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1.
The influence of biogenic emissions on tropospheric ozone production over Saxony (Germany) is studied using a coupled numerical modelling system. Emissions of hydrocarbons from forest areas as well as biogenic NO are considered. In an additional study the effect of VOC-emissions from rape fields on the ozone behaviour is estimated.  相似文献   

2.
A two-dimensional model of radiative, dynamical and photochemical processes in the atmosphere has been developed and used for the simulation of ozone distribution. The results of numerical simulations are compared with LIARS and TOMS measurements. The comparison shows that the overall agreement between simulated and LIARS stratospheric ozone data is within 5–15% for almost all of the stratosphere except for the high latitudes of the winter hemisphere. This kind of disagreement is a common problem for all 2-D models, which cannot resonably reproduce planetary and gravity wave breaking processes over high latitudes. Validation of the simulated total ozone against TOMS data also shows a good overall agreement. The the total ozone difference between the 2-D model results and TOMS measurements is within 5–10% in both Northern and Southern hemispheres during all seasons except 40°S-60°S from June to October. In this region, the difference between simulated and TOMS total ozone is 30%.  相似文献   

3.
Radio noise continuum emissions observed in metric and deca-metric wave frequencies are, in general, associated with actively varying sunspot groups accompanied by the S-component of microwave radio emissions. It is known that these continuum emission sources, often called type I storm sources, are often associated with type III burst storm activity from metric to hectometric wave frequencies. This storm activity is, therefore, closely connected with the development of these continuum emission sources.It is shown that the S-component emission in microwave frequencies generally precedes by several days the emission of these noise continuum storms of lower frequencies. In order for these storms to develop, the growth of sunspot groups into complex types is very important with the increase of the average magnetic field intensity and area of these groups. In particular, the types of these groups such as and are very important on the generation of noise continuum storm sources and sharp increase of the flux of these continuum emissions. This fact suggests that sunspot magnetic configuration and its variation, both space and time, are very effective on the growth of the sources for these noise continuum emissions.Although we have not known yet the true mechanism of these emissions, it is very likely that energetic electrons, 10 to 100 keV, accelerated in association with the variation of sunspot magnetic fields, are responsible as the sources of those radio emissions. Furthermore it seems that these electrons are contributing to the emission of type III burst storms, which are associated with the noise continuum storm sources. In explaining the origin of these storms, some plasma processes must be taken into consideration. Furthermore, it should be remarked that the storage mechanism of the electrons mentioned above plays an important role in generating both the noise continuum emissions and type III burst storms, because on-fringe type III bursts are all generated above these noise continuum storms sources. After reviewing the theories of these noise continuum storm emissions, a model is briefly considered to explain the relation between these continuums and type III bursts, and a discussion is given on the role of energetic electrons on these two emissions. It is pointed out that instabilities associated with these electrons and their relation to their own stabilizing effects are important in interpreting both of these storm emissions.Astrophysics and Space Science Review Paper.  相似文献   

4.
The rate of production of NO in the thermosphere is expected to vary greatly over the course of an 11-year solar cycle because the fluxes of both extreme ultraviolet radiation and auroral particles are known to increase substantially from solar minimum to solar maximum. In the stratosphere, NO participates in a catalytic cycle which constitutes the dominant photochemical destruction mechanism for stratospheric ozone. If appreciable long range transport of NO from the thermosphere to the upper stratosphere occurs, its effects should therefore be manifested in upper atmospheric ozone density variations over the 11-year solar cycle. In this paper, model predictions of the seasonal and latitudinal variations in upper stratospheric O3 associated with NO transport for different levels of solar activity are compared to satellite observations of upper stratospheric ozone abundances.  相似文献   

5.
The objective of this work is to study the influence of three mechanisms in the high surface concentration of the Spanish EMEP stations. These mechanisms are: Photochemical production from organic compounds and nitrogen oxides, exchange of air between the Planetary Boundary Layer and the free troposphere and the advection of ozone. To do this we have designed a new method that use multivariate analysis and the average ozone concentrations, NOx concentrations, lenght of the air mass trajectories reaching the stations and emissions of NOx. Results suggest that high surface ozone concentrations are controled by photochemical production if the source is close to the station. If the distance from the source to the station rises, the influence of the NOx emissions become more important.  相似文献   

6.
Modeling mineral dust emissions from Chinese and Mongolian deserts   总被引：6，自引：0，他引：6  
The present study investigates the frequency and intensity of mineral dust emissions over the deserts of eastern Asia from 1996 to 2001. Mineral dust emissions are simulated using a physical dust emission scheme over a region extending from 35.5°N to 47°N and from 73°E to 125°E. The input parameters required by the dust emission model are (1) surface features data including aerodynamic roughness length, soil dry size distribution and texture; and (2) meteorological surface data, mainly wind speed, soil moisture and snow cover. The way by which these surface features and meteorological data can be assessed is described and discussed. The influence of soil moisture and snow cover is taken into account and their effects on simulated dust emission are quantified.The simulations reproduce on a daily basis the location and intensity of the severe events of April 1998 and spring 2001 as recorded by the meteorological stations and/or described in various studies. Based on 6 yr of simulations, the main dust source regions are identified and their relative contributions to the total dust emissions are quantified.The seasonal cycle of the dust storms frequency is well reproduced with a maximum in spring. The simulations suggest that it is mainly controlled by the emissions occurring in the Taklimakan desert in latter spring and in summer, and by those occurring in the northern deserts of China in winter. The Taklimakan desert appears to be the most frequent and steady source of dust emissions during the studied period. On the other hand, in the Gobi desert, only a few dust emission events are simulated, but the dust amount emitted during each event is generally very large. In the northern deserts of China, dust emissions are frequent and their intensity is variable.These results show an important annual and inter-annual variability of the emitted dust (between 100 Mt yr− 1 and 460 Mt yr− 1), mainly controlled by the occurrence of severe events in the Gobi desert and in the northern deserts of China.  相似文献   

7.
Insight into the causes of the annual and semi-annual ozone oscillations may be gained from the analysis of photochemical model behavior. In this paper, the monthly variations of the ozone mixing ratio computed by the two-dimensional photochemical model of Garcia and Solomon (1983, J. geophys. Res. 88, 1379) are Fourier-analyzed and compared with SBUV observations of ozone mixing ratio. Remarkably good qualitative agreement between the model calculations and the observations is found. Analysis of computed transport and chemical production and destruction rates reveals the causes of the modelled seasonal ozone variations.

It will be shown that at high latitudes and low altitudes, modelled ozone abundances increase in the winter due to transport and decrease in the summer due to chemical destruction. In the middle stratosphere, the calculated annual ozone variation is largely due to the annual variation in the odd-oxygen production rate, and in the upper stratosphere, the computed annual ozone variation is caused by the large calculated annual oscillation in temperature. Comparison between the model and observations suggests that the equatorial semi-annual oscillation above 10 mb is caused mainly by the semi-annual temperature and wind oscillation (SAO). Below 10 mb the computed equatorial ozone variation is caused by the increased rates of odd-oxygen production associated with the semi-annual zenith crossings of the Sun. Finally, the calculated polar semi-annual ozone oscillations are found to be caused by modulation of the radiatively driven middle-stratospheric ozone variation by temperature dependent chemical destruction processes.  相似文献   


8.
Numerous fluorescent emissions from the Herzberg bands of molecular oxygen lie in the spectral region 242–300 nm. This coincides with the wavelength range used by orbiting spectrometers which observe the Rayleigh backscattered spectrum of the earth for the purpose of monitoring the vertical distribution of stratospheric ozone. Model calculations indicate that Herzberg band emissions in the dayglow could provide significant contamination of the ozone measurements if the quenching rate of O2(A3Σ) is sufficiently small. This is especially true near 255 nm, where the most intense fluorescent emissions relative to the Rayleigh scattered signal are located and where past satellite measurements show a persistent excess radiance above that expected for a pure ozone absorbing and molecular scattering atmosphere. However, very small quenching rates are adequate to reduce the dayglow emission to negligible levels. Available laboratory data have not definitely established the quenching on the rate of O2(A3Σ) as a function of vibrational level, and such information is required before the Herzberg band contributions can be evaluated with confidence.  相似文献   

9.
Geographical sources of surface ozone in five Spanish EMEP stations are studied using the air mass trajectories that arrive at the stations together with the CPFs (Conditional Probability Functions). Results show that regions with strong NOx emissions placed far away the stations are the main sources of ozone in Spain. So, the center of Europe and the middle Mediterranean area are the two main geographical sources of surface ozone in Spain.  相似文献   

10.
The properties of a sample of extragalactic OH maser sources over a wide spectral range are discussed. Based on a sample of 22 maser galaxies it is shown that OH, HCN, and x-ray emission are closely related. On the other hand, these emissions depend on the mass of the galactic nucleus. It is shown that the broadening of the OH emission line is caused by the rotation of the circumnuclear disk, dense regions of which serve as the sources of OH and HCN emission. X-ray heating can excite OH and HCN molecules.  相似文献   

11.
Xun Zhu  Jeng-Hwa Yee 《Icarus》2007,189(1):136-150
A one-dimensional photochemical-transport model for the martian lower atmosphere has been developed to study the diurnal cycles of wave-photochemistry coupling. The model self-consistently calculates water vapor mixing ratio profiles, which exhibit strong vertical and diurnal variations mainly due to the high sensitivity of the saturation vapor pressure to temperature variation. The dynamical coupling of water vapor caused by the temperature variation induced by tidal waves, vertical transport parameterized by eddy diffusion, and linear relaxation introduced in condensation-sublimation processes all have similar timescales of diurnal variation. This leads to a significant asymmetric distribution of water vapor concentration as a function of local time. As a result, the net effect of the temperature variation by tidal waves depletes the water vapor concentration in its diurnal mean. The coupling processes also deplete the diurnally averaged HOx concentration, which in turn leads to significant enhancements of both ozone concentration and the associated airglow emissions in the martian atmosphere. The model also shows explicitly the importance of photochemical-transport coupling to the airglow emissions and its implications in species retrievals when the photochemical times of the excited states are comparable to the timescale of diurnal variation.  相似文献   

12.
We present absolute abundances and latitudinal variations of ozone and water in the atmosphere of Mars during its late northern spring (Ls=67.3°) shortly before aphelion. Long-slit maps of the a1Δg state of molecular oxygen (O2) and HDO, an isotopic form of water, were acquired on UT January 21.6 1997 using a high-resolution infrared spectrometer (CSHELL) at the NASA Infrared Telescope Facility. O2(a1Δg) is produced by ozone photolysis, and the ensuing dayglow emission at 1.27 μm is used as a tracer for ozone. Retrieved vertical column densities for ozone above ∼20 km ranged between 1.5 and 2.8 μm-atm at mid- to low latitudes (30°S-60°N) and decreased outside that region. A significant decrease in ozone density is seen near 30°N (close to the subsolar latitude of 23.5°N). The rotational temperatures retrieved from O2(a-X) emissions show a mean of 172±2.5 K, confirming that the sensed ozone lies in the middle atmosphere (∼24 km). The ν1 fundamental band of HDO near 3.67 μm was used as a proxy for H2O. The retrieved vertical column abundance of water varies from 3 precipitable microns (pr-μm) at ∼30°S to 24 pr-μm at ∼60°N. We compare these results with current photochemical models and with measurements obtained by other methods.  相似文献   

13.
In this study we present the diurnal and monthly variations in the surface ozone concentrations of five Spanish remote stations belonging to the EMEP network. In two of the stations, a maximum in the afternoon is presented because of the turbulent mixing producing appreciable downward ozone flux. In other two stations no maxima are produced. In one of them this result is due to the strong westerly winds that dominate the air flow and the low solar insolation. In the other station the reason are two phenomena: the mountain induced flow regime that produce high concentrations during the night and the photochemical production that results in high concentrations during the afternoon.Four of the five considered stations show the typical natural spring maximum. This maximum extends into summer in two of the stations. In one of the stations the maximum is reached in summer and it is due to the proximity of the station to strong nitrogen oxide emission areas.  相似文献   

14.
The relativistic beaming model has been successfully used to explain many of the observational properties of active galactic nuclei. In this model the total emission is formed by two components, one beamed, one unbeamed. However, the exact contribution from each component in unresolved sources is still not clear. In the radio band, the core and extended emissions are clearly separated. We adopt the method proposed by Kembhavi to separate the two contributions in the X-ray emissions in a sample of 19 gamma-ray loud blazars. It is clearly shown that the beamed emission dominates the X-ray flux and the unbeamed X-ray emission is correlated with the extended radio emission of the considered objects. We also find that the ratio of the beamed to the unbeamed X-ray luminosity is correlated with the X-ray spectral index, an effect that should be a consequence of the underlying X-ray emission mechanism.  相似文献   

15.
P. Kaufmann 《Solar physics》1996,169(2):377-388
The time profiles of electromagnetic fluxes at hard X-rays and short microwaves are signatures of the energy conversion mechanisms at the origin of solar flares. The distinction between continuum and discrete energy production brings drastic conceptual consequences for the interpretation of the energy conversion processes. As more sensitive detectors were used on measurements with higher time resolution, the notion of continuum energy release in the impulsive phase is being replaced by the concept of repetitive energy production or Elementary Flare Bursts manifested at hard X-rays and by rapid time structures in microwave emissions. These discrete time structures are now known to be as short as tens of milliseconds, and part of their emissions are possibly produced by the same populations of accelerated electrons. Fast spikes, with mm-wave emission fluxes increasing for shorter wavelengths, simultaneous with hard X-rays, bring severe constraints for interpretation. This problem is reviewed, with the suggestion of a possible significant burst emission component in the sub-mm-IR range, due to primeval short-lived explosive compact sources, for which there are still no diagnostics.Dedicated to Cornelis de Jager  相似文献   

16.
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17.
Fluctuations in the brightness of the background radiation can lead to confusion with real point sources. This type of confusion with background emission is relevant when making infrared (IR) observations with relatively large beam sizes, since the amount of fluctuation tends to increase with the angular scale. To quantitively assess the effect of the background emission on the detection of point sources for current and future far-IR observations by space-borne missions such as Spitzer , ASTRO-F , Herschel and Space Infrared Telescope for Cosmology and Astrophysics ( SPICA ), we have extended the Galactic emission map to a higher level of angular resolution than that of the currently available data. Using this high-resolution map, we estimate the sky confusion noise owing to the emission from interstellar dust clouds or cirrus, based on fluctuation analysis and detailed photometry over realistically simulated images. We find that the confusion noise derived by simple fluctuation analysis agrees well with the results from realistic simulations. Although sky confusion noise becomes dominant in long wavelength bands  (>100 μm)  with 60–90 cm aperture missions, it is expected to be two orders of magnitude lower for the next generation of space missions (with larger aperture sizes) such as Herschel and SPICA .  相似文献   

18.
A review is given of the stratospheric budgets of odd oxygen, odd nitrogen, nitrous oxide, methane and carbonyl sulfide. The stratospheric column production rate of NO by the reaction N2O + O(1D) → 2 NO is 1.1–1.9 × 108 molecules cm?2 s?1. The stratospheric loss rates for N2O, CH4 and COS are equal to 0.9–1.4 × 109, 1 × 1010 and 0.5 × 107 molecules cm?2 s?1, respectively. From currently available information on the global distributions of N2O and CH4 there are some indications of about two times smaller OH concentrations below 35 km than those which are calculated based on the latest compilation of kinetic data.Most significantly, however, it is shown that photochemical models and available ozone observations cannot be reconciled and that there may be particularly severe problems in the 25–35 km region. This issue is thoroughly discussed.Volcanic emissions of SO2 to the stratosphere may locally lead to much enhanced ozone concentrations and heating rates. These may influence the dynamic behaviour of volcanic plumes before their dispersion over large volumes of the stratosphere.  相似文献   

19.
Fluorescent emissions from nitric oxide appear imposed upon the Rayleigh backscattered spectrum of the earth's atmosphere between 250 and 300 nm in wavelength. Satellite instruments designed to monitor the global ozone distribution can routinely observe these signals although techniques for exploiting the data are not yet available. Application of a radiative transfer equation developed for an atmosphere including absorption by ozone, molecular scattering, and nitric oxide fluorescence shows the three most prominent NO emissions relative to the 250–300 nm backscattered sunlight to be the (1,4), (1,6), and (0,3) gamma bands. Analysis of the contribution function for each emission band indicates that the fluorescent signals can provide useful information on the magnitude and variability of nitric oxide between 40 and 140 km in altitude.  相似文献   

20.
In Paper I, we presented a detailed formulation of the relativistic shocks and synchrotron emission in the context of gamma-ray burst (GRB) physics. To see how well this model reproduces the observed characteristics of the GRBs and their afterglows, here we present the results of some simulations based on this model. They are meant to reproduce the prompt and afterglow emissions in some intervals of time during a burst. We show that this goal is achieved for both short and long GRBs and their afterglows, at least for part of the parameter space. Moreover, these results are evidence of the physical relevance of the two phenomenological models we have suggested in Paper I for the evolution of the active region – synchrotron emitting region in a shock. The dynamical active region model seems to reproduce the observed characteristics of prompt emissions and late afterglow better than the quasi-steady model which is more suitable for the onset of afterglows. Therefore, these simulations confirm the arguments presented in Paper I about the behaviour of these models based on their physical properties.  相似文献   

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