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1.
Pesticides and herbicides including organochlorine compounds have had extensive current and past application by Queensland's intensive coastal agriculture industry as well as for a wide range of domestic, public health and agricultural purposes in urban areas. The persistent nature of these types of compounds together with possible continued illegal use of banned organochlorine compounds raises the potential for continued long-term chronic exposure to plants and animals of the Great Barrier Reef. Sediment and seagrass samples were collected from 16 intertidal and 25 subtidal sampling sites between Torres Strait and Townsville, near Mackay and Gladstone, and in Hervey and Moreton Bays in 1997 and 1998 and analysed for pesticide and herbicide residues. Low levels of atrazine (0.1–0.3 μg kg−1), diuron (0.2–10.1 μg kg−1), lindane (0.08–0.19 μg kg−1), dieldrin (0.05–0.37 μg kg−1), DDT (0.05–0.26 μg kg−1), and DDE (0.05–0.26 μg kg−1) were detected in sediments and/or seagrasses. Contaminants were mainly detected in samples collected along the high rainfall, tropical coast between Townsville and Port Douglas and in Moreton Bay. Of the contaminants detected, the herbicide diuron is of most concern as the concentrations detected have some potential to impact local seagrass communities.  相似文献   

2.
The contamination of organochlorine pesticides (OCPs) in sediments from the Wu-Shi River estuary was investigated to evaluate the pollution potentials and distribution of OCPs in central Taiwan. A total of 19 sediment samples were collected at five sampling stations along the River estuary. The concentrations of OCPs were in the range of 0.99–14.5 ng/g-dry weight (dw) for ΣHCH (-, β-, γ-, δ-HCH), 0.46–13.4 ng/g-dw for Σcyclodiene and 0.53–11.4 ng/g-dw for ΣDDT (p,p′-DDD, p,p′-DDE, p,p′-DDT). The mean concentrations of ΣHCH, Σcyclodiene and ΣDDT were 3.79, 4.87 and 2.51 ng/g-dw, respectively. The total concentrations of OCPs correspond to 1.73–71.9 μg/g-OC when normalized to TOC contents. Among the organochlorine pesticides, endosulfan sulfate, β-HCH, and p,p′-DDD were the most dominant compounds in the sediments with the average concentrations of 1.97, 3.43 and 2.08 ng/g, respectively. Also, different contamination patterns among sampling seasons were observed. The measured concentrations of OCPs collected in spring were higher than those in autumn and winter. A linear relationship between sediment characteristics and OCP residues was also demonstrated. The results obtained in this study show that there still exist a variety of organochlorine pesticide residues in the sediments from the near shore of central Taiwan.  相似文献   

3.
Concentrations of polychlorinated biphenyls (PCBs), dichlorodiphenyltrichloroethane (DDT) and its metabolites, chlordane-related compounds (CHLs), mirex, hexachlorocyclohexane isomers (HCHs), dieldrin, and hexachlorobenzene (HCB) were determined in blubber of harbor seals (Phoca vitulina concolor) from the northwestern Atlantic coast. PCBs, DDTs, and CHLs were the major persistent organochlorines in harbor seal blubber, while mirex, HCHs, dieldrin, and HCB were minor contaminants. Highest concentrations were found in the adult males, followed by the pups, yearlings, adult females, and fetuses. DDT and PCB concentrations have declined from the high levels reported in the early 1970s, but no declines were observed in our samples over the ten-year period 1991-2001. DDT/PCB ratios were indicative of a more rapid decline of DDTs than PCBs, while ratios of p,p'-DDE/DDT were indicative of a metabolic "weathering" of DDT. The population appears to be susceptible to disease outbreaks, as evidenced by a recurrence of viral epizootics since the late 1970s. The PCB burdens in these seals are similar to levels reported in seals from polluted regions of Europe and Asia, and exceed the estimated threshold levels for adverse reproductive and immune system effects in the species.  相似文献   

4.
The levels of HCH isomers, HCB and summation DDTs were determined in five species of Baltic fish collected during 1995-2006. Some downward time trends of HCH isomer, pp'-DDE and pp'-DDD concentrations in Baltic fish were observed; in contrast, HCB and DDT concentrations did not exhibit any obvious trend. Concentrations of summation HCHs expressed on a lipid weight basis were very similar in all species studied. In contrast, concentrations of summation DDTs varied in tested species. The most abundant HCH isomer was beta-HCH and among DDT-related compounds, pp'-DDE prevailed. In our investigations the sampling sites were not a crucial factor for organochlorine pesticide concentrations and patterns observed in fish, but the occurrence of several inter-species differences in the bioaccumulation features of OC pesticides were observed. For cod there was a positive correlation between fish size (length) and summation DDT concentration. In herring, sprat and salmon samples, summation DDT concentrations were negatively correlated with fat content.  相似文献   

5.
The concentration ranges of chlorinated hydrocarbons in marine fish were HCB (0.03–9.5 ppb), Lindane (0.02–5.3 ppb), Endosulphan (0.21–4.9 ppb), DDT (0.50–18.6 ppb), Aldrin (0.05–54.6 ppb) and PCB (4.78–225 ppb). Fish contained higher concentrations of Aldrin, Heptachlor, HCB and Lindane than shellfish, while a reverse trend was observed for DDT and PCBs. The concentrations of residues obtained were found to be lower than those reported in literature for industrialized countries. Predator fish species were found to concentrate more residues in muscle tissue than plankton feeders. The DDT/PCB values were less than 1 indicating a predominance of industrial activities over agricultural activities as the source of contamination of the marine environment. The fish Galeoides decadactylus is a potential bio-indicator for chlorinated hydrocarbons pollution monitoring in the study area.  相似文献   

6.
Polychlorinated biphenyls (PCBs) and organochlorine (OC) pesticide levels were determined in blubber samples collected from stranded and incidentally by-caught Hector’s (Cephalorhynchus hectori hectori) and Maui’s (Cephalorhynchus hectori maui) dolphins from New Zealand waters between 1997 and 2009. PCBs (45 congeners) and a range of OC pesticides including dieldrin, hexachlorocyclohexane (HCH) and dichlorodiphenyltrichloroethane (DDT), along with its metabolites DDE and DDD were determined. OC pesticides dieldrin, p,p′-DDE, p,p′-DDD and p,p′-DDT were present at the highest concentrations. Sum DDT concentrations ranged from 93.7 to 8210 (Mean = 1358, S.D = 1974) and 252.4 to 57,390 (Mean = 12,389, S.D = 18,161) μg/kg wet weight in females and males, respectively. Similarly, Σ45CB concentrations ranged from 45.5 to 981.3 (Mean = 333.2, S.D = 265.8) and 60.5 to 5574 (Mean = 1833, S.D = 1659) μg/kg wet weight in females and males, respectively. The transfer of ΣDDTs and summed PCBs (both as ΣICES7CBs and Σ45CBs) between a pregnant female and her unborn fetus was calculated at 5.7% and 4.3%, respectively. As the fetus was close to term, this likely represents the degree of placental transfer. Concentrations of OC pesticides determined in the present study are higher than those previously reported for Hector’s dolphins. Sum DDT and DDE/ΣDDT levels calculated reveal New Zealand’s legacy of DDT usage, particularly off the east coast of the South Island.  相似文献   

7.
Jin Y  Hong SH  Li D  Shim WJ  Lee SS 《Marine pollution bulletin》2008,57(6-12):775-781
To assess the levels of organochlorine compounds (OCs) in the Chinese coastal environment, monitoring study using bivalves was conducted in 2005. A total of 21 bivalve samples covering the northeastern coast of China were collected and analyzed. Organochlorine compounds were widely distributed in the Chinese coastal environment, with dichlorodiphenyltrichloroethane (DDT) contamination being particularly prevalent. The overall concentrations of PCBs, DDTs, HCHs, chlordane compounds (CHLs), dieldrin, and endosulfans in bivalves were in the ranges of 3.27-25.4, 54.8-2680, 1.42-25.5, n.d. (not detected)-2.28, n.d.-4.02, and n.d.-9.55 ng g(-1) on a dry weight basis, respectively. The concentrations of DDT and HCH compounds are relatively higher than those from the coastal areas of other Asian countries. DDT metabolites were predominant, suggesting that the degradation of DDT is in progress in the Chinese coastal environment. Still, however, DDTs of high concentration exceeding 1000 ng g(-1) were observed at 19% of the stations surveyed. Among HCH compounds, beta-HCH, which is an isomer with strong persistency, was observed predominantly. Compositions of DDT and HCH compounds imply that fresh input of the two compounds into the Chinese coasts is possibly low.  相似文献   

8.
During August-September 1993, a joint Russian-United States expedition to the Bering and Chukchi Seas took place. Surface water samples were collected from 21 sites and separated into dissolved (duplicates) and suspended solids; 19 sediment and 6 air samples were also collected. These samples were analysed for 19 organochlorine pesticides, 11 chlorobenzenes and 113 PCB congeners. The report provides data on selected compounds which occured in > or = 75% of the water samples. Highest water concentrations were observed for HCH in open waters north and south of the Bering Strait, both regions being similar (alpha-HCH; 2.2 ng/L and lindane: 0.35 ng/L). Air levels observed were also constant (alpha-HCH; 0.041 ng/m3, lindane: 0.0093 ng/m3). Suspended solids and air particulares contributed little to the concentrations in their respective media, an observation common to all analytes except for the PCBs and the DDT residues. The sum of PCB concentrations in water were higher in the Bering Sea area compared to the Chukchi Sea (1.0 vrs 0.67 ng/L) and lower for air (0.46 vrs 0.23 ng/m3). Sum of DDT in water was higher in the Bering Sea than in the Chukchi Sea (0.23 vrs 0.15 ng/L) while in sediments and air, the Bering Sea concentrations were lower (0.95 vrs 1.6 ng/g and 36 vrs 56 pg/m3, respectively). Other organochlorine compounds for which data are presented include: pp'-DDE, pp'-DDT, dieldrin, HCB, 3 chlorobenzenes and 3 PCB congeners. Fluxes of all these chemicals through the Berin Strait are estimated; they ranged from 57 t/a (alpha-HCH) through 26 t/a (for sum of PCBs) to 0.2 t/a (pp'-DDE, dieldrin and 1,2,3-trichlorobenzene). Fugacity ratios for the HCHs and PCBs indicate the alpha-HCH is degassing in both the Bering and Chukchi Seas and that the gamma-isomer is degassing in the Bering Sea and is close to equilibrium (weakly absorbing) in the Chuchi Sea; the sum of PCBs are strongly absorbing in both areas.  相似文献   

9.
Organochlorine compounds (OCs) were determined in the five species of sturgeons collected from coastal waters of Caspian Sea in Kazakhstan, Azerbaijan, Turkmenistan and Iran during 2001 and 2002 to understand their status of contamination and accumulation features. Among OCs examined, concentrations of DDTs (DDT and its metabolites) were predominant in all the sturgeon samples with concentrations ranging from 73 to 31,000 ng/g on lipid weight basis, followed by PCBs, CHLs, HCHs, HCB, dieldrin, TCPMOH, and heptachlor epoxide in order. The concentrations of OCs in beluga (Huso huso) were the highest among all the five species. When comparing residue levels among same species, OC residues were highest in sturgeons from Azerbaijan and Kazakhstan and lowest in Turkmenistan. However, the concentrations of HCHs, dieldrin, and heptachlor epoxide in sturgeons showed less geographical variability.  相似文献   

10.
《Marine pollution bulletin》2009,58(6-12):775-781
To assess the levels of organochlorine compounds (OCs) in the Chinese coastal environment, monitoring study using bivalves was conducted in 2005. A total of 21 bivalve samples covering the northeastern coast of China were collected and analyzed. Organochlorine compounds were widely distributed in the Chinese coastal environment, with dichlorodiphenyltrichloroethane (DDT) contamination being particularly prevalent. The overall concentrations of PCBs, DDTs, HCHs, chlordane compounds (CHLs), dieldrin, and endosulfans in bivalves were in the ranges of 3.27–25.4, 54.8–2680, 1.42–25.5, n.d. (not detected)–2.28, n.d.–4.02, and n.d.–9.55 ng g−1 on a dry weight basis, respectively. The concentrations of DDT and HCH compounds are relatively higher than those from the coastal areas of other Asian countries. DDT metabolites were predominant, suggesting that the degradation of DDT is in progress in the Chinese coastal environment. Still, however, DDTs of high concentration exceeding 1000 ng g−1 were observed at 19% of the stations surveyed. Among HCH compounds, β-HCH, which is an isomer with strong persistency, was observed predominantly. Compositions of DDT and HCH compounds imply that fresh input of the two compounds into the Chinese coasts is possibly low.  相似文献   

11.
Bivalves (Crassostrea rizhophorae, Isognomon alatus, Codakia orbicularis Linné, and Tellina fausta) and sediment samples collected from 12 locations along the Dominican Republic coastline were used to assess the degree of nearshore contamination by selected chlorinated hydrocarbons and heavy metals. Concentrations of total chlordanes, DDTs and PCBs ranged from 0.51 to 7.47 ng/g, < MDL to 30.9 ng/g and 11.3 to 82.3 ng/g, and from < MDL to 1.73 ng/g, 0.21 to 12.5 ng/g and 0.46 to 41.9 ng/g in bivalves and surface sediments, respectively. The concentration ranges of predominantly anthropogenic Cu, Pb and Zn were 3.08–866 μg/g, 0.08–1.46 μg/g and 22.9–4380 μg/g in bivalve soft parts and 1.01–111 mg/g, 0.420–134 μg/g and 1.96–277 μg/g in surface sediments, respectively. Mercury concentrations ranged from 0.290 to 7.02 μg/g and from 0.096 to 0.565 μg/g in both matrices. The relatively high Hg concentrations found in bivalves from two stations in Bahia Samana, near to a known source of past Hg contamination in the sediments, require a more in-depth survey of the area. In general the concentrations of selected chlorinated hydrocarbons and trace metals, compared with those reported for the same matrices in the Caribbean and west Atlantic coastal areas, show at present the existence of only very localized contamination problems in the Dominican Republic.  相似文献   

12.
Surface waters collected along the salinity gradient of the Hudson River estuary in four cruises between 1995 and 1997 were size-fractionated into particulate (>0.45 μm), ‘dissolved' (<0.45 μm), colloidal (10 kDa, 0.45 μm) and low molecular weight (<10 kDa) phases. Dissolved Cd concentrations (range: 0.11–1.19 nM) in surface waters of the estuary appear to have decreased fourfold (from an average of 2.36 to 0.61 nM) over a 23-year period, since the initial analysis of samples collected in the 1970s by Klinkhammer and Bender [Estuar. Coastal Shelf Sci. 12 (1981) 629–643]. This interannual decline reflects improvement in sewage treatment and the elimination of industrial Cd sources to the Hudson River estuary. In contrast, dissolved Mn levels (range: 0.033–1.46 μM) have remained relatively constant over the same period of time, suggesting that anthropogenic sources have very limited impact on Mn concentrations in the estuary. The concentrations of both Cd and Mn appeared to strongly depend on the season and/or river discharge. The highest concentrations were detected under low freshwater discharge, implying that limited hydraulic flushing allows a build-up of metals in the water column. Although the decline in Cd levels within the estuary reflects a reduction in the magnitude of anthropogenic inputs, mass balance estimates indicated that current sources of Cd to the estuary include sewage discharges (in the lower estuary around Manhattan) and diagenetic remobilization from industrial Cd deposited in sediments nearly 2 decades ago (in the upper estuary near Foundry Cove). Moreover, under low river discharge, the sources considered in our model (sewage, riverine input, atmospheric deposition, and benthic fluxes) could account for no more than 60% of the Cd exported from the lower estuary to the ocean. This suggests that undefined sources such as ground water and inputs from other watersheds (e.g., Long Island Sound and Newark Bay) may potentially influence the water quality of the New York Harbor. The size-fractionated metal concentrations indicated that most of the traditionally defined ‘dissolved' Cd and Mn consisted of <10 kDa molecular weight species. High molecular weight colloidal species of Mn accounted for about 50% of the dissolved fraction at the riverine end-member and <5% at intermediate and high salinities. Colloidal Cd accounted for <6% of the dissolved phase throughout the estuary. Unlike the non-conservative excess (relative to ideal dilution of river water and seawater) of dissolved Mn observed along the estuary, high molecular weight colloidal Mn appeared to be removed at the head of the estuary. The small contribution of colloidal Cd and Mn to the ‘dissolved' phase suggests that remobilization from suspended particulate phases and/or from sediments occurs through the formation of small molecular weight species.  相似文献   

13.
Zinc in muscle tissue from 28 species of fish, three species of sharks and rays, two species of squid and cuttlefish, and three species of crustacea collected from Cleveland Bay, together with some measurements made on oysters and mangrove flora and fauna are reported. In the fish species the mean Zn concentration in muscle tissue was 4.83 ± 2.82 μg/g wet weight, slightly lower than zinc measurements (7 μg/g wet weight) made in 14 fish species collected from the bay in 1975. Zinc in sharks and rays ranged from 3.5 to 7.2 μg/g wet wt, in squid and cuttlefish 13–16 μg/g wet wt, and in crustacea levels ranged from 14 to 18 μg/g wet wt. Zinc levels in fish varied between species with concentrations well below the ANZECC Maximum Residue Limit of zinc in seafood (150 μg/g wet wt). Although lower zinc concentrations were found in oysters collected from the Townsville Harbour area (2080 μg/g wet wt), compared with previous measurements made 25 years ago at this site, these levels are still above the Maximum Residue Limit for zinc in oysters (1000 μg/g wet wt). Concentrations of zinc in oysters from Orpheus Island (2547 μg/g wet wt), about 74 km away from industrial and urban activity, are also above the safe guideline values. Horseshoe Bay oysters transplanted to Ross Creek accumulated zinc at a rate of about 100 μg/g of oyster tissue per week, suggesting that dissolved zinc levels at this site are elevated, and that oysters rapidly accumulate zinc. Highest concentrations of zinc in mangrove leaves (30–65 μg/g dry wt) occurred in Osbornia octodonta, Exocaria agalocha, and Aegialitus annulata, compared with Ceriops tagal, and Avicennia marina (5–10 μg/g dry wt). No significant difference in zinc concentration occurred between leaves and litter fall for most of these species, with the sole exception of Exocaria, which showed almost a twofold increase in concentration. In seven species of mangrove fauna levels of zinc were very uniform and close to 50 μg/g (dry wt) Telescopium telescopium from the mouth of the Ross Estuary was the exception with levels at 400 μg/g (dry wt).  相似文献   

14.
A steady-state nonequilibrium fugacity model incorporating the oceanographic dimensions of the environment receiving a sewage discharge from Sydney, Australia was used to predict the environmental fate of a range of chlorohydrocarbon contaminants. The model showed advection in water to be the dominant removal process, accounting for all except 1–2% of the contaminants discharged. With the exception of the more water soluble dieldrin, the major portion of contaminant present in the area was held in the sediments. Bioconcentration and sediment sorption models were used with levels detected in the biota and sediments to calculate the ambient water concentrations of the chlorohydrocarbon contaminants. The ambient water concentrations calculated using these models were in general agreement within a factor of about 2 in all but one case, and that was in agreement within an order of magnitude. The fugacity model was also used to estimate the rates of discharge of each of the contaminants. These were chlordane 83–640, DDT 150, dieldrin 1400–1500, hexachlorobenzene 360–400 and PCBs 55–96 g day−1. Comparisons of the calculated ambient concentrations of each compound in the water and in fish in waters adjacent to the discharge point before and after its relocation from a cliff-face to a deepwater site indicated that relocation should result in an order of magnitude reduction.  相似文献   

15.
Lake Koronia, a Ramsar site, is shallow, polymictic, hypertrophic and until recently was aerially the fourth largest lake in Greece. Although exceeding 5 m in the past, lake depth has declined progressively from 3.8 m in 1980 to < 1 m in 1997, reducing surface area and water volume by 50% and 80%, respectively. Specific conductivityincreased from 1300 μS cm−1 in 1977 to >6000 μS cm−1 in 1991. Increased phosphate concentrations from the late 1970's (8–45 μg L−1) to the late 1990's (100–1000 μg L−1) document that the previously eutrophic system with a limited littoral zone switched to hypertrophy dominated by massive cyanobacteria blooms. Oxygen saturation of the water column increased progressively from about 80% in 1983 to full saturation about 1993, after which it decreased progressively to only 20% saturation in 1997. In spite of cyanobacteria dominance, community metabolism of the lake switched from progressively increasing autotrophy to rapidly advancing heterotrophy associated with progressive water-level reduction leading to fish extirpation in the lake.  相似文献   

16.
Kurt PB  Ozkoc HB 《Marine pollution bulletin》2004,48(11-12):1076-1083
A mussel and seawater monitoring survey was conducted at six sampling points between Yalikoy (Ordu) and Sinop in 1999-2000 along the Mid-Black Sea Coast of Turkey in order to assess concentrations of organochlorine pesticides (OCs) and polychlorinated biphenyls (PCBs). Chlorinated pesticides and PCBs were measured in the mussel Mytilus Galloprovincialis and in seawater. In the mussel samples, the most common pollutants in terms of average concentration per g of wet weight (ww), were DDT (max. 1800 pg/gww, min. 240 pg/gww) and its metabolites DDD (max. 5400 pg/gww, min. 240 pg/gww) and DDE (max. 2800 pg/gww, min. 70 pg/gww). Also, dieldrin, heptachlor and HCB were notable contaminants in the mussel samples. PCBs were determined in none of the biota or seawater samples. The concentrations of the OCs and PCBs in mussels were higher in coastal areas receiving river discharges and close to the largest city of the region, Samsun (especially in sampling points in the harbour area). The well-known long persistence of DDTs and other chlorinated compounds was confirmed by residues of these pollutants measured in mussels. On the other hand, even though the usage of such kind of persistent compounds in Turkey was banned, there may still be illegal usage and it is not certain whether the application of these compounds did end in the region.  相似文献   

17.
Concentrations of chlorinated hydrocarbons (DDT and metabolites, PCBs, aldrin, dieldrin, HCB and BHCs) have been determined in the tissues of five species of marine animals sampled in selected areas of the central Mediterranean.  相似文献   

18.
The concentration of cadmium in sexually mature Nucella lapillus was investigated around the coast of Wales. Higher concentrations of cadmium were found in whelks located in the Bristol Channel compared with Cardigan Bay Nucella. Accumulation and toxicity of cadmium were investigated at 50–600 μg Cd l−1 over a period of 21 days. At the lower concentrations of 50–100 μg Cd l−1 all Nucella survived the 21 days of experimentation. The rate of cadmium uptake after exposure to cadmium was inconsistent and not related to the degree of site contamination. At all sites the concentration of cadmium in Nucella, after treatment with 50–600 μg Cd l−1 for 21 days, was significantly different from controls, but after 7 days it varied with the site and cadmium concentration. Only samples collected at Fishguard, Dale, and Swansea survived 21 days at 600 μg Cd l−1. Tissue cadmium concentrations did not significantly effect the whole body concentration of zinc.  相似文献   

19.
Deposition samples were taken at a height of 2367 m above sea level (m.a.s.l.) on the Island of Tenerife from May 1999 until July 2000 and analysed for 19 polychlorinated biphenyl (PCB) congeners, hexachlorobenzene (HCB), hexachlorocyclohexanes (HCH) and DDTs. This site is located above the inversion layer, so samples represent background concentrations of the free troposphere. The average deposition fluxes of HCB, total HCH, DDTs and PCBs were 86, 400, 110 and 780 ng m(-2) yr(-1), respectively, being lower than those reported at sea level in continental or marine areas. All compounds are generally found in higher abundance in the wet precipitation samples. However, these samples only represent a fraction, e.g. 33%, of the total deposition load. Annual mass balance calculations show that wet precipitation is essentially responsible for the deposition of the low molecular weight OC whereas dry deposition accounts for more than 50% of the higher molecular weight PCBs.  相似文献   

20.
Persistent organochlorine compound concentrations were determined for 23 surface sediment samples collected from Alexandria Harbor, Egypt. Total PCB concentrations ranged from 0.9 to 1210 ng/g with four to seven Cl-substituted biphenyls being the most prevalent PCBs congeners. Different PCB congener distribution patterns were observed, probably reflecting different inputs and attenuation at various locations. Total DDT concentrations varied from <0.25 ng/g to 885 ng/g. The ratios of DDTs (2,4′- and 4,4′-DDT)/total DDTs (DDTs plus metabolites) in sediment samples from certain sites were 0.86 or higher, indicating little attenuation or recent input of DDT. Total chlordane (the sum of heptachlor and its epoxide, oxy-, γ- and -chlordane and cis+trans-nonachlor) ranged from <0.25 to 44 ng/g with the highest concentration found in the Arsenal Basin. The geographic distributions of PCBs, total DDTs and total chlordane were similar. Chlorinated benzenes (CBs), hexachlorocyclohexanes (HCHs), aldrin, dieldrin, endrin, chloropyrifos, endosulfan, mirex and pentachloroanisole were below detection limits or detected at low concentrations in most of the samples. Sites that were contaminated with high concentrations of organochlorine compounds were associated with dense population and low energy environment. The contamination levels of PCBs, total DDTs and total chlordane were in high range compared to other locations worldwide.  相似文献   

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