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1.
大气湿沉降向太湖水生生态系统输送氮的初步估算   总被引：30，自引：3，他引：27  
测定和分析了2002年7月至2003年6月太湖周边地区太湖站、拖山岛、东山站、无锡、苏州、湖州、常州等7个站点大气降水化学组成,计算了水气界面TN、NH4 -N、NO3--N、T1N、TON的湿沉降率。结果表明,大气降水的TN浓度变化范围为2.06±0.30(常州)-3.71±0.43(拖山岛),太湖流域大气降水已呈富营养化水质的特征;大气降水TN、NH4 -N、NO3--N、TIN、TON的年均湿沉降率分别为2806.75kg/km2、1458.81kg/km2、631.67kg/km2、2090.48kg/km2和716.28kg/km2;每年由湿沉降直接进入太湖水体的TN约为6562.2t,NH4 -N为3410.7t,NO3--N为1476.8t,TIN为4887.5t,TON为1674.7t;TN占入湖河道年输入污染物总量的13.6%.大气湿沉降中,TIN对TN的贡献比较大,平均约占TN的78.78%.TIN的湿沉降率具有季节性分布,夏季高,春季次之,冬秋季低。这种现象无疑对太湖水体的蓝藻爆发和富营养化具有潜在的促进作用.  相似文献   

2.
The aim of the atmospheric nitrogen inputs into the coastal ecosystem (ANICE) project is to improve transport–chemistry models that estimate nitrogen deposition to the sea. To achieve this, experimental and modelling work is being conducted which aims to improve understanding of the processes involved in the chemical transformation, transport and deposition of atmospheric nitrogen compounds. Of particular emphasis within ANICE is the influence of coastal zone processes. Both short episodes with high deposition and chronic nitrogen inputs are considered in the project. The improved transport–chemistry models will be used to assess the atmospheric inputs of nitrogen compounds into the European regional seas (the North Sea is studied as a prototype) and evaluate the impact of various emission reduction strategies on the atmospheric nitrogen loads. Assessment of the impact of atmospheric nitrogen on coastal ecosystems will be based on comparisons of phytoplankton nitrogen requirements, other external nitrogen inputs to the ANICE area of interest and the direct nitrogen fluxes provided by ANICE. Selected results from both the experimental and modelling components are presented here. The experimental results show the large spatial and temporal variability in the concentrations of gaseous nitrogen compounds, and their influences on fluxes. Model calculations show the strong variation of both concentrations and gradients of nitric acid at fetches of up to 25 km. Aerosol concentrations also show high temporal variability and experimental evidence for the reaction between nitric acid and sea salt aerosol is provided by size-segregated aerosol composition measured at both sides of the North Sea. In several occasions throughout the experimental period, air mass back trajectory analysis showed connected flow between the two sampling sites (the Weybourne Atmospheric Observatory on the North Norfolk coast of the UK and Meetpost Noordwijk, a research tower at 9 km off the Dutch coast). Results from the METRAS/SEMA mesoscale chemistry transport model system for one of these cases are presented. Measurements of aerosol and rain chemical composition, using equipment mounted on a commercial ferry, show variations in composition across the North Sea. These measurements have been compared to results obtained with the transport–chemistry model ACDEP which calculates the atmospheric inputs into the whole North Sea area. Finally, the results will be made available for the assessment of the impact of atmospheric nitrogen on coastal ecosystems.  相似文献   

3.
李静  陈光杰  黄林培  孔令阳  索旗  王旭  朱云  张涛  王露 《湖泊科学》2023,35(6):2170-2184
区域增温和大气氮沉降作用已成为高山湖泊面临的重要环境胁迫,已有高山湖泊生物群落响应的长期模式研究主要集中于藻类而缺乏更高营养级生物(如浮游动物)的系统调查。本研究选择滇西北地区深水型的高山湖泊沃迪错开展沉积物调查,通过多指标分析(总氮、总磷、叶绿素a、氮稳定同位素等)并结合区域气候重建记录,识别近两百年来该湖泊及流域环境的变化历史,进一步利用枝角类群落指标(物种组成、生物量等)定量评价了湖泊生物群落的响应模式与驱动因子。结果表明,湖泊营养水平(如总氮浓度)和初级生产力(叶绿素a浓度等)在过去近两百年总体呈上升趋势。相关分析显示,大气氮沉降和流域外源输入是影响总氮上升的主要因素,同时区域增温和营养盐富集促进了湖泊初级生产力的不断上升。自1960s以来区域升温明显,湖泊营养水平和叶绿素a浓度呈现加速上升的趋势。钻孔中枝角类群落以浮游属种(Daphnia longispina等)为优势种,在1900AD以前D.longispina相对丰度较为稳定(40.83%±8.02%),之后出现下降趋势且在1948—1965年间明显下降,之后再次明显上升并成为主要优势种。排序分析显示,气温、叶绿素a和总...  相似文献   

4.
亚热带地区典型水库流域氮、磷湿沉降及入湖贡献率估算   总被引：1，自引：0，他引：1  
为了探究汤浦水库流域氮、磷湿沉降对水库水体营养的贡献率,本研究对2014 2015年的汤浦水库流域4个采样点的雨水及3条溪流进行样品收集,测定其中磷和不同形态氮的质量浓度,分析汤浦水库流域大气湿沉降中氮、磷营养盐的分布特征,并估算氮、磷营养盐湿沉降对汤浦水库入库负荷的贡献率.结果表明:湿沉降中总氮(TN)平均浓度为1.02±0.58 mg/L,氨氮、硝态氮和有机氮浓度占TN浓度的比例分别为60.65%、34.07%和5.28%;总磷(TP)平均浓度为0.033±0.028 mg/L.4个采样点湿沉降中氮、磷浓度均表现为冬春季(少雨季)高、夏秋季(多雨季)低.空间上,王化点位的各形态氮和总磷浓度显著高于其他3个采样点.TN和TP年均湿沉降通量约为18.15和0.62 kg/(hm~2·a),年均沉降总量为834.94和28.39 t;库区TN和TP水面湿沉降量为24.14和0.82 t,直接贡献率占河流输入的1.77%和3.07%.湿沉降来源的氮、磷营养盐随河流输入的间接贡献率为8.3%和4.6%.综上所述,氮、磷湿沉降是水库外源营养的重要输入部分,深入掌握其时空分布特征及入库贡献率是进一步加强流域管理和减轻水库外源营养输入的重要前提.  相似文献   

5.
Little is known about the distribution and risk levels of nutrients and organic matter(OM) in the surface sediment of shallow submerged macrophyte-dominated lakes. In the current study, sixty surface sediment samples were collected from Xukou Bay, a typical submerged macrophyte-dominated zone in Lake Taihu, China. A 60-day degradation experiment of Potamogeton malaianus, a dominant species in the bay,was done in the laboratory. The results demonstrated that the ranges of total nitrogen(TN) and t...  相似文献   

6.
A. O. Pektas 《水文科学杂志》2017,62(10):1694-1703
Suspended sediment modelling is a quite significant issue in hydrology. The prediction of suspended sediment has taken the attention of several scientists in water resources. With extrapolation, the forecasting ability of the employed forecasting model beyond the calibration range is investigated. In the present study, different smoothing parameters are used to differentiate the kurtosis of the local critical points (local minima and maxima). The two models used are an artificial neural network (ANN) model and a multiple linear regression (MLR) model for prediction in order to examine the model extrapolation ability. The ANN model provides closer estimations to the observed peaks, being higher than the corresponding MLR ones. For the local minima, the ANN predictions are higher than the MLR predictions. As there are limited local points, all the remaining ANN predictions are lower than the MLR ones except for one point.  相似文献   

7.
济南市不同区域水生生物与水环境因子的响应关系   总被引：2，自引：2，他引：0  
水生生物与水环境因子是水生态系统中重要的组成部分,研究水生生物与水环境因子的响应关系对制定水生态系统修复方案具有重要意义.于2014年5、8和10月,对济南市水生态系统进行野外采样调查.共设36个采样点,采集鱼类、底栖动物、浮游动物和浮游植物四种生物,并测定了26个水环境因子.采用Spearman相关分析法、小提琴图法和冗余分析法,筛选主要的水环境因子,分析济南市水生生物丰富度和主要水环境因子的分布特征,以及两者间的相互关系.结果表明,共筛选出6个主要的水环境因子,分别为流量（Flow）、溶解氧（DO）、栖息地质量指数（QHEI）、电导率（Cond）、化学需氧量（COD）和总氮（TN）.黄河区Flow、DO、QHEI和水生生物丰富度均较高,小清河区COD、TN、Cond和水生生物丰富度最低.黄河区Cond与鱼类丰富度呈显著相关,城区TN与底栖动物丰富度呈显著相关,小清河区COD、DO和QHEI对水生生物丰富度有显著影响,徒骇马颊河区TN对水生生物丰富度有显著影响.该研究为济南市水生态修复方案的制定提供参考,也为其他城市水生态文明建设提供一种思路.  相似文献   

8.
水生植被对于维持水生态系统结构和功能稳定性具有举足轻重的作用,而重建水生植物被认为是污染湖泊生态修复的重要手段.氮素是水生态系统重要的限制性元素之一,根着挺水植物生长发育无疑将深刻地影响着沉积物氮的迁移转化过程,但水生植物不同生长阶段对沉积物氮的需求和植物代谢强度均不同,目前对挺水植物完整生长过程中沉积物氮组分及含量变化认识仍十分不足.本研究通过为期120d的沉积物柱芯培养和水槽模拟试验,探究巢湖芦苇恢复完整生长过程中沉积物总氮(TN)、无机氮(TIN)与可转化态氮(TF-N)的变化及其关键调控因子.结果表明,芦苇完整生长过程将持续激发沉积物氮活性,沉积物TIN与TF-N含量逐渐增加,而沉积物TN和非可转化态氮(NTF-N)含量显著降低.模拟试验期间,指数型增长的芦苇生物量提高了沉积物铵态氮(NH_4~+-N)和硝态氮(NO_3~--N)含量,但亚硝态氮(NO_2~--N)含量却逐渐降低;与第0天相比,第120天沉积物离子交换态氮(IEF-N)、碳酸盐结合态氮(CF-N)、铁锰氧化态氮(IMOF-N)和有机态及硫化物结合态氮(OSF-N)含量分别增加了 1.10、3.40、3.60和1.40倍,这主要受芦苇吸收利用、根系代谢强化根际沉积物氧化还原电势和改变pH微环境共同驱动.在第120天,沉积物NH_4~+-N和NO_3~--N含量急剧升高,分别是第90天的9.43和2.22倍,表明芦苇衰亡凋落过程将向沉积物释放大量的TIN,故需要综合采取湖泊物理—生态工程手段来有效管控芦苇枯落物,从而提升水生植被修复效果并构建长效稳态机制.  相似文献   

9.
A nitrogen mass balance, realized for the lower Oglio River basin (Po River Plain, northern Italy), suggested an elevated impact of agricultural activities in this watershed. Livestock manure, synthetic fertilizers, biological fixation, atmospheric deposition, and wastewater sludge contributed 51, 34, 12, 2, and 1% of total N (TN) input, respectively (basin average 450 kg N ha?1 arable land (AL) year?1, overall input 100 115 t N year?1). Crop uptake, ammonia volatilization and denitrification in soils contributed 65, 21, and 14%, respectively, of TN output (basin average 270 kg N ha?1 AL year?1, overall output 60 060 t N year?1). N inputs exceeded outputs by 40 056 t N year?1, resulting in a basin average surplus of about 180 kg N ha?1 AL year?1. About 34% of the N surplus was exported annually from the basin while the remaining amount (about 26 800 t N year?1) underwent other unaccounted for processes within the watershed. The relevance of nitrogen removal via denitrification in aquatic compartments within the watershed was evaluated. Denitrification in the secondary drainage network can represent a relevant nitrogen sink due to great linear extension (over 12 500 km), with estimated nitrogen loss up to 8500 t N year?1. Denitrification in the riverbed and in perifluvial wetlands have the potential to remove only a small fraction of the nitrogen surplus (<3%). Evidence suggests the relevance of groundwater as a site of nitrogen accumulation.  相似文献   

10.
Although acidifying deposition in western North America is lower than in many parts of the world, many high‐elevation ecosystems there are extremely sensitive to acidification. Previous studies determined that the Mount Zirkel Wilderness Area (MZWA) has the most acidic snowpack and aquatic ecosystems that are among the most sensitive in the region. In this study, spatial and temporal variability of ponds and lakes in and near the MZWA were examined to determine their sensitivity to acidification and the effects of acidic deposition during and after snowmelt. Within the areas identified as sensitive to acidification based on bedrock types, there was substantial variability in acid‐neutralizing capacity (ANC), which was related to differences in hydrological flowpaths that control delivery of weathering products to surface waters. Geological and topographic maps were of limited use in predicting acid sensitivity because their spatial resolution was not fine enough to capture the variability of these attributes for lakes and ponds with small catchment areas. Many of the lakes are sensitive to acidification (summer and autumn ANC < 100 µeq L?1), but none of them appeared to be threatened immediately by episodic or chronic acidification. In contrast, 22 ponds had minimum ANC < 30 µeq L?1, indicating that they are extremely sensitive to acidic deposition and could be damaged by episodic acidification, although net acidity (ANC < 0) was not measured in any of the ponds during the study. The lowest measured pH value was 5·4, and pH generally remained less than 6·0 throughout early summer in the most sensitive ponds, indicating that biological effects of acidification are possible at levels of atmospheric deposition that occurred during the study. The aquatic chemistry of lakes was dominated by atmospheric deposition and biogeochemical processes in soils and shallow ground water, whereas the aquatic chemistry of ponds was also affected by organic acids and biogeochemical processes in the water column and at the sediment–water interface. These results indicate that conceptual and mechanistic acidification models that have been developed for lakes and streams may be inadequate for predicting acidification in less‐understood systems such as ponds. Copyright © 2004 John Wiley & Sons, Ltd.  相似文献   

11.
水库水体污染控制及富营养化防治是保障城市原水供应安全的重要环节.本研究针对金泽水源水库太浦河来水氮、磷浓度较高的特点,自行设计建设了5个面积均为240 m~2的生态净化模拟试验池(A、B、C、D和对照)开展模拟试验,研究了不同水库形态、水生植物种植面积比例及种植方式对水体氮、磷污染物去除的影响.结果表明,通过模拟试验池的生态净化,原水中铵态氮(NH_4~+-N)、总磷(TP)和总氮(TN)的平均去除率分别为50.36%、53.73%和22.25%,C池TN和NH_4~+-N去除率最高分别达到了24.97%和54.61%,D池TP去除率最高,达到62.16%,水体溶解氧(DO)平均浓度提高了1.11 mg/L,平均透明度提高了27.6 cm,均显著高于对照池.水库形态结构、水生植物面积比例及种植方式对水体氮、磷污染物净化效果影响明显,增大水库浅水区面积能有效提高对水体氮、磷污染物的去除能力,增加水生植物种植面积能有效提高水体氮污染物去除和DO、透明度的提升能力,采用浮床种植方式能有效提高水体磷污染物去除和透明度提升能力.本研究结果能为金泽水源水库及其他类似水库的设计和建设提供科学依据.  相似文献   

12.
The European Union's Water Framework Directive (WFD) requires that all Member States within the European Union determine reference conditions for aquatic ecosystems to provide a baseline against which to measure the effects of past and present activities. Reference conditions are subsequently used to classify the ecological status of European waters. The decisions regarding environmental status will be important future elements in the management of European coastal waters. We have developed a number of classification scenarios for total nitrogen (TN) in the overlying waters of the southern part of Roskilde Fjord, Denmark, taking as our basis a palaeoecological reconstruction of fluctuations in TN between 1850 and 1995. We present a provisional classification scheme for the ecological status of Roskilde Fjord, sensu the WFD. Decision(s) regarding the deviation from reference conditions will give a wide range of apparent ecological status from good, through moderate and poor, to bad depending upon the definition of an acceptable deviation from reference conditions. The determination of an acceptable deviation will ultimately be a political decision, and will result in a wide range in the protection of coastal waters in Europe. There is still, however, an urgent need for a sound scientific documentation of the various scenarios for the implementation of the WFD.  相似文献   

13.
基于洱海水生态特征的流域最大日负荷总量控制   总被引：1，自引：1，他引：0  
基于洱海水生态历史数据及现状资料,采用概率密度分布曲线法及水生生物基准相结合的方式计算洱海总氮(TN)、总磷(TP)、高锰酸盐指数(COD_(Mn))和氨氮(NH_3-N)的控制目标,目标值分别为0.36、0.026、4和0.28 mg/L.再根据该水质目标,得到洱海的最大日负荷(TMDL)总量.TMDL总量采用线性规划法计算,其中污染物响应系数矩阵通过MIKE 21二维水质模型计算所得.安全容余(MOS)则通过一阶误差分析法确定.经过一系列的计算,最终确定洱海的TMDL总量控制计划.计算结果表明,洱海TN、TP、COD_(Mn)和NH_3-N的TMDL总量分别为2005.989、149.671、19258.844和1348.119 kg/d,其MOS所占比例分别为6.152%、5.570%、4.380%和5.021%,表明洱海农业面源污染为该流域主要的污染形式,其允许最大排放量约占全部允许排放量的90%左右.  相似文献   

14.
The simulation of karstic aquifers is difficult using traditional groundwater numerical simulators, as the exact knowledge of the hydraulic characteristics of the physical system in small scale is rarely available and the numerical simulators produce results of limited reliability. In the present work, artificial neural networks (ANNs) are utilized to predict the response of a karstic aquifer, using the hydraulic head change per time step rather than the hydraulic head itself as output parameter of the network. As it will be demonstrated, in the first case a better approximation of the physical system's response is achieved as the change of the hydraulic head is more naturally connected to the input parameters of the network, which model the aquatic equilibrium of the system. The correlation of rainfall and hydraulic head change per time step was initially used to determine the time lag of the rainfall input data, which represents the time needed by the rainfall to percolate and reach the water table. In a second step, a differential evolution (DE) algorithm is utilized for the optimal selection of rainfall time lag as well as ANN's architecture and training parameters. Although a time consuming procedure, the improvement obtained suggests that the empirical determination of the ANN parameters and structure is not always sufficient and an optimization procedure, which minimizes the training and evaluation errors of the ANN, may provide substantially better simulation results. The optimized networks were finally used for midterm predictions (30 to 90 days ahead) of the hydraulic head, showing the ability of the ANN with hydraulic head change as output parameter to provide predictions with high accuracy at the end of the considered time period. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

15.
In the Rhode River estuarine/watershed area, increased acidity of precipitation from atmospheric acidic deposition has deleterious effects on the freshwater ecosystems. One of the characteristics of an acidic watershed is the mobilization of aluminum from soils to aquatic environment. Increased concentrations of aluminum in surface waters are toxic to living organisms. Detection of long-term changes of acidity and elevated Al concentrations in surface and soil waters is a central issue. In this present paper, the dynamics ofAl speciation in the shallow ground waters from Rhode River watershed 110 (la) were investigated. This research provides a unique, regional analysis of important controls on the transport of Al speciation through the rural watershed of the Chesapeake Bay.  相似文献   

16.
An application of the artificial neural network (ANN) approach for predicting mean grain size using electric resistivity data from Bam city is presented. A feed forward back propagation network was developed employing 45 sets of input data. The input variables in the ANN model are the electrical resistivity, water table as a Boolean value and depth; the output is the mean grain size. To demonstrate the authenticity of this approach, the network predictions are compared with those from interpolation methods and the same data. This comparison shows that the ANN approach performs better results. The predicted and observed mean grain size values were compared and show high correlation coefficients. The ANN approach maps show a high degree of correlation with well data based grain size maps and can therefore be used conservatively to better understand the influence of input parameters on sedimentological predictions.  相似文献   

17.
A generalized watershed model was used to evaluate the effects of global climate changes on the hydrologic responses of freshwater ecosystems. The Enhanced Trickle Down (ETD) model was applied to W-3 watershed located near Danville, Vermont. Eight years of field data was used to perform model calibration and verification and the results were presented in Nikolaidis et al., (1993). Results from the Goddard Institute for Space Studies (GISS) and the Geophysical Fluid Dynamics Laboratory (GFDL) general circulation models which simulated the doubling of present day atmospheric CO2 scenarios were used to perform the hydrologic simulations for the W-3 watershed. The results indicate that the W-3 watershed will experience increases in annual evapotranspiration and decreases in annual outflow and soil moisture. Stochastic models that simulate collective statistical properties of meteorological time series were developed to generate data to drive the ETD model in a Monte-Carlo fashion for quantification of the uncertainty in the model predictions due to input time series. This coupled deterministic and stochastic model was used to generate probable scenarios of future hydrology of the W-3 watershed. The predicted evapotranspiration and soil moisture under doubling present day atmospheric CO2 scenarios exceed the present day uncertainty due to input time series by a factor greater than 2. The results indicate that the hydrologic response of the W-3 watershed will be significantly different than its present day response. The Enhanced Trickle Down model can be used to evaluate land surface feedbacks and assessing water quantity management in the event of climate change.  相似文献   

18.
The Turkey Lakes Watershed (TLW) study is a federal, interdepartmental study established in 1979 to investigate the effects of acid rain on terrestrial and aquatic ecosystems. The 10.5 km2 watershed, located in the Eastern Temperate Mixed Forest on the Canadian Shield, has been the site of multidisciplinary studies on biogeochemical and ecological processes conducted across plot to catchment scales. The whole-ecosystem investigative approach was adopted from the outset and has allowed research to evolve from its original (and continuing) acidification focus to include investigations on the effects of climate change, forest harvesting and other forest ecosystem perturbations. The extensive scientific and support infrastructure allows for collection of a comprehensive data record essential for understanding long-term environmental trends. Data include atmospheric deposition, meteorology, stream hydrology and chemistry, soil, pore and ground water properties, understory and overstory vegetation, lake and outflow physical and chemical properties, and aquatic macroinvertebrate and fish community composition and abundance. These data have contributed to over 400 published research papers and graduate theses. The watershed has also figured prominently in many continent-wide comparisons advancing fundamental watershed theory. The knowledge gained at TLW has influenced pollutant emission and natural resource management policies provincially, nationally and internationally.  相似文献   

19.
白洋淀是雄安新区的核心生态功能区.为探究白洋淀不同植物群落区表层沉积物碳(C)氮(N)磷(P)化学计量特征,采集了96组表层沉积物样品开展对比分析.研究表明:白洋淀湿地表层沉积物总有机碳(TOC)含量均值为39.64 g/kg,范围为14.4～ 136.82 g/kg,总氮(TN)和总磷(TP)均值分别为2.62和0....  相似文献   

20.
Although artificial neural networks (ANNs) have been applied in rainfall runoff modelling for many years, there are still many important issues unsolved that have prevented this powerful non‐linear tool from wide applications in operational flood forecasting activities. This paper describes three ANN configurations and it is found that a dedicated ANN for each lead‐time step has the best performance and a multiple output form has the worst result. The most popular form with multiple inputs and single output has the average performance. In comparison with a linear transfer function (TF) model, it is found that ANN models are uncompetitive against the TF model in short‐range predictions and should not be used in operational flood forecasting owing to their complicated calibration process. For longer range predictions, ANN models have an improved chance to perform better than the TF model; however, this is highly dependent on the training data arrangement and there are undesirable uncertainties involved, as demonstrated by bootstrap analysis in the study. To tackle the uncertainty issue, two novel approaches are proposed: distance analysis and response analysis. Instead of discarding the training data after the model's calibration, the data should be retained as an integral part of the model during its prediction stage and the uncertainty for each prediction could be judged in real time by measuring the distances against the training data. The response analysis is based on an extension of the traditional unit hydrograph concept and has a very useful potential to reveal the hydrological characteristics of ANN models, hence improving user confidence in using them in real time. Copyright © 2006 John Wiley & Sons, Ltd.  相似文献   

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