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1.
The continental shelf and slope of southern Central Chile have been subject to a number of international as well as Chilean research campaigns over the last 30 years. This work summarizes the geologic setting of the southern Central Chilean Continental shelf (33°S–43°S) using recently published geophysical, seismological, sedimentological and bio-geochemical data. Additionally, unpublished data such as reflection seismic profiles, swath bathymetry and observations on biota that allow further insights into the evolution of this continental platform are integrated. The outcome is an overview of the current knowledge about the geology of the southern Central Chilean shelf and upper slope. We observe both patches of reduced as well as high recent sedimentation on the shelf and upper slope, due to local redistribution of fluvial input, mainly governed by bottom currents and submarine canyons and highly productive upwelling zones. Shelf basins show highly variable thickness of Oligocene-Quaternary sedimentary units that are dissected by the marine continuations of upper plate faults known from land. Seismic velocity studies indicate that a paleo-accretionary complex that is sandwiched between the present, relatively small active accretionary prism and the continental crust forms the bulk of the continental margin of southern Central Chile.  相似文献   

2.
The Pampas plain (30°–41°S) has historically been considered as a sector that evolved independently from the adjacent Andean ranges. Nevertheless, the study of the Pampas showed that it is reasonable to expect an important influence from the Andes into the extraandean area. The Pampas plain can be divided into two sectors: the northern portion, adjacent to the Pampean Ranges, has been studied by Davila (2005, 2007, 2010). The southern sector (34°–41°S) is the objective of the present work. The study of this area allowed to characterize two separate foreland basins: the Southern Pampa basin and the Northern Patagonian basin. The infill is composed of Late Miocene and Pliocene units, interpreted as distal synorogenic sequences associated with the late Cenozoic Andean uplift at this latitudinal range. These foreland basins have been defined based on facies changes, distinct depositional styles, along with the analysis of sedimentary and isopach maps. The basins geometries are proposed following De Celles and Gilles (1996) taking into account the infill geometry, distribution and grain size. In both cases, these depocenters are located remarkably far away from the Andean tectonics loads. Therefore they cannot be explained with short-wave subsidence patterns. Elastic models explain the tectonic subsidence in the proximal depocenters but fail to replicate the complete distal basins. These characteristics show that dynamic subsidence is controlling the subsidence in the Southern Pampas and Northern Patagonian basins.  相似文献   

3.
The aim of this study is the synthesis of CuSeO3·2H2O (chalcomenite analog), ZnSeO3·2H2O, and ZnSeO3·H2O and the investigation of their solubility in water. CuSeO3·2H2O has been synthesized from solutions of Cu nitrate and Na selenite, while Zn selenites were synthesized from solutions of Zn nitrate and Na selenite. The samples obtained have been examined with X-ray diffraction and infrared and Raman spectroscopy. The solubility has been determined using the isothermal saturation method in ampoules at 25°C. The solubility has been calculated using the Geochemist’s Workbench (GMB 9.0) software package. Solubility products have been calculated for CuSeO3·2H2O (10–10.63), ZnSeO3·2H2O (10–8.35), and ZnSeO3·H2O (10–7.96). The database used comprises thermodynamic characteristics of 46 elements, 47 base particles, 48 redox pairs, 551 particles in solution, and 624 solid phases. The Eh–pH diagrams of the Zn–Se–H2O and Cu–Se–H2O systems were plotted for the average contents of these elements in underground water in oxidation zones of sulfide deposits.  相似文献   

4.
The paper presents data on the major-component, trace-element, and mineralogical composition of plutonic rocks, and the composition of their minerals, from the Sierra Leone region in the crest zone of the Mid-Atlantic Ridge between the Strakhov and Bogdanov fracture zones. According to their relations with seafloor structures, the rock associations are subdivided into those of rift valleys and nontransform offset zones. The troctolites and olivine gabbro composing the rift association were produced early in the fractionation course of oceanic tholeiite melt in unstationary and relatively small magmatic chambers. Most rocks beneath the nontransform offset zones crystallized during the long-lasting fractionation of the melt in large chambers hosted in serpentinized peridotites. This part consists of various cumulates, ranging from troctolites to gabbroids. Where deep tectonic detachments entered partly consolidated portions of the chambers, the melt interacted with the wall rocks. Fluid that was generated via the dehydration of serpentine and concentrated hydrophile elements, locally modified the composition of the melt and resulted in amphibole-bearing rocks. Under stress, the intercumulus melts were squeezed into tectonically weakened zones, mixed there, and also interacted with the wall rocks. These mix melts produced (with the participation of fractional crystallization) mineralized Fe-Ti gabbroids. Residual portions of the melts generated most of the diorites and plagiogranites. The high-Na diorites likely crystallized from acid melts that were derived via the partial melting of older gabbroids where aqueous fluids circulated; these fluids were generated by the deserpenitization of the host rocks in tectonized zones cutting through the chambers.  相似文献   

5.
At the southern part of the East Pacific Rise (EPR), between 6°S and 30°S a survey on volcanic and hydrothermal activity was performed and samples were obtained by means of TV-controlled grab.This paper deals with altered and mineralized basalt sampled between 7°S and 23°S from five sites in a hydrothermal field.These basalts of tholeitic composition are vitreous to holocrystaline. They have suffered pervasive alteration during which rock-forming minerals (pyroxene, plagioclase) have been replaced by kaolinite, chlorite and smectite. As a consequence, strong depletion of Ca, Cr, Ni, Mg, Sr and Al took place, accompanied by an enrichment of Fe, Cu, Co, Mo, Zn, and Pb. The ore mineral assemblage is rather uniform and consists of pyrite, marcasite, wurtzite, sphalerite, chalcopyrite, covellite and goethite.The igneous and hydrothermal activities can be subdivided into different stages: lithification, high-temperature alteration (<400 C), medium to low temperature alteration and two substages of ore formation (250°C – 150°C and <150°C, respectively).This active present-day ore deposition is interpreted in terms of a peripheral zone of a volcanic-hosted ore mineralisation. It may be compared with fossil ophiolite-hosted massive sulfides that formed throughout the Alpine (e.g. Arabia, Cyprus) as well as Caledonian orogeny (e.g. Scandinavia).
Zusammenfassung Im Südteil des East Pacific Rise (EPR) zwischen 6°S und 30°S wurde eine Übersichtsbeprobung in einem Gebiet starker vulkanischer und hydrothermaler Aktivität durchgeführt. Diese Studie befaßt sich mit alterierten und mineralisierten Basalten die in einem Hyrothermalfeld, an 5 Positionen zwischen 7°S und 23°S genommen wurden. Die tholeiitischen Basalte sind z.T. hyalin. z.T. holokristallin strukturiert. Im Verlauf der sehr starken Alteration wurden die Minerale Pyroxen und Plagioklas in Kaolinit, Chlorit und Smektit ungewandelt. Dieser Verdrängungsprozeß wurde von einer starken Abreicherung an Ca, Cr, Ni, Mg, Sr, Al und einer Anreicherung an Fe, Cu, Co, Mo, Zn und Pb begleitet. Die Vererzung zeigt eine einfache Mineralvergesellschaftung mit Pyrit, Markasit, Wurtzit, Sphalerit, Chalkopyrit, Covellin und Geothit.Die magmatische und hydrothermale Aktivität läßt sich in verschiedene Stadien untergliedern: Basaltentstehung, Hochtemperturalteration (< 400°), Mittelbis Tieftemperaturalteration und Vererzung mit 2 Substadien (250°C–150°C, < 150°C).Diese rezenten Vererzungen lassen sich interpretieren als die Randzone einer vulkanitgebundenen Erzmineralisation. Sie läßt sich mit fossilen Vertretern ophiolit-gebundener massiver Sulfiderze, wie sie im Verlauf den alpidischen (z.B. Arab.-Halbinsel, Zypern) und kaledonischen Orogenese (z.B. Norwegen) entstanden sind, vergleichen.
Résumé Une étude des activités volcanique et hydrothermale a été effectuée dans la partie sud de l'East Pacific Rise, entre 6° et 30° de latitude sud. Des échantillons y ont été prélevés au moyen d'un engin dirigé par TV.La présente note se rapporte aux basaltes altérés et minéralisés récoltés en cinq points d'un champ hydrothermal, entre 7°S et 23°S.Ces basaltes, de composition tholéiitique sont tantôt vitreux, tantôt holocristallins. Ils ont été le siège d'une forte altération hydrothermale au cours de laquelle les minéraux de la roche (pyroxène, plagioclase) ont été remplacés par de la kaolinite, de la chlorite et de la smectite. Il en est résulté un appauvrissement marqué en Ca, Cr, Ni, Mg, Sr et Al, accompagné d'un enrichissement en Fe, Cu, Co, Mo, Zn et Pb. La minéralisation présente une association simple à pyrite, marcassite, wurtzite, sphalérite, covelline et goethite.On peut distinguer plusieurs stades d'activité magmatique et hydrothermale: formation du basalte, altération de haute température (<400°C), altération de moyenne à basse température avec deux stades de minéralisation (250-150°C; <150°C). Ces dépôts de la nature actuelle peuvent s'interpréter comme la zone périphérique d'une aire de minéralisation volcanogène. On peut les comparer à des gisements fossiles de sulfures massifs liés à des ophiolites, comme il s'en est formé au cours des orogenèses alpine (p. ex.: péninsule arabique, Chypre) et calédonienne (p. ex.: Norvège).
»East Pacific Rise (EPR)« 6° 30° . , 7° 23° . , . , , . , Cr, Ni, Mg, Sr, Al Fe, u, , Mo, Zn Pb. , , , , , . : , ( 400°), (250°–150°, <150°) . , , . , , (.: , ) (.: ).
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6.
《Applied Geochemistry》1997,12(4):383-395
594 sediment samples from the Galapagos Rift System (GRS) and the crest of the East Pacific Rise (EPR) were chemically analyzed for 12 elements. Carbonate-free compositional datasets associated with each of 3 regions, the GRS, the EPR 2°N–4°S and the EPR 10°S–42°S, were separately subjected to endmember analysis. The compositions of endmember estimates were constructed for each dataset. These composition largely confirmed theidentities of endmembers that had previously been inferred from the varimax rotated loadings of a conventional factor analysis (of the correlation matrices) of the same 3 datasets.In view of the widely-reported unreliability of the correlation structure of compositional data, the confirmation by endmember analysis of the results of a factor analysis is itself quite remarkable. However, the particular advantage of endmember analysis is that the chemical compositions of extreme sources are estimated, and may readily be interpreted. The samples in the dataset can then be expressed as mixtures of these extreme sources. By contrast, the varimax rotated loadings of a factor analysis indicate only those elements that are associated together on a single factor which may or may not be an endmember, the composition of which nevertheless remains unknown.  相似文献   

7.
Patagonia, including the island of Tierra del Fuego, lies in southernmost South America at the junction of the South American, Antarctic, and Scotia tectonic plates. Historical and instrumental records have documented several local earthquakes of damaging magnitude, posing a threat to the rapidly growing population of 300,000 and the expanding industrial and service infrastructure. Short and inaccurate instrumental records of local seismic events and a diffuse epicenter distribution not clearly related to the recognized seismogenic structures have hindered an adequate evaluation of the seismic hazard for this region. To improve this situation, a paleoseismological study was carried out on two gravelly strandplains on the Atlantic coast of Patagonia. Surveying combined ground-probing radar, vertical electric sounding, and seismic refraction. Coseismic normal faults buried beneath the strandplain bodies were revealed and related to the morphology of the strandplains. The faults have probable ages between 0.9 and 6.4 kyr BP and a recurrence rate of about 1 kyr. The more likely source for these structures is the Magallanes-Fagnano fault, a continental transform fault that crosses Tierra del Fuego. The distance of more than 300 km from the buried coseismic structures to the trace of the Magallanes-Fagnano fault argues for high-magnitude earthquake activity on this fault throughout the Holocene. Urban development on soft glacial and alluvial substrates increases the hazard.  相似文献   

8.
Our newly obtained data on the geochemistry and age of plagiogranite-gabbronorite association in the oceanic core complex of the Mid-Atlantic Ridge (MAR) at 5°10′S suggest close genetic relations between these rocks in this segment of the ridge. The U/Pb zircon age of an oceanic plagiogranite (OPG) sample is 1.059 ± 0.055 Ma and is in good agreement with the zircon age of plutonic rocks in the oceanic core complex of northern MAR. A distinctive geochemical feature of the rocks is their unusually depleted 87Sr/86Sr and 143Nd/144Nd ratios, which suggest that the plutonic rocks of the gabbronorite-plagiogranite association in MAR at 5°10′S could be derived from the most strongly depleted mantle reservoir of all known to occur beneath the axial MAR zone. The COMAGMAT-5.2 numerical thermodynamic simulation of the possible crystallization links between the plagiogranite and gabbronorite from the MAR segment at 5°10′S led us to conclude that the leading role in the origin of the plagiogranite was played by a two-stage process: the partial melting of the gabbronorite and the subsequent fractionation of the newly generated melt. The regional differences between the isotopic-geochemical parameters of MAR plagiogranites can, perhaps, reflect local specifics of so-called hydrothermal anatexis, such as the geochemical features of the rocks involved in this process and the parameters of the hydrothermal process, for example, variations in the W/R ratio.  相似文献   

9.
The understanding of the mechanisms of the selenium behavior under near-surface conditions is an urgent problem of modern mineralogy and geochemistry, and is very important for solving environmental problems. The objective of this study is to synthesize analogs of ahlfeldite and cobaltomenite and to estimate their solubility in water. These analogs have been synthesized by mixing aqueous solutions of cobalt and nickel nitrates, respectively, and sodium selenite acidified with a solution of nitric acid. The obtained samples have been identified by X-ray diffraction and IR spectroscopy. The solubility has been determined by the isothermal saturation method in ampoules at 25°C, while the solubility products have been calculated using the Geochemist’s Workbench (GMB 7.0) software package. The solubility products of ahlfeldite and cobaltomenite are 10?9.20 and 10?9.44, respectively. The Eh-pH diagrams were calculated and plotted with the GMB 7.0 software package. The Eh-pH diagrams of the Ni-Se-H2O and Co-Se-H2O systems have been calculated for the average contents of these elements in underground water and their contents in acidic water of the oxidation zone of sulfide deposits. The formation of ahlfeldite and cobaltomenite under near-surface conditions is discussed.  相似文献   

10.
Arrival-times of local events recorded in northern Chile and southern Bolivia were used to determine the P velocity structure above the subducted Nazca plate. The data were recorded between June and November 1994 by the French “Lithoscope” network: 41 vertical and 14 three-component short-period seismic stations were installed along a 700 km long profile crossing the main structures of the Andean chain, from the Coastal Cordillera to the Subandean Zone. The inversion method used is a modified version of Thurber’s 3D iterative simultaneous inversion code. The results were compared with a model obtained from previous German nearby refraction seismic studies and supplemented by field geological observations.The relocated seismicity is consistent with an ∼30° dipping slab between 0 and 170 km depth. We found a variation of about 30 km of the Moho depth along the profile. The crustal thickness is about 47 km under the Coastal Cordillera, 70 km under the Western Cordillera and the western part of the Eastern Cordillera, and 60–65 km beneath the Altiplano. Close to the surface, a good agreement between the velocity model and the geological structures is observed. Generally, in the upper crust, high velocities coincide with zones where basement is present near the surface. Low velocities are well correlated with the presence of very thick sedimentary basins or volcanic material. At greater depth, the trend of the velocity model is consistent with the existence of asymmetrical west-dipping imbricated blocks, overthrusting toward the east, which explain the asymmetrical pattern of the sedimentary basins. Beneath the Western Cordillera, the active volcanic arc, a large zone of low velocity is observed and interpreted to be due to partially molten material. A clear velocity contrast appears between the western and eastern parts of the upper mantle beneath the Andes; this geometry suggests the existence of a low velocity wedge in the mantle above the slab and the presence of a thick old lithosphere in the eastern part of the Andes.  相似文献   

11.
Understanding the mechanisms of arsenic’s behavior under near-surface conditions is one of the actual problems of contemporary mineralogy and geochemistry and is important for solving environmental problems. The aim of this study is to synthesize analogs of erythrite and annabergite and to investigate their solubility in water. These phases have been synthesized by the boiling-dry of aqueous solutions of cobalt and nickel nitrates mixed with sodium hydroarsenate alkalized with NaOH. The samples obtained have been identified with electron microprobe, X-ray diffraction, and IR spectroscopy. Solubility has been determined by the isothermal saturation method in ampoules at 25°C. The solubility has been calculated using the Geochemist’s Workbench (GMB 7.0) software package. The measured solubilities of erythrite and annabergite are 10?35.76 and 10?36.43, respectively. Eh-pH diagrams were calculated and plotted using the GMB 7.0 software package. The database comprises the thermodynamic parameters of 46 elements, 47 main particles, 48 redox pairs, 552 particles in solution, 624 solid phases, and 10 gases. The Eh-pH diagrams of the Ni-As-H2O and Co-As-H2O systems were plotted for the average contents of these elements in the acidic waters in the oxidation zones of sulfide deposits. The formation of erythrite and annabergite under near-surface conditions is discussed.  相似文献   

12.
Data presented in the paper suggest significant differences between the thermodynamic conditions under which magmatic complexes were formed in MAR at 29°–34° N and 12°–18° N. The melts occurring at 29°–34° N were derived by the melting of a mantle source with a homogeneous distribution of volatile components and arrived at the surface without significant fractionation, likely, due to their rapid ascent. The MAR segments between 12° and 18° N combine contrasting geodynamic environments of magmatism, which predetermined the development of a large plume region with the widespread mixing of the melting products of geochemically distinct mantle sources. At the same time, this region is characterized by conditions favorable for the origin of localized zones of anomalous plume magmatism. These sporadic magmatic sources were spatially restricted to MAR fragments with the Hess crust, whose compositional and mechanical properties were, perhaps, favorable for the focusing and localization of plume magmatism. The plume source between 12° and 18°N beneath MAR may be geochemically heterogeneous.  相似文献   

13.
The paper presents characteristics of the Nd and Sr isotopic systems of ultrabasic rocks, gabbroids, plagiogranites, and their minerals and data on He and hydrocarbons in fluid inclusions in the same samples. The materials presented in this publication were obtained by studying samples dredged from the MAR crest zone at 5°–6° N (U/Pb zircon dating, geochemical and petrological-mineralogical studies). It was demonstrated that the variations in the isotopic composition of He entrapped in the rocks and minerals were controlled by variable degrees of mixing of juvenile He, which is typical of basaltic glass of MAR (DM source) and atmospheric He. An increase in the fraction of atmospheric He in the plutonic rocks and, to a lesser degree, in their minerals reflects the involvement of seawater or the hydrated material of the oceanic crust in the magmatic and postmagmatic processes. This conclusion finds further support in a positive correlation between the fraction of mantle He (R) and the 87Sr/86Sr ratio. The high-temperature hydration of ultrabasic rocks (amphibolization) was associated with an increase in the fraction of mantle He, while their low-temperature hydration (serpentinization) was accompanied by a drastic decrease in this fraction and a significant increase in the 87Sr/86Sr ratio. The insignificant variations in the 143Nd/144Nd (close to 0.5130) and 87Sr/86Sr (0.7035) in most of the gabbroids and plagiogranites, as well as the fraction of mantle He in these rocks, amphibolites, and their ore minerals, indicate that the melts were derived from the depleted mantle. Similar?Nd values of the gabbroids, plagiogranites, and fresh harzburgites (6.77–8.39) suggest that these rocks were genetically related to a single mantle source. The value of ?Nd = 2.62 of the serpentinized lherzolites likely reflects relations of these relatively weakly depleted mantle residues to another source. The aforementioned characteristics of the rocks generally reflect the various degrees of mixing of components of the depleted mantle with crustal components (seawater) during the metamorphic and hydrothermal processes that accompanied the formation of the oceanic crust.  相似文献   

14.
《International Geology Review》2012,54(14):1691-1719
This study investigates the formation of lower oceanic crust and geochemical variations of basalts along the Central Indian Ridge (CIR, lat. 7°45′–17°10′ S). Harzburgites, various gabbroic cumulates, medium- to fine-grained oxide gabbros, diabases, and pillow basalts were recovered by dredging from segment ends such as ridge-transform intersections (RTIs), non-transform discontinuities (NTDs), and transform offset areas. The occurrence of both harzburgites and gabbroic rocks with minor basalts at all segments ends, and leucogabbro intrusive into harzburgite at the 12°45′ S NTD indicates that oceanic crust at segment ends exposes mantle-derived harzburgites and gabbroic intrusions with a thin basaltic cover due to sparse magmatic activity. Basalts collected along the entire ridge show wide compositional variations between N (normal)- and E (enriched)-mid-ocean ridge basalt (MORB). T (transitional)-MORBs with enriched affinities are more prominent than N-MORBs. There is no tendency of enrichment towards specific directions. (La/Sm)N variations in MORB along the CIR (8°–21°S) fluctuates at a regional scale with local high positive anomalies reflecting compositional heterogeneity of the sub-CIR mantle domain.  相似文献   

15.
The paper presents newly obtained original data on the morphology, internal structure (as seen in cathodoluminescence images, CL), and composition of more than 400 zircon grains separated from gabbroids and plagiogranites (OPG) sampled at the axial zone of the Mid-Atlantic Ridge (MAR). The zircons were analyzed for REE by LA-ICP-MS and for Hf, U, Th, Y, and P by EPMA. Magmatic zircon in the gabbroids crystallized from differentiating magmatic melt in a number of episodes, as follows from systematic rimward increase in the Hf concentration, and also often from the simultaneous increase in the (U + Th) and (Y + P) concentrations. These tendencies are also discernible (although much less clearly) in zircons from the OPG. Zircon in the OPG is depleted in REE compared to the least modified zircons in the gabbro, which suggests that the OPG were derived via partial melting of gabbro in the presence of seawater-derived concentrated aqueous salt fluid. Another reason for the REE depletion might be simultaneous crystallization of zircon and apatite. The CL-dark sectors, which are found in practically all of the magmatic zircon grains, have Y/P (a.p.f.u.) ? 1 which most likely resulted from OH accommodation in the zircon structure, a fact suggesting that the OPG parental melt contained water. High-temperature hydrothermal processes induced partial to complete recrystallization of zircon (via dissolution-reprecepitation), a process that was associated with ductile and brittle deformations of the zircon-hosting rocks. The morphology of the hydrothermal zircons varies depending on pH and silica activity in the fluid from weakly corroded subhedral crystals with typical vermicular microtopography of the crystal faces to completely modified grains of colloform structure. Geochemically, the earlier hydrothermal transformations of the zircons resulted in their enrichment in La and other LREE, except only Ce, whose concentration, conversely, decreases compared to that of the unmodified magmatic zircons. The hydrothermal zircon displays a reduced Ce anomaly and its most altered domains typically host minute inclusions of xenotime, U and Th oxides and silicates, and occasionally also baddeleyite, which suggests that the hydrothermal fluid was reduced and highly alkaline. These features were acquired by the seawater-derived fluid when it circulated within the axial MAR zone area due to phase separation in the H2O–NaCl system and particularly as a result of fluid interaction with the abyssal peridotites of oceanic core complexes. Our data demonstrate that zircon is a sensitive indicator of tectonic and physicochemical processes in the oceanic crust.  相似文献   

16.
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17.
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18.
Following the recommendation of the International Commission on Stratigraphy (16 votes Yes [94%], 1 abstention, 2 votes not received), the Global boundary Stratotype Section and Point (GSSP) for the base of the Turonian Stage of the Cretaceous System is defined as the base of bed 86 of the Bridge Creek Limestone Member of the Greenhorn Limestone Formation at the western end of the Denver and Rio Grande Railroad cut near the north boundary of the Pueblo Reservoir State Park Recreation Area, west of Pueblo, Colorado, USA. This GSSP horizon is also exposed and protected in the adjacent state recreation area. It coincides with the first occurrence of the ammonite Watinoceras devonense, is in the middle of a global positive excursion in Carbon-13 isotopes, and is bracketed by widespread bentonites that have yield edages of 93 to 93.5 Ma.  相似文献   

19.
The further development of Peyve’s concept of deep faults in the Earth’s crust and brittle part of the lithosphere is discussed. Three aspects are accentuated in this paper: (1) the modern definition of the term deep fault; (2) the parameters of deep faults as ruptures of the geological medium and three-dimensional, often boundary, geological bodies; and (3) reactivation of deep faults, including the development of this process in real time. Peyve’s idea of deep faults readily fitted into the concept of new global tectonics (plate tectonics). This was facilitated, first of all, by the extensive efforts made to elaborate Peyve’s ideas by a large group of researchers at the Geological Institute of the Russian Academy of Sciences (GIN RAS) and other scientists. At present, the term deep fault has been extended and transformed to cover three-dimensional geological bodies; the geological and geophysical properties and parameters of these bodies, as well as their reactivation (recurrent activation) in real time, have been studied.  相似文献   

20.
Zabuye Salt Lake in Tibet, China is a carbonate-type salt lake, which has some unique characteristics that make it different from other types of salt lakes. The lake is at the latter period in its evolution and contains liquid and solid resources. Its brine is rich in Li, B, K and other useful minor elements that are of great economic value. We studied the concentration behavior of these elements and the crystallization paths of salts during isothermal evaporation of brine at 15°C and 25°C. The crystallization sequence of the primary salts from the brine at 25°C is halite (NaCl) → aphthitalite (3K2SO4·Na2SO4) → zabuyelite (Li2CO3)→ trona (Na2CO3·NaHCO3·2H2O) → thermonatrite (Na2CO3·H2O) → sylvite (KCl), while the sequence is halite (NaCl) → sylvite (KCl) → trona (Na2CO3·NaHCO3·2H2O) → zabuyelite (Li2CO3) → thermonatrite (Na2CO3·H2O) → aphthitalite (3K2SO4·Na2SO4) at 15°C. They are in accordance with the metastable phase diagram of the Na+, K+-Cl?, CO32?, SO42?-H2O quinary system at 25°C, except for Na2CO3·7H2O which is replaced by trona and thermonatrite. In the 25°C experiment, zabuyelite (Li2CO3) was precipitated in the early stage because Li2CO3 is supersaturated in the brine at 25°C, in contrast with that at 15°C, it precipitated in the later stage. Potash was precipitated in the middle and late stages in both experiments, while boron was concentrated in the early and middle stages and precipitated in the late stage.  相似文献   

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