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1.
Measurements of cosmic-ray produced53Mn are reported for a series of lunar surface samples down to a depth of 416 g/cm2. These results clearly illustrate the decrease in activity with depth as the incident galactic cosmic rays are absorbed. Below 60 g/cm2 the production rate decreases exponentially with a mean length, λ, of about 220 g/cm2. These results indicate that, at the Apollo 15 site, the lunar regolith has been unmixed, on a meter scale, for the last 5 my. The neutron activation technique for53Mn, which allowed samples smaller than 200 mg to be used for these measurements, is described.  相似文献   

2.
Cosmic-ray-produced53Mn (t1/2 = 3.7 × 106years) has been determined by neutron activation in nine Allan Hills-77 meteorites. Additionally,36Cl (1/2 = 3.0 × 105years) has been measured in seven of these objects using tandem accelerator mass spectrometry. These results, along with14C (t1/2 = 5740years) and26Al (7.2 × 105 years) concentrations determined elsewhere, yield terrestrial ages ranging from 0.1 × 105 to 7 × 105 years. Weathering was not found to result in53Mn loss.  相似文献   

3.
Cosmogenic radionuclides, including22Na,26Al and54Mn, were measured in a sample of the recently-fallen Malakal hypersthene chondrite. The high26Al activity, 79 ± 2 dpm/kg, greatly exceeds the levels expected from elemental production rates, shielding considerations, or comparisons with other ordinary chondrites, and can only be explained by exposure to a uniquely high cosmic-ray flux. Calculations including noble gas,3H, and53Mn data from other laboratories require a two-stage irradiation. Malakal's most probable history is: exposure in excess of 4 m.y. to an effective cosmic-ray flux approximately three times that experienced by other chondrites, an orbit change (very possibly caused by a collision), and a final period of about 2 m.y. during which it was exposed to a “normal” cosmic-ray flux.  相似文献   

4.
The concentrations of222Rn and226Ra in the water column and in the sediments of Santa Barbara and San Nicolas Basins have been measured semi-annually over the last four years. Approximately one-third of excess radon profiles obtained in the water column in these basins can be adequately fit with a one-dimensional eddy diffusion-decay model. Exponential profiles in the center of San Nicolas Basin yield a vertical eddy diffusivity of 26±16 cm2/s and 3.4±1.0 cm2/s for Santa Barbara Basin. The application of a two-dimensional eddy diffusion-decay model to profiles obtained in the center and on the margins of San Nicolas Basin produces a better fit than is found using a one-dimensional vertical eddy diffusivity. The two-dimensional model for San Nicolas Basin predicts a vertical eddy diffusivity of 17 cm2/s and a horizontal eddy diffusivity of 105 cm2/s. These values are in reasonable agreement with those predicted from the vertical buoyancy gradient and the horizontal length scale.The vertically integrated radon excess (standing crop) in the water column of Santa Barbara Basin averages 53±23 atoms/m2 s. This is in good agreement with the flux across the sediment-water interface of 60±15 atoms/m2 s, calculated by measuring radon emanation in the sediments as a function of depth and applying a molecular diffusion-reaction model. Hence, one-dimensional molecular diffusion accurately predicts the flux of radon from the laminated Santa Barbara Basin sediments. In San Nicolas Basin the integrated radon excess in the water column is 376±143 atoms/m2 s, but the diffusive randon flux from San Nicolas Basin sediments averages only 190±53 atoms/m2 s. This descrepancy indicates that a non-diffusive process, probably macrofaunal irrigation, supplies much of the flux of radon from San Nicolas Basin sediments.  相似文献   

5.
Four cores recovered within the framework of the INTERPOL Project have been analysed for their grain size and geochemistry; sediment accumulation rates (SARs) were also determined from 210Pb and 137Cs profiles. Two cores are representative of the Axios and Aliakmon Rivers depositional environment, whilst the third core represents the Pinios River province; the fourth core represents an environment of outer shelf relict sands. Apparent SARs ranged between 0.667 g cm−2 yr−1 (Axios and Aliakmon Rivers) and 0.414 g cm−2 yr−1 (Pinios River). Trawling activities and biomixing are critical processes that may be responsible for the mixing of the surface sediments, as observed from the excess 210Pb profiles. The thickness of the surface mixed layer was 4.5 cm in the vicinity of Axios and Aliakmon Rivers and in the area of Pinios River, 3.75 cm on the outer shelf and 1 cm in the area where no trawling was observed. Sediment accumulation appeared to be regulated by variations in the riverine discharge, shelf transport pathways and winnowing processes. Major element variations, such as Si, Al, Ti, V and Ni, were dominated by terrigenous supply as aluminosilicate minerals and quartz, whereas most Ca and Sr were biogenic. Si/Al and Ca/Al ratios have been used to express changes in sediment accumulation and winnowing. Redox processes were depicted by Mn, which showed an increase in the depth of its redoxcline, from 1 cm in inshore stations to 2 cm on the outer shelf. Si/Al ratios follow the Ca/Al ratios and can be used to assess percentage winnowing in the sediment. Increases in these ratios indicate a decrease in sediment input rates and are seen in the upper parts of most of the cores. Anthropogenic or ‘excess’ metal contents have been calculated from Zn/V and Pb/V ratios. Their distributions in the cores showed that by far the highest contamination is associated with the Axios River output, whilst sediments influenced by the Pinios River were relatively uncontaminated.  相似文献   

6.
Activities of a suite of radioisotopes ranging in half-life from 5.6 days (52Mn) to 3.7 m.y. (53Mn) have been measured in the Dhajala chondrite. The results show that all the radioactivities are close to the expected levels except54Mn and 22Na. Their activities are higher than those based on the interplanetary fluxes at 1 A.U. near the ecliptic, expected immediately before the fall of Dhajala, corresponding to the time of solar minimum. Furthermore, activity ratios of 54Mn/53Mn and 22Na/26Al are higher by 30–50% than expected. The departure from the expected values is discussed in terms of spatial variations of cosmic rays based on the computed orbital parameters of the meteoroid. If the galactic cosmic ray fluxes in the equatorial region (±15°) are assumed to be the same as in the ecliptic plane then these results suggest higher fluxes by 33 ± 7% at heliographic latitudes 15–40°S, during solar minimum.  相似文献   

7.
Cosmic-ray-produced53Mn (t1/2 = 3.7 × 106years) has been measured in twenty Antarctic meteorites by neutron activation analysis.36Cl (t1/2 = 3.0 × 105years) has been measured in fourteen of these objects by tandem accelerator mass spectrometry. Cosmic ray exposure ages and terrestrial ages of the meteorites are calculated from these results and from rare gases.14C (t1/2 = 5740years) and26Al (t1/2 = 7.2 × 105years) data. The terrestrial ages range from 3 × 104 to 5 × 105 years. Many of the L3 Allan Hills chrondrites seem to be a single fall based on these results. In addition,10Be (t1/2 = 1.6 × 106years) and36Cl have been measured in six Antarctic ice samples. The first measurements of10Be/36Cl ratios in the ice core samples demonstrate a new dating method for ice.  相似文献   

8.
The contents of spallogenic53Mn and target elements for its production were determined in 80- to 400-mg samples from 13 different locations of the LL6 chondrite St. Severin, along the 34.8-cm drill core AIII. The53Mn content increases from the surface to the center of the stone by ≈30%. The variation with depth is satisfactorily described by several models, presuming that appropriate primary and secondary particle fluxes are chosen. The53Mn saturation activities (53Mn*) are linearly correlated with the spallogenic3He/21Ne and22Ne/21Ne ratios, which suggests the possibility to eliminate uncertainties in the determination of53Mn cosmic ray exposure ages arising from depth effects and terrestrial residence times.  相似文献   

9.
Three ferromanganese nodules handpicked from the tops of 2500 cm2 area box cores taken from the north equatorial Pacific have been analysed for their U-Th series nuclides.230Thexc concentrations in the surface 1–2 mm of the top side of the nodules indicate growth rates of 1.8–4.6 mm/106 yr. In two of the nodules a significant discontinuity in the230Thexc depth profile has been observed at ～0.3 m.y. ago, suggesting that the nodule growth has been episodic. The concentration profiles of231Paexc (measured via227Th) yield growth rates similar to the230Thexc data. The bottom sides of the nodules display exponential decrease of230Thexc/232Th activity ratio with depth, yielding growth rates of 1.5–3.3 mm/106 yr.The230Thexc and231Paexc concentrations in the outermost layer of the bottom face are significantly lower than in the outermost layer of the top face. Comparison of the extrapolated230Thexc/232Th and230Thexc/231Paexc activity ratios for the top and bottom surfaces yields an “age” of (5?15) × 104 yr for the bottom relative to the top. This “age” most probably represents the time elapsed since the nodules have attained the present orientation.The210Pb concentration in the surface ～0.1 mm of the top side is in large excess over its parent226Ra. Elsewhere in the nodule, up to ～1 mm depth in both top and bottom sides,210Pb is deficient relative to226Ra, probably due to222Rn loss. The absence of210Pbexc below the outermost layer of the top face rules out the possibility of a sampling artifact as the cause of the observed exponentially decreasing230Thexc and231Paexc concentration profiles. The flux of210Pbexc to the nodules ranges between 0.31 and 0.58 dpm/cm2 yr. The exhalation rate of222Rn, estimated from the226Ra-210Pb disequilibrium is ～570 dpm/cm2 yr from the top side and >2000 dpm/cm2 yr from the bottom side.226Ra is deficient in the top side relative to230Th up to ～0.5–1 mm and is in large excess throughout the bottom. The data indicate a net gain of226Ra into the nodule, corresponding to a flux of (24?46) × 10?3 dpm/cm2 yr. On a total area basis the gain of226Ra into the nodules is <20% of the226Ra escaping from the sediments. A similar gain of228Ra into the bottom side of the nodules is reflected by the high228Th/232Th activity ratios observed in the outermost layer in contact with sediments.  相似文献   

10.
The distribution of “ash” (the non-combustible fraction of marine suspended matter) and concentrations of particulate Al, Ca, Fe, Cr, Ni, Cu, Sr and234Th in surface waters and of210Pb,230Th and234Th in two vertical profiles (385–4400 m) of the Indian Ocean are reported.The ash concentrations in surface waters follow the primary productivity pattern, with higher abundances in samples south of 40°S and lower concentrations in the equatorial and subtropical regions. Opaline silica and CaCO3 are the dominant components of the ash in samples from >40°S and from 7°N to 39°S, respectively. Aluminosilicates are only a minor constituent of the surface particulate matter. The metal/Al ratios in the surface particles are significantly higher compared to their corresponding crustal ratios for all the metals analyzed in this work. Comparison of enrichment factors between marine aerosols, plankton and surface oceanic particles, seem to indicate that this high metal/Al ratio in surface particles most likely arises from their involvement in marine biogeochemical cycles. Particulate234Th activity in surface waters parallels the ash abundance implying that its scavenging efficiency from surface waters depends on the particulate concentration.The particulate230Th and210Pb concentration profiles increase monotonously with depth. It is difficult to ascribe this increase to a process other than the in-situ vertical scavenging of230Th and210Pb from the water column by settling particles. The mean settling velocities of particles calculated from the particulate230Th data using a one-dimensional settling model is about 2 × 10?3 cm/s. The settling velocity computed from the particulate230Th profiles does not appear to be compatible with the particulate210Pb depth profiles; one possible explanation to account for the disparity would be that230Th and210Pb are scavenged by different size populations of particles.On the whole, the geographic distribution of particulate matter, their composition and settling velocities in the Atlantic, Pacific and Indian Oceans are similar indicating that they are controlled by quite similar processes in the marine hydrosphere.  相似文献   

11.
Cosmic-ray-produced53Mn (t1/2 = 3.7 × 106years) was measured in individual and groups of deep-sea iron and stony spherules by highly sensitive neutron activation analysis. The activities found were less than 20 dpm53Mn/kg Fe (10?5?10?6 dpm53Mn/sample) in iron spherules except one iron spherule whose activity was 241 ± 73 dpm53Mn/kg Fe. These low activities may indicate evaporative loss of53Mn due to heating in the earth's atmosphere. On the other hand, all stony spherules contained 200–260 dpm53Mn/kg Fe which is similar to chondritic values. These spherules may be ablation debris from large objects.  相似文献   

12.
Ti-V plots and the petrogenesis of modern and ophiolitic lavas   总被引：10，自引：0，他引：10  
Radioactive and stable cosmogenic nuclides have been determined in the various fragments of the Kirin chondrite (H5). Experimental results obtained from our samples are described and compared with similar data obtained in other laboratories. Cosmogenic54Mn,22Na,60Co,26Al,53Mn,40K (in the metal phase), and light noble gases were measured. Based on these data, the irradiation history of this meteorite can be explained in terms of (1) a multi-stage exposure which involves a first-stage irradiation for 107 years and a second stage for about 4×105 years, and (2) depth effects in the productions of the nuclides in 4π(second stage) and 2π(first stage) geometries. These conclusions are consistent with those of our previous work which was based on a limited number of samples.  相似文献   

13.
Seven vertical profiles of226Ra have been measured along an east-west traverse at about 30°N from San Diego to northwest of Hawaii. These profiles show that there is a distinct core of Ra maximum spreading westward as a tongue in the northeast Pacific deep water. This core starts in the east with 21.1 Ra units (1Ra unit= 10?14g/kg) at 3.9 km depth at about 130°W, and deepens westward to 4.1 km with its Ra reduced to 18.3 units at 150°W. A similar core with some uncertainty due to possible sampling errors extends westward near the bottom at 5.2 km depth from 19.4 Ra units at 150°W to 15.9 units at about 180° longitude. In addition, these profiles appear to be correlated with each other in structure above the cores of Ra maximum. These cores indicate that the Ra input depends locally on the type and composition of sediments and so the flux varies over the ocean bottom. On the basis of a one-dimensional diffusion-decay model, a horizontal diffusion coefficient of 106 cm2/sec has been computed along these cores. Although this value appears to be slightly lower, it is not inconsistent with those derived from other physical methods.  相似文献   

14.
The Apollo 16 soils have the largest low energy neutron fluences (up to 1017 n/cm2, E < 0.18eV) yet observed in lunar samples. Variations in the isotopic ratios 158Gd/157Gd and 150Sm/149Sm (up to 1.9% and 2.0% respectively) indicate that the low energy neutron fluence in the Apollo 16 drill stem increases with depth throughout the section sampled. Such a variation implies that accretion has been the dominant regolith “gardening” process at this location. The data may be fit by a model of continuous accretion of pre-irradiated material at a rate of ～70 g/(cm2 · 108yr) or by models involving as few as two slabs of material in which the first slab could have been deposited as long as 109 yr ago.The ratio of the number of neutrons captured per atom by Sm to the number captured per atom by Gd is lower than in previously measured lunar samples, which implies a lower energy neutron spectrum at this site. The variation of this ratio with chemical composition is qualitatively similar to that predicted by Lingenfelter, Canfield and Hampel.Variations are observed in the ratio 152Gd/160Gd which are fluence correlated and probably result from neutron capture by151Eu.  相似文献   

15.
The density, and therefore the pressure, of CO2 fluid inclusions in minerals can be estimated from the Fermi diad splitting of Raman spectra of CO2. An accurate determination of the pressure of CO2 fluid inclusions enables the estimation of the depth origin of rocks from the deep Earth. A micro-Raman densimeter was applied to ultramafic–mafic xenoliths sampled along the Ohku coast of Oki-Dogo Island in the Sea of Japan (East Sea). The density of CO2 fluid inclusions in the mafic granulite was 1.02–1.05 g/cm3, while those of lherzolites were 0.98–1.02 g/cm3. In contrast, the density of CO2 fluid inclusions measured in olivine gabbro, clinopyroxenite, and harzburgite were lower ranging from 0.86–to 0.99 g/cm3. Taking into account the temperature condition estimated using a pyroxene thermometer, the mafic granulite originated from a depth of 27–30 km and the lherzolites from 25–29 km. The overlapping depth of 27–29 km can be interpreted as the depth including the Moho discontinuity under Oki-Dogo Island 3.3 Ma. This estimation is consistent with geophysical observations.  相似文献   

16.
Water samples collected at the 21°N hydrothermal site on the East Pacific Rise crest, including Deep-Tow and hydrocast samples collected in 1977 and three hot vent water samples collected recently with the submersible “Alvin”, contain significant additions of3He,4He, and Mn. Although the vent water collections were at least 50-fold diluted with ambient seawater, they are up to 53 times enriched in3He and 7.4 times enriched in4He relative to saturated seawater, with concentrations of total dissolvable manganese (TDM) up to 310 μg/kg.3He and4He covary in the vent samples, with3He/4He about 8 times the atmospheric ratio, reflecting a mantle helium source. In contrast to the helium isotopes the Mn/3He ratio in the vent samples is variable, ranging from 4.3 × 104 up to 1.0 × 105 g/cm3. Profiles of3He/4He and TDM in the water column at 21°N show a sharp maximum ofδ(3He) = 47%and TDM= 0.69 μg/kg, much higher than the average values of 34% and 0.2 μg/kg for the deep water in this region. This spike in3He and Mn occurs at 2400 m depth, 200 m above the level of the 21°N vents, and 100 m higher than any local bathymetry, evidence for upward transport of the hydrothermal discharge via rising plumes of hot vent water. Two of the 21°N Deep-Tow samples associated with small (?0.010°C) temperature anomalies hadδ(3He) = 38%and TDM= 0.28 and 0.58 μg/kg, also slightly elevated relative to background. The Deep-Tow and hydrocast samples have lower Mn/3He ratios than average vent samples due to Mn removal by scavenging. Comparison of vent samples and water column measurements at 21°N indicate that the pure vent water could be detected using3He and Mn even when diluted ～105 times with seawater, confirming that these two tracers are extremely sensitive indicators of submarine hydrothermal activity.  相似文献   

17.
The thermoluminescence (TL) of various plagioclase feldspars embedded in a thick target of 150 kg of artificial lunar soil was measured after a 600-MeV proton irradiation. No correlation was observed between the parameters of the characteristic feldspar glow peak and the anorthite contents. The relative TL sensitivities of the individual plagioclase variants were measured and found to be practically the same for60Co-γ- and 600-MeV proton-irradiated samples.The TL intensity distribution within the target arrangement, converted to a 2π isotropic p-influx, resulted in an approximate TL depth profile of a thermally undisturbed lunar soil bomarded by galactic cosmic protons. The undisturbed TL intensity at a depth of 28 g/cm2 (? 17 cm) decreased to 39% at a depth of 106 g/cm2 (? 60 cm). For the evaluation of the temperature gradients by TL in lunar samples the experimental data at the sites of Taurus-Littrow and of Hadley-Rille yielded minimum depth intervals for sampling of ～ 20 cm and ～ 40 cm respectively, presuming an error of ± 15% in the TL determination. Certain aspects are seen by using the relation TL intensity/22Na-activity ratio versus depth (thus representing the total ionization profile) to establish22Na depth profiles.  相似文献   

18.
Data for the diffusion of cations in pyroxenes are relevant to a variety of sub-solidus processes including order-disorder and exsolution. Similar data must also be available if the reliability of geobarometers and geothermometers involving pyroxenes is to be assessed. Two types of diffusion experiment have been performed to determine cation diffusion rates in pyroxenes: (1) interdiffusion between single crystals of diopside and polycrystalline sinters enriched in Al and Fe, and (2) interdiffusion between single crystals of diopside and a glass of the same composition which was isotopically enriched in26Mg and43Ca. Following high-temperature annealing for periods up to several hundred hours, analysis of the diffusion couples, using an electron microprobe and an ion microprobe respectively, failed to show any measurable diffusion profiles. From these “null result” experiments the diffusion coefficients (D) for Al and Fe in diopside are estimated to be less than4×10?14cm2s?1 at 1200°C, and values ofD for Ca and Mg in diopside are estimated to be less than7 × 10?14cm2s?1 at 1250°C. These rates are significantly slower than published tracer-type diffusion data for Ca and Al.A review of studies of order-disorder, microstructural coarsening, and diffusion in pyroxenes suggest that activation energies for cation exchange are typically in excess of 60 kcal mol?1. Transport rates will be assisted, and activation energies lowered by sample non-stoichiometry, inhomogeneities, high dislocation densities and the presence of water.The collective data for Al, Mg and Ca diffusion in diopside indicate diffusion coefficients? 10?15cm2s?1 at 1200°C. A comparison with data for diffusion in garnet, olivine and spinel suggests that pyroxenes may have the highest blocking temperatures.  相似文献   

19.
Vertical eddy diffusivities (Kv's) have been estimated at fourteen widely separated locations from fourteen222Rn profiles and two228Ra profiles measured near the ocean floor as part of the Atlantic and Pacific GEOSECS programs. They show an inverse proportionality to the local buoyancy gradient [(g/?)(??pot/?z)] calculated from hydrographic measurements. The negative of the constant of proportionality is the buoyancy flux [?Kv(g/?)(??pot/?z)] which has a mean of ?4 × 10?6 cm2/sec3. Our results suggest that the buoyancy flux varies very little near the ocean floor. Kv's for the interior of the deep Pacific calculated from the relationship Kv = (4 × 10?6cm2/sec3)/[(g/?)(??pot/?z)] agree well with published estimates. Kv's calculated for the pycnocline are one to two orders of magnitude smaller than upper limits estimated from tritium and7Be distributions.Heat fluxes calculated with the model Kv's obtained from the222Rn profiles average 31 μcal cm?2 sec?1 in the Atlantic Ocean and 8 μcal cm?2 sec?1 in the Pacific Ocean.  相似文献   

20.
Many glacial deposits in the Quartermain Mountains, Antarctica present two apparent contradictions regarding the degradation of unconsolidated deposits. The glacial deposits are up to millions of years old, yet they have maintained their meter‐scale morphology despite the fact that bedrock and regolith erosion rates in the Quartermain Mountains have been measured at 0·1–4·0 m Ma?1. Additionally, ground ice persists in some Miocene‐aged soils in the Quartermain Mountains even though modeled and measured sublimation rates of ice in Antarctic soils suggest that without any recharge mechanisms ground ice should sublimate in the upper few meters of soil on the order of 103 to 105 years. This paper presents results from using the concentration of cosmogenic nuclides beryllium‐10 (10Be) and aluminum‐26 (26Al) in bulk sediment samples from depth profiles of three glacial deposits in the Quartermain Mountains. The measured nuclide concentrations are lower than expected for the known ages of the deposits, erosion alone does not always explain these concentrations, and deflation of the tills by the sublimation of ice coupled with erosion of the overlying till can explain some of the nuclide concentration profiles. The degradation rates that best match the data range 0·7–12 m Ma?1 for sublimation of ice with initial debris concentrations ranging 12–45% and erosion of the overlying till at rates of 0·4–1·2 m Ma?1. Overturning of the tills by cryoturbation, vertical mixing, or soil creep is not indicated by the cosmogenic nuclide profiles, and degradation appears to be limited to within a few centimeters of the surface. Erosion of these tills without vertical mixing may partially explain how some glacial deposits in the Quartermain Mountains maintain their morphology and contain ground ice close to the surface for millions of years. Copyright © 2010 John Wiley & Sons, Ltd.  相似文献   

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