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1.
A calculation method for determining the amount of Rn isotopes and daughter products at the start of measurement (CRAS) is proposed as a more accurate means of estimating the initial Rn concentration in soil gas. The CRAS utilizes the decay law between 222Rn and 220Rn isotopes and the daughter products 218Po and 216Po, and is applicable to α-scintillation counter measurements. As Rn is both inert and chemically stable, it is useful for fault investigation based on the soil gas geochemistry. However, the total number of α particles emitted by the decay of Rn has generally been considered to be proportional to the initial Rn concentration, without considering the gas condition with respect to radioactive equilibrium. The CRAS method is shown to be effective to derive Rn concentration for soil gases under both nonequilibrium conditions, in which the total number of decays increases with time, and equilibrium conditions, which are typical of normal soil under low gas flux. The CRAS method in conjunction with finite difference method simulation is applied to the analysis of two active fault areas in Japan, and it is demonstrated that this combination could detect the sharp rises in 222Rn concentrations associated with faults. The method also allows the determination of fault geometry near the surface based on the asymmetry variation of the Rn concentration distribution when coupled with a numerical simulation of 222Rn transport. The results for the new method as applied to the two case studies are consistent with the data collected from the geological survey. It implies that the CRAS method is suitable for investigating the fault system and interstitial gas mobility through fractures. The present analyses have also demonstrated that high Rn concentrations require the recent and repeated accumulation of 222Rn parents (230Th and 226Ra) in fault gouges through deep gas release during fault movement.  相似文献   

2.
The combined use of geophysical and soil gas composition exploration methods allows to rapidly obtain at relative low cost information that might be related to seismic activity conditions. In this study, we carried out geochemical soil gas sampling (222Rn, 220Rn and CO2), electrical resistivity tomography and seismic refraction profiles in two selected zones near the town of Amer in the Spanish Pyrenees, where the presence of recent fractures is evident in the field. Data analysis clearly reveals anomalous values for each gas at specific positions along the electrical imaging transects. Geomorphologic and hydrogeologic data and the integration of geophysical data and soil gas measurements indicate that: (1) endogene gases radon (222Rn) and carbon dioxide (CO2) are released from the meta-sedimentary basement rocks across the main fractured zones with higher permeability values, while lower Cenozoic detrital sedimentary formations act as an impervious boundary; (2) sites with highest radon concentrations (52?kBq?m?3) coincide with the zones in the Amer fault showing more recent geomorphic evidence of activity, and more specifically with those areas covered by thinner surficial formations; (3) the lowest 222Rn values (0.2?C0.4?kBq?m?3) were recorded just on the master active fault plane. This pattern could be explained by a dilution effect resulting from high rates of soil CO2 efflux (267?g?m?2?day?1); (4) soil thoron (220Rn) activity is maximum (143?kBq?m?3) in areas with high surficial fracturing; (5) groundwater pumping may cause important distortions in the natural flow dynamics and in the measured concentrations of gases. The agreement between the different data (geochemical, geophysical, and hydrogeological) and field observations (geology and geomorphology) leads us to propose a preliminary tectonic-gravitational model for the study area.  相似文献   

3.
本文是为了确定在卢氏盆地内被第四系覆盖的黄村断裂的位置、断裂性质,分析黄村断裂与其北侧的乔家窑地热异常的关系。断裂构造是深部氡气汇集和迁移的主要通道,氡气沿断裂向上迁移,在地表浅部形成氡异常。土壤氡气异常可揭示隐伏断裂构造的位置、产状和活动性。黄村断裂通过卢氏乔家窑一带,为第四系沉积物所覆盖。沿垂直断裂走向方向布置4条测线。应用瞬时土壤测氡仪进行了野外现场测量,测试了土壤氡气浓度,确定土壤氡气异常,分析黄村断裂位置、产状和活动性。结果表明:黄村断裂带上方土壤氡气具有异常显示,异常位置与断层位置具有较好的一致性。沿QJ12测线,从南向北,土壤氡气异常形态为低-高-较高-较低-低的峰值形态。在断层带上方氡气峰值异常高于背景值的1.5倍以上,异常峰多数为2个测点以上组成。土壤氡气变化特征表明黄村断裂具有较强的活动性。利用土壤氡气异常分析了黄村断裂深部结构特征,给出了主断裂面与次级断裂面产状和位置。结合土壤氡气异常,分析了乔家地热形成机理。初步研究结果表明,豫西基底构造具有多期活动性,活化区域内的压扭性断裂,可转变为局部张性断裂,控制水热、成矿物质的迁移和富集。  相似文献   

4.
The structure of the acoustic basement of the eastern part of the St. Paul multifault transform fracture system hosts rift paleovalleys and a paleonodal depression that mismatch the position of the currently active zones. This displacement zone, which is composed of five fault troughs, is unstable in terms of the position of the rift segments, which jumped according to redistribution of stresses. The St. Paul system is characterized by straightening of the transform transition between two remote segments of the Mid-Atlantic Ridge (MAR). The eastern part of the system contains anomalous bright-spot-like reflectors on the flattened basement, which is a result of atypical magmatism, that forms the standard ridge relief of the acoustic basement. Deformations of the acoustic basement have a presedimentation character. The present-day deformations with lower amplitude in comparison to the basement are accompanied by acoustic brightening of the sedimentary sequence. The axial Bouguer anomalies in the east of the system continue to the north for 120 km from the active segments of the St. Paul system. Currently seismically active segments of the spreading system are characterized by increasing amplitudes of the E–W displacement along the fault troughs. Cross-correlation of the lengths of the active structural elements of the MAR zone (segments of the ridge and transform fracture zones of displacement) indicates that, statistically, the multifault transform fracture system is a specific type of oceanic strike-slip faults.  相似文献   

5.
地震活动断裂带能够向大气释放大量的温室气体、放射性气体和有毒气体(CO_2、CH_4、Rn和Hg),并对大气环境的影响产生复杂的影响。利用静态暗箱法,对汶川M_s8.0地震破裂带CO_2、Rn和Hg脱气强度进行实地测量,并计算了CO_2和Hg脱气对大气的年贡献量。结果表明:(1)破裂带土壤气中CO_2、CH_4、Rn和Hg异常浓度最大值分别可以达到7.98%、2.38%、524.30k Bq/m~3和161.00ng/m~3;破裂带CO_2、Rn和Hg脱气平均通量是34.95g·m~(-2)d~(-1)、36.11m Bq·m~(-2)s~(-1)和26.56ng·m~(-2)h~(-1),最大值分别达到259.23g·m~(-2)d~(-1)、580.35m Bq·m~(-2)s~(-1)和387.67ng·m~(-2)h~(-1);(2)汶川Ms8.0地震破裂带向大气脱气的CO_2年贡献量是0.95Mt,Hg的年贡献量是15.94kg。汶川Ms8.0地震破裂带破裂CO_2、CH_4、Rn和Hg等的脱气强度,不仅与破裂带渗透率有关,还与断裂带浅部存在的气藏、煤层以及磷矿层等气体源有重要的联系。  相似文献   

6.
Published reports show that 222Rn contents of soil gas can increase under snow-covered or frozen soils. By utilizing these observations and results of field tests described here, it can be stated that U prospecting with 222Rn in frozen terrain is practicable.Rn profiles in frozen and snow-covered soils over U mineralization in the Bancroft area of Ontario outlined known radioactive zones more clearly than did scintillometer profiles.Tests in Gatineau Park, Quebec, in the proximity of a radioactive pegmatite dike showed that lake ice acts as a restrictive barrier to Rn movement from lake waters beneath. Water samples, collected and allowed to freeze in plastic bottles, retained dissolved Rn quite effectively thus permitting sample collection and storage under the most severe winter conditions. Rn sampling of through-ice lake waters is therefore a feasible prospecting tool.Samples of spring run-off (snow-melt) waters and slushy snow collected from within a known weakly radioactive zone near South March, Ontario, were shown to contain less Rn than found in the same stream waters in the summer. No pronounced Rn degassing event of frozen soils was apparent early in the spring thaw in percolating run-off waters draining from the zone. The usefulness of spring thaw hydrogeochemistry using Rn is discussed.  相似文献   

7.
The mechanism of222Rn release into fracture fluids by direct alpha-recoil, lattice and grain boundary/micro-crack diffusion is discussed. Experimental measurements of222Rn release into surrounding air and water phases have been made for crystalline rock specimens with well defined surface areas. The222Rn flux from an infinite plane surface and hence the effective diffusion length of222Rn in the rock matrix has been estimated.The222Rn flux from plane crystalline rock surfaces has been used in conjunction with a simple hydrological model of the reservoir to calculate the222Rn content of the return fluids of a geothermal doublet circulation system. For given production rate and piezometric difference between the injection and production wells, the222Rn content of the return fluid is dependent upon the distribution of flow path lengths and fracture apertures in the reservoir. Matching of the calculated and experimental222Rn contents of the return fluids has been used to select appropriate parameters for the reservoir model and hence to estimate the extent of the heat-transfer surface. The model estimates the fracture width of the flow paths, total swept surface area and fracture volume within the reservoir.  相似文献   

8.
《Applied Geochemistry》1986,1(6):647-657
The mechanism of222Rn release into fracture fluids by direct alpha-recoil, lattice and grain boundary/micro-crack diffusion is discussed. Experimental measurements of222Rn release into surrounding air and water phases have been made for crystalline rock specimens with well defined surface areas. The222Rn flux from an infinite plane surface and hence the effective diffusion length of222Rn in the rock matrix has been estimated.The222Rn flux from plane crystalline rock surfaces has been used in conjunction with a simple hydrological model of the reservoir to calculate the222Rn content of the return fluids of a geothermal doublet circulation system. For given production rate and piezometric difference between the injection and production wells, the222Rn content of the return fluid is dependent upon the distribution of flow path lengths and fracture apertures in the reservoir. Matching of the calculated and experimental222Rn contents of the return fluids has been used to select appropriate parameters for the reservoir model and hence to estimate the extent of the heat-transfer surface. The model estimates the fracture width of the flow paths, total swept surface area and fracture volume within the reservoir.  相似文献   

9.
刘江  张进江  郭磊  戚国伟 《岩石学报》2014,30(7):1899-1908
晚中生代,内蒙古大青山依次经历晚侏罗世盘羊山逆冲推覆、早白垩世呼和浩特变质核杂岩伸展、早白垩世大青山逆冲推覆断层及早白垩世以来高角度正断层复杂构造演化。其中,呼和浩特变质核杂岩韧性剪切带的冷却时间和抬升机制的制约尚不明确。本文在野外考察和显微构造分析基础上,采用逐步加热40Ar-39Ar定年法对韧性剪切带内不同单矿物的冷却年龄进行了测定。角闪石、白云母、黑云母和钾长石单矿物40Ar-39Ar冷却年龄处于120~116Ma之间。结合已有年龄数据及单矿物封闭温度,构建了韧性剪切带的冷却曲线。结果表明,韧性剪切带在122~115Ma期间存在一个明显的快速冷却过程。这一阶段快速冷却是与变质核杂岩拆离断层相关核部杂岩拆离折返作为大青山逆冲推覆断层上盘抬升的结果。  相似文献   

10.
《Applied Geochemistry》1995,10(4):437-446
This is the first study on Pb stable isotopes in fault gouges and their parent rocks. We analyzed the composition of Pb isotopes and contents of U and Pb in 10 pairs of fault gouges and their parent rocks collected along several active faults in central Japan. Thorium-232-208Pb ages of two fault systems were determined as pre-Tertiary, which are consistent with the data from KAr ages and geological considerations.Naturally, the235U207Pb system is of little use for dating because the magnitude of difference in207Pb/204Pb between gouges and parent rocks is too small. It is found that the206Pb/204Pb can indicate the contribution of206Pb resulting from excess supplies of226Ra and222Rn along the fault. The excess206Pb accumulation rate corresponds to the average222Rn concentration in soil gas or groundwater through geological time since the gouge formation. A comparison of Quaternary fault activity and estimated Tertiary activity reveals the characteristics of each fault system.  相似文献   

11.
In the Alban Hills area, strong areally diffuse and localised spot degassing processes occur (Tivoli, Cava dei Selci, Solforata, Tor Caldara). The gas comprises a large proportion of CO2, with minor CH4, H2S and Rn. These advective features are generated by fluid leakage from buried reservoirs hosted in the structural highs of the Mesozoic carbonate basement. Gas migration towards the surface is controlled by fault and fracture systems bordering the structural highs of the carbonate formations (e.g. Ciampino high). His release is triggered when the total pressure of the fluid phase exceeds the hydrostatic pressure, thus forming a free gas phase. Furthermore, both the sudden and catastrophic, and slow and continuous gas release at surface, of naturally occurring toxic species (CO2, H2S and Rn) poses a serious health risk to people living in this geologically active area.This paper presents data obtained from soil gas and gas flux surveys, as well as gas isotopes analyses, which suggest the presence of a deep origin gas flux enriched in carbon dioxide and minor species (CH4 and H2S), as well as a channelled migration of geogas mixtures having a Rn component which is not produced in situ.In regards to the health risk to local inhabitants, it was found that some anomalous areas had been zoned as parkland while others had been heavily developed for residential purposes. For example, many new houses were found to have been built on ground which has soil gas CO2 concentrations of over 70% and a CO2 flux of about 0.7 kg m−2 day−1, as well as radon values of more than 250 kBq/m3. In addition, an indoor radon survey has been conducted in selected houses in the town of Cava dei Selci to search for a possible correlation between the local geology and the radon concentration in indoor air. Preliminary results indicate high indoor values at ground floor levels (up to 1000 Bq/m3) and very high values in the cellars (up to 250.000 Bq/m3). It is recommended that land-use planners incorporate soil gas and/or gas flux measurements in the environmental assessment of areas of possible risk (i.e. volcanic or structurally active areas).  相似文献   

12.
The spatio-temporal variations of soil gas in the seismic fault zone produced by the 12 May 2008 Wenchuan Ms 8.0 earthquake were investigated based on the field measurements of soil gas concentrations after the main shock. Concentrations of He, H2, CO2, CH4, O2, N2, Rn, and Hg in soil gas were measured in the field at eight short profiles across the seismic rupture zone in June and December 2008 and July 2009. Soil-gas concentrations of more than 800 sampling sites were obtained. The data showed that the magnitudes of the He and H2 anomalies of three surveys declined significantly with decreasing strength of the aftershocks with time. The maximum concentrations of He and H2 (40 and 279.4 ppm, respectively) were found in three replicates at the south part of the rupture zone close to the epicenter. The spatio-temporal variations of CO2, Rn, and Hg concentrations differed obviously between the north and south parts of the fault zone. The maximum He and H2 concentrations in Jun 2008 occurred near the parts of the rupture zone where vertical displacements were larger. The anomalies of He, H2, CO2, Rn, and Hg concentrations could be related to the variation in the regional stress field and the aftershock activity.  相似文献   

13.
《Applied Geochemistry》1996,11(4):497-510
Radon emanation has been observed to be anomalously high along active faults in many parts of the world. We tested this relationship by conducting and repeating soil-air radon surveys with a portable radon meter across several faults in California. The results confirm the existence of fault-associated radon anomalies, which show characteristic features that may be related to fault structures but vary in time due to other environmental changes, such as rainfall. Across two creeping faults in San Juan Bautista and Hollister, the radon anomalies showed prominent double peaks straddling the fault-gouge zone during dry summers, but the peak-to-background ratios diminished after significant rain fall during winter. Across a locked segment of the San Andreas fault near Olema, the anomaly has a single peak located several meters southwest of the slip zone associated with the 1906 San Francisco earthquake. Across two fault segments that ruptured during the magnitude 7.5 Landers earthquake in 1992, anomalously high radon concentration was found in the fractures three weeks after the earthquake. We attribute the fault-related anomalies to a slow vertical gas flow in or near the fault zones. Radon generated locally in subsurface soil has a concentration profile that increases three orders of magnitude from the surface to a depth of several meters; thus an upward flow that brings up deeper and radon-richer soil air to the detection level can cause a significantly higher concentration reading. This explanation is consistent with concentrations of carbon dioxide and oxygen, measured in soil-air samples collected during one of the surveys.  相似文献   

14.
通过二维、三维地震资料解释与构造解析,明确了塔里木盆地塔中北坡发育多条北东向、北东东向走滑断裂带,在平面和剖面上识别出了6种走滑断裂活动的标志。研究表明,塔中北坡走滑断裂在剖面上呈直立断层、花状构造,北东向走滑断裂下部表现为明显挤压隆升,而上部则表现为继承性张扭负花状构造,具有"下拱上掉"的特征,表明了断裂的多期走滑活动。总体上可划分为中奥陶世末—志留纪压扭走滑断层、晚泥盆世—早石炭世张扭走滑断层和晚二叠世末逆冲断层三期,它们在空间上相互叠置。研究认为走滑断裂的变形强度控制了奥陶系裂缝及缝洞型储层发育范围,走滑断裂的分段性对优质缝洞型储层发育具有较强的控制作用。提出了在变形强度大的裂缝发育区、走滑断裂拉张部位的断洼区,以及受后期张扭走滑断裂叠加改造的断槽部位的串珠状地震反射异常体发育区,是下步寻找天然气规模储量的有利勘探方向。  相似文献   

15.
210Po and 210Pb measurements of soils delineated uranium anomalies at three out of four test sites in Ontario, Canada. Measurements were made of 210Po in solutions produced by both complete digestion and partial leaching of soil samples. Direct plating of 210Po onto metal plates was followed by measuring the alpha activity. Subsequent plating of 210Po in-grown from 210Pb in solution several months later confirmed the anomalies.The 210Po and 210Pb anomalies at three of the test sites coincided with 226Ra and 222Rn anomalies. Samples from the fourth uranium occurrence associated with a known 222Rn anomaly failed to show either a 226Ra anomaly on the one hand, or 210Po or 210Pb anomalies on the other. This suggests that the 210Po and 210Pb anomalies were probably produced by the decay of 226Ra contained within secondary dispersion haloes.Although anomalies due to the 210Po and 210Pb products of 222Rn have now been documented, prospecting methods based on their use as direct tracers of the migration paths of 222Rn require much further development.  相似文献   

16.
210Po and 210Pb measurements of soils delineated uranium anomalies at three out of four test sites in Ontario, Canada. Measurements were made of 210Po in solutions produced by both complete digestion and partial leaching of soil samples. Direct plating of 210Po onto metal plates was followed by measuring the alpha activity. Subsequent plating of 210Po in-grown from 210Pb in solution several months later confirmed the anomalies.The 210Po and 210Pb anomalies at three of the test sites coincided with 226Ra and 222Rn anomalies. Samples from the fourth uranium occurrence associated with a known 222Rn anomaly failed to show either a 226Ra anomaly on the one hand, or 210Po or 210Pb anomalies on the other. This suggests that the 210Po and 210Pb anomalies were probably produced by the decay of 226Ra contained within secondary dispersion haloes.Although anomalies due to the 210Po and 210Pb products of 222Rn have now been documented, prospecting methods based on their use as direct tracers of the migration paths of 222Rn require much further development.  相似文献   

17.
Data are presented on the molecular composition of drill-mud gas from the lower sedimentary section (1800–3987 m) of the SAFOD (San Andreas Fault Observatory at Depth) Main Hole measured on-line during drilling, as well as C and H isotope data from off-line mud gas samples. Hydrocarbons, H2 and CO2 are the most abundant non-atmospheric gases in drill-mud when drilling seismogenic zones. Gas influx into the well at depth is related to the lithology and permeability of the drilled strata: larger formation gas influx was detected when drilling through organic-rich shales and permeable sandstones. The SAF (San Andreas Fault), encountered between approximately 3100 m and 3450 m borehole depth, is generally low in gas, but is encompassed by two gas-rich zones (2700–2900 m and below 3550 m) at the fault margins with enhanced 222Rn activities and distinct gas compositions. Within the fault, two interstratified gas-rich lenses (3150–3200 m and 3310–3340 m) consist of CO2 and hydrocarbons (upper zone), but almost exclusively of hydrocarbons (lower zone).  相似文献   

18.
As natural gas becomes increasingly important in our daily life, studies have been carried out on trace elements such as mercury and arsenic within it. Other than those, the existence of radioactive gaseous radon from the combustion of natural gas indoors can cause severe diseases and damages to body organs, putting a hazardous impact on human health. At the same time, the radon can also corrode gas production and transportation equipment. A review of the literature on radon concentrations in natural gas produced from gas reservoirs in China and other countries have been studied. Radon is a decay product from 238U, which is closely related to the accumulation and migration of organic matter during diagenesis. Gas recovered from reservoirs with higher than average natural 238U contains higher than average levels of 222Rn. Massive fault systems and fracture zones appear to play a significant role in radon concentrations in natural gas.  相似文献   

19.
基于土壤氡气测量识别甘肃北山南缘隐伏断裂   总被引：1，自引：0，他引：1  
李杰彪  周志超  云龙  苏锐  郭永海 《地质学报》2022,96(6):2240-2250
我国高放废物地质处置库首选预选区位于甘肃北山南缘，区内分布有多条大型非活动断裂构造，这些断裂很可能成为未来放射性核素迁移的主要通道。断裂在向地表延伸过程中，受第四系覆盖等因素影响，造成关键构造部位隐伏地下而难以识别。本文以北山地区新场地段南部红旗山和前红泉断裂为研究对象，采用土壤中氡气测量方法，探讨了大型断裂构造中隐伏段落的识别及其指示的水文地质意义。结果表明：土壤中氡气测量对于识别北山南缘隐伏断裂具有很好的指示意义，是传统地质调查方法的一种重要补充；红旗山和前红泉断裂裂隙系统整体开启性均较差，裂隙系统不发育，影响范围较小，不具备形成较大规模储水空间的可能性。不同断裂带土壤氡浓度背景值差异较大，可根据土壤氡浓度累积频率分布图确定背景值；土壤氡浓度等值线分布图对判断隐伏断裂位置具有一定的指示作用。对于压剪性断裂而言，主断裂多沿氡气高异常与低异常边界分布或表现为氡气中等异常，而两侧的次级断裂表现为氡气高异常。  相似文献   

20.
Soil-gas radon concentrations and exhalation rates have generally been observed to be anomalously high along active faults in many parts of the world. The soil-gas method is based on the principle that faults and fractures in rocks are highly permeable pathways along which gases can migrate upward from deep crust and mantle to soil cover, retaining their source signatures. The present study summarizes the influence of fault zones on anomalous radon concentrations in soil by integrated geophysical and geo-structural analyses in three study areas of Central-Northern Calabria (Southern Italy). Soil-gas radon surveys have been carried out by means of an alpha scintillation counting system, at 12,509 locations between 2002 and 2004. A geostatistical approach has been used to estimate the spatial distribution of soil radon concentrations. Relations among soil-gas distribution and geo-structural features have been evaluated by ordinary multi-Gaussian kriging. Highest soil radon concentrations (ca. 90 kBq m?3) have been measured in the Rossanese sector. In the three study areas, no appreciable differences can be noticed among lithotypes, with the highest concentration values (ca. 89 kBq m?3) measured in alluvial deposit and in clay. Measurements of soil-gas radon reveal anomalies clearly connected to the tectonic structures. Increased signals are linearly distributed along regional WNW–ESE trending shear zones, with main pathways of concentration also recognizable along the E–W fault system in the Rossanese sector, the N–S fault system in the Crati Graben and the Catanzaro Trough, and the NE–SW fault system in the Catanzaro Trough. The distribution of epicentres of historical earthquakes occurred between 1184 and 2001 confirms the recent activity of the same fault systems. Soil-gas radon concentrations generally increase, as expected, with decreasing distance to the faults.  相似文献   

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