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1.
Soil moisture is an important variable in explaining hydrological processes at hillslope scale. The distribution of soil moisture along a hillslope is related to the spatial distribution of the soil properties, the topography, the soil depth, and the vegetation. In order to investigate the factors affecting soil moisture, various environmental data were collected from a humid forest hillslope in this study. Several factors (the wetness index; the contributing area; the local slope; the soil depth; the composition of sand, silt, and clay; the scaling parameter; the hydraulic conductivity; the tree diameter at breast height; and the total weighted basal area) were evaluated for their effect on soil moisture and its distribution over the hillslope at depths of 10, 30, and 60 cm. Both linear correlation analysis and empirical orthogonal function analysis indicated that the soil texture was a dominant factor in soil moisture distribution. The impact of soil hydraulic conductivity was important for all soil moisture ranges at a depth of 30 cm, but those at 10 and 60 cm were limited to very wet and dry conditions, respectively. The relationships of the various factors with the spatial variability of soil moisture indicated the existence of a threshold soil moisture that is related to the composition of the soil and the factors related to the distribution of water in the study area.  相似文献   

2.
Rainwater harvesting through modified contour ridges known as dead level contours has been practiced in Zimbabwe in the last two decades. Studies have shown marginal soil moisture retention benefits for using this technique while results on crop yield benefits are lacking. This paper presents results from a field study for assessing the impact of dead level contours on soil moisture and crop yield carried out from 2009 to 2011 within the Limpopo River Basin. The experiments were carried out on two study sites; one containing silt loam soil and another containing sandy soil. Three treatments constituting dead level contoured plots, non-contoured plots and plots with the traditional graded contours were used on each site. All the three treatments were planted with a maize crop and managed using conventional farming methods. Planting, weeding and fertiliser application in the three treatments were done at the same time. Crop monitoring was carried out on sub plots measuring 4 m by 4 m established in every treatment. The development of the crop was monitored until harvesting time with data on plant height, leaf moisture and crop yield being collected. An analysis of the data shows that in the site with silt loam soil more soil moisture accumulated after heavy rainfall in dead level contour plots compared to the control (no contours) and graded contour plots (P < 0.05). However the maize crop experienced an insignificantly (P > 0.05) higher yield in the dead level contoured treatment compared to the non-contoured treatment while a significantly (P < 0.05) higher yield was obtained in the dead level contoured treatment when compared with a graded contoured treatment. Different results were obtained from the site with sandy soil where there was no significant difference in soil moisture after a high rainfall event of 60 mm/day between dead level contour plots compared to the control and graded contour plots. The yield from the dead level contoured treatment and that from the graded contoured treatment were comparable and both not significantly (P > 0.05) higher than that from the non-contoured treatment. This suggests that adopting dead level contours as an in situ rainwater harvesting technique results in crop yield benefits in fields with soil type conditions that enable runoff generation but is not likely to have benefit in soils with low runoff generation.  相似文献   

3.
An accurate prediction of solute infiltration in a soil profile is important in the area of environmental science, groundwater and civil engineering. We examined the infiltration pattern and monitored the infiltration process using a combined method of dye tracer test and electrical resistivity tomography (ERT) in an undisturbed field soil (1 m × 1 m). A homogeneous matrix flow was observed in the surface soil (A horizon), but a preferential flow along macropores and residual rock structure was the dominant infiltration pattern in the subsurface soil. Saturated interflow along the slopping boundaries of A and C1 horizons and of an upper sandy layer and a lower thin clay layer in the C horizon was also observed. The result of ERT showed that matrix flow started first in A horizon and then the infiltration was followed by the preferential flows along the sloping interfaces and macropores. The ERT did not show as much detail as the dye‐stained image for the preferential flow. However, the area with the higher staining density where preferential flow was dominant showed a relatively lower electrical resistivity. The result of this study indicates that ERT can be applied for the monitoring of solute transportation in the vadose zone. Copyright © 2010 John Wiley & Sons, Ltd.  相似文献   

4.
Preferential flow is known to influence hillslope hydrology in many areas around the world. Most research on preferential flow has been performed in temperate regions. Preferential infiltration has also been found in semi‐arid regions, but its impact on the hydrology of these regions is poorly known. The aim of this study is to describe and quantify the influence of preferential flow on the hillslope hydrology from small scale (infiltration) to large scale (subsurface stormflow) in a semi‐arid Dehesa landscape. Precipitation, soil moisture content, piezometric water level and discharge data were used to analyse the hydrological functioning of a catchment in Spain. Variability of soil moisture content during the transition from dry to wet season (September to November) within horizontal soil layers leads to the conclusion that there is preferential infiltration into the soils. When the rainfall intensity is high, a water level rapidly builds up in the piezometer pipes in the area, sometimes even reaching soil surface. This water level also drops back to bedrock within a few hours (under dry catchment conditions) to days (under wet catchment conditions). As the soil matrix is not necessarily wet while this water layer is built up, it is thought to be a transient water table in large connected pores which drain partly to the matrix, partly fill up bedrock irregularities and partly drain through subsurface flow to the channels. When the soil matrix becomes wetter the loss of water from macropores to the matrix and bedrock decreases and subsurface stormflow increases. It may be concluded that the hillslope hydrological system consists of a fine matrix domain and a macropore domain, which have their own flow characteristics but which also interact, depending on the soil matrix and macropore moisture contents. The macropore flow can result in subsurface flow, ranging from 13% contribution to total discharge for a large event of high intensity rainfall or high discharge to 80% of total discharge for a small event with low intensity rainfall or low discharge. During large events the fraction of subsurface stormflow in the discharge is suppressed by the large amount of surface runoff. Copyright © 2008 John Wiley & Sons, Ltd.  相似文献   

5.
6.
Many studies have focused on the amount of stemflow in different forests and for different rainfall events, but few studies have focused on how stemflow intensity varies during events or the infiltration of stemflow into the soil. Stemflow may lead to higher water delivery rates at the base of the tree compared with throughfall over the same area and fast and deeper infiltration of this water along roots and other preferential flow pathways. In this study, stemflow amounts and intensities were measured and blue dye experiments were conducted in a mature coniferous forest in coastal British Columbia to examine double funnelling of stemflow. Stemflow accounted for only 1% of precipitation and increased linearly with event total precipitation. Funnelling ratios ranged from less than 1 to almost 20; smaller trees had larger funnelling ratios. Stemflow intensity generally was highest for periods with high‐intensity rainfall later in the event. The maximum stemflow intensities were higher than the maximum precipitation intensities. Dye tracer experiments showed that stemflow infiltrated primarily along roots and was found more frequently at depth than near the soil surface. Lateral flow of stemflow was observed above a dense clay layer for both the throughfall and stemflow experiments. Stemflow appeared to infiltrate deeper (122 cm) than throughfall (85 cm), but this difference was in part a result of site‐specific differences in maximum soil depth. However, the observed high stemflow intensities combined with preferential flow of stemflow may lead to enhanced subsurface stormflow. This suggests that even though stemflow is only a very minor component of the water balance, it may still significantly affect soil moisture, recharge, and runoff generation. Copyright © 2016 John Wiley & Sons, Ltd.  相似文献   

7.
This study examined the effects of different soil texture configurations on water movement and solute transport to provide a reliable scientific basis for the application of negative‐pressure irrigation (NPI) technology. HYDRUS‐2D was used to analyse water movement and solute transport under NPI. The main results are as follows: (a) HYDRUS‐2D can be used to simulate water movement and solute transport under NPI, as there was good agreement between the simulated and measured values for water contents, NaCl concentrations, cumulative water infiltration, and wetting distances in the horizontal and vertical directions; the Nash–Sutcliffe efficiency coefficients were in the range of 0.94–0.97. (b) Layered soils have obvious effects on water movement under NPI. With the emitter position in the loam layer, when a coarse texture of loamy sand was present below the loam layer (namely, L‐LS), irrigation water accumulated in the topsoil, and this led to an increase in evaporation compared with the homogeneous loam profile. However, fine texture silty loam or silty clay loam layers beneath the loam layer (namely, L‐SiL or L‐SiCL, respectively) was more conducive to water infiltration into the lower layer, and this increased the amount of water infiltration and simultaneously reduced the surface evaporation effectively. (c) Layered soils have obvious effects on solute transport under NPI, and salt accumulation will readily occur in the clay‐rich soil layer at the interface. The maximum soil salt accumulation of L‐LS occurred above the soil interface between the two soil layers with a value of 21.80 g/kg; however, for L‐SiCL and L‐SiL, the maximum salt accumulation occurred below the soil interface between the two soil layers, with values of 23.80 g/kg and 20.08 g/kg, respectively. (d) Interlayered soils showed remarkable changes in the water infiltration characteristics and salt‐leaching intensities under NPI, and the properties for the soil profile with a silty loam interlayer were better than those for the soil profile with a silty clay loam interlayer. The soil profile with a loamy sand interlayer had the lowest amount of water infiltration, which resulted in reductions of the salt‐leaching intensities. Thus, NPI is clearly not suitable for loamy sand soil. Overall, the results demonstrated that soil texture configurations affected water movement and solute transport under NPI. Therefore, careful consideration should be given to the use of NPI to achieve target soil water and solution conditions and reduce water loss.  相似文献   

8.
We studied the temporal patterns of tracer throughput in the outflow of large (30 cm diameter by 38 cm long) undisturbed cores from the Panola Mountain Research Watershed, Georgia. Tracer breakthrough was affected by soil structure and rainfall intensity. Two rainfall intensities (20 and 40 mm hr−1) for separate Cl and Br amended solutions were applied to two cores (one extracted from a hillslope soil and one extracted from a residual clay soil on the ridge). For both low and high rainfall intensity experiments, preferential flow occurred in the clay core, but not in the hillslope core. The preferential flow is attributed to well‐developed interpedal macrochannels that are commonly found in structured clay soils, characteristic of the ridge site. However, each rainfall intensity exceeded the matrix infiltration capacity at the top of the hillslope core, but did not exceed the matrix infiltration capacity at the middle and bottom of the hillslope core and at all levels in the clay core. Localized zones of saturation created when rainfall intensity exceeds the matrix infiltration capacity may cause water and tracer to overflow from the matrix into macrochannels, where preferential flow occurs to depth in otherwise unsaturated soil. Copyright © 1999 John Wiley & Sons, Ltd.  相似文献   

9.
The loss of P in overland flow from most cultivated soils is controlled by erosion, and in‐turn soil moisture. We evaluated the effect of soil moisture on erosion and P transport in overland flow by applying rainfall (7 cm h?1) to packed soil boxes (1 m long and 0·15 m wide) and field plots (1 and 10 m long by 1 m wide) of silt loams in a central Pennsylvania (USA) catchment. Flow from packed soil boxes took longer to initiate as antecedent soil moisture decreased from field capacity (2 min) to air dried (8 to 9 min). Even in the more complex field plots (i.e. soil heterogeneity and topography), the wetter site (1 by 10 m plot; 70% field capacity) produced flow more quickly (3 min) and in greater volume (439 L) than the drier site (1 by 10 m plot; 40% field capacity, 15 min, and 214 L, respectively). However, less suspended sediment was transported from wetter soil boxes (1·6 to 2·5 g L?1) and field plots (0·9 g L?1) than drier boxes (2·9 to 4·2 g L?1) and plots (1·2 g L?1). Differences are attributed to their potential for soil aggregate breakdown, slaking and dispersion, which contribute to surface soil sealing and crusting, as dry soils are subject to rapid wetting (by rainfall). During flow, selective erosion and antecedent moisture conditions affected P transport. At field capacity, DRP and PP transport varied little during overland flow. Whereas P transport from previously dry soil decreased rapidly after the initiation of flow (6 to 1·5 mg TP L?1), owing to the greater slaking and dispersion of P‐rich particles into flow at the beginning than end of the flow event. These results indicate that soil moisture fluctuations greatly effect erosion and P transport potential and that management to decrease the potential for loss should consider practices such as conservation tillage and cover crops, particularly on areas where high soil P and erosion coincide. Copyright © 2002 John Wiley & Sons, Ltd.  相似文献   

10.
ABSTRACT

Infiltration plays a fundamental role in streamflow, groundwater recharge, subsurface flow, and surface and subsurface water quality and quantity. In this study, adaptive neuro-fuzzy inference system (ANFIS), support vector machine (SVM) and random forest (RF) models were used to determine cumulative infiltration and infiltration rate in arid areas in Iran. The input data were sand, clay, silt, density of soil and soil moisture, while the output data were cumulative infiltration and infiltration rate, the latter measured using a double-ring infiltrometer at 16 locations. The results show that SVM with radial basis kernel function better estimated cumulative infiltration (RMSE = 0.2791 cm) compared to the other models. Also, SVM with M4 radial basis kernel function better estimated the infiltration rate (RMSE = 0.0633 cm/h) than the ANFIS and RF models. Thus, SVM was found to be the most suitable model for modelling infiltration in the study area.  相似文献   

11.
Changes in hydrologic flowpaths have important impacts on the timing, magnitude and hydrochemistry of run‐off during snowmelt in forested catchments, but how flowpaths are affected by variation in winter climate and the irregular presence of soil frost remains poorly understood. The depth and extent of soil frost may be expected to increase as snowpack decreases or develops later because of climate change. In this study, we used end‐member mixing analysis to determine daily contributions of snow, forest floor soil water and groundwater to stream run‐off during snowmelt under different soil frost regimes resulting from interannual and elevational variation at the Hubbard Brook Experimental Forest in New Hampshire, USA. We observed greater routing of run‐off through forest floor flowpaths during early snowmelt in 2011, when the snowpack was deep and soil frost was minimal, compared with the early snowmelt in 2012 under conditions of deep and extensive soil frost. The results indicate that widespread soil frost that penetrated the depth of the forest floor decreased the flow signal through the shallowest subsurface flowpaths, but did not reduce overall infiltration of melt waters, as the contribution from the snow‐precipitation end‐member was similar under both conditions. These results are consistent with development of granular soil frost which permits vertical infiltration of melt waters, but either reduces lateral flow in the forest floor or prevents the solute exchange that would produce the typical chemical signature of shallow subsurface flowpaths in streamwater. Copyright © 2016 John Wiley & Sons, Ltd.  相似文献   

12.
13.
Soils derived from different lithologies and their controls on preferential flow remain underexplored in forested landscapes. In the same lithology, the propensity for preferential flow occurrence at different hillslope positions also remains largely elusive. By utilizing a soil moisture response time method, we compared preferential flow occurrence between a shale site (Shale Hills, silt loam soils) and a sandstone site (Garner Run, sandy loam soils) at four hillslope positions: ridge-top, North- and South-facing mid-slopes and toe slope, for over 2 years. The catchments are neighbouring and covered by temperate forest. For the four hillslope positions, Shale Hills had higher preferential flow frequencies compared to Garner Run. Between these two catchments, the South-facing mid-slope sites showed the highest contrasts in preferential flow frequency (33.5% of events at Shale Hills vs. 8.8% at Garner Run) while the ridge-top sites showed the lowest contrasts (18.7 vs. 13.2%). Additionally, over the unfrozen period, for seven out of eight monitoring sites, drier antecedent conditions tended to be more favourable for preferential flows to occur, with significant (p < .01) relationships at two sites. Except for the South-facing mid-slope sites, both Shale Hills and Garner Run had two preferential flow pathways. The characteristic preferential flow pathways at Shale Hills were the Bw and C horizons, and for Garner Run, preferential flow moved from the E/AE horizon to the Bw horizon. This study shows that shale-derived soils tended to have higher preferential flow occurrence than sandstone soils, but hillslope positions exhibit different levels of contrasts. More effort should be paid to study the impact of lithology on preferential flows in the context of land surface modelling and biogeochemical reactions to improve ecosystem services of headwater catchments.  相似文献   

14.
The effect of super absorbent polyacrylate (SAP) hydrogel amendment to different soil types on plant available water (PAW), evapotranspiration and survival of Eucalyptus grandis, Eucalyptus citriodora, Pinus caribaea, Araucaria cunninghamii, Melia volkensii, Grevillea robusta, Azadirachta indica, Maesopsis eminii and Terminalia superba was investigated. The seedlings were potted in 3 kg size polythene bags filled with sand, loam, silt loam, sandy loam and clay soils, amended at 0 (control), 0.2 and 0.4% w/w hydrogel. The tree seedlings were allowed to grow normally with routine uniform watering in a glass house set up for a period of eight weeks, after which they were subjected to drought conditions by not watering any further. The 0.4% hydrogel amendment significantly (p < 0.05) increased the PAW by a factor of about three in sand, two fold in silt loam and one fold in sandy loam, loam and clay soils compared to the control. Similarly, the addition of either 0.2 or 0.4% hydrogel to the five soil types resulted in prolonged tree survival compared to the controls. Araucaria cunninghammi survived longest at 153 days, while Maesopsis eminii survived least (95 days) in sand amended at 0.4% after subjection to desiccation. Evapotranspiration was reduced in eight of the nine tree species grown in sandy loam, loam, silt loam and clay soils amended at 0.4% hydrogel. It is probable that soil amendment with SAP decreased the hydraulic soil conductivity that might reduce plant transpiration and soil evaporation.  相似文献   

15.
Many investigations show relationships between topographical factors and the spatial distribution of soil moisture in catchments. However, few quantitative analyses have been carried out to elucidate the role of different hydrological processes in the spatial distribution of topsoil moisture in catchments. A spatially distributed rainfall—runoff model was used to investigate contributions of subsurface matric flow, macropore flow and surface runoff to the spatial distribution of soil moisture in a cultivated catchment. The model results show that lateral subsurface flow in the soil matrix or in macropores has a minor effect on the spatial distribution of soil moisture. Only when a perched groundwater table is maintained long enough, which is only possible if the subsurface is completely impermeable, may a spatial distribution in moisture content occur along the slope. Surface runoff, producing accumulations of soil moisture in flat flow paths of agricultural origin (field boundaries), was demonstrated to cause significant spatial variations in soil moisture within a short period after rainfall (<2 days). When significant amounts of surface runoff are produced, wetter moisture conditions will be generated at locations with larger upstream contributing areas. Copyright © 2001 John Wiley & Sons, Ltd.  相似文献   

16.
Sampling of soil pore moisture in the vadose zone underneath land disposal facilities (landfills and surface impoundments) for hazardous waste has been suggested as an "early warning system" to detect leakage from these facilities. Some states require vadose zone moisture sampling at such sites. Given a leak of a particular size, mathematical models can estimate the necessary moisture sample volume collection times and lysimeter spacings to guarantee detection of the leak in a homogeneous medium. Examination of 47 hazardous waste sites existing in 1984 indicated the most were located in areas with water tables too shallow to permit vadose zone detection monitoring. Several of the 47 sites had soils that could be described as loamy sand, silt loam or silty clay. Using these three soils as examples, the process of lysimeter leak-detector network design has been illustrated. For a particular loamy sand with a saturates hydraulic conductivity of 10-6 cm/ sec, the maximum ceramic lysimeter spacing is 15.5 feet at a depth of 30 feet to collec a moisture sample of 10 mL in one week from a 1 ft2 leak. For a silt loam, maximum lysimeter spacing would be 17 feet at depth of 15 feet. For silty clays, the maximum lysimeter spacing is 7 feet at a depth of 2 feet; maximum emplacement depth is about 9 feet. Calculations show that in some soils, suction lysimeters will not be able to collect usable moisture samples. Since soil properties vary widely and lysimeter spacing is strongly dependent on soil-moisture characteristics appropriate soil measurements and modeling must be performed at each disposal facility to estimate lysimete performance and to select locations for emplacement.  相似文献   

17.
Todd Redding  Kevin Devito 《水文研究》2010,24(21):2995-3010
Rainfall simulation experiments by Redding and Devito ( 2008 , Hydrological Processes 23: 4287–4300) on two adjacent plots of contrasting antecedent soil moisture storage on an aspen‐forested hillslope on the Boreal Plain showed that lateral flow generation occurred only once large soil storage capacity was saturated combined with a minimum event precipitation of 15–20 mm. This paper extends the results of Redding and Devito ( 2008 , Hydrological Processes 23: 4287–4300) with detailed analysis of pore pressure, soil moisture and tracer data from the rainfall simulation experiments, which is used to identify lateral flow generation mechanisms and flow pathways. Lateral flow was not generated until soils were wet into the fine textured C horizon. Lateral flow occurred dominantly through the clay‐rich Bt horizon by way of root channels. Lateral flow during the largest event was dominated by event water, and precipitation intensity was critical in lateral flow generation. Lateral flow was initiated as preferential flow near the soil surface into root channels, followed by development of a perched water table at depth, which also interacted with preferential flow pathways to move water laterally by the transmissivity feedback mechanism. The results indicate that lateral flow generated by rainfall on these hillslopes is uncommon because of the generally high available soil moisture storage capacity and the low probability of rainfall events of sufficient magnitude and intensity. Copyright © 2010 John Wiley & Sons, Ltd.  相似文献   

18.
Soil erosion by water in abandoned dry terraces is one of the most important environmental problems in semiarid areas, enhancing biological degradation and reducing possible resources that can be obtained. However, little is known about the effects of the types of lithology and soil properties on the early stages of soil erosion. Therefore, the main aim of this research was to assess the effect of different lithologies (marls, limestones, and metamorphic—phyllites, schists, and greywackes—materials) and soil properties on the early stages of soil erosion by water in abandoned dry terraces, compared with similar terraces still in agricultural use. Soil analyses (texture, aggregate stability, and bulk density) and 22 rainfall simulations were carried out under dry conditions. During the experiments, local inclination, vegetation and stone cover, total organic matter, and antecedent soil moisture were also quantified. The results showed that the highest soil loss (41.41 g/m2 in cultivated plots and 17.05 g/m2 in the abandoned plots) and runoff (3.79 L/m2 in the abandoned plot) occurred on marl substrata. Marls also showed the shallowest infiltration front (9 cm) and lowest infiltration rate (4.3 cm/min). Limestones and, especially, metamorphic areas, showed a lower degree of soil erosion, higher infiltration rates, and deeper infiltration fronts.  相似文献   

19.
Surface infiltration and internal drainage properties of five soil types from arid drylands of South Africa were studied under double ring infiltrometer, rainfall simulation plots (1 m2) and instantaneous drainage plots (9 m2). Changes in soil water content during 40 minute rainfall simulation for a rainstorm with average intensity of 1.61 mm min?1 and 30 day drainage period were measured at various depths by 1.5 m long capacitance soil water measuring (DFM) probe. Different (P < 0.05) mean surface steady infiltration rate ranged from 0.05 to 4.47 mm min?1 and had a negative power relationship (R 2 = 0.65) with horizon clay plus fine silt content. Power regression (R 2 ≥ 86%) described rainstorm infiltration and obtained steady rates within an average time of 15 minutes. Mean total infiltrated soil water content was lowest (P < 0.05) from surface horizons with either 47.7% clay plus fine silt content or bulk density of 1.91 g cm?3 and exchangeable sodium of not less than 44 mg kg?1. Surface horizons with lower surface bulk density and total sand fraction of more than 72% had infiltrated depth and mean total infiltrated soil water content up to 40 cm deeper and 0.55 mm mm?1 greater, respectively. Drainage rate at drained upper limit calculated from the Wilcox drainage model (R 2 ≤ 0.97%) was 0.2 mm day?1 or less were from underlying horizons with either clay plus fine silt of 45% or soft calcium carbonate. Higher drainage rate with accumulative drainage amount greater than 60 mm were from soil profile horizons with clay plus fine silt content of less than 20% and above unity steady infiltration rates. Rainstorm infiltration and drainage rates was shown to depend on permeability and coarseness of the respective soil surface and subsurface horizons; a phenomenon critical for harnessing rain and flood water to recharge groundwater. Copyright © 2016 John Wiley & Sons, Ltd.  相似文献   

20.
Using a Simple Soil Column Method to Evaluate Soil Phosphorus Leaching Risk   总被引:3,自引:0,他引:3  
The impacts of soil P leaching on water eutrophication have widely been concerned. However, there is no dependable method to quantitatively estimate the P leaching risk of soils. In this study, a simple soil column method was developed using two calcareous Fluvisols, silt loam and loam. The soil column was 20 cm in length and 5 cm in diameter, and distilled water was continuously supplied from the top. The volume and dissolved reactive P (DRP) concentrations of leachate were measured. Results showed that DRP concentrations in leachate increased slowly for the low soil Olsen‐P levels but rapidly for the high Olsen‐P levels. According to these two‐phase changes in the DRP versus soil Olsen‐P contents, the thresholds of P leaching risk were estimated to be 41.1 and 62.3 mg P kg?1 (Olsen‐P) for silt loam and loam, respectively. The P leaching intensity of soils increased by 3‐ to 540‐fold if the soil Olsen‐P contents accumulated from 6.6 to 155.5 mg P kg?1. The outcomes derived from this study regarding the determination of P leaching threshold and intensity by the soil column method also need a further verification on more soils with a wide range of physical and chemical properties.  相似文献   

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