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1.
The available observational data on the pollution of tributaries and areas of the Caspian Sea by petroleum hydrocarbons and products are examined. The possible petroleum input from sources in the sea is assessed using up-to-date data of satellite observations of sea surface pollution by oil films. The hydroecological CNPSi-model is applied to studying water pollution processes by petroleum hydrocarbons in ten areas chosen in the Caspian Sea and the subsequent biodegradation of those pollutants. The model calculations of the within-year dynamics of petroleum hydrocarbon concentrations use mean annual observational data on within-year variations in water mediium characteristics (water temperature, light intensity, and transparency), as well as the morphometric parameters of sea areas (the area, mean depth, and water volumes). The characteristics of water exchange between the areas were evaluated using a hydrodynamic model. The model calculations were used to characterize the within-year variations in petroleum hydrocarbon concentrations, the biomasses of petroleum-oxidizing bacteria, the characteristics of their oxidation activity and bioproduction, and the internal fluxes of petroleum hydrocarbons (their input from various sources, horizontal and vertical transport, and biotransformation) in different sea areas. Calculation results were used to compile annual balances for the processes of input and consumption of petroleum hydrocarbons in the chosen and aggregated sea areas.  相似文献   

2.
The conditions of transformations of biogenic substances and the redistribution of their concentrations in the shelf water of Sakhalin Island are studied. Preliminary works have given the results for the water area of La Perouse Strait and Aniva Bay (the Sea of Okhotsk), while this paper gives such results for Tatar Strait (the Sea of Japan). Three electronic instruments of oceanographic studies are applied: an adapted version of Bergen Oceanic Model (for the reconstruction of the space and time distribution of seawater temperature, salinity, and density; the circulation intensity of water masses; and water exchange parameters with nearby water areas and within the strait); GIS “Sakhalin Shelf” (for the reconstruction of annual variations in thermohaline characteristics on a standard grid and horizons of oceanographic stations, and the parameters of the aquatic environment); hydroecological CNPSi-model (for studying the annual dynamics of biogenic element compounds, the biomasses, biohydrochemical activity and bioproduction of microorganisms—bacteria, phytoplankton, and zooplankton, taking part in transformation of biogenic substances and petroleum hydrocarbons, as well as the internal fluxes of biogenic substances governed by the activity of microorganisms and the external load on the marine ecosystem). The results of modeling the spatial transport of biogenic substances through the outer boundaries of Tatar Strait water area and the boundaries of the three areas identified within it are presented and discussed.  相似文献   

3.
Literary data have been used to assess the inflow of petroleum hydrocarbons (with river runoff, precipitation, wastewaters, sea transport, and at ice thawing) into different regions of the White Sea. The hydroecological CNPSi-model was used as an instrument to reproduce the annual dynamics of hydrocarbon concentrations at their parallel inflow and subsequent transformation in the waters of the nine White Sea regions (the bays of Kandalaksha, Onega, Dvina, and Mezen; the Solovetskie Islands; the deep-water part: Bassein, Gorlo, Voronka, and Chupa Bay). The calculations were based on normal annual values of monthly variations of water temperature, light intensity, and transparency, the morphometric parameters of the regions (water areas, mean depths, and water volumes) and water exchange between the regions and with the Barents Sea (calculated by a hydrodynamic model). The calculated concentrations of hydrocarbons, the biomasses and activity characteristics of hydrocarbon-oxidizing bacteria have been analyzed (their values were estimated for the 2-m surface water layer). The results of calculations were used to evaluate hydrocarbon balances for regions and the sea as a whole. The calculations demonstrate the balanced character of hydrocarbon fluxes, the balance discrepancy for the regions being <0.1–16.1%.  相似文献   

4.
The White Sea is a natural analogue of arctic seas. The pollution of the sea by petroleum hydrocarbons is not high now. However, the load on sea ecosystem can increase in the nearest future because of the anticipated industrial development in its watershed, including an increase in oil, coal, and diamond production. The specific features of the nature of arctic marine systems (hydrological, ice, hydrobiological, hydrochemical, and radiation regimes), and the poor knowledge of the conditions of dispersion, transformation, and utilization of petroleum hydrocarbons in such seas make their ecological studies especially important. Petroleum hydrocarbon concentrations in the waters of tributaries and water areas of the White Sea (for 1980–2006 and 1989–2006, respectively) were evaluated using literary and authors’ data. Analysis of the collected materials shows that the majority of petroleum hydrocarbons enter the sea’s water areas with river runoff. Petroleum hydrocarbon concentrations were evaluated in major tributaries of the sea, including the rivers of Northern Dvina, Onega, Mezen, Niva, Kem, and Keret, delivering petroleum hydrocarbons into the bays of Dvina, Onega, Mezen, and Kandalaksha, water area near the Solovetskie Islands, and Chupa Bay, respectively (Bay — Gulf). Model calculations should yield within-year variations in petroleum hydrocarbon concentrations in different part of the sea (under a correctly specified load) and the conditions of their biotransformation and horizontal transport through the boundaries between areas within the sea.  相似文献   

5.
This study has no analogues in terms of methodology, as it uses three electronic instruments for studying the oceanographic regime of Tatar Strait. GIS “Sakhalin Shelf” was used to reconstruct annual variations in hydrological and hydrochemical characteristics of the marine environment at standard horizons of oceanographic stations in fixed geographic coordinates. An adapted version of the Oceanic Model created in Bergen University was used to reconstruct the spatial and temporal distribution of seawater temperature and salinity, to calculate the density and the circulation rate of water masses and water exchange parameters between the strait and nearby water areas and between regions within the strait. The hydroecological CNPSi-model was next used to assess the annual dynamics of concentrations of biogenic element compounds; the biomasses, biohydrochemical activity, and bioproductivity of microorganisms (heterotrophic bacteria, three phytoplankton and two zooplankton groups), involved in transformation of biogenic substances, as well as the internal fluxes of biogenic substances, governed by microorganism activity and the external load onto the marine ecosystem. Analysis of calculation results made it possible to reveal new features in water circulation in the strait (including those for winter) and, for the first time, to analyze the transport regime of biogenic substances through the external boundaries of Tatar Strait and through the boundaries of three regions identified within the strait.  相似文献   

6.
Statistical modeling and GIS “Sakhalin Shelf” are used to restore the annual variations of water temperature and salinity at standard oceanographic stations in Tatar Strait, where observation series are about 45 years long. Numerical modeling techniques with the help of Bergen University model are used to restore the spatial fields of water temperature and salinity. Analysis of calculation results made it possible to identify new features of the hydrological regime in the strait, in particular, during winter, for which no generalizations have been made before.  相似文献   

7.
Variability of dense water formation in the Ross Sea   总被引:1,自引:0,他引:1  
This paper presents results from a model study of the interannual variability of high salinity shelf water (HSSW) properties in the Ross Sea. Salinity and potential temperature of HSSW formed in the western Ross Sea show oscillatory behaviour at periods of 5–6 and 9 years superimposed on long-term fluctuations. While the shorter oscillations are induced by wind variability, variability on the scale of decades appears to be related to air temperature fluctuations. At least part of the strong decrease of HSSW salinities deduced from observations for the period 1963–2000 is shown to be an aliasing artefact due to an undersampling of the periodic signal. While sea ice formation is responsible for the yearly salinity increase that triggers the formation of HSSW, interannual variability of net freezing rates hardly affects changes in the properties of the resulting water mass. Instead, results from model experiments indicate that the interannual variability of dense water characteristics is predominantly controlled by variations in the shelf inflow through a sub-surface salinity and a deep temperature signal. The origin of the variability of inflow characteristics to the Ross Sea continental shelf can be traced into the Amundsen and Bellingshausen Seas. The temperature anomalies are induced at the continental shelf break in the western Bellingshausen Sea by fluctuations of the meridional transport of circumpolar deep water with the eastern cell of the Ross Gyre. In the Amundsen Sea, upwelling due to a persistently cyclonic wind field carries the signal into the surface mixed layer, leading to fluctuations of the vertical heat flux, anomalies of brine release near the sea ice edge, and consequently to a sub-surface salinity anomaly. With the westward flowing coastal current, both the sub-surface salinity and deep temperature signals are advected onto the Ross Sea continental shelf. Convection carries the signal of salinity variability into the deep ocean, where it interacts with modified circumpolar deep water upwelled onto the continental shelf as the second source water mass of HSSW. Sea ice formation on the Ross Sea continental shelf thus drives the vertical propagation of the signal rather than determining the signal itself.  相似文献   

8.
The state of the marine environment (the temperature, light intensity, transparency, biogenic load) in Tatar Strait was assessed based on mean annual data from literary sources and with the use of GIS “Sakhalin Shelf.” The entire strait was divided into three regions (northern, southwestern, and southeastern), and water exchange between them for each month was estimated by using Bergen Oceanic Model. The information about the state of the marine environment and water exchange characteristics was used as input data for a hydroecological model, which enabled the assessment of annual variations of biogenic substance concentrations and biomasses of microorganisms (heterotrophic bacteria, three groups of phytoplankton, and two groups of zooplankton) in the strait regions chosen. The development conditions of microorganism biomasses within the year can be characterized by their activity indices (specific growth rates), the values of internal fluxes of biogenic substances, and calculated bioproductivity values. The calculated biogenic substance concentrations and phytoplankton bioproductivity values showed good agreement with the estimates for the Sea of Japan and Tatar Strait available from the literature.  相似文献   

9.
An igneous intrusion of 94m thick was discovered intruding into the Silurian sandstone from Tazhong 18 Well. The petroleum previously preserved in the Silurian sandstone reservoir was altered into black carbonaceous bitumen by abnormally high heat stress induced by the igneous intrusion. The reflectance of the carbonaceous bitumen reaches as high as 3.54%, indicating that the bitumen had evolved into a high thermal evolution level. Similar to the Silurian samples from the neighboring Tazhong 11, Tazhong 12, Tazhong 45 and Tazhong 47 wells, the distribution of C27, C28 and C29 steranes of the carbonaceous bitumen is still “V”-shaped and can still be employed as an efficient parameter in oil source correlation. The “V”-shaped distribution indicates that the hydrocarbons from the Tazhong 18 and the neighboring wells were all generated from the Middle-Upper Ordovician hydrocarbon source rocks. However, the oil source correlation parameters associated with and terpanes had been changed greatly by the high heat stress and can no longer be used in oil source correlation. The δ 13C values of the petroleum from the neighboring wells are between −32.53%. and −33.37%., coincident with those of the Paleozoic marine petroleum in the Tarim Basin. However, the δ 13C values of the carbonaceous bitumen from the Tazhong 18 Well are between −27.18%. and −29.26%., isotopically much heavier than the petroleum from the neighboring wells. The content of light hydrocarbons (nC14nC20) of the saturated hydrocarbon fraction in the carbonaceous bitumen is extremely higher than the content of heavy hydrocarbons. The light/heavy hydrocarbon ratios (ΣnC21 nC22 + are between 4.56 and 39.17. In the saturated fraction, the even numbered hydrocarbons are predominant to the odd numbered, and the OEP (Odd to Even Predominance) values are between 0.22 and 0.49. However, the content of light hydrocarbons in the petroleum from the neighboring wells is relatively low and the content of the even numbered hydrocarbons is almost equal to that of the odd numbered. Compared with the samples from the neighboring wells, the abundance of non-alkylated aromatic hydrocarbons, such as phenanthrenes, and polycyclic aromatic hydrocarbons (PAHs), such as fluoranthane, pyrene, benzo[a]anthracene and benzofluoranthene, are relatively high. Supported by the National Key Basic Research and Development Project (Grant No. 2005CB422103)  相似文献   

10.
Data of long-term observations of Roshydromet and the studies of the authors’ studies of hydrochemical, hydrobiological, and bioassaying characteristics and appropriate publications in the areas of megalopolises—the cities of Rostov-on-Don and Novosibirsk are analyzed. Similar and distinctive characteristics of water quality by these ecological-toxicological characteristics are identified; trends in the long-term year-to-year variations in water quality are established, criteria and characteristics reflecting the effect of cities on water bodies in their territory are determined. The identity of some chemical-toxicological criteria and the characteristics of the influence of cities in southern Russia and Siberia on water bodies suggest that they can also be used in urban area in other regions. The Lower Don is used as an example to show that water pollution by metals is mostly due to wastewater discharge, while water pollution by petroleum products and sulfates has no direct relation to that.  相似文献   

11.
Nitrate concentrations in streamwater of agricultural catchments often exhibit interannual variations, which are supposed to result from land‐use changes, as well as seasonal variations mainly explained by the effect of hydrological and biogeochemical cycles. In catchments on impervious bedrock, seasonal variations of nitrate concentrations in streamwater are usually characterized by higher nitrate concentrations in winter than in summer. However, intermediate or inverse cycles with higher concentrations in summer are sometimes observed. An experimental study was carried out to assess the mechanisms that determine the seasonal cycles of streamwater nitrate concentrations in intensive agricultural catchments. Temporal and spatial patterns of groundwater concentrations were investigated in two adjacent catchments located in south‐western Brittany (France), characterized by different seasonal variations of streamwater nitrate concentrations. Wells were drilled across the hillslope at depths ranging from 1·5 to 20 m. Dynamics of the water table were monitored and the groundwater nitrate and chloride concentrations were measured weekly over 2 years. Results highlighted that groundwater was partitioned into downslope domains, where denitrification induced lower nitrate concentrations than into mid‐slope and upslope domains. For one catchment, high subsurface flow with high nitrate concentrations during high water periods and active denitrification during low water periods explained the higher streamwater nitrate concentrations in winter than in summer. For the other catchment, the high contribution of groundwater with high nitrate concentrations smoothed or inverted this trend. Increasing bromide/chloride ratio and nitrate concentrations with depth argued for an effect of past agricultural pressure on this catchment. The relative contribution of flows in time and correlatively the spatial origin of waters, function of the depth and the location on the hillslope, and their chemical characteristics control seasonal cycles of streamwater nitrate concentrations and can influence their interannual trends. Copyright © 2004 John Wiley & Sons, Ltd.  相似文献   

12.
As a critical water discharge term in basin‐scale water balance, accurate estimation of evapotranspiration (ET) is therefore important for sustainable water resources management. The understanding of the relationship between ET and groundwater storage change can improve our knowledge on the hydrological cycle in such regions with intensive agricultural land usage. Since the 1960s, the North China Plain (NCP) has experienced groundwater depletion because of overexploitation of groundwater for agriculture and urban development. Using meteorological data from 23 stations, the complementary relationship areal evapotranspiration model is evaluated against estimates of ET derived from regional water balance in the NCP during the period 1993–2008. The discrepancies between calculated ET and that derived by basin water balance indicate seasonal and interannual variations in model parameters. The monthly actual ET variations during the period from 1960 to 2008 are investigated by the calibrated model and then are used to derive groundwater storage change. The estimated actual ET is positively correlated with precipitation, and the general higher ET than precipitation indicates the contributions of groundwater irrigation to the total water supply. The long term decreasing trend in the actual ET can be explained by declining in precipitation, sunshine duration and wind speed. Over the past ~50 years, the calculated average annual water storage change, represented by the difference between actual ET and precipitation, was approximately 36 mm, or 4.8 km3; and the cumulative groundwater storage depletion was approximately 1700 mm, or 220 km3 in the NCP. The significantly groundwater storage depletion conversely affects the seasonal and interannual variations of ET. Irrigation especially during spring cause a marked increase in seasonal ET, whereas the rapid increasing of agricultural coverage over the NCP reduces the annual ET and is the primary control factor of the strong linear relationship between actual and potential ET. Copyright © 2013 John Wiley & Sons, Ltd.  相似文献   

13.
The available observational data on variations of oil hydrocarbon concentrations in White Sea tributaries and in individual parts of the sea are analyzed, and the contributions of different external sources to marine environment pollution are evaluated. The results of calculations are used to determine the possible total input of hydrocarbons from additional potential sources—internal natural (production by microorganisms) and external anthropogenic (navigation and sea shipping), which are most active in the summer and autumn. The hydroecological CNPSi-model is used to reproduce the processes of pollution of nine areas in the White Sea by oil hydrocarbons and their subsequent biodegradation in the marine environment. The annual dynamics of hydrocarbon concentrations was calculated using the long-term annual observations of monthly variations of the temperature, light intensity, and transparency of water, data on the morphometry of sea areas (the squares, mean depths, and water volumes) and water exchange between the chosen areas, calculated by a hydrodynamic model. For large bays (Dvina, Kandalaksha), the calculated concentrations of oil hydrocarbons are shown to be in agreement with the available estimates (the mean and maximal concentrations). The annual variations of oil hydrocarbon concentrations; the biomasses, oxidation activity and bioproduction characteristics of oil hydrocarbon-oxidizing bacteria are characterized. The calculated internal fluxes of oil hydrocarbons (the inputs from different sources, horizontal transport, and biotransformation) were used to calculate their annual balances for individual areas and the sea as a whole, showing the balanced character of their fluxes with the total balance discrepancies for individual areas varying within 0.3–4.1%.  相似文献   

14.
Sea level trends and interannual variability at Antalya and Menteş tide gauges are investigated during the 1985–2001 period, quantifying the roles of atmospheric, steric and local land motion contributions. Tide gauge sea level measurements, temperature/salinity climatologies and GPS data are used in the analyses and the results are compared with the output of a barotropic model forced by atmospheric pressure and wind. The overall sea level trends at two tide gauges collocated with GPS are in the range of 5.5 to 7.9 mm/yr during the study period, but showing different behaviour in the sub-periods 1985–1993 and 1993–2001 due to variations in the contributing factors both in space and time. After the removal of the atmospheric forcing and steric contribution from sea level records, the resulting trends vary between 1.9 to 4.5 mm/yr in Antalya and −1.2 to −11.6 mm/yr in Menteş depending on the period considered. Vertical land movement estimated from GPS data seems to explain the high positive residual trend in Antalya during the whole period. On the other hand, the source of the highly negative sea level trend of about −14 mm/yr in Menteş during 1985–1993 could not be resolved with the available datasets. Interannual variability of wind and atmospheric pressure appear to dominate the sea level at both tide gauges during the study period. Atmospheric and steric contributions together account for ∼50% of the total sea level variance at interannual time scales. Mass induced sea level variations which were not considered in this study may help to close the sea level trend budgets as well as to better explain the interannual sea level variance.  相似文献   

15.
The article gives the results of studying the concentration and composition of aliphatic and polycyclic aromatic hydrocarbons in suspension in surface waters at sections from the English Channel and Skagerak Strait to various regions of the Baltic Sea (2010–2015) and in water and bottom sediments of the southeastern part of the sea in the water area of the Kravtsovskoe field (2008–2015). In recent years, the surface waters of open areas of the Baltic Sea showed a decrease in hydrocarbon concentrations down to background levels (12–33 μg/L). The maximal concentration of hydrocarbons (in excess of the MAC) was recorded in different seasons in navigation areas, including the English Channel and Pregola R. mouth. In the zone of the Kravtsovskoe field, the concentration and composition of hydrocarbons in water depends on their inflow from the bank, and the same characteristics in bottom sediments, on the rate of their leakage from sediment stratum. A decline in these processes have led to a decrease in hydrocarbon concentrations in the sediments of a local area near D-6 platform to background levels (5–7 μg/g) and to the predominance of terrigenous, rather than petroleum, alkanes in hydrocarbon compositions.  相似文献   

16.
The levels of selected organic markers, including 17 polycyclic aromatic hydrocarbons (PAHs), 16 of which are classified as priority pollutants by the US-EPA and perylene, aliphatic hydrocarbons (total and linear alkanes) and petroleum biomarkers (hopanes and steranes), were measured in suspended particulate matter (SPM) of the Mundaú-Manguaba estuarine-lagoon system (MMELS) in northeastern Brazil and the Paraíba do Sul River (PSR) estuary in southeastern Brazil, both of which are affected by sugarcane agriculture and urbanization. A total of 33 surface water samples of SPM were collected (22 from the MMELS and 11 from the PSR). The ∑16PAH ranged from 221 to 1243 ng g−1 in the MMELS and from 228 to 1814 ng g−1 in the PSR. Hopane and sterane concentrations in the PSR were higher than in the MMELS due to the input from petrogenic sources in PSR. The contributions of higher plants were also observed by n-alkane analyses. The PAH isomeric ratios indicated that the SPM from MMELS showed characteristics of combustion from biomass or petroleum and PSR was associated to petrogenic input, either from combustion or from unburned petroleum. Three sampling sites located near to the sugarcane plant and mouth of the rivers showed higher PAH concentrations and may largely be considered as highly contaminated. However, levels of n-alkanes and petroleum biomarkers in both study areas were relatively low.  相似文献   

17.
Soil moisture is an important driver of growth in boreal Alaska, but estimating soil hydraulic parameters can be challenging in this data-sparse region. Parameter estimation is further complicated in regions with rapidly warming climate, where there is a need to minimize model error dependence on interannual climate variations. To better identify soil hydraulic parameters and quantify energy and water balance and soil moisture dynamics, we applied the physically based, one-dimensional ecohydrological Simultaneous Heat and Water (SHAW) model, loosely coupled with the Geophysical Institute of Permafrost Laboratory (GIPL) model, to an upland deciduous forest stand in interior Alaska over a 13-year period. Using a Generalized Likelihood Uncertainty Estimation parameterisation, SHAW reproduced interannual and vertical spatial variability of soil moisture during a five-year validation period quite well, with root mean squared error (RMSE) of volumetric water content at 0.5 m as low as 0.020 cm3/cm3. Many parameter sets reproduced reasonable soil moisture dynamics, suggesting considerable equifinality. Model performance generally declined in the eight-year validation period, indicating some overfitting and demonstrating the importance of interannual variability in model evaluation. We compared the performance of parameter sets selected based on traditional performance measures such as the RMSE that minimize error in soil moisture simulation, with one that is designed to minimize the dependence of model error on interannual climate variability using a new diagnostic approach we call CSMP, which stands for Climate Sensitivity of Model Performance. Use of the CSMP approach moderately decreases traditional model performance but may be more suitable for climate change applications, for which it is important that model error is independent from climate variability. These findings illustrate (1) that the SHAW model, coupled with GIPL, can adequately simulate soil moisture dynamics in this boreal deciduous region, (2) the importance of interannual variability in model parameterisation, and (3) a novel objective function for parameter selection to improve applicability in non-stationary climates.  相似文献   

18.
 Volcanic lakes have a wide range of characteristics, and we make an attempt to delineate the limiting physical conditions for several lake classes. The ratio between heat input and heat dissipation capacity of a lake constrains the temperature for perfectly mixed steady-state volcanic lakes. Poorly mixed lakes are also conditioned by this ratio, but their temperature structure is also strongly influenced by the hydrodynamics resulting from different mechanisms of heat transfer. The steady-state temperatures of volcanic lakes are largely determined by the magnitude of the volcanic heat influx relative to the surface area of the lake. Small lakes have only a small capacity for heat dissipation and their temperature rises quickly with only small heat inputs; large lakes are buffered against variations in heat input. Both the heat dissipation and meteoric water input into a lake are functions of lake surface area and therefore each lake water temperature demands a certain precipitation rate for mass conservation, independent of lake size. The results of energy/mass-balance modeling shows that under common atmospheric conditions, most steady-state volcanic lakes are unlikely to maintain a temperature in excess of 45–50  °C. Validation of the volcanic lake model was performed using published data from Yugama Lake (Japan) and the Keli Mutu lakes (Indonesia). Also, the model was applied to 24 natural systems to provide a baseline assessment of energy fluxes under the model assumptions so future work on those systems can identify nuances in individual systems that deviate from the simple model conditions. We recommend the model for use in assessing temperature variations and volcanic lake stability in settings with known physical and atmospheric conditions. Application of the energy/mass balance calculations of model lakes provides a genetic classification scheme largely based on physical process parameters. Received: 28 February 1996 / Accepted: 23 November 1996  相似文献   

19.
Bioconcentration factors (Kbc) for petroleum hydrocarbons, PAHs, LABs and biogenic hydrocarbons in Mytilus edulis were measured in field experiments using time-integrating water samplers. Seven deployments at five sites gave lipid weight Kbcs for total hydrocarbons ranging from 0.99 × 106 to 3.1 × 106 (mean 1.6 × 106)—a narrower range than has been obtained previously. Bioconcentration factors for the PAHs were similar to those for total hydrocarbons where the major hydrocarbon source was oil. However, at other sites the factors for PAHs were an order of magnitude lower than those for petroleum and for hydrocarbons originating from algae. Compositional profiles for the linear alkyl benzenes (LABs) suggested that these compounds were assimilated primarily from the dissolved phase, despite their greater abundance on particles.  相似文献   

20.
The natural surface films in the Eastern Mediterranean appear to be badly polluted with petroleum hydrocarbons, and sub-surface oil/water emulsions are also important contributors to the interface chemistry in certain areas. High levels of non-natural hydrocarbons are present in the lipids of some near-surface zooplankton from this regions, suggesting that these animals store and concentrate the pollutant hydrocarbons.  相似文献   

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