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1.
The sediments from Lake Bosumtwi, Ghana contain a unique record of fine-scale (mm to sub-mm) laminations, which will provide a valuable annual chronometer for reconstructing paleoenvironmental changes in West Africa covering much of the last 1 Ma. Comparisons of laminae counts to independent 210Pb dates and the rise in anthropogenic “bomb” radiocarbon support the interpretation of the laminations in the uppermost sediments as registering annual events. Radiocarbon dates on in-situ fish-bone collagen are in agreement with varve counts, further supporting the annual nature of our varve chronology. Over the instrumental period (1925–1999), dark-varve thickness measurements are correlated with local rainfall (r = 0.54) and appear able to resolve decadal-scale changes in precipitation. The relationship between varve thickness and rainfall provides support for our interpretation that dark-colored varve thickness records catchment runoff during the rainy season rather than dust flux during the dry season. Dark laminae alternate with organic and carbonate-rich light laminae formed during the fall period of enhanced productivity. Downcore, varves undergo significant microstratigraphic and geochemical variations, but retain the same pattern of alternating clastic and organic-rich laminae, providing support that the laminae may represent annual time markers for reconstructions of the deeper part of the record.  相似文献   

2.
Two varve counts made nearly 20 yrs apart and by different authors in the small and well sheltered meromictic lake of Valkiajärvi were compared with a view to establishing how similar, or otherwise, these two independent varve chronologies might be. The results were significant, the difference between the two varve counts being less than 2% for most of the sediment length, even though the average varve thickness was only 0.3 mm. The continuous and essentially uniform varve record - so far the longest in Finland - covers 8400 yrs and could be applied for accurate dating of palaeoenvironmental indicators in the sediment. As an example, we present a varve-dated pollen diagram for Lake Valkiajärvi.In addition, some magnetic parameters (susceptibility, ARM, SIRM) were measured on the sediment sequence to support the stratigraphic division and correlation of the cores, and to outline the development of the basin since the last deglaciation. Magnetic variables reflected mainly the variation in minerogenic material in the sediment, and were therefore related to changes in the catchment. The magnetic parameters also showed a drastic change some 6000 yrs ago, the reason for which, unfortunately, is still not fully understood.  相似文献   

3.
This study assesses Little Ice Age (LIA) lake sediment morphological and geochemical records and moraine chronologies in the upper Fraser River watershed, British Columbia, Canada, to resolve differences in paleoenvironmental interpretation and to clarify sediment production and sediment delivery processes within alpine geomorphic systems. Moose Lake (13.9 km2), situated at 1032 m a.s.l., contains a partially varved record indicating variable rates of accumulation during the last millennium that, in general, coincide with previously documented LIA glacial advances in the region and locally. Dendrochronological assessment of forefield surfaces in the headwaters of the catchment (Reef Icefield) shows that periods of moraine construction occurred just prior to ad 1770, ad 1839 and ad 1883, and some time before ad 1570. Taken collectively, increases in varve thickness within eight Moose Lake sediment cores coincide with documented glacier advances over the twelfth through fourteenth centuries, the eighteenth century, and nineteenth through twentieth centuries. Glacial activity during the sixteenth century is also indicated. While varve thickness variations in proximal and distal sediments clearly reflect glacial activity upstream of Moose Lake, the intermediate varve record is relatively insensitive to these decadal and longer‐term catchment processes. Variations in Ca and related elements derived from glaciated carbonate terrain within the Moose River sub‐catchment (including Reef Icefield) indicate gradually increasing delivery from these sources from the twelfth through twentieth centuries even where the varve thickness record is unresponsive. Elevated carbonate concentrations confirm glacial activity c. ad 1200, ad 1500, ad 1750, and ad 1900.  相似文献   

4.
Lithostratigraphic analyses of a sub-annually laminated core from Ranu Lamongan, a maar lake on the island of Java, document considerable changes in the lake’s chemistry and water balance over the past ca. 800 calendar years. Composition of the dark (clastics) and light (diatoms and/or calcium carbonate minerals) couplets suggests that these laminations form in response to seasonal changes in rainfall and water-column overturn in the lake. Calcium carbonate is not continuous in the core, and when it occurs it varies, sometimes abruptly, in carbonate phase and elemental composition (low Mg-calcite Mg-calcite, and aragonite). A significant correlation between Mg/Ca changes and δ18O variations in authigenic calcium carbonate suggest the basin is highly sensitive to hydrologic variation. Lithologic data suggest calcium carbonate precipitates and thus records hydrologic conditions during the dry season – a season in which rainfall anomalies are highly correlated with the phase of ENSO. Our carbonate-based record of Mg/Ca shows variability in evaporative concentration on a quasi-seasonal frequency for the past ca. 800 years. Our record shows two multi-decadal periods of drought – ca. 1275–1325 and ca. 1450–1650 CE – the latter of which was especially strong and/or prolonged. Our record also shows a possible change in drought frequency at around 1650 CE, in which periods of calcium carbonate precipitation and Mg/Ca change shifted from multi-decadal to interannual variability. Given the strong correlations between modern-day drought in East Java and ENSO variability, our drought record may indicate a regime shift in the behavior of the ENSO system about 350 years ago. Finally, comparisons between our record and others suggest that variation in ENSO on centennial and sub-centennial scales is not strongly associated with changes in the global mean climate state.  相似文献   

5.
Past atmospheric Pb deposition in Lake Qinghai,northeastern Tibetan Plateau   总被引：2，自引：0，他引：2  
Two short sediment cores were recovered from sub-basins of Lake Qinghai, China and were analyzed for concentrations of Pb and 16 other elements to determine historic, regional atmospheric Pb deposition on the Tibetan Plateau. Core chronologies, dating back to the eighteenth century, were established using activities of 210Pb and 137Cs. The 17 elements were divided into three principal components. Variations in concentrations of PC1 elements (Al, Cr, Cu, Fe, K, Mn, Ni, and Ti) demonstrate different patterns between the two cores, and are attributed to different sediment sources in the two sub-basins. PC2 elements (Ba, Ca, Na, and Sr) may be associated with the degree of catchment weathering and/or water chemistry. Four elements (Pb, Zn, P, and Co) are related to both PC1 and PC2, and reflect a mixture of natural and anthropogenic sources. The PC3 element is Mg in the north sub-basin, and is perhaps related to aragonite precipitation and/or increased farming. Elevated Pb concentrations in uppermost sediments of both cores signify a recent regional/global increase in anthropogenic Pb release into the environment. After subtracting lithogenic Pb, derived from rock weathering and/or dust and normalized to the background immobile element Ti, results suggest that excess, anthropogenic Pb is transferred to the lake and its sediments predominantly via the atmosphere. This anthropogenic atmospheric Pb is comparable in magnitude and displays similar variation patterns in the two cores, reflecting regional atmospheric deposition and local erosion. The average anthropogenic Pb deposition rate in Lake Qinghai since the 1960s has been ~12.2 ± 3.5 mg/m2/a, comparable with atmospheric Pb fluxes reported for sites elsewhere in the northern hemisphere.  相似文献   

6.
A 336-year floating varve chronology from Lake Holzmaar (Eifel, Western-Germany) covering the recent period has been established by microfacies analysis of thin sections. This sequence terminates 23 cm below the core top. In the top 23 cm, the varves are disturbed. By means of linear regression, the varve sequence was dated to the period AD 1607–1942. The influences of climatic variability and anthropogenic activities in the lakes catchment (e.g., forestry, agriculture) on lithology, fabric, and microfossil content of the varve sublaminae could be discriminated by applying statistical analyses (ordination and clustering) to the combination of the sublaminae in the varves and their thickness. Four clusters are obtained. Cluster 1 indicates cold springs, and shorter, cooler summers reflected primarily in below-average varve thickness (VT) for two stable phases: from AD 1650–1700 (during the Maunder Minimum) and from AD 1750–1785. Cluster 2 indicates years with conditions transitional to that indicated by cluster 1, characterized by vigorous and prolonged spring circulation with massive blooms of the nordic-alpine Aulacoseira subarctica. The samples assigned to Cluster 3 and Cluster 4 show the imprint of anthropogenic influences. Cluster 3 (AD 1795–1815 and AD 1825–1885) is characterized by above-average VT due to high detritus input throughout the year. The increased soil erosion can be linked to anthropogenic deforestation as a consequence of the production increase of the Eifelian iron industry at the end of the 18th century. This input dampens the climatic signal of a colder Dalton Minimum, which is reflected in a short drop in VT centered around AD 1810. At about AD 1885, Cluster 4 conditions, characterized by increased nutrient concentrations, low detritus input, and longer periods of stable summer stratification, become the stable state in Lake Holzmaar. They indicate the response of the lake to natural reforestation and the use of artificial fertilizers in the catchment, which began, according to historical records, in the 1850s in the Eifel region. The prolonged, stable summer stratification periods may be the first indication of the modern warming trend. A drop in VT centered around AD 1890 and recurring cluster-1 conditions may indicate the Damon Minimum.  相似文献   

7.
Image analysis as a method to quantify sediment components   总被引：1，自引：0，他引：1  
Varved lake sediments, with their annual to seasonal resolution, have a high potential for inferring past environmental and climatic conditions. To fully utilize the information present in varved records, high-resolution analyses, which often are time-consuming and difficult to perform, are desirable. The investigation reported here aims at (i) developing image analysis as a method for estimating annual accumulation rates of sediment components such as minerogenic matter, organic matter and biogenic silica, and (ii) assessing the relative importance of these components for changes in varve thickness. Image analysis was used to digitize the grey-scale variations and to measure the varve thickness of 540 varves (476-1015 AD) from Lake Kassjön in northern Sweden. From the 35 cm long digitized sediment sequence, 108 consecutive five-year samples were cut out quantitatively, and relationships between grey-scale variations and sediment dry mass and individual sediment components were assessed. There is a strong correlation between corrected grey-scale (i.e. the product of grey-scale and varve thickness) and the dry mass accumulation rate (r = 0.90, p < 0.001). With a stepwise multiple regression a significant model (R2 = 0.81) between corrected grey-scale and the accumulation rates of minerogenic matter (r = 0.90, p < 0.001) and biogenic silica (r 0.26, p < 0.012) was obtained. Considering the minor contribution and weak significance of biogenic silica, image analysis can be used as a fast and non-destructive method to infer past annual accumulation rates of dry mass and minerogenic matter in Kassibn. The model of the relationship between changes in varve thickness, and water content and accumulation rates of sediment components has little predictive power (R2 = 0.45). The result shows that the varve thickness in Kassjön, at least during the period 476-1015 AD, is not determined by a single sediment component but partly depends on interactions between the major sediment components.  相似文献   

8.
The least annual precipitation in the western interior of North America occurs in the northern Great Plains, including an area that encompasses parts of south-eastern Alberta, south-western Saskatchewan and eastern Montana. During 1999–2001, most climate stations in this region had record low precipitation. This paper examines this three-year drought in the context of historical climate records from Medicine Hat, Alberta and Havre, Montana and summer (June–July) and annual (August–July) precipitation reconstructed from standardized tree-ring widths (residual chronologies) from Pinus contorta (lodgepole pine) sampled in the Cypress Hills of Alberta and Saskatchewan and the Bears Paw Mountains of north-central Montana. Drought is operationally defined as precipitation in the lower 10th and 20th percentiles. Plots of reconstructed precipitation and cumulative departure from median values indicate a shift in climate variability prior to the twentieth century, when EuroCanadians settled in this region. The eighteenth and nineteenth centuries are characterized by sustained periods of progressively wetter and drier conditions, including prolonged drought. Various archival sources document the significant impacts of these prolonged droughts. While drought was frequent in the twentieth century, it tended to be of short duration and the impacts also were ameliorated by intervening periods of relatively high precipitation. Increasing aridity in response to global warming could expose a larger area of the northern Great Plains to the impacts of drought.  相似文献   

9.
In this paper, the relationships between paleo-precipitation and the regional influence of El Nino Southern Oscillation (ENSO) in South America are assessed from a high-resolution calendar varve-thickness record. Two short laminated sediment cores (53 and 61 cm length) from Lago Puyehue (40° S) are analysed by continuous varve measurements through the last 600 years. The calendar varve years are determined by the occurrence of graded planktonic-rich layers. The annual sediment accumulation rates are reconstructed by using the standard varve-counting methods on thin sections. The 1980–2000 varve-thickness record is interpreted in terms of climate through correlation with limnological and local monthly instrumental climate databases. The comparison between the standardized varve thickness with the instrumental records reveals a strong correlation (r = 0.75, р = 0.07) between the total varve thickness and the austral autumn/winter precipitation. We argue that strong austral winter winds and precipitation are the forcing factors for the seasonal turn-over and phytoplankton increase in the lake sediments. During strong El Nino events the precipitation and the winds decrease abnormally, hence reducing the thickness of the biogenic sediments deposited after the winter turn-over. Our results show one significant regional maximum peak of winter precipitation (>900 mm) in the mid 20th century and a significant period with lower winter precipitation (<400 mm) before the 15th century, i.e., the late Medieval Warm Period. The first peak in the mid 20th century is confirmed by the regional precipitation database. The influence of ENSO cycles over the last 600 years is assessed by spectral analysis in Fagel et al. (2007). The possible influence of the regional volcanism and/or the seismic activity on the local climate record is also discussed. This is the sixth in a series of eight papers published in this special issue dedicated to the 17,900 year multi-proxy lacustrine record of Lago Puyehue, Chilean Lake District. The papers in this special issue were collected by M. De Batist, N. Fagel, M. -F. Loutre and E. Chapron.  相似文献   

10.
阿尼玛卿山地祁连圆柏径向生长对气候的响应   总被引：2，自引：0，他引：2  
通过对阿尼玛卿山地5 个坡面20 个祁连圆柏树轮宽度标准年表的分析, 发现公共区间内各树木年轮宽度标准年表中的信噪比SNR 和样本总解释量EPS 值都较高, 说明年表中都含有较强的环境信息; 树轮宽度年表之间的平均相关为0.35 (大多达到95%的置信程度), 具有较好的区域一致性。聚类分析使树木年轮宽度年表分成东、西两大部分, 而年表的第一主分量显示出: 西部树轮的指数序列明显长于东部即树木生长有自西向东扩展的趋势, 并且东、西区域树木生长变化的特征年变化具有同步性。东、西树轮宽度年表中第一主分量和第二主分量与气候因子的相关和响应都表现出一定的相似性, 但第二主分量对气候因子响应的差异性更显著。西部树木生长PCI 的主要限制因子是温度, 尤其当年春末夏初及前一年秋季温度影响最大, 同样降水也起着重要的作用, 西部树木生长PC2 的主要限制因子是降水量; 而东部树木生长PC1 主要受降水的制约, 第二主分量PC2 的响应分析显示出气候的滞后影响(树木前期生长) 是非常重要的限制因子。  相似文献   

11.
Sediments from a 3 ha lake (75 °34.34N, 89 °18.55W) from the coastal region of northern Devon Island, Nunavut, Canada, contain discrete laminations in the deepest part of the basin. The laminations are varves as indicated by the correspondence between counts and thickness measurements of the couplets and 210Pb dating. A 14 cm core representing 150 years of sedimentation contained laminated couplets consisting of a lighter inorganic layer with a higher percentage of calcium and magnesium, alternating with fine darker bands, typically more cohesive, and comprising higher proportions of silica and carbon. A reddish oxidation zone with higher iron and aluminum frequently separates the laminations. The dark layer represents a biogenic component deposited in summer and is made cohesive by bacterial filaments among the other particles. The light inorganic layer represents clastic deposition from allochthonous sources. Deposition rates were relatively consistent through the core with an increase in varve thickness in the 1950s. Diatom concentrations in the sediments increased by two orders of magnitude in this century, with major increases in the 1920s and 1950s. The increase in varve thickness and diatom abundance coincides with an increase in summer melt percentage in an ice core from the Devon Island Ice Cap (Koerner, 1977). The relatively high sedimentation rate (0.15 cm yr-1) coupled with the consistency of deposition makes this lake a significant indicator for recent climate changes of the Canadian Arctic Archipelago.  相似文献   

12.
树木年轮记录的天山北坡中部过去338 a降水变化   总被引：5，自引：1，他引：4  
 利用位于天山北坡中部9个气象站的降水资料与采自该地区的21个树木年轮年表序列进行分析。结果表明,9个气象站上年8月到当年7月的平均降水量与树木年轮标准化年表具有很好的相关性,最高单相关达到0.612（P<0.0001）。分析发现,生长季前期及春材形成期的降水变化对天山山区树木年轮径向生长量起着决定性作用。用四工河东白杨沟、呼图壁河赛热克巴依萨依、呼图壁河希热克久热特、四工河西白杨沟、奎屯河兰能果尔南5个标准化年表较好地重建了天山北坡中部近338 a来上年8月到当年7月的降水量,重建方程的方差解释量达到60.0%,经过统计检验和历史资料验证,表明重建序列是可靠的。对过去338 a天山北坡中部降水变化的特征分析表明,近338 a间,天山北坡中部降水大体经历了8个偏干和8个偏湿阶段,偏湿年份与偏干年份基本持平。最长的偏干阶段是1705—1750年,最干旱的阶段为1960—1989年,最干旱年份是1796年、1944年和1974年,降水偏少程度均大于27%;最长的偏湿阶段是1917—1959年,1690—1904年间为降水最为丰沛的时期。天山北坡中部338 a降水具有两年左右的变化准周期,在1751年发生了明显的由少到多的突变,在1958年前后发生了明显的由多到少的突变。  相似文献   

13.
A composite record of varve sedimentation is presented from high arctic meromictic Lake C2. The combination of a short runoff and sediment transport season with the strong density stratification of the lake lead to the formation of annual sediment couplets. This conclusion was confirmed by 210Pb determinations. High intra-lake correlation of the varves allowed the construction of a composite record of varve sedimentation from overlapping segments of multiple sediment cores. Cross-dating between core segments isolated counting errors in individual cores, that could be attributed to minor sediment disturbances and vague structures. Resolving counting errors by cross-dating reduced the chronological error of the composite series to an estimated ±57 years.The Lake C2 series is the first non-ice cap, high resolution late-Holocene environmental record from the Canadian high arctic. The composite varve series compares favorably with other high resolution proxies from the arctic, in particular with the ice core records from Devon Island and Camp Century, Greenland. A general correspondence between the varve record and other North American proxies for the little Ice Age period (1400–1900 AD) suggests that the Lake C2 record is sensitive to large-scale synoptic changes.This is the tenth in a series of papers published in this issue on the Taconite Inlet Lakes Project. These papers were collected by Dr R. S. Bradley.  相似文献   

14.
The temporal variability and severity of pre-instrument record summer droughts in the Ohio River Valley (Illinois, Indiana, and Ohio, USA) are not well understood. This study attempts to help fill this gap in Ohio Valley drought knowledge by using tree-ring chronologies from Illinois, Indiana, and Ohio to reconstruct summer (June through August) PDSI. We found that recent meteorological droughts of 1988 and 2012 are not unusual in the context of those reconstructed for the interval of 1680–2012. Droughts prior to 1895 (when the instrument-based record began) were more severe and lasted, on average, 1.5 times longer than those after 1895. The North American Drought Atlas represents droughts well for this region, but we found that drought severity was not homogeneous across the three sites. This indicates drought in the Ohio River Valley should be examined at a sub-regional level and suggests a need for a finer spatial representation of tree-ring chronologies in the Ohio Valley. Given the context of historical drought variability, the reconstructions suggest this region should be prepared for droughts that may be more severe and longer lasting than those recently observed.  相似文献   

15.
范子昂  魏文寿  陈峰  袁玉江 《中国沙漠》2012,32(4):996-1002
 利用采自腾格里沙漠东缘的贺兰山油松树轮样本,建立树轮宽度年表。通过相关普查发现,贺兰山油松树轮宽度差值年表与腾格里沙漠东缘当年5月至7月的降水存在显著的正相关,相关系数为0.606（P<0.001）。利用贺兰山北部的树轮宽度差值年表,可较好地重建腾格里沙漠东缘近231 a来当年5月至7月的降水变化,交叉检验表明,降水重建结果稳定可靠。通过与腾格里沙漠南缘地区树轮降水重建序列对比分析,发现腾格里沙漠边缘区的树轮重建降水的干湿阶段变化具有良好的同步性,并对西北地区极端干旱历史事件有良好响应。  相似文献   

16.
Sources and chronologies of metal contamination were studied in sediment cores of three lakes of the Rouyn-Noranda mining area (Québec, Canada) affected by atmospheric deposition of anthropogenic contaminants. One of the three lakes also received acid mine drainage. The sediments were dated using 210Pb and 137Cs and analysed for stable Pb isotope ratios and for total concentrations of 15 elements (Ag, Al, Au, Ca, Cu, Cd, Fe, Hg, Mn, Ni, P, Pb, S, Ti, Zn). Stable lead isotopic signatures helped to determine the quantitative contributions of different industrial Pb sources to our sampling sites. This source apportionment showed the dominant influence of the Rouyn-Noranda copper smelter in airborne Pb emissions for the decades following 1926, when industrialization began in the region. The smelter source had a low ratio of 206Pb/207Pb ranging between 0.90 and 1.05, as typical of the Abitibi Archean sulphides. The relationships between element (metal) sedimentary fluxes and anthropogenic Pb fluxes allowed us to infer the origin of the anthropogenic source. These relationships strongly suggest that the copper smelter was (and may still be) an atmospheric source of Cd, Cu, Pb, Zn, Ag and Hg to the surrounding lakes. Our study indicates that the efforts made by the Rouyn-Noranda copper smelter to reduce airborne emissions of metals have been translated in reduced atmospheric metal loadings to the surrounding lakes.  相似文献   

17.
天山北坡东部地区树轮宽度年表特征分析   总被引：8，自引：5，他引：3  
通过对天山北坡东部地区8个树轮宽度标准化年表的有关参数的对比,证明苏巴什沟与白杨河沟年表包含有较多的气候信息,8个树轮宽度标准化年表的互相关系数平均值达0.530,其中白杨河沟与苏巴什沟年表的相关系数高达0.725。说明所采样本对该区域的气候具有较好的代表性。再将8个树轮宽度标准化年表与附近的奇台县、木垒县两个气象站1961—2007年逐月降水和平均最低气温,及单月降水和单月气温进行相关分析。结果表明,天山东部地区白杨河沟的树轮宽度生长与上年7月至当年6月的降水呈正相关,其相关系数为0.597,显著性水平达0.000006,与当年6月平均最低气温呈负相关,相关系数为-0.437,显著性水平达0.001,上述均具有明确的树木生理学意义。研究还发现,在0.05显著性水平上,8个年表的树轮宽度指数变化以2~3 a的变化准周期最为多见,苏巴什沟、大东沟及白杨河沟年表以11 a准周期多见。就整个地区而言,天山北坡东部地区8个年表中低频气候信息一般多于高频气候信息。  相似文献   

18.
Annually-laminated clastic sediments preserve a high resolution proxy record of paleoclimate, provided that allochthonous sedimentation represents a response to meteorological forcing of watershed sediment transfer. Here, we demonstrate this linkage, and illustrate a calibration process using the most recent 40 years of a varve record from Lake C2 (82°50 N; 78°00 W), three years of field measurements, and meteorological data for 1951–92 from nearby AES weather station Alert. Field measurements were used to correlate proxies of the energy available for snowmelt (e.g. air temperature) and daily suspended sediment discharge (SSQ). Our calibration was extended through use of weather data from Alert. Both mean daily air temperature at Echo, and daily SSQ, were well correlated with air temperature at 600 m above Alert, as obtained from the 1200 Z (0800 LST) rawinsonde sounding. Accordingly, we used pooled 1990 and 1992 Alert 600 m data to predict the lagged daily sediment discharge into Lake C2 (adj. r 2=0.43). Daily values were summed each year in order to produce an annual series of predicted sediment transfer to the lake. The original varve chronology was based on eight sediment cores recovered from the deep basin of the lake (>80 m). Although low-frequency fluctuations of the varve and predicted SSQ series agree, slight tuning of the varve record optimizes the correlation between them. Adjustments were based on examination of weather data for specific years, reexamination of sediment core thin sections, and by aligning fluctuations in the two series which closely matched. Although the original chronology is reasonably well correlated with 600 m temperatures at Alert (for JJA mean, r=0.41, significant at 0.01), the adjusted chronology is both better correlated and contains a more precise climate signal (r=0.54 for July mean, significant at 0.01). This is the first calibrated varve record produced from Arctic lake sediments, and demonstrates that varves from Lake C2 contain a paleoclimatic record. We believe the post-facto manipulations required to produce the adjusted varve chronology are reasonable given the uncertainties inherent in varve counting, and the lack of any independent corroborating chronostratigraphic markers.This is the ninth in a series of papers published in this issue on the Taconite Inlet Lakes Project. These papers were collected by Dr R. S. Bradley.  相似文献   

19.
Several cores were compared to elucidate the grade of mercury retention in sediments of the Baltic Sea near Oulu, Finland. The known history of the mercury discharge to waste water from a chlor-alkali plant, the primary pollution source, was compared to that in the sedimentary record. One core was dated by lead-210 and varve counts. During the past thirty years, the rate of sedimentation was up to 10 mm per year corresponding to a dry matter accumulation rate of about 3 kg m–2a–1. Under these conditions, most of the mercury reaching the sediment was retained. Correspondingly, the mercury levels in fish were considerably lower, with a delay of some five years.The present mercury content of the upper layers is some 1/4 or 1/5 that of the late 1970's, but it is still some twentyfold compared to levels at the beginning of the century. The extent to which the present mercury level in the sediment represents the various phases of industrial emission remains unsolved due to the origin of mercury in this sea area from several other sources and due to difficulties in exact core correlations from different years.  相似文献   

20.
Post-depositional mobility of137Cs,239+240Pu and210Pb was assessed in six small lake basins by comparing sedimentary nuclide profiles with their known fallout history. Laminae couplets, when present, were determined to be varves because the137Cs and239+240Pu 1963 fallout peaks are present in laminae couplets corresponding to years 1962–1964. There is no evidence of mobility of210Pb, because 1) mass accumulation rates based on210Pb agree with those based on137Cs and239+240Pu peak depths and with those based on varve counts, and 2)210Pb ages agree with varve ages. Significant mobility of137Cs is evident from the penetration of137Cs to depths 15–20 cm deeper than239+240Pu. Deep penetration of137Cs in spite of a sharp gradient below the peak is interpreted by a numerical model to suggest that137Cs is present in two distinct forms in these sediments, 67–82% as an immobile form and 18–33% reversibly adsorbed with a K d of approximately 5000. The profiles can be interpreted equally well assuming a small portionof the total137Cs was present as an extremely mobile phase (K d 5000) in the months to years following peak fallout, slowly becoming more strongly adsorbed. High NH 4 + concentrations in porewaters may enhance diffusion of the mobile form of137Cs, but not of the immobile form of137Cs that defines the sharp gradient. Mobility of137Cs is likely also enhanced by the low clay content and the high porosity of these sediments. Thus the first detection of137Cs in the sediments cannot automatically be assumed to correspond to a date of 1952 (initial testing of thermonuclear weapons), although the depth of the peak can be assumed to correspond to 1963 (the year of maximum fallout from testing of thermonuclear weapons).239+240Pu is a more reliable sediment chronometer than137Cs because it is significantly less mobile.This is the sixth of a series of papers to be published by this journal following the 20 th anniversary of the first application of210Pb dating of lake sediments. Dr P.G. Appleby is guest editing this series.  相似文献   

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