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1.
Vertical profiles of210Pb and230Th in the deep water were analyzed by using a simple one-dimensional model. Both nuclides are considered to settle down with the velocity of 1×10–4 cm/sec. The diameter of particle corresponding to the velocity is calculated to be 5, while only about 10 % of the nuclides can be collected on filter paper with a pore size of 0.5. It is supposed that the nuclides exist in particulate materials which is changeable in size. This suggestion is supported from the following evidences. (1) The directly observed behavior of marine snow and the size distribution of particles observed with a coulter counter. (2) The existence of many chemical elements of which residence time is about 150 years. (3) Their possible existence as eutectic solid phases in the seawater. (4) The consistency of the observed accumulation rate of pelagic sediments with that estimated from the settling velocity. (5) The consistency of the decomposition rate of organic matter in the deep water estimated from the oxygen comsumption with that from the settling velocity.  相似文献   

2.
Sediment trap experiments were carried out in two oceans, the eastern Pacific Ocean and the Antarctic Ocean, which have very different biological productivities. The natural radionuclides,234Th,210Po and210Pb were used as tracers of reactive metals. Larger particulate fluxes of these radionuclides were found in the seas where total mass fluxes were larger, although the concentrations of these radionuclides in the settling particles were somewhat smaller. The concentrations of234Th in the settling particles varied widely and irregularly with depth, whereas the concentrations of210Po and210Pb in the settling particles steadily increased with increasing water depth. The ratios of210Po/210Pb in the settling particulates were larger than unity which the ratio of234Th/excess210Po as larger than234Th/210Po in the deep water. These results suggest that, when the particles sink through the water column, these radionuclides are being absorbed by settling particles in the order234Th>210Po>210Pb. The observed particulate fluxes of210Pb are about one eighth of those calculated from the disequilibria between226Ra and210Pb at the stations in the subtropical eastern Pacific, although the observed fluxes are the same as the calculated ones in the northern North Pacific and the Antarctic Ocean. Thus, there must be a horizontal flow carrying these reactive metals from the oligotorophic ocean to the biologically productive ocean where the metals are removed by settling particles even in deep water.  相似文献   

3.
This article summarizes the author's work on210Pb and210Po distributions in the marine environment for which the Okada Prize of the Oceanographical Society of Japan was awarded. In this review, the work of other investigators and the studies now going on are also included. The210Pb concentration in the surface water of the ocean is controlled by the atmospheric flux of210Pb and productivity. The disequilibrium between226Ra and210Pb in the deep sea reveals that the oceanic residence time of lead is less than a hundred years rather than of the order of thousands of years as thought before based on stable lead measurement in ocean water. Particulate removal of210Pb from the water column is likely to be the major cause of the deficiency of210Pb in the water, however more investigations would be needed to clarify the detailed removal mechanism of210Pb. The experiments on particulate flux by using sediment traps will provide an unique opportunity to examine this. 210Pb in excess of226Ra in sediment is useful for geochronology of shallow water sediments and the study on bioturbation rates on the deep sea sediments.  相似文献   

4.
U–Th decay series isotopes, δ18O and Si measurements in the river estuarine waters and sediments of the polluted Hooghly estuary as well as the surface waters of the Bay of Bengal, its high salinity end member, are reported. Dissolved Si indicates that there are probably two mixing regimes, dissolved U behaviour is nonconservative and δ18O behaves conservatively in the overall estuarine region. Isotopes of reactive elements, viz. 234Th and 210Po, are removed from the estuarine waters in <2 days and <1 month, respectively, which is due to high suspended matter (30–301 mg l−1). 228Ra and 226Ra are profusely released into the estuarine waters in the low to mid-salinity regions.As expected, the opposite trend is observed in the case of estuarine sediments and suspended matter. Reactive isotopes of Th, 210Pb and 210Po are enriched, whereas Ra isotopes are depleted with respect to their parent nuclides in the estuarine sediments and suspended matter. 232Th/Al ratio appears well suited to study the distribution and mixing of the bed load sediments of the Ganga–Brahmaputra (G–B) and the Hooghly rivers with those from other rivers on the Bay of Bengal floor.  相似文献   

5.
The stability constants for sulfate, chloride and hydroxide ions with cerium (III) in the solution at ionic strength of 0.67 have been determined by cation exchange method, the values of 1 and 2 for sulfate complexes of cerium being 40±13 and 453±140, respectively and those for chloride complexes being 1.28±0.23 and 0.56±0.076, respectively. The values of 1, 2 and 3 for hydroxide complexes of cerium were (4.5±0.9)×107, (3.3±0.7)×1014 and (1.8±0.7)×1023, respectively.Using the above constants the ratios of individual chemical species of144Ce were calculated in a solution at ionic strength of 0.67 containing sulfate and chloride ions approximately the same as in seawater of 35 %. The result of calculation indicates that the dominant species of144Ce in this solution is Ce(OH)3 0 at pH 8.  相似文献   

6.
The physico-chemical states of artificial radionuclides,90Sr,137Cs and144Ce in seawater were investigated by radiochemical analysis of filtered and unfiltered seawater. The difference of radionuclide concentrations between unfiltered and filtered seawaters was defined as the particulate form radioisotope and its particle ratio was discussed.Practically no particulate90Sr, greater than 0.22 in size, was observed in both coastal and open seawaters, but some of137Cs seemed to be insoluble in some circumstances, especially in coastal waters. A considerable amount of144Ce was found to be particulate.An estimation of the radionuclides in particulate form was made for Kashima-nada seawaters collected in 1970 to 1972, and it was shown that the possible occurrence of particulate radionuclides, greater than 0.22 in size, were 1% or less for90Sr and 6% for137Cs. In the coastal water, 80 % of144Ce were seemed to be in particulate form, but in the open seawater only a few%. The influences of suspended materials to137Cs and144Ce concentration levels in seawater were not negligible and further investigations are desirable.  相似文献   

7.
The downward short- and long-wave radiation fluxes at the sea surface (S, L) were measured aboard the R/VHakuho Maru, University of Tokyo, for the period of 117 days on six cruises from 1981 to 1985 in the western North Pacific near Japan. The upward fluxes of short- and long-wave radiation (S, L) were calculated by Payne's (1972) table and the Stefan-Boltzmann's law, respectively. The sensible and laten heat fluxes (Q h ,Q e ) were also estimated from an aerodynamic bulk method.From April to August, the daily mean value ofS varied with the amplitude of 100200 Wm–2. The value ofS was estimated approximately 6% ofS in all seasons. The difference betweenL andL was so small that the net radiation flux (Q n ) was dominated byS. In addition, the net heat flux at the sea surface was also dominated byS due to small values ofQ h andQ e , and then the ocean was warmed at the rate of 111 Wm–2 in April and 63 Wm–2 in August in the Oyashio Area, and 132 Wm–2 in May and 164 Wm–2 in June in the Kuroshio Area, respectively.From September to March, a remarkable negative correlation between the day to day variation ofS and that ofL was observed except when an intense cold air outbreak occurred. It was found that the correlation was caused by the cloud climatological feature of the western North Pacific in this period.S was not a dominant factor in the net heat flux. The value ofQ h +Q e in the Kuroshio Area ranged from 260 Wm–2 to 630 Wm–2, much larger thanQ n which ranged from –8 Wm–2 to 92 Wm–2 in the leg mean values (each leg period was about 10 days). Then the ocean was cooled at the rate of –160–620 Wm–2 during this period. The net heat flux in the Kuroshio Area averaged over five legs from late November to February was –473 Wm–2. This value is 50100% larger than the climatological values reported so far.The temporal and spatial variability of radiation fluxes and heat fluxes during each leg was also discussed.  相似文献   

8.
A new set of empirical formulas for the production rate and the number concentration of sea-water droplets on the sea surface are proposed, synthesizing past observation data of sea-salt particles in the sea and water droplets in wind-wave tanks. A new levelz c is introduced as the effective wind-sea surface where seawater droplets are produced. The new formulas are expressed in linear functions in logarithmic scales ofu*2/v p , a parameter to describe overall conditions of airsea boundary processes, whereu * is the friction velocity of air,v the kinematic viscosity of air and p the peak angular frequency of wind-wave part of wave spectra. A model of coexistence of spray droplets and suspended particles near the sea surface is proposed. As for the independent parameter, a comparison between the uses ofu*2/v p and ofu * 3 which was the traditional way of parameterization excluding wave measure, shows that the advantage of usingu*2/v p is statistically significant with a confidence limit 89% in F-test.  相似文献   

9.
The plot of210Pb activity against depth in carbonate sands on the Virgin Island Bank is a negative asymmetric hyperbolic curve. As depth increases, an initial rapid decrease in210Pb activity caused by the decay of unsupported210Pb and226Ra is followed by increasing activity as a result of210Pb achieving equilibrium with ingrowing230Th. As this curve is time dependent, an estimate of the relative ages in carbonate sequences and the rates of net carbonate accumulation can be made. The ease of210Pb activity determinations makes this procedure an attractive method in obtaining carbonate sand accumulation rates.  相似文献   

10.
Microbial mats were collected from a variety of sites near hydrocarbon vents along the slope in the northern Gulf of Mexico and, for comparison, from Warm Mineral Springs, Florida, USA. A predominant microorganism in each of the mats was the giant bacterium,Beggiatoa. Diameters of the bacterial filaments ranged from about 6 µm to approximately 200 µm. The latter organisms are the largest prokaryotic organisms yet found. All filaments over about 10 µm in diameter contained a large central vacuole, producing a cell with the cytoplasm as a cylindrical tube underlying the cytoplasmic membrane. Sulfur globules were confined to this peripheral layer. Push cores often contained pyrite tubules whose appearance is suggestive of aBeggiatoa origin. Determinations of 13C inBeggiatoa mats from vents along the Louisiana slope yielded values in the range of –26.6 to –27.9 (PDB), suggesting an unusually high degree of isotope fractionation (–24.9) relative to the carbon source in the ambient seawater, which is typical of sulfur-oxidizing chemoautotrophs. The presence of SO (elemental sulfur) within cells ofBeggiatoa resulting from oxidation of H2S supports the importance of bacterial sulfate reduction processes in the underlying vents for the sustenance of theBeggiatoa mats.  相似文献   

11.
Some experiments were carried out to explain thein situ phenomena that the number of coliform organisms decreased rapidly from estuaries to offshore, and also at deeper layer, and that the appearance of coliform types varied.In natural seawater, experimental results did not show thatEscherichia coli was extinct by self-purification or anti-biosis action of seawater, but it showed that this organism decreased mainly because of their starvation caused by lack of nourishment. Although the decreasing rate of bacterial density was delayed in enriched seawater, addition of nutrient even at the time of bacterial extinction promoted the appearance of variated form of this bacteria with floc formation.Flocculation of bacterial cells was influenced by quality and quantity of added nutrients. Temperature was shown to have an effect on the floc formation, but appearance of variated form in flocculated cells ofE. coli was not affected by temperature. Flocculated particles of coliform bacteria were adsorbed on suspended particles in seawater and precipitated rapidly. This phenomenon seems to be a cause of the rapid disappearance of coliform bacteria in coastal waters.In bottom deposits the coliform bacteria probably survive longer as physiologically variated forms when suitable nutrients were supplied.  相似文献   

12.
Stability constants were determined for60Co (II)-amino acid complexes in sodium perchlorate media at an ionic strength=0.67, using cation exchange resins. Stability constants were, for Co(II)-phenylalanine, log 1=4.4, log 2=8.2, log 3=11.7, for Co(II)-histidine, log 1=7.4. for Co(II)-valine, log 1=4.3, log 2=8.5, for Co(II)-proline, log 1=4.1, and for Co(II)-tyrosine, log 1=7.2, respectively. The abundance of Co(II)-amino acid complexes in seawater was calculated from these stability constants on the basis of chemical equilibrium, assuming the concentration of individual amino acid to be 10–7 to 10–8 mol l–1. It was inferred that the Co(II)-amino acid complexes are probably not formed abundantly in seawater while inorganic species of60Co(II) may still be dominant for a short period of time after discharge into seawater as liquid waste.  相似文献   

13.
The selectivity of amino acid assimilation by marine bacteria was examined using seven kinds of14C-amino acids and the acid hydrolysate of14C-labelled proteins. It was found that the net assimilation and respiration by marine bacteria followed MICHAELIS-MENTEN kinetics for all of amino acids used in our experiments. Maximum velocities of amino acids were 0.01 to 0.19g carbon/hour per 2×107 cells for net assimilation and less than 0.18g carbon/hour per 2×107 cells for respiration at 20C. The velocity of gross assimilation was found with the following order: phenylalanine>valine, glutamic acid>serine, arginine>tryptophan>glycine. The assimilation velocities of amino acids in these laboratory works showed almost the same order as those in field experiments. The assimilation velocity of an amino acid was influenced by coexisting another amino acids or glucose. The assimilation velocity in lower substrate range of amino acids was directly proportional to the number of bacterial cells in the range from 6×102 to 3×104 cells per ml. No linear relation between the assimilation velocity of amino acids and reciprocal of absolute temperature was found, but a marked bending was observed at 15 to 20C. The velocity at the optimum temperature was three to six times of that at 5C.  相似文献   

14.
Local balance in the air-sea boundary processes   总被引：2，自引：0，他引：2  
A combination of the three-second power law, presented in part I for wind waves of simple spectrum, and the similarity of the spectral form of wind waves, leads to a new concept on the energy spectrum of wind waves. It is well substantiated by data from a wind-wave tunnel experiment.In the gravity wave range, the gross form of the high frequency side of the spectrum is proportional tog u * –4, whereg represents the acceleration of gravity,u * the friction velocity, the angular frequency, and the factor of proportionality is 2.0×l0–2. The wind waves grow in such a way that the spectrum slides up, keeping its similar form, along the line of the gross form, on the logarithmic diagram of the spectral density,, versus. Also, the terminal value of, at the peak frequency of the fully developed sea, is along a line of the gradient ofg 2 –5.The fine structure of the spectrum from the wind-wave tunnel experiment shows a characteristic form oscillating around the –4-line. The excess of the energy density concentrates around the peak frequency and the second- and the third-order harmonics, and the deficit occurs in the middle of these frequencies. This form of the fine structure is always similar in the gravity wave range, in purely controlled conditions such as in a wind-wave tunnel. Moving averages of these spectra tend very close to the form proportional to –5.As the wave number becomes large, the effect of surface tension is incorporated, and the –4-line in the gravity wave range gradually continues to a –8/3-line in the capillary wave range, in accordance with the wind-wave tunnel data. Likewise, the –5-line gradually continues to a –7/3-line.Also, through a discussion on these results, is suggested the existence of a kind of general similarity in the structure of wind wave field.  相似文献   

15.
Dependences have been determined which connect the parameters of the dispersion relation of the lowest mode of internal waves with the integral characteristics of the seasonal thermocline when 10 min30 min, 20 mh150 m, and 0·4 m2/s2 Q5·2 m2/s2.Translated by Mikhail M. Trufanov.  相似文献   

16.
The chemical states of iron in near-shore and deep-sea sediments were investigated by means of57Fe Mössbauer spectroscopy in combination with selective and nonselective chemical leachings. As far as a limited number of the sediments analyzed are concerned, Mössbauer spectra of near-shore sediments consist of high-spin paramgnetic ferrous (=1.13 mm/s, Eq=2.65 mm/s) and paramagnetic ferric (=0.35 mm/s, Eq=0.64 mm/s) components, while those of deep-sea sediments are composed of high-spin paramagnetic ferrous, paramagnetic ferrous, paramagnetic ferric and magnetic ferric (0.4 mm/s,H510 KG) components. The Fe2+/Fe3+ ratios of deepsea sediments are much smaller than those in near-shore sediments, while the total contents of iron in the former are much higher than those in the latter. This is principally due to the high contents of authigenic ferric oxides in deep-sea sediments. Further, in the aluminosilicate fraction, the Fe2+/Fe3+ ratios of deep-sea sediments are also smaller than those of near-shore sediments. This is probably attributed to high contents of clay minerals and authigenic aluminosilicates in deep-sea sediments relative to near-shore ones. The magnetic components in deepsea sediments are attributable to hematite, magnetite and/or maghemite.  相似文献   

17.
Information on the distribution of dissolved Folin phenol active substances (FPAS) such as tannin and lignin in the seawater along the west coast of India is provided. Notable amounts of FPAS (surface concentrations: 80 g/l to 147 g/l and bottom concentrations: 80 g/l to 116 g/l) were detected in the seawater along the coast. The distribution pattern brings about a general depth-wise decrease. A seaward decrease was observed in the southern stations whereas reverse was the case in northern stations. A significant negative correlation was observed between FPAS concentration and dissolved oxygen in sub-surface samples. The appreciable amounts of FPAS detected in the coastal waters indicate the presence of organic matter principally originating from terrestrial (upland and coastal marsh) ecosystems in the marine environment. In this context, they may be used as tracers to determine the fate of coastalborn dissolved organic matter in the ocean and to determine directly the relationship between allochthonous and autochthonous organic matter.  相似文献   

18.
The development process of wind-waves of which spectral peak distributes from 0.6 cps to 9.3 cps will be discussed on the basis of the wind tunnel experiments and of the field observations performed at Lake Biwa. The characteristics of power and slope spectra are here presented. The development process of these wind-waves is characterized by three stages;i.e. initial-wavelets, transition stage and sea-waves. In the wind tunnel experiments, the transition from the stage of the initial-wavelets to the transition stage occurs when the wave spectral peak arrives at the line 6.40×10–4 k –2cm2·sec (wherek is wave number) or when the slope spectral density at the frequencyf max becomes larger than 6.40×10–4 sec. In the stage of sea-waves, the component wave of a wave-spectral peak is steepest in the component waves. And the wave spectral peak develops along the line 1.02×102 f –6 cm2·sec (wheref is the frequency corresponding to the wave numberk) untill it reaches the line 33.3f –4cm2·sec, and thereafter develops along the latter line, which indicates the constant density of slope spectrum. It is suggested that the nonlinearity of wind-waves must become stronger as wind-waves develop. The effective momentum flux ws from the air flow to wind-waves in this stage is evaluated to be about 49% of the total stress 0.  相似文献   

19.
Nitrogen isotope compositions of particulate organic matter and nitrate were analyzed for seawater sampled at five stations at the Alaskan Gyre, Western Subarctic Gyre and East China Sea, focusing on the samples from the surface to 5000 m water to characterize the nitrogen cycling in the subarctic North Pacific Ocean and its marginal sea. The 15N of particulate organic matter showed little agreement with a conceptual closed model that interprets isotopic variation as being caused by isotope discrimination on nitrate utilization. The 15N and 13C of particulate organic matter varied with the water depth. A correlation between isotope compositions and C/N elemental ratio was found generally at all stations, although some irregular data were also found in deep layers. We developed a hypothetical nitrogen balance model based on N2 fixation and denitrification in seawater and attempted to apply it to distinguish nutrient cycling using both 15N-NO3 – and N* variation in seawater. This model was applied to the observed data set of 15N-NO3 – and N* in the North Pacific water and estimated the 15N-NO3 – of primordial nitrate in the North Pacific deep water as 4.8. The North Pacific intermediate water for all stations showed similar 15N-NO3 – and N* values of 6 and –3 µmol/kg, respectively, suggesting a similar nitrogen biogeochemistry. In the East China Sea, analysis showed evidence of water exchange with the North Pacific intermediate water but a significant influence of nitrogen from the river runoff was found in depths shallower than 400 m.  相似文献   

20.
Using climatological atlas data and historical hydrographic data, the relationship between dynamic height anomaly D and acoustic round-trip travel time in the Pacific Ocean is investigated. A tight, linear relation is found in a region centered on the Kuroshio and Kuroshio Extension. In this region, the slopem of the relation is approximately –50 dyn m s–1, about equal to the value expected for first-baroclinicmode response and twice as large as the value form in the Gulf Stream region of the Atlantic Ocean. The value ofm in the Pacific generally increases in magnitude towards the south and with increasing depth to which the integrals for D and are carried. It is changed only slightly by correcting for the temperature and salinity march of the seasons in the surface layer. The Kuroshio region is established as one in which the record of from an inverted echo sounder can be interpreted reliably in terms of D. An inverted echo sounder can also be used in this way in a number of other regions of the Pacific, although the available hydrographic data sets are too sparse to establish their boundaries clearly.  相似文献   

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