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1.
Five samples from historical lava flows on Mt. Etna, which had previously been used in a palaeointensity study, were examined using a combination of rock magnetic and microscopic techniques to elucidate the causes of failure of palaeointensity determination. The samples were characterised using a combination of low-temperature susceptibility (LT-), Bitter pattern imaging and scanning electron microscope (SEM). High-temperature susceptibility curves and hysteresis loops had been previously measured by Calvo et al. (2001). Of the five samples only one gave an accurate palaeointensity. This sample was deuterically oxidised and consisted of large exsolved ore grains. It was only possible to distinguish this sample either optically or magnetically from a similar sample by the LT- warming curves; the unsuccessful sample displayed alteration in the LT- warming curves, which was not readily observed in the high temperature susceptibility curves. It is proposed that the measurement of LT- curves before and after heating could be a more sensitive method of determining suitability for palaeointensity determination than previous rock magnetic pre-selection techniques.  相似文献   

2.
Low-temperature oxidation under atmospheric conditions affects the magnetic properties of magnetite in natural rocks: the coercivities of magnetite grains increase and other parameters change accordingly. It was recently shown that heating to 150°C largely removes the effects of low-temperature oxidation (van Velzen and Zijderveld, 1995). Heating may therefore serve as a detection tool for the presence of the effect of low-temperature oxidation. In the present study, a collection of loess and paleosol samples from various loess regions of the world is examined for the influence of low-temperature oxidation. In all samples of the collection a decrease of coercivities was found after heating to 150°C. Generally loess samples were affected to a larger extent than paleosol samples. The original range of remanent coercivities(B cr)of 21-58 mT changed to 20-42 mT after heating. The IRM capacity of the samples decreased from 0 up to 25%. ARM showed changes between a decrease of 10% and an increase of 15%. The grain-size indicative parameter IRM/ARM is considerably influenced by the heating and therefore by low-temperature oxidation. The changes in susceptibility are limited and will not influence the interpretation of large-scale features of the susceptibility record as a paleoclimate proxy. Small variations, however, may be obscured by the varying influence of oxidation in the outcrop, which can significantly modify the rock-magnetic record. Rock-magnetic parameters used to determine magnetic mineral content and grain sizes should be corrected for the effect of low-temperature oxidation. To this end heating to 150°C is recommended. The occurrence of the changes is in itself already an indication for the presence of magnetite. Low-temperature oxidation will not only be due to recent weathering in the outcrop, but also to earlier oxidation processes in the source area, during transport and deposition of the loess and during pedogenesis. Truly fresh sediment samples are only influenced by this earlier oxidation. In that case heating will reveal the degree of ancient low-temperature oxidation, which may be related to climate at the time of deposition and pedogenesis.  相似文献   

3.
Our study concerned magnetic properties of soil profiles taken from polluted regions of Eastern Ukraine around the industrial centres Krivyj Rig, Mariupol and Komsomolsk. Soils represent chernozem and podzoluvisol. The low-field magnetic susceptibility shows enhancement in the topsoil caused by contamination by coarse-grain magnetite connected with industrial pollution. Magnetic mineralogy was determined by means of thermal demagnetisation of SIRM, monitoring of susceptibility changes during warming from ?196°C to room temperature and heating to 700°C, and Mössbauer analysis. Granulometry of magnetic particles was investigated by determination of hysteresis parameters, susceptibility, M s , SIRM and ARM ratios and frequency dependence of susceptibility. The chemical parameters, namely pH, organic carbon and iron content in different pedogenic and lithogenic minerals, measured for particular horizons determined pedogenic characteristic of soil profiles. Our study showed that differences in magnetic parameters of non-polluted and polluted soil profiles are not limited to the topsoil, but reach deep layers of the parent material. Industrial pollution promotes formation of the so-called “pedogenic” SP and SD particles in these layers.  相似文献   

4.
Summary Using four samples of basaltic rocks from the Bohemian Massif, Nos 201, 202, 206 and 218, the curves of rotational moments in a magnetic field of 4 × 105 A/m were studied as a function of the degree of oxidation of titanomagnetites. The amplitudes of the individual harmonics were determined by harmonic analysis for samples oxidized to various degrees. It was found that the proportion of the harmonic A 1 withsin increases with the degree of oxidation. Simultaneously, the anisotropy of the magnetic susceptibility changes in a field of 60 A/m and the structure changes from linearly parallel to plane parallel.  相似文献   

5.
Magnetic susceptibility (MS) of natural specimens of hematite and goethite is studied under continuous heating with various additives: with carbon (sugar), nitrogen (carbamide), and elemental sulfur. It is found that heating of hematite with carbon above 450°C results in the formation of single-domain magnetite, while the magnetic susceptibility rises by a factor of 165. The increase in magnetic susceptibility on heating of hematite with nitrogen above 540°C reflects the generation of a single-domain maghemite with the Curie point of about 650°C, which is stable to heating. After the first heating, the magnetic susceptibility increases by 415 times. The subsequent cycle of thermal treatment results in the transition of maghemite to hematite, a decrease of MS, and an increase of coercivity. Heating with sulfur produces a stable single-domain magnetite at a temperature above the Curie point, which is manifested in the cooling curves. Here, the MS increases by a factor of 400. The heating curves for goethite exhibit a sharp drop in susceptibility to a temperature of 350–360°C, which reflects the transition of hematite to goethite. Heating of hematite with carbon produces stable maghemite at above 530°C, and with sulphur and nitrogen, it produces magnetite. When heated with pyrite, hematite reduces to magnetite under the action of sulfur released from pyrite.  相似文献   

6.
Magnetic Characteristics of Different Soil Types from Bulgaria   总被引：3，自引：0，他引：3  
Magnetic studies of different soil types can provide valuable information about palaeoenvironmental conditions at the time they were formed. Results of investigations of rock-magnetism of genetically different soil types, which developed over varying time intervals (Meadow Chernozem - formed during the last 6000 years BP; Leached Cinnamonic soil - formed since the 3rd-2nd century BC and Pellic Vertisoil - the oldest, formed since the Late Pliocene) are presented. The soil profiles of the Leached Cinnamonic and Pellic Vertisoil are characterized by lower values of magnetic susceptibility, as compared to that of the parent materials. It is shown that using percentage frequency-dependent susceptibility (Xfd%) and viscous remanent magnetization (VRM), pedogenic alteration could be detected even in such circumstances. The variations of the parameters measured along the depth of the studied Meadow Chernozem soil profile are characterized by gradual smooth magnetic enhancement, pointing to the absence of secondary redistribution of pedogenic magnetites. In contrast to this case, the two other profiles (Leached Cinnamonic and Pellic Vertisoil) show magnetically enhanced lower (illuvial) horizons due to processes of acid destruction and re-precipitation of the original pedogenic ferromagnetic minerals down the profiles. These specific magnetic properties are of particular importance in using susceptibility variations as a palaeoclimatic proxy record.  相似文献   

7.
Frequency-dependent magnetic susceptibility, its anisotropy (AMS), its temperature variation, natural remanent magnetization and time-dependent isothermal remanent magnetization as well as M?ssbauer spectroscopy of a small collection of Celtic and Mediaeval graphitic pottery from Southern Bohemia were investigated. The mineral composition of the pottery is dominated by fragments of quartz, accompanied mainly by various silicates from granitoids and paragneisses, or by calcite, within the plastic component being probably illite but also graphite. No ferrimagnetic minerals were found in optical microscope, among Fe-oxides only limonite was observed, even though the bulk susceptibility of the pottery varies in the orders of 10?4 to 10?2 [SI]. This may indicate presence of ferromagnetic particles in the ultrafine (superparamagnetic, SP) state, which is confirmed by frequency-dependent susceptibility ranging from 3% to almost 16%. The low temperature susceptibility vs. temperature curves are only moderately sloped, showing the Verwey transition only in one case. The high temperature curves mostly show presence of two magnetic phases, maghemite and magnetite. Cooling curves show distinctly lower susceptibilities than the heating curves indicating instability of the assemblage of ferrimagnetic minerals, particularly in temperatures slightly under 700 °C. M?ssbauer spectroscopy confirmed the results of the frequency-dependent susceptibility, showing the increase of ferrimagnetic sextets in the spectra measured at 4.2K, likely indicating maghemite as the distinct ferrimagnetic phase. The frequency-dependent AMS indicates preferred orientation of SP1,16 particles, coaxiality between SP1,16 grain AMS and whole specimen AMS indicate that all grains, ultrafine and coarser ones, were oriented by the same process, i.e. copying the pottery structure created during wheel-turning.  相似文献   

8.
Anisotropy of magnetic susceptibility (AMS) of the middle Tertiary Bloodgood Canyon and Shelley Peak Tuffs of the Mogollon-Datil volcanic field has been used to (1) evaluate the ability of AMS to constrain flow lineations in low-susceptibility ash-flow tuffs; (2) establish a correlation between magnetic fabric, magnetic mineralogy, tuff facies, and characteristics of the depositional setting; and (3) constrain source locations of the tuffs. The tuffs are associated with the overlapping Bursum caldera and Gila Cliff Dwellings basin. The high-silica Bloodgood Canyon Tuff fills the Gila Cliff Dwellings basin and occurs as thin outcrops outside of the basin. The older Shelley Peak Tuff occurs as thin outcrops both along the boundary between the two structures, and outside of the complex. AMS data were collected from 16 sites of Bloodgood Canyon Tuff basin fill, 19 sites of Bloodgood Canyon Tuff outflow, and 11 sites of Shelley Peak Tuff. Sites were classified on the basis of within-site clustering of orientations of principal susceptibility axes, based on the categories of Knight et al. (1986). Most microscopically visible oxide minerals in the Bloodgood Canyon Tuff outflow and basin fill, and in the Shelley Peak Tuff are members of the hematite-ilmenite solid solution series. However, IRM acquisition data indicate that Bloodgood Canyon Tuff basin fill and Shelley Peak Tuff have magnetic mineralogy dominated by single- or pseudo-single-domain magnetite, and that the magnetic mineralogy of the Bloodgood Canyon Tuff outflow is dominated by hematite. Hematite in Bloodgood Canyon Tuff outflow is likely to be the result of deuteric and/or low-temperature alteration of magnetite and iron silicate minerals. Bulk magnetic susceptibility is higher in magnetite-dominated ash-flow tuff (Bloodgood Canyon Tuff basin fill and Shelley Peak Tuff) than it is in hematite-dominated ash-flow tuff (Bloodgood Canyon Tuff outflow). Bloodgood Canyon Tuff outflow has the highest total anisotropy (H) of the three units, followed by Shelley Peak Tuff and Bloodgood Canyon Tuff basin fill. All three ash-flow tuffs are genearlly characterized by oblate susceptibility ellipsoids, with those of the Bloodgood Canyon Tuff basin fill nearest to spherical. At high values of total anisotropy, Shelley Peak Tuff susceptibility ellipsoids attain a prolate shape; those of Bloodgood Canyon Tuff outflow attain an increasingly oblate shape. Three factors may influence differences in total anisotropy and susceptibility ellipsoid shape: (1) ash which travelled the greatest distance before deposition may show the best development of magnetic fabric, particularly of magnetic lineation; (2) deposition of ash in a closed basin may inhibit laminar flow throughout the sheet and the resulting development of flow textures; and (3) replacement of magnetite and iron silicates preferentially oriented within the foliation plane by hematite with strong crystalline anisotropy may enhance the magnetic susceptibility within that plane. Scatter in AMS axis orientation within sites may result from: (1) greater orientation inaccuracy in block-sampled than in fielddrilled samples; (2) rheomorphism; and (3) low accuracy of AMS measurement in low-susceptibility ashflow tuffs. Evaluation of flow lineation based on AMS of sites with well-clustered K 1 axes indicates that (1) Bloodgood Canyon Tuff basin fill flowed along a generally northwest-southeast azimuth; (2) Shelley Peak Tuff located on the boundary of the Bursum caldera and the Gila Cliff Dwellings basin flowed along a nearly east-west azimuth; and (3) Bloodgood Canyon Tuff outflow sites have K 1 susceptibility axes generally radial to the Bursum-Gila Cliff Dwellings complex, but within-site scatter of K 1 orientations is generally too large to draw conclusions about flow lineation orientation. Limited petrographic work on pilot thin sections adds flow direction information to AMS-derived flow lineation information.  相似文献   

9.
Several events of anthropogenic impacts on the floodplain river sediments of the Danube along a section near the town of Oryakhovo (NW Bulgaria) have been detected using magnetic technique. In the field, magnetic susceptibility was measured using three susceptibility meters – MS2D, KT-5 and SM30. The differences in the surface susceptibility values measured with the different instruments are ascribed to the various penetration depths which depend on several parameters like sensor diameter, frequency and field strength. This is supported by the detailed laboratory study on penetration depth and sensitivity of the new SM30 susceptibility meter and the comparison with the already existing data for the other two sensors. Boundaries between different flooding events are clearly linked with significant variability of the measured susceptibility values corresponding to one and the same level. Sediment cores, taken at different distances from the water level, show the history of depositional events and corresponding degree of anthropogenic pollution. Identification of the magnetic phases responsible for the signal was carried out by means of thermomagnetic (T) curves. The main carrier is magnetite with Tc of 580°C or oxidized magnetite with Tc of 600°C. A second kink at about 300°C is better expressed for samples with lower susceptibilities. It may correspond to several minerals, e.g. maghemite, pyrrothite, titanomagnetite, as well as different mineral transformations of paramagnetic minerals (decomposition, dehydroxilation, etc. for example siderite, lepidocrocite). The samples showing strong magnetic enhancement are characterized by the predominance of magnetite. Optical microscopy on magnetic extracts shows the presence of small spherical particles, typical for the anthropogenic magnetic phases from high-temperature technological processes. Well expressed susceptibility variations along the cores suggest the presence of several stages of different degree of pollution, covering an estimated period of about 30 years.  相似文献   

10.
The relation of the maximal daily average values of the relativistic electron fluxes with an energy higher than 2 MeV, obtained from the measurements on GOES geostationary satellites, during the recovery phase of magnetic storms to the solar wind parameters and magnetospheric activity indices has been considered. The parameters of Pc5 and Pi1 geomagnetic pulsations and the relativistic electron fluxes during the prestorm period and the main phase of magnetic storms have been used together with the traditional indices of geomagnetic activity (A E, K p, D st). A simple model for predicting relativistic electron fluxes has been proposed for the first three days of the magnetic storm recovery phase. The predicted fluxes of the outer radiation belt relativistic electrons well correlate with the observed values (R ∼ 0.8–0.9).  相似文献   

11.
杭州城区土壤的磁性与磁性矿物学及其环境意义   总被引：18，自引：0，他引：18       下载免费PDF全文
对杭州城区四个不同功能区块土壤进行了系统的环境磁学测定,结果表明城市土壤的磁化率平均值为128×10-8m3·kg-1,频率磁化率平均值3.6%(样品数=182),城市土壤呈现明显的磁性增强. 城市土壤的磁化率与频率磁化率呈极显著指数负相关,表明城市土壤磁性增强明显区别于自然成土过程引起的以超顺磁性(SP)颗粒为主的表土磁性增强机理. 统计分析表明,城市土壤磁化率与软剩磁和饱和等温剩磁(SIRM)呈显著直线正相关,说明亚铁磁性矿物是城市土壤剩余磁性的主要载体. 综合等温剩磁获得曲线、热磁曲线、磁滞回线等岩石磁学测定和SEM/EDX分析,城市土壤的磁性矿物以磁铁矿和赤铁矿为主,磁性矿物以假单畴-多畴（PSD-MD）颗粒存在,粒度明显大于成土过程形成的磁性颗粒,这些磁性颗粒主要来自燃料燃烧、汽车尾气等环境污染物. 因此,城市土壤磁测可作为城市土壤污染监测、污染空间分布和污染物来源判断的新手段.  相似文献   

12.
The natural remanent magnetization of andesitic pumice emitted during the 1985 eruption of the Nevado del Ruiz volcano (Colombia) has a direction opposite to the present geomagnetic field. The self-reversing mechanism can be re-activated in the laboratory during cycles of heating and subsequent cooling in air and zero magnetic field. Laboratory-produced thermoremanent magnetization is dominated by the same self-reversal process in fields up to several mT. Microchemical, optical and Curie temperature analyses indicate that the ferromagnetic minerals are members of the magnetite-ulvöspinel and hematite-ilmenite series with average compositions of Fe2.73Ti0.27O4 and Fe1.38Ti0.62O3, respectively. In analogy with the magnetic behaviour of synthetically grown antiferromagnetic-ferromagnetic FeMn-FeNi films, the self-reversal can probably be interpreted in terms of an exchange field acting between a Ti-poor canted antiferromagnetic and a Ti-rich ferrimagnetic phase in the hemoilmenite grains.  相似文献   

13.
Existing activity indices (magnetic indices like AE, Kp, Dst or indices based on solar wind parameters) are poor predictors of the instantaneous magnetospheric configuration. We suggest a new activity index - the MT-index. It is defined as the invariant latitude of the isotropic boundary (IB) of \uparrow100 keV protons reduced to the midnight meridian. This IB is a low-altitude signature of the boundary between regions of adiabatic and chaotic regimes of particle motion in the tail current sheet which is controlled by the magnetic field in the equatorial near-Earth tail (at 5-10Re). We have investigated the local time and activity dependence of the IB latitude based on data from about 2000 orbits of NOAA spacecraft. By finding the formula to reduce the IB latitude to midnight meridian, we then evaluate the accuracy of the derived index. We compared the MT-index with the magnetic field measured simultaneously by geosynchronous GOES-2 spacecraft and showed that, unlike the traditional indices, the MT-index displays a good correlation (r\uparrow0.9) with the magnetic field inclination in the nightside portion of the geosynchronous orbit. It is, thus, a good measure to characterize quantitatively the tailward stretching of the tail magnetic field. Based on the measured MT value, a simple numerical procedure is suggested to choose the version of the T89 magnetospheric model. We conclude that the MT-index is the best known predictor of the instantaneous magnetic configuration in the near-Earth magnetotail. It may be available on a regular basis and can be implemented for scientific studies.  相似文献   

14.
At moderate temperatures, the elastic properties of natural MgAl2O4 spinel differ in several significant ways from properties of synthetic spinels. Below 1000 K, the ultrasonic resonant frequencies of an ordered natural spinel change significantly after heat treatment; at higher temperatures, both types of spinels have similar resonant responses. The temperature derivatives of the elastic constants of an ordered spinel also differ from those of disordered spinels at moderate temperatures; again, at higher temperatures, both types of spinels have similar behaviors. The Raman spectra also differ below 1000 K for ordered natural and disordered spinels and are similar at higher temperatures and after cooling to ambient temperature. We associate these changes in ultrasonic resonance and Raman spectra of spinel with cation disordering at high temperature which may be quenched by cooling. We deduce estimates of the inversion parameter from the relative intensities of the two A1g Raman modes in very good agreement with estimates made from other measurements. We find thatC 11 andC 12 decrease by 4 and 8%, respectively, with 20% inversion in spinel;C 44 is less sensitive to cation order. These results imply that previous measurements of the adiabatic elastic constants of spinels at ambient conditions have been affected by the state of cation disorder of the specimen.  相似文献   

15.
北京房山岩体的磁组构特征及其 对岩体侵位的约束   总被引：3，自引：0，他引：3       下载免费PDF全文
岩浆岩的磁组构与岩浆流动、侵位时应力和冷凝后遭受后期构造改造作用有关.本文分析了北京房山岩体东山口-凤凰亭剖面岩石磁化率各向异性(AMS)变化.热磁曲线和磁滞回线分析显示,岩石的主要载磁矿物为多畴磁铁矿颗粒.AMS磁化率椭球体呈压扁状,磁面理发育且产状陡倾,磁化率各向异性度P值平均值高达1.189.自边缘相(东山口)到中心相(凤凰亭),岩石磁化率椭球的扁率E值和形状因子T值逐渐减小,说明磁组构主要反映岩浆流动和岩体侵位时近NNE-SSW方向的挤压作用,在侵位冷凝后并没有遭受到明显的构造改造.  相似文献   

16.
In the past the global, fully coupled, time-dependent mathematical model of the Earths thermo-sphere/ionosphere/plasmasphere (CTIP) has been unable to reproduce accurately observed values of the maximum plasma frequency, foF2, at extreme geophysical locations such as the Argentine Islands during the summer solstice where the ionosphere remains in sunlight throughout the day. This is probably because the seasonal dependence of thermospheric cooling by 5.3 m nitric oxide has been neglected and the photodissociation of O2 and heating rate calculations have been over-simplified. Now we have included an up-to-date calculation of the solar EUV and UV thermospheric heating rate, coupled with a new calculation of a diurnally varying O2 photodissociation rate, in the model. Seasonally dependent 5.3 m nitric oxide cooling is also included. With these important improvements, it is found that model values of foF2 are in substantially better agreement with observation. The height of the F2-peak is reduced throughout the day, but remains within acceptable limits of values derived from observation, except at around 0600 h LT. We also carry out two studies of the sensitivity of the upper atmosphere to changes in the magnitude of nitric oxide cooling and photodissociation rates. We find that hmF2 increases with increased heating, whilst foF2 falls. The converse is true for an increase in the cooling rate. Similarly increasing the photodissociation rate increases both hmF2 and foF2. These changes are explained in terms of changes in the neutral temperature, composition and neutral wind.  相似文献   

17.
Magnetic parameters and their environmental implications of sediments in a core (PD) from the Pearl River Delta, South China, indicate that ferrimagnetic minerals with low coercivity, such as magnetite, dominate the magnetic properties although small amounts of Fe-sulphides occur. The fraction of Fe-sulphides increases and becomes the dominant minerals determining the magnetic characteristics in grey-black organic-rich clay horizons, indicating an anoxic, sulphate-reducing swamp environment resulting from a marine regression. In the "Huaban clay" , hard magnetic minerals, such as hematite and goethite, largely control the magnetic properties of the sediments and imply a long period of exposure and weathering. Where magnetite is the main magnetic mineral, its fraction and grain size determine properties such as magnetic susceptibility (κ ) and saturation isothermal remanent magnetization (SIRM). Ratios of SIRM/κ and χarm/SIRM reflect changes in sea level with high SIRM/κ and χarm/SIRM correlating with a smaller magnetic mineral grain size and rising sea level. Based on downcore variations of these environmental magnetic parameters along with sediment characteristics and microfauna, the sedimentary environment of the Pearl River Delta area can be divided into two main cycles of transgression and regression during the late Pleistocene and Holocene with more sub-cycles of sea level fluctuation during each transgression.  相似文献   

18.
Abstract

The heat transfer by a rotating, differentially-heated annulus of fluid is measured throughout the high amplitude wave regime. Only Δrw T was varied (although v(T15 ).K(T15 ) varied by 46%), and it is found that Nu = C1(λ)Ra? away from the symmetry and low amplitude to wave transition curves and this is independent of ω. (λ is the wavelength.) On the wave side of these transition curves a region exists in which Nu (symmetry) λ Nu λ C1(λ)Ra?. The local heat transfer rate also varies strongly with wave phase.

Using a selection of measured internal thermal fields in the steady, high amplitude wave regime, the side-wall thermal boundary layer structure is examined. It is found that Nu, = C2·Gr2 A2; both C 2 and A 2 are independent of ω and λ to first order. For the time mean profiles, A 2 ≈ 0.25; in the high heat transfer portion of the wave A 2 < ¼ and in the low heat transfer portion of the wave A 2 > ?. These relations hold over most of the vertical extent of the side walls. The deviations of the boundary layers from the above behavior which occur on the remainder of the walls is illustrated. The average thicknesses of the wall boundary layers ∞ Ra?¼ except in that phase of the wave in which the wall to mid-gap temperature difference is the largest.  相似文献   

19.
During revisiting the Upper Pleistocene Pekla loess-soil section located on the Sea of Azov coast of the Taman Peninsula, its lower 6 m were continuously sampled, which led to an increase in the age range from ∼50 to 400 ka. The detailed rock magnetic study of the structure, grain-size, and concentrations of magnetic mineral (natural remanent magnetization (NRM) carrier) in the collected rock samples revealed regular changes in rock magnetic characteristics along the section and their correlation with climatic fluctuations. Magnetite and hematite both deposited during the transport of sedimentary material and formed during pedogenesis, which involved the entire section to a varying extent, represent the main magnetic minerals in the examined rocks. Automorphic paleosoils that were formed during warm and humid periods corresponding to odd stages of the MIS scale are characterized by elevated concentrations of magnetic mineral (NRM, magnetic susceptibility (K lf), saturation isothermal remanent magnetization (SIRM), and anhysteresis (ideal) remanent magnetization (ARM)) parameters and share of superparamagnetic particles (up to 80%, according to elevated values of the frequency-dependent magnetic susceptibility K td) as well as by lowered rigidity parameter (B cr) and grain size (ARM/K parameter). Such changes in the paleosoils may be explained by the occurrence of newly formed fine-grained magnetite particles close in size to its superparamagnetic and single-domain varieties due to the activation of bio/geochemical processes during warm stages. The growth of the above-mentioned rock magnetic parameters in automorphic soils may be considered as serving a quantitative criterion for defining the boundary between warm and cold periods even in poorly developed soils.  相似文献   

20.
This study reports systematic analysis of air pollution concentration by particulate matter (PM) in relation to annual changes of metrological conditions. The concentration of PM collected on filters was evaluated by magnetic properties. Long series of filters collected during 1977, 1980, 1981 and 1985 in Warsaw have been used for measurement. Such long time series allowed a better determination of correlation between seasonal susceptibility changes and meteorological conditions and to verify the repeatability of annual behavior. The magnetic susceptibility normalized by mass (??) has been used as a proxy of pollution. Monthly variations of ?? (??m) demonstrated slow and small seasonal changes disturbed by quick, high peaks. The filters with high susceptibilities contain a mixture of magnetic single and multidomain grains which is characteristic for anthropogenic pollution, with the frequency-dependent susceptibility ??fd being less than 4%. The low susceptibility samples are characterized by admixture of small amount of pseudo-single domain (PSD) and possible small amount of superparamagnetic (SP) grains. Detailed analysis of reduced mean monthly susceptibility ??R revealed that temperature and absolute humidity correlate positively in cold period of year and negatively in warm months. The linear correlation coefficients range from 0.7 to 0.9 and from 0.3 to 0.4 for negative and positive linear correlation, respectively. The dispersion of pollutants in a city depends on the way of ventilation. The big cities like Warsaw are urban heat islands which act the most effective way for the warm period and for the cold time. The correlation of ??R with absolute humidity is similar to that for temperature but for different reasons. The presence of big amount of water vapor particles in the atmosphere can favor the adhesion of smaller ferromagnetic grains to their surface which can accelerate the process of falling down of such agglomerates. Such a process can take place during wintertime. We do not observe clear correlation between ??R and precipitation.  相似文献   

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