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1.
The occurrence of estrogens in the aquatic environment has become a major concern worldwide because of their strong endocrine disrupting potency. In this study, concentrations of four estrogenic compounds, estrone (E1), 17β-estradiol (E2), 17α-ethynylestradiol (EE2), estriol (E3) were determined with liquid chromatography-tandem mass spectrometry analyses in surface water from South China Sea, and distributions and potential risks of their estrogenic activity were assessed. The estrogenic compounds E1, E2 and E3 were detected in most of the samples, with their concentrations up to 11.16, 3.71 and 21.63 ng L−1. However, EE2 was only detected in 3 samples. Causality analysis, EEQ values from chemical analysis identified E2 as the main responsible compounds. Based on the EEQ values in the surface water, high estrogenic risks were in the coastal water, and low estrogenic risks in the open sea.  相似文献   

2.
The range of relative sea level rise in the northwestern South China Sea since the Last Glacial Maximum was over 100 m. As a result, lowland regions including the Northeast Vietnam coast, Beibu Gulf, and South China coast experienced an evolution from land to sea. Based on the principle of reconstructing paleogeography and using recent digital elevation model, relative sea level curves, and sediment accumulation data, this paper presents a series of paleogeographic scenarios back to 20 cal. ka BP for the northwestern South China Sea. The scenarios demonstrate the entire process of coastline changes for the area of interest. During the late glacial period from 20 to 15 cal. ka BP, coastline slowly retreated, causing a land loss of only 1×104 km2, and thus the land-sea distribution remained nearly unchanged. Later in 15–10 cal. ka BP coastline rapidly retreated and area of land loss was up to 24×104km2, causing lowlands around Northeast Vietnam and South China soon to be underwater. Coastline retreat continued quite rapidly during the early Holocene. From 10 to 6 cal. ka BP land area had decreased by 9×104km2, and during that process the Qiongzhou Strait completely opened up. Since the mid Holocene, main controls on coastline change are from vertical crustal movements and sedimentation. Transgression was surpassed by regression, resulting in a land accretion of about 10×104km2. Supported by Key Laboratory of Marginal Sea Geology, Chinese Academy of Sciences (Grant No. MSGL0711), the Guangdong Natural Science Foundation (Grant No. 04001309) and Open Fund of the Key Laboratory of Marine Geology and Environment, Chinese Academy of Sciences (Grant No. MGE2007KG04)  相似文献   

3.
Sea fog is typically formed and developed under a set of favorable environmental conditions, which are associated with the station pressure changes, sea level pressure, winds, temperature, water vapor supply, and sea surface temperature. Understanding of these environmental factors during the evolution of a sea fog episode is crucial for forecasting the occurrence and severity of sea fogs over the ocean and adjacent coastal areas. In this study, the large-scale environment variability of six fog events over the Yellow Sea was investigated. It was realized in the present study that the northwest Pacific Ocean high (NPH) is vital to fog formation over the Yellow Sea. In our study, six fog cases can be basically divided into two types: (1) pressure-weakening type, (2) pressure-strengthening type. The former type happened in spring and the latter type in summer. Prevailing southerly winds, accompanied with the well-positioned NPH, may supply a large amount of warm water vapor for the fog formation and maintenance. The intensity of the air temperature inversion is stronger in summer cases than that in spring ones. The wind direction change from south to north and the unstable lower atmosphere may lead to fog’s dissipation. This study may provide a comprehensive understanding of sea fog’s onset, maintenance, and dissipation over the Yellow Sea.  相似文献   

4.
Radium-226 (226Ra) activities were measured in the surface water samples collected from the Arctic Ocean and the Bering Sea during the First Chinese National Arctic Research Expedition. The results showed that 226Ra concentrations in the surface water ranged from 0.28 to 1.56 Bq/m3 with an average of 0.76 Bq/m3 in the Arctic Ocean, and from 0.25 to 1.26 Bq/m3 with an average of 0.71 Bq/m3 in the Bering Sea. The values were obviously lower than those from open oceans in middle and low latitudes, indicating that the study area may be partly influenced by sea ice meltwater. In the Bering Sea, 226Ra in the surface water decreased northward, probably as a result of the exchange between the 226Ra-deficient sea ice meltwater and the 226Ra-rich Pacific water. In the Arctic Ocean, 226Ra in the surface water increased northward and eastward. This spatial distribution of 226Ra reflected the variation of the 226Ra-enriched river component in the water mass of the Arctic Ocean. The vertical profiles of 226Ra in the Canadian Basin showed a concentration maximum at 200 m, which could be attributed to the inputs of the Pacific water or/and the bottom shelf water with high 226Ra concentration. This conclusion was consistent with the results from 2H, 18O tracers.  相似文献   

5.
A detailed stable isotopic study based on benthic foraminifera from 1165 samples of ODP Site 1148 (18° 50.17.3’N, 116° 33.93’E, water depth 3308.3 m), northern South China Sea, provides an excellent oxygen isotopic record with an average resolution of 30 ka. It contains the most continuous δ18O data with highest resolution for the whole Neogene sequence in the world. The δ18O curve shows a step-like increasing upwards and records 5 increases, 3 decreases and 2 stable stages during the Neogene, reflecting the general trend of global cooling. Among these events the δ18O decrease at 17.2–14.5 Ma, and two δ18O increases at 14.5-13.6 and 3.0-2.4 Ma are most marked and globally comparable. The intervals at 13.6-10.2 and 6.0-3.0 Ma with the lowest-amplitude and least fluctuation in δ18O represent the most stable bottom water periods for the South China Sea.  相似文献   

6.
Based on the stable isotopic analysis of more than 1000 samples of planktonic and benthic foraminifers from ODP Site 1148 in the northern South China Sea (SCS), the oxygen isotope stratigraphy has been applied to the last 3 million years for the first time in the SCS. Furthermore, the paleoceanographic changes in the northern SCS during the last 6 million years have been unraveled. The benthic foraminiferal δ18O record shows that before δ3.1 Ma the SCS was much more influenced by the warm intermediate water of the Pacific. The remarkable decrease in the deepwater temperature of the SCS during the period of 3.1-2.5 Ma demonstrates the formation of the Northern Hemisphere ice-sheet. However, the several sea surface temperature (SST) reductions during the early and middle Pliocene, reflected by the planktonic foraminiferal δ18O, might be related to the ice-sheet growth in the Antarctic region. Only those stepwise and irreversible SST reductions during the period of δ2.2-0.9 Ma could be related to the formation and growth of the Northern Hemisphere ice-sheet.  相似文献   

7.
The most important source of dissolved manganese, Mn(II), to the Dead Sea is by upward diffusion from bottom sediments. This source contributes about 80 tons of Mn(II) each year. The concentration of dissolved manganese in the Dead Sea is extraordinarily high (7.03 mg 1?1). It appears that the content (some 1.026 × 106 tons) of dissolved manganese in the sea has remained constant during 1977–1979, although oxygen was introduced into deeper layers during the deepening of the pycnocline (1977–1978) and during the overturn of its water masses in the winter of 1978/79. The rate of oxidation of Mn(II) in Dead Sea water is extremely slow hence Mn(II) may practically be considered as the stable form of Mn in Dead Sea waters. Dilution by fresh water causes a pH rise and may facilitate faster oxidation of the dissolved divalent manganese. It is shown here that the shape of the Mn(II) profile, observed in the lake during 1963, may have developed by oxidation of Mn(II) in the more diluted upper layers and subsequent reduction of the oxidation products in the anoxic and more saline deeper layers during 260 years of continuous meromixis.  相似文献   

8.
The effect of monsoon, coastal current and temperature on the distribution and seasonal variations of Calanus sinicus abundance were studied. The samples from the northwest continental shelf of South China Sea were collected with 505 μm planktonic nets from July 2006 to October 2007. The abundance of C. sinicus made up 34.28% and 12.34% of all copepods in spring and summer, respectively. The distribution of C. sinicus varied seasonally and regionally. The distribution of C. sinicus ranged between east inshore and offshore waters from the Leizhou Peninsula to Hainan Island, with a mean of 23.00 (±77.78) ind. m−3 in spring. In summer it had a mean of 13.74 (±45.10) ind. m−3 occurring only in the east inshore waters from Leizhou Peninsula to Hainan Island. C. sinicus was not abundant during autumn and winter seasons. The surveyed area was divided into three sub-regions based on topographical analysis and water mass, region I (included the east inshore waters of Leizhou Peninsula), region II (included the east inshore waters of Hainan Island) and region III (included the offshore waters from Leizhou Peninsula to Hainan Island). The average abundance of C. sinicus within region I was determined to be 115.63 (±145.93) and 68.12 (±84.00) ind. m−3 in spring and summer, respectively, values higher than those of regions II and III. Our findings suggested that C. sinicus was transported from the East China Sea to the northwest continental shelf of South China Sea by the Guangdong Coastal Current, which was driven by the northeast monsoon in spring. The presence of a cold eddy, in addition to coastal upwelling driven by the southwest monsoon, provided suitable survival conditions for C. sinicus in summer. This species disappeared in autumn due to high temperatures (>27 °C) and did not begin to enter into the northwest continental shelf of South China Sea from the East China Sea during the period of investigation in winter. The frequency of C. sinicus was low in region III during the year as a result of the South China Sea Warm Current and pelagic waters with high temperature during the spring and summer months.  相似文献   

9.
Sediment components and their fluxes of Cores MD12-3428(water depth: 903 m), MD12-3433(water depth: 2125 m),and MD12-3434(water depth: 2995 m), obtained along a transect on the continental slope of the northern South China Sea, have been conducted to reveal the spatiotemporal variations and the controlling factors of the sediment components and of their fluxes.Results show that deep-sea sediments in the northern South China Sea are composed mainly of terrigenous(59–89%) and carbonate(6–38%) particles, with minor components of opal(1.6–9.4%) and organic matter(0.7–1.9%). Fluxes of terrigenous and carbonate particles reach up to 2.4–21.8 and 0.4–6.5 g cm–2 kyr–1, respectively, values that are one to two orders of magnitude higher than the fluxes of opal and organic matter. Temporal variations of the percentages and fluxes of deep-sea sediment components have displayed clear glacial-interglacial cyclicity since the last glaciation. Terrigenous, opal, and organic matter percentages and their fluxes increas clearly during marine isotope stage 2, while carbonate percentages and fluxes show an opposite variation pattern or are characterized by an unremarkable increase. This implies that deep-sea carbonate in the South China Sea is affected by the dilution of terrigenous inputs during the sea-level lowstand. With increasing water depth along the transect, the terrigenous percentage increases but with largely decreased fluxes. Both the percentage and flux of carbonate decrease, while the percentages and fluxes of opal and organic matter display much more complicated variational features. The spatiotemporal variations of deep-sea sediment components and of their fluxes since the last glaciation in the northern South China Sea are strongly controlled by sea-level fluctuations. Simultaneously, terrigenous supply associated with monsoonal rainfall, marine primary productivity,and the dilution effect between terrigenous and biogenic particles, also play interconnected roles in the sediment accumulation processes.  相似文献   

10.
The high-resolution quantitative analysis of the planktonic foraminifera and the δ18O records of the section between 96.49– 137.6 mcd at ODP Site 1144 on the continental slope of northern South China Sea reveals an abrupt cooling event of sea surface temperature (SST) during the last interglacial (MIS 5.5, i.e. 5e). The dropping range of the winter SST may come to 7.5°C corresponding to 1.2‰ of the δ18O value of sea surface water. This event is comparable with those discovered in the west Europe and the northern Atlantic Ocean, but expressed in a more intensive way. It is inferred that this event may have been induced by middle- to low-latitude processes rather than by polar ice sheet change. Since the Kuroshio-index speciesPulleniatina obliquiloculata displayed the most distinct change at the event, it may also be related to the paleoceanographic change of the low-latitude area in the western Pacific Ocean. This event can be considered as one of “Younger Dryas-style coolings” and is indicative of climate variability of the last interglacial stage.  相似文献   

11.
The surface water of the Japan Sea contained226Ra of70 ± 4dpm m−3 which was nearly equal to that of the surface water in the North Pacific. The concentration of226Ra in the Japan Sea deep water below 500 m was151 ± 8dpm m−3, showing a vertically and regionally small variation. This concentration of226Ra in the deep water is unexpectedly high, because the Japan Sea deep water has a higher Δ14 C value by about 50‰ than the Atlantic deep water containing the same226Ra. One of the causes to be considered is larger contribution of226Ra from biogenic particles dissolving in the Japan Sea deep water, but the Japan Sea is not so fertile in comparison to the Bering Sea. The other more plausible cause is the internal ventilation of the Japan Sea water, which means that the residence time of the Japan Sea Proper water is considerably long although the water is vertically mixed fairly well especially in winter. The ventilation may supply some amounts of radiocarbon and oxygen but does not change the inventory of226Ra. The residence times of the Japan Sea deep water and of water within the Japan Sea are calculated by solving simultaneous equations for226Ra and14C with a three-box model to be 300–400 years and 700–1000 years, respectively.  相似文献   

12.
A typical area, Gaomi City in China, was chosen to discuss the enrichment process of groundwater fluorine in sea water intrusion area. The groundwater had fluorine levels of 0.09–10.99 mg/L, with an average concentration of 1.38 mg/L. The high-fluorine groundwater was mainly distributed in the unconsolidated Quaternary sediments, where concentrations in 83.6% of the samples exceeded the national limit of 1.0 mg/L. The groundwater in the Quaternary sediments also had higher levels of Cl−, TDS, Mg2+, and pH and lower levels of Ca2+, Co, Ni, and Cu than that in the bedrock. The groundwater fluorine levels in the Quaternary sediments are positively correlated with Cl−, TDS, Mg2+, pH, and negatively correlated with Ca2+, γCa2+/γMg2+, Co, Ni, Cu. Geochemical indices of Cl− and TDS indicate sea water intrusion in the Quaternary high-fluorine groundwater area (F− > 1.0 mg/L), while they do not indicate any intrusion in the bedrock area. The chemical weathering of minerals was intensified with the intrusion of sea water. Cation exchange was confirmed to occur in the Quaternary sediments and was promoted by sea water intrusion. Cation exchange consumes part of groundwater Ca2+ and permits more F− dissolving. Consequently, in the Quaternary sediments, the groundwater was supersaturated with CaF2 minerals and undersaturated with MgF2 minerals when F− > 1.0 mg/L, while CaF2 and MgF2 minerals both are undersaturated when F− < 1.0 mg/L. Thus, the chemical weathering of minerals and cation exchange caused by sea water intrusion are the crucial processes controlling the groundwater fluorine levels, which should be considered when the groundwater fluorine enrichment mechanism is discussed along coastal zones.  相似文献   

13.
Strontium, neodymium isotopic compositions and trace elements of the detrital sediments of Core NS90-103 from South China Sea were analyzed. The results show that the87Sr/86Sr ratios of the detritus during the last glacial range from 0.722 4 to 0.723 0. They are significantly higher than those during the Holocene and the maximum of the last interglacial, which range from 0.721 0 to 0.721 7. This indicates stronger continental weathering during the last glacial. On the other hand, the143Nd/144Nd ratios of these detritus are higher during the last glacial too, similar to the variation of the87Sr/86Sr ratios. The trace element geochemistry of these detritus indicates that more authigenic sediments, such as ferromanganese, during the last glacial may partly contribute to the increase of143Nd/144Nd ratios. Furthermore, much more detritus from continent of South China to the north of the South China Sea may probably contribute to143Nd/144Nd ratios increase during the last glacial, which was the result of the enhancement of northeast monsoon.  相似文献   

14.
中国近海海平面变化特征分析   总被引：6，自引：1，他引：5       下载免费PDF全文
用经验正交函数分析方法,对中国近海14年多的测高海平面同化格网资料进行分析,给出了黄海、东海和南海各海平面变化主要主成分的空间变化和时间变化特征.用标准Morlet小波变换方法分析了各海区主成分时间变化序列的时频特征.分析结果表明,各主成分的空间分布特征与当地的海洋环流或洋流特征相对应.时频分析结果显示,中国近海海平面变化的显著周期主要为年周期信号.其次,黄海和东海还显示准2个月的非稳态信号,东海和南海具有较显著的半年周期信号,东海半年周期信号的能量不稳定.此外,在南海及台湾东部海域,首次发现存在较为显著的准540天周期信号,其动力学机制目前尚不明确.坎门和西沙验潮站资料的时频特征分析也验证了该信号的存在.最后本文给出了中国近海海平面在1993~2007年间的平均上升速率和其区域分布特征.  相似文献   

15.
Measurement of228Ra activities in the upper 300 m water column was conducted at two stations in the South China Sea using an MnO2-fiber extraction/β-counting technique of228Ac. Results showed that228Ra activities ranged from 0.38 to 3.60 Bq · m-3. The vertical profiles of228Ra at the time-series station favored a steady state assumption. Based on a one-dimensional steady state model,228Ra-nitrate coupled approach was applied to stations NS97-43, NS99-53 (T1), NS99-53 (T2). New production thus quantified were 4.4, 5.1 and 5.7 mmolC · m-2 · d-1, respectively,f ratios in the South China Sea were estimated from the derived new production and the documented primary productivity in the regime, to be 0.12–0.15.  相似文献   

16.
Fog is an atmospheric phenomenon that has important environmental consequences related to visibility, air quality and climate change on local and regional scales. The formation of radiation fog results from a complex balance between surface radiative cooling, turbulent mixing in the surface layer, aerosol growth by deliquescence and activation of fog droplets. During the ParisFog field experiment, out of 16 events forecasted for radiation fog, activated fog materialized in seven events, while in five other events the visibility dropped to 1–2 km but haze particle size remained below the critical size of activation. To better understand the conditions that lead to or do not lead to sustained fog droplet activation, we performed a comparative study of dynamic, thermal, radiative and microphysical processes occurring between sunset and fog (or quasi-fog) onset. We selected two radiation fog events and two quasi-radiation fog events that occurred under similar large-scale conditions for this comparative study. We identified that aerosol growth by deliquescence and droplet activation actually occurred in both quasi-fog events, but only during <1 h. Based on ParisFog measurements, we found that the main factors limiting sustained activation of droplets at fog onset in the Paris metropolitan area are (1) lack of mixing in the surface layer (typically wind speed <0.5 ms?1), (2) relative humidity exceeding 90 % throughout the residual layer, (3) low cooling rate in the surface layer (typically less than ?1 °C per hour on average) due to weak radiative cooling (0 to ?30 Wm?2) and near zero sensible heat fluxes, and (4) a combination of the three factors listed above during the critical phase of droplet activation preventing the transfer of cooling from the surface to the liquid layer. In addition, we found some evidence of contrasted aerosol growth by deliquescence under high relative humidity conditions in the four events, possibly associated with the chemical nature of the aerosols, which could be another factor impacting droplet activation.  相似文献   

17.
The South China Sea is a large marginal sea surrounded by land masses and island chains, and characterized by complex bathymetry and irregular coastlines. An unstructured-grid SUNTANS model is employed to perform depth-averaged simulations of the circulation in the South China Sea. The model is tidally forced at the open ocean boundaries using the eight main tidal constituents as derived from the OSU Tidal Prediction Software. The model simulations are performed for the year 2005 using a time step of 60 s. The model reproduces the spring-neap and diurnal and semidiurnal variability in the observed data. Skill assessment of the model is performed by comparing model-predicted surface elevations with observations. For stations located in the central region of the South China Sea, the root mean squared errors (RMSE) are less than 10 % and the Pearson’s correlation coefficient (r) is as high as 0.9. The simulations show that the quality of the model prediction is dependent on the horizontal grid resolution, coastline accuracy, and boundary locations. The maximum RMSE errors and minimum correlation coefficients occur at Kaohsiung (located in northern South China Sea off Taiwan coast) and Tioman (located in southern South China Sea off Malaysia coast). This may be explained with spectral analysis of sea level residuals and winds, which reveal dynamics at Kaohsiung and Tioman are strongly influenced by the seasonal monsoon winds. Our model demonstrates the importance of tidally driven circulation in the central region of the South China Sea.  相似文献   

18.
通过对南海北部陆坡下部ODPl148站位沉积物中陆源矿物组分的含量、堆积速率、粒度、石英氧同位素及石英扫描电镜的分析,探讨南海沉积演化及其构造响应.结果显示,根据综合指标的变化特征可将南海海盆的沉积演化划分为5个阶段:扩张初期(34～28.5 Ma)、构造活动剧烈期(28.5～23 Ma)、构造活动减弱期(23～16....  相似文献   

19.
South China Sea   总被引：8，自引：0，他引：8  
The South China Sea is poorly understood in terms of its marine biota, ecology and the human impacts upon it. What is known is most often contained in reports and workshop and conference documents that are not available to the wider scientific community. The South China Sea has an area of some 3.3 million km2 and depths range from the shallowest coastal fringe to 5377 m in the Manila Trench. It is also studded with numerous islets, atolls and reefs many of which are just awash at low tide. It is largely confined within the Tropic of Cancer and, therefore, experiences a monsoonal climate being influenced by the Southwest Monsoon in summer and the Northeast Monsoon in winter. The South China Sea is a marginal sea and, therefore, largely surrounded by land. Countries that have a major influence on and claims to the sea include China, Malaysia, the Philippines and Vietnam, although Thailand, Indonesia and Taiwan have some too. The coastal fringes of the South China Sea are home to about 270 million people that have had some of the fastest developing and most vibrant economies on the globe. Consequently, anthropogenic impacts, such as over-exploitation of resources and pollution, are anticipated to be huge although, in reality, relatively little is known about them. The Indo-West Pacific biogeographic province, at the centre of which the South China Sea lies, is probably the world's most diverse shallow-water marine area. Of three major nearshore habitat types, i.e., coral reefs, mangroves and seagrasses, 45 mangrove species out of a global total of 51, most of the currently recognised 70 coral genera and 20 of 50 known seagrass species have been recorded from the South China Sea. The island groups of the South China Sea are all disputed and sovereignty is claimed over them by a number of countries. Conflicts have in recent decades arisen over them because of perceived national rights. It is perhaps because of this that so little research has been undertaken on the South China Sea. What data are available, however, and if Hong Kong is used, as it is herein, as an indicator of what the perturbations of other regional cities upon the South China Sea are like, then it is impacted grossly and an ecological disaster has probably already, but unknowingly, happened.  相似文献   

20.
High-resolution δ13C records are presented for the Miocene benthic foraminifersCibicidoides wuellerstorfi andC. kullenbergi (24-5 Ma) and the planktonic foraminiferGlobigerinoides sacculifer (18-5 Ma) from ODP Site 1148A (18° 50.17’N, 116° 33.93’E, water depth 3308.3 m), northern South China Sea. The general pattern of parallel benthic and planktonic δ13C shows a decrease trend of δ13C values from the early-middle Miocene to the middle-late Miocene. Two distinct δ13C positive excursions at 23.1-22.2 and 17.3-13.6 Ma, and two negative excursions at 10.2-9.4 and 6.9-6.2 Ma have been recognized. All these events are cosmopolitan, providing the good data for the stratigraphic correlation of the South China Sea with the global oceans as well as for studying the changes of the global carbon reservoir and its corresponding climate.  相似文献   

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