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1.
This paper presents the results of the studies of aerosol optical properties measured using lidars and sun photometers. We describe two case studies of the combined measurements made in two coastal zones in Crete in 2006 and in Rozewie on the Baltic Sea in 2009. The combination of lidar and sun photometer measurements provides comprehensive information on both the total aerosol optical thickness in the entire atmosphere as well as the vertical structure of aerosol optical properties. Combination of such information with air mass back-trajectories and data collected at stations located on the route of air masses provides complete picture of the aerosol variations in the study area both vertically and horizontally. We show that such combined studies are especially important in the coastal areas where depending on air mass advection directions and altitudes the influence of fine or coarse mode (in this case possibly sea-salt) particles on the vertical structure of aerosol optical properties is an important issue to consider.  相似文献   

2.
Agriculture crop residue burning in tropics is an important source of atmospheric aerosols and monitoring their long-range transport is an important element in climate change studies. Synchronous measurements using micro-pulsed lidar, MICROTOPS-II sun photometer, multi-filter rotating shadow band radiometer (MFRSR) on aerosol optical depth and ground reaching solar irradiance were carried at an urban location in central region of India. Aerosol backscatter profiles obtained from micro-pulse lidar showed elevated aerosol layers up to ～3 km on certain days during October 2007. Satellite data observations on aerosol properties suggested transport of particles from agriculture crop residue burning in Indo-Gangetic Plains over large regions. Radiative forcing of aerosols estimated from SBDART model with input information on aerosol chemical properties, aerosol optical depth and single scattering albedo and broadband solar irradiance measurements using MFRSR showed good correlation (R=0.98).  相似文献   

3.
This paper presents the measurements of a vertical structure of aerosol optical properties performed during the MACRON (Maritime Aerosol, Clouds and Radiation Observation in Norway) campaign, which took place in July and August 2007 at ALOMAR observatory on Andøya island (69.279°N, 16.009°E, elevation 380 m a.s.l.). The mean value of the aerosol optical thickness (AOT) at 500 nm during campaign was 0.12. Significant increase of the AOT above longtime mean value was observed on 7 and 8 August 2007 when the AOT exceeded 0.4 at 500 nm. Analyses of back trajectories show the aerosol transported from over Africa and Central Europe. The aerosol extinction coefficient obtained from the synergy of ceilometer and sun photometer observations reached 0.05–0.08 km?1 (at 1064 nm) in the dust layer. The single scattering albedo at the ALOMAR observatory decreased during the dust episode to 0.93–0.94, which indicates some absorptive aerosols in the lower PBL.  相似文献   

4.
Error analysis of multi-wavelength sun photometry   总被引：6，自引：0，他引：6  
The error terms involved in precision multi-wavelength sun photometry, as used to study atmospheric aerosols, are analyzed. The error terms treated include instrumental errors, calibration errors, and errors imposed by the atmosphere. It is shown that in order to derive accurate aerosol parameters, one must exercise great care in the photometer calibration. A procedure for accurate calibration is described, based on an intercalibration between extrapolations of the extraterrestrial solar spectral irradiance and irradiance of a standard lamp. Methods are described to assess, and reduce, uncertainties brought about by diffuse radiation in the photometer's field of view, temporal variations in aerosol optical depth, and gaseous absorption features at the operating wavelength. It is shown that if care is taken sun photometry can be used to derive monochromatic aerosol optical depth to an accuracy of several thousandths.  相似文献   

5.

In this paper we have analyzed aerosol distribution over the Tibetan Plateau by using the global monthly mean satellite data of Stratospheric Aerosol and Gas Experiment II (SAGE II). The results are as follows: (1) Stratospheric aerosol optical depth can oscillate in the four seasons. It means that the aerosol optical depth is the thickest in winter and a little thinner in spring and the thinnest in summer and then a little thicker in autumn. We have found that the oscillation is caused by the oscillation of tropopause in different seasons. (2) Stratospheric aerosol comes mainly from sprays of volcano. After eruption of Mount Pinatubo aerosol optical depth in stratosphere over the Tibetan Plateau increases 10 times compared with before. (3) The characteristic of aerosol vertical distribution over the Tibetan Plateau is that there is an extremely high value at the altitude of 70 hPa. The most interesting thing is that the extremely high value can oscillate between 50 hPa and 100 hPa. We have verified that the oscillation is a unique characteristic over the Tibetan Plateau by comparing it with South China and North China. Then the radiative forcing and regional climate response over the Tibetan Plateau of aerosol are investigated. We have discovered such things as followed by: (1) The radiative forcing is positive because the parameterized aerosol optical depth is less than 0.14 which is the optical depth of the uniform background boundary aerosol layer. It is 0–3 W/m2 in January and 0–4 W/m2 in April and less than 3 W/m2 in July and 3–6 W/m2 in October. (2) Ground temperature rises 0.1–0.2 K in October which is the biggest increasing magnitude, and 0.01–0.02 in July which is the smallest one. It rises about 0.05-0.01 K in January and April. (3) Air temperature near the earth’s surface and the one at the altitude of 500 hPa rise too, but the increasing magnitude is less than the former one.

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6.
Summary The phenomenon of the green flash at sunset (or sunrise) is reviewed. Several possible mechanisms that have been put forth to explain the green flash are discussed. A quantitative model for the phenomenon is then described, which includes parameters that are representative for a polar atmosphere (low humidity and small aerosol optical depth). It is supposed that the primary mechanism responsible for causing the green flash are natural molecular disperion, and, the filtering action imposed by the atmosphere for low elevation angles. Results from the model indicate that a green rim of vertical extent 0.15 milliradians would appear at the upper limb of the sun during sunset or sunrise. The theoretical results are compared with observations of a green flash made at wintertime in interior Alaska.  相似文献   

7.
Aerosol particle size distribution and chemical properties are important in studies related to human health and climate. The present study describes an analysis of aerosol mass loading, Aerosol Optical Depth (AOD), black carbon aerosol mass concentration and carbon monoxide over tropical urban region of Hyderabad, India, during March 2006, coinciding with active forest fires season over India. Aerosol optical depth, particulate matter mass loading and carbon monoxide were observed to be high on days with air mass coming from north of the study area. Spatial occurrence of forest fires was analysed using MODIS daytime data and DMSP-OLS nighttime data sets. Aerosol optical depth measured using Microtops-II sunphotometer correlated well with MODIS derived AOD values. Results of the study suggested that synoptic meteorological conditions play an important role in the observed aerosol properties over the study area during the forest fire season.  相似文献   

8.
In this paper, optical measurements of aerosol properties made during a ship cruise from Poland to Antarctic Station in September and October 2006, and during the cruise back to Gdynia in April and May 2007 are described. A large gradient of pollution between the clear South Atlantic and the dusty North Atlantic was observed. The maximum of aerosol optical thickness at a wavelength of 500 nm reached 0.4 at 20°N in September 2006 and 0.3 at 40°N in May 2007, respectively. Strong Saharan dust transport is suggested as an explanation for the small values of Ångström exponent observed (values of 0.2 and 0.4 on these respective dates). On the Southern Hemisphere the aerosol optical thickness at 500 nm ranged from 0.05 to 0.2. Significant increases of the aerosol optical thickness were associated with strong wind and sea salt production. Good agreement was found when the in situ measurements of aerosol optical thickness were compared to satellite retrievals and modelling results.  相似文献   

9.
Reflectance measurements of both the visible and infrared bands of passive remote sensing sensors are widely used to retrieve aerosol optical depth(AOD) information. This is performed commonly for data obtained over both ocean and land, and these measurements allow for the off line development of a lookup table using radiative transfer models. Owing to molecular and aerosol effects, the reflected light received by the sensor is usually highly polarized. The linear polarization effect may be up to 100%, and the polarization factor of a sensor optical system will change the total intensity as well as the polarization status of the signal reaching the detector. The detector response will be different when the incident light polarization status changes, even if the total intensity remains constant. However, if the polarization calibration is neglected, it will cause obvious errors in the aerosol data retrieval. This is especially true for aerosol optical depth retrieval over an ocean. This measurement relies directly on the reflectance output of the sensor. Cases involving land surfaces are not discussed herein because the inhomogeneous properties conceal the error due to polarization. Taking the 550 and 860 nm bands as examples, the difference between the real top-of-atmosphere(TOA) reflectance and the reflectance reaching the detector is calculated using three different sensor polarization standards according to the Sea-viewing Wide Field-of-view Sensor(Sea Wi FS) and Moderate Resolution Imaging Spectroradiometer(MODIS) standards. The differences in AOD retrieval are also demonstrated using the lookup table developed previously from a vector radiative transfer code. The results reveal that under a normal situation in which the AOD is 0.15, the maximum AOD retrieval error could reach 0.04 in 550 nm but only 0.02 in 860 nm for the dust aerosol model. For the soot aerosol model, the maximum AOD retrieval error is 0.1 in 550 nm and 0.12 in 860 nm, indicating that the lack of polarization calibration will lead to large errors in aerosol retrieval over an ocean.  相似文献   

10.
A joint United States/Russian/French collaborative experiment was undertaken in March 1993 and March 1996. Projects LODE I and II (Lake Owens Dust Experiments) took place on the anthropogenically desertified playa (dry lakebed) and surrounding regions of Owens Lake, in east-central California. One of the five parts of Project LODE was to determine relationships between optical depth and flux of dust emitted from the dry lake. Project LODE II included subsequent dust plume measurements and size distributions obtained through April 1996, to further refine the flux measurements for distinct mineral aerosol source regions at Owens Lake. Size distributions of dust aerosol were determined and aerosol optical depths were calculated from sunphotometer solar extinction measurements taken downwind in plumes coming from the emissive areas of Owens Lake. This source was visually observed for 10 measured dust storms. The plume mass was calculated to be 1·5 × 109 g using ground-based measurements and ≥1·6 × 109 g from satellite data. Project LODE II results were found to be consistent with LODE I results for the south end of the playa, but flux values were found to be reduced for the northeastern portion of the playa by comparison. Vertical flux values estimated by sunphotometry were found to be consistent with values estimated via a micrometeorological method. Copyright © 1999 John Wiley & Sons, Ltd.  相似文献   

11.
An algorithm based on simulated satellite signal calculated by the 6S radiative transfer model has been developed in order to retrieve the aerosol optical thickness of dust over the Atlantic ocean. The algorithm is applied to the visible channel of Geostationary Operational Environmental Satellite (GOES 8) images. The inversion uses a look-up table giving the satellite signal intensity as a function of surface albedo, viewing geometry, solar illumination and the optical properties of the aerosols. The study consists of assessing the feasibility of monitoring and mapping the transport of suspended particles across the Atlantic from the Sahara to the Caribbean. The study area is between 10 and 25 N and 30 and 65 W. The optical thickness of aerosols has been calculated over a period of 11 days between 10th and 20th of June 1997 for the 14:15 UT GOES image acquisition. The calculated aerosol optical thickness ranges from 0.0 to 0.81 with an important event of dust presence occurring between 13th and 16th of June. The retrieved aerosol optical thickness is in good agreement with the values obtained between 14h UT and 15h UT from ground based sun photometer measurements on the island of Guadeloupe, and a coefficient correlation (R2) of 0.88 has been found between the data sets.  相似文献   

12.
Six years of spectral aerosol optical depth (AOD) measurements have been analyzed from a tropical coastal site, Trivandrum (8.55°N, 76.9°E, 3 m msl) to infer on the seasonal changes in the microphysical properties of columnar aerosols, by examining the derivatives of the Angstrom wavelength exponent (α) in the wavelength domain (α′λ) as well as in AOD domain (α′τ) and by retrieving the columnar size distribution by numerical inversion of the AODs. The inference of the changes in the aerosol microphysics drawn from the features of the derivatives α′λ and α′τ is consistent with the pattern revealed by the aerosol properties obtained from the columnar size distributions retrieved from the AOD spectra as well as from the surface measurements of mass-size distributions, which are supported by the back-trajectory cluster analysis and the results of chemical species analysis.  相似文献   

13.
We examine the impact of the Atmospheric Brown Clouds on the direct radiative forcing of the Himalayan foothills and the Indo-Gangetic Plains (IGP) regions, home for over 500 million S. Asians. The NASA-Terra MODIS satellite data reveal an extensive layer of aerosols covering the entire IGP and Himalayan foothills region with seasonal mean AODs of about 0.4 to 0.5 in the visible wavelengths (0.55 micron), which fall among the largest seasonal mean dry season AODs for the tropics. We show new surface data which reveal the presence of strongly absorbing aerosols that lead to a large reduction in solar radiation fluxes at the surface during the October to May period. The three-year mean (2001 to 2003) October to May seasonal and diurnal average reduction in surface solar radiation for the IGP region is about 32 (±5) W m−2 (about 10% of TOA insolation or 20% of surface insolation). The forcing efficiency (forcing per unit optical depth) is as large as −27% (note that the forcing is negative) of top-of-atmosphere (TOA) solar insolation, and exceeds the forcing efficiency that has been observed for other polluted regions in America, Africa, East Asia, and Europe. General circulation model sensitivity studies suggest that both the local and remote influence of the aerosol induced radiative forcing is to strengthen the lower atmosphere inversion, stabilize the boundary layer, amplify the climatological tendency for a drier troposphere, and decrease evaporation. These aerosol-induced changes could potentially increase the life times of aerosols, make them more persistent, and decrease their single scattering albedos, thus potentially leading to a detrimental positive feedback between aerosol concentrations, aerosol forcing, and aerosol persistence. In addition, both the model studies and observations of pan evaporation suggest that the reduction in surface solar radiation may have led to a reduction in surface evaporation of moisture. These results suggest the vulnerability of this vital region to air pollution related direct and indirect (through climate changes) impacts on agricultural productivity of the region.  相似文献   

14.
This study contains a comparative analysis of aerosol optical thickness (AOT) between numerical calculations obtained from the Navy Aerosol Analysis and Prediction System (NAAPS) model and direct observations from the AERONET robotic network and the Saharan Aerosol over WArsaw (SAWA) field campaign. AOT was calculated for 500 nm wavelength. The comparison shows underestimation of the total aerosol optical thickness simulated by NAAPS. The correlation coefficients between model and observation oscillates between 0.57 and 0.72. Results of seven-year (1998–2004) NAAPS simulation of aerosol components (sea salt, mineral dust, sulphate, and smoke) show large temporal and spatial variability of the aerosol optical thickness over Europe. The least polluted region is the Iberian Peninsula, while the highest aerosol burdens occurred in Central Europe, mostly due to anthropogenic sulphate particles. Finally, the analysis of mineral dust transport shows frequent episodes of Saharan dust inflow over Central Europe. There are about 20 days a year (4 days in May) when instantaneous AOT associated with mineral dust aerosol increases over 0.1.  相似文献   

15.
Continuous measurements of solar spectral radiation using the Multi-filter Rotating Shadow Band Radiometer (MFRSR) are performed at the Actinometric Station of the National Observatory of Athens (ASNOA). The present study utilizes three clear-sky days of continuous observations, from local sunrise to local sunset, in order to investigate the daily variation of the radiation components (diffuse, global and direct-beam) as well as their ratios (diffuse-to-global, DGR, and diffuse-to-direct-beam, DDR) under different atmospheric conditions. Both ratios have received great scientific interest, especially for investigating solar irradiance modifications under various atmospheric conditions, aerosol load and optical properties. Apart from this, the present study shows that the DDR can constitute a measure of atmospheric turbidity when it is determined at longer wavelengths, while the DGR cannot. The effect of the solar zenith angle (SZA) on both ratios is significant at the shorter wavelengths with varying sensitivities depending on the aerosol field and sun elevation. The present study confirms the results obtained by previous solar irradiance measurements in Athens and also those computed via radiative transfer codes and sheds light on the scientific knowledge of the use of spectral DDR as an atmospheric turbidity index.  相似文献   

16.
This work estimates the Ångström turbidity coefficients and investigates the variation of the aerosol optical depth (AOD) in the Athens area, during different atmospheric conditions. The AOD is estimated in the wavelength band of 400–670 nm from direct-beam spectral irradiance measurements using ground-based instrumentation, during an experimental campaign performed in the period 22 September–1 October 2002. All data were collected under clear-sky conditions near the city center of Athens; the AODs were estimated relative to the local zenith to avoid the influence of the optical air mass. The study shows that the AOD is influenced by wind regime and traffic in the Athens area. The Angstrom's turbidity coefficients and the AOD values were found to be higher under the influence of South-sector winds compared to those from the North-sector. Under South-sector low winds, the pollutants are accumulated in the Athens basin. On the contrary, the North-sector winds clean the atmosphere.  相似文献   

17.
Two sounding rockets equipped with photometers and particle detectors have been flown into proton auroras. The measured altitude dependence of the proton flux is compared with calculations based upon known energy-range relations for protons in air. Expressions suitable for numerical calculations of Doppler profiles at arbitrary angles to the geomagnetic field and at different heights within an aurora are developed. Profiles due to some typical proton spectra have been calculated and it is shown that altitude profiles at some wavelengths are more sensitive to the shape of the proton spectrum than are profiles at other wavelengths. Variations in the H <beta> Doppler profile versus height for several angles with the magnetic field is studied. Profiles, as generated by the actually measured protons in the energy range 1 keV to 1 MeV, have been calculated and are compared with direct optical measurements made by ground and rocket photometers. The rocket photometers took measurements at different wavelengths within the Doppler profile. The correspondence between calculations and measurements is generally good. The total H <beta> is calculated and fair agreement with the measured intensity is found.  相似文献   

18.
A theoretical model based on some physical assumptions has been integrated to study the scattering of solar radiation by aerosol particulates of any size present in the atmosphere. Using this model, which incorporates multiple scattering, scattered fluxes of radiation with varying optical depths and also the optical depth versus wavelengths are computed. The present results are found to be in close agreement with the observations of the Pre-Indian Ocean Experiment (INDOEX) 1996. This provides evidence of the direct effect of aerosol particulates on the radiative forcing of the atmosphere.  相似文献   

19.
Aerosol optical properties have been studied for spring seasons when increased values of PM10 are registered. Measurements of aerosol optical properties were taken by collocated lidar and sun-photometers at Belsk, Poland, and Minsk, Belarus. A significant increase of registered aerosol optical thickness (AOT) was found during episodes with elevated PM10 concentrations. An increase of AOT at 1020 nm amounted to 50% in the case of Minsk and 18% in the case of Belsk, while an increase of AOT at 400 nm was 66% and 33%, respectively. We noted an increase of Ångström exponent by 6% at both stations and no significant increase of single scattering albedo. The LIDAR measurements together with NAAPS model results and backtrajectory analysis suggest that both the biomass burning products and the Saharan dust are responsible for increased PM10 concentrations and large AOT values during spring time. The smoke aerosol is transported over Central Europe mainly in the boundary layer, increasing both PM10 concentration and AOT. The dust aerosol transported in the free troposphere slightly affects the AOT values only. Statistically significant correlation between PM10 concentration and AOT was found during reporting period.  相似文献   

20.
Extensive and collocated measurements of several aerosol parameters were made over the eastern Arabian Sea, during the inter-monsoon and summer monsoon seasons of 2003 as a part of the Arabian Sea Monsoon Experiment (ARMEX). Associated with the seasonal changes in the synoptic wind fields from northeasterly/easterly to westerly/northwesterly, the aerosol characteristics and columnar optical depth show large variations. Consequently, the atmospheric forcing is found to increase from March to April and then to decrease consistently towards June. However, the magnitude of the forcing efficiency of aerosols continuously decreases from winter to summer. Such temporal changes in radiative forcing need to be accounted for in reducing the uncertainty in aerosol climate impact.  相似文献   

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