共查询到10条相似文献，搜索用时 157 毫秒
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将广泛应用于东亚地区的LLA(Lurmann Lloyd Atkinson)化学机制耦合到欧拉型区域空气质量模式(RAQM),并考虑区域污染物长期模拟研究中降水随时间变化的非均匀性,讨论了湍流参数化过程中相似理论在近地层和全边界层的应用对湍流垂直扩散系数(Kz)与干沉降速度(V),O3与NOx浓度的影响。结果表明,全边界层应用相似理论明显低估了Kz值,近地层50m处Kz值被低估20%以上,750m处其值被低估约70%;O3、NOx的干沉降速度在日本东部与南部海域被低估了10%以上,在朝鲜半岛东部和西部海域模拟值普遍偏高。Kz和干沉降速度的不同直接影响污染物的浓度和沉降量分布。Kz值的被低估对NOx浓度有明显影响,在近地层50m处NOx浓度最大可增加约30%,整个边界层中NOx平均浓度除台湾省东北海域外普遍增加5%~20%。O3浓度则受干沉降作用的影响较大。虽然近地层、全边界层分别应用相似理论都较好地模拟了O3与NOx峰值浓度出现的时间,但相似理论应用于全边界层会引起较大的误差。即使是大区域、长期空气质量模拟研究,也建议相似理论仅应用于近地层,且模式第一层高度应设置在常通量层内。 相似文献
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采用地形坐标系下适合于复杂地形且满足地-气耦合的静力学三维中-β尺度气象预报模式,使用08时的实测流场经变分法初始化后得到的初始流场,模拟研究了上海地区的局地流场时空演变特征。模式较细致地考虑了湍流、长短波辐射、凝结、蒸发、地表热力平衡等因子,在此基础上,使用有限元法数值求解一阶闭合的三维欧拉平流扩散方程,模拟了上海地区的SO2浓度分布。结果表明:上海的局地流场具有明显的日变化特征,受海陆温差的影响明显,日间风速较夜间风速大,风向呈顺时针旋转;在不稳定层结情况下,高架点源排放的高空污染物对地面的污染物浓度有贡献,会造成地面污染物浓度升高。 相似文献
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嵌套网格空气质量预报模式系统的发展与应用 总被引：74，自引：4，他引：74
主要综述中国科学院大气物理研究所自主开发的嵌套网格空气质量预报模式系统(NAQPMS,Nested Air Quality Prediction Modeling System)的历史发展与应用情况.模式发展伊始为欧拉污染物输送实用模型,利用其研究东亚硫氧化物的跨国输送问题,得出中国对于周边国家的输送量不大的结论; 在系统中嵌入适合东亚的起沙机制模块,用来模拟沙尘发生、输送及沉降等过程,估算亚洲大陆沙尘气溶胶对海洋地区的输送与沉降通量,为研究海洋生物地球化学循环提供基础数据; 利用该系统研究沙尘及其土壤粒子对酸雨的中和作用,发现沙尘输送对东亚酸雨的分布影响很大; 发展城市尺度高分辨率气象和空气质量预报技术,使模式水平分辨率达到500 m,并应用于台北高浓度臭氧和PM10的模拟; 研究和集成区域及城市尺度大气污染预报理论和模拟技术,研制成目前的嵌套网格空气质量预报模式系统,以探讨不同尺度各种污染(如沙尘暴、城市光化学烟雾、酸雨、高浓度悬浮颗粒物等)的变化规律.在模式系统中初步建立资料同化模块,开展大气化学成分及沙尘输送模拟的资料同化研究.系统已经在北京、上海、深圳、郑州等城市环境监测中心实施空气质量的实时预报.未来,系统将集成到全球环境大气输送模式(GEATM),以实现从城市群到全球具有双向耦合功能的模式系统. 相似文献
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In this paper a 3-D mesoscale PBL dynamic prognostic model for a coastal region with complex terrain was developed to simulate the 3-D flow field under a local sea-land breeze circulation. The output from the PBL model was used as an input to an Eulerian numerical model which can be used to simulate finely the temporal and spatial distributions of an air pollutant (SO2) during a sea-land breeze developing in a coastal region. With respect to its use as a diagnostic model, only a few data would be required to simulate the background winds controlled by a larger scale synoptic system, and then provide initial winds for the PBL model.Having linked the three models and defined the coefficients of turbulent diffusion in a simple form, an integrated 3-D numerical air quality model suitable for the coastal environment was designed. The period of May 29, 1986 was selected for simulating and analysing the distribution of air pollutants over the coastal area of Bohai-sea in Northern China. The results indicated that the calculated concentrations corresponded with the observed ones on the whole. Thus this linked model has been shown to be feasible and useful in practice. 相似文献
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Yang Fanglin 《大气科学进展》1991,8(2):149-164
The stability of large-scale horizontal motion in the atmosphere is discussed in this paper by using qualitative analysis theory of non-linear ordinary differential equations. Both the non-linear distribution of basic Zephyr flow and the variation of geostrophic vorticity along the latitude (f=f0 + βδy ) are all included in this paper's mathematical model so as to analogue the background field of large-scale horizontal air motion more really in the rotating reference frame of the earth. Some significant results are drawn out from this paper and the conclusions of Li(1986)'s and Wan et al.(1990)'s are extended widely. 相似文献
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Modeling of Regional High Ozone Episode Observed at Two Mountain Sites (Mt. Tai and Huang) in East China 总被引：3，自引：0，他引：3
Zifa Wang Jie Li Xiquan Wang Pakpong Pochanart Hajime Akimoto 《Journal of Atmospheric Chemistry》2006,55(3):253-272
A high O3 episode was observed during 23–25 May 2004 at two high-mountain sites reflecting the regional pattern of air pollutants over East China. This episode lasted about three days with the maximum hourly O3 mixing ratios reaching 111 and 114 ppbv at Mt. Tai and Huang, respectively. Backward trajectories and meteorological analysis indicated that regional transport, associated with a weak high pressure system over the East China Sea, might play an important role in the formation of this high ozone episode. The nested air quality prediction modeling system (NAQPMS) was applied to investigate the formation and evolution of this high O3 event. The comparison of model results with observations showed that NAQPMS successfully reproduced the main observed patterns of O3 and meteorological parameters during the simulated period. The model results with emission over the Yangtze Delta and the East Central China switched on/off clearly showed that ozone and its precursors transported from the Yangtze Delta and the East Central China enhanced the high ozone episode at two sites, with a contribution of 20%–50% during the episode. In addition, based on process analysis with the model, chemical production and regional transport appeared to be the main causes of high ozone episode involving a large amount of high-ozone air masses and precursors transported from the surrounding areas. The horizontal transport is more active during the period of high ozone episode than that during the non-episode at Mt. Tai as well as Mt. Huang. 相似文献
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Described is a system for analyzing and forecasting the air quality in the central regions of Russia, During the operation of the system, the detailed meteorological information provided by the WRF-ARW model is used by the CHIMERE chemistry transport model for simulating the processes of transport, chemical transformation, and deposition of atmospheric minor constituents. Considered is the quality of retrieved and forecasted (with the lead time up to three days) concentrations of O3, NO2, NO, CO, and PM10. The presented verification scores of pollutant concentrations demonstrate a relative success of the system. Demonstrated is a need in improving the data on the emissions of the air pollutants used for simulations. A procedure for the statistical correction of computed concentrations is described and verification scores of its results are given. 相似文献
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Summary The three-dimensional long-range transport model EURAD has been applied to two episodes in 1986 to study the transport and transformation of air pollutants over Europe under different meteorological conditions. The spring episode is characterized by varying meteorological conditions over Europe and transport of pollutants is complex. The summer episode is suitable to study the enhanced formation of photooxidants as an almost stagnant high pressure system over central Europe favoured the accumulation of pollutants. Available observations from several monitoring networks in Europe are used to evaluate the near surface concentration predictions of the model. This is possible for the sulfur species, O3 and NO2 for the central part of the modelling domain. It is shown that O3 and NO2 trends in the western part of the model domain are estimated reasonably well. The strong bias for underpredicting NO2 in the eastern part of the domain reflects the quality of emission data for the two regions of the modelling area. Typically for regional scale Eulerian transport models when applied on larger grid sizes, EURAD overpredicts the observed minima and underpredicts the high observations. This is particularly true for O3 but also detectable in the sulfate comparisons. Several sensitivity simulations for both episodes were performed to test numerical algorithms, parameterizations or emission data. Results from these simulations clearly show the important role of cloud related processes during the spring time for the sulfur species. Further testing and assessment of cloud parameterizations and emission data for transport models is anticipated.With 22 Figures 相似文献
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Observed pollutants are of both primary and secondary origins, influenced by local topography and meteorology. Identifying
sources and relative contribution often require vast detailed data collection and complicated models. This study applied a
statistical time series analysis to two selected pollution events, spring and fall, at two sites in northern Taiwan. Vector
moving average representations were used to quantitatively examine relationships among chemical pollutants and estimate their
lifetimes. Results from impulse responses show that wind direction change alters the characteristic of pollution observed
in opposite sites of Taipei City, from chemical dominant system to transport dominant one and vice versa. Chemicals are clearly
separated into photochemical pollutants and primary pollutants. Results pointed out that Taipei City is the major source of
photochemical smog, but not these primary pollutants. Derived chemical lifetimes at same location vary from 20% to four times
under different meteorological condition. Estimated concentrations of hydroxyl radical range between 2 to 8 × 107 cm−3. Photochemical pollutants are responsible for parts of PM10 collected in both station observed. Oxidation of SO2 is only important in PM10 observed at one station. This study provides a simpler tool to derive information usually from
complex models, therefore, is suitable as complement in decision-making process. 相似文献