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1.
The radiogenic and primordial noble gas content of the atmospheres of Venus, Earth, and Mars are compared with one another and with the noble gas content of other extraterrestial samples, especially meteorites. The fourfold depletion of 40Ar for Venus relative to the Earth is attributed to the outgassing rates and associated tectonics and volcanic styles for the two planets diverging significantly within the first billion or so years of their history, with the outgassing rate for Venus becoming much less than that for the Earth at subsequent times. This early divergence in the tectonic style of the two planets may be due to a corresponding early onset of the runaway greenhouse on Venus. The 16-fold depletion of 40Ar for Mars relative to the Earth may be due to a combination of a mild K depletion for Mars, a smaller fraction of its interior being outgassed, and to an early reduction in its outgassing rate. Venus has lost virtually all of its primordial He and some of its radiogenic He. The escape flux of He may have been quite substantial in Venus' early history, but much diminished at later times, with this time variation being perhaps strongly influenced by massive losses of H2 resulting from efficient H2O loss processes.Key trends in the primordial noble gas content of terrestial planetary atmospheres include (1) a several orders of magnitude decrease in 20Ne and 36Ar from Venus to Earth to Mars; (2) a nearly constant 20Ne/36Ar ratio which is comparable to that found in the more primitive carbonaceous chondrites and which is two orders of magnitude smaller than the solar ratio; (3) a sizable fractionation of Ar, Kr, and Xe from their solar ratios, although the degree of fractionation, especially for 36Ar/132Xe, seems to decrease systematically from carbonaceous chondrites to Mars to Earth to Venus; and (4) large differences in Ne and Xe isotopic ratios among Earth, meteorites, and the Sun. Explaining trends (2), (2) and (4), and (1) pose the biggest problems for the solar-wind implantation, primitive atmosphere, and late veneer hypotheses, respectively. It is suggested that the grain-accretion hypothesis can explain all four trends, although the assumptions needed to achieve this agreement are far from proven. In particular, trends (1), (2), (3), and (4) are attributed to large pressure but small temperature differences in various regions of the inner solar system at the times of noble gas incorporation by host phases; similar proportions of the host phases that incorporated most of the He and Ne on the one hand (X) and Ar, Kr, and Xe on the other hand (Q); a decrease in the degree of fractionation with increasing noble-gas partial pressure; and the presence of interstellar carriers containing isotopically anomalous noble gases.Our analysis also suggests that primordial noble gases were incorporated throughout the interior of the outer terrestial planets, i.e., homogeneous accretion is favored over inhomogeneous accretion. In accord with meteorite data, we propose that carbonaceous materials were key hosts for the primordial noble gases incorporated into planets and that they provided a major source of the planets' CO2 and N2.  相似文献   

2.
Abstract— The trapped noble gas record of 57 enstatite chondrites (E chondrites) has been investigated. Basically, two different gas patterns have been identified dependent on the petrologic type. All E chondrites of type 4 to 6 show a mixture of trapped common chondritic rare gases (Q) and a subsolar component (range of elemental ratios for E4–6 chondrites: 36Ar/132Xe = 582 ± 270 and 36Ar/84Kr = 242 ± 88). E3 chondrites usually contain Q gases, but also a composition with lower 36Ar/132Xe and 36Ar/84Kr ratios, which we call sub‐Q (36Ar/132Xe = 37.0 ± 18.0 and 36Ar/84Kr = 41.7 ± 18.1). The presence of either the subsolar or the sub‐Q signature in particular petrologic types cannot be readily explained by parent body metamorphism as postulated for ordinary chondrites. We therefore present a different model that can explain the bimodal distribution and composition of trapped heavy noble gases in E chondrites. Trapped solar noble gases have been observed only in some E3 chondrites. About 30% of each group, EH3 and EL3 chondrites, amounting to 9% of all analyzed E chondrites show the solar signature. Notably, only one of those meteorites has been explicitly described as a regolith breccia.  相似文献   

3.
《Icarus》2003,165(2):326-339
The origin of the terrestrial atmosphere is one of the most puzzling enigmas in the planetary sciences. It is suggested here that two sources contributed to its formation, fractionated nebular gases and accreted cometary volatiles. During terrestrial growth, a transient gas envelope was fractionated from nebular composition. This transient atmosphere was mixed with cometary material. The fractionation stage resulted in a high Xe/Kr ratio, with xenon being more isotopically fractionated than krypton. Comets delivered volatiles having low Xe/Kr ratios and solar isotopic compositions. The resulting atmosphere had a near-solar Xe/Kr ratio, almost unfractionated krypton delivered by comets, and fractionated xenon inherited from the fractionation episode. The dual origin therefore provides an elegant solution to the long-standing “missing xenon” paradox. It is demonstrated that such a model could explain the isotopic and elemental abundances of Ne, Ar, Kr, and Xe in the terrestrial atmosphere.  相似文献   

4.
Abstract— This work reports on the noble gas inventory of 3 new acapulcoites, 3 brachinites, 2 new eucrites from the Dar al Gani region in Libya, the unique achondrite Dar al Gani (DaG) 896 from the same locality, the new eucrite‐like achondrite Northwest Africa (NWA) 011, and the controversial sample Tafassasset. We determined cosmic ray exposure and gas retention ages, evaluated shielding conditions, and discuss the trapped noble gas component of the specimens. All exposure ages are within the known range of stony meteorites and partly confirm previously established age clusters. Shielding conditions vary, suggesting substantial shielding for all 3 brachinites and Tafassasset. We cannot exclude, however, that the Mg‐rich composition of brachinites simply simulates heavy shielding. Regarding the trapped component, we found Q‐like compositions only for the acapulcoite Thiel Mountains (TIL) 99002. The brachinite Elephant Moraine (EET) 99402 yields a high, subsolar 36Ar/132Xe ratio of ?400 along with a slightly elevated 84Kr/132atio, indicating minor atmospheric contamination. All the other samples, particularly the eucrite DaG 983, are characterized by clearly elevated Ar/Kr/Xe ratios due to significant terrestrial alteration. Tafassasset exhibits noble gas parameters that are different from those of CR chondrites, including a relatively high cosmic ray exposure age, the absence of a solar component, low 132Xe concentrations, a low trapped 36Ar/132Xe ratio of ?30, and a noticeable amount of radiogenic 129Xe. Similar attributes have been observed for some primitive achondrites. These attributes are also consistent with the metamorphic character of the sample. We, therefore, consider Tafassasset's noble gas record to be inconclusive as to its classification (primitive achondrite versus metamorphosed CR chondrite).  相似文献   

5.
Abstract– Enstatite chondrites (ECs) were subjected to noble gas analyses using stepped crushing and pyrolysis extraction methods. ECs can be classified into subsolar gas‐carrying and subsolar gas‐free ECs based on the 36Ar/84Kr/132Xe ratios. For subsolar gas‐free ECs, elemental ratios, and Xe isotopic compositions indicate that Q gas is the dominant trapped component, the Q gas concentration can be correlated with the petrologic type, reasonably explained by gas release from a common EC parental material during subsequent heating. Atmospheric Xe with sub‐Q elemental ratios is found in Antarctic E3s at 600–800 °C and through crushing. The 132Xe released in these fractions accounts for 30–60% of the bulk concentrations. Hence, the sub‐Q signature is generally due to contamination of elementally fractionated atmosphere. Subsolar gas is mainly released (up to 78% of the bulk 36Ar) at 1300–1600 °C and through crushing, suggesting that enstatite and friable phases are the host phases. Subsolar gas is isotopically identical to solar gas, but elementally fractionated. These observations are consistent with a previous study, which suggested that subsolar gas could be fractionated solar wind having been implanted into chondrule precursors ( Okazaki et al. 2001 ). Unlike subsolar gas‐free ECs, the primordial gas concentrations of subsolar gas‐carrying ECs are not simply correlated with the petrologic type. It is inferred that subsolar gas‐rich chondrules were heterogeneously distributed in the solar nebula and accreted to form subsolar gas‐carrying ECs. Subsequent metamorphic and impact‐shock heating events have affected noble gas compositions to various degrees.  相似文献   

6.
Abstract— The noble gases He, Ne, Ar, Kr, and Xe were measured in 27 individual Antarctic micrometeorites (AMMs) in the size range 60 to 250 μm that were collected at the Dome Fuji Station. Eleven of the AMMs were collected in 1996 (F96 series) and 16 were collected in 1997 (F97 series). One of the F97 AMMs is a totally melted spherule, whereas all other particles are irregular in shape. Noble gases were extracted using a Nd‐YAG continuous wave laser with an output power of 2.5‐3.5 W for ?5 min. Most particles released measurable amounts of noble gases. 3He/4He ratios are determined for 26 AMMs ((0.85‐9.65) × 10?4). Solar energetic particles (SEP) are the dominant source of helium in most AMMs rather than solar wind (SW) and cosmogenic He. Three samples had higher 3He/4He ratios compared to that of SW, showing the presence of spallogenic 3He. The Ne isotopic composition of most AMMs resembled that of SEP as in the case of helium. Spallogenic 21Ne was detected in three samples, two of which had extremely long cosmic‐ray exposure ages (> 100 Ma), calculated by assuming solar cosmic‐ray (SCR) + galactic cosmic‐ray (GCR) production. These two particles may have come to Earth directly from the Kuiper Belt. Most AMMs had negligible amounts of cosmogenic 21 Ne and exposure ages of <1 Ma. 40Ar/36Ar ratios for all particles (3.9–289) were lower than that of the terrestrial atmosphere (296), indicating an extraterrestrial origin of part of the Ar with a very low 40Ar/36Ar ratio plus some atmospheric contamination. Indeed, 40Ar/36Ar ratios for the AMMs are higher than SW, SEP, and Q‐Ar values, which is explained by the presence of atmospheric 40Ar. The average 38Ar/36Ar ratio of 24 AMMs (0.194) is slightly higher than the value of atmospheric or Q‐Ar, suggesting the presence of SEP‐Ar which has a relatively high 38Ar/36Ar ratio. According to the elemental compositions of the heavy noble gases, Dome Fuji AMMs can be classified into three groups: chondritic (eight particles), air‐affected (nine particles), and solar‐affected (eight particles). The eight AMMs classified as chondritic preserve the heavy noble gas composition of primordial trapped component due to lack of atmospheric adsorption and solar implantation. The average of 129Xe/132Xe ratio for the 16 AMMs not affected by atmospheric contamination (1.05) corresponds to the values in matrices of carbonaceous chondrites (?1.04). One AMM, F96DK038, has high 129Xe/132Xe in excess of this ratio. Our results imply that most Dome Fuji AMMs originally had chondritic heavy noble gas compositions, and carbonaceous chondrite‐like objects are appropriate candidate sources for most AMMs.  相似文献   

7.
Abstract Noble gases and N were analyzed in handpicked metal separates from lunar soil 68501 by a combination of step-wise combustions and pyrolyses. Helium and Ne were found to be unfractionated with respect to one another when normalized to solar abundances, for both the bulk sample and for all but the highest temperature steps. However, they are depleted relative to Ar, Kr and Xe by at least a factor of 5. The heavier gases exhibit mass-dependent fractionation relative to solar system abundance ratios but appear unfractionated, both in the bulk metal and in early temperature steps, when compared to relative abundances derived from lunar ilmenite 71501 by chemical etching, recently put forward as representing the abundance ratios in solar wind. Estimates of the contribution of solar energetic particles (SEP) to the originally implanted solar gases, derived from a basic interpretation of He and Ne isotopes, yield values of about 10%. Analysis of the Ar isotopes requires a minimum of 20% SEP, and Kr isotopes, using our preferred composition for solar wind Kr, yield a result that overlaps both of these values. It is possible to reconcile the data from these gases if significant loss of solar wind Ar, Kr and presumably Xe has occurred relative to the SEP component, most likely by erosive processes that are mass independent, although mass-dependent losses (Ar > Kr > Xe) cannot be excluded. If such losses did occur, the SEP contribution to the solar implanted gases must have been no more than a few percent. Nitrogen is a mixture of indigenous meteoritic N, whose isotopic composition is inferred to be relatively light, and implanted solar N, which has probably undergone diffusive redistribution and fractionation. If the heavy noble gases have not undergone diffusive loss, then N/Ar in the solar wind can be inferred to be at least several times the accepted solar ratio. The solar wind N appears, even after correction for fractionation effects, to have a minimum δ15N value ≥+150‰ and a more probable value ≥+200‰.  相似文献   

8.
Analysis of abundance patterns of rare gases Ne22, Ar36, Kr84 and Xe130 on Earth and in ordinary and carbonaceous chondrites is presented. A mechanism of chemical adsorption of rare gases at the planetesimal stage during their accretion is proposed to generate the abundance pattern of the heavy rare gases on the Earth. The calculated values for Xe and Kr agree well with the observed values whereas for Ar, the agreement is poor.  相似文献   

9.
Abstract— We investigated the characteristics and history of lunar meteorites Queen Alexandra Range 93069, Yamato 793169 and Asuka 881757 based on the abundances of all stable noble gas isotopes, the concentrations of the radionuclides 10Be, 26Al, 36Cl, and 81Kr, and the abundances of Mg, Al, K, Ca, Fe, Cl, Sr, Y, Zr, Ba, and La. Based on the solar wind and cosmic-ray irradiations, QUE 93069 is the most mature lunar meteorite studied up to now. The 40Ar/36Ar ratio of the trapped component is 1.87 ± 0.16. This ratio corresponds to a time when the material was exposed to solar and lunar atmospheric volatiles ～400 Ma ago. On the other hand, Yamato 793169 and Asuka 881757 contain very little or no solar noble gases, which indicates that these materials resided in the top layer of the lunar regolith only briefly or not at all. For all lunar meteorites, we observe a positive correlation of the concentrations of cosmic-ray produced with trapped solar noble gases. The duration of lunar regolith residence for the lunar meteorites was calculated based on cosmic-ray produced 21Ne, 38Ar, 78Kr, 83Kr, and 126Xe and appropriate production rates that were derived based on the target element abundances and the shielding indicator 131Xe/126Xe. For QUE 93069, Yamato 793169, and Asuka 881757, we obtained 1000 ± 400 Ma, 50 ± 10 Ma, and <1 Ma, respectively. Both Asuka 881757 and Yamato 793169 show losses of radiogenic 4He from U and Th decay and Yamato 793169 also 40Ar loss from K-decay. For Asuka 881757, we calculate a K-Ar gas retention age of 3100 ± 600 Ma and a 244Pu-136Xe fission age of 4240 ± 170 Ma. This age is one of the oldest formation ages ever observed for a lunar basalt. The exposure history of QUE 93069 after ejection from the Moon was derived from the radionuclide concentrations: ejection 0.16 ± 0.03 Ma ago, duration of Moon-Earth transit 0.15 ± 0.02 Ma and fall on Earth <0.015 Ma ago. This ejection event is distinguished temporally from those which produced the other lunar meteorites. We conclude that six to eight events are necessary to eject all the known lunar meteorites.  相似文献   

10.
Abstract— Elemental and isotopic compositions of the noble gases have been determined in six North American tektites (4 bediasites and 2 georgiaites) and one Ivory Coast tektite. Radiogenically produced 4He may explain the large 4He/36Ar ratios measured relative to air, despite significant diffusive losses. The Ne isotopic composition is enriched in 20Ne consistent with a single stage mass fractionation process. The enormous 20Ne/36Ar enrichments observed in all tektite samples, similar to those reported from other tektites and impact glasses, are attributed to atmospheric diffusion into the samples following solidification. The North American tektites show a systematic increase in 84Kr/36Ar and 132Xe/36Ar relative to air, with enrichments greater than those determined for any other tektite group or terrestrial samples other than shales. These enrichments are inconsistent with existing models of dissolving Kr and Xe in tektite glass without elemental fractionation at atmospheric pressures equivalent to ∼40 km altitude. The Kr and Xe isotopic compositions are indistinguishable from atmospheric within experimental uncertainty.  相似文献   

11.
Origin of the atmospheres of the terrestrial planets   总被引：1，自引：0，他引：1  
A.G.W. Cameron 《Icarus》1983,56(2):195-201
The monotonic decrease in the atmospheric abundance of 36Ar per gram of planet in the sequence, Venus, Earth, and Mars has been assumed to reflect some conditions in the primitive solar nebula at the time of formation of the planetary atmospheres, having to do either with the composition of the nebula itself or the composition of the trapped gases in small solid bodies in the nebula. Behind such hypotheses lies the assumption that planetary atmospheres steadily gain components. However, not only can gases enter atmospheres; they may also be lost from atmospheres both by adsorption into the planetary interior and by loss into space as a result of collisions with minor and major planetesimals. In this paper a necessarily qualitative discussion is given of the problem of collisions with minor planetesimals, a process called atmospheric cratering or atmospheric erosion, and a discussion is given of atmospheric loss accompanying collision of a planet with a major planetesimal, such as may have produced the Earth's Moon.  相似文献   

12.
Abstract— We have measured Ne, Ar, Kr and Xe in Si2O3 “smokes” that were condensed on Al substrates, vapor-deposited with various mixtures of CH4, NH3, H2O and noble gases at 10 K and subsequently irradiated with 1 MeV protons to simulate conditions during grain mantle formation in interstellar clouds. The noble gases were analyzed using conventional stepwise heating and static noble gas mass spectrometry. Neither Ne nor Ar is retained by the samples upon warming to room temperature, but Xe is very efficiently trapped and retained. Kr is somewhat less effectively retained, typically depleted by factors of about 10–20 relative to Xe. Isotopic fractionation favoring the heavy isotopes of Xe and Kr of about 5–10‰/amu is observed. Correlations between the specific chemistry of the vapor deposition and heavy noble gas retention are most likely the result of competition by the various species for irradiation-produced trapping sites. The concentration of Xe retained by some of these smokes exceeds that observed in phase Q of meteorites and, like phase Q, they do not seem to be carriers of the light noble gases. Such artificially prepared material may, therefore, offer clues concerning the incorporation of the heavy planetary noble gases in meteoritic material and the nature of phase Q.  相似文献   

13.
《Icarus》1986,66(2):195-210
A model for the selective loss of noble gases by thermal escape of the gases from planetesimals as they grow to form the terrestrial planets has been developed. The initial elemental and isotopic abundance ratios are assumed to be solar. Competition between gravitational binding and escape determines the degree of fractionation that occurs. Two classes of planetesimals can be formed on a time scale consistent with modern models of accretion. One class is depleted in neon and, in some cases, partly in 36Ar. The other class is neon rich. Subject to the validity of some assumptions regarding loss of planetary atmospheres following collisions between very large embryo planets and a strong radial dependence in the rate of accumulation of neon-rich planetesimals, the mechanism can account for all known properties of the noble gas volatiles on the terrestrial planets except one. This is the 36Ar/38Ar ratios for Earth and Mars which are predicted to be much lower than observed. This failure is probably fatal for the hypothesis.  相似文献   

14.
Abstract– Noble gas isotopic compositions were measured for a eucritic pebble and bulk material of a silicate–metal mixture from the Vaca Muerta mesosiderite as well as pyroxene and plagioclase separated from the eucritic pebble by total melting and stepwise heating methods. Trapped noble gases were degassed completely by a high‐temperature thermal event, probably at the formation of the Vaca Muerta parent body (VMPB). The presence of fissiogenic Xe isotopes from extinct 244Pu in the bulk samples might be a result of rapid cooling from an early high‐temperature metamorphism. High concentrations of cosmogenic noble gases enabled us to determine precise isotopic ratios of cosmogenic Kr and Xe. Spallogenic Ne from Na and unique Ar isotopic compositions were observed. The 81Kr‐Kr exposure age of 168 ± 8 Myr for the silicate pebble is distinctly longer than the age of 139 ± 8 Myr for the bulk samples. The precursor of the pebble had been irradiated on the surface of the VMPB for more than 60 Myr (first stage irradiation), with subsequent incorporation into bulk materials approximately 4 Gyr ago. The Vaca Muerta meteorite was excavated from the VMPB 140 Myr ago (second stage irradiation). Relative diffusion rates among the cosmogenic Ar, Kr, and Xe based on data obtained by stepwise heating indicate that Kr and Xe can be partially retained in pyroxene and plagioclase under the condition that resets the K‐Ar system. This result supports the presence of fission Xe and of excess concentration of cosmogenic Kr, which could have survived the thermal event approximately 3.8 Gyr ago.  相似文献   

15.
Abstract— Isotopic abundances of the noble gases were measured in the following Martian meteorites: two shock glass inclusions from Elephant Moraine (EET) 79001, shock vein glass from Shergotty and Yamato (Y) 793605, and whole-rock samples of Allan Hills (ALH) 84001 and Queen Alexandra Range (QUE) 94201. These glass samples, when combined with literature data on a separate single glass inclusion from EET 79001 and a glass vein from Zagami, permit examination in greater detail of the isotopic composition of Ne, Ar, Kr, and Xe trapped from the Martian atmosphere. The isotopic composition of Martian Ne, if actually present in these glasses, remains poorly defined. The 40Ar/36Ar ratio of trapped Martian atmospheric Ar is probably considerably lower than the nominal ratio of 3000 measured by Viking, and data on impact glasses suggest a value of ～1900. The atmospheric 36Ar/38Ar ratio is ≤4.0. Martian atmospheric Kr may be enriched in lighter isotopes by ～0.5%/amu compared to both solar-wind Kr and to the Martian composition previously reported. The isotopic composition of Xe in these glasses agrees with that previously reported in the literature. The Martian atmospheric 36Ar/132Xe and 84Kr/132Xe elemental ratios are higher than those reported by Viking by factors of ～2.5–1.6 (depending on the 40Ar/36Ar ratio adopted) and ～1.8, respectively, and are discussed in a separate paper. Cosmogenic gases indicate space exposure ages of 2.7 ± 0.6 Ma for QUE 94201 and Shergotty and 14 ± 1 Ma for ALH 84001. Small amounts of 21Ne produced by energetic solar protons may be present in QUE 94201 but are not present in ALH 84001 or Y-793605. The space exposure age for Y-793605 is 4.9 ± 0.6 Ma and appears to be distinctly older than the ages for basaltic shergottites. However, uncertainties in cosmogenic production rates still makes somewhat uncertain the number of Martian impact events required to produce the exposure ages of Martian meteorites.  相似文献   

16.
As planetary embryos grow, gravitational stirring of planetesimals by embryos strongly enhances random velocities of planetesimals and makes collisions between planetesimals destructive. The resulting fragments are ground down by successive collisions. Eventually the smallest fragments are removed by the inward drift due to gas drag. Therefore, the collisional disruption depletes the planetesimal disk and inhibits embryo growth. We provide analytical formulae for the final masses of planetary embryos, taking into account planetesimal depletion due to collisional disruption. Furthermore, we perform the statistical simulations for embryo growth (which excellently reproduce results of direct N-body simulations if disruption is neglected). These analytical formulae are consistent with the outcome of our statistical simulations. Our results indicate that the final embryo mass at several AU in the minimum-mass solar nebula can reach about ∼0.1 Earth mass within 107 years. This brings another difficulty in formation of gas giant planets, which requires cores with ∼10 Earth masses for gas accretion. However, if the nebular disk is 10 times more massive than the minimum-mass solar nebula and the initial planetesimal size is larger than 100 km, as suggested by some models of planetesimal formation, the final embryo mass reaches about 10 Earth masses at 3-4 AU. The enhancement of embryos’ collisional cross sections by their atmosphere could further increase their final mass to form gas giant planets at 5-10 AU in the Solar System.  相似文献   

17.
We report new data from Pesyanoe‐90,1 (dark lithology) on the isotopic signature of solar wind (SW) Xe as recorded in this enstatite achondrite which represents a soil‐breccia of an asteroidal regolith. The low temperature (≤800°C) steps define the Pesyanoe‐S xenon component, which is isotopically consistent with SW Xe reported for the lunar regolith. This implies that the SW Xe isotopic signature was the same at two distinct solar system locations and, importantly, also at different times of solar irradiation. Further, we compare the calculated average solar wind “SW‐Xe” signature to Chass‐S Xe, the indigenous Xe observed in SNC (Mars) meteorites. Again, a close agreement between these compositions is observed, which implies that a mass‐dependent differential fractionation of Xe between SW‐Xe and Chass‐S Xe is >1.5%o per amu. We also observe fractionated (Pesyanoe‐F) Xe and Ar components in higher temperature steps and we document a fission component due to extinct 244Pu. Interestingly, the Pesyanoe‐F Xe component is revealed only at the highest temperatures (>1200°C). The Pesyanoe‐F gas reveals Xe isotopic signatures that are consistent with lunar solar energetic particles (SEP) data and may indicate a distinct solar energetic particle radiation as was inferred for the moon. However, we cannot rule out fractionation processes due to parent body processes. We note that ratios 36Ar/38Ar≤5 are also consistent with SEP data. Calculated abundances of the fission component correlate well with radiogenic 40Ar concentrations, revealing rather constant 244Pu/K ratios in Pesyanoe, and separates thereof, and indicate that both components were retained. We identify a nitrogen component (δ15N = 44%o) of non‐solar origin with an isotopic signature distinct from indigenous N (δ15N = ?33%o). While large excesses at 128Xe and 129Xe are observed in the lunar regolith samples, these excesses in Pesyanoe are small. On the other hand, significant 126Xe isotopic excesses, comparable to relative excesses observed in lunar soils and breccias, are prominent in the intermediate temperature steps of Pesyanoe‐90,1.  相似文献   

18.
Abstract— Noble gases were measured in the Kapoeta achondrite by means of step-wise closed-system acid-etching with H2SO3. Isotopic ratios indicate that He, Ne and Ar are primarily solar in origin, although elemental abundance ratios indicate that the He and Ne have been significantly depleted relative to the Ar. Xenon is dominated by a typical trapped meteoritic component, and the same is probably true for Kr. The initial 11% of the Ar released from the sample by acid etching has a cumulative 36Ar/38Ar ratio of 5.58 ± 0.03, which indicates that the solar wind at some time in the past had a 36Ar/38Ar ratio significantly above previous values suggested for this ratio.  相似文献   

19.
Abstract— The Xe contents in 25 individual stratospheric interplanetary dust particles were measured in two different laboratories using focused laser micro‐gas extraction and (1) a conventional low‐blank magnetic sector mass spectrometer (Washington University), and (2) a resonance ionization time of flight mass spectrometer (RELAX‐University of Manchester). Data from both laboratories yielded a remarkably similar upper‐limit 132Xe concentration in the IDPs (>2.7, 6.8 and 2.2 × 10?8ccSTP/g for Washington University Run 1, Washington University Run 2 and University of Manchester analyses, respectively), which is up to a factor of five smaller than previous estimates. The upper‐limit 132Xe/36Ar ratio in the IDPs (132Xe/36Ar > ?8 × 10?4for Run 1 and 132Xe/36Ar > ?19 × 10?4for Run 2), computed using 36Ar concentration data reported elsewhere is consistent with a mixture between implanted solar wind, primordial, and atmospheric noble gases. Most significantly, there is no evidence that IDPs are particularly enriched in primordial noble gases compared to chondritic meteorites, as implied by previous work.  相似文献   

20.
Abstract— In this paper, we present concentration and isotopic composition of the light noble gases He, Ne, and Ar as well as of 84Kr, 132Xe, and 129Xe in bulk samples of 33 Rumuruti (R) chondrites. Together with previously published data of six R chondrites, exposure ages are calculated and compared with those of ordinary chondrites. A number of pairings, especially between those from Northwest Africa (NWA), are suggested, so that only 23 individual falls are represented by the 39 R chondrites discussed here. Eleven of these meteorites, or almost 50%, contain solar gases and are thus regolithic breccias. This percentage is higher than that of ordinary chondrites, howardites, or aubrites. This may imply that the parent body of R chondrites has a relatively thick regolith. Concentrations of heavy noble gases, especially of Kr, are affected by the terrestrial atmospheric component, which resides in weathering products. Compared to ordinary chondrites, 129Xe/132Xe ratios of R chondrites are high.  相似文献   

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