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1.
This study contains a comparative analysis of aerosol optical thickness (AOT) between numerical calculations obtained from the Navy Aerosol Analysis and Prediction System (NAAPS) model and direct observations from the AERONET robotic network and the Saharan Aerosol over WArsaw (SAWA) field campaign. AOT was calculated for 500 nm wavelength. The comparison shows underestimation of the total aerosol optical thickness simulated by NAAPS. The correlation coefficients between model and observation oscillates between 0.57 and 0.72. Results of seven-year (1998–2004) NAAPS simulation of aerosol components (sea salt, mineral dust, sulphate, and smoke) show large temporal and spatial variability of the aerosol optical thickness over Europe. The least polluted region is the Iberian Peninsula, while the highest aerosol burdens occurred in Central Europe, mostly due to anthropogenic sulphate particles. Finally, the analysis of mineral dust transport shows frequent episodes of Saharan dust inflow over Central Europe. There are about 20 days a year (4 days in May) when instantaneous AOT associated with mineral dust aerosol increases over 0.1.  相似文献   

2.
In this paper, optical measurements of aerosol properties made during a ship cruise from Poland to Antarctic Station in September and October 2006, and during the cruise back to Gdynia in April and May 2007 are described. A large gradient of pollution between the clear South Atlantic and the dusty North Atlantic was observed. The maximum of aerosol optical thickness at a wavelength of 500 nm reached 0.4 at 20°N in September 2006 and 0.3 at 40°N in May 2007, respectively. Strong Saharan dust transport is suggested as an explanation for the small values of Ångström exponent observed (values of 0.2 and 0.4 on these respective dates). On the Southern Hemisphere the aerosol optical thickness at 500 nm ranged from 0.05 to 0.2. Significant increases of the aerosol optical thickness were associated with strong wind and sea salt production. Good agreement was found when the in situ measurements of aerosol optical thickness were compared to satellite retrievals and modelling results.  相似文献   

3.
Aerosol optical properties have been studied for spring seasons when increased values of PM10 are registered. Measurements of aerosol optical properties were taken by collocated lidar and sun-photometers at Belsk, Poland, and Minsk, Belarus. A significant increase of registered aerosol optical thickness (AOT) was found during episodes with elevated PM10 concentrations. An increase of AOT at 1020 nm amounted to 50% in the case of Minsk and 18% in the case of Belsk, while an increase of AOT at 400 nm was 66% and 33%, respectively. We noted an increase of Ångström exponent by 6% at both stations and no significant increase of single scattering albedo. The LIDAR measurements together with NAAPS model results and backtrajectory analysis suggest that both the biomass burning products and the Saharan dust are responsible for increased PM10 concentrations and large AOT values during spring time. The smoke aerosol is transported over Central Europe mainly in the boundary layer, increasing both PM10 concentration and AOT. The dust aerosol transported in the free troposphere slightly affects the AOT values only. Statistically significant correlation between PM10 concentration and AOT was found during reporting period.  相似文献   

4.
Aerosol optical thickness (AOT) and seasonal variation of AOT over Belsk, Poland, in the UV wavelength range (310–380 nm) have been analysed using results of measurements by Brewer spectrophotometer No. 064 and Cimel sunphotometer data for the 2002–2007 period. The comparison of AOT derived from direct Sun measurements by Brewer spectrophotometer in the 310–320 nm range and retrieved from Cimel measurements at longer wavelengths shows good correlation (R = 0.96), with overestimation of retrieved values compared to the measured ones by about 6%. Basing on aerosol microphysical properties taken from almucantar retrievals and Mie theory, optical properties of aerosol in the UV range has been calculated. Analysis of seasonal variation of AOT at Belsk reveals two maxima: in April and July–August. Analysis of back-trajectories in conjunction with analysis of fire maps from Fire Information For Resource Management System shows that these seasonal maxima are connected with seasonal biomass burning in Eastern and Southern Europe.  相似文献   

5.
Sun-photometer measurements at Hefei, an urban site located in central East China, were examined to investigate the variations of aerosol loading and optical properties. It is found that aerosol optical thickness (AOT) keeps higher in winter/spring and gets relatively lower in summer/autumn. The large AOT in winter is caused by anthropogenic sulfate/nitrate aerosols, while in spring dust particles elevate the background aerosol loading and the excessive fine-mode particles eventually lead to severe pollution. There is a dramatic decline of AOT during summer, with monthly averaged AOT reaching the maximum in June and soon the minimum in August. Meanwhile, aerosol size decreases consistently and single scattering albedo (SSA) reaches its minimum in July. During summertime large-sized particles play a key role to change the air from clean to mild-pollution situation, while the presence of massive small-sized particles makes the air being even more polluted. These complicated summer patterns are possibly related to the three key processes that are active in the high temperature/humidity environment concentrating on sulfate/nitrate aerosols, i.e., gas-to-particle transformation, hygroscopic growth, and wet scavenging. Regardless of season, the increase of SSA with increasing AOT occurs across the visible and near-infrared bands, suggesting the dominant negative/cooling effect with the elevated aerosol loading. The SSA spectra under varying AOT monotonically decrease with wavelength. The relatively large slope arises in summer, reinforcing the dominance of sulfate/nitrate aerosols that induce severe pollution in summer season around this city.  相似文献   

6.
This paper investigates the annual cycle in aerosol optical thickness (AOT) and Angstrom exponent in Darwin, Australia, a coastal site in the Tropical Warm Pool where the major aerosol sources are biomass burning and sea salt. We have used radiometer measurements from the Tropical Western Pacific Atmospheric Radiation Measurement facility for the period March 2002–June 2003. Strong seasonal cycles in AOT and Angstrom exponent were observed, peaking during the burning season (May–November). Investigation of the spectral dependence of optical thickness showed that the Angstrom formula can be satisfactorily fitted to the AOT data during the burning season but not on summer and autumn afternoons due to the presence of sea salt aerosols.  相似文献   

7.

In this paper we have analyzed aerosol distribution over the Tibetan Plateau by using the global monthly mean satellite data of Stratospheric Aerosol and Gas Experiment II (SAGE II). The results are as follows: (1) Stratospheric aerosol optical depth can oscillate in the four seasons. It means that the aerosol optical depth is the thickest in winter and a little thinner in spring and the thinnest in summer and then a little thicker in autumn. We have found that the oscillation is caused by the oscillation of tropopause in different seasons. (2) Stratospheric aerosol comes mainly from sprays of volcano. After eruption of Mount Pinatubo aerosol optical depth in stratosphere over the Tibetan Plateau increases 10 times compared with before. (3) The characteristic of aerosol vertical distribution over the Tibetan Plateau is that there is an extremely high value at the altitude of 70 hPa. The most interesting thing is that the extremely high value can oscillate between 50 hPa and 100 hPa. We have verified that the oscillation is a unique characteristic over the Tibetan Plateau by comparing it with South China and North China. Then the radiative forcing and regional climate response over the Tibetan Plateau of aerosol are investigated. We have discovered such things as followed by: (1) The radiative forcing is positive because the parameterized aerosol optical depth is less than 0.14 which is the optical depth of the uniform background boundary aerosol layer. It is 0–3 W/m2 in January and 0–4 W/m2 in April and less than 3 W/m2 in July and 3–6 W/m2 in October. (2) Ground temperature rises 0.1–0.2 K in October which is the biggest increasing magnitude, and 0.01–0.02 in July which is the smallest one. It rises about 0.05-0.01 K in January and April. (3) Air temperature near the earth’s surface and the one at the altitude of 500 hPa rise too, but the increasing magnitude is less than the former one.

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8.
We present the results of a Schumann resonance monitoring campaign held at Lehta observatory, Karelia, Russia during July–August, 1998. Three electromagnetic (EM) field components were recorded simultaneously: the vertical electric and two orthogonal magnetic fields. This paper demonstrates advantages of the Poynting vector (PV) technique when studying the space–time dynamics of the worldwide thunderstorm activity from a single observatory. Analysis of the diurnal PV patterns revealed a night-time peak in African thunderstorm activity. This maximum occurs around 02:00–03:00 UT and reaches 1/3 of regular afternoon level. The Schumann resonance structure was discovered in the spectra of the wave arrival angles.  相似文献   

9.
Measurements of both broadband and spectral UV radiation have been carried out at Lhasa (29°40′N, 91°08′E, 3648 m above sea level) on the Tibetan Plateau, using a moderate bandwidth filter instrument (NILUV) and a Fixed Imaging Compact Spectrometer (FICS). In this paper, the erythemal UV dose rates deduced from broadband measurements during the period from 1 July 1996 to 10 December 1997 are presented. The observed highest erythemal UV dose rate is 500 (or 458) mW/m2 in July 1996 (or 1997), and the corresponding daily erythemal UV dose can reach up to 7.60 (or 7.00) kJ/m2 and 9.18 (or 8.96) kJ/m2, respectively, for the monthly mean and the monthly maximum. Comparisons with the UV levels at other locations at similar latitudes show that both the monthly mean and monthly maximum erythemal UV doses at Lhasa can be higher by a factor of 1.3–1.5 than those at San Diego (32°05′N, 117°1′W) in summer (from May to August), and exceed the corresponding values at Perth (32°0′S, 115°8′E) in the southern hemisphere summer (from November to February) by a factor of 1.2–1.4. Comparisons of both the broadband measurements and spectral measurements with the outputs of a discrete ordinate method (DOM) radiative transfer model have also been conducted. The results from the comparisons of broadband measurements with model outputs show that a 15, 11 and 10% agreement may be achieved around solar noon (with solar zenith angle smaller than 60°), respectively, for global irradiances in the 305, 320 and 340 mm channels, whilst the corresponding agreements are about 8 and 4% for the erythemal UV dose rate and the 340–305 nm ratio, respectively. The comparisons of the measured spectral irradiance with model calculations indicate that large discrepancies may appear at wavelengths shorter than 310 nm and longer than 380 nm. However, a 10% agreement may be generally achieved in UVA for solar zenith angle lower than 55°C. The corresponding agreement is about 20 and 5%, respectively, for UVB and the erythemal UV dose rate.  相似文献   

10.
In April 2010, volcanic ash from the Eyjafjalla volcano in Iceland strongly impacted aviation in Europe. In order to prevent a similar scenario in the future, a threshold value for safe aviation based on actual mass concentrations was introduced (2 mg m−3 in Germany). This study contrasts microphysical and optical properties of volcanic ash and mineral dust and assesses the detectability of potentially dangerous ash layers (mass concentration larger than 2 mg m−3) from a pilot’s perspective during a flight. Also the possibility to distinguish between volcanic ash and other aerosols is investigated. The visual detectability of airborne volcanic ash is addressed based on idealized radiative transfer simulations and on airborne observations with the DLR Falcon gathered during the Eyjafjalla volcanic ash research flights in 2010 and during the Saharan Mineral Dust Experiments in 2006 and 2008. Mineral dust and volcanic ash aerosol both show an enhanced coarse mode (>1 μm) aerosol concentration, but volcanic ash aerosol additionally contains a significant number of Aitken mode particles (<150 nm) not present in mineral dust. Under daylight clear-sky conditions and depending on the viewing geometry, volcanic ash is visible already at mass concentrations far below what is currently considered dangerous for aircraft engines. However, it is not possible to visually distinguish volcanic ash from other aerosol layers or to determine whether a volcanic ash layer is potentially dangerous (mass concentration larger or smaller than 2 mg m−3). Different appearances due to microphysical differences of both aerosol types are not detectable by the human eye. Nonetheless, as ash concentrations can vary significantly over distances travelled by an airplane within seconds, this visual threat evaluation may contribute greatly to the short-term response of pilots in ash-contaminated air space.  相似文献   

11.
An unusual intense dust storm occurred over North-East region of India on 17 March 2009, which was analyzed using multi-satellite data sets. Terra MODIS AOD550 showed high values on 17 March 2009 with low values of Angstrom exponent (α), suggesting coarse mode particle loading in the atmosphere. NCEP temperature and relative humidity anomalies showed high temperature and low humidity during March 2009. Dry weather conditions due to deficit rainfall during January–March 2009 and higher winds resulted in unusual dust storm over the region. Satellite observations of aerosol optical depth variations suggested increased aerosol loading in March 2009 due to dust storm.  相似文献   

12.
High-field torque-meter measurements of diamagnetic susceptibility anisotropy of a suite of samples of Carrara marble, axially shortened by amounts up to 50% at (1.5–3.0) · 108 Pa confining pressure and at 20–500°C (mainly 400°C), have been compared with optical measurements of preferred crystallographic orientation. A revised value for the susceptibility anisotropy of calcite has been obtained from studies of single crystals, and it has been shown to be almost independent of the state of intracrystalline plastic strain. From the measured anisotropy of calcite, quantitative comparison of optical and magnetic fabric measurements is possible. It is found that these measurements agree and the implications of the observed progressive development of fabric intensity with strain are discussed.  相似文献   

13.
This work estimates the Ångström turbidity coefficients and investigates the variation of the aerosol optical depth (AOD) in the Athens area, during different atmospheric conditions. The AOD is estimated in the wavelength band of 400–670 nm from direct-beam spectral irradiance measurements using ground-based instrumentation, during an experimental campaign performed in the period 22 September–1 October 2002. All data were collected under clear-sky conditions near the city center of Athens; the AODs were estimated relative to the local zenith to avoid the influence of the optical air mass. The study shows that the AOD is influenced by wind regime and traffic in the Athens area. The Angstrom's turbidity coefficients and the AOD values were found to be higher under the influence of South-sector winds compared to those from the North-sector. Under South-sector low winds, the pollutants are accumulated in the Athens basin. On the contrary, the North-sector winds clean the atmosphere.  相似文献   

14.
The spatial distribution of the aerosol optical depth during the northern winter, along the West coast of India and over the oceanic environments of the Arabian Sea and the South-West Indian Ocean (between 60°E–78°E and 15°N–20°S), has been investigated using co-ordinated ground-based and ship-borne measurements carried out during January–March of 1998 and 1999 under the Indian Ocean Experiment (INDOEX). In this paper apart from the expected results, an interesting observation is presented of enhanced aerosol activity in the mid Arabian Sea, far removed from the continent. Its implications are discussed.  相似文献   

15.
Solar irradiance, skylight, and aureole intensities were measured early in spring 1981 in Kensington, Australia. The aerosol optical thickness, the aureole intensities, and the scattering phase function at 5° suggest that scattering was due to aerosols of very small sizes. The estimates of the weighted aerosol mean square radius,p 2, seem to lead to the same conclusion.  相似文献   

16.
The lidar ratios at 500 and 1020 nm were derived from POM 01L sun-sky scanning photometer measurements taken at Belsk Geophysical Observatory (long. 20°47′, lat. 51°50′) in the period from 2002 to 2006. The most frequently occurring lidar ratio values for the study period are 50 sr and 30 sr at 500 nm and 1020 nm, respectively. Calculations of lidar ratios for summer and winter seasons have been made as well. Back trajectory analysis was also performed to final aerosol source of origin.  相似文献   

17.
A joint United States/Russian/French collaborative experiment was undertaken in March 1993 and March 1996. Projects LODE I and II (Lake Owens Dust Experiments) took place on the anthropogenically desertified playa (dry lakebed) and surrounding regions of Owens Lake, in east-central California. One of the five parts of Project LODE was to determine relationships between optical depth and flux of dust emitted from the dry lake. Project LODE II included subsequent dust plume measurements and size distributions obtained through April 1996, to further refine the flux measurements for distinct mineral aerosol source regions at Owens Lake. Size distributions of dust aerosol were determined and aerosol optical depths were calculated from sunphotometer solar extinction measurements taken downwind in plumes coming from the emissive areas of Owens Lake. This source was visually observed for 10 measured dust storms. The plume mass was calculated to be 1·5 × 109 g using ground-based measurements and ≥1·6 × 109 g from satellite data. Project LODE II results were found to be consistent with LODE I results for the south end of the playa, but flux values were found to be reduced for the northeastern portion of the playa by comparison. Vertical flux values estimated by sunphotometry were found to be consistent with values estimated via a micrometeorological method. Copyright © 1999 John Wiley & Sons, Ltd.  相似文献   

18.
In this study, long‐term discharge data and climate records, such as temperature and precipitation during 1977–2006, have been used to define basin climatic and hydrologic regimes and changes. Discharge analyses at four key gauging stations (Eagle, Stevens Village, Nenana, and Pilot Station) in the Yukon River Basin show that the runoff in the cold season (November to April) is low with small variations, whereas it is high (28 500–177 000 ft3/s; 810–5000 m3/s) with high fluctuations in the warm season (May to October). The Stevens Village Station is in the upper basin and has similar changes with the flow near basin outlet. Flow increases in May (61 074 ft3/s; 1729 m3/s) and September (23 325 ft3/s; 660 m3/s); and decreases in July (35 174 ft3/s; 996 m3/s) and August (6809 ft3/s; 193 m3/s). Discharge in May at the Pilot Station (near the basin outlet) shows a positive trend (177 000 ft3/s; 5010 m3/s). Daily flow analyses show high fluctuation during the warm season and very low flow during the cold season; the 10‐year average analyses of daily flow at Pilot Station show a small increase in the peak and its timing shifted to a little earlier date. The annual flow, average of 227 900 ft3/s (6450 m3/s) with high inter‐annual fluctuations, has increased by 18 200 ft3/s (or 8%; 520 m3/s) during 1977–2006. From 1977 to 2006, basin air temperature in June has increased by 3.9 °F (2.2 °C) and decreased by 10.5 °F (5.8 °C) in January. A strong and positive correlation exists between air temperature in April and discharge in May, whereas a strong and negative correlation relates August temperature and September discharge. Negative trend during 1977–2006 is observed for precipitation in June (0.6 in.; 15 mm) with a confidence over 93%. Precipitation in August and September has strong and positive correlations with discharge in September and October at basin outlet; the precipitation in other months has weak correlation with the discharge. The mean annual precipitation during 1977–2006 increased by 1.1 in. (or 8%; 28 mm), which contributes to the annual flow increase during the study period. Copyright © 2012 John Wiley & Sons, Ltd.  相似文献   

19.
Activity size distribution of the short-lived radon progeny in indoor air was measured continuously over several weeks. Two different measurement techniques were used: a direct measurement with a low-pressure Berner cascade impactor for attached fraction of 214Pb and 214Bi (≥100 nm) and an indirect determination based on measurement with a wire screen diffusion battery (unattached fraction 0.5–5 nm, 218Po, 214Pb). In parallel, the meteorological parameters like temperature, humidity were registered. Measured activity size distribution of radon progeny can be approximated by a sum of three log-normal distributions modes (nucleation, accumulation and coarse). The greatest activity fraction was adsorbed on aerosol particles in the accumulation size range (100–1000 nm) with activity median aerodynamic diameters (AMADa) and geometric standard deviations (GSD a ) values of 250–500 nm, and 1.5–3.5, respectively. The influence of the weather conditions on the activity of the accumulation particles was not significant. In contrast to the results of measurements a small but significant fraction of the radon progeny (average value 5 %) was attached to coarse particles (>1000 nm). This fraction varied between 0 and 10 %. On the other hand, although the amount of unattached activities not more 10 % of the total activity, but is considered to yield about 50 % of the total radiation dose. The mean thermodynamic equivalent diameters of 218Po and 214Pb were determined to be 1.28 and 1.30 nm with relative mean geometric standard deviations of 1.30 and 1.24, respectively. Based on the obtained results of radon progeny size distributions (attached and unattached), the total deposition fractions of the human lung were evaluated by using a lung deposition model.  相似文献   

20.
Atmospheric aerosol particle size distribution data derived from almucantar scans performed by the CIMEL sunphotometer at Belsk, Poland, in 2005 are used for the estimation of aerosol optical thickness (AOT) in the UV range by applying the Mie theory. The results obtained are compared with the direct Sun measurement data from the CIMEL sunphotometer and collocated Brewer spectrophotometer No. 064, as well as with AOT obtained by Angström extrapolation from the direct Sun measurements performed by the CIMEL sunphotometer in the visible range of wavelengths. Mean differences between calculated and measured values of AOT are up to about 8% in the UV-B range, which is close to the measurement uncertainty of the Brewer spectrophotometer and much less than that obtained by means of Angstrom extrapolation (over 24% in the UV-B range).  相似文献   

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