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1.
The warm circumnuclear dust in the inner cometary coma reradiates in the IR in the wavelength range of the ground state rotational band of the dominant atmospheric molecule, H2O. However, the interaction of this radiation with H2O has hitherto not been taken into account in cometary atmospheric models. Here we have extended our earlier two-phase, multifluid model of the dusty atmosphere by including this effect. Although this IR radiation initially pumps the rotational levels of H2O, frequent intermolecular collisions in the inner coma transfer this energy from rotational modes to translational modes. As a result the temperature in the innermost coma no longer decreases to about 10 K, as predicted by the earlier models, but reaches a minimum of only about 120 K.  相似文献   

2.
The combination of a time-dependent spherically symmetric hydrodynamic model of stellar atmosphere pulsation and a radiation transport code, which incorporates maser saturation theory, enabled us to synthesise maps and spectra of H2O maser emission from the circumstellar envelopes of long period variable stars. The synthetic maps and spectra compare favourably with observed 22, 321 and 325 GHz H2O maser emission. As is observed in H2O maser regions the peak emission occurs between 3–8 stellar radii from the star. The calculated H2O maser regions are in conditions of nH2 = 106 − 108 cm−3, assuming a fractional abundance of 10−4; kinetic temperatures of 550–3000 K; dust ensemble temperatures of 500–1200 K and an accelerating velocity field. The IR radiation field is explicitly included in the radiation transport model, incorporating the latest absorption efficiency data for silicates from Draine. We reproduce the features seen in high angular resolution MERLIN spectral line datacubes. This shows that a mass outflow model which extends the photosphere using pulsations and incorporates radiation pressure on silicate based dust particles can produce the observed data on small (10-mas) angular scales. This revised version was published online in September 2006 with corrections to the Cover Date.  相似文献   

3.
Loss of water from Venus. I. Hydrodynamic escape of hydrogen   总被引：1，自引：0，他引：1  
A one-dimensional photochemical-dynamic model is used to study hydrodynamic loss of hydrogen from a primitive, water-rich atmosphere on Venus. The escape flux is calculated as a function of the H2O mixing ratio at the atmospheric cold trap. The cold-trap mixing ratio is then related in an approximate fashion to the H2O concentration in the lower atmosphere. Hydrodynamic escape should have been the dominant loss process for hydrogen when the H2O mass mixing ratio in the lower atmosphere exceeded ～0.1. The escape rate would have depended upon the magnitude of the solar ultraviolet flux and the atmospheric euv heating efficiency and, to a lesser extent, on the O2 content of the atmosphere. The time required for Venus to have lost the bulk of a terrestrial ocean of water is on the order of a billion years. Deutrium would have been swept away along with hydrogen if the escape rate was high enough, but some D/H enrichment should have occurred as the escape rate slowed down.  相似文献   

4.
Density profiles for CO, O, and O2 in the Cytherean atmosphere above 90 km are plotted with eddy diffusion coefficient (K) as a parameter, subject to the constraint that the mixing ratios of CO and O2 approach their observed value or values under the observed upper limit at the lower boundary. It is then shown that the value of K puts upper limits on the amount of hydrogen (in the form of H2O, HCl, and H2) the atmosphere near 90km can contain. This value is a function of the density and temperature of hydrogen at the critical level and the magnitude of the total escape flux, where unspecified flux mechanisms other than thermal are postulated ad hoc. In general these constraints call for large values of K to accomodate the atomic hydrogen produced by measured mixing ratios of HCl and H2O. Hence they constrain thee amount of O in the upper atmosphere to values well under 1% at 130 km unless there are very large hydrogen escape fluxes, 107 cm?2sec?1 or larger. The freedom to assume arbitrary amounts of H2 in the atmosphere is also restricted. We suggest either very effective escape mechanisms—despite low exospheric hydrogen densities—or novel excitation mechanisms for O(33S) and O(35S) in the upper atmosphere.  相似文献   

5.
An ultraviolet spectral probe for a hydrogen-rich planetary atmosphere, such as that of Jupiter, is suggested, utilizing discrete lines in the H2staggered+ 2pπu?1sσg electronic transition. For the Jovian atmosphere, the dominant mechanism for exciting H2+ to its 2pπu state appears to be photoexcitation, principally through absorption of the solar Lyman-α line. We estimate that the Jovian column emission rate of the H2+ 2pπu(ν′ = 2, J′ = 1) →1sσg(ν″ = 18,J″ = 0) fluorescent line at 1236.6 Å is if1 photon cmsu-2 secsu-1; i.e., that if1 photon secsu-1 of this radiation would strike a 15-cm diameter mirror in a Jupiter fly-by at an impact parameter of 3 × 105km. The critical role of corrections to the Born-Oppenheimer approximation in the use of an H2+ probe is discussed.  相似文献   

6.
Europa is bombarded by intense radiation that erodes the surface, launching molecules into a thin “atmosphere” representative of surface composition. In addition to atoms and molecules created in the mostly water ice surface such as H2O, O2, H2, the atmosphere is known to have species representative of trace surface materials. These trace species are carried off with the 10-104 H2O molecules ejected by each energetic heavy ion, a process we have simulated using molecular dynamics. Using the results of those simulations, we found that a neutral mass spectrometer orbiting ∼100 km above the surface could detect species with surface concentrations above ∼0.03%. We have also modeled the atmospheric spatial structure of the volatile species CO2 and SO2 under a variety of assumptions. Detections of these species with moderate time and space resolution would allow us to constrain surface composition, chemistry and to study space weathering processes.  相似文献   

7.
To explain the observed abundances of CO2 in Titan's atmosphere, a relatively high water deposition into the atmosphere needs to be invoked due to the importance of H2O photolysis in CO2 production. A likely source of H2O is icy dust particles from space. This paper considers the direct dust input to Titan's atmosphere from the interplanetary environment, and also ejecta particles from micrometeoroid impacts with the icy satellites Hyperion, Iapetus and Phoebe. It is found that the likely mass influx to Titan is 10–16 to 10–15 kg m–2 s–1. This mass influx is an order of magnitude too low to explain the observed levels of CO2 in Titan's atmosphere in the context of a recent photochemical model. This leads one to speculate as to the likelihood of one large impact to Titan in the recent past;i.e., that the atmosphere is not in equilibrium but is cnrrently losing CO2.  相似文献   

8.
SCIAMACHY (SCanning Imaging Absorption spectrometer for Atmospheric CHartographY) is a space based spectrometer designed to measure sunlight transmitted, reflected and scattered by the Earth atmosphere or surface. It is a contribution to the Envisat-1 satellite to be launched in late 1999.SCIAMACHY measurements will provide amounts and distribution of 03, BrO, OCl0, ClO, S02, H2CO, N02, CO, CO2, CH4, H2O, N20, pressure, temperature, aerosol, radiation, cloud cover and cloud top height from atmospheric measurements in nadir, limb and occultation geometry.By the combination of the near simultaneous limb and nadir observations SCIAMACHY is one of a limited number of instruments which is able to detect tropospheric column amounts of 03, N02, CO, CH4, H2O, N20, S02, H2CO, and BrO down to the planetary boundary layer under cloud free conditions.  相似文献   

9.
Despite several spacecraft encounters and numerous groundbased investigations, we still do not know much about Jupiter's deep atmosphere; in fact, the Galileo probe results were so different than anyone had anticipated, that we understand even less about this planet's atmosphere now than before the Galileo mission. We formulate four basic questions in Section 1.3, which, if solved, would help to better understand the chemistry and dynamics in Jupiter's atmosphere. We believe that three out of the four questions (explanation of NH3 altitude profile, characterization of hot spots, altitude below which the atmosphere is uniformly mixed) may be solved from passive sounding of Jupiter's deep (∼ tens of bars) atmosphere via a radio telescope orbiting the planet. Question nr. 4 (the water abundance in Jupiter's deep atmosphere) has been singled out by the Solar System Exploration Decadal Survey as a key question, since the water abundance in Jupiter's deep atmosphere is tied in with planet formation models. In this paper we investigate the sensitivity of microwave retrievals to the composition of Jupiter's deep atmosphere, in particular the water abundance. Based upon present uncertainties in the ammonia abundance and other known and unknown absorbers, including uncertainties in clouds (density and index of refraction), and uncertainties in the thermal structure and lineshape profiles, we conclude that the retrieval of water at depth from microwave spectra (disk-averaged and locally) will be highly uncertain. We show that, if the H2O lineshape profile would be accurately known (laboratory data are needed!), an atmosphere with a near-solar H2O abundance can likely be distinguished from one with an abundance of 10-20×solar O based upon the difference in their microwave spectra at wavelengths ?50 cm. This would be sufficient to distinguish between some proposed scenarios by which Jupiter acquired its inventory of volatile elements heavier than helium. If, in addition, limb-darkening measurements are obtained (again, the H2O lineshape profile should be known), tighter constraints on the H2O abundance can be obtained (see also Janssen et al., 2004, this issue).  相似文献   

10.
An accessible model for interstellar OH/H2O maser associations is presented. It can be classified into radiative pumping model. It can close the dynamical cycle of H2O and OH species, and can give an interpretation on interstellar OH/H2O associations. A reasonable scheme for both regeneration and destruction of interstellar H2O and OH molecules is argued. Our model has overcome the defects of former radiative models, and is compatible with astronomical conditions. It is shown that the rotational population of H2O and OH in these regions is much less affected by collisions than by radiation. Some experiments have confirmed our proposal.  相似文献   

11.
Joel S. Levine 《Icarus》1976,28(2):165-169
The presence of 28% argon on Mars as calculated by Levine and Riegler and indirectly inferred from Soviet Mars-6 lander data has important implications for the outgassing history of H2O, CO2, and N2 on Mars. Even if the terrestrial volatile outgassing ratio is only approximately valid for Mars, then large quantities of H2O [of the order of 105 gcm?2 (about 108 more H2O than is currently present in the Martian atmosphere)] and about 104 gcm?2 of CO2 (about 103 times more CO2 than found at present in the Martian atmosphere) and some 450 gcm?2 of N2 may have outgassed over the history of Mars.  相似文献   

12.
The evolution of the martian atmosphere with regard to its H2O inventory is influenced by thermal loss processes of H, H2, nonthermal atmospheric loss processes of H+, H2+, O, O+, CO2, and O2+ into space, as well as by chemical weathering of the surface soil. The evolution of thermal and nonthermal escape processes depend on the history of the intensity of the solar XUV radiation and the solar wind density. Thus, we use actual data from the observation of solar proxies with different ages from the Sun in Time program for reconstructing the Sun's radiation and particle environment from the present to 3.5 Gyr ago. The correlation between mass loss and X-ray surface flux of solar proxies follows a power law relationship, which indicates a solar wind density up to 1000 times higher at the beginning of the Sun's main sequence lifetime. For the study of various atmospheric escape processes we used a gas dynamic test particle model for the estimation of the pick up ion loss rates and considered pick up ion sputtering, as well as dissociative recombination. The loss of H2O from Mars over the last 3.5 Gyr was estimated to be equivalent to a global martian H2O ocean with a depth of about 12 m, which is smaller than the values reported by previous studies. If ion momentum transport, a process studied in detail by Mars Express is significant on Mars, the water loss may be enhanced by a factor of about 2. In our investigation we found that the sum of thermal and nonthermal atmospheric loss rates of H and all nonthermal escape processes of O to space are not compatible with a ratio of 2:1, and is currently close to about 20:1. Escape to space cannot therefore be the only sink for oxygen on Mars. Our results suggest that the missing oxygen (needed for the validation of the 2:1 ratio between H and O) can be explained by the incorporation into the martian surface by chemical weathering processes since the onset of intense oxidation about 2 Gyr ago. Based on the evolution of the atmosphere-surface-interaction on Mars, an overall global surface sink of about 2×1042 oxygen particles in the regolith can be expected. Because of the intense oxidation of inorganic matter, this process may have led to the formation of considerable amounts of sulfates and ferric oxides on Mars. To model this effect we consider several factors: (1) the amount of incorporated oxygen, (2) the inorganic composition of the martian soil and (3) meteoritic gardening. We show that the oxygen incorporation has also implications for the oxidant extinction depth, which is an important parameter to determine required sampling depths on Mars aimed at finding putative organic material. We found that the oxidant extinction depth is expected to lie in a range between 2 and 5 m for global mean values.  相似文献   

13.
Exchange of CO2 and H2O between the Mars regolith and the atmosphere-cap system plays an important role in governing the evolution of the martian atmosphere and the martian climate. Most of the exchangeable CO2 (perhaps one or two orders of magnitude more than the atmospheric inventory) is currently adsorbed on the deep regolith, and can be “cryopumped” to a large quasipermanent CO2 cap (not now present) during lowest Mars obliquity (θ). During the obliquity driven regolith-cap CO2 exchange cycle, the atmospheric pressure varies harmonically between ~0.1 mb (lowest Θ) and ? 20 mb (highest Θ). The regolith buffer plays only a small or negligible role in the seasonal CO2 pressure variations caused by atmosphere-cap exchange because adsorption greatly inhibits diffusion of the seasonal “pressure wave” into the regolith. In contrast, thermally driven H2O seasonal exchange between the atmosphere and regolith appears to be in large part responsible for observed seasonal variations in the small atmospheric H2O inventory. Long term exchange of H2O may be dominated by transfer between the polar caps and ice in the regolith. Available and potential tests of regolith-atmospheric-cap volatile exchange models using ground-based and spacecraft-based techniques are discussed.  相似文献   

14.
The atmospheric transmission window at 2.7 μm in Jupiter's atmosphere was observed at a spectral resolution of 0.1 cm?1 from the Kuiper Airborne Observatory. From analysis of the CH4 abundance (～80m-am) and the H2O abundance (<0.0125cm-am) it was determined that the penetration depth of solar flux at 2.7 μm is near the base of the NH3 cloud layer. The upper limit to H2O at 2.7 μm and other recent results suggest that photolytic reactions in Jupiter's lower troposphere may not be as significant as was previously thought. The search for H2S in Jupiter's atmosphere yielded an upper limit of ～0.1cm-am. The corresponding limit to the elemental abundance ratio [S]/[H] was ～1.7 × 10?8, about 10?3 times the solar value. Upon modeling the abundance and distribution of H2S in Jupiter's atmosphere it was concluded that, contrary to expectations, sulfur-bearing chromophores are not present in significant amounts in Jupiter's visible clouds. Rather, it appears that most of Jupiter's sulfur is locked up as NH4SH in a lower cloud layer. Alternatively, the global abundance of sulfur in Jupiter may be significantly depleted.  相似文献   

15.
We report laboratory studies on the 0.8 MeV proton irradiation of ices composed of sulfuric acid (H2SO4), sulfuric acid monohydrate (H2SO4·H2O), and sulfuric acid tetrahydrate (H2SO4·4H2O) between 10 and 180 K. Using infrared spectroscopy, we identify the main radiation products as H2O, SO2, (S2O3)x, H3O+, , and . At high radiation doses, we find that H2SO4 molecules are destroyed completely and that H2SO4·H2O is formed on subsequent warming. This hydrate is significantly more stable to radiolytic destruction than pure H2SO4, falling to an equilibrium relative abundance of 50% of its original value on prolonged irradiation. Unlike either pure H2SO4 or H2SO4·H2O, the loss of H2SO4·4H2O exhibits a strong temperature dependence, as the tetrahydrate is essentially unchanged at the highest irradiation temperatures and completely destroyed at the lowest ones, which we speculate is due to a combination of radiolytic destruction and amorphization. Furthermore, at the lower temperatures it is clear that irradiation causes the tetrahydrate spectrum to transition to one that closely resembles the monohydrate spectrum. Extrapolating our results to Europa’s surface, we speculate that the variations in SO2 concentrations observed in the chaotic terrains are a result of radiation processing of lower hydration states of sulfuric acid and that the monohydrate will remain stable on the surface over geological times, while the tetrahydrate will remain stable in the warmer regions but be destroyed in the colder regions, unless it can be reformed by other processes, such as thermal reactions induced by diurnal cycling.  相似文献   

16.
Mm-wave spectra of HDO in the Venus mesosphere (65-100 km) were obtained over the period March 1998 to June 2004. Each spectrum is a measurement of the hemispheric-average H2O vapor mixing ratio in the Venus mesosphere. Observations were conducted for wide ranges of Venus solar elongations (46° W to 47° E), and fractional disk illuminations (f=0% to 99%), yielding water vapor abundances on 17 dates and over a full range of local solar time (LST) at the sub-Earth point on Venus. Our mesopheric H2O values are more numerous and far more precise than the earliest mm-derived H2O measurements [Encrenaz, Th., Lellouch, E., Paubert, G., Gulkis, S., 1991. First detection of HDO in the atmosphere of Venus at radio wavelengths: An estimate of the H2O vertical distribution. Astron. Astrophys. 246, L63-L66; Encrenaz, Th., Lellouch, E., Cernicharo, J., Paubert, G., Gulkis, S., Spilker, T., 1995. The thermal profile and water abundance in the Venus mesosphere from H2O and HDO millimeter observations. Icarus 117, 162-172], allowing an analysis of variability that was previously impossible. Measured 65-100 km H2O ranged from 0.0±0.06 to 3.5±0.3 ppmv, with significantly different variability than found in previous infrared (lower altitude, cloudtop) studies. Strong global variability on a 1-2 month timescale is clear and unambiguous. A limited number of excellent s/n measurements tentatively indicate the 1-2 month variability manifests most rapidly as change in the lower mesosphere, and more slowly as change in the upper mesosphere. Neither long term (1998-2004) nor diurnal variability in 65-100 km H2O is evident. While six-year and/or diurnal variabilities are not ruled out, they are weaker than the 1-2 month timescale variation. These conclusions are supported by initial (2004) sub-mm measurements.  相似文献   

17.
《Icarus》1986,67(1):19-36
A quantitative model of the state, distribution, and migration of water in the shallow Martian regolith is presented. Reported results are confined to the region of the planet greater than 40° lat. The calculations take into account (1) expected thermal variations at all depths, latitudes, and times resulting from seasonal and astronomically induced insolation variations; (2) variations in atmospheric PH2O and PCO2 resulting from polar insolation variations and regolith adsorptive equilibria; (3) feedback effects related to latent heat and albedo variations resulting from condensation of atmospheric constituents; (4) two possible regolith mineralogies; (5) variable total H2O content of the regolith; (6) kinetics of H2O transport through the Martian atmosphere and regolith; and (7) equilibrium phase partitioning of H2O between the condensed, adsorbed, and vapor phases. Results suggest that the adsorptive capacity of the regolith is important in controlling the state and distribution of high-latitude H2O; unweathered mafic silicates favor the development of shallow ground ice at all temperate and polar latitudes, while heavily weathered clay-like regolith materials leads to a deeper ground ice interface and far more extensive quantities of adsorbed H2O. The capacity of the high-latitude regolith for storage of H2O and the total mass of H2O exchanged between the atmosphere, polar cap, and subsurface over an obliquity cycle is found to be relatively independent of mineralogy. The maximum exchanged volume is found to be 3.0 × 104 km3 of ice per cycle. Implications for the history of the polar caps and the origin of the layered terrain are discussed. Results also suggest that seasonal thermal waves act to force adsorbed H2O into the solid phase over a wide variety of latitude/obliquity conditions. Seasonal phase cycling of regolith H2O is most common at high latitudes and obliquities. Such phase behavior is highly dependent on regolith mineralogy. In a highly weathered regolith, adsorbed H2O is annually forced into the solid phase at all latitudes ≥40° at obliquities greater than approximately 25°. Seasonal adsorption-freezing cycles which are predicted here may produce geomorphologic signatures not unlike those produced by terrestrial freeze-thaw cycles.  相似文献   

18.
A two-dimensional kinetic model calculation for the water group species (H2O, H2, O2, OH, O, H) in Europa's atmosphere is undertaken to determine its basic compositional structure, gas escape rates, and velocity distribution information to initialize neutral cloud model calculations for the most important gas tori. The dominant atmospheric species is O2 at low altitudes and H2 at higher altitudes with average day-night column densities of 4.5×1014 and 7.7×1013 cm−2, respectively. H2 forms the most important gas torus with an escape rate of ∼2×1027 s−1 followed by O with an escape rate of ∼5×1026 s−1, created primarily as exothermic O products from O2 dissociation by magnetospheric electrons. The circumplanetary distributions of H2 and O are highly peaked about the satellite location and asymmetrically distributed near Europa's orbit about Jupiter, have substantial forward clouds extending radially inward to Io's orbit, and have spatially integrated cloud populations of 4.2×1033 molecules for H2 and 4.0×1032 atoms for O that are larger than their corresponding populations in Europa's local atmosphere by a factor of ∼200 and ∼1000, respectively. The cloud population for H2 is a factor of ∼3 times larger than that for the combined cloud population of Io's O and S neutral clouds and provides the dominant neutral population beyond the so-called ramp region at 7.4-7.8 RJ in the plasma torus. The calculated brightness of Europa's O cloud on the sky plane is very dim at the sub-Rayleigh level. The H2 and O tori provide a new source of europagenic molecular and atomic pickup ions for the thermal plasma and introduce a neutral barrier in which new plasma sinks are created for the cooler iogenic plasma as it is transported radially outward and in which new sinks are created to alter the population and pitch angle distribution of the energetic plasma as it is transported radially inward. The europagenic instantaneous pickup ion rates are peaked at Europa's orbit, dominate the iogenic pickup ion rates beyond the ramp region, and introduce new secondary plasma source peaks in the solution of the plasma transport problem. The H2 torus is identified as the unknown Europa gas torus that creates both the observed loss of energetic H+ ions at Europa's orbit and the corresponding measured ENA production rate for H.  相似文献   

19.
The penetration in the terrestrial atmosphere of solar radiation corresponding to the spectral range of the Schumann-Runge bands of molecular oxygen is analyzed between 1750 and 2050 Å. The variation of the absorption cross section with temperature is taken into account and it is shown that average O2 absorption cross sections cannot lead to correct photodissociation coefficients. Reduction factors are defined in order to simplify the computation of the molecular oxygen photodissociation and to permit a simple determination of the photodissociation coefficients of any minor constituent with smoothly varying absorption cross section. Examples are given for O2, H2O, CO2, N2O, HNO3 and H2O2. Numerical approximations are developed for three types of spectral subdivisions: Schumann-Runge band intervals, 500 cm?1 and 10 Å intervals. The approximations are valid from the lower thermosphere down to the stratosphere and they can be applied for a wide range of atmospheric models and solar zenith distances.  相似文献   

20.
A 1-D collisional Monte Carlo model of Europa's atmosphere is described in which the sublimation and sputtering sources of H2O molecules and their molecular fragments are accounted for as well as the radiolytically produced O2. Dissociation and ionization of H2O and O2 by magnetospheric electron, solar UV-photon and photo-electron impact, and collisional ejection from the atmosphere by the low-energy plasma are taken into account. Reactions with the surface are discussed, but only adsorption and atomic oxygen recombination are included in this model. The size of the surface-bounded oxygen atmosphere of Europa is primarily determined by a balance between atmospheric sources from irradiation of the satellite's icy surface by the high-energy magnetospheric charged particles and atmospheric losses from collisional ejection by the low-energy plasma, photo- and electron-impact dissociation, and ionization and pick-up from the surface-bounded atmosphere. A range of sources rates for O2 to H2O are used with a larger oxygen-to-water ratio than suggested by laboratory measurements in order to account for differences in adsorption onto grains in the regolith. These calculations show that the atmospheric composition is determined by both the water and oxygen photochemistry in the near-surface region, escape of suprathermal oxygen and water into the jovian system, and the exchange of radiolytic water products with the porous regolith. For the electron impact ionization rates used, pick-up ionization is the dominant oxygen loss process, whereas photo-dissociation and atmospheric sputtering are the dominant sources of neutral oxygen for Europa's neutral torus. Including desorption and loss of water enhances the supply of oxygen species to the neutral torus, but hydrogen produced by radiolysis is the dominant source of neutrals for Europa's torus in these models.  相似文献   

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