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1.
The composition and distribution of particles of native iron in eight sections of the Cretaceous-Danian sediments in the Caucasus, Crimea and Kopet Dagh were studied using thermomagnetic analysis up to 800°C. Iron particles are found in 330 of 571 tested samples, their percentage varies from 10−5 to 0.05%, and their distribution is bimodal. It was established that the Santonian sediments of the Caucasus and Kara-Kala are enriched with the iron particles; the upper boundary of these sediments is marked by a sharp drop in the iron content at approximately 84 Ma, which coincides with the upper boundary of the Dzhalal hyperchron. The variations in the Curie point of iron from 680°C up to 780°C reflect the fluctuations of the nickel admixture. A peak of the elevated iron content with nearly constant nickel of 5% was found in all studied sections, i.e., this is a global effect. The global pattern of the distribution and composition of the iron particles clearly indicates that their origin is associated with cosmic dust. At the same time, the particles of Ni-Fe alloy and pure nickel are very rare, and their concentration does not correlate with the content of iron particles. Apparently, there are very few Ni-Fe and pure nickel particles in cosmic dust, and, most likely, the particles of Ni-Fe alloy are mainly due to impact events.  相似文献   

2.
Thermomagnetic and microprobe analyses are carried out and a set of magnetic characteristics are measured for 25 meteorites and 3 tektites from the collections of the Vernadsky Geological Museum of the Russian Academy of Sciences and Museum of Natural History of the North-East Interdisciplinary Science Research Institute, Far Eastern Branch of the Russian Academy of Sciences. It is found that, notwithstanding their type, all the meteorites contain the same magnetic minerals and only differ by concentrations of these minerals. Kamacite with less than 10% nickel is the main magnetic mineral in the studied samples. Pure iron, taenite, and schreibersite are less frequent; nickel, various iron spinels, Fe-Al alloys, etc., are very rare. These minerals are normally absent in the crusts of the Earth and other planets. The studied meteorites are more likely parts of the cores and lower mantles of the meteoritic parent bodies (the planets). Uniformity in the magnetic properties of the meteorites and the types of their thermomagnetic (MT) curves is violated by secondary alterations of the meteorites in the terrestrial environment. The sediments demonstrate the same monotony as the meteorites: kamacite is likely the only extraterrestrial magnetic mineral, which is abundant in sediments and associated with cosmic dust. The compositional similarity of kamacite in iron meteorites and in cosmic dust is due to their common source; the degree of fragmentation of the material of the parent body is the only difference.  相似文献   

3.
Thermodynamic conditions (first of all, temperature) are the main dynamic factors in the transformation process of ferrous to ferric iron (TFFI). TFFI usually takes place within a temperature range of 473–843 K (most active at temperatures above 673 K) and does not require presence of the oxidizing agents above 673 K. Analysis of the chemical composition of different rocks and minerals indicates that only for some sedimentary rocks is the relative content of ferrous iron oxide less than its value in magnetite, and this value is minimal for oceanic sediments. The relative content of ferrous iron oxide in oceanic magmatic rocks exceeds this value in continental magmatic rocks and depends on the rate of rock cooling. An investigation of the role of the titanium oxide content of different rocks on stability of ferrous iron oxide against its transformation to ferric iron oxide shows that a significant correlation (r = 0.79) does exist between the relative content of ferrous iron oxide and ratio of TiO2/Fe2O3. Temperature within the solar nebula at location of the Earth was within the temperature range of the TFFI. During the Earth accretion and its early evolution, ferric iron oxide was unstable and most likely did not exist. The first magnetic minerals containing ferric iron could have appeared only after the Earth’s surface had cooled below ∼843 K. The formation of the first Algoma-type banded iron formations could be used as a marker of the Earth’s surface cooling below ∼843 K.  相似文献   

4.
This article considers the process of entry of cosmic substance into the Earth’s atmosphere and the further evolution of the formed extraterrestrial aerosol. It is shown that meteorite-derived aerosol generated in the atmosphere may affect the Earth’s climate in two ways: (a) particles of meteoric haze may serve as condensation nuclei in the troposphere and stratosphere; (b) charged meteor particles residing in the mesosphere may markedly change (by a few percent) the total atmospheric resistance and, thereby, affect the global current circuit. Changes in the global electric circuit, in turn, may influence cloud formation processes. The obtained results argue for the fact that the meteoric dust in the Earth’s atmosphere is potentially one of the important climate-forming agents. It is shown that the amount of interstellar dust in the Earth’s atmosphere is too small to have a considerable affect on atmospheric processes.  相似文献   

5.
Thermomagnetic and microprobe studies of native iron in the terrestrial upper-mantle hyperbasites (xenoliths in basalts), Siberian traps, and oceanic basalts are carried out. The results are compared to the previous data on native iron in sediments and meteorites. It is established that in terms of the composition and grain size and shape, the particles of native iron in the terrestrial rocks are close to each other and to the extraterrestrial iron particles from sediments and meteorites. This suggests that the sources of the origin of these particles were similar; i.e., the formation conditions in the Earth were close to the conditions in the meteorites’ parent bodies. This similarity is likely to be due to the homogeneity of the gas and dust cloud at the early stage of the solar system. The predominance of pure native iron in the sediments can probably be accounted for by the fact that interstellar dust is mostly contributed by the upper-mantle material of the planets, whereas the lower-mantle and core material falls on the Earth mainly in the form of meteorites. A model describing the structure of the planets in the solar system from the standpoint of the distribution of native iron and FeNi alloys is proposed.  相似文献   

6.
The data on the distribution of native iron particles in sediments yielded by thermomagnetic analysis are explored. It is shown that the accumulation of iron particles in sediments is statistically inversely linked with the rate of sedimentation and the frequency of geomagnetic reversals and statistically directly linked to the intensity of the geomagnetic field. These dependences highlight the predominance of cosmic iron particles in the studied sediments.  相似文献   

7.
Results of investigation of the cosmic matter in the transitional clay layer at the Cretaceous-Paleogene boundary in the Gams section, Eastern Alps, are presented. A great diversity of iron microspherules and particles of different morphologies, pure nickel spherules, awaruite (Fe3Ni) particles, and diamond crystals are discovered. Iron microspherules are also met in the overlying Paleocene deposits, but their diversity there is not great. The discovered metallic microspherules and particles are described, their chemical compositions are presented, and their origin is discussed.  相似文献   

8.
The thermomagnetic and microprobe analyses of sedimentary samples from DSDP 386, 387, 391A, and 391C boreholes in the northwestern Atlantic reveal the ubiquitous occurrence of particles of native iron. The concentrations of native iron are bimodal everywhere with the zero mode necessarily present. The nickel admixture in native iron forms two groups, one represented by pure iron and the comprising native iron with 5–6% Ni. The redeposition of iron particles manifests itself in the correlation between the concentrations of these particles and terrestrial minerals (magnetite), as well as in the equalization and reduction of the concentration of the iron particles. Pyrite and pyrrhotite are widespread in the studied sediments, and the distribution of native iron does not depend on the presence of pyrite (i.e., on redox conditions) in them. At the same time, the distributions of pyrite and particles of magnetite + titanomagnetite are inversely correlated, which can probably be accounted for by the partial dissolution of magnetite and titanomagnetite in the reducing conditions. The increased concentration of particles of volcanogenic homogeneous titanomagnetite is revealed in the volcanoclastic turbidites of the Oligocene and early and middle Miocene age at the base of the Bermuda Rise (borehole 386). The titanomagnetite composition is characteristic of the basalts of plume magmatism; it corresponds to the depth of the magmatic source in the interval of 50–25 km.  相似文献   

9.
The unit for detecting thermal neutrons, which makes it possible to study variations in cosmic rays of the interplanetary and geophysical origin, has been created at the high altitude cosmic ray station (3340 m above sea level) near the Earth’s crust fault. It has been established that variations in thermal neutrons are of the same nature as high-energy variations registered with a neutron supermonitor in the absence of seismic activity. The flux of thermal neutrons from the Earth’s crust during seismic activity in December 2006 has been registered for the first time. The flux value is higher than the background level by 5–6%. The method for detecting the flux of thermal neutrons from the Earth’s crust with the simultaneous registration of high-energy neutrons has been proposed.  相似文献   

10.
The changes of magnetic susceptibility(κ) are correlated with those of corresponding sedimentological, geochemical, mineralogical and biological results, which verifies thatκ can be taken as one of the environmental proxies. However, usually the exact origin of magnetic signal is poorly understood, and is difficult to relate with the environmental evolution. Magnetic properties of material derived from the catchment and sedimentary environment may affect the accumulation, preservation, or authigenesis and diagenesis of magnetic minerals. In the Lake Hulun region in Inner Mongolia, it is found that muddy sediments, deposited during high water level period (corresponding to humid climate), have comparatively highκ values. In contrast, the sandy sediments, deposited during low water level period (corresponding to arid climate), have lowκ values. Detailed rock magnetic investigation confirms that detrital magnetite derived from volcanic rocks in the catchment exists in both muddy and sandy sediments. During high water level period, secondary ferrimagnetic iron sulphide was produced in muddy sediments under relatively reductive conditions. Ferrimagnetic iron sulphide, coexisting with detrital magnetite, predominates the magnetic properties of muddy sediments, resulting in increasingκ. This paper reveals the significance of authigenic ferrimagnetic iron sulphide produced after sediment deposition.  相似文献   

11.
59Ni in 0.4 g of nickel from deep-sea sediments was measured with an extremely low-level X-ray spectrometer. The obtained specific activity was (5.9 ± 1.8) × 10?2 dpm/kg sediments. The59Ni activity induced by proton and alpha particle irradiation in outer space can be estimated as 300 dpm/kg dust. Hence, the content of extraterrestrial dust in deep-sea sediments was not more than 200 ppm.  相似文献   

12.
The paper continues a cycle of petromagnetic investigations of epicontinental deposits at the Mesozoic-Cenozoic (K/T) boundary and is devoted to the study of the Gams section (Austria). Using thermomagnetic analysis, the following magnetic phases are identified: goethite (T C = 90–150°C), hemoilmenite (T C = 200?300°C), metallic nickel (T C = 350–360°C), magnetite and titanomagnetite (T C = 550–610°C), Fe-Ni alloy (T C = 640–660°C), and metallic iron (T C = 740–770°C). Their concentrations are determined from M(T). In all samples, ensembles of magnetic grains have similar coercivity spectra and are characterized by a high coercivity. An exception is the lower coercivity of the boundary clay layer due to grains of metallic nickel and iron. With rare exceptions, the studied sediments are anisotropic and generally possess a magnetic foliation, which indicates a terrigenous accumulation of magnetic minerals. Many samples of sandy-clayey rocks have an inverse magnetic fabric associated with the presence of acicular goethite. The values of paramagnetic and diamagnetic components in the deposits are calculated. According to the results obtained, the K/T boundary is marked by a sharp increase in the concentration of Fe hydroxides. The distribution of titanomagnetite reflects its dispersal during eruptive activity, which is better expressed in the Maastrichtian and at the base of the layer J. The along-section distribution of metallic iron, most likely of cosmic origin, is rather uniformly chaotic. The presence of nickel, most probably of impact origin, is a particularly local phenomenon as yet. The K/T boundary is not directly related to an impact event.  相似文献   

13.
Interstitial water samples from the Guatemala Basin and the coast of Baja California have been analyzed for manganese, iron, copper, nickel and nitrate. The data provide a systematic look at changes in trace metal diagenesis proceeding from red clay to highly reducing nearshore sediments.In red clay sediments, the nitrate concentrations suggest that only aerobic respiration is occurring. Manganese and iron are below detection. Nickel concentrations remain the same as in bottom seawater but copper shows a pronounced maximum just at the sediment/water interface. Proceeding to hemipelagic sediments, denitrification becomes increasingly important and manganese and iron remobilization occur in the sediments.The linear manganese and nitrate profiles suggest regions of production or consumption separated by zones of diffusion. This differs from the conventional picture of a continuous series of reactions within the sediments. Manganese reduction always occurs before iron reduction. The pore water nickel correlates well with manganese in these sediments, suggesting that nickel is associated with MnO2 in the solid phase. The pore water flux ratio of manganese and nickel agrees well with the ratio in solid phase authigenic oxides. Copper still displays a core top concentration maximum as well as a second maximum associated with the remobilized manganese. The calculated ratio of the Cu/C flux ratios support the argument for copper remobilization during organic carbon oxidation. Comparison of the upward and downward diffusive fluxes with the rate of copper buried by sedimentation shows that at least half of the copper buried must be of diagenetic origin and less than 25% of the copper reaching the sediments is buried.  相似文献   

14.
Andrew Lane 《Ocean Dynamics》2005,55(5-6):541-548
The development and application of a Lagrangian particle-tracking model to simulate sediment transport in the Mersey Estuary (UK) is described. Each of the particles (up to a million in total) is advected horizontally by the 3-D tidal currents. Related vertical movements are: (1) downwards by settlement at a prescribed velocity w s and (2) both upwards and downwards by a distance related to the vertical eddy diffusivity. In a novel departure from traditional practice, where initial distributions of surficial sediments are specified, all particles are introduced at the seaward boundary of the model. Provenance studies indicate surficial sediments are overwhelmingly of marine origin. For the predominant fine sediments, ‘cyclical convergence’ in suspended sediment concentrations is approximated after about two spring-neap tidal cycles. Comparisons are shown between the suspended sediment concentrations and net deposition rates computed by this model against observed values and earlier computations utilising both 1-D and 3-D Eulerian models. While all of these results are in broad agreement, the flexibility of the Lagrangian approach for simulating flocculation, consolidation and mixed sediments illustrates its future potential.  相似文献   

15.
Results of petromagnetic studies of epicontinental sediments at the Mesozoic-Cenozoic (K/T) boundary are generalized. Their analysis shows that an abrupt rise in the concentration of iron hydroxides is confined to this boundary. Their concentration is highest at the base of the boundary layer and drops by more than two times at it top. As distinct from iron hydroxides, other magnetic minerals were variously accumulated, depending on their origin and local deposition conditions of terrigenous material (for example, accumulation of particles of metallic iron and nickel, aerial transport of titanomagnetite grains of volcanic origin, and deposition of terrigenous particles of magnetite and ilmenite).  相似文献   

16.
The work reported here confirms the existence of (largely) unmelted micrometeorites in sediments from seasonal lakes on the Greenland ice sheet. Approximately1/3 of the dark and irregularly shaped particles selected from disaggregated sediments had sufficient contents of Ne to permit measurement of isotopic compositions. The sediments consisted of a mixture of biologically derived contaminants and minor amounts of terrestrial minerals and extraterrestrial fragments. Although terrestrial mineral contamination varied by a factor of 20 for the two different sediments, a yield of 1000 cosmic particles/kg of wet cryoconite was found for both samples. The isotopic compositions of the Ne in both rounded and irregular (25% of total) particles that contained enough gas to measure were non-terrestrial, plotting in a field defined by solar wind (SW), solar energetic particle (SEP) and spallation. Exposure ages ranged from < 0.5 Ma to 20 Ma, consistent with previous estimates from10Be and26Al measurements of larger spherules removed from similar sediments. Comparison of the Ne data with compositional-morphological data demonstrates the general validity of criteria previously used to identify extraterrestrial particles; however, two particles identified as of probable terrestrial origin by three independent, experienced meteorite petrologists were shown by the Ne data to be extraterrestrial and probably extraterrestrial, respectively. Future studies of Greenland micrometeorites are outlined and improved collection techniques are discussed.  相似文献   

17.
This paper reports the first Raman study of a representative set of interplanetary dust particles (IDPs) belonging to different infrared spectral classes. Six different groups of Raman spectra can be discerned among the 20 IDPs studied. All particles, except the four belonging to group 6, exhibit the Raman signature of poorly crystallized carbonaceous material. The degree of “disorder” of this material, as evidenced by the width and relative strength of the two first-order Raman bands at 1360 relative cm−1 and 1600 relative cm−1, varies among particles from different spectral groups (increasing from group 1 to group 5). The most ordered carbonaceous material, with an estimated upper crystallite size limit of 60Å(group 1), is found in particles that tend to show deuterium depletions and that have infrared spectra characteristic of olivines. Raman spectra of particles belonging to groups 2, 3 and 4 (none of which have FTIR spectra characteristic of olivines) show clear evidence for the presence of carbonaceous material, although the “degree of order” is noticeably less than for carbons in group 1 particles. All seven particles with documented deuterium enrichments [1,2] fall into these three intermediate Raman groups. This relationship of the hydrogen isotopic compositions with the Raman data suggests different carbonaceous carrier phases for deuterium depletions and enrichments. Particles from Raman groups 5 and 6, whose spectra show little or no evidence for the presence of carbonaceous material, show deuterium abundances within the range of terrestrial rocks. In general, there is no obvious relationship between Raman groups and infrared classes which are based on the 10 μm absorption band due to silicates. In part, this is due to the fact that no Raman bands for silicates are seen, although silicates are known to be present from infrared and analytical electron microscopic measurements. The lack of silicate bands indicates that the silicate grains are coated with and/or imbedded in a carbonaceous material, which is presumably the reason that the particles look black in the visible. Several particles also show broad visible laser-induced photoluminescence, which is also probably produced by a carbonaceous component.  相似文献   

18.
Magnetic signature of different vegetation species in polluted environment   总被引：2，自引：0，他引：2  
Detailed magnetic study on vegetation samples from several strongly polluted and clean sites in Bulgaria is carried out in order to evaluate suitability of different species as passive dust collectors in magnetometry. From each location, available species among lichens, mosses, poplar leaves, dandelion, needles have been sampled. Magnetic susceptibility calculated on mass-specific basis shows wide variability between diamagnetic signal up to 846 × 10−8 m3/kg. Lichens and mosses are found to be the species, showing magnetic signals with the strongest contrast between clean and polluted environment. The main magnetic phase is magnetite-like according to the results from thermomagnetic analysis of susceptibility on magnetic extracts. Scanning electron microscopy (SEM) microphotographs reveal the presence of abundant particulate matter on vegetation surface both with anthropogenic (spherules) and lithogenic origin. Magnetic grain size deduced by the ratio of saturation remanent magnetization (SIRM) and mass-specific magnetic susceptibility (χ) and coercivities (Bc and Bcr) suggest that different species accumulate preferentially small SD-like grains from pollution emissions. Contrasting relationship of the ratio of anhysteretic remanent magnetization (ARM) and χ for polluted vs clean sites deduced by needles and lichens may be related to transformation of the accumulated dust particles within lichens’ tissue. This finding indicates that the exact species used as biological dust collector is of importance when studying spatial grain size distribution of magnetic dust particles. Pilot study on polycyclic aromatic hydrocarbons (PAH) content and its relation to magnetic parameters shows good correspondence between high levels of PAHs and high SIRM values for locations affected by non-ferrous industrial production.  相似文献   

19.
The possible mechanism by which cosmic rays affect the formation of neutral water droplets and ice crystals in the Earth’s atmosphere has been considered. This mechanism is based on changes in atmospheric transparency and vertical temperature distribution. It has been indicated that a change in the optical thickness for visible and IR radiation by several percents, which can take place when cosmic-ray particles penetrate into the atmosphere, results in a change in the temperature vertical distribution, affecting the growth of water droplets, concentration of active condensation nuclei, and the formation of ice particles. This mechanism makes it possible to explain the correlation between the intensity of galactic cosmic rays at low altitudes and the absence of this correlation at middle altitudes.  相似文献   

20.
The results of magnetic and microprobe studies of the rock sequences in the Mezmaiskaya cave at the unique multilayer Paleolithic site are discussed. The magnetic properties of rocks are analyzed for 17 layers (upwards from layer 4 to layer 1\1) dated from over 73 ka ago to recent times. The rocks of layer 1C (Early Upper Paleolithic, ∼38 ka) are found to have the highest magnetic susceptibility (K) (up to 2500 × 10−6 SI), which is related to the intensive activity of [Homo sapiens]. The minimum K corresponds to the rocks of layer 2, which is overlain by layer 1D. The sizes of magnetic grains vary throughout the rock section. The largest grains are found in the middle part of the section in the Middle Paleolithic layers 2B3, 2B2, 2B1, 2A, and 2. The superparamagnetic fraction is identified in all layers. This fact supports the view that the cave was open as early as the formation of layer 4. According to the thermomagnetic data on the saturation magnetization and the temperature curves of magnetic susceptibility, magnetite is the main carrier of the rock magnetization; some samples contain iron hydroxides. Samples with iron sulfides (pyrite) are abundant. The study of the hysteresis parameters of rocks showed that the question on whether sulfide-bearing rocks are suitable for reliable paleomagnetic determinations requires further laboratory research into the origin of magnetite in the rocks. The chemical composition of rocks composing layer 2B3 and layers 1D (∼39 ka) and 2B1 (∼45 ka), in which the presence of volcanic ash has been previously established according to the presence of volcanic glass, was determined by detailed microprobe analysis. A wide variety of chemical elements (up to 18 items) was recognized in layers 1D and 2B1. The iron, titan, chrome, manganese content, and concentrations of other components vary from grain to grain. The microprobe analysis of samples from layers 1D and 2B1 revealed a set of magnetic particles with compositions characteristic of volcanic rocks, which supports the ash origin of these layers. Layer 2B3 is established not to be volcanic ash. The results on the volcanic glass in the rocks of layers 1D and 2B1 were published by Golovanova and her colleagues in Current Anthropology in October 2010 [Golovanova et al., 2010].  相似文献   

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