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1.
Weekly bulk aerosol samples collected at Funafuti, Tuvalu (8°30S, 179°12E), American Samoa (14°15S, 170°35W), and Rarotonga (21°15S, 159°45W), from 1983 through most of 1987 have been analyzed for nitrate and other constituents. The mean nitrate concentration is about 0.11 g m–3 at each of these stations: 0.107±0.011 g m–3 at Funafuti; 0.116±0.008 at American Samoa; and 0.117±0.010 at Rarotonga. Previous measurements of mineral aerosol and trace metal concentrations at American Samoa are among the lowest ever recorded for the near-surface troposphere and indicate that this region is minimally affected by transport of soil material and pollutants from the continents. Consequently, the nitrate concentration of 0.11 g m–3 can be regarded as the natural level for the remote marine boundary layer of the tropical South Pacific Ocean. In contrast, over the tropical North Pacific which is significantly impacted by the transport of material from Asia and North America, the mean nitrate concentrations are about three times higher, 0.29 and 0.36 g m–3 at Midway and Oahu, respectively. The major sources of the nitrate over the tropical South Pacific are still very uncertain. A very significant correlation between the nitrate concentrations at American Samoa and the concentrations of 210Pb suggests that transport from continental sources might be important. This continental source could be lightning, which occurs most frequently over the tropical continents. A near-zero correlation with 7Be indicates that the stratosphere and upper troposphere are probably not the major sources. A significant biogenic source would be consistent with the higher mean nitrate concentrations, 0.16 to 0.17 g m–3, found over the equatorial Pacific at Fanning Island (3°55N, 159°20W) and Nauru (0°32S, 166°57E). The lack of correlation between nitrate and nss sulfate at American Samoa does not necessarily preclude an important role for marine biogenic sources.  相似文献   

2.
Observations made with a monostatic sodar and from a 120 m instrumented tower have been used to study the variations in the atmospheric boundary layer at Tarapur (19° 50 N, 72° 41 E) during the solar eclipse of February 16, 1980. Atmospheric instability was reduced below normal values during the eclipse but the atmosphere at no time became stable.  相似文献   

3.
Wind velocities within a plant canopy are much more strongly skewed than those of the air flow above. We have examined the governing Eulerian equations for the velocity products u i, u j uk using data from a wind tunnel study with an artificial canopy consisting of an array of 5 cm lengths of monofilament fishing line, and from measurements in corn (Zea mays L).Simple parameterizations for pressure-velocity correlations, and for the quadruple velocity products allowed reasonably accurate calculations of the third moments using measured profiles of the mean velocity, variance and covariance fields. Comparisons of individual terms in the rate equations for ovu i, u j u krevealed that diffusion (from above) and mean shear were most important in creating large skewness in the canopy. A drag term also contributed but was of lesser importance. These terms were balanced by return-to-isotropy and a turbulence interaction term. A quasi-Gaussian approximation considerably underestimated the magnitude of the fourth moments within the canopy.  相似文献   

4.
Springtime measurements of NOx, ozone, PAN,J(NO2), and other compounds were made near Ny-Ålesund,Svalbard (78°54N, 11°53E), in 1994 and Poker Flat,Alaska (65°08N, 147°29W), in 1995. At Svalbard medianmixing ratios for PAN and NOx of 237 and 23.7 pptv,respectively, were observed. The median mixing ratios at Poker Flat for PANand NOx were 79.5 and 85.9 pptv, respectively. These data areused to estimate thermal PAN decomposition using several differentapproaches. At Svalbard PAN decomposition was very small, while at PokerFlat up to 30 pptv/h PAN decomposed. At both sites the NOx/PANratio increased with temperature between –10 and 20°C implyingthat PAN decomposition is an important NOx source. In-situozone production was calculated from the measured NO, NO2,O3, J(NO2), and temperature data, using thesteady state assumption Median ozone production was 605 pptv/h at PokerFlat, and one order of magnitude smaller at Svalbard during the daytime.Only at Poker Flat could a direct influence on the diurnal ozone cycle beobserved from in-situ production. These results imply that PAN decompositionis a major source of NOx in the high latitude troposphere, andthat this contributes to the observed spring maximum in surface ozone.  相似文献   

5.
Surfaces fluxes, turbulent kinetic energy and Flux Richardson number are calculated for three typical sea breeze days characterizing three types of sea breeze onset at an inland station Kharagpur (22°21 N, 87°19 E), 80 km inland, one of the sites for MONTBLEX (MONsoon Trough Boundary Layer EXperiment), in India. The sea breeze onset is associated with a decrease in momentum and heat fluxes and an increase in moisture flux. The turbulent kinetic energy shows quite a significant value even in the late afternoon. The surface layer becomes nearly stable even before sunset, due to the passage of the sea breeze.  相似文献   

6.
Summary The Balkan Peninsula is situated in the impact zone of Saharan dust storms. The case of Saharan dust transport to Belgrade in the period of 14–17 April 1994 is analyzed using the Eta model for synoptic and meso scale processes. Air back trajectories are calculated at six model levels from 434 up to 5129m with horizontal grid resolutions of 1°×1° and 10×10. Following cyclonic circulation the dust was picked up from North Africa, and transported over Mediterranean. Simultaneously, according to the analysis of the three lowest trajectories, transport of trace metals from Macedonia and southern Serbia by the Koshava wind might be dominant in the observed episode. Turbulent flow enhanced the coagulation process of initially clean dust particles with particles containing Pb and Cd. The coagulation and scavenging processes below and in clouds increased deposition rates of Pb and Cd in Belgrade in the course of wet removal, and consequently trough resuspension processes. Dry deposition samples contained characteristic particles up to 30µm in diameter with Fe content of 11 to 15 atomic% and significant ratio Si/Fe of 3 to 5, determined for selected single particles by the SEM/EDX method. Following dry and wet deposition of Cd and Pb, a residual effect of dustfall is noticed throughout the vegetational period.  相似文献   

7.
Summary A classification scheme for cold surges occurring along the Front Range of the Rocky Mountains has been developed using NMC surface and upper air data. A separation is seen in the data between cases with parent anticyclones that moved from Canada south into the United States (Northern type) and those which moved from the Eastern Pacific Ocean east into the central US (Western type). The Northern surges are further broken down into three types, A, B and B, when the degree of southward motion of the anticyclone and the leading edge of the cold air is considered. An anticyclone movement south of 40°N distinguishes type A, while anticyclone tracks remaining north of 40°N characterize types B and B. The leading edge of the surge (the surge line) associated with the type A anticyclone travels south of 25N, while the type B anticyclones produce two distinct surge line movements, one remaining north of 25°N and the other moving south of 25°N. It is not possible to break down the Western surges into distinct types. As a rule, the anticyclones associated with Western surges remain between 50°N and 30°N, with the surge line moving south to 18°N on average.Though the classification scheme is developed in a relatively subjective manner, the statistical robustness of the scheme is verified through application of the nonparametric Mann-Whitney test. Results of the test clearly provide support for the division of the surges that was obtained.With 16 Figures  相似文献   

8.
Meteorological measurements taken at the Näsudden wind turbine site during slightly unstable conditions have been analyzed. The height of the convective boundary layer (CBL) was rather low, varying between 60 and 300 m. Turbulence statistics near the ground followed Monin-Obukhov similarity, whereas the remaining part of the boundary layer can be regarded as a near neutral upper layer. In 55% of the runs, horizontal roll vortices were found. Those were the most unstable runs, with -z i/L > 5. Spectra and co-spectra are used to identify the structures. Three roll indicators were identified: (i) a low frequency peak in the spectrum of the lateral component at low level; (ii) a corresponding increase in the vertical component at mid-CBL; (iii) a positive covariance {ovvw} together with positive wind shear in the lateral direction (V/z) in the CBL. By applying these indicators, it is possible to show that horizontal roll circulations are likely to be a common phenomenon over the Baltic during late summer and early winter.  相似文献   

9.
Sublimation and melt disturb the environmental information obtained from ice core records in the Andes. In two case studies we demonstrate to what extent these post-depositional processes may remove major parts of the accumulated snow cover. Dark ash layers from the Tungurahua eruption changed the albedo of surface snow on Chimborazo glacier (6268 m, 1°30 S,78°36 W, Ecuador) between two ice core drilling campaigns and forced substantial melt. Re-distribution and washout of the chemical constituents shifted the concentration profiles obtained in December 1999 as compared to an equivalent core drilled in December 2000. The stable isotope records showed that approximately the water equivalent (weq) of an annual layer had melted, and that the percolating melt water penetrated within the firn layer to a depth of at least 16.5 m without refreezing. In the second example, from a site on the dry axis between the tropical and extra-tropical precipitation belts, significant loss of accumulated snow layers occurred by sublimation. A surface experiment at Cerro Tapado glacier (5536 m, 30°08 S,69°55 W, Chile) revealed that losses of 2 mm weq (5 mm snow) per day occurred during the dry period following the 1997/98 El Niño. This loss generally included the entire surface layer enriched in stable isotopes, and thus caused minimal disturbance of the isotopic signature (and hence climatic information) of the net accumulation, yet chemical constituents again experienced considerable changes in concentration. From annual layer counting and direct dating it is obvious that the major part of the accumulated ice on both glaciers is younger than 100 years; however, isotopic and chemical variations at least in the basal ice from Cerro Tapado clearly point to climate conditions different from the recent centuries. This evidence is supported by mass balance considerations derived from a glacier-climate model. The possibility of a third type of disturbance aside from sublimation and melting – in this case a significant hiatus in the environmental chronology – also deserves consideration for other icecore records from this region. Potential disruptions or discontinuities need to be carefully evaluated given the profound changes in climatic and glaciological conditions since the Last Glacial Maximum throughout Holocene times.  相似文献   

10.
Summary A simple parameterization for the estimation of turbulent kinetic energy (TKE) and momentum flux profiles under near-neutral stratification based on sodar measurements of the vertical velocity variance has been tested using data from the LINEX-2000 experiment. Measurements included operation of a phased-array Doppler sodar DSDPA.90 and of a sonic anemometer USA-1 mounted at a meteorological tower at a height of 90m. Good agreement has been found between the TKE and momentum flux values derived from the sonic and sodar data (with correlation coefficients r>0.90 and a slope of the regression lines of about 1.01.1) suggesting the possible use of sodar measurements of w 2 to derive turbulence parameter profiles above the tower range.  相似文献   

11.
This study examines the statistical properties of the concentration derivative, , for a dispersing plume in a near-neutrally stratified atmospheric surface layer. Towards this goal, the probability density function (pdf) of , and the conditional pdf of given a fixed concentration level, , have been measured. These pdfs are found to be modeled well by a generalizedq-Gaussian (gqG) distribution with intermittency exponent,q, equal to 0.3 and 3/4, respectively. These results highlight the strong intermittency effect (patchiness) of the small-scale concentration eddy structures in the plume. The distribution of time intervals between successive high peaks in the squared derivative process, x2, is found to be well approximated by a power-law distribution, implying that occurrences of these high peaks are much more clustered than would be predicted by a Poisson or shot-noise process. The results are used to improve models for the joint pdf of and , and for the expected number of upcrossings per unit time interval of a fixed concentration level that have been proposed by Kristensenet al. (1989). The predictions of the improved models are in accord with observations, and suggest that the intercorrelation between and must be explicitly incorporated if good estimates of the upcrossing intensity are to be obtained.  相似文献   

12.
The use of ultrasonic anemometers under cloudy weather conditions is often doubted, even rejected or not discussed in the literature. To investigate the influence of liquid water content on the behaviour of sonic anemometers a small intercomparison experiment using an ultrasonic anemometer, a fast response propeller anemometer, and a Particulate Volume Monitor was performed at the German Environmental Research Station Schneefernerhaus near the top of Mt. Zugspitze. The results obtained under different conditions (dry/cloudy) give no significant hint on such an influence.  相似文献   

13.
Summary A time series and extreme value analysis of maximum precipitation for distinct time intervals from 10 minutes to 1 day have been deduced for the observatory Zagreb-Gri ( = 45°49 and = 15°59,H s = 157 m) for the period between 1908 and 1985. The Spearman rank correlation test revealed that the short-term precipitation maxima series for the time intervals of 10 to 30 minutes and 8 to 24 hours indicate no significant trend for the 95 percent probability level. The 40-minute to 4-hour precipitation maxima exhibited an increaese in recent time. Annual maximumt-minute precipitation was estimated using the Gumbel distribution for sets of data gradually prolonged with 10-year steps towards the past. The ratios (q) of maximum precipitation estimates for the shorter periods and of estimates for the reference period (1908–1985) have been calculated. Their positions according to the confidence interval on the reference estimates were determined. Confident extreme value estimates could be obtained using at least the 50–60 year data series.With 3 Figures  相似文献   

14.
Flux densities of carbon dioxide were measured over an arid, vegetation-free surface by eddy covariance techniques and by a heat budget-profile method, in which CO2 concentration gradients were specified in terms of mixing ratios. This method showed negligible fluxes of CO2, consistent with the bareness of the experimental site, whereas the eddy covariance measurements indicated large downward fluxes of CO2. These apparently conflicting observations are in quantitative agreement with the results of a recent theory which predicts that whenever there are vertical fluxes of sensible or latent heat, a mean vertical velocity is developed. This velocity causes a mean vertical convective mass flux (= cw for CO2, in standard notation). The eddy covariance technique neglects this mean convective flux and measures only the turbulent flux c w. Thus, when the net flux of CO2 is zero, the eddy covariance method indicates an apparent flux which is equal and opposite to the mean convective flux, i.e., c w = – c w. Corrections for the mean convective flux are particularly significant for CO2 because cw and c w are often of similar magnitude. The correct measurement of the net CO2 flux by eddy covariance techniques requires that the fluxes of sensible and latent heat be measured as well.  相似文献   

15.
The commonly measured value of in the relaxed eddy accumulationmethod of about 0.56is shown to arise from the non-Gaussiannature of turbulence. Fourth-orderGram–Charlier functions forthe two-dimensional probability distributionsof variation in the horizontal component of wind velocityand concentrations of water vapour, carbondioxide and methane with respect to thevertical component of wind velocity are used to examinethe value of .An analytical solution for ispresented in terms of fourth-order moments.Under mean conditions, this solution givesa value for of0.557. Variation of is shown to be controlledprimarily by the ratio of the mean ofc'w3 (where c'is relevant to the entity of interest andw' is vertical component of windvelocity) to the correlationcoefficient between the entity concentrationand vertical component of wind velocity.  相似文献   

16.
Measurements of the concentrations of carbonyl sulfide (COS) in the marine atmosphere were made over a period of two years in the southern Indian Ocean (Amsterdam Island, 37°50 S–77°31 E; March 1987–February 1988 and April 1989–February 1990). The mean atmospheric COS concentration for the whole period was 475±48 pptv (n=544). Atmospheric COS concentrations show no significant seasonal variation with a summer to winter ratio of 1.05. Taking into account the observed variability of the atmospheric COS concentration (10%), a value of 1.4 yr is estimated as a lower limit for the atmospheric COS lifetime. A comparison of the COS data at Amsterdam Island with those obtained in the Southern Hemisphere in the past 12 yr does not reveal any significant trend in the tropospheric background COS mixing ratio.  相似文献   

17.
Summary The seasonal and diurnal variations in the vertical component of the atmospheric electric field, air temperature, relative humidity and horizontal wind speed were studied using the surface data for the two periods (1936–40) and (1962–66) recorded at the tropical urban station, Colaba, Bombay (18°51N, 72°49E, 11 m ASL), located on the west coast of India.The atmospheric electric field during the latter period (1962–66) is significantly higher (up to 42.3%) than the earlier period (1936–40). This has been attributed to the enhanced particulate concentrations in the atmosphere. The increase noticed in the atmospheric electric field is a maximum during winter and minimum during the monsoon. The atmospheric electric field exhibited a marked semi-diurnal oscillation with peaks at 0900 LST and 2200 LST during winter, premonsoon and post-monsoon seasons of both the periods. During the monsoon season the double oscillation is not marked.The variations noticed in the surface air temperature and the relative humidity are in agreement with those observed in the atmospheric electric field. The horizontal wind speed showed a decrease which has been attributed to the surface roughness resulting from urbanization.With 7 Figures  相似文献   

18.
Wind characteristics in the lowest 340 m (agl) of the atmospheric boundary layer at Pune (18°32N, 73°51E, 559 m ASL) have been investigated using the pilot balloon wind observations obtained during the summer monsoon seasons of 1976, 1979 and 1980. Variations in the zonal and meridional components of wind at the surface, 40, 150 and 340 m (agl) have been described. Frequency distribution of the zonal component showed an unimodal character at the surface, which gradually approached a multimodal character at 340 m. The distribution pattern of the wind components was, by and large, normal. Spectral analysis of the wind components showed that the spectral energy was predominantly shared by 5–7 and 2–3 day periods.  相似文献   

19.
Daily measurements of atmospheric concentrations of dimethylsulfide (DMS) were carried out for two years in a marine site at remote area: the Amsterdam Island (37°50S–77°31E) located in the southern Indian Ocean. DMS concentrations were also measured in seawater. A seasonal variation is observed for both DMS in the atmosphere and in the sea-surface. The monthly averages of DMS concentrations in the surface coastal seawater and in the atmosphere ranged, respectively, from 0.3 to 2.0 nmol l-1 and from 1.4 to 11.3 nmol m-3 (34 to 274 pptv), with the highest values in summer. The monthly variation of sea-to-air flux of DMS from the southern Indian Ocean ranges from 0.7 to 4.4 mol m-2 d-1. A factor of 2.3 is observed between summer and winter with mean DMS fluxes of 3.0 and 1.3 mol m-2 d-1, respectively.  相似文献   

20.
Summary Spectral measurements were made of solar ultraviolet-B (UVB) irradiance at Sutton Bonington (52° 50N, 1° 15W) under cloudless skies using a Licor LI 1800 scanning spectroradiometer. The finite bandpass of the instrument and the steep shape of the UVB spectra caused overestimation of irradiance at short wavelengths. Spectra were corrected mathematically for these effects.The corrected spectra were compared to estimates of global UVB irradiance as a function of zenith angle and amount of ozone. Comparisons were made at 300 nm, 310 nm and 320 nm. Estimates were significantly greater (p = 0.05) than the measurements except at 320 nm where differences were not significant. The differences may have been the result of overestimation of UVB at short wavelengths, since some of the assumptions on which the estimates were based may not be valid for Sutton Bonington conditions.
Zusammenfassung Unter wolkenlosem Himmel wurden in Sutton Bonington (52° 50N, 1° 15W) mittels eines Licor LI 1800 Spektroradiometer-Scanners Spektralmessungen von Ultraviolett-B (UVB)-Strahlung durchgeführt. Die endliche Bandbreite des Instruments und der steile Anstieg der UVB-Spektren führten zu einer Überschätzung der Strahlung im kurzwelligen Bereich. Die Spektren wurden in dieser Hinsicht mathematisch korrigiert.Die korrigierten Spektren wurden mit den Schätzwerten der globalen UVB-Strahlung — als Funktion von Zenithwinkel und Ozonmenge — bei 300nm, 310nm und 320nm verglichen. Hiebei erwiesen sich die Schätzwerte wesentlich höher (p = 0,05) als die Meßwerte, nur bei 320nm waren die Unterschiede nicht signifikant. Die Unterschiede könnten aus der Überschätzung von UVB im kurzwelligen Bereich resultieren, da einige der Schätzungsvoraussetzungen auf die Bedingungen in Sutton Bonington nicht zutreffen dürften.

On leave from Department of Agronomy and Soils, Washington State University, Pullman, WA, U.S.A.

With 4 Figures  相似文献   

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