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1.
Over the last 100?years, Arctic warming has resulted in a longer growing season in boreal and tundra ecosystems. This has contributed to a slow northward expansion of the boreal forest and a decrease in the surface albedo. Corresponding changes to the surface and atmospheric energy budgets have contributed to a broad region of warming over areas of boreal forest expansion. In addition, mesoscale and synoptic scale patterns have changed as a result of the excess energy at and near the surface. Previous studies have identified a relationship between the positioning of the boreal forest-tundra ecotone and the Arctic frontal zone in summer. This study examines the climate response to hypothetical boreal forest expansion and its influence on the summer Arctic frontal zone. Using the Weather Research and Forecasting model over the Northern Hemisphere, an experiment was performed to evaluate the atmospheric response to expansion of evergreen and deciduous boreal needleleaf forests into open shrubland along the northern boundary of the existing forest. Results show that the lower surface albedo with forest expansion leads to a local increase in net radiation and an average hemispheric warming of 0.6°C at and near the surface during June with some locations warming by 1–2°C. This warming contributes to changes in the meridional temperature gradient that enhances the Arctic frontal zone and strengthens the summertime jet. This experiment suggests that continued Northern Hemisphere high-latitude warming and boreal forest expansion might contribute to additional climate changes during the summer.  相似文献   

2.
Using the CAM3.0 model, we investigated the respective effects of aerosol concentration increasing and decadal variation of global sea surface temperature(SST) around year 1976/77 on the East Asian precipitation in boreal summer. By doubling the concentration of the sulfate aerosol and black carbon aerosol separately and synchronously in East Asia(100-150 °E, 20-50 °N), the climate effects of these aerosols are specifically investigated. The results show that both the decadal SST changing and aerosol concentration increasing could lead to rainfall decreasing in the center of East Asia, but increasing in the regions along southeast coast areas of China. However, the different patterns of rainfall over ocean and lower wind field over Asian continent between aerosol experiments and SST experiments in CAM3.0 indicate the presence of different mechanisms. In the increased aerosol concentration experiments, scattering effect is the main climate effect for both sulfate and black carbon aerosols in the Eastern Asian summer. Especially in the increased sulfate aerosol concentration experiment, the climate scattering effect of aerosol leads to the most significant temperature decreasing, sinking convection anomalies and decreased rainfall in the troposphere over the central part of East Asia. However, in an increased black carbon aerosol concentration experiment, weakened sinking convection anomalies exist at the southerly position. This weakened sinking and its compensating rising convection anomalies in the south lead to the heavy rainfall over southeast coast areas of China. When concentrations of both sulfate and black carbon aerosols increase synchronously, the anomalous rainfall distribution is somewhat like that in the increased black carbon concentration aerosol experiment but with less intensity.  相似文献   

3.
Dimethylsulphide (DMS) is an important sulphur‐containing trace gas produced by enzymatic cleavage of its precursor compound, dimethylsulphoniopropionate (DMSP), which is released by marine phytoplankton in the upper ocean. After ventilation to the atmosphere, DMS is oxidised to form sulphate aerosols which in the unpolluted marine atmosphere are a major source of cloud condensation nuclei (CCN). Because the micro‐physical properties of clouds relevant to climate change are sensitive to CCN concentration in air, it has been postulated that marine sulphur emissions may play a rôle in climate regulation. The Subantarctic Southern Ocean (41–53°S) is relatively free of anthropogenic sulphur emissions, thus sulphate aerosols will be mainly derived from the biogenic source of DMS, making it an ideal region in which to evaluate the DMS‐climate regulation hypothesis. We have extended a previous modelling analysis of the DMS cycle in this region by employing a coupled general circulation model (CGCM) which has been run in transient mode to provide a more realistic climate scenario. The CGCM output provided meteorological data under the IPCC/IS92a radiative forcing scenario. A DMS production model has been forced with the CGCM climate data to simulate the trend in the sea‐to‐air DMS flux for the period 1960 to 2080, corresponding to equivalent CO2 tripling relative to pre‐industrial levels. The results confirm a minor but non‐negligible increase in DMS flux in this region, in the range +1% to +6% predicted over the period simulated. Uncertainty analysis of the DMS model predictions have confirmed the positive sign for the change in DMS flux, that is a negative DMS feedback on warming.  相似文献   

4.
Aerosol particles are of particular importance because of their impacts on cloud development and precipitation processes over land and ocean. Aerosol properties as well as meteorological observations from the Department of Energy Atmospheric Radiation Measurement(ARM) platform situated in the Southern Great Plains(SGP) are utilized in this study to illustrate the dependence of continental cloud condensation nuclei(CCN) number concentration(NCCN) on aerosol type and transport pathways. ARM-SGP observations from the 2011 Midlatitude Continental Convective Clouds Experiment field campaign are presented in this study and compared with our previous work during the 2009–10 Clouds, Aerosol, and Precipitation in the Marine Boundary Layer field campaign over the current ARM Eastern North Atlantic site. Northerly winds over the SGP reflect clean, continental conditions with aerosol scattering coefficient(σ_(sp)) values less than 20 Mm~(-1) and NCCNvalues less than 100 cm~(-3). However, southerly winds over the SGP are responsible for the observed moderate to high correlation(R)among aerosol loading(σ_(sp) 60 Mm~(-1)) and NCCN, carbonaceous chemical species(biomass burning smoke), and precipitable water vapor. This suggests a common transport mechanism for smoke aerosols and moisture via the Gulf of Mexico,indicating a strong dependence on air mass type. NASA MERRA~(-2) reanalysis aerosol and chemical data are moderately to highly correlated with surface ARM-SGP data, suggesting that this facility can represent surface aerosol conditions in the SGP, especially during strong aerosol loading events that transport via the Gulf of Mexico. Future long-term investigations will help to understand the seasonal influences of air masses on aerosol, CCN, and cloud properties over land in comparison to over ocean.  相似文献   

5.
It is well known that the emissions of hot gases from various power stations and other industrial sources in the regional atmosphere cause decrease in rainfall around these complexes. To overcome this shortage, one method is to introduce artificially conducive aerosol particles in the atmosphere using aeroplane to increase rainfall. To prove the feasibility of this idea, in this paper, a nonlinear mathematical model is proposed involving five dependent variables, namely, the volume density of water vapour, number densities of cloud droplets and raindrops, and the concentrations of small and large size conducive aerosol particles. It is assumed that two types of aerosol particles are introduced in the regional atmosphere, one of them is of small size CCN type which is conducive to increase cloud droplets from vapour phase, while the other is of large size and is conducive to transform the cloud droplets to raindrops. The model is analyzed using stability theory of differential equations and computer simulation. The model analysis shows that due to the introduction of conducive aerosol particles in the regional atmosphere, the rainfall increases as compared to the case when no aerosols are introduced in the atmosphere of the region under consideration. The computer simulation confirms the analytical results.  相似文献   

6.
Ground-based aerosol instrumentation covering particle size diameters from 25 nm to 32 µm was deployed to determine aerosol concentration and cloud condensation nuclei (CCN)-activation properties at water vapor supersaturations in the range of S = 0.20–1.50 % in the remote Brazilian northeast semi-arid region (NEB) in coastal (maritime) and continental (inland) regimes. The instruments measured aerosol number concentration and activation spectra for CCN and revealed that aerosol properties are sensitive with respect to the sources as a function of the local wind circulation system. The observations show that coastal aerosol total number concentrations are above 3,000 cm?3 on average, exhibiting concentration peaks depending on the time of the day in a consistent daily pattern. The variation on aerosol concentration has also influences on the fraction of particles active as CCN. At 1.0 % water vapor supersaturation, the fraction can reach as high as 80 %. Inland aerosol total concentrations were about 1,800–1,900 cm?3 and did not show much diurnal variation. The fraction of particles active as CCN observed inland depend on the history of the air masses, and was much higher when air masses were originated over the sea. It was found that (NH4)2SO4 and NaCl are the major soluble inorganic fraction of the aerosols at the coast. The major fraction of NaCl was present in the coarse mode, while ammonium sulfate dominates the inorganic fraction at the submicron range, with about 10 % of the total aerosol mass at 0.32 µm. Inorganic compounds are almost absent in particles with sizes around 0.1 μm. The study suggests that the air masses with high concentration of CCN originate at the sea. The feasible explanation lies in the fact that the NEB’s beaches have a particular morphology that produces a wide surf zone and creates a large load of aerosols when combined with strong and permanent winds of the region.  相似文献   

7.
In this study, we investigated the response of trees growing at the cold margins of the boreal forest to climate variation in the 20th century. Working at eight sites at and near alpine and arctic treeline in three regions in Alaska, we compared tree growth (from measured tree ring-widths) to historical climate data to document how growth has responded to climate variation in the 20th century. We found that there was substantial regional variability in response to climate variation. Contrary to our expectations, we found that after 1950 warmer temperatures were associated with decreased tree growth in all but the wettest region, the Alaska Range. Although tree growth increased from 1900–1950 at almost all sites, significant declines in tree growth were common after 1950 in all but the Alaska Range sites. We also found that there was substantial variability in response to climate variation according to distance to treeline. Inverse growth responses to temperature were more common at sites below the forest margin than at sites at the forest margin. Together, these results suggest that inverse responses to temperature are widespread, affecting even the coldest parts of the boreal forest. Even in such close proximity to treeline, warm temperatures after 1950 have been associated with reduced tree growth. Growth declines were most common in the warmer and drier sites, and thus support the hypothesis that drought-stress may accompany increased warming in the boreal forest.  相似文献   

8.
Climate Change and People-Caused Forest Fire Occurrence in Ontario   总被引：2，自引：0，他引：2  
Climate change that results from increasing levels of greenhouse gases in the atmosphere has the potential to increase temperature and alter rainfall patterns across the boreal forest region of Canada. Daily output from the Canadian Climate Centre coupled general circulation model (GCM) and the Hadley Centre's HadCM3 GCM provided simulated historic climate data and future climate scenarios for the forested area of the province of Ontario, Canada. These models project that in climates of increased greenhouse gases and aerosols, surface air temperatures will increase while seasonal precipitation amounts will remain relatively constant or increase slightly during the forest fire season. These projected changes in weather conditions are used to predict changes in the moisture content of forest fuel, which influences the incidence of people-caused forest fires. Poisson regression analysis methods are used to develop predictive models for the daily number of fires occurring in each of the ecoregions across the forest fire management region of Ontario. This people-caused fire prediction model, combined with GCM data, predicts the total number of people-caused fires in Ontario could increase by approximately 18% by 2020–2040 and50% by the end of the 21st century.  相似文献   

9.
There are many indicators that human activity may change climate conditions all around the globe through emissions of greenhouse gases. In addition, aerosol particles are emitted from various natural and anthropogenic sources. One important source of aerosols arises from biomass burning, particularly in low latitudes where shifting cultivation and land degradation lead to enhanced aerosol burden. In this study the counteracting effects of greenhouse gases and aerosols on African climate are compared using climate model experiments with fully interactive aerosols from different sources. The consideration of aerosol emissions induces a remarkable decrease in short-wave solar irradiation near the surface, especially in winter and autumn in tropical West Africa and the Congo Basin where biomass burning is mainly prevailing. This directly leads to a modification of the surface energy budget with reduced sensible heat fluxes. As a consequence, temperature decreases, compensating the strong warming signal due to enhanced trace gas concentrations. While precipitation in tropical Africa is less sensitive to the greenhouse warming, it tends to decrease, if the effect of aerosols from biomass burning is taken into account. This is partly due to the local impact of enhanced aerosol burden and partly to modifications of the large-scale monsoon circulation in the lower troposphere, usually lagging behind the season with maximum aerosol emissions. In the model equilibrium experiments, the greenhouse gas impact on temperature stands out from internal variability at various time scales from daily to decadaland the same holds for precipitation under the additional aerosol forcing. Greenhouse gases and aerosols exhibit an opposite effect on daily temperature extremes, resulting in an compensation of the individual responses under the combined forcing. In terms of precipitation, daily extreme events tend to be reduced under aerosol forcing, particularly over the tropical Atlantic and the Congo basin. These results suggest that the simulation of the multiple aerosol effects from anthropogenic sources represents an important factor in tropical climate change, hence, requiring more attention in climate modelling attempts.  相似文献   

10.
The Russian boreal forest contains about 25% of the global terrestrial biomass, and even a higher percentage of the carbon stored in litter and soils. Fire burns large areas annually, much of it in low-severity surface fires – but data on fire area and impacts or extent of varying fire severity are poor. Changes in land use, cover, and disturbance patterns such as those predicted by global climate change models, have the potential to greatly alter current fire regimes in boreal forests and to significantly impact global carbon budgets. The extent and global importance of fires in the boreal zone have often been greatly underestimated. For the 1998 fire season we estimate from remote sensing data that about 13.3 million ha burned in Siberia. This is about 5 times higher than estimates from the Russian Aerial Forest Protection Service (Avialesookhrana) for the same period. We estimate that fires in the Russian boreal forest in 1998 constituted some 14–20% of average annual global carbon emissions from forest fires. Average annual emissions from boreal zone forests may be equivalent to 23–39% of regional fossil fuel emissions in Canada and Russia, respectively. But the lack of accurate data and models introduces large potential errors into these estimates. Improved monitoring and understanding of the landscape extent and severity of fires and effects of fire on carbon storage, air chemistry, vegetation dynamics and structure, and forest health and productivity are essential to provide inputs into global and regional models of carbon cycling and atmospheric chemistry.  相似文献   

11.
Abstract This paper describes the effect of the presence of water-soluble organic compounds (WSOC) in aerosol particles on the aerosol critical supersaturation as defined by the Köhler theory and on cloud condensation nuclei (CCN) number concentration. Taking into account both the soluble mass increase and the surface tension depression due to WSOC, we calculated a substantial decrease of the aerosol critical supersaturation, which results in a large increase in CCN number concentration. CCN supersaturation spectra were computed for three different aerosol types: marine, rural and urban. The increase of CCN number concentration in the presence of WSOC (with respect to the case when only the inorganic aerosol compounds are considered) varies with aerosol type, with an increase up to 13% in the marine case, up to 97% in the rural case, and up to 110% in the urban case, for the supersaturation range typical of atmospheric conditions.  相似文献   

12.
In this work we propose and test a method to calculate cloud condensation nuclei (CCN) spectra based on aerosol number size distributions and hygroscopic growth factors. Sensitivity studies show that this method can be used in a wide variety of conditions except when the aerosol consist mainly of organic compounds. One crucial step in the calculations, estimating soluble ions in an aerosol particle based on hygroscopic growth factors, is tested in an internal hygroscopic consistency study. The results show that during the second Aerosol Characterization Experiment (ACE-2) the number concentration of inorganic ions analyzed in impactor samples could be reproduced from measured growth factors within the measurement uncertainties at the measurement site in Sagres, Portugal.
CCN spectra were calculated based on data from the ACE-2 field experiment at the Sagres site. The calculations overestimate measured CCN spectra on average by approximately 30%, which is comparable to the uncertainties in measurements and calculations at supersaturations below 0.5%. The calculated CCN spectra were averaged over time periods when Sagres received clean air masses and air masses influenced by aged and recent pollution. Pollution outbreaks enhance the CCN concentrations at supersaturations near 0.2% by a factor of 3 (aged pollution) to 5 (recent pollution) compared to the clean marine background concentrations. In polluted air masses, the shape of the CCN spectra changes. The clean spectra can be approximated by a power function, whereas the polluted spectra are better approximated by an error function.  相似文献   

13.
We propose a climate stabilizing feedback loop involving biogenic sulfur. The mechanism is similar to the "CLAW" hypothesis (Charlson et al., 1987) but does not require the active participation of the ocean biota. The magnitude of the feedback response in this loop is derived by convective transport of biogenic sulfur over tropical oceans into the middle and high troposphere. Once aloft, the sulfur is oxidized into low-volatile species which nucleate new particles that later subside back into the subtropical marine boundary layer (MBL) and serve as cloud condensation nuclei (CCN). The MBL clouds are susceptible to albedo modification by changes in CCN concentrations (Platnick and Twomey, 1995). We envision that as global temperatures rise the sea surface warms, convective mass transport of sulfur will rise and the increased mass of sulfur in the upper troposphere will lead to higher numbers of particles or a shift in the particle size distribution to larger sizes. In either case, there is an increase in the number of particles large enough to act as CCN in the air subsiding backinto the MBL. The increase in CCN increases the cloud albedo, decreases the solar input to the surface and the temperature decreases. More measurements are needed to confirm whether the magnitude of increased sulfur carried through the loop as a function of increased sea surface temperature is sufficient to close the loop and regulate the climate.  相似文献   

14.
A set of vertical profiles of aerosol number concentrations, size distributions and cloud condensation nuclei(CCN)spectra was observed using a passive cloud and aerosol spectrometer(PCASP) and cloud condensation nuclei counter, over the Tongliao area, East Inner Mongolia, China. The results showed that the average aerosol number concentration in this region was much lower than that in heavily polluted areas. Monthly average aerosol number concentrations within the boundary layer reached a maximum in May and a minimum in September, and the variations in CCN number concentrations at different supersaturations showed the same trend. The parameters c and k of the empirical function N = c S~kwere 539 and1.477 under clean conditions, and their counterparts under polluted conditions were 1615 and 1.42. Measurements from the airborne probe mounted on a Yun-12(Y12) aircraft, together with Hybrid Single-Particle Lagrangian Integrated Trajectory model backward trajectories indicated that the air mass from the south of Tongliao contained a high concentration of aerosol particles(1000–2500 cm~(-3)) in the middle and lower parts of the troposphere. Moreover, detailed intercomparison of data obtained on two days in 2010 indicated that the activation efficiency in terms of the ratio of NCCNto N_a(aerosols measured from PCASP) was 0.74(0.4 supersaturations) when the air mass mainly came from south of Tongliao, and this value increased to 0.83 on the relatively cleaner day. Thus, long-range transport of anthropogenic pollutants from heavily polluted mega cities,such as Beijing and Tianjin, may result in slightly decreasing activation efficiencies.  相似文献   

15.
Growth of fine aerosol particles is investigated during the Aerosol–CCN–Cloud Closure Experiment campaign in June2013 at an urban site near Beijing. Analyses show a high frequency(~ 50%) of fine aerosol particle growth events, and show that the growth rates range from 2.1 to 6.5 nm h~(-1) with a mean value of ~ 5.1 nm h~(-1). A review of previous studies indicates that at least four mechanisms can affect the growth of fine aerosol particles: vapor condensation, intramodal coagulation,extramodal coagulation, and multi-phase chemical reaction. At the initial stage of fine aerosol particle growth, condensational growth usually plays a major role and coagulation efficiency generally increases with particle sizes. An overview of previous studies shows higher growth rates over megacity, urban and boreal forest regions than over rural and oceanic regions. This is most likely due to the higher condensational vapor, which can cause strong condensational growth of fine aerosol particles.Associated with these multiple factors of influence, there are large uncertainties for the aerosol particle growth rates, even at the same location.  相似文献   

16.
Over the last century, the Arctic has warmed at twice the rate of the planet as a whole. Observational evidence indicates that this rapid warming is affecting the tundra and boreal forest biomes by changing their structure and geographic distribution. A global climate model (GCM) was used to explore the atmospheric response to boreal forest expansion by applying a one-grid cell shift of the forest into tundra. This subtle shift is meant to represent the expansion that would occur this century rather than more extreme scenarios predicted by dynamic vegetation models. Results show that this shift causes an average annual warming of 0.3 °C over the region because of a reduction in the surface albedo and an increase in net radiation. A warming of ~1.0 °C occurs in spring when the forest masks the higher albedo snow-covered surface and results in snowmelt and a reduction in cloud cover. Results fail to show a larger-scale dynamical response although some warming of the lower and mid troposphere occurs in July. No changes were found in the position or strength of the Arctic frontal zone as some studies have indicated will occur with a shift in the boreal forest-tundra boundary. These findings suggest that coupled model simulations that predict larger changes in vegetation distribution are likely overemphasizing the amount of Arctic warming that will occur this century. These findings also indicate that a realistic dynamical response to subtle land cover change might not be correctly simulated by GCMs run at coarse spatial resolutions.  相似文献   

17.
By analyzing airborne observations over North China from 30 flights during spring and autumn of 2005-2007, characteristics of the vertical distributions of aerosol and cloud condensation nuclei (CCN) at 0.3% supersaturation in various locations of North China are investigated. The measurement samplings were conducted over different surfaces such as plains, plateau, and sea. The results show that the number concentration of accumulation mode aerosols was greater in autumn than in spring, but the reverse is true for CCN. This means that more aerosols with diameters smaller than 100 nm could be activated as CCN in spring, and this could induce higher aerosol activation efficiency. The aerosol activation efficiency over the plains near the Taihang Mountain was greater in spring than in autumn, and it was greater over sea than over land. The aerosol activation efficiency above the boundary layer over the Bashang Plateau was very low. Based on a fit of the negative exponential vertical distributions of aerosol and CCN, a spatial parameterization model of aerosol and CCN as well as aerosol activation efficiency over North China was proposed. The results show that aerosol activation efficiency was not clearly dependent on altitude because it was mainly affected by regional physical and chemical characteristics of aerosols and the ambient atmospheric conditions. The mean aerosol activation efficiency is 0.66, with values of 0.70 and 0.53 in spring and autumn,respectively.  相似文献   

18.
Effects of aerosol radiative forcing on the diurnal and seasonal cycles of precipitation over West Africa and eastern Atlantic Ocean are investigated for the boreal summer season: June–July–August. An eight year (2000–2007) average of GCM simulated rainfall data is compared with the corresponding TRMM rainfall data. The comparison shows that the amplitude of the diurnal cycles of rainfall over land and ocean are reasonably well simulated. Over land, the phase of the simulated diurnal cycle of precipitation peaks several hours earlier than that of the TRMM data. Corresponding differences over the ocean(s) are relatively smaller. Some of the key features of the aerosol induced model simulated field anomalies are: (a) aerosol direct radiative forcing which increases the atmospheric stability and reduces the daytime moist convection and convective precipitation; (b) the aerosol induced changes in the diurnal cycle of precipitation are out of phase with those of the TRMM data over land, but are in-phase over the ocean; (c) aerosols reduce the amplitude of the diurnal cycle of precipitation over land and enhance it over ocean. However, the phase of the diurnal cycle is not affected much by the aerosol radiative forcing both over land and ocean. During the boreal summer, aerosol radiative forcing and induced circulation and precipitation cool the Sahel and the southern part of Sahara desert more than the adjacent areas to the north and south, thereby shifting the peak meridional temperature gradient northward. Consequently, an anomalous easterly jet is found north of its climatological location. This anomalous jet is associated with increased cyclonic circulation to the south of its axis, resulting in an anomalous monsoon rain belt in the Sahel.  相似文献   

19.
Although it is believed that organic aerosols play a key role in cloud nucleation and make an important contribution to the cloud condensation nuclei (CCN) population, their specific species remain poorly characterized. This paper reviews the current knowledge of organic acids (mainly formic, acetic, pyruvic and oxalic acids). Without specification, organic acids in this paper refer to these four organic acids in the gas and aerosol phases. This paper analyzes the extent to which organic acids act as CCN and compares the physical and chemical properties of organic acids with those of CCN. The results show that aerosol formate and acetate concentrations range from 0.02 to 5.3 nmol m−3 and from 0.03 to 12.4 nmol m−3, respectively, and that between 34 to 77% of formate and between 21 to 66% of acetate are present in the fine fraction of aerosols. It was found that although most (98–99%) of these volatile organic acids are present in the gas phase, their concentrations in the aerosol particles are sufficient to make them a good candidate for CCN. The results also show that organic acids may make an important contribution to the formation of CCN in some special sources such as vegetation emissions and biomass-burning. Organic acids are expected to contribute significantly to the estimates of indirect (cloud-mediated) forcing due to aerosols.  相似文献   

20.
A semi-empirical model has been developed to reproduce glacial–interglacial changes of continental dust and marine sodium concentrations (factor of ∼50 and ∼5, respectively) observed in inland Antarctic ice cores. The model uses conceptual pathways of aerosols within the high troposphere; assumes the dry deposition of impurities on the Antarctic surface; uses estimates of aerosol transit times taken independent of climate; assumes a temperature-dependent removal process during aerosol pathways from the mid-latitudes. The model is fitted to the data over the last four climate cycles from Vostok and EPICA Dome C Antarctic sites. As temperature is cooling, the aerosol response suggests different modes of climate couplings between latitudes, which can be continuous or below temperature thresholds for sodium and dust, respectively. The model estimates a southern South America dust source activity two to three times higher for glacial periods than for the Holocene and a glacial temperature over the Southern Ocean 3–5 °C cooler. Both estimates appear consistent with independent observations. After removal of temperature effects, dust and sodium residuals for both sites show orbital frequencies in opposite phase at the precession timescale. Such long-term insolation-related modulation of terrestrial and marine aerosol input, could provide a chemical pacemaker useful for refining ice core chronologies.  相似文献   

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