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1.
In this study, an optimized single-channel phoswich well detector design has been proposed and assessed in order to improve beta–gamma coincidence measurement sensitivity of xenon radioisotopes. This newly designed phoswich well detector consists of a plastic beta counting cell (BC404) embedded in a CsI (Tl) crystal coupled to a photomultiplier tube. The BC404 is configured in a cylindrical pipe shape to minimise light collection deterioration. The CsI (Tl) crystal consists of a rectangular part and a semi-cylinder scintillation part as a light reflector to increase light gathering. Compared with a PhosWatch detector, the final optimized detector geometry showed 15 % improvement in the energy resolution of a 131mXe 129.4 keV conversion electron peak. The predicted beta–gamma coincidence efficiencies of xenon radioisotopes have also been improved accordingly.  相似文献   

2.
This paper describes a method to calibrate a neutron capture sonde equipped with a high resolution γ-ray detector, and analyze log data. The method utilizes the 1460.8-keV passive γ-ray of 40K, the 770.3-keV capture γ-ray of 39K, and a capture γ-ray from a target element. An equation containing the spectral line intensities for the two capture γ-rays, nuclear capture data, and the detector efficiency function expresses the concentration of the target element as a multiple of the 39K concentration. The concentration of 39K is easily deduced from the 40K concentration, which is calculated directly from the line intensity for the 1460.8-keV γ-ray in a passive γ-ray spectrum.The calibration automatically adjusts to changes in the neutron transport properties of the logged medium that may result, for example, from variations in the H density and the concentrations of neutron poisons. Fluctuations in the neutron source output are similarly accommodated. The calibration utilizes U.S. Department of Energy (DOE) passive γ-ray calibration standards that contain well established concentrations of K, U, and Th. The passive γ-rays from K, U, and Th (and the U and Th decay progenies) provide data for the detector efficiency function determination.Data for proof-of-principle demonstrations of the method were acquired by logging boreholes penetrating the shallow subsurface at a DOE waste site with a simple, reliable neutron capture logging system. The system had a 252Cf source and a high purity germanium (HPGe) detector. Time gating could not be used to sort signals originating from capture and activation, but the excellent energy resolution permitted capture γ-ray identifications based solely on the γ-ray energies. Cl, H, and other elements were detected and assessed.A conventional calibration and data analysis method was also employed. The method was specific to Cl and was based on measurements in two Cl-impregnated concrete blocks. Cl concentrations inferred with this method were often consistent with the concentrations determined with the new method. When the two methods produced different Cl concentrations, the discrepancies could be explained by variations in formation parameters.  相似文献   

3.
The resonance transition 2P-2S of the atomic hydrogen (Lyman-alpha emission) is the strongest and most conspicuous feature in the solar EUV spectrum. The Lyman-alpha radiation transfer depends on the resonance scattering from the hydrogen atoms in the atmosphere and on the O2 absorption. Since the Lyman-alpha extinction in the atmosphere is a measure for the column density of the oxygen molecules, the atmospheric O2 density and temperature profiles can be calculated thereof. A detector of solar Lyman-alpha radiation was manufactured in the Stara Zagora Department of the Solar-Terrestrial Influences Laboratory (STIL). Its basic part is an ionization camera, filled in with NO. A 60 V power supply is applied to the chamber. The produced photoelectric current from the sensor is fed to a two-channel amplifier, providing analog signal. The characteristics of the Lyman-alpha detector were studied. It passed successfully all tests and the results showed that the so-designed instrument could be used in rocket experiments to measure the Lymanalpha flux. From the measurements of the detector, the Lyman-alpha vertical profile can be obtained. Programs are created to compute the O2 density, atmospheric power and temperature profiles based on Lymanalpha data. The detector design appertained to ASLAF project (Attenuation of the Solar Lyman-Alpha Flux), a scientific cooperation between STIL—Bul.Acad.Sci., Stara Zagora Department and the Atmospheric Physics Group at the Department of Meteorology (MISU), Stockholm University, Sweden. The joint project was part of the rocket experiment HotPay I, in the ALOMAR eARI Project, EU’s 6th Framework Programme, Andøya Rocket Range, Andenes, Norway. The project is partly financed by the Bulgarian Ministry of Science and Education.  相似文献   

4.
Superficial volcanic manifestations occurred at Soufriere de Guadeloupe in 1976–1977. Superficial phenomena started on July 8, and had been preceded the previous year by a seismovolcanic crisis of exceptional amplitude for the Caribbean region. The essentially phreatic manifestations were accompanied by an extraordinarily high number of recorded quiakes: 16,467 earthquakes in 21 months, 153 of which classified as clearly perceived. The epicentral area covered about 30 km2, and the seismic energy released reached a total of 1018 erg. Thirty-six volcanic tremors accompanied violent superficial manifestations, and 26 strong phreatic eruptions have been observed. The important role played by seismology as a crisis detector for this type of volcanoes has been clearly shown.  相似文献   

5.
The energy released in a spontaneous decay process of natural radionuclides is the main source of the total radiation dose to human beings. Natural radionuclides are widely distributed in soil, rocks, air, and groundwater. In present investigation, the analysis of terrestrial radionuclides such as 226Ra, 232Th, and 40K in soil and sand of Chattarpur area of southeastern coast of Odisha has been carried out using NaI(Tl) gamma ray detector. The higher activity concentrations of naturally occurring radionuclides have been reported from the study area. The gamma radiationdose originating from the terrestrial radionuclides was found to vary from 95 to 1813 nGy/h with an average of 700 nGy/h. This study is important to generate a baseline data of radiation exposure in the area. Health hazard effects due to natural radiation exposure are discussed in details.  相似文献   

6.
The Wilson electron synchrotron at Cornell University has recently undergone modifications which enable it to produce a highly collimated X-ray beam of 1015 photons (s mrad. 10% bandwidth)?1 in the range from 1 to 40 keV (12.4 to 0.31 Å wavelength). It is expected that a monochromatic beam produced from this source will have at least a hundred times the intensity of the X-rays from a rotating anode source. It is hoped that the use of a position-sensitive detector will improve the detection efficiency by another factor of a hundred over photographic film. If these improvements are realized, it should be possible to conduct real-time or nearly real-time diffraction experiments in the diamond anvil cell. The technique will be used to collect data for experiments in which slower data collecting would mean missing transient phenomena. The technique will also be useful for making studies during conditions that cause deterioration of the experimental apparatus such as graphitization of the diamonds or creep of the metal parts.  相似文献   

7.
The Wide-Angle Airborne Laser Ranging System (WA-ALRS) is aninstrument developed at IGN with the aim of measuring landsubsidence with sub-cm accuracy. The instrument provides rangemeasurements that are used to estimate the co-ordinates of aground-based network of cube-corner retroreflectors (CCRs).Millimeter accuracy on relative radial co-ordinates has beendemonstrated in a ground-based experiment and centimeter accuracyhas been obtained in a recent airborne experiment. The mainlimitation in the latter experiment came from the low link budgetat longer distances. In this paper we analyze the performanceexpected with two different detector modules (avalanchephotodiodes with amplifiers). Laboratory measurements are used tocharacterize detector parameters and estimate ranging accuracy.Numerical simulations predict a 2–3 mm accuracy in the verticalco-ordinate with these detectors combined to a 2-km aircraftaltitude, a 20 laser beam divergence, a 250-m CCR separation and 103 measurements per CCR.  相似文献   

8.
Malachite green (MG), a traditional agent used in aquaculture although is not approved; its low cost and high efficacy make illicit use likely. We developed a small‐scale, simple, and sensitive dispersive liquid–liquid microextraction procedure for the assay of trace amounts of MG in aquatic environment of Trout fish. Fiber optic‐linear array detection spectrophotometry with charge‐coupled device detector benefiting from a microcell was used for this purpose. The method is based on enhancement effect of an anionic surfactant on the extraction of MG in to very fine multidroplets of microextraction solvent which made assisted by disperser solvent. Under the optimum conditions, the enrichment factor 77.5 was obtained from a 5‐mL water sample. The calibration graph was linear up to 5 × 10?7 mol L?1 with detection limit of 1 × 10?8 mol L?1. The relative standard deviation for seven replicate measurements of 4 × 10?7 and 5 × 10?8 mol L?1 of MG were 3.3 and 4.5%, respectively.  相似文献   

9.
The activity concentrations of 226Ra and 228Ac in weathered Japanese soils from two selected prefectures have been measured using a γ-ray spectroscopy system with high purity germanium detector. The uranium, thorium, and rare earth elements (REEs) concentrations were determined from the same soil samples using inductively coupled plasma mass spectrometry (ICP-MS). For example, granitic rocks contain higher amounts of U, Th, and light REEs compared to other igneous rocks such as basalt and andesites. Therefore, it is necessary to understand the interaction between REEs and nature of soils since soils are complex heterogeneous mixture of organic and inorganic solids, water, and gases. In this paper, we will discuss about distribution pattern of 238U and 232Th along with REEs in soil samples of weathered acid rock (granite) collected from two prefectures of Japan: Hiroshima and Miyagi.  相似文献   

10.
The aim of this study is to assess the performance of linear discriminate analysis, support vector machines (SVMs) with linear and radial basis, classification and regression trees and random forest (RF) in the classification of radionuclide data obtained from three different types of rocks. Radionuclide data were obtained for metamorphic, sedimentary and igneous rocks using gamma spectroscopic method. A P-type high-purity germanium detector was used for the radiometric study. For analysis purpose, we have determined activity concentrations of 232Th, 226Ra and 40K radionuclides, published elsewhere (Rafique et al. in Russ Geol Geophys 55:1073–1082, 2014), in different rock samples and built the classification model after pre-processing the data using three times tenfold cross-validation. Using this model, we have classified the new samples into known categories of sedimentary, igneous and metamorphic. The statistics depicts that RF and SVM with radial kernel outperform as compared to other classification methods in terms of error rate, area under the curve and with respect to other performance measures.  相似文献   

11.
Monitoring of Xe and Kr radionuclides was conducted from August 2006 to 30 July 2008 within the framework of ISTC Project #2133. Cherepovets City in Vologda Province and St. Petersburg were chosen as monitoring locations. Kr–Xe concentrate samples were obtained as a result of processing of several thousand m3 of atmospheric air. New results of 85Kr monitoring show, that for last 15 years, the 85Kr volumetric activity in the atmospheric air of the northwest region of Russia has increased approximately 50% and has achieved a level of 1.5 Bq/m3. This value correlates well with similar data for Western Europe and Japan. The xenon fraction (80–160 cm3 under STP) is adsorbed on charcoal in the ampoule, which is measured in the well of HPGe gamma detector. Minimum detectable concentration (MDC) of 133Xe for this technique is 0.008 mBq/m3, and it is the most sensitive method used today. The 133Xe concentration in the atmospheric air of Cherepovets City varied in the monitoring period ranging from 0.09 to 2.5 mBq/m3. During the period of March 2007–30 July 2008, 133Xe activity concentration in the atmospheric air of St. Petersburg changed from background values (0.2–0.3 mBq/m3) to 185 mBq/m3 and for approximately 20% of the samples 135Xe was also measured with the 135Xe/133Xe activity ratio varied within the range of 0.03–3.5.  相似文献   

12.
In the present study, experiments have been carried out to calibrate LR-115 alpha detector films in bare and cup-mode exposure for the measurement of radon and thoron concentrations in soil gas. Results showed non-uniformity in track formation on the films in bare-mode exposure. However, in cup-mode exposure the non-uniformity was reduced to a greater extent. The calibration factors obtained for radon in bare- and cup-mode exposures are 0.049 and 0.034 tr. cm?2 per Bq m?3 d, respectively. An attempt has been made to calibrate the radon-thoron discriminative cup with LR-115 films for simultaneous measurements of radon and thoron. This paper also presents the preliminary results of radonthoron monitoring in Tatun volcanic areas of northern Taiwan for the first time using radon-thoron discriminators with LR-115 films. The results show that the safe temperature to install the LR-115 films in volcanic areas is ≤ 65°C and thoron concentration in the study area is low.  相似文献   

13.
This report describes the construction and properties of a Ge(Li) bore hole probe for in situ gamma ray spectrometry. The probe has the form of a cylinder 8.9 cm in diameter and 160 cm long. It contains a 22 cm3 coaxial Ge(Li) detector, cooled by liquid nitrogen. Holding time of the assembled probe is in excess of ten hours, energy resolution is 2.3 keV for 122 keV photons and 2.6 keV for 1333 keV photons. The probe has been used in field experiments in the Ranstad uranium mine and for the study of neutron activation spectra obtained in bore hole models. Results from these experiments are presented and discussed. It is stressed that the Ge(Li) probe gives promise to become a powerful tool in bore hole activation analysis.  相似文献   

14.
— Indoor radon radioactivity in the rooms on the ground floor and first floor of the Physics Department, Faculty of Science, Universiti Brunei Darussalam was measured using a system that consists of an air filter pump, ZnS detector, photomultiplier tube and counter. Ground floor rooms' radon radioactivity was found to be about three times higher than that of the first floor. The maximum ground floor indoor radioactivity is only 0.39 Bqm?3, a value relatively low and safe compared to the mean outdoor radon concentration of 1.41 Bqm?3 measured (HU and TAN, 2000). The main source of radon emanation originates from the ground soil rather than the building materials.  相似文献   

15.
We present a new LA–ICP–MS system for zircon fission‐track (FT) and U–Pb double dating, whereby a femtosecond laser combined with galvanometric optics simultaneously ablates multiple spots to measure average surface U contents. The U contents of zircon measured by LA–ICP–MS and standardized with the NIST SRM610 glass are comparable to those measured by the induced FT method, and have smaller analytical errors. LA–ICP–MS FT dating of seven zircon samples including three IUGS age standards is as accurate as the external detector method, but can give a higher‐precision age depending on the counting statistics of the U content measurement. Double dating of the IUGS age standards gives FT and U–Pb ages that are in agreement. A chip of the Nancy 91500 zircon has a homogeneous U content of 84 ppm, suggesting the possibility of using this zircon as a matrix‐matched U‐standard for FT dating. When using the Nancy 91500 zircon as a U‐standard, a zeta calibration value of 42–43 year cm2 for LA–ICP–MS FT dating is obtained. While this value is strictly valid only for the particular session, it can serve as a reference for other studies.  相似文献   

16.
In some volcanic systems, thoron and radon activity and CO2 flux, in soil and fumaroles, show a relationship between (220Rn/222Rn) and CO2 efflux. It is theorized that deep, magmatic sources of gas are characterized by high 222Rn activity and high CO2 efflux, whereas shallow sources are indicated by high 220Rn activity and relatively low CO2 efflux. In this paper we evaluate whether the observed inverse relationship is a true geochemical signal, or potentially an analytical artifact of high CO2 concentrations. We report results from a laboratory experiment using the RAD7 radon detector, known 222Rn (radon) and 220Rn (thoron), and a controllable percentage of CO2 in the carrier gas. Our results show that for every percentage of CO2, the 220Rn reading should be multiplied by 1.019, the 222Rn radon should be multiplied by 1.003 and the 220Rn/222Rn ratio should be multiplied by 1.016 to correct for the presence of the CO2.  相似文献   

17.
Chromatographic analyses of fumarolic gases, collected in sampling bottles containing an alkaline solution, have been carried out using a thermal conductivity detector and a flame ionization detector, after catalytic conversion of CO and CH4. The latter method enables the concentration of carbon monoxide to be measured with sufficient accuracy for use in a CO-CO2-H2-H2O geothermometer. Application of this geothermometer to fumaroles in the crater of Solfatara in the Campi Flegrei, Italy, indicates that they are fed from a steam reservoir at 250±15 °C and at 10–36±2atm of oxygen. On the other hand, the CH4-CO2-H2-H2O geothermobarometer seems to re-equilibrate at superficial temperatures and cannot be used for infering thermodynamic conditions at depth. Regular sampling of these fumaroles together with a geothermometric interpretation of the gas analyses provides a means of monitoring, with comparative accuracy, the chemical and thermal evolution of the hydrothermal reservoir below the Solfatara crater. Such monitoring would probably detect an increase in temperature at depth and the injection of magmatic gas into the reservoir.  相似文献   

18.
The natural radioactivity due to radium, thorium, and potassium in building material samples contribute to the radiation dose received by human beings significantly. It is essential to evaluate the activity levels of these nuclides for the assessment of natural radiation dose. Activity concentrations of the gamma emitting primordial radionuclides 232Th, 226Ra, and 40K were measured using high resolution gamma spectrometry technique with high purity germanium (HPGe) detector in building materials: sand, brick, granite, cement and rock, collected from various areas of Gulbarga and Koppal districts. The standard ASTM procedure was followed for the sample preparation. The distribution of radionuclides and variation in activity concentration depend upon the rock formation and the geological properties of the region. The activity of the three radionuclides, 232Th, 226Ra, and 40K, were found to be in the range of 3.1–227.1, 1.6–111, and 23.2–1505 Bq/kg, respectively. The dose related radiological parameters were also calculated for all the samples and the observations show that the activity concentrations of the radionuclides are well within the UNSCEAR limits.  相似文献   

19.
Accurate characterization of contaminant mass in zones of low hydraulic conductivity (low k) is essential for site management because this difficult‐to‐treat mass can be a long‐term secondary source. This study developed a protocol for the membrane interface probe (MIP) as a low‐cost, rapid data‐acquisition tool for qualitatively evaluating the location and relative distribution of mass in low‐k zones. MIP operating parameters were varied systematically at high and low concentration locations at a contaminated site to evaluate the impact of the parameters on data quality relative to a detailed adjacent profile of soil concentrations. Evaluation of the relative location of maximum concentrations and the shape of the MIP vs. soil profiles led to a standard operating procedure (SOP) for the MIP to delineate contamination in low‐k zones. This includes recommendations for: (1) preferred detector (ECD for low concentration zones, PID or ECD for higher concentration zones); (2) combining downlogged and uplogged data to reduce carryover; and (3) higher carrier gas flow rate in high concentration zones. Linear regression indicated scatter in all MIP‐to‐soil comparisons, including R2 values using the SOP of 0.32 in the low concentration boring and 0.49 in the high concentration boring. In contrast, a control dataset with soil‐to‐soil correlations from borings 1‐m apart exhibited an R2 of ≥0.88, highlighting the uncertainty in predicting soil concentrations using MIP data. This study demonstrates that the MIP provides lower‐precision contaminant distribution and heterogeneity data compared to more intensive high‐resolution characterization methods. This is consistent with its use as a complementary screening tool.  相似文献   

20.
In the Long Valley caldera, where seismicity has continued essentially uninterrupted since mid-1980 and uplift is documented, samples of water from hot, warm, and cold springs have been collected since September, 1982, and their222Rn concentrations analyzed. Concurrently, rocks encompassing the hydrologic systems feeding the springs were analyzed for their radioelement contents, because their uranium is the ultimate source of the222Rn in the water.The222Rn concentration in the springs varies inversely with their temperature and specific conductance. High concentrations (1500 to 2500 picocuries per liter) occur in dilute cold springs on the margins of the caldera, while low contents (12 to 25 pCi/l) occur in hot to boiling springs. Springwater radon concentrations also correlate slightly with the uranium content of the encompassing rocks.A continuous monitoring system was installed in August, 1983, at a spring issuing from basalt, to provide hourly records of radon concentration. A gamma detector is submerged in a natural pool, and we have observed that the radioactivity measured in this manner is due almost entirely to the222Rn concentration of the water. Initial operation shows diurnal and semidiurnal variations in the222Rn concentration of the springwater that are ascribed to earth tides, suggesting that those variations are responding to small changes in stress in the rocks encompassing the hydrologic system.  相似文献   

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