperature were increasing and alongshore windstress was low. Across the six years of the study, we found that cancrid crab larvae had a more even seasonal availability than larvae of non-cancrid species, which settled in greatest numbers during the early portion of the upwelling season. Sea urchins settled in greatest numbers during the later part of the upwelling season. Together these patterns demonstrate the taxon-specific way that inter-annual variability in larval supply is forced by the coincidence of larval availability with favorable physical transport mechanisms.  相似文献   

20.
The results of measurements of the CO content in the atmospheric thickness by the method of solar molecular-absorption spectroscopy are presented. Over 87 months of observations, the annual mean CO content decreased by ～19% at a mean rate of changes equal to ?(0.14 ± 0.02) atm cm per year. Maxima and minima of seasonal variations most often fall on February and September, respectively. The mean overall amplitude of changes in the CO content during the annual cycle is about 50% of the mean value. The Fourier analysis revealed variations in the CO composition with periods from 3 to 84 months. A simple statistical model satisfactorily describes time changes in the CO content in the atmospheric thickness. The results of measurements of the CO content in the atmospheric thickness are compared with the data of CO measurements in samples of surface air at stations of the Global Atmospheric Watch.  相似文献   

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