共查询到20条相似文献，搜索用时 750 毫秒
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一、前言工业及交通运输中排放出一定量的HNO_3(硝酸气体)和NH_3(氨气)。同时,土壤中也散发出大量的NH_3。与SO_2一样,过量的HNO_3和NH_3气体也会对人类及其他 相似文献
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实际大气中受扰动的饱和气块发生凝结后 ,凝结水会部分脱离气块。以前研究饱和湿大气的Brunt V is l 频率 (N2 m)没有考虑凝结水的部分脱离 ,相当位温 (θe)也忽略了饱和气块的混合比的作用。文中针对这些不足 ,在假设饱和空气中只存在气液转换条件下 ,推导出液态水部分脱离气块的、更符合实际情况的N2 m 表达式和修正的饱和湿大气θe 表达式。新的N2 m 表达式增加了部分脱离气块的液态水的作用项 ,新的θe 表达式中包含有饱和气块的混合比 ,并对有关的表达式分别作了讨论和比较 相似文献
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通过对2016年4—10月份德州台站3种雨量传感器观测的降水量进行偏差、相对偏差及标准差,分析分钟、小时降水量及降水起始时间。结果表明:4—10月份DSC2观测总降水量最多,其次是备SL3-1,新SL3-1最少;在小—中雨时,新SL3—1观测的降水量最准确,在大—暴雨时,称重DSC2观测的降水量最准确;除在1.0mm以下的间歇性降水外,DSC2降水起始和输出时间比新SL3—1平均晚3min左右;新SL3—1和备SL3—1虽然型号相同,但仪器稳定性也存在差异,新SL3—1的稳定性要好于备SL3—1。 相似文献
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防止雨量自记纸受潮膨胀的方法在雨后或有雾的早晨 ,雨量自记迹线常有数小时的缓缓上升现象 ,除确有雾量外 ,大多是因空气湿度大 ,自计纸受潮膨胀而造成的非正常现象。为避免出现这种情况 ,可事先在雨量自计纸背面涂少许蜡 (注意不能影响到正面笔尖的正常划线 )即可避免。日照药液使用两次的方法一些观测员常把涂刷日照纸后剩余的有效药液倒掉 ,这实在有些可惜。将剩下的药液倒入棕色瓶中 (可用盛日照药的棕色空瓶 ,洗净晾干 ,外边再糊一层黑纸 ) ,存放在不常开的柜子里或无光照、气温较低的地方 ,10天以后 ,把保存的药液摇晃均匀 ,再涂刷日… 相似文献
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根据2003年北京夏季近地面大气光化学污染物观测资料,对中国气象局培训中心(代表站)O3超标日浓度、O3前体物浓度、不同天气条件下O3浓度分布特征等进行分析。结果表明:中国北京夏季NO2,NO,CO的浓度特征与日本神奈川县相似,白天(16:00以前)如果NO2/NO超过29,则容易出现O3超标;VOC浓度的高低影响O3浓度;当处于暖湿气流控制,地面为小风或静风、气温较高、湿度较大的多云天气时,易出现O3超标情况。这些污染物发生的特点和规律对北京大气光化学污染的研究和防治具有借鉴意义。 相似文献
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THE IMPACT OF RELATIVE HUMIDITY ON THE RADIATIVE PROPERTY AND RADIATIVE FORCING OF SULFATE AEROSOL* 
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下载免费PDF全文 With the data of complex refractive index of sulfate aerosol,the radiative properties of the aerosol under 8 relative humidity conditions are calculated in this paper.By using the concentration distribution from two CTM models and LASG GOALS/AGCM,the radiative forcing due to hygroscopic sulfate aerosol is simulated.The results show that:(1)With the increase of relative humidity,the mass extinction coefficiency factor decreases in the shortwave spectrum;single scattering albedo keeps unchanged except for a little increase in longwave spectrum,and asymmetry factor increases in whole spectrum.(2)Larger differences occur in radiative forcingsimulated by using two CTM data,and the global mean forcing is -0.268 and -0.816 W/m2,respectively.(3)When the impact of relative humidity on radiative property is taken into account,the distribution pattern of radiative forcing due to the wet particles is very similar to that of dry sulfate,but the forcing value decreases by 60%. 相似文献
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Lei WANG Qing BAO Wei-Chyung WANG Yimin LIU Guo-Xiong WU Linjiong ZHOU JiANDong LI Hua GONG Guokui NIAN Jinxiao LI Xiaocong WANG Bian HE 《大气科学进展》2019,(7):697-710
Cloud dominates influence factors of atmospheric radiation, while aerosol–cloud interactions are of vital importance in its spatiotemporal distribution. In this study, a two-moment(mass and number) cloud microphysics scheme, which significantly improved the treatment of the coupled processes of aerosols and clouds, was incorporated into version 1.1 of the IAP/LASG global Finite-volume Atmospheric Model(FAMIL1.1). For illustrative purposes, the characteristics of the energy balance and cloud radiative forcing(CRF) in an AMIP-type simulation with prescribed aerosols were compared with those in observational/reanalysis data. Even within the constraints of the prescribed aerosol mass, the model simulated global mean energy balance at the top of the atmosphere(TOA) and at the Earth's surface, as well as their seasonal variation, are in good agreement with the observational data. The maximum deviation terms lie in the surface downwelling longwave radiation and surface latent heat flux, which are 3.5 W m-2(1%) and 3 W m-2(3.5%), individually. The spatial correlations of the annual TOA net radiation flux and the net CRF between simulation and observation were around 0.97 and 0.90, respectively. A major weakness is that FAMIL1.1 predicts more liquid water content and less ice water content over most oceans. Detailed comparisons are presented for a number of regions, with a focus on the Asian monsoon region(AMR). The results indicate that FAMIL1.1 well reproduces the summer–winter contrast for both the geographical distribution of the longwave CRF and shortwave CRF over the AMR. Finally, the model bias and possible solutions, as well as further works to develop FAMIL1.1 are discussed. 相似文献
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Modeling Study of the Impact of Heterogeneous Reactions on Dust Surfaces on Aerosol Optical Depth and Direct Radiative Forcing over East Asia in Springtime 下载免费PDF全文
下载免费PDF全文 The spatial distributions and interannual variations of aerosol concentrations,aerosol optical depth(AOD) ,aerosol direct radiative forcings,and their responses to heterogeneous reactions on dust surfaces over East Asia in March 2006-10 were investigated by utilizing a regional coupled climate-chemistry/aerosol model. Anthropogenic aerosol concentrations(inorganic+carbonaceous) were higher in March 2006 and 2008,whereas soil dust reached its highest levels in March 2006 and 2010,resulting in stronger aerosol radiative forcings in these periods.The domain and five-year(2006-10) monthly mean concentrations of anthropogenic and dust aerosols,AOD,and radiative forcings at the surface(SURF) and at the top of the atmosphere(TOA) in March were 2.4μg m-3,13.1μg m-3,0.18,-19.0 W m-2,and-7.4 W m-2,respectively.Heterogeneous reactions led to an increase of total inorganic aerosol concentration;however,the ambient inorganic aerosol concentration decreased,resulting in a smaller AOD and weaker aerosol radiative forcings.In March 2006 and 2010,the changes in ambient inorganic aerosols,AOD,and aerosol radiative forcings were more evident.In terms of the domain and five-year averages,the total inorganic aerosol concentrations increased by 13.7%(0.17μg m-3) due to heterogeneous reactions,but the ambient inorganic aerosol concentrations were reduced by 10.5%(0.13μg m-3) .As a result,the changes in AOD,SURF and TOA radiative forcings were estimated to be-3.9%(-0.007) ,-1.7%(0.34 W m-2) ,and-4.3%(0.34 W m-2) ,respectively,in March over East Asia. 相似文献
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基于国际大气化学-气候模式比较计划模式数据评估中国沙尘气溶胶直接辐射强迫 总被引：2，自引：0，他引：2
目前气候模式对沙尘气溶胶直接辐射强迫模拟仍有很大不确定性,多模式对比有助于定量评估不确定范围。国际大气化学—气候模式比较计划（Atmospheric Chemistry and Climate Model Intercomparison Project,ACCMIP）旨在评估当前模式对短寿命大气成分辐射强迫和气候效应的模拟能力。基于7个ACCMIP模式模拟的中国地区沙尘气溶胶浓度,我们评估了中国区域沙尘气溶胶直接辐射强迫和不确定性范围。结果显示,中国区域沙尘气溶胶年排放总量为215±163 Tg a-1,区域年均地表浓度为41±27 μg m-3,柱浓度为9±4 kg m-2,光学厚度为0.09±0.05。中国区域年均沙尘气溶胶产生的大气顶短波、长波和总辐射强迫分别为-1.3±0.8 W m-2、0.7±0.4 W m-2和-0.5±0.7 W m-2;地表短波、长波和总的辐射强迫值为-1.5±1.0 W m-2、1.8±0.9 W m-2和0.2±0.2 W m-2。沙尘气溶胶长波辐射强迫对沙尘浓度的垂直分布敏感。高层沙尘气溶胶浓度越大,其在大气顶产生更强的正值长波辐射强迫。然而,沙尘气溶胶短波辐射强迫主要受整层沙尘柱浓度控制,对沙尘浓度的垂直分布较不敏感。本文结果可为中国沙尘气溶胶的气候模拟提供参考。 相似文献
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基于云和地球辐射能量系统观测数据集（CERES),对比分析了耦合模式比较计划第五（CMIP5）和第六阶段（CMIP6）模拟的历史大气层顶和地表辐射收支的年际变化和空间分布,明确了多模式间不确定性大的关键区域。结果表明：在年际尺度上,除地表向上长波辐射外,CMIP6的辐射分量的集合均值较CMIP5更接近于CERES观测值,全球地表向下短波辐射的高估和大气逆辐射的低估在CMIP6中分别降低了1.9 W/m2和3.3 W/m2。除大气逆辐射外,CMIP6的辐射分量在多模式间的一致性较CMIP5提高。在北极,CMIP6对大气层顶反射短波、大气层顶出射长波和地表向下短波辐射的模拟偏差较CMIP5大。在南北纬60°,CMIP6对大气逆辐射的模拟偏差较CMIP5大。其他区域CMIP6的辐射分量更接近CERES观测值。CMIP6模拟的地表向下短波辐射和大气逆辐射的不确定性较大区域面积较CMIP5减小,但不确定性极大区域面积无变化。地表净辐射的不确定性空间分布在两代CMIP间变化甚小。青藏高原、赤道太平洋、热带雨林、阿拉伯半岛和南极洲沿海依然是地球系统模式模拟辐射收支不确定性极大的关键区域。 相似文献
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A coupled meteorology and aerosol/chemistry model WRF-Chem(Weather Research and Forecast model coupled with Chemistry) was used to conduct a pair of simulations with present-day(PD) and preindustrial(PI) emissions over East Asia to examine the aerosol indirect effect on clouds.As a result of an increase in aerosols in January,the cloud droplet number increased by 650 cm-3 over the ocean and East China,400 cm-3 over Central and Southwest China,and less than 200 cm-3 over North China.The cloud liquid water path(LWP) increased by 40-60 g m-2 over the ocean and Southeast China and 30 g m-2 over Central China;the LWP increased less than 5 g m-2 or decreased by 5 g m-2 over North China.The effective radius(Re) decreased by more than 4 μm over Southwest,Central,and Southeast China and 2μm over North China.In July,variations in cloud properties were more uniform;the cloud droplet number increased by approximately 250-400 cm-3,the LWP increased by approximately 30-50 g m-2,and Re decreased by approximately 3 ?m over most regions of China.In response to cloud property changes from PI to PD,shortwave(SW) cloud radiative forcing strengthened by 30 W m-2 over the ocean and 10 W m-2 over Southeast China,and it weakened slightly by approximately 2-10 W m-2 over Central and Southwest China in January.In July,SW cloud radiative forcing strengthened by 15 W m-2 over Southeast and North China and weakened by 10 W m-2 over Central China.The different responses of SW cloud radiative forcing in different regions was related to cloud feedbacks and natural variability. 相似文献
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Anthropogenic aerosols play an important role in the atmospheric energy balance. Anthropogenic aerosol optical depth (AOD) and its accompanying shortwave radiative forcing (RF) are usually simulated by nu- merical models. Recently, with the development of space-borne instruments and sophisticated retrieval algorithms, it has become possible to estimate aerosol radiative forcing based on satellite observations. In this study, we have estimated shortwave direct radiative forcing due to anthropogenic aerosols over oceans in all-sky conditions by combining clouds and the Single Scanner Footprint data of the Clouds and Earth’s Radiant Energy System (CERES/SSF) experiment, which provide measurements of upward shortwave fluxes at the top of atmosphere, with Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol and cloud products. We found that globally averaged aerosol radiative forcing over oceans in the clear-sky conditions and all-sky conditions were -1.03±0.48 W m-2 and -0.34 ±0.16 W m-2, respectively. Direct radiative forcing by anthropogenic aerosols shows large regional and seasonal variations. In some regions and in particular seasons, the magnitude of direct forcing by anthropogenic aerosols can be comparable to the forcing of greenhouse gases. However, it shows that aerosols caused the cooling effect, rather than warming effect from global scale, which is different from greenhouse gases. 相似文献
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Assuming spheroidal and spherical particle shapes for mineral dust aerosols, the effect of particle shape on dust aerosol optical depth retrievals, and subsequently on instantaneous shortwave direct radiative forcing (SWDRF) at the top of the atmosphere (TOA), is assessed based on Moderate Resolution Imaging Spectroradiometer (MODIS) data for a case study. Specifically, a simplified aerosol retrieval algorithm based on the principle of the Deep Blue aerosol retrieval method is employed to retrieve dust aerosol optical depths, and the Fu-Liou radiative transfer model is used to derive the instantaneous SWDRF of dust at the TOA for cloud-free conditions. Without considering the effect of particle shape on dust aerosol optical depth retrievals, the effect of particle shape on the scattering properties of dust aerosols (e.g., extinction efficiency, single scattering albedo and asymmetry factor) is negligible, which can lead to a relative difference of at most 5% for the SWDRF at the TOA. However, the effect of particle shape on the SWDRF cannot be neglected provided that the effect of particle shape on dust aerosol optical depth retrievals is also taken into account for SWDRF calculations. The corresponding results in an instantaneous case study show that the relative differences of the SWDRF at the TOA between spheroids and spheres depend critically on the scattering angles at which dust aerosol optical depths are retrieved, and can be up to 40% for low dust-loading conditions. 相似文献
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使用RegCM4.6区域气候模式，选取Emanuel和Mix（Grell+Emanuel）两种积云对流参数化方案，以2016年为例，分别对中国地区云短波辐射强迫及其涉及的物理量进行数值模拟，揭示其时空分布特征，并探究两种积云对流参数方案模拟效果的差异及其原因。结果表明：从季节平均来看，全国地表云短波辐射强迫均为负值，云对地表为冷却效应，冬季最小，春夏季较大。塔里木盆地四季均为辐射强迫低值区，夏季冷却效应最弱，辐射强迫绝对值低于40 W·m-2；全天空地表净短波辐射分布也呈显著季节差异，除夏季外均呈由南向北逐渐递减的分布趋势；晴空地表净短波辐射在横断山脉处和塔里木盆地处均比较低，其中春季最为明显；两个方案所得的季节空间分布特征大致相同，但在数值上存在差异。春季时全国大部分地区全天空地表净短波辐射通量差异最大，在55 W·m-2左右，晴空地表净短波辐射通量在青藏高原处差异在60W·m-2左右。 相似文献