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1.
We investigated the provenance of organic matter in the inner fjord area of northern Patagonia, Chile (～44–47°S), by studying the elemental (organic carbon, total nitrogen), isotopic (δ13C, δ15N), and biomarker (n-alkanoic acids from vascular plant waxes) composition of surface sediments as well as local marine and terrestrial organic matter. Average end-member values of N/C, δ13C, and δ15N from organic matter were 0.127±0.010, ?19.8±0.3‰, and 9.9±0.5‰ for autochthonous (marine) sources and 0.040±0.018, ?29.3±2.1‰, and 0.2±3.0‰ for allochthonous (terrestrial) sources. Using a mixing equation based on these two end-members, we calculated the relative contribution of marine and terrestrial organic carbon from the open ocean to the heads of fjords close to river outlets. The input of marine-derived organic carbon varied widely and accounted for 13–96% (average 61%) of the organic carbon pool of surface sediments. Integrated regional calculations for the inner fjord system of northern Patagonia covered in this study, which encompasses an area of ～4280 km2, suggest that carbon accumulation may account for between 2.3 and 7.8×104 ton C yr?1. This represents a storage capacity of marine-derived carbon between 1.8 and 6.2×104 ton yr?1, which corresponds to an assimilation rate of CO2 by marine photosynthesis between 0.06 and 0.23×106 ton yr?1. This rate suggests that the entire fjord system of Patagonia, which covers an area of ～240,000 km2, may represent a potentially important region for the global burial of marine organic matter and the sequestration of atmospheric CO2.  相似文献   

2.
This study involved a baseline evaluation of fluvial carbon export and degas rates in three nested rural catchments (1 to 80 km2) in Taboão, a representative experimental catchment of the Upper Uruguay River Basin. Analyses of the carbon content in stream waters and the catchment carbon yield were based on 4‐year monthly in situ data and statistical modeling using the United States Geological Survey load estimator model. We also estimated p CO2 and degas fluxes using carbonate equilibrium and gas‐exchange formulas. Our results indicated that the water was consistently p CO2 saturated (~90% of the cases) and that the steep terrain favors high gas evasion rates. The mean calculated fluvial export was 5.4 tC·km?2·year?1 with inorganic carbon dominating (dissolved inorganic carbon:dissolved organic carbon ratio >4), and degas rates (~40 tC km?2·year?1) were nearly sevenfold higher than the downstream export. The homogeneous land use in this nested catchment system results in similar water‐quality characteristics, and therefore, export rates are expected to be closely related to the rainfall–runoff relationships at each scale. Although the sampling campaigns did not fully reproduce storm‐event conditions and related effects such as flushing or dilution of in‐stream carbon, our results indicated a potential link between dissolved inorganic carbon and slower hydrological pathways related to subsurface water storage and movement.  相似文献   

3.
An excess of fine sediment (grain size <2 mm) supply to rivers leads to reservoir siltation, water contamination and operational problems for hydroelectric power plants in many catchments of the world, such as in the French Alps. These problems are exacerbated in mountainous environments characterized by large sediment exports during very short periods. This study combined river flow records, sediment geochemistry and associated radionuclide concentrations as input properties to a Monte Carlo mixing model to quantify the contribution of different geologic sources to river sediment. Overall, between 2007 and 2009, erosion rates reached 249 ± 75 t km?2 yr?1 at the outlet of the Bléone catchment, but this mean value masked important spatial variations of erosion intensity within the catchment (85–5000 t km?2 yr?1). Quantifying the contribution of different potential sources to river sediment required the application of sediment fingerprinting using a Monte Carlo mixing model. This model allowed the specific contributions of different geological sub‐types (i.e. black marls, marly limestones, conglomerates and Quaternary deposits) to be determined. Even though they generate locally very high erosion rates, black marls supplied only a minor fraction (5–20%) of the fine sediment collected on the riverbed in the vicinity of the 907 km2 catchment outlet. The bulk of sediment was provided by Quaternary deposits (21–66%), conglomerates (3–44%) and limestones (9–27%). Even though bioengineering works conducted currently to stabilize gullies in black marl terrains are undoubtedly useful to limit sediment supply to the Bléone river, erosion generated by other substrate sources dominated between 2007 and 2009 in this catchment. Copyright © 2011 John Wiley & Sons, Ltd.  相似文献   

4.
Total organic carbon fluxes of the Red River system (Vietnam)   总被引：1，自引：0，他引：1       下载免费PDF全文
Riverine transport of organic carbon from terrestrial ecosystems to the oceans plays an important role in the global carbon cycle. The Red River is located in Southeast Asia where river discharge, sediment loads and fluxes of elements (carbon, nitrogen and phosphorus) associated with suspended solids have been dramatically altered over past decades as a result of reservoir impoundment and land use, population, and climate change. Dissolved organic carbon (DOC) and particulate organic carbon (POC) concentrations were measured monthly at four stations of the Red River system from January 2008 to December 2010. The results reveal that POC changed synchronically with total suspended solids (TSS) concentration and with the river discharge, whereas no clear trend was observed for DOC concentration. The mean value of total organic carbon (TOC = DOC + POC) flux in the delta of the Red River was 31.5 × 1013 ± 4.0 × 1013 MgC.yr?1 (range 27.9–35.8 × 1013 MgC.yr?1 which leads to a specific TOC flux of 2012 ± 255 kgC.km?2.yr?1 during this 2008–2010 period. About 80% of the TOC flux was transferred to the estuary during the rainy season as a consequence of the higher river water discharge. The high mean value of the POC:Chl‐a ratio (1585 ± 870 mgC.mgChl‐a?1) and the moderate C:N ratio (7.3 ± 0.1) in the water column system suggest that organic carbon in the Red River system is mainly derived from erosion and soil leaching in the basin. The effect of two new dam impoundments in the Red River was also observable with lower TOC fluxes in 2010 compared with 2008. Copyright © 2017 John Wiley & Sons, Ltd.  相似文献   

5.
This paper aims to provide an overview of regional carbon fluxes and budgets in the marginal seas adjacent to China.The "China Seas" includes primarily the South China Sea, East China Sea, Yellow Sea, and the Bohai Sea. Emphasis is given to CO_2 fluxes across the air-sea interface and their controls. The net flux of CO_2 degassing from the China Seas is estimated to be9.5±53 Tg C yr~(-1). The total riverine carbon flux through estuaries to the China Seas is estimated as 59.6±6.4 Tg C yr~(-1). Chinese estuaries annually emit 0.74±0.02 Tg C as CO_2 to the atmosphere. Additionally, there is a very large net carbon influx from the Western Pacific to the China Seas, amounting to ～2.5 Pg C yr~(-1). As a first-order estimate, the total export flux of particulate organic carbon from the upper ocean of the China Seas is 240±80 Tg C yr~(-1). This review also attempts to examine current knowledge gaps to promote a better understanding of the carbon cycle in this important region.  相似文献   

6.
Glacial erosion rates are estimated to be among the highest in the world. Few studies have attempted, however, to quantify the flux of sediment from the periglacial landscape to a glacier. Here, erosion rates from the nonglacial landscape above the Matanuska Glacier, Alaska are presented and compare with an 8‐yr record of proglacial suspended sediment yield. Non‐glacial lowering rates range from 1·8 ± 0·5 mm yr?1 to 8·5 ± 3·4 mm yr?1 from estimates of rock fall and debris‐flow fan volumes. An average erosion rate of 0·08 ± 0·04 mm yr?1 from eight convex‐up ridge crests was determined using in situ produced cosmogenic 10Be. Extrapolating these rates, based on landscape morphometry, to the Matanuska basin (58% ice‐cover), it was found that nonglacial processes account for an annual sediment flux of 2·3 ± 1·0 × 106 t. Suspended sediment data for 8 years and an assumed bedload to estimate the annual sediment yield at the Matanuska terminus to be 2·9 ± 1·0 × 106 t, corresponding to an erosion rate of 1·8 ± 0·6 mm yr?1: nonglacial sources therefore account for 80 ± 45% of the proglacial yield. A similar set of analyses were used for a small tributary sub‐basin (32% ice‐cover) to determine an erosion rate of 12·1 ± 6·9 mm yr?1, based on proglacial sediment yield, with the nonglacial sediment flux equal to 10 ± 7% of the proglacial yield. It is suggested that erosion rates by nonglacial processes are similar to inferred subglacial rates, such that the ice‐free regions of a glaciated landscape contribute significantly to the glacial sediment budget. The similar magnitude of nonglacial and glacial rates implies that partially glaciated landscapes will respond rapidly to changes in climate and base level through a rapid nonglacial response to glacially driven incision. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

7.
Recently, researchers have recognized the significant role of small mountainous river systems in the transport of carbon from terrestrial environments to the ocean, and the scale of such studies have ranged from channel bed units to continents. In temperate zones, these mountain river systems commonly drain catchments that are largely forested. However, the magnitude of carbon export from rivers draining old‐growth redwood forests has not been evaluated to date. Old‐growth redwood stands support some of the largest quantities of biomass in the world, up to 350 000 Mg of stem biomass km‐2 and soil organic carbon can reach 46 800 Mg km‐2. In north coastal California, suspended sediment samples were collected at three gaging stations for two to four years on streams draining old‐growth redwood forests. Carbon content, determined through loss‐on‐ignition tests, was strongly correlated with turbidity, and continuous turbidity records from the gaging stations were used to estimate annual carbon exports of 1 · 6 to 4 · 2 Mg km‐2 yr‐1. These values, representing 13 to 33% of the suspended sediment load, are some of the highest percentages reported in the global literature. The fraction of organic carbon as part of the suspended sediment load decreased with discharge, but reached an asymptote of 5 to 10% at flows 10 to 20 times the mean annual flows. Although larger rivers in this region exhibit high sediment yields (up to 3600 Mg km‐2 yr‐1), mainly attributed to high rates of uplift, mass movement, and timber harvest, the small pristine streams in this study have sediment yields of only 8 to 100 Mg km‐2 yr‐1. Because the current extent of old‐growth redwood stands is less than 5% of its pre‐European‐settlement distribution, the present organic carbon signature in suspended sediment loads in this region is likely different from that in the early 20th century. Published 2015. This article is a U.S. Government work and is in the public domain in the USA.  相似文献   

8.
Black marls form very extensive outcrops in the Alps and constitute some of the most eroded terrains, thus causing major problems of sedimentation in artificial storage systems (e.g. reservoirs) and river systems. In the experimental catchments near Draix (France), soil erosion rates have been measured in the past at the plot scale through a detailed monitoring of surface elevation changes and at the catchment scale through continuous monitoring of sediment yield in traps at basin outlets. More recently, erosion rates have been determined by means of dendrogeomorphic techniques in three monitored catchments of the Draix basin. A total of 48 exposed roots of Scots pine have been sampled and anatomical variations in annual growth rings resulting from denudation analysed. At the plot scale, average medium‐term soil erosion rates derived from exposed roots vary between 1·8 and 13·8 mm yr?1 (average: 5·9 mm yr?1) and values are significantly correlated with slope angle. The dendrogeomorphic record of point‐scale soil erosion rates matches very well with soil erosion rates measured in the Draix basins. Based on the point‐scale measurements and dendrogeomorphic results obtained at the point scale, a linear regression model involving slope angle was derived and coupled to high‐resolution slope maps obtained from a LiDAR‐generated digital elevation model so as to generate high‐resolution soil erosion maps. The resulting regression model is statistically significant and average soil erosion rates obtained from the areal erosion map (5·8, 5·2 and 6·2 mm yr?1 for the Roubine, Moulin and Laval catchments, respectively) prove to be well in concert with average annual erosion rates measured in traps at the outlet of these catchments since 1985 (6·3, 4·1 and 6·4 mm yr?1). This contribution demonstrates that dendrogeomorphic analyses of roots clearly have significant potential and that they are a powerful tool for the quantification and mapping of soil erosion rates in areas where measurements of past erosion is lacking. Copyright © 2011 John Wiley & Sons, Ltd.  相似文献   

9.
Rainfall, peak discharges, and suspended sediment transport were surveyed for 280 events in three small (0.8 to 10 km2) catchments in a hilly area derived from Neogene marls, silts, and sands. Under similar hydrological input conditions, stream flow behaviour and sediment delivery differed considerably from one catchment to another, depending on topography, lithology, land use, and especially sediment availability. Analytical treatment of data showed a good fit between sediment yield and peak flow discharge. Less good, although still significant, was the correlation between sediment concentration and discharge values for different flow stages. Rainfall peak/basin lag time and rainfall/discharge showed poor or no correlation, mainly due to strong variations in rainfall distribution. Sediment concentration in the catchments varied enormously according to season, from zero up to 334 g 1?1; sediment yield was 160-900 tonnes km?2 yr?1 in the two major catchments, and over 5200 tonnes km?2 yr?1 in the headwater catchment, stressing the importance of small tributaries not only in inducing floods in downstream channels, but also in sediment supply.  相似文献   

10.
Cultivated fields have been shown to be the dominant sources of sediment in almost all investigated UK catchments, typically contributing 85 to 95% of sediment inputs. As a result, most catchment management strategies are directed towards mitigating these sediment inputs. However, in many regions of the UK such as the Nene basin there is a paucity of sediment provenance data. This study used the caesium‐137 (137Cs) inventories of lake and floodplain cores as well as the 137Cs activities of present day sediment to determine sediment provenance. Sediment yields were also reconstructed in a small lake catchment. Low 137Cs inventories were present in the lake and floodplain cores in comparison to the reference inventory and inventories in cores from other UK catchments. Caesium‐137 activities in the present day sediments were low; falling close to those found in the channel bank catchment samples. It was estimated that 60 to 100% of the sediment in the Nene originated from channel banks. Pre‐1963 sediment yields were approximately 11.2 t km?2 yr?1 and post‐1963 was approximately 11.9 t km?2 yr?1. The lack of increased sediment yield post‐1963 and low sediment yield is unusual for a UK catchment (where a yield of 28 to 51 t km?2 yr?1 is typical for a lowland agricultural catchment), but is explained by the low predicted contribution of sediment from agricultural topsoils. The high channel bank contribution is likely caused by the river being starved of sediment from topsoils, increasing its capacity to entrain bank material. The good agreement between the results derived using cores and recently transported sediments, highlight the reliability of 137Cs when tracing sediment sources. However, care should be taken to assess the potential impacts of sediment particle size, sediment focusing in lakes and the possible remobilization of 137Cs from sedimentary deposits. Copyright © 2016 John Wiley & Sons, Ltd.  相似文献   

11.
Widespread, intense rainfall over the Upper Rio Chagres watershed (414 km2) in central Panama during December 2010 triggered numerous landslides that introduced large numbers of trees to the river network. We flew by helicopter along the mainstem Upper Chagres and the adjacent margins of Lake Alhajuela, into which the Upper Chagres flows, in February and June 2011. We used low‐elevation video photography from these flights to tally the number of wood pieces stored along the lake margin and within the channel, and the number of landslides reaching the mainstem. We used these tallies with ground‐verified estimates of average wood piece size and landslide surface area, and assumptions about wood density, carbon content, and aboveground biomass, to develop a first‐order estimate of carbon export in the form of wood from the Upper Chagres following the 2010 storms. Based on the wood tally, we estimate 9 · 6 to 16 Mg C/km2 export, and from the landslide tally we estimate 24 Mg C/km2. We believe the landslide tally provides a more accurate minimum estimate of carbon export from the Upper Chagres during the December 2010 storms. These values are an order of magnitude higher than limited data for average or background rates of wood‐based carbon export from other catchments, but two orders of magnitude lower than wood‐based carbon export during extreme storms in Taiwan. The findings suggest that duration of flood flow above a threshold for mobilizing wood within the channel network exerts a more important control on wood export from the Upper Chagres than magnitude of flood peak. Copyright © 2013 John Wiley & Sons, Ltd.  相似文献   

12.
The Yellow River transports a large amount of sediment and particulate organic carbon (POC), which is thought to mainly derive from erosion of the Chinese Loess Plateau (CLP). However, the compositions, sources and erosional fluxes of POC in the Yellow River remain poorly constrained. Here we combined measurements of mineralogy, total organic carbon content (OCtotal), stable organic carbon isotopes (δ13Corg), radiocarbon (14C) activity of organic matter in bulk suspended sediments collected seasonally from the upper and middle Yellow River, to quantify the compositions and fluxes of the POC and to assess its sources (biospheric and petrogenic POC, i.e. POCbio and POCpetro, respectively). The results showed that the POC loading of sediments was controlled by mineralogy, grain size and specific surface area of loess particles. The Fmod of POC (0.71 to 0.31) can be explained by mixing of POCpetro with modern and aged POCbio. A binary mixing model based on the hyperbolic relationship of the Fmod and OCtotal revealed a wide range of ages of POCbio from 1300 to 11100 14C years. Relative to the upstream station, the annual POCbio and POCpetro fluxes in the Yellow River are more than doubled after it flows crossing the CLP within 35% drainage area gain, resulting in POCbio and POCpetro yields of the CLP at 3.50 ± 0.59 and 0.48 ± 0.49 tC/km2/yr, respectively. POC flux seasonal variation revealed that monsoon rainfall exerts a first-order control on the export of both POCbio and POCpetro from the CLP to the Yellow River, resulting in more than 90% of the annual POC exported during the monsoon season. Around one third of annual POC erosional flux was transported during a storm event period, highlighting the important role of extreme events in POC export in this large river. © 2020 John Wiley & Sons, Ltd.  相似文献   

13.
High‐resolution historical (1942) and recent (1994) digital terrain models were derived from aerial photographs along the Big Sur coastline in central California to measure the long‐term volume of material that enters the nearshore environment. During the 52‐year measurement time period, an average of 21 000 ± 3100 m3 km?1 a?1 of material was eroded from nine study sections distributed along the coast, with a low yield of 1000 ± 240 m3 km?1 a?1 and a high of 46 700 ± 7300 m3 km?1 a?1. The results compare well with known volumes from several deep‐seated landslides in the area and suggest that the processes by which material is delivered to the coast are episodic in nature. In addition, a number of parameters are investigated to determine what influences the substantial variation in yield along the coast. It is found that the magnitude of regional coastal landslide sediment yield is primarily related to the physical strength of the slope‐forming material. Coastal Highway 1 runs along the lower portion of the slope along this stretch of coastline, and winter storms frequently damage the highway. The California Department of Transportation is responsible for maintaining this scenic highway while minimizing the impacts to the coastal ecosystems that are part of the Monterey Bay National Marine Sanctuary. This study provides environmental managers with critical background data on the volumes of material that historically enter the nearshore from landslides, as well as demonstrating the application of deriving historical digital terrain data to model landscape evolution. Published in 2005 by John Wiley & Sons, Ltd.  相似文献   

14.
Nitrogen (N) and phosphorus (P) dynamics in the Kuparuk River in arctic Alaska were characterized in a 3‐year study using routine samples near the mouth of the river at the Arctic Ocean, synoptic whole‐river surveys, and temporally intense sampling during storms in three headwater basins. The Lower Kuparuk River has low nitrate concentrations (mean [NO3]‐N] = 17 µg l?1 ± 1·6 SE) and dissolved inorganic N (DIN, mean [N] = 31 µg l?1 ± 1·2 SE) compared with rivers in more temperate environments. Organic forms constituted on average 90% of the N exported to the Arctic Ocean, and high ratios of dissolved organic N (DON) to total dissolved N (TDN) concentrations (mean 0·92) likely result from waterlogged soils formed by reduced infiltration due to permafrost and low hydrologic gradients. Annual export of TDN, DON, and particulate N averaged 52 kg km?2, 48 kg km?2, and 4·1 kg km?2 respectively. During snowmelt, the high volume of runoff typically results in the highest nutrient loads of the year, although high discharge during summer storms can result in substantial nutrient loading over short periods of time. Differences in seasonal flow regime (snowmelt versus rain) and storm‐driven variation in discharge appear to be more important for determining nutrient concentrations than is the spatial variation in processes along the transect from headwaters towards the ocean. Both the temporal variation in nitrate:DIN ratios of headwater streams and the spatial variation in nitrate:DIN between larger sub‐basins and smaller headwater catchments is likely controlled by shifts in nitrification and soil anoxia. Copyright © 2008 John Wiley & Sons, Ltd.  相似文献   

15.
Estimates of greenhouse gas evasion from rivers have been refined over the past decades to constrain their role in global carbon cycle processes. However, despite 55% of the human population living in urban areas, urban rivers have had limited attention. We monitored carbon dynamics in an urbanized river (River Kelvin, 331 km2, UK) to explore the drivers of dissolved carbon lateral and vertical export. Over a 2-year sampling period, riverine methane (CH4) and carbon dioxide (CO2) concentrations were consistently oversaturated with respect to atmospheric equilibria, leading to continual degassing to the atmosphere. Carbon stable isotopic compositions (δ13C) indicated that terrestrially derived carbon comprised most of the riverine CH4 and dissolved CO2 (CO2*) load while dissolved inorganic carbon (DIC) from groundwater was the main form of riverine DIC. The dynamics of CH4, CO2*, and DIC in the river were primarily hydrology-controlled, that is, [CH4] and [CO2*] both increased with elevated discharge, total [DIC] decreased with elevated discharge while the proportion of biologically derived DIC increased with increasing discharge. The concentration of dissolved organic carbon (DOC) showed a weak relationship with river hydrology in summer and autumn and was likely influenced by the combined sewer overflows. Carbon emission to the atmosphere is estimated to be 3.10 ± 0.61 kg C·m−2·yr−1 normalized to water surface area, with more than 99% emitted as CO2. Annual carbon loss to the coastal estuary is approximately 4.69 ± 0.70 Gg C yr−1, with annual DIC export approximately double that of DOC. Per unit area, the River Kelvin was a smaller carbon source to the atmosphere than natural rivers/streams but shows elevated fluxes of DIC and DOC under comparable conditions. This research illustrates the role urban systems may have on riverine carbon dynamics and demonstrates the potential tight link between urbanization and riverine carbon export.  相似文献   

16.
The transport and yield of suspended sediment (SS) in catchments all over the world have long been topics of great interest. This paper addresses the scarcity of information on SS delivery and its environmental controls in small catchments, especially in the Atlantic region. Five steep catchments in Gipuzkoa (Basque Country) with areas between 56 and 796 km2 that drain into the Bay of Biscay were continuously monitored for precipitation, discharge and suspended sediment concentration (SSC) in their outlets from 2006 to 2013. Environmental characteristics such as elevation, slope, land‐use, soil depth and erodibility of the lithology were also calculated. The analysis included consideration of uncertainties in the SSC calibration models in the final suspended sediment yield (SSY) estimations. The total delivery of sediments from the catchments into the Bay of Biscay and its standard deviation was 272 200 ± 38 107 t yr.?1, or 151 ± 21 t km?2 yr.?1, and the SSYs ranged from 46 ± 0.48 to 217 ± 106 t km?2 yr.?1. Hydroclimatic variables and catchment areas do not explain the spatial variability found in SSY, whereas land‐use (especially non‐native plantations) and management (human impacts) appear to be the main factors that control this variability. Obtaining long‐term measurements on sediment delivery would allow for the effects of environmental and human induced changes on SS fluxes to be better detected. However, the data provided in this paper offer valuable and quantitative information that will enable decision‐makers to make more informed decisions on land management while considering the effects of the delivery of SS. Copyright © 2016 John Wiley & Sons, Ltd.  相似文献   

17.
This study uses long‐term records of stream chemistry, discharge and air temperature from two neighbouring forested catchments in the southern Appalachians in order to calculate production of dissolved CO2 and dissolved inorganic carbon (DIC). One of the pair of catchments was clear‐felled during the period of the study. The study shows that: (1) areal production rates of both dissolved CO2 and DIC are similar between the two catchments even during and immediately after the period of clear‐felling; (2) flux of total inorganic carbon (dissolved CO2+ DIC) rises dramatically in response to a catchment‐wide acidification event; (3) DIC and dissolved CO2 are dominantly released on the old water portion of the discharge and concentrations peak in the early autumn when flows in the study catchments are at their lowest; (4) total fluvial carbon flux from the clear‐felled catchment is 11·6 t km−2 year−1 and for the control catchment is 11·4 t km−2 year−1. The total inorganic carbon flux represents 69% of the total fluvial carbon flux. The method presented in the study provides a useful way of estimating inorganic carbon flux from a catchment without detailed gas monitoring. The time series of dissolved CO2 at emergence to the stream can also be a proxy for the soil flux of CO2. Copyright © 2005 John Wiley & Sons, Ltd.  相似文献   

18.
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19.
The impact of intensive farming on chemical weathering in the Critical Zone is still an open question. Extensively instrumented and monitored over the last 50 years, the Orgeval Critical Zone Observatory (CZO) in France is an observation site impacted by intensive farming since the 1960s. The Orgeval observatory represents an ideal place to study the response and resilience capability of the Critical Zone under agricultural stress. This paper investigates the chemical composition of different water bodies in two nested catchments of the Orgeval CZO, including rainfall, springs, rivers, and rocks, over one and half hydrological year. We show that elemental and strontium isotopic ratios are powerful to constrain the origin of the elements. The results show that the river chemistry at the outlet of the two nested catchments is dominated by rain inputs (particularly atmospheric dust dissolution) and the chemical weathering of limestone and gypsum. Fertilizer input is clearly visible, although the distinction between gypsum dissolution and fertilizer inputs needs more investigation. The mixtures of water masses inferred from our data are in good agreement with the hydrological context of the watershed, that is, a multilayered aquifer structure. At the main outlet of the CZO, we estimate that the input of ocean‐derived solutes through rainfall represents 7 t km?2 year?1, on the same order of magnitude as the net fertilizer input (10 t km?2 year?1), and that rock weathering releases 50 t km?2 year?1. Including previously published physical erosion rates, we estimate that the total denudation rate (physical and chemical) of the Orgeval CZO is 20 mm (1,000 year)?1, which, along with the entire Seine watershed, is among the lowest chemical denudation rates for carbonate terrains under temperate climate. Chemical denudation is about 10 times higher than physical erosion in the Orgeval CZO. The consumption of CO2 by rock weathering is estimated to be between 265.103 and 360.103 molC km2 year?1, similar for the two nested catchments. Compared with the rivers, the springs show a higher CO2 consumption rate that suggests, as pointed out earlier, a enhancement of carbonate dissolution linked to nitrification and thus fertilizer application. The hyporheic zone appears to be a hot spot in the carbon cycle at the Orgeval CZO. This study sheds light on the complex, anthropocenic, interplay between geology, climate, and human activities that characterize and that take place in intensive agriculture regions.  相似文献   

20.
We measured spatial and temporal variations in carbon concentrations, isotopic compositions and exports during a complete hydrological cycle in nine watercourses draining a lowland forested podzolized catchment, flowing into the Arcachon lagoon (France). In addition, integrated fluxes of CO2 across the water-atmosphere interface were estimated to assess the relative importance of CO2 evasion versus lateral carbon transport at the catchment scale. Watercourse similarities and specificities linked to the local catchment characteristics are discussed and compared with other riverine systems. Low concentrations of suspended particulate matter and particulate organic carbon (POC) were generally measured in all the watercourses (8.4 ± 3.4 and 1.6 ± 0.6 mg L?1, respectively), reflecting limited mechanical soil erosion. The generally high POC content in the suspended matter (20 %), low Chl a concentrations (1.3 ± 1.4 μg L?1) and the relatively constant δ13C-POC value (near ?28 ‰) throughout the year reveal this POC originates from terrestrial C3 plant and soil detritus. The presence of podzols leads to high levels of dissolved organic carbon (DOC; 6.6 ± 2.2 mg L?1). Similarly, high dissolved inorganic carbon (DIC) concentrations were measured in the Arcachon lagoon catchment (5.9 ± 2.2 mg L?1). The δ13C-DIC value around ?20 ‰ throughout the year in many small watercourses reveals the predominance of terrestrial carbon mineralisation and silicate rock weathering in soils as the major DIC source. With pCO2 between 1,000 and 10,000 ppmv, all watercourses were a source of CO2 to the atmosphere, particularly during the low river stage. Organic carbon parameters remained relatively stable throughout the year, whereas DIC parameters showed strong seasonal contrasts closely linked to the hydrological regime and hyporheic flows. In total, the carbon export from the Arcachon watershed was estimated at 15,870 t C year?1 or 6 t C km?2 year?1, mostly exported to the lagoon as DOC (35 %), DIC (24 %) and lost as CO2 degassing to the atmosphere (34 %).  相似文献   

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