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1.
The characteristics of net radiation (Rn)(0.3--10 μm) in Lhasa and Haibei in the Tibetan Plateau were analyzed based on long-term in-situ measurements of surface radiation data. The monthly average of daily Rn reached a minimum during the winter period followed by an increase until May and then a decline until January. This variation is consistent with solar activity. The annual mean daily total Rn values were 0.92 MJ m-2 d-1 and 0.66 MJ m-2d-1 in Lhasa and Haibei, respectively. A relationship between Rn and broadband solar radiation (Rs) was demonstrated by a good linear correlation at the two sites. Rn can be an accurate estimate from Rs. The estimated Rn values were similar to the observed values, and the relative deviations between the estimates and measurements of Rn were 2.8% and 3.8% in Lhasa and Haibei, respectively. The application of the Rn estimating model to other locations showed that it could provide acceptable estimated Rn values from the Rs data. Furthermore, we analyzed the influence of clouds on Rn by different clear index (Ks), defined as the ratio of Rs to the extraterrestrial solar irradiance on a horizontal surface. The results indicate that more accurate results are associated with increased cloudy conditions. The influence of the albedo was also considered, but its inclusion in the model resulted in only a slight improvement. Because surface albedo is not usually measured, an expression based solely on global solar radiation could be of more extensive use.  相似文献   

2.
Results from large-eddy simulations and field measurements have previously shown that the velocity field is influenced by the boundary layer height, z i , during close to neutral, slightly unstable, atmospheric stratification. During such conditions the non-dimensional wind profile, φ m , has been found to be a function of both z/L and z i /L. At constant z/L, φ m decreases with decreasing boundary layer height. Since φ m is directly related to the parameterizations of the air–sea surface fluxes, these results will have an influence when calculating the surface fluxes in weather and climate models. The global impact of this was estimated using re-analysis data from 1979 to 2001 and bulk parameterizations. The results show that the sum of the global latent and sensible mean heat fluxes increase by 0.77 W m−2 or about 1% and the mean surface stress increase by 1.4 mN m−2 or 1.8% when including the effects of the boundary layer height in the parameterizations. However, some regions show a larger response. The greatest impact is found over the tropical oceans between 30°S and 30°N. In this region the boundary layer height influences the non-dimensional wind profile during extended periods of time. In the mid Indian Ocean this results in an increase of the mean annual heat fluxes by 2.0 W m−2 and an increase of the mean annual surface stress by 2.6 mN m−2.  相似文献   

3.
Profiles of wind and turbulence over an urban area evolve with fetch in response to surface characteristics. Sodar measurements, taken on 22 April 2002 during the Salford Experiment in the UK (Salfex), are here related to upstream terrain. A logarithmic layer up to z = 65m was observed in all half-hour averaged profiles. Above this height the profile showed a different vertical gradient, suggesting a change in surface cover upstream. The drag coefficient varied by a factor of two over only a 20° direction change. Turbulence intensity (σ x ) for each wind component (x) decreased with height, but the ratio suggested an underestimate of σ u compared to previous results. Mean urban and suburban cover fraction within the source area for each height decreased sharply between z = 20 and 50m, increasing slightly above. The near-convergence of cover fractions thus occured for source areas of minimum length ≈ 2,200 m. In comparison, the mean length scale of heterogeneity L P was calculated from surface cover data to be 1,284 m, and the corresponding mean blending height h b was 175 m. Finally, the mean streamline angle, α, was negative and the magnitude decreased with height. An exponential fit to α for z ≤ 65m gave an e-folding height scale of 159 m. A simple relationship between this height scale and L P was assumed, giving L P ≈ 1,080 m, which is in reasonable agreement with the estimate from surface cover type. The results suggest that more emphasis is required on modelling and measuring surface-layer flow over heterogeneous urban canopies.  相似文献   

4.
To understand the response of the Greenland ice sheet to climate change the so-called ablation zone is of particular importance, since it accommodates the yearly net surface ice loss. In numerical models and for data analysis, the bulk aerodynamic method is often used to calculate the turbulent surface fluxes, for which the aerodynamic roughness length (z 0) is a key parameter. We present, for the first time, spatial and temporal variations of z 0 in the ablation area of the Greenland ice sheet using year-round data from three automatic weather stations and one eddy-correlation mast. The temporal variation of z 0 is found to be very high in the lower ablation area (factor 500) with, at the end of the summer melt, a maximum in spatial variation for the whole ablation area of a factor 1000. The variation in time matches the onset of the accumulation and ablation season as recovered by sonic height rangers. During winter, snow accumulation and redistribution by snow drift lead to a uniform value of z 0≈ 10−4 m throughout the ablation area. At the beginning of summer, snow melt uncovers ice hummocks and z 0 quickly increases well above 10−2 m in the lower ablation area. At the end of summer melt, hummocky ice dominates the surface with z 0 > 5  ×  10−3 m up to 60 km from the ice edge. At the same time, the area close to the equilibrium line (about 90 km from the ice edge) remains very smooth with z 0 = 10−5 m. At the beginning of winter, we observed that single snow events have the potential to lower z 0 for a very rough ice surface by a factor of 20 to 50. The total surface drag of the abundant small-scale ice hummocks apparently dominates over the less frequent large domes and deep gullies. The latter results are verified by studying the individual drag contributions of hummocks and domes with a drag partition model.  相似文献   

5.
A time series of microwave radiometric profiles over Arctic Canada’s Cape Bathurst (70°N, 124.5°W) flaw lead polynya region from 1 January to 30 June, 2008 was examined to determine the general characteristics of the atmospheric boundary layer in winter and spring. A surface based or elevated inversion was present on 97% of winter (January–March) days, and on 77% of spring (April–June) days. The inversion was the deepest in the first week of March (≈1100 m), and the shallowest in June (≈250 m). The mean temperature and absolute humidity from the surface to the top of the inversion averaged 250.1 K (−23.1°C), and 0.56 × 10−3 kg m−3 in winter, and in spring averaged 267.5 K (−5.6°C), and 2.77 × 10−3 kg m−3. The median winter atmospheric boundary-layer (ABL) potential temperature profile provided evidence of a shallow, weakly stable internal boundary layer (surface to 350 m) topped by an inversion (350–1,000 m). The median spring profile showed a shallow, near-neutral internal boundary layer (surface to 350 m) under an elevated inversion (600–800 m). The median ABL absolute humidity profiles were weakly positive in winter and negative in spring. Estimates of the convergence of sensible heat and water vapour from the surface that could have produced the turbulent internal boundary layers of the median profiles were 0.67 MJ m−2 and 13.1 × 10−3 kg m−2 for the winter season, and 0.66 MJ m−2 and 33.4 × 10−3 kg m−2 for the spring season. With fetches of 10–100 km, these accumulations may have resulted from a surface sensible heat flux of 15–185 W m−2, plus a surface moisture flux of 0.001–0.013 mm h−1 (or a latent heat flux of 0.7–8.8 W m−2) in winter, and 0.003–0.033 mm h−1 (or a latent heat flux of 2–22 W m−2) in spring.  相似文献   

6.
Summary  Turbulent fluxes of CO2 were continuously measured by eddy correlation for three months in 1997 over a gramineous fen in a high-arctic environment at Zackenberg (74°28′12″N, 20°34′23″W) in NE-Greenland. The measurements started on 1 June, when there was still a 1–2 m cover of dry snow, and ended 26 August at a time that corresponds to late autumn at this high-arctic site. During the 20-day period with snow cover, fluxes of CO2 to the atmosphere were small, typically 0.005 mg CO2 m−2 s−1 (0.41 g CO2 m−2 d−1), wheres during the thawed period, the fluxes displayed a clear diurnal variation. During the snow-free period, before the onset of vegetation growth, fluxes of CO2 to the atmosphere were typically 0.1 mg CO2 m−2 s−1 in the afternoon, and daily sums reached values up to almost 9 g CO2 m−2 d−1. After 4 July, downward fluxes of CO2 increased, and on sunny days in the middle of the growing season, the net ecosystem exchange rates attained typical values of about −0.23 mg m−2 s−1 at midday and max values of daily sums of −12 g CO2 m−2 d−1. Throughout the measured period the fen ecosystem acted as a net-sink of 130 g CO2 m−2. Modelling the ecosystem respiration during the season corresponded well with eddy correlation and chamber measurements. On the basis of the eddy correlation data and the predicted respiration effluxes, an estimate of the annual CO2 balance the calender year 1997 was calculated to be a net-sink of 20 g CO2 m−2 yr−1. Received October 6, 1999 Revised May 2, 2000  相似文献   

7.
This paper presents meteorological measurements made during the antarctic summer period, on two 9 m and 3 m towers, on the rocky and ice shelf terrains of the Indian antarctic stations Maitri and Dakshin Gangotri, respectively. The measurements of fluctuations in temperature and wind speed made with relatively lesser precision instrumentation pertain to smaller wave numbers ~10-2 m-1 appropriate to outer scale L 0 of the atmospheric turbulence spectrum. Autocorrelation analysis of the fluctuations in temperature and wind speed has been performed. A new autoregressive scheme has been developed to represent the computed autocorrelation functions by a Yule statistical model, and to estimate the correlation period T 0 of the turbulent medium. Height profiles of outer scale L 0 of turbulence may be given in terms of T 0 and mean wind speed u. Further, the similarity theory of Monin-Obukhov has been used to compute height profiles of temperature structure parameter C T 2. At Maitri, values of L 0 and C T 2 are higher between 03–22 h local time than between 22–03 h. Values of L 0 and C T 2 are smaller over the ice shelf terrain of the Dakshin Gangotri station, compared to those over the rocky terrain of the Maitri station.  相似文献   

8.
We use a reduced complexity climate model with a three-dimensional ocean component and realistic topography to investigate the effect of stratification-dependent mixing on the sensitivity of the North Atlantic subpolar gyre (SPG), and the Atlantic meridional overturning circulation (AMOC), to idealized CO2 increase and peaking scenarios. The vertical diffusivity of the ocean interior is parameterized as κ ∼ N −α, where N is the local buoyancy frequency. For all parameter values 0 ≤ α ≤ 3, we find the SPG, and subsequently the AMOC, to weaken in response to increasing CO2 concentrations. The weakening is significantly stronger for α ≥ αcr ≈ 1.5. Depending on the value of α, two separate model states develop. These states remain different after the CO2 concentration is stabilized, and in some cases even after the CO2 concentration has been decreased again to the pre-industrial level. This behaviour is explained by a positive feedback between stratification and mixing anomalies in the Nordic Seas, causing a persistent weakening of the SPG.  相似文献   

9.
Rainfall variability and kinetic energy in Southern Nigeria   总被引：1，自引：1，他引：0  
A decreasing trend of rainfall has been observed in West Africa, where rainfall erosivity is also considered to be high. Therefore, this study was carried out to evaluate the variability of rainfall and its erosivity in two contrasting zones in southern Nigeria between 1977 and 1999 to understand the implications of climate variability on rainfall erosivity. The study sites were Ibadan, a sub-humid zone, and Port-Harcourt, a humid zone. Time of occurrence of rainfall, rainfall amount (A), intensity (I 15 and I 30), kinetic energy (E) and rainfall erosivity factor (R), were evaluated. Kinetic energy was estimated with Brown–Foster (BF) equation, making the rainfall erosivity (product of kinetic energy and intensity) to be designated as EI 30-BF and EI 15-BF. The frequency of rainfall during daylight (06:00–18:00 h) was 48% for Ibadan and 69% for Port-Harcourt. There were time-specific differences in daily rainfall occurrence between the zones, suggesting a strong influence of local effects on rainfall generation, such as, relief in Ibadan and proximity to the sea in Port-Harcourt. Annual E was 213 MJ ha−1for Ibadan and 361 MJ ha−1 for Port-Harcourt. Ibadan had a significantly higher daily E than Port-Harcourt because of higher intensity while Port-Harcourt had significantly higher annual E than Ibadan because of higher annual rainfall amount. Annual erosivity at Ibadan using the EI 30-BF was 9,742 MJ mm ha−1 h−1 whereas it was 15,752 MJ mm ha−1 h−1 at Port-Harcourt. Using the EI 15-BF, Ibadan had an annual value of 14,806 MJ mm ha−1 h−1 while Port-Harcourt had 20,583 MJ mm ha−1 h−1. Thus, annual rainfall erosivity was significantly higher in the humid than the sub-humid zone because of higher amount of rainfall but the reverse was the case with daily erosivity because of higher intensities in the sub-humid zone. Rainfall intensity was, therefore, a key measure of erosivity. There was a strong positive relationship between rainfall erosivity and rainfall amount. Between 1977 and 1988, 50–88% of the 12 years had rainfall erosivity which exceeded the long-term average but rainfall erosivity was less than the long-term average between 1989 and 1999. This suggested a decreasing trend in erosivity due to the decreasing trend in rainfall amount in West Africa. However, the trend did not imply lesser soil erosion and environmental degradation risks.  相似文献   

10.
Aerosol and rain samples were collected between 48°N and 55°S during the KH-08-2 and MR08-06 cruises conducted over the North and South Pacific Ocean in 2008 and 2009, to estimate dry and wet deposition fluxes of atmospheric inorganic nitrogen (N). Inorganic N in aerosols was composed of ~68% NH4+ and ~32% NO3– (median values for all data), with ~81% and ~45% of each species being present on fine mode aerosol, respectively. Concentrations of NH4+ and NO3− in rainwater ranged from 1.7–55 μmol L−1 and 0.16–18 μmol L−1, respectively, accounting for ~87% by NH4+ and ~13% by NO3− of total inorganic N (median values for all data). A significant correlation (r = 0.74, p < 0.05, n = 10) between NH4+ and methanesulfonic acid (MSA) was found in rainwater samples collected over the South Pacific, whereas no significant correlations were found between NH4+ and MSA in rainwater collected over the subarctic (r = 0.42, p > 0.1, n = 6) and subtropical (r = 0.33, p > 0.5, n = 6) western North Pacific, suggesting that emissions of ammonia (NH3) by marine biological activity from the ocean could become a significant source of NH4+ over the South Pacific. While NO3− was the dominant inorganic N species in dry deposition, inorganic N supplied to surface waters by wet deposition was predominantly by NH4+ (42–99% of the wet deposition fluxes for total inorganic N). We estimated mean total (dry + wet) deposition fluxes of atmospheric total inorganic N in the Pacific Ocean to be 32–64 μmol m−2 d−1, with 66–99% of this by wet deposition, indicating that wet deposition plays a more important role in the supply of atmospheric inorganic N than dry deposition.  相似文献   

11.
High-resolution water vapour measurements made by the Atmospheric Radiation Measurement (ARM) Raman lidar operated at the Southern Great Plains Climate Research Facility site near Lamont, Oklahoma, U.S.A. are presented. Using a 2-h measurement period for the convective boundary layer (CBL) on 13 September 2005, with temporal and spatial resolutions of 10 s and 75 m, respectively, spectral and autocovariance analyses of water vapour mixing ratio time series are performed. It is demonstrated that the major part of the inertial subrange was detected and that the integral scale was significantly larger than the time resolution. Consequently, the major part of the turbulent fluctuations was resolved. Different methods to retrieve noise error profiles yield consistent results and compare well with noise profiles estimated using Poisson statistics of the Raman lidar signals. Integral scale, mixing-ratio variance, skewness, and kurtosis profiles were determined including error bars with respect to statistical and sampling errors. The integral scale ranges between 70 and 130 s at the top of the CBL. Within the CBL, up to the third order, noise errors are significantly smaller than sampling errors and the absolute values of turbulent variables, respectively. The mixing-ratio variance profile rises monotonically from ≈0.07 to ≈3.7 g2 kg−2 in the entrainment zone. The skewness is nearly zero up to 0.6 z/z i , becomes −1 around 0.7–0.8 z/z i , crosses zero at about 0.95 z/z i , and reaches about 1.7 at 1.1 z/z i (here, z is the height and z i is the CBL depth). The noise errors are too large to derive fourth-order moments with sufficient accuracy. Consequently, to the best of our knowledge, the ARM Raman lidar is the first water vapour Raman lidar with demonstrated capability to retrieve profiles of turbulent variables up to the third order during daytime throughout the atmospheric CBL.  相似文献   

12.
The Summer Surface Energy Balance of the High Antarctic Plateau   总被引：1，自引：0，他引：1  
The summertime surface energy balance (SEB) at Kohnen station, situated on the high Antarctic plateau (75°00′ S, 0°04′ E, 2892m above sea level) is presented for the period of 8 January to 9 February 2002. Shortwave and longwave radiation fluxes were measured directly; the former was corrected for problems associated with the cosine response of the instrument. Sensible and latent heat fluxes were calculated using the bulk method, and eddy-correlation measurements and the modified Bowen ratio method were used to verify these calculated fluxes. The calculated sub-surface heat flux was checked by comparing calculated to measured snow temperatures. Uncertainties in the measurements and energy-balance calculations are discussed. The general meteorological conditions were not extraordinary during the period of the experiment, with a mean 2-m air temperature of −27.5°C, specific humidity of 0.52×10−3kg kg−1 and wind speed of 4.1ms−1. The experiment covered the transition period from Antarctic summer (positive net radiation) to winter (negative net radiation), and as a result the period mean net radiation, sensible heat, latent heat and sub-surface heat fluxes were small with values of −1.1, 0.0, −1.0 and 0.7 Wm−2, respectively. Daily mean net radiation peaked on cloudy days (16 Wm−2) and was negative on clear-sky days (minimum of −19 W m−2). Daily mean sensible heat flux ranged from −8 to +10 Wm−2, latent heat flux from −4 to 0 Wm−2 and sub-surface heat flux from −8 to +7 Wm−2.  相似文献   

13.
Previous measurements of urban energy balances generally have been limited to densely built, central city sites and older suburban locations with mature tree canopies that are higher than the height of the buildings. In contrast, few data are available for the extensive, open vegetated types typical of low-density residential areas that have been newly converted from rural land use. We made direct measurements of surface energy fluxes using the eddy-covariance technique at Greenwood, a recently developed exurban neighbourhood near Kansas City, Missouri, USA, during an intensive field campaign in August 2004. Energy partitioning was dominated by the latent heat flux under both cloudy and near clear-sky conditions. The mean daytime Bowen ratio (β) values were 0.46, 0.48, and 0.47 respectively for the cloudy, near clear-sky and all-sky conditions. Net radiation (R n ) increased rapidly from dawn (−34 and −58W m−2) during the night to reach a maximum (423 and 630W m−2) after midday for cloudy and near clear-sky conditions respectively. Mean daytime values were 253 and 370W m−2, respectively for the cloudy and near clear-sky conditions, while mean daily values were 114 for cloudy and 171W m−2 for near clear-sky conditions, respectively. Midday surface albedo values were 0.25 and 0.24 for the cloudy and near clear-sky conditions, respectively. The site exhibited an angular dependence on the solar elevation angle, in contrast to previous observations over urban and suburban areas, but similar to vegetated surfaces. The latent heat flux (Q E ), sensible heat flux (Q H ), and the residual heat storage ΔQ s terms accounted for between 46–58%, 21–23%, and 18–31% of R n , respectively, for all-sky conditions and time averages. The observed albedo, R n , and Q E values are higher than the values that have been reported for suburban areas with high summer evapotranspiration rates in North America. These results suggest that the rapidly growing residential areas at the exurban fringe of large metropolitan areas have a surface energy balance that is more similar to the rural areas from which they were developed than it is to the older suburbs and city centres that make up the urban fabric to which they are being joined.  相似文献   

14.
The present study investigates the chemical composition of wet atmospheric precipitation samples on a daily and an intra-event timescales in Opme, an experimental meteorological station located near Clermont-Ferrand, France. The samples have been collected from November 2005 to October 2007. A total of 217 rainwater samples, integrated for 24 h, were collected and analyzed for pH, conductivity, Na+, K+, Mg2+, NH4+, Ca2+, Cl−, NO3− , SO42− , PO43− and HCO3−. The composition of the rainwater collected appeared to be controlled by the following potential sources: neutralisation process (association among calcium, ammonium with nitrate and sulphate), marine and terrestrial sources. In order to determine the role of long-range transport, the integrated events were classified according to four origins of air-masses: (1) West, (2) North and East, (3) South including Iberian and Italian Peninsulae and (4) local. This analysis allows identifying the source areas of the different association of elements defined. Although calcium is always dominant, total content of rainfall is variable and neutralisation process can be more or less efficient and specific. Rainout (long-range transport) and washout (below-cloud scavenging) were investigated through intra-event measurements of chemical species. Four rain-events have been selected according to the four classes of origins of air-masses. It appears that the first fractions are responsible for an important part of the chemical content of the whole event. Terrestrial species, locally emitted, induce the neutralisation process of acid species. Local meteorological conditions, such as wind’s speed and direction, play an important role as they could provoke recharges of the below cloud air column during the event.  相似文献   

15.
A suite of active and passive remote sensing instruments and in-situ sensors deployed at the SIRTA Observatory (Instrumented Site for Atmospheric Remote Sensing Research), near Paris, France, for a period of six months (October 2006–March 2007) document simultaneously radiative, microphysical and dynamic processes driving the continental-fog life cycle. The study focuses on a 6-day period between 23 and 29 December 2006 characterized by several stratus-cloud lowering and lifting events and almost 18 h of visibility below 1 km. Conceptual models and different possible scenarios are presented here to explain the formation, the development and the dissipation phases of three major stratus–fog events and to quantify the impact of each driving process. For example, slowly evolving large-scale conditions characterized by a slow continuous cloud-base lowering, followed by a rapid transient period conductive to fog formation and dissipation, are observed for cases 1 and 3. During this stable period, continuous cloud-top radiative cooling (≈ −160 Wm−2) induces a progressive and slow lowering of the cloud base: larger droplets at cloud top (cloud reflectivity approximately equals to −20 dBZ) induce slow droplet fall to and beyond cloud base (Doppler velocity ≈ −0.1 ms−1), cooling the sub-cloud layer by evaporation and lowering the saturation level to 100 m (case 1) or to the surface (cases 2 and 3). Suddenly, a significant increase in Doppler velocity magnitude ≈ −0.6 ms−1 and of turbulent kinetic energy dissipation rate around 10−3 m2s−3 occurs at cloud base (case 1). These larger cloud droplets reach the surface leading to fog formation over 1.5 h. The Doppler velocity continues to increase over the entire cloud depth with a maximum value of around −1 ms−1 due to the collection of fog droplets by the drizzle drops with high collection efficiency. As particles become larger, they fall to the ground and lead to fog dissipation. Hence, falling particles play a major role in both the formation and also in the dissipation of the fog. These roles co-exist and the balance is driven by the characteristics of the falling particles, such as the concentration of drizzle drops, the size distribution of drizzle drops compared to fog droplets, Doppler velocity and thermodynamic state close to the surface.  相似文献   

16.
Measurements of atmospheric turbulence made during the Surface Heat Budget of the Arctic Ocean Experiment (SHEBA) are used to examine the profile stability functions of momentum, φ m , and sensible heat, φ h , in the stably stratified boundary layer over the Arctic pack ice. Turbulent fluxes and mean meteorological data that cover different surface conditions and a wide range of stability conditions were continuously measured and reported hourly at five levels on a 20-m main tower for 11 months. The comprehensive dataset collected during SHEBA allows studying φ m and φ h in detail and includes ample data for the very stable case. New parameterizations for φ m (ζ) and φ h (ζ) in stable conditions are proposed to describe the SHEBA data; these cover the entire range of the stability parameter ζ = z/L from neutral to very stable conditions, where L is the Obukhov length and z is the measurement height. In the limit of very strong stability, φ m follows a ζ 1/3 dependence, whereas φ h initially increases with increasing ζ, reaches a maximum at ζ ≈ 10, and then tends to level off with increasing ζ. The effects of self-correlation, which occur in plots of φ m and φ h versus ζ, are reduced by using an independent bin-averaging method instead of conventional averaging.  相似文献   

17.
The scaling laws of the vertical (F wc ) and longitudinal (F uc ) velocity-scalar cospectra within the inertial subrange are explored using dimensional arguments and a simplified cospectral budget in the canopy sublayer above three distinct forested ecosystems. The cospectral budget was shown to be consistent with plausible scaling laws originating from dimensional considerations. Using the analytical solution to the novel cospectral budget, it was shown that F wc (k) and F uc (k) are governed by the linear superposition of two terms that scale as k −2/3−α and k −β , where k is the wavenumber, −α is the exponent of the velocity spectrum, and β( ≥ 7/3) depends on the ratio of the similarity constants for the pressure-scalar covariance and the flux transport terms. It was also demonstrated that, when the magnitude of the mean scalar concentration gradient is large, the k −2/3−α term dominates the velocity-scalar cospectral budget. For such a case, correcting for biases emerging from high frequency losses in eddy-covariance scalar flux measurements can be readily formulated by using the measured velocity spectral exponent in the inertial subrange.  相似文献   

18.
Aerosol dispersion in the area surrounding an existing biological treatment facility is investigated using large-eddy simulation, with the objective to investigate the applicability of computational fluid dynamics to complex real-life problems. The aerosol sources consist of two large aeration ponds that slowly diffuse aerosols into the atmosphere. These sources are modelled as dilute concentrations of a non-buoyant non-reacting pollutant diffusing from two horizontal surfaces. The time frame of the aerosol release is restricted to the order of minutes, justifying a statistically steady inlet boundary condition. The numerical results are compared to wind-tunnel experiments for validation. The wind-tunnel flow characteristics resemble neutral atmospheric conditions with a Reynolds number, based on the boundary-layer thickness, of Re δ ≈ 2 × 105. The numerical inflow conditions are based upon the wind-tunnel flow field. The predicted decay of both the mean and root-mean-square concentrations are in good agreement with experimental data; at 3 m from the ground, the plume mean concentration 200 m downwind of the source is approximately 2% of the source strength. The numerical data in the near-surface layer (0–50 m from the ground) correspond particularly well with the wind-tunnel data. Tentative deposition simulations suggest that there seems to be little difference in the deposition rates of large (1.8 × 10−5 m) and small (3 × 10−6 m) particles in the near-field under the flow conditions considered.  相似文献   

19.
In situ AGAGE GC-MS measurements of methyl bromide (CH3Br) and methyl chloride (CH3Cl) at Mace Head, Ireland and Cape Grim, Tasmania (1998–2001) reveal a complex pattern of sources. At Mace Head both gases have well-defined seasonal cycles with similar average annual decreases of 3.0% yr−1 (CH3Br) and 2.6% yr−1 (CH3Cl), and mean northern hemisphere baseline mole fractions of 10.37 ± 0.05 ppt and 535.7 ± 2.2 ppt, respectively. We have used a Lagrangian dispersion model and local meteorological data to segregate the Mace Head observations into different source regions, and interpret the results in terms of the known sources and sinks of these two key halocarbons. At Cape Grim CH3Br and CH3Cl also show annual decreases in their baseline mixing ratios of 2.5% yr−1 and 1.5% yr−1, respectively. Mean baseline mole fractions were 7.94 ± 0.03 ppt (CH3Br) and 541.3 ± 1.1 ppt (CH3Cl). Although CH3Cl has astrong seasonal cycle there is no well-defined seasonal cycle in the Cape Grim CH3Br record. The fact that both gases are steadily decreasing in the atmosphere at both locations implies that a change has occurred which is affecting a common, major source of both gases (possibly biomass burning) and/or their major sink process (destruction by hydroxyl radical).  相似文献   

20.
Dispersion estimates with a Gaussian plume model are often incorrect because of particle settling (β), deposition (γ) or the vertical gradient in diffusivity (K v (z) = K 0 + μz). These “non-Gaussian” effects, and the interaction between them, can be evaluated with a new Hankel/Fourier method. Due to the deepening of the plume downwind and reduced vertical concentration gradients, these effects become more important at greater distance from the source. They dominate when distance from the source exceeds L β = K 0 U/β 2, L γ  = K 0 U/γ 2 and L μ = K 0 U/μ 2 respectively. In this case, the ratio β/μ plays a central role and when β/μ = 1/2 the effects of settling and K gradient exactly cancel. A general computational method and several specific closed form solutions are given, including a new dispersion relation for the case when all three non-Gaussian effects are strong. A more general result is that surface concentration scales as C(x) ~ γ −2 whenever deposition is strong. Categorization of dispersion problems using β/μ, L γ and L μ is proposed.  相似文献   

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