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1.
Most hillslope studies examining the interplay between climate and earth surface processes tend to be biased towards eroding parts of landscapes. This limitation makes it difficult to assess how entire upland landscapes, which are mosaics of eroding and depositional areas, evolve physio‐chemically as a function of climate. Here we combine new soil geochemical data and published 10Be‐derived soil production rates to estimate variations in chemical weathering across two eroding‐to‐depositional hillslopes spanning a climate gradient in southeastern Australia. At the warmer and wetter Nunnock River (NR) site, rates of total soil (–3 to –14 g m‐2 yr‐1; negative sign indicates mass loss) and saprolite (–18 to –32 g m‐2 yr‐1) chemical weathering are uniform across the hillslope transect. Alternatively, the drier hillslope at Frog's Hollow (FH) is characterized by contrasting weathering patterns in eroding soils (–30 to –53 g m‐2 yr‐1) vs. depositional soils (+91 g m‐2 yr‐1; positive sign indicates mass addition). This difference partly reflects mineral grain size sorting as a result of upslope bioturbation coupled with water‐driven soil erosion, as well as greater vegetative productivity in moister depositional soils. Both of these processes are magnified in the drier climate. The data reveal the importance of linking the erosion–deposition continuum in hillslope weathering studies in order to fully capture the coupled roles of biota and erosion in driving the physical and chemical evolution of hillslopes. Our findings also highlight the potential limitations of applying current weathering models to landscapes where particle‐sorting erosion processes are active. Copyright © 2018 John Wiley & Sons, Ltd.  相似文献   

2.
Landscapes evolve in response to external forces, such as tectonics and climate, that influence surface processes of erosion and weathering. Internal feedbacks between erosion and weathering also play an integral role in regulating the landscapes response. Our understanding of these internal and external feedbacks is limited to a handful of field‐based studies, only a few of which have explicitly examined saprolite weathering. Here, we report rates of erosion and weathering in saprolite and soil to quantify how climate influences denudation, by focusing on an elevation transect in the western Sierra Nevada Mountains, California. We use an adapted mass balance approach and couple soil‐production rates from the cosmogenic radionuclide (CRN) 10Be with zirconium concentrations in rock, saprolite and soil. Our approach includes deep saprolite weathering and suggests that previous studies may have underestimated denudation rates across similar landscapes. Along the studied climate gradient, chemical weathering rates peak at middle elevations (1200–2000 m), averaging 112·3 ± 9·7 t km–2 y–1 compared to high and low elevation sites (46·8 ± 5·2 t km?2 y?1). Measured weathering rates follow similar patterns with climate as those of predicted silica fluxes, modeled using an Arrhenius temperature relationship and a linear relationship between flux and precipitation. Furthermore, chemical weathering and erosion are tightly correlated across our sites, and physical erosion rates increase with both saprolite weathering rates and intensity. Unexpectedly, saprolite and soil weathering intensities are inversely related, such that more weathered saprolites are overlain by weakly weathered soils. These data quantify exciting links between climate, weathering and erosion, and together suggest that climate controls chemical weathering via temperature and moisture control on chemical reaction rates. Our results also suggest that saprolite weathering reduces bedrock coherence, leading to faster rates of soil transport that, in turn, decrease material residence times in the soil column and limit soil weathering. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

3.
Soil‐covered upland landscapes constitute a critical part of the habitable world. Our understanding of how they evolve as a function of different climatic, tectonic and geological regimes is important across a wide range of disciplines and depends, in part, on understanding the links between chemical and physical weathering processes. Extensive previous work has shown that soil production rates decrease with increasing soil column thickness, but chemical weathering rates were not measured. Here we examine a granitic, soil‐mantled hillslope at Point Reyes, California, where soil production rates were determined using in situ produced cosmogenic nuclides (10Be and 26Al), and we quantify the extent as well as the rates of chemical weathering of the saprolite from beneath soil from across the landscape. We collected saprolite samples from the base of soil pits and analysed them for abrasion pH as well as for major and trace elements by X‐ray fluorescence spectroscopy, and for clay mineralogy by X‐ray diffraction spectroscopy. Our results show for the first time that chemical weathering rates decrease with increasing soil thickness and account for 13 to 51 per cent of total denudation. We also show that spatial variation in chemical weathering appears to be topographically controlled: weathering rate decreases with slope across the divergent ridge and increases with upslope contributing area in the convergent swale. Furthermore, to determine the best measure for the extent of saprolite weathering, we compared four different chemical weathering indices – the Vogt ratio, the chemical index of alteration (CIA), Parker's index, and the silicon–aluminium ratio – with saprolite pH. Measurements of the CIA were the most closely correlated with saprolite pH, showing that weathering intensity decreases linearly with an increase in saprolite pH from 4·7 to almost 7. Data presented here are among the first to couple directly rates of soil production and chemical weathering with how topography is likely to control weathering at a hillslope scale. Copyright © 2006 John Wiley & Sons, Ltd.  相似文献   

4.
Landscapes in areas of active uplift and erosion can only remain soil‐mantled if the local production of soil equals or exceeds the local erosion rate. The soil production rate varies with soil depth, hence local variation in soil depth may provide clues about spatial variation in erosion rates. If uplift and the consequent erosion rates are sufficiently uniform in space and time, then there will be tendency toward equilibrium landforms shaped by the erosional processes. Soil mantle thickness would adjust such that soil production matched the erosion. Previous work in the Oregon Coast Range suggested that there may be a tendency locally toward equilibrium between hillslope erosion and sediment yield. Here results from a new methodology based on cosmogenic radionuclide accumulation in bedrock minerals at the base of the soil column are reported. We quantify how soil production varies with soil thickness in the southern Oregon Coast Range and explore further the issue of landscape equilibrium. Apparent soil production is determined to be an inverse exponential function of soil depth, with a maximum inferred production rate of 268 m Ma?1 occurring under zero soil depth. This rate depends, however, on the degree of weathering of the underlying bedrock. The stochastic and large‐scale nature of soil production by biogenic processes leads to large temporal and spatial variations in soil depth; the spatial variation of soil depth neither supports nor rejects equilibrium morphology. Our observed catchment‐averaged erosion rate of 117 m Ma?1 is, however, similar to that estimated for the region by others, and to soil production rates under thin and intermediate soils typical for the steep ridges. We suggest that portions of the Oregon Coast Range may be eroding at roughly the same rate, but that local competition between drainage networks and episodic erosional events leads to landforms that are out of equilibrium locally and have a spatially varying soil mantle. Copyright © 2001 John Wiley & Sons, Ltd.  相似文献   

5.
Soil depth and soil production are highly complicated phenomena, generated from a complex interaction of physical, biological and chemical processes. It has, nevertheless, become increasingly clear that soil formation rates are closely related to chemical weathering rates. Somewhat paradoxically, it is likewise becoming apparent that such biogeochemical reactions as slowly transform rock to soil are limited by physical processes, such as flowing water and the formation of fractures. We have formulated a theoretical approach that relates soil formation rates to chemical weathering rates, and those, likewise, to solute transport rates. For such a theoretical framework to be relevant, the solute transport rates cannot equal those of the flowing water, as is the case in Gaussian solute transport. Rather, solute transport must be slowed in accordance with heavy‐tailed solute arrival time distributions. The inference is that the traditional advection–dispersion equation formulation for solute transport is inadequate in the typically heterogeneous geological media that weather to form soils. Here we examine the implications of this soil production model on the assumption of the approach to steady state. Particularly at slow erosion rates we find that many soil columns are not in equilibrium. This tendency may be accentuated in dry climates. Copyright © 2017 John Wiley & Sons, Ltd.  相似文献   

6.
Cosmogenic nuclides in rock, soil, and sediment are routinely used to measure denudation rates of catchments and hillslopes. Although it has been shown that these measurements are prone to biases due to chemical erosion in regolith, most studies of cosmogenic nuclides have ignored this potential source of error. Here we quantify the extent to which overlooking effects of chemical erosion introduces bias in interpreting denudation rates from cosmogenic nuclides. We consider two end‐member effects: one due to weathering near the surface and the other due to weathering at depth. Near the surface, chemical erosion influences nuclide concentrations in host minerals by enriching (or depleting) them relative to other more (or less) soluble minerals. This increases (or decreases) their residence times relative to the regolith as a whole. At depth, where minerals are shielded from cosmic radiation, chemical erosion causes denudation without influencing cosmogenic nuclide buildup. If this effect is ignored, denudation rates inferred from cosmogenic nuclides will be too low. We derive a general expression, termed the ‘chemical erosion factor’, or CEF, which corrects for biases introduced by both deep and near‐surface chemical erosion in regolith. The CEF differs from the ‘quartz enrichment factor’ of previous work in that it can also be applied to relatively soluble minerals, such as olivine. Using data from diverse climatic settings, we calculate CEFs ranging from 1.03 to 1.87 for cosmogenic nuclides in quartz. This implies that ignoring chemical erosion can lead to errors of close to 100% in intensely weathered regolith. CEF is strongly correlated with mean annual precipitation across our sites, reflecting climatic influence on chemical weathering. Our results indicate that quantifying CEFs is crucial in cosmogenic nuclide studies of landscapes where chemical erosion accounts for a significant fraction of the overall denudation. Copyright © 2012 John Wiley & Sons, Ltd.  相似文献   

7.
Spatially discontinuous permafrost conditions frequently occur in the European Alps. How soils under such conditions have evolved and how they may react to climate warming is largely unknown. This study focuses on the comparison of nearby soils that are characterised by the presence or absence of permafrost (active‐layer thickness: 2–3 m) in the alpine (tundra) and subalpine (forest) range of the Eastern Swiss Alps using a multi‐method (geochemical and mineralogical) approach. Moreover, a new non‐steady‐state concept was applied to determine rates of chemical weathering, soil erosion, soil formation, soil denudation, and soil production. Long‐term chemical weathering rates, soil formation and erosion rates were assessed by using immobile elements, fine‐earth stocks and meteoric 10Be. In addition, the weathering index (K + Ca)/Ti, the amount of Fe‐ and Al‐oxyhydroxides and clay minerals characteristics were considered. All methods indicated that the differences between permafrost‐affected and non‐permafrost‐affected soils were small. Furthermore, the soils did not uniformly differ in their weathering behaviour. A tendency towards less intense weathering in soils that were affected by permafrost was noted: at most sites, weathering rates, the proportion of oxyhydroxides and the weathering stage of clay minerals were lower in permafrost soils. In part, erosion rates were higher at the permafrost sites and accounted for 79–97% of the denudation rates. In general, soil formation rates (8.8–86.7 t/km2/yr) were in the expected range for Alpine soils. Independent of permafrost conditions, it seems that the local microenvironment (particularly vegetation and subsequently soil organic matter) has strongly influenced denudation rates. As the climate has varied since the beginning of soil evolution, the conditions for soil formation and weathering were not stable over time. Soil evolution in high Alpine settings is complex owing to, among others, spatio‐temporal variations of permafrost conditions and thus climate. This makes predictions of future behaviour very difficult. Copyright © 2016 John Wiley & Sons, Ltd.  相似文献   

8.
This study presents a semi-empirical model for quantifying the reduction in the mechanical strength of bedrock beneath actively eroding soil-mantled hillslopes. The strength reduction of bedrock controls the rate of physical disintegration of saprolite, which supplies fresh minerals that are then exposed to intense chemical weathering in soil sections. To determine the values of parameters employed in the model requires knowledge of the denudation rate of the hillslope, the thickness of the soil and saprolite layers, the strength of fresh bedrock, and the threshold strength for physical erosion at the uppermost face of the saprolite. These parameters can be obtained from cosmogenic nuclide analyses for quartz samples from the soil–saprolite boundary and basic field- and laboratory-based investigations. Further testing of the model within a diverse range of climatic, tectonic, and lithologic environments is likely to provide clues to the mechanisms responsible for local and regional variations in the rates of soil production and chemical weathering upon hillslopes.  相似文献   

9.
Soil-covered upland landscapes comprise a critical part of the habitable world and our understanding of their evolution as a function of different climatic, tectonic, and geologic regimes is important across a wide range of disciplines. Soil production and transport play essential roles in controlling the spatial variation of soil depth and therefore hillslope hydrological processes, distribution of vegetation, and soil biological activity. Field-based confirmation of the hypothesized relationship between soil thickness and soil production is relatively recent, however, and here we quantify a direct, material strength-based influence on variable soil production across landscapes. We report clear empirical linkages between the shear strength of the parent material (its erodibility) and the overlying soil thickness. Specifically, we use a cone penetrometer and a shear vane to determine saprolite resistance to shear. We find that saprolite shear strength increases systematically with overlying soil thickness across three very different field sites where we previously quantified soil production rates. At these sites, soil production rates, determined from in situ produced beryllium-10 (10Be) and aluminum-26 (26Al), decrease with overlying soil thickness and we therefore infer that the efficiency of soil production must decrease with increasing parent material shear strength. We use our field-based data to help explain the linkages between biogenic processes, chemical weathering, hillslope hydrology, and the evolution of the Earth's surface. © 2019 John Wiley & Sons, Ltd.  相似文献   

10.
We report erosion rates and processes, determined from in situ‐produced beryllium‐10 (10Be) and aluminum‐26 (26Al), across a soil‐mantled landscape of Arnhem Land, northern Australia. Soil production rates peak under a soil thickness of about 35 cm and we observe no soil thicknesses between exposed bedrock and this thickness. These results thus quantify a well‐defined ‘humped’ soil‐production function, in contrast to functions reported for other landscapes. We compare this function to a previously reported exponential decline of soil production rates with increasing soil thickness across the passive margin exposed in the Bega Valley, south‐eastern Australia, and found remarkable similarities in rates. The critical difference in this work was that the Arnhem Land landscapes were either bedrock or mantled with soils greater than about 35 cm deep, with peak soil production rates of about 20 m/Ma under 35–40 cm of soil, thus supporting previous theory and modeling results for a humped soil production function. We also show how coupling point‐specific with catchment‐averaged erosion rate measurements lead to a better understanding of landscape denudation. Specifically, we report a nested sampling scheme where we quantify average erosion rates from the first‐order, upland catchments to the main, sixth‐order channel of Tin Camp Creek. The low (～5 m/Ma) rates from the main channel sediments reflect contributions from the slowly eroding stony highlands, while the channels draining our study area reflect local soil production rates (～10 m/Ma off the rocky ridge; ～20 m/Ma from the soil mantled regions). Quantifying such rates and processes help determine spatial variations of soil thickness as well as helping to predict the sustainability of the Earth's soil resource under different erosional regimes. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

11.
It has been hypothesized that many soil profiles reach a steady‐state thickness. In this work, such profiles were simulated using a one‐dimensional model of reaction with advective and diffusive solute transport. A model ‘rock’ is considered, consisting of albite that weathers to kaolinite in the presence of chemically inert quartz. The model yields three different steady‐state regimes of weathering. At the lowest erosion rates, a local‐equilibrium regime is established where albite is completely depleted in the weathering zone. This regime is equivalent to the transport‐limited regime described in the literature. With an increase in erosion rate, transition and kinetic regimes are established. In the transition regime, both albite and kaolinite are present in the weathering zone, but albite does not persist to the soil–air interface. In the weathering‐limited regime, here called the kinetic regime, albite persists to the soil–air interface. The steady‐state thickness of regolith decreases with increasing erosion rate in the local equilibrium and transition regimes, but in the kinetic regime, this thickness is independent of erosion rate. Analytical expressions derived from the model are used to show that regolith production rates decrease exponentially with regolith thickness. The steady‐state regolith thickness increases with the Darcy velocity of the pore fluid, and in the local equilibrium regime may vary markedly with small variations in this velocity and erosion rate. In the weathering‐limited regime, the temperature dependences for chemical weathering rates are related to the activation energy for the rate constant for mineral reaction and to the ΔH of dissolution, while for local equilibrium regimes they are related to the ΔH only. The model illustrates how geochemical and geomorphological observations are related for a simple compositional system. The insights provided will be useful in interpreting natural regolith profiles. Copyright © 2010 John Wiley & Sons, Ltd.  相似文献   

12.
Knowing little about how porosity and permeability are distributed at depth, we commonly develop models of groundwater by treating the subsurface as a homogeneous black box even though porosity and permeability vary with depth. One reason for this depth variation is that infiltrating meteoric water reacts with minerals to affect porosity in localized zones called reaction fronts. We are beginning to learn to map and model these fronts beneath headwater catchments and show how they are distributed. The subsurface landscapes defined by these fronts lie subparallel to the soil-air interface but with lower relief. They can be situated above, below, or at the water table. These subsurface landscapes of reaction are important because porosity developed from weathering can control subsurface water storage. In addition, porosity often changes at the weathering fronts, and when this affects permeability significantly, the front can act like a valve that re-orients water flowing through the subsurface. We explore controls on the positions of reaction fronts under headwater landscapes by accounting for the timescales of erosion, chemical equilibration, and solute transport. One strong control on the landscape of subsurface reaction is the land surface geometry, which is in turn a function of the erosion rate. In addition, the reaction fronts, like the water table, are strongly affected by the lithology and water infiltration rate. We hypothesize that relationships among the land surface, reaction fronts, and the water table are controlled by feedbacks that can push landscapes towards an ‘ideal hill’. In this steady state, reaction-front valves partition water volumes into shallow and deep flowpaths. These flows dissolve low- and high-solubility minerals, respectively, allowing their reaction fronts to advance at the erosion rate. This conceptualization could inform better models of subsurface porosity and permeability, replacing the black box.  相似文献   

13.
Investigations to understand linkages among climate, erosion and weathering are central to quantifying landscape evolution. We approach these linkages through synthesis of regolith data for granitic terrain compiled with respect to climate, geochemistry, and denudation rates for low sloping upland profiles. Focusing on Na as a proxy for plagioclase weathering, we quantified regolith Na depletion, Na mass loss, and the relative partitioning of denudation to physical and chemical contributions. The depth and magnitude of regolith Na depletion increased continuously with increasing water availability, except for locations with mean annual temperature < 5 °C that exhibited little Na depletion, and locations with physical erosion rates < 20 g m? 2 yr? 1 that exhibited deep and complete regolith Na depletion. Surface Na depletion also tended to decrease with increasing physical erosion. Depth-integrated Na mass loss and regolith depth were both three orders of magnitude greater in the fully depleted, low erosion rate sites relative to other locations. These locations exhibited strong erosion-limitation of Na chemical weathering rates based on correlation of Na chemical weathering rate to total Na denudation. Sodium weathering rates in cool locations with positive annual water balance were strongly correlated to total Na denudation and precipitation, and exhibited an average apparent activation energy (Ea) of 69 kJ mol? 1 Na. The remaining water-limited locations exhibited kinetic limitation of Na weathering rates with an Ea of 136 kJ mol? 1 Na, roughly equivalent to the sum of laboratory measures of Ea and dissolution reaction enthalpy for albite. Water availability is suggested as the dominant factor limiting rate kinetics in the water-limited systems. Together, these data demonstrate marked transitions and nonlinearity in how climate and tectonics correlate to plagioclase chemical weathering and Na mass loss.  相似文献   

14.
The ridgelines of mountain ranges are a source of geomorphic information unadulterated by the arrival of sediment from upslope. Studies along ridgecrests, therefore, can help identify and isolate the controls on important regolith properties such as thickness and texture. A 1.5 km section of ridgeline in the Sierra Nevada (CA) with a tenfold decrease in erosion rate (inferred from ridgetop convexity) provided an opportunity to conduct a high‐resolution survey of regolith properties and investigate their controls. We found that regolith along the most quickly eroding section of the ridge was the rockiest and had the lowest clay concentrations. Furthermore, a general increase in regolith thickness with a slowing of erosion rate was accompanied by an increase in biomass, changes in vegetation community, broader ridgeline profiles, and an apparent increase in total available moisture. The greatest source of variation in regolith thickness at the 10–100 m scale, however, was the local topography along the ridgeline, with the deepest regolith in the saddles and the thinnest on the knobs. Because regolith in the saddles had higher surface soil moisture than the knobs, we conclude that the hydrological conditions primarily driven by local topography (i.e. rapid vs. slow drainage and water‐storage potential) provide the fundamental controls on regolith thickness through feedbacks incorporating physical weathering by the biota and chemical weathering. Moreover, because the ridgeline saddles are the uppermost extensions of first‐order valleys, we propose that the fluvial network affects regolith properties in the furthest reaches of the watershed. Copyright © 2015 John Wiley & Sons, Ltd.  相似文献   

15.
Past variations in climate and tectonics have led to spatially and temporally varying erosion rates across many landscapes. In this contribution I examine methods for detecting and quantifying the nature and timing of transience in eroding landscapes. At a single location, cosmogenic nuclides can detect the instantaneous removal of material or acceleration of erosion rates over millennial timescales using paired nuclides. Detection is possible only if one of the nuclides has a significantly shorter half‐life than the other. Currently, the only practical way of doing this is to use cosmogenic in situ carbon‐14 (14C) alongside a longer lived nuclide, such as beryllium‐10 (10Be). Hillslope information can complement or be used in lieu of cosmogenic information: in soil mantled landscapes, increased erosion rates can be detected for millennia after the increase by comparing relief and ridgetop curvature. This technique will work as long as the final erosion rate is greater than twice the initial rate. On a landscape scale, transience may be detected based upon disequilibria in channel profiles or ridgetops, but transience can be sensitive to the nature of transient forcing. Where forcing is periodic, landscapes display differing behavior if forcing is driven by changes in base level lowering rates versus changes in the efficiency of either channel or hillslope erosion (e.g. driven by climate change). Oscillations in base level lowering lead to basin averaged erosion rates that reflect a long term average erosion rate despite strong spatial heterogeneity in local erosion rates. This averaging is reflected in 10Be concentrations in stream sediments. Changes in hillslope sediment transport coefficients can lead to large fluctuations in basin averaged erosion rates, which again are reflected in 10Be concentrations. The variability of erosion rates in landscapes where both the sediment transport and channel erodibility coefficients vary is dominated by changes to the hillslope transport coefficient. Copyright © 2016 John Wiley & Sons, Ltd.  相似文献   

16.
The evolution of volcanic landscapes and their landslide potential are both dependent upon the weathering of layered volcanic rock sequences. We characterize critical zone structure using shallow seismic Vp and Vs profiles and vertical exposures of rock across a basaltic climosequence on Kohala peninsula, Hawai’i, and exploit the dramatic gradient in mean annual precipitation (MAP) across the peninsula as a proxy for weathering intensity. Seismic velocity increases rapidly with depth and the velocity–depth gradient is uniform across three sites with 500–600 mm/yr MAP, where the transition to unaltered bedrock occurs at a depth of 4 to 10 m. In contrast, velocity increases with depth less rapidly at wetter sites, but this gradient remains constant across increasing MAP from 1000 to 3000 mm/yr and the transition to unaltered bedrock is near the maximum depth of investigation (15–25 m). In detail, the profiles of seismic velocity and of weathering at wet sites are nowhere monotonic functions of depth. The uniform average velocity gradient and the greater depths of low velocities may be explained by the averaging of velocities over intercalated highly weathered sites with less weathered layers at sites where MAP > 1000 mm/yr. Hence, the main effect of climate is not the progressive deepening of a near‐surface altered layer, but rather the rapid weathering of high permeability zones within rock subjected to precipitation greater than ~1000 mm/yr. Although weathering suggests mechanical weakening, the nearly horizontal orientation of alternating weathered and unweathered horizons with respect to topography also plays a role in the slope stability of these heterogeneous rock masses. We speculate that where steep, rapidly evolving hillslopes exist, the sub‐horizontal orientation of weak/strong horizons allows such sites to remain nearly as strong as their less weathered counterparts at drier sites, as is exemplified by the 50°–60° slopes maintained in the amphitheater canyons on the northwest flank of the island. Copyright © 2017 John Wiley & Sons, Ltd.  相似文献   

17.
We present a study to estimate the large-scale landscape history of a continental margin, by establishing a source-to-sink volume balance between the eroding onshore areas and the offshore basins. Assuming erosion as the primary process for sediment production, we strive to constrain a numerical model of landscape evolution that balances the volumes of eroded materials from the continent and that deposited in the corresponding basins, with a ratio imposed for loss of erosion products. We use this approach to investigate the landscape history of Madagascar since the Late Cretaceous. The uplift history prescribed in the model is inferred from elevations of planation surfaces formed at various ages. By fitting the volumes of terrigenous sediments in the Morondava Basin along the west coast and the current elevation of the island, the landscape evolution model is optimized by constraining the erosion law parameters and ratios of sediment loss. The results include a best-fit landscape evolution model, which features two major periods of uplift and erosion during the Late Cretaceous and the middle to late Cenozoic. The model supports suggestions from previous studies that most of the high topography of the island was constructed since the middle to late Miocene, and on the central plateau the erosion has not reached an equilibrium with the high uplift rates in the late Cenozoic. Our models also indicate that over the geological time scale a significant portion of materials eroded from Madagascar was not archived in the offshore basin, possibly consumed by chemical weathering, the intensity of which might have varied with climate.  相似文献   

18.
We present a model of chemical reaction within hills to explore how evolving porosity (and by inference, permeability) affects flow pathways and weathering. The model consists of hydrologic and reactive-transport equations that describe alteration of ferrous minerals and feldspar. These reactions were chosen because previous work emphasized that oxygen- and acid-driven weathering affects porosity differently in felsic and mafic rocks. A parameter controlling the order of the fronts is presented. In the absence of erosion, the two reaction fronts move at different velocities and the relative depths depend on geochemical conditions and starting composition. In turn, the fronts and associated changes in porosity drastically affect both the vertical and lateral velocities of water flow. For these cases, estimates of weathering advance rates based on simple models that posit unidirectional constant-velocity advection do not apply. In the model hills, weathering advance rates diminish with time as the Darcy velocities decrease with depth. The system can thus attain a dynamical steady state at any erosion rate where the regolith thickness is constant in time and velocities of both fronts become equal to one another and to the erosion rate. The slower the advection velocities in a system, the faster it attains a steady state. For example, a massive rock with relatively fast-dissolving minerals such as diabase – where solute transport across the reaction front mainly occurs by diffusion – can reach a steady state more quickly than granitoid rocks in which advection contributes to solute transport. The attainment of a steady state is controlled by coupling between weathering and hydrologic processes that force water to flow horizontally above reaction fronts where permeability changes rapidly with depth and acts as a partial barrier to fluid flow. Published 2020. This article is a U.S. Government work and is in the public domain in the USA.  相似文献   

19.
Increased erosion associated with land use change often alters the flux of sediments and nutrients, but few studies have looked at the interaction between these disrupted cycles. We studied the effects of gully erosion on carbon and nitrogen storage in surface soil/sediment and herbaceous vegetation and on C and N mineralization in a headwater catchment used for cattle grazing. We found significantly lower C and N stored in an incising gully compared with an intact valley. This storage was significantly higher in an adjacent stabilizing gully, although not to the levels found in the intact valley. The intact valley had two to four times higher soil/sediment concentrations of total organic C, total N and Colwell extractable P than the incising gully. Lower storage was not explained by differences in vegetation biomass density or silt and clay content. Vegetation accounted for only 8% of C and 2% of N storage. Although not a significant store in itself, vegetation has an important indirect role in restoring and maintaining soil/sediment C and N stocks in eroding areas. We found significant linear relationships between C and N mineralization rates and soil/sediment C and N content, with lower rates occurring in the eroded sediment. These findings support our initial hypothesis that gully erosion reduces C and N storage and mineralization rates in eroding catchments. The implications of this study include a change to the quality of eroded sediments in headwater catchments, causing C‐poorer and N‐poorer sediments to be exported but overall loads to increase. Copyright © 2013 John Wiley & Sons, Ltd.  相似文献   

20.
The clay mineralogy of Tulare Lake sediment was examined to investigate hydroclimatic and environmental changes in the southern Sierra Nevada Mountains (SNM) since the most recent glacial maximum. Evolution of clay mineral assemblages elucidates significant changes in weathering, erosion, and hydroclimatic condition in the catchment. During the last glacial period (24.4–15.1 cal ka BP), low illite content implies less physical erosion of the granitic batholith rocks and a cold and arid environment in the southern SNM. Abrupt increases of illite content at 21.8–20.8 and 17.6 cal ka BP resulted from the glacier advances to the ablation zone and illite-rich glacier flour was transported down to the lake. The gradual increase of smectite induced by progressive depletion of illite-rich glacier flour from 17.6 cal ka BP toward the end of this period indicates climate was beginning to get warm and wet. From 11.9 to 5.3 cal ka BP, two warm and wet periods (10.7–9.4 and 8.2–5.2 cal ka BP) were characterized by high smectite/illite content ratios and low illite crystallinity values, suggesting intensive rainfall precipitation and more physical erosion in the highland and lowland catchment as well as more smectite formation in the terrace soils. Since the last glacial period, physical erosion, in comparison to the chemical weathering, was the dominant process responding to the hydroclimatic change in the Tulare Lake catchment. Moderate to weak chemical weathering was signified by the mostly low illite chemical weathering index of the core sediments. Such results suggest that vegetation cover in the southern SNM was low and limited.  相似文献   

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