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1.
Eddy fluxes of CO2 estimated using a sonic anemometer and a closed-path analyser were, on average, 16% lower than those obtained with the same anemometer and an adjacent open-path CO2 analyser. Covariances between vertical windspeed and CO2 density from the closed-path analyser were calculated using data points for CO2 that were delayed relative to anemometer data by the time required for a parcel of air to travel from the tube inlet to the CO2 sensor. Air flow in the intake tube was laminar. Densities of CO2 that had been corrected for spurious fluctuations arising from fluctuations in temperature and humidity were used in the flux calculations. Corrections for the cross-sensitivity of CO2 analysers to water vapour were also incorporated. Spectral analysis of the corrected CO2 signal from the closed-path analyser showed that damping of fluctuations in the sampling tube at frequencies f > 0.1 Hz caused the apparent loss in flux. The measured losses can be predicted accurately using theory that describes the damping of oscillations in a sampling tube. High-frequency response of the closed-path system can be improved substantially by ensuring turbulent flow in the tube, using a combination of high volumetric flow rate and small tube diameter. The analysis of attenuation of turbulent fluctuations in flow through tubes is applicable to the measurement of fluxes of other minor atmospheric constituents using the eddy covariance method.  相似文献   

2.
We have examined the potential of using a closed-path sensor to accurately measure eddy fluxes of CO2. Five inlet tubeflow configurations were employed in the experimental setup. The fluxes of CO2 were compared against those measured with an open-path sensor. Sampling air through an intake tube causes a loss of flux, due to the attenuation of CO2 density fluctuations. Adjustments need to be made to correct for this loss and to account for density effects due to the simultaneous transfer of heat and water vapor. Theory quantifying these effects is discussed.The raw CO2 flux measured with the closed-path sensor was smaller than that measured with the open-path sensor by about 15% (on average) for the turbulent tubeflow configurations with a short (3 m) intake tube, by 31% for turbulent tubeflow with a longer (6 m) intake tube and by 24% for laminar tubeflow. The difference was, in part, caused by tube attenuation of the CO2 density fluctuations and inadequate sensor time response. The elimination of the flux adjustment for the simultaneous transfer of sensible heat (i.e., the attenuation of ambient temperature fluctuations in the intake tube) generally accounted for the rest of this difference.The raw flux measured with the closed-path sensor was corrected for frequency response and density effects. Except in the case of laminar tubeflow, the corrected closed-path flux agreed consistently with the corrected open-path flux within a few percent (<5%). These results suggest that closed-path sensors, with appropriate corrections, can be used to measure CO2 flux accurately. Recommendations are included on selecting an optimum flow configuration to minimize the effect of sampling air through a tube.Published as Paper No. 9938, Journal Series, Nebraska Agricultural Research Division.  相似文献   

3.
In the context of CO2 surface exchange estimation, an analysis combining the basic principles of diffusion and scalar conservation shows that the mixing ratio is the appropriate variable both for defining the (eddy covariance) turbulent flux and also for expressing the relationship between the turbulent flux and surface exchange in boundary-layer budget equations. Other scalar intensity variables sometimes chosen, both the CO2 density and molar fraction, are susceptible to the influence of surface exchange of heat and water vapour. The application of a hypsometric analysis to the boundary-layer “control volume” below the tower measurement height reveals flaws in previously applied approaches: (a) incompressibility cannot be assumed to simplify mass conservation (the budget in terms of CO2 density); (b) compressibility alone makes the analysis of mass conservation vulnerable to uncertainties associated with resultant non-zero vertical velocities too small to measure or model over real terrain; and (c) the WPL (Webb et al. (1980) Quart J Roy Meteorol Soc 106:85–100) “zero dry air flux” assumption is invalidated except at the surface boundary. Nevertheless, the definition and removal of the WPL terms do not hinge upon this last assumption, and so the turbulent CO2 flux can be accurately determined by eddy covariance using gas analysers of either open- or closed-path design. An appendix discusses the necessary assumptions and appropriate interpretations for deriving the WPL terms.  相似文献   

4.
An eddy covariance system using a closed-path CO2analyser was constructed for long-term CO2flux measurements above a forest, and its total frequency response was valuated experimentally. The amplitude and phase responses of the system wereexamined through a preliminary test, in which a prescribed pattern of CO2fluctuation was input to the system. The result showed that the amplitude of the output from the system was attenuated as frequency increased, with a half-power frequency of 0.3 Hz. The phase was delayed by the air sampling through a long tube, but the delay in phase decreased asfrequency increased. We then presented a new technique for the correction of flux loss due to the inadequate system response for the eddy covariance measurements of CO2 flux. Using the present system and the correction technique, diurnal variations in CO2 flux were measured over a temperate deciduous forest on three days in 1997. The results were compared with the CO2fluxes measured with a fast response open-path gas analyser. The CO2fluxes from the closed-path system agreed with those from the open-path system after the Webb, Pearman and Leuning correction was made for the latter. In the present test over a forest, the contribution of the frequency-response correction to the CO2fluxes was small and its averaged percentage was only 3%in the daytime. However, the percentage would likely increase, if the system were applied to a shorter vegetation site where high frequency components are more important. The comparison confirmed that we can obtain correct measurements of CO2flux using the present closed-path system and the correction technique.  相似文献   

5.
Comparison was made of the flux measurements of a closed-path CO2/H2O analyzer and an open-path H2O analyzer above a clover field and the forest floor of a Douglas-fir stand. The attenuation of the gas concentration fluctuations caused by the sampling tube of the closed-path analyzer resulted in underestimation of the H20 flux above both surfaces. The degree of underestimation above the clover field depended on wind speed, but was smaller than that calculated from the transfer function for laminar flow in a circular tube and the scalar cospectrum in the neutral and unstable surface layer. Above the forest floor CO2 fluctuations led those of H2O by 0.7s. The implications of this are discussed regarding the determination of the time delay caused by the sampling tube of the closedpath analyzer. The day-time CO2 efflux from the forest floor, averaged over three days, was 0.043 mg/(m2s).  相似文献   

6.
We present an approach for assessing the impact of systematic biases in measured energy fluxes on CO2 flux estimates obtained from open-path eddy-covariance systems. In our analysis, we present equations to analyse the propagation of errors through the Webb, Pearman, and Leuning (WPL) algorithm [Quart. J. Roy. Meteorol. Soc. 106, 85–100, 1980] that is widely used to account for density fluctuations on CO2 flux measurements. Our results suggest that incomplete energy balance closure does not necessarily lead to an underestimation of CO2 fluxes despite the existence of surface energy imbalance; either an overestimation or underestimation of CO2 fluxes is possible depending on local atmospheric conditions and measurement errors in the sensible heat, latent heat, and CO2 fluxes. We use open-path eddy-covariance fluxes measured over a black spruce forest in interior Alaska to explore several energy imbalance scenarios and their consequences for CO2 fluxes.  相似文献   

7.
A Simple Method of Estimating Scalar Fluxes Over Forests   总被引：1，自引：0，他引：1  
A simple aerodynamic-variance method is proposed to fill gaps in continuous CO2 flux measurements in rainy conditions, when open-path analysers do not function. The method requires turbulent conditions (friction velocity greater than 0.1 ms–1), and uses measurements of mean wind speed, and standard deviations of temperature and CO2 concentration fluctuations to complement, and at times replace, eddy-covariance measurements of friction velocity, sensible heat flux and CO2 flux. Friction velocity is estimated from the mean wind speed with a flux-gradient relationship modified for the roughness sublayer. Since normalised standard deviations do not follow Monin-Obukhov similarity theory in the roughness sublayer, a simple classification scheme according to the scalar turbulence scale was used. This scheme is shown to produce sensible heat and CO2 flux estimates that are well correlated with the measured values.  相似文献   

8.
Energy and CO2 fluxes are commonly measured above plant canopies using an eddy covariance system that consists of a three-dimensional sonic anemometer and an H2O/CO2 infrared gas analyzer. By assuming that the dry air is conserved and inducing mean vertical velocity, Webb et al. (Quart. J. Roy. Meteorol. Soc. 106, 85-100, 1980) obtained two equations to account for density effects due to heat and water vapour transfer on H2O/CO2 fluxes. In this paper, directly starting with physical consideration of air-parcel expansion/compression, we derive two alternative equations to correct for these effects that do not require the assumption that dry air is conserved and the use of the mean vertical velocity. We then applied these equations to eddy flux observations from a black spruce forest in interior Alaska during the summer of 2002. In this ecosystem, the equations developed here led to increased estimates of CO2 uptake by the vegetation during the day (up to about 20%), and decreased estimates of CO2 respiration by the ecosystem during the night (approximately 4%) as compared with estimates obtained using the Webb et al. approach.  相似文献   

9.
We investigated the ‘local’ and ‘global’ similarity of vertical turbulent transfer of heat, water vapour, and CO2 within an urban surface layer. The results were derived from field measurements in a residential area of Tokyo, Japan during midday on fair-weather days in July 2001. In this study, correlation coefficients and quadrant analysis were used for the evaluation of ‘global’ similarity and wavelet analysis was employed for investigating ‘local’ similarity. The correlation coefficients indicated that the transfer efficiencies of water vapour and CO2 were generally smaller than that of heat. Using wavelet analysis, we found that heat is always efficiently transferred by thermal and organized motions. In contrast, water vapour and CO2, which are passive quantities, were not transferred as efficiently as heat. The quadrant analyses showed that the heat transfer by ejection exceeded that by sweep, and the ratios of ejection to sweep for water vapour and CO2 transfer were less than that for heat. This indicated that heat is more efficiently transferred by upward motions and supported the findings from wavelet analysis. The differences of turbulent transfer between heat and both CO2 and water vapour were probably caused both by the active role of temperature and the heterogeneity in the source distribution of scalars  相似文献   

10.
Spectra of CO2 and water vapour fluctuations from measurements made in the marine atmospheric surface layer have been analyzed. A normalization of spectra based on Monin–Obukhov similarity theory, originally developed for wind speed and temperature, has been successfully extended also to CO2 and humidity spectra. The normalized CO2 spectra were observed to have somewhat larger contributions from low frequencies compared to humidity spectra during unstable stratification. However, overall, the CO2 and humidity spectra showed good agreement as did the cospectra of vertical velocity with water vapour and CO2 respectively. During stable stratification the spectra and cospectra displayed a well-defined spectral gap separating the mesoscale and small-scale turbulent fluctuations. Two-dimensional turbulence was suggested as a possible source for the mesoscale fluctuations, which in combination with wave activity in the vertical wind is likely to explain the increase in the cospectral energy for the corresponding frequency range. Prior to the analysis the turbulence time series of the density measurements were converted to time series of mixing ratios relative to dry air. Some differences were observed when the spectra based on the original density measurements were compared to the spectra based on the mixing ratio time series. It is thus recommended to always convert the density time series to mixing ratio before performing spectral analysis.  相似文献   

11.
When density fluctuations of scalars such as CO2 are measured with open-path gas analyzers, the measured vertical turbulent flux must be adjusted to take into account fluctuations induced by ‘external effects’ such as temperature and water vapour. These adjustments are needed to separate the effects of surface fluxes responsible for ‘natural’ fluctuations in CO2 concentration from these external effects. Analogous to vertical fluxes, simplified expressions for separating the ‘external effects’ from higher-order scalar density turbulence statistics are derived. The level of complexity in terms of input to these expressions are analogous to that of the Webb–Pearman–Leuning (WPL), and are shown to be consistent with the conservation of dry air. It is demonstrated that both higher-order turbulent moments such as the scalar variances, the mixed velocity-scalar covariances, and the two-scalar covariance require significant adjustments due to ‘external effects’. The impact of these adjustments on the turbulent CO2 spectra, probability density function, and dimensionless similarity functions derived from flux-variance relationships are also discussed.  相似文献   

12.
Components of the surface energy balance of a mature boreal jack pine forest and a jack pine clearcut were analysed to determine the causes of the imbalance that is commonly observed in micrometeorological measurements. At the clearcut site (HJP02), a significant portion of the imbalance was caused by: (i) the overestimation of net radiation (R n ) due to the inclusion of the tower in the field of view of the downward facing radiometers, and (ii) the underestimation of the latent heat flux (λE) due to the damping of high frequency fluctuations in the water vapour mixing ratio by the sample tube of the closed-path infrared gas analyzer. Loss of low-frequency covariance induced by insufficient averaging time as well as systematic advection of fluxes away from the eddy-covariance (EC) tower were discounted as significant issues. Spatial and temporal distributions of the total surface-layer heat flux (T), i.e. the sum of sensible heat flux (H) and λE, were well behaved and differences between the relative magnitudes of the turbulent fluxes for several investigated energy balance closure (C) classes were observed. Therefore, it can be assumed that micrometeorological processes that affected all turbulent fluxes similarly did not cause the variation in C. Turbulent fluxes measured at the clearcut site should not be forced to close the energy balance. However, at the mature forest site (OJP), loss of low-frequency covariance contributed significantly to the systematic imbalance when a 30-min averaging time was used, but the application of averaging times that were long enough to capture all of the low-frequency covariance was inadequate to resolve all of the high-frequency covariance. Although we found qualitative similarity between T and the net ecosystem exchange (NEE) of carbon dioxide (CO2), forcing T to closure while retaining the Bowen ratio and applying the same factor to CO2 fluxes (F C ) cannot be generally recommended since it remains uncertain to what extent long wavelength contributions affect the relationship between T, F C and C.  相似文献   

13.
An open path,fast response infrared absorption gas analyzer for H2O and CO2   总被引：1，自引：0，他引：1  
An open path infrared absorption based instrument for fast response measurements of H2O and CO2 fluctuations is described. This instrument performed reliably in several field experiments in both terrestrial and marine environments, on both fixed (tower) and mobile (boat, plane) flux platforms. Noise levels for H2O and CO2 concentrations were less than 10 mg/m3 and 300 g/m3, respectively for frequencies between 0.005 and 10 Hz. Drifts in instrument output, associated with changes in instrument temperature, are compensated for electronically.  相似文献   

14.
Evapotranspiration is a source of water vapour to the atmosphere, and as a crucial indicator of landscape behaviour its accurate measurement has widespread implications. Here we investigate errors that are prevalent and systematic in the closed-path eddy-covariance measurement of latent heat flux: the attenuation of fluxes through dampened cospectral power at high frequencies. This process is especially pronounced during periods of high relative humidity through the adsorption and desorption of water vapour along the tube walls. These effects are additionally amplified during lower air temperature conditions. Here, we quantify the underestimation of evapotranspiration by a closed-path system by comparing its flux estimate to simultaneous and adjacent measurements from an open-path sensor. We apply models relating flux loss to relative humidity itself, to the lag time of the cross-correlation peak between the water vapour and vertical wind velocity signals, and to models of cospectral attenuation relative to the cospectral power of simultaneous sensible heat-flux measurements. We find that including the role of temperature in modifying the attenuation–humidity relationship is essential for unbiased flux correction, and that physically based cospectral attenuation methods are effective characterizers of closed-path instrument signal loss relative to the unattenuated flux value.  相似文献   

15.
We present turbulence spectra and cospectra derived from long-term eddy-covariancemeasurements (nearly 40,000 hourly data over three to four years) and the transferfunctions of closed-path infrared gas analyzers over two mixed hardwood forests inthe mid-western U.S.A. The measurement heights ranged from 1.3 to 2.1 times themean tree height, and peak vegetation area index (VAI) was 3.5 to 4.7; the topographyat both sites deviates from ideal flat terrain. The analysis follows the approach ofKaimal et al. (Quart. J. Roy. Meteorol. Soc. 98, 563–589, 1972) whose results were based upon 15 hours of measurements atthree heights in the Kansas experiment over flatter and smoother terrain. Both thespectral and cospectral constants and stability functions for normalizing and collapsingspectra and cospectra in the inertial subrange were found to be different from those ofKaimal et al. In unstable conditions, we found that an appropriate stabilityfunction for the non-dimensional dissipation of turbulent kinetic energy is of the form () = (1 - b-)-1/4 - c-, where representsthe non-dimensional stability parameter. In stable conditions, a non-linear functionGxy() = 1 + bxyc xy (cxy < 1) was found to benecessary to collapse cospectra in the inertial subrange. The empirical cospectralmodels of Kaimal et al. were modified to fit the somewhat more (neutraland unstable) or less (stable) sharply peaked scalar cospectra observed over forestsusing the appropriate cospectral constants and non-linear stability functions. Theempirical coefficients in the stability functions and in the cospectral models varywith measurement height and seasonal changes in VAI. The seasonal differencesare generally larger at the Morgan Monroe State Forest site (greater peak VAI) andcloser to the canopy.The characteristics of transfer functions of the closed-path infrared gas analysersthrough long-tubes for CO2 and water vapour fluxes were studied empirically. This was done by fitting the ratio between normalized cospectra of CO2 or watervapour fluxes and those of sensible heat to the transfer function of a first-order sensor.The characteristic time constant for CO2 is much smaller than that for water vapour. The time constant for water vapour increases greatly with aging tubes. Three methods were used to estimate the flux attenuations and corrections; from June through August, the attenuations of CO2 fluxes are about 3–4% during the daytime and 6–10% at night on average. For the daytime latent heat flux (QE), the attenuations are foundto vary from less than 10% for newer tubes to over 20% for aged tubes. Correctionsto QE led to increases in the ratio (QH + QE)/(Q* - QG) by about 0.05 to0.19 (QH is sensible heat flux, Q* is net radiation and QG is soil heat flux),and thus are expected to have an important impact on the assessment of energy balanceclosure.  相似文献   

16.
Atmospheric CO2 removal is currently receiving serious consideration as a supplement or even alternative to emissions reduction. However the possible consequences of such a strategy for the climate system, and particularly for regional changes to the hydrological cycle, are not well understood. Two idealised general circulation model experiments are described, where CO2 concentrations are steadily increased, then decreased along the same path. Global mean precipitation continues to increase for several decades after CO2 begins to decrease. The mean tropical circulation shows associated changes due to the constraint on the global circulation imposed by precipitation and water vapour. The patterns of precipitation and circulation change also exhibit asymmetries with regard to changes in both CO2 and global mean temperature, but while the lag in global precipitation can be ascribed to different levels of CO2 at the same temperature state, the regional changes cannot. Instead, ocean memory and heat transfer are important here. In particular the equatorial East Pacific continues to warm relative to the West Pacific during CO2 ramp-down, producing an anomalously large equatorial Pacific sea surface temperature gradient and associated rainfall anomalies. The mechanism is likely to be a lag in response to atmospheric forcing between mixed-layer water in the east Pacific and the sub-thermocline water below, due to transport through the ocean circulation. The implication of this study is that a CO2 pathway of increasing then decreasing atmospheric CO2 concentrations may lead us to climate states during CO2 decrease that have not been experienced during the increase.  相似文献   

17.
Abstract

Fluxes of temperature, water vapour, O3, SO2 and CO2 were estimated from the measurement of their variances, taken over a wetland region in northern Ontario (Canada) during the summer of 1990 and over a deciduous forest when it was fully leafed during the summer of 1988 and when it was leafless during the winter of 1990. A set of flux‐variance relations was employed, including empirical forms of universal functions that could be adjusted with some constants. Results from the present study show that these constants needed to be adjusted with site‐specific data in order to achieve a closer agreement between estimated and observed fluxes. Best estimates were obtained for the fluxes of temperature and water vapour and it was found that the flux estimates of O3, SO2 and CO2 correlated better with water vapour than with temperature. For these trace gases the flux‐variance method yielded estimates of dry deposition velocities that were either comparable with or larger than those obtained from a resistance analogue model. Both methods yielded values that overestimated the observed dry deposition velocities. The employment of the flux‐variance method in an operational network would require the use of fast‐response sensors and a practical method for reducing the noise level of the measured variances.  相似文献   

18.
Vertical turbulent fluxes of water vapour, carbon dioxide, and sensible heat were measured from 16 August to the 28 September 2006 near the city centre of Münster in north-west Germany. In comparison to results of measurements above homogeneous ecosystem sites, the CO2 fluxes above the urban investigation area showed more peaks and higher variances during the course of a day, probably caused by traffic and other varying, anthropogenic sources. The main goal of this study is the introduction and establishment of a new gap filling procedure using radial basis function (RBF) neural networks, which is also applicable under complex environmental conditions. We applied adapted RBF neural networks within a combined modular expert system of neural networks as an innovative approach to fill data gaps in micrometeorological flux time series. We found that RBF networks are superior to multi-layer perceptron (MLP) neural networks in the reproduction of the highly variable turbulent fluxes. In addition, we enhanced the methodology in the field of quality assessment for eddy covariance data. An RBF neural network mapping system was used to identify conditions of a turbulence regime that allows reliable quantification of turbulent fluxes through finding an acceptable minimum of the friction velocity. For the data analysed in this study, the minimum acceptable friction velocity was found to be 0.15 m s−1. The obtained CO2 fluxes, measured on a tower at 65 m a.g.l., reached average values of 12 μmol m−2 s−1 and fell to nighttime minimum values of 3 μmol m −2 s−1. Mean daily CO2 emissions of 21 g CO2 m−2d −1 were obtained during our 6-week experiment. Hence, the city centre of Münster appeared to be a significant source of CO2. The half-hourly average values of water vapour fluxes ranged between 0.062 and 0.989 mmol m−2 s−1and showed lower variances than the simultaneously measured fluxes of CO2.  相似文献   

19.
A large-eddy simulation model developed at the National Center for Atmospheric Research (NCAR) is extended to simulate the transport and diffusion of C18OO, H218O and 13CO2 in the atmospheric boundary layer (ABL). The simulation results show that the 18O compositions of leaf water and the ABL CO2 are moderately sensitive to wind speed. The variations in the 18O composition of water vapour are an order of magnitude greater than those in the 13C and 18O compositions of CO2 both at turbulent eddy scales and across the capping inversion. In a fully-developed convective ABL, these isotopic compositions are well mixed as with other conserved atmospheric quantities. The Keeling intercepts determined with the simulated high-frequency turbulence time series do not give a reliable estimate of the 18O composition of the surface water vapour flux and may be a reasonable approximation to the 13C and 18O compositions of the surface CO2 flux in the late afternoon only after a deep convective ABL has developed. We suggest that our isotopic large-eddy simulation (ISOLES) model should be a useful tool for testing and formulating research hypotheses on land–air isotopic exchanges.  相似文献   

20.
A land-surface model (LSM) is coupled with a large-eddy simulation (LES) model to investigate the vegetation-atmosphere exchange of heat, water vapour, and carbon dioxide (CO2) in heterogeneous landscapes. The dissimilarity of scalar transport in the lower convective boundary layer is quantified in several ways: eddy diffusivity, spatial structure of the scalar fields, and spatial and temporal variations in the surface fluxes of these scalars. The results show that eddy diffusivities differ among the three scalars, by up to 10–12%, in the surface layer; the difference is partly attributed to the influence of top-down diffusion. The turbulence-organized structures of CO2 bear more resemblance to those of water vapour than those of the potential temperature. The surface fluxes when coupled with the flow aloft show large spatial variations even with perfectly homogeneous surface conditions and constant solar radiation forcing across the horizontal simulation domain. In general, the surface sensible heat flux shows the greatest spatial and temporal variations, and the CO2 flux the least. Furthermore, our results show that the one-dimensional land-surface model scheme underestimates the surface heat flux by 3–8% and overestimates the water vapour and CO2 fluxes by 2–8% and 1–9%, respectively, as compared to the flux simulated with the coupled LES-LSM.  相似文献   

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