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1.
Water draining from a large agricultural catchment of 1 110 km2 in southwest France was sampled over an 18‐month period to determine the temporal variability in suspended sediment (SS) and dissolved (DOC) and particulate organic carbon (POC) transport during flood events, with quantification of fluxes and controlling factors, and to analyze the relationships between discharge and SS, DOC and POC. A total of 15 flood events were analyzed, providing extensive data on SS, POC and DOC during floods. There was high variability in SS, POC and DOC transport during different seasonal floods, with SS varying by event from 513 to 41 750 t; POC from 12 to 748 t and DOC from 9 to 218 t. Overall, 76 and 62% of total fluxes of POC and DOC occurred within 22% of the study period. POC and DOC export from the Save catchment amounted to 3090 t and 1240 t, equivalent to 1·8 t km?2 y?1 and 0·7 t km?2 y?1, respectively. Statistical analyses showed that total precipitation, flood discharge and total water yield were the major factors controlling SS, POC and DOC transport from the catchment. The relationships between SS, POC and DOC and discharge over temporal flood events resulted in different hysteresis patterns, which were used to deduce dissolved and particulate origins. In both clockwise and anticlockwise hysteresis, POC mainly followed the same patterns as discharge and SS. The DOC‐discharge relationship was mainly characterized by alternating clockwise and anticlockwise hysteresis due to dilution effects of water originating from different sources in the whole catchment. Copyright © 2011 John Wiley & Sons, Ltd.  相似文献   

2.
Waterborne carbon (C) export from terrestrial ecosystems is a potentially important flux for the net catchment C balance and links the biogeochemical C cycling of terrestrial ecosystems to their downstream aquatic ecosystems. We have monitored hydrology and stream chemistry over 3 years in ten nested catchments (0.6–15.1 km2) with variable peatland cover (0%–22%) and groundwater influence in subarctic Sweden. Total waterborne C export, including dissolved and particulate organic carbon (DOC and POC) and dissolved inorganic carbon (DIC), ranged between 2.8 and 7.3 g m–2 year–1, representing ~10%–30% of catchment net ecosystem exchange of CO2. Several characteristics of catchment waterborne C export were affected by interacting effects of peatland cover and groundwater influence, including magnitude and timing, partitioning into DOC, POC, and DIC and chemical composition of the exported DOC. Waterborne C export was greater during the wetter years, equivalent to an average change in export of ~2 g m–2 year–1 per 100 mm of precipitation. Wetter years led to a greater relative increase in DIC export than DOC export due to an inferred relative shift in dominance from shallow organic flow pathways to groundwater sources. Indices of DOC composition (SUVA254 and a250/a365) indicated that DOC aromaticity and average molecular weight increased with catchment peatland cover and decreased with increased groundwater influence. Our results provide examples on how waterborne C export and DOC composition might be affected by climate change. Copyright © 2012 John Wiley & Sons, Ltd.  相似文献   

3.
The China Seas include the South China Sea, East China Sea, Yellow Sea, and Bohai Sea. Located off the Northwestern Pacific margin, covering 4700000 km~2 from tropical to northern temperate zones, and including a variety of continental margins/basins and depths, the China Seas provide typical cases for carbon budget studies. The South China Sea being a deep basin and part of the Western Pacific Warm Pool is characterized by oceanic features; the East China Sea with a wide continental shelf, enormous terrestrial discharges and open margins to the West Pacific, is featured by strong cross-shelf materials transport; the Yellow Sea is featured by the confluence of cold and warm waters; and the Bohai Sea is a shallow semiclosed gulf with strong impacts of human activities. Three large rivers, the Yangtze River, Yellow River, and Pearl River, flow into the East China Sea, the Bohai Sea, and the South China Sea, respectively. The Kuroshio Current at the outer margin of the Chinese continental shelf is one of the two major western boundary currents of the world oceans and its strength and position directly affect the regional climate of China. These characteristics make the China Seas a typical case of marginal seas to study carbon storage and fluxes. This paper systematically analyzes the literature data on the carbon pools and fluxes of the Bohai Sea,Yellow Sea, East China Sea, and South China Sea, including different interfaces(land-sea, sea-air, sediment-water, and marginal sea-open ocean) and different ecosystems(mangroves, wetland, seagrass beds, macroalgae mariculture, coral reefs, euphotic zones, and water column). Among the four seas, the Bohai Sea and South China Sea are acting as CO_2 sources, releasing about0.22 and 13.86–33.60 Tg C yr~(-1) into the atmosphere, respectively, whereas the Yellow Sea and East China Sea are acting as carbon sinks, absorbing about 1.15 and 6.92–23.30 Tg C yr~(-1) of atmospheric CO_2, respectively. Overall, if only the CO_2 exchange at the sea-air interface is considered, the Chinese marginal seas appear to be a source of atmospheric CO_2, with a net release of 6.01–9.33 Tg C yr~(-1), mainly from the inputs of rivers and adjacent oceans. The riverine dissolved inorganic carbon (DIC) input into the Bohai Sea and Yellow Sea, East China Sea, and South China Sea are 5.04, 14.60, and 40.14 Tg C yr~(-1),respectively. The DIC input from adjacent oceans is as high as 144.81 Tg C yr~(-1), significantly exceeding the carbon released from the seas to the atmosphere. In terms of output, the depositional fluxes of organic carbon in the Bohai Sea, Yellow Sea, East China Sea, and South China Sea are 2.00, 3.60, 7.40, and 5.92 Tg C yr~(-1), respectively. The fluxes of organic carbon from the East China Sea and South China Sea to the adjacent oceans are 15.25–36.70 and 43.93 Tg C yr~(-1), respectively. The annual carbon storage of mangroves, wetlands, and seagrass in Chinese coastal waters is 0.36–1.75 Tg C yr~(-1), with a dissolved organic carbon(DOC) output from seagrass beds of up to 0.59 Tg C yr~(-1). Removable organic carbon flux by Chinese macroalgae mariculture account for 0.68 Tg C yr~(-1) and the associated POC depositional and DOC releasing fluxes are 0.14 and 0.82 Tg C yr~(-1), respectively. Thus, in total, the annual output of organic carbon, which is mainly DOC, in the China Seas is 81.72–104.56 Tg C yr~(-1). The DOC efflux from the East China Sea to the adjacent oceans is 15.00–35.00 Tg C yr~(-1). The DOC efflux from the South China Sea is 31.39 Tg C yr~(-1). Although the marginal China Seas seem to be a source of atmospheric CO_2 based on the CO_2 flux at the sea-air interface, the combined effects of the riverine input in the area, oceanic input, depositional export,and microbial carbon pump(DOC conversion and output) indicate that the China Seas represent an important carbon storage area.  相似文献   

4.
Estimates of greenhouse gas evasion from rivers have been refined over the past decades to constrain their role in global carbon cycle processes. However, despite 55% of the human population living in urban areas, urban rivers have had limited attention. We monitored carbon dynamics in an urbanized river (River Kelvin, 331 km2, UK) to explore the drivers of dissolved carbon lateral and vertical export. Over a 2-year sampling period, riverine methane (CH4) and carbon dioxide (CO2) concentrations were consistently oversaturated with respect to atmospheric equilibria, leading to continual degassing to the atmosphere. Carbon stable isotopic compositions (δ13C) indicated that terrestrially derived carbon comprised most of the riverine CH4 and dissolved CO2 (CO2*) load while dissolved inorganic carbon (DIC) from groundwater was the main form of riverine DIC. The dynamics of CH4, CO2*, and DIC in the river were primarily hydrology-controlled, that is, [CH4] and [CO2*] both increased with elevated discharge, total [DIC] decreased with elevated discharge while the proportion of biologically derived DIC increased with increasing discharge. The concentration of dissolved organic carbon (DOC) showed a weak relationship with river hydrology in summer and autumn and was likely influenced by the combined sewer overflows. Carbon emission to the atmosphere is estimated to be 3.10 ± 0.61 kg C·m−2·yr−1 normalized to water surface area, with more than 99% emitted as CO2. Annual carbon loss to the coastal estuary is approximately 4.69 ± 0.70 Gg C yr−1, with annual DIC export approximately double that of DOC. Per unit area, the River Kelvin was a smaller carbon source to the atmosphere than natural rivers/streams but shows elevated fluxes of DIC and DOC under comparable conditions. This research illustrates the role urban systems may have on riverine carbon dynamics and demonstrates the potential tight link between urbanization and riverine carbon export.  相似文献   

5.
We measured spatial and temporal variations in carbon concentrations, isotopic compositions and exports during a complete hydrological cycle in nine watercourses draining a lowland forested podzolized catchment, flowing into the Arcachon lagoon (France). In addition, integrated fluxes of CO2 across the water-atmosphere interface were estimated to assess the relative importance of CO2 evasion versus lateral carbon transport at the catchment scale. Watercourse similarities and specificities linked to the local catchment characteristics are discussed and compared with other riverine systems. Low concentrations of suspended particulate matter and particulate organic carbon (POC) were generally measured in all the watercourses (8.4 ± 3.4 and 1.6 ± 0.6 mg L?1, respectively), reflecting limited mechanical soil erosion. The generally high POC content in the suspended matter (20 %), low Chl a concentrations (1.3 ± 1.4 μg L?1) and the relatively constant δ13C-POC value (near ?28 ‰) throughout the year reveal this POC originates from terrestrial C3 plant and soil detritus. The presence of podzols leads to high levels of dissolved organic carbon (DOC; 6.6 ± 2.2 mg L?1). Similarly, high dissolved inorganic carbon (DIC) concentrations were measured in the Arcachon lagoon catchment (5.9 ± 2.2 mg L?1). The δ13C-DIC value around ?20 ‰ throughout the year in many small watercourses reveals the predominance of terrestrial carbon mineralisation and silicate rock weathering in soils as the major DIC source. With pCO2 between 1,000 and 10,000 ppmv, all watercourses were a source of CO2 to the atmosphere, particularly during the low river stage. Organic carbon parameters remained relatively stable throughout the year, whereas DIC parameters showed strong seasonal contrasts closely linked to the hydrological regime and hyporheic flows. In total, the carbon export from the Arcachon watershed was estimated at 15,870 t C year?1 or 6 t C km?2 year?1, mostly exported to the lagoon as DOC (35 %), DIC (24 %) and lost as CO2 degassing to the atmosphere (34 %).  相似文献   

6.
To investigate the effects of anthropogenic activity, namely, land use change and reservoir construction, on particulate organic carbon (POC) transport, we collected monthly water samples during September 2007 to August 2009 from the Longchuanjiang River to understand seasonal variations in the concentrations of organic carbon species and their sources and the yield of organic and inorganic carbon from the catchment in the Upper Yangtze basin. The contents of riverine POC, total organic carbon and total suspended sediment (TSS) changed synchronously with water discharge, whereas the contents of dissolved organic carbon had a small variation. The POC concentration in the suspended sediment decreased non‐linearly with increasing TSS concentration. Higher molar C/N ratio of particulate organic matter (average 77) revealed that POC was dominated by terrestrially derived organic matter in the high flows and urban wastewaters in the low flows. The TSS transported by this river was 2.7 × 105 t/yr in 2008. The specific fluxes of total organic carbon and dissolved inorganic carbon (DIC) were 5.6 and 6 t/km2/yr, respectively, with more than 90% in the high flow period. A high carbon yield in the catchment of the upper Yangtze was due to human‐induced land use alterations and urban wastes. Consistent with most rivers in the monsoon climate regions, the dissolved organic carbon–POC ratio of the export flux was low (0.41). Twenty‐two percent (0.9 t/km2/yr) of POC out of 4 t/km2/yr was from autochthonous production and 78% (3.1 t/km2/yr) from allochthonous production. The annual sediment load and hence the organic carbon flux have been affected by environmental alterations of physical, chemical and hydrological conditions in the past 50 years, demonstrating the impacts of human disturbances on the global and local carbon cycling. Finally, we addressed that organic carbon flux should be reassessed using adequate samples (i.e. at least two times in low‐flow month, four times in high‐flow month and one time per day during the flood period), daily water discharge and sediment loads and appropriate estimate method. Copyright © 2011 John Wiley & Sons, Ltd.  相似文献   

7.
Spatial and temporal variability of hydrological responses affecting surface water dissolved organic carbon (DOC) concentrations are important for determining upscaling patterns of DOC export within larger catchments. Annual and intra‐annual variations in DOC concentrations and fluxes were assessed over 2 years at 12 sites (3·40–1837 km2) within the River Dee basin in NE Scotland. Mean annual DOC fluxes, primarily correlated with catchment soil coverage, ranged from 3·41 to 9·48 g m?2 yr?1. Periods of seasonal (summer–autumn and winter–spring) DOC concentrations (production) were delineated and related to discharge. Although antecedent temperature mainly determined the timing of switchover between periods of high DOC in the summer‐autumn and low DOC in winter‐spring, inter‐annual variability of export within the same season was largely dependent on its associated water flux. DOC fluxes ranged from 1·39 to 4·80 g m?2 season?1 during summer–autumn and 1·43 to 4·15 g m?2 season?1 in winter–spring.Relationships between DOC areal fluxes and catchment scale indicated that mainstem fluxes reflect the averaging of highly heterogeneous inputs from contrasting headwater catchments, leading to convergent DOC fluxes at catchment sizes of ca 100 km2. However, during summer–autumn periods, in contrast to winter–spring, longitudinal mainstem DOC fluxes continue to decrease, most likely because of increasing biological processes. This highlights the importance of considering seasonal as well as annual changes in DOC fluxes with catchment scale. This study increases our understanding of the temporal variability of DOC upscaling patterns reflecting cumulative changes across different catchment scales and aids modelling of carbon budgets at different stages of riverine systems. Copyright © 2010 John Wiley & Sons, Ltd.  相似文献   

8.
Detailed knowledge of the flood period of Arctic rivers remains one of the few factors impeding rigorous prediction of the effect of climate change on carbon and related element fluxes from the land to the Arctic Ocean. In order to test the temporal and spatial variability of element concentration in the Ob River (western Siberia) water during flood period and to quantify the contribution of spring flood period to the annual element export, we sampled the main channel year round in 2014–2017 for dissolved C, major, and trace element concentrations. We revealed high stability (approximately ≤10% relative variation) of dissolved C, major, and trace element concentrations in the Ob River during spring flood period over a 1‐km section of the river channel and over 3 days continuous monitoring (3‐hr frequency). We identified two groups of elements with contrasting relationship to discharge: (a) DIC and soluble elements (Cl, SO4, Li, B, Na, Mg, Ca, P, V, Cr, Mn, As, Rb, Sr, Mo, Ba, W, and U) negatively correlated (p < 0.05) with discharge and exhibited minimal concentrations during spring flood and autumn high flow and (b) DOC and particle‐reactive elements (Al, Fe, Ti, Y, Zr, Nb, Cs, REEs, Hf, Tl, Pb, and Th), some nutrients (K), and metalloids (Ge, Sb, and Te), positively correlated (p < 0.05) with discharge and showed the highest concentrations during spring flood. We attribute the decreased concentration of soluble elements with discharge to dilution by groundwater feeding and increased concentration of DOC and particle‐reactive metals with discharge to leaching from surface soil, plant litter, and suspended particles. Overall, the present study provides first‐order assessment of fluxes of major and trace elements in the middle course of the Ob River, reveals their high temporal and spatial stability, and characterizes the mechanism of river water chemical composition acquisition.  相似文献   

9.
The Yellow River transports a large amount of sediment and particulate organic carbon (POC), which is thought to mainly derive from erosion of the Chinese Loess Plateau (CLP). However, the compositions, sources and erosional fluxes of POC in the Yellow River remain poorly constrained. Here we combined measurements of mineralogy, total organic carbon content (OCtotal), stable organic carbon isotopes (δ13Corg), radiocarbon (14C) activity of organic matter in bulk suspended sediments collected seasonally from the upper and middle Yellow River, to quantify the compositions and fluxes of the POC and to assess its sources (biospheric and petrogenic POC, i.e. POCbio and POCpetro, respectively). The results showed that the POC loading of sediments was controlled by mineralogy, grain size and specific surface area of loess particles. The Fmod of POC (0.71 to 0.31) can be explained by mixing of POCpetro with modern and aged POCbio. A binary mixing model based on the hyperbolic relationship of the Fmod and OCtotal revealed a wide range of ages of POCbio from 1300 to 11100 14C years. Relative to the upstream station, the annual POCbio and POCpetro fluxes in the Yellow River are more than doubled after it flows crossing the CLP within 35% drainage area gain, resulting in POCbio and POCpetro yields of the CLP at 3.50 ± 0.59 and 0.48 ± 0.49 tC/km2/yr, respectively. POC flux seasonal variation revealed that monsoon rainfall exerts a first-order control on the export of both POCbio and POCpetro from the CLP to the Yellow River, resulting in more than 90% of the annual POC exported during the monsoon season. Around one third of annual POC erosional flux was transported during a storm event period, highlighting the important role of extreme events in POC export in this large river. © 2020 John Wiley & Sons, Ltd.  相似文献   

10.
We analyzed variation of channel–floodplain suspended sediment exchange along a 140 km reach of the lower Amazon River for two decades (1995–2014). Daily sediment fluxes were determined by combining measured and estimated surface sediment concentrations with river–floodplain water exchanges computed with a two‐dimensional hydraulic model. The average annual inflow to the floodplain was 4088 ± 2017 Gg yr?1 and the outflow was 2251 ± 471 Gg yr?1, respectively. Prediction of average sediment accretion rate was twice the estimate from a previous study of this same reach and more than an order of magnitude lower than an estimate from an earlier regional scale study. The amount of water routed through the floodplain, which is sensitive to levee topography and increases exponentially with river discharge, was the main factor controlling the variation in total annual sediment inflow. Besides floodplain routing, the total annual sediment export depended on the increase in sediment concentration in lakes during floodplain drainage. The recent increasing amplitude of the Amazon River annual flood over two decades has caused a substantial shift in water and sediment river–floodplain exchanges. In the second decade (2005–2014), as the frequency of extreme floods increased, annual sediment inflow increased by 81% and net storage increased by 317% in relation to the previous decade (1995–2004). Copyright © 2017 John Wiley & Sons, Ltd.  相似文献   

11.
The ongoing regression of sea ice cover is expected to significantly affect the fate of organic carbon over the Arctic continental shelves. Long-term moored sediment traps were deployed in 2005–2006 in the Beaufort Sea, Northern Baffin Bay and the Laptev Sea to compare the annual variability of POC fluxes and to evaluate the factors regulating the annual cycle of carbon export over these continental shelves. Annual POC fluxes at 200 m ranged from 1.6 to 5.9 g C m−2 yr−1 with the highest export in Northern Baffin Bay and the lowest export over the Mackenzie Shelf in the Beaufort Sea. Each annual cycle exhibited an increase in POC export a few weeks before, during, or immediately following sea ice melt, but showed different patterns over the remainder of the cycle. Enhanced primary production, discharge of the Lena River, and resuspension events contributed to periods of elevated POC export over the Laptev Sea slope. High POC fluxes in Northern Baffin Bay reflected periods of elevated primary production in the North Water polynya. In the Beaufort Sea sediment resuspension contributed to most of the large export events. Our results suggest that the outer shelf of the Laptev Sea will likely sustain the largest increase in POC export in the next few years due to the large reduction in ice cover and the possible increase in the Lena River discharge. The large differences in forcing among the regions investigated reinforce the importance of monitoring POC fluxes in the different oceanographic regimes that characterize the Arctic shelves to assess the response of the Arctic Ocean carbon cycle to interannual variability and climate change.  相似文献   

12.
Carbon transported by rivers is an important component of the global carbon cycle. Here, we report on organic carbon transport along the third largest river in China, the Songhua River, and its major tributaries. Water samples were collected seasonally or more frequently to determine dissolved organic carbon (DOC) and particulate organic carbon (POC) concentrations and C/N and stable carbon isotopic ratios. Principal component analysis and multiple regression analysis of these data, in combination with hydrological records for the past 50 years, were used to determine the major factors influencing the riverine carbon fluxes. Results indicate that the organic carbon in the Songhua River basin is derived mainly from terrestrial sources. In the 2008–2009 hydrological year, the mean concentrations of DOC and POC were 5.87 and 2.36 mg/L, and the estimated fluxes of the DOC and POC were 0.30 and 0.14 t·km?2·year?1, respectively. The riverine POC and DOC concentrations were higher in subcatchments with more cropland, but the area‐specific fluxes were lower, owing to decreased discharge. We found that hydrological characteristics and land‐use type (whether forest or cropland) were the most important factors influencing carbon transport in this system. Agricultural activity, particularly irrigation, is the principal cause of changes in water discharge and carbon export. Over the last 50 years, the conversion of forest to cropland has reduced riverine carbon exports mainly through an associated decrease in discharge following increased extraction of water for irrigation.  相似文献   

13.
Seasonal changes in water quality were measured in samples taken at various distances from shallow water across mudflat to mangroves during flood period and from mangroves across mudflat to shallow water during ebb period in a subtropical mangrove estuary (Zhangjiang Estuary, Fujian, China). The TN (total dissolved nitrogen), TP (total dissolved phosphorus), COD (chemical oxygen demand), and DOC (dissolved organic carbon) contents during the flood period were significantly higher than those during the ebb period. In contrast, the opposite was true for the POC (particulate organic carbon) content and transparency. The mangroves at Zhangjiang Estuary may trap nutrients at rates of 90.5 g N/m2/yr, 2.2 g TP/m2/yr, and 13.7 g C/m2/yr in the form of DOC, and export POC at a rate of 81.8 g/m2/yr. Our results support the hypothesis that the maintenance of estuarine water quality by mangroves occurs during flood periods.  相似文献   

14.
Evaluating the role of fluvial transfer of terrestrial organic carbon (OC) and subsequent burial in the global carbon cycle requires the sources and fluxes of fluvial OC to be assessed, which remains poorly constrained in the Huanghe (Yellow River). Here, we report the elemental, stable isotopic, and radiocarbon activity of particulate organic carbon (POC) sampled at the outlet of Huanghe in 2012–2013. We show that the Huanghe riverine POC can be explained by binary mixing of fossil (POCfossil) and non‐fossil (POCnon‐fossil) components, the former may reach ~40% of the total POC. The Huanghe POCnon‐fossil is mostly sourced from C3 plants, with a mean residence time of c. 2200 years. The current human‐controlled hydrological regime strongly influenced the POC sources, transport modes, and fluxes. In 2012–2013, the Huanghe delivered 0.73 Tg (1 Tg = 1012 g) of POC to the sea, and about 28% of the annual POC flux occurred within a short human induced flood event. Globally, the Huanghe should be one of the largest rivers in the transfer and re‐burial of fossil OC. However, the fate of Huanghe fossil OC is still unconstrained and needs to be further investigated. Copyright © 2015 John Wiley & Sons, Ltd.  相似文献   

15.
The stable isotopic composition of dissolved inorganic carbon (δ13C‐DIC) was investigated as a potential tracer of streamflow generation processes at the Sleepers River Research Watershed, Vermont, USA. Downstream sampling showed δ13C‐DIC increased between 3–5‰ from the stream source to the outlet weir approximately 0·5 km downstream, concomitant with increasing pH and decreasing PCO2. An increase in δ13C‐DIC of 2·4 ± 0·1‰ per log unit decrease of excess PCO2 (stream PCO2 normalized to atmospheric PCO2) was observed from downstream transect data collected during snowmelt. Isotopic fractionation of DIC due to CO2 outgassing rather than exchange with atmospheric CO2 may be the primary cause of increased δ13C‐DIC values downstream when PCO2 of surface freshwater exceeds twice the atmospheric CO2 concentration. Although CO2 outgassing caused a general increase in stream δ13C‐DIC values, points of localized groundwater seepage into the stream were identified by decreases in δ13C‐DIC and increases in DIC concentration of the stream water superimposed upon the general downstream trend. In addition, comparison between snowmelt, early spring and summer seasons showed that DIC is flushed from shallow groundwater flowpaths during snowmelt and is replaced by a greater proportion of DIC derived from soil CO2 during the early spring growing season. Thus, in spite of effects from CO2 outgassing, δ13C of DIC can be a useful indicator of groundwater additions to headwater streams and a tracer of carbon dynamics in catchments. Copyright © 2007 John Wiley & Sons, Ltd.  相似文献   

16.
Total organic carbon fluxes of the Red River system (Vietnam)   总被引：1，自引：0，他引：1       下载免费PDF全文
Riverine transport of organic carbon from terrestrial ecosystems to the oceans plays an important role in the global carbon cycle. The Red River is located in Southeast Asia where river discharge, sediment loads and fluxes of elements (carbon, nitrogen and phosphorus) associated with suspended solids have been dramatically altered over past decades as a result of reservoir impoundment and land use, population, and climate change. Dissolved organic carbon (DOC) and particulate organic carbon (POC) concentrations were measured monthly at four stations of the Red River system from January 2008 to December 2010. The results reveal that POC changed synchronically with total suspended solids (TSS) concentration and with the river discharge, whereas no clear trend was observed for DOC concentration. The mean value of total organic carbon (TOC = DOC + POC) flux in the delta of the Red River was 31.5 × 1013 ± 4.0 × 1013 MgC.yr?1 (range 27.9–35.8 × 1013 MgC.yr?1 which leads to a specific TOC flux of 2012 ± 255 kgC.km?2.yr?1 during this 2008–2010 period. About 80% of the TOC flux was transferred to the estuary during the rainy season as a consequence of the higher river water discharge. The high mean value of the POC:Chl‐a ratio (1585 ± 870 mgC.mgChl‐a?1) and the moderate C:N ratio (7.3 ± 0.1) in the water column system suggest that organic carbon in the Red River system is mainly derived from erosion and soil leaching in the basin. The effect of two new dam impoundments in the Red River was also observable with lower TOC fluxes in 2010 compared with 2008. Copyright © 2017 John Wiley & Sons, Ltd.  相似文献   

17.
Rivers of South and Southeast Asia disgorge large suspended sediment loads, reflecting exceptionally high rates of erosion promoted by natural processes (tectonic and climatic) and anthropogenic (land‐use change) activities that are characteristic of the region. While particulate carbon and nitrogen fluxes have been characterized in some large Asian rivers, less is known about the headwater systems where much sediment and organic material are initially mobilized. This study, conducted in the 74‐km2 Mae Sa Experimental Catchment in northern Thailand, shows that the Sa River is an important source for particulate organic carbon (POC) and particulate organic nitrogen (PON) transported to larger river systems and downstream reservoirs. However, the yields during three years of investigation varied greatly: 5.0–22.3 Mg POC km?2 y?1 and 0.48–2.02 Mg PON km?2 y?1. The 22.3 Mg POC km?2 y?1 yield is the highest reported for any river on the Asian continent. Stream samples collected during 12 storms showed that almost 3% of the total suspended solid load is POC 0.7 µm to 2.0 mm in size. This percentage is higher than other values for most large rivers on the continent. Further, we documented a strong pulse hysteretic behaviour in the stream, whereby peak fluxes of POC and PON are often delayed (anticlockwise hysteresis) or accelerated (clockwise hysteresis) relative to stream flow peaks (or are complex), complicating the prediction of storm‐based or annual particulate carbon and nitrogen fluxes. Stream turbidity and total suspended sediment are reasonable proxies for POC and PON concentrations, while stream discharge is not a good predictor variable. Observed C:N ratios for measured particulate samples range from 3 to 83, with the high‐end values likely associated with fresh (non‐decomposed) vegetative material greater than 2 mm in diameter. The C:N ratio (weighted based on three sediment sizes) for 12 events ranges from 7.5 to 15.3. These modest values reflect the relatively low C:N ratios for small size fractions (0.7–0.63 µm) that comprise 50–90% of the TSS load in the events. Overall, organic material <0.63 µm contribute about 75% of the total POC load and 80% of the PON load. The annual C:N ratio for the river is approximately 10–11. Collectively, our findings indicate the occasionally high yields make the Sa River—and potentially other similar headwater rivers—a hot spot for POC and PON transported to downstream water bodies. Complex hysteresis patterns and high year‐to‐year variability hinders our ability to calculate and predict these yields without continuous, automated monitoring of discharge and turbidity. Copyright © 2016 John Wiley & Sons, Ltd.  相似文献   

18.
The purposes of this study were to assess if Lake Apopka (FL, USA) was autotrophic or heterotrophic based on the partial pressure of dissolved carbon dioxide (pCO2) in the surface water and to evaluate factors that influence the long-term changes in pCO2. Monthly average pH, alkalinity and other limnological variables collected between 1987 and 2006 were used to estimate dissolved inorganic carbon (DIC), pCO2 and CO2 flux between surface water and atmosphere. Results indicated that average pCO2 in the surface water was 196 μatm, well below the atmospheric pCO2. Direct measurements of DIC concentration on three sampling dates in 2009 also supported pCO2 undersaturation in Lake Apopka. Supersaturation in CO2 occurred in this lake in only 13% of the samples from the 20-year record. The surface-water pCO2 was inversely related to Chl a concentrations. Average annual CO2 flux was 28.2 g C m−2 year−1 from the atmosphere to the lake water and correlated significantly with Chl a concentration, indicating that biological carbon sequestration led to the low dissolved CO2 concentration. Low pCO2 and high invasion rates of atmospheric CO2 in Lake Apopka indicated persistent autotrophy. High rates of nutrient loading and primary production, a high buffering capacity, a lack of allochthonous loading of organic matter, and the dominance of a planktivorous–benthivorous fish food web have supported long-term net autotrophy in this shallow subtropical eutrophic lake. Our results also showed that lake restoration by the means of nutrient reduction resulted in significantly lower total phosphorus (TP) and Chl a concentrations, and higher pCO2.  相似文献   

19.
Drifting sediment traps were deployed at 9 stations in May-June (ice-covered conditions) and July-August (ice-free conditions) 2004 in the Chukchi Sea to investigate the variability in export fluxes of biogenic matter in the presence and absence of sea ice cover. Measurements of chlorophyll-a (Chl-a), particulate organic carbon (POC), particulate nitrogen (PN), phytoplankton, zooplankton fecal pellets, and the stable carbon isotope composition (δ13C) of the sinking material were performed along Barrow Canyon (BC) and a parallel shelf-to-basin transect from East Hanna Shoal (EHS) to the Canada Basin. POC export fluxes were similarly high in the presence (378±106 mg C m−2 d−1) and in the absence of ice cover (442±203 mg C m−2 d−1) at the BC stations, while fluxes were significantly higher in the absence (129±98 mg C m−2 d−1) than in the presence of ice cover (44±29 mg C m−2 d−1) at the EHS stations. The C/N ratios and δ13C values of sinking organic particles indicated that POC export fluxes on the Chukchi continental shelf were mostly composed of freshly produced labile material, except at the EHS stations under ice cover where the exported matter was mostly composed of refractory material probably advected into the EHS region. Chl-a fluxes were higher under ice cover than in ice-free water, however, relatively low daily loss rates of Chl-a and similar phytoplankton carbon fluxes in ice-covered and ice-free water suggest the retention of phytoplankton in the upper water column. An increase in fecal pellet carbon fluxes in ice-free water reflected higher grazing pressure in the absence of ice cover. Elevated daily loss rates of POC at the BC stations confirmed other indications that Barrow Canyon is an important area of carbon export to the basin and/or benthos. These results support the conclusion that there are large spatial and temporal variations in export fluxes of biogenic matter on the Chukchi continental shelf, although export fluxes may be similar in the presence and in the absence of ice cover in highly productive regions.  相似文献   

20.
Global climate change and diverse human activities have resulted in distinct temporal–spatial variability of watershed hydrological regimes, especially in water‐limited areas. This study presented a comprehensive investigation of streamflow and sediment load changes on multi‐temporal scales (annual, flood season, monthly and daily scales) during 1952–2011 in the Yanhe watershed, Loess Plateau. The results indicated that the decreasing trend of precipitation and increasing trend of potential evapotranspiration and aridity index were not significant. Significant decreasing trends (p < 0.01) were detected for both the annual and flood season streamflow, sediment load, sediment concentration and sediment coefficient. The runoff coefficient exhibited a significantly negative trend (p < 0.01) on the flood season scale, whereas the decreasing trend on the annual scale was not significant. The streamflow and sediment load during July–August contributed 46.7% and 86.2% to the annual total, respectively. The maximum daily streamflow and sediment load had the median occurrence date of July 31, and they accounted for 9.7% and 29.2% of the annual total, respectively. All of these monthly and daily hydrological characteristics exhibited remarkable decreasing trends (p < 0.01). However, the contribution of the maximum daily streamflow to the annual total progressively decreased (?0.07% year?1), while that of maximum daily sediment load increased over the last 60 years (0.08% year?1). The transfer of sloping cropland for afforestation and construction of check‐dams represented the dominant causes of streamflow and sediment load reductions, which also made the sediment grain finer. Copyright © 2015 John Wiley & Sons, Ltd.  相似文献   

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