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1.
Springtime measurements of NOx, ozone, PAN,J(NO2), and other compounds were made near Ny-Ålesund,Svalbard (78°54N, 11°53E), in 1994 and Poker Flat,Alaska (65°08N, 147°29W), in 1995. At Svalbard medianmixing ratios for PAN and NOx of 237 and 23.7 pptv,respectively, were observed. The median mixing ratios at Poker Flat for PANand NOx were 79.5 and 85.9 pptv, respectively. These data areused to estimate thermal PAN decomposition using several differentapproaches. At Svalbard PAN decomposition was very small, while at PokerFlat up to 30 pptv/h PAN decomposed. At both sites the NOx/PANratio increased with temperature between –10 and 20°C implyingthat PAN decomposition is an important NOx source. In-situozone production was calculated from the measured NO, NO2,O3, J(NO2), and temperature data, using thesteady state assumption Median ozone production was 605 pptv/h at PokerFlat, and one order of magnitude smaller at Svalbard during the daytime.Only at Poker Flat could a direct influence on the diurnal ozone cycle beobserved from in-situ production. These results imply that PAN decompositionis a major source of NOx in the high latitude troposphere, andthat this contributes to the observed spring maximum in surface ozone.  相似文献   

2.
Since April 1986, measurements of the CO2 concentration in the surface air have been conducted at the Meteorological Research Institure (MRI, 36°04 N, 140°07 E, 25 m above sea level) in Tsukuba, located 50 km northeast of Tokyo, Japan. The CO2 data measured over times between 11:00 Japan Standard Time (JST) and 16:00 JST (C N ) were considered to be representative of the air (within a few ppmv) in the planetary boundary layer. To evaluate the representative CO2 level on a spatial scale larger than that of the C N record, the CO2 data with hour-to-hour variation less than 1 ppmv were selected (C P ). Comparison of these data with those of Ryori (39°02 N, 141°50 E), a continental station operated by the Japan Meteorological Agency, indicates that the C P record provides a representative CO2 level in the air on spatial scales of at least a few hundred kilometers.The C N record allows an investigation of the internanual changes in photosynthesis/respiration against changes in climatological parameters. Within a small temperature anomaly (ca.±1 °C) respiration is sensitive to the temperature change, while photosynthesis is less sensitive. When the temperature anomaly is large, however, photosynthesis and respiration tend to be competitive.  相似文献   

3.
Weekly bulk aerosol samples collected at Funafuti, Tuvalu (8°30S, 179°12E), American Samoa (14°15S, 170°35W), and Rarotonga (21°15S, 159°45W), from 1983 through most of 1987 have been analyzed for nitrate and other constituents. The mean nitrate concentration is about 0.11 g m–3 at each of these stations: 0.107±0.011 g m–3 at Funafuti; 0.116±0.008 at American Samoa; and 0.117±0.010 at Rarotonga. Previous measurements of mineral aerosol and trace metal concentrations at American Samoa are among the lowest ever recorded for the near-surface troposphere and indicate that this region is minimally affected by transport of soil material and pollutants from the continents. Consequently, the nitrate concentration of 0.11 g m–3 can be regarded as the natural level for the remote marine boundary layer of the tropical South Pacific Ocean. In contrast, over the tropical North Pacific which is significantly impacted by the transport of material from Asia and North America, the mean nitrate concentrations are about three times higher, 0.29 and 0.36 g m–3 at Midway and Oahu, respectively. The major sources of the nitrate over the tropical South Pacific are still very uncertain. A very significant correlation between the nitrate concentrations at American Samoa and the concentrations of 210Pb suggests that transport from continental sources might be important. This continental source could be lightning, which occurs most frequently over the tropical continents. A near-zero correlation with 7Be indicates that the stratosphere and upper troposphere are probably not the major sources. A significant biogenic source would be consistent with the higher mean nitrate concentrations, 0.16 to 0.17 g m–3, found over the equatorial Pacific at Fanning Island (3°55N, 159°20W) and Nauru (0°32S, 166°57E). The lack of correlation between nitrate and nss sulfate at American Samoa does not necessarily preclude an important role for marine biogenic sources.  相似文献   

4.
A two-dimensional atmospheric boundary-layer model is applied to the Nanticoke region on the northern shore of Lake Erie (80 ° 03W and 42 ° 50N) to simulate numerically the observed wind and temperature profiles. In general, the profiles predicted by the model agree reasonably well with the observed profiles.  相似文献   

5.
This study examines the statistical properties of the concentration derivative, , for a dispersing plume in a near-neutrally stratified atmospheric surface layer. Towards this goal, the probability density function (pdf) of , and the conditional pdf of given a fixed concentration level, , have been measured. These pdfs are found to be modeled well by a generalizedq-Gaussian (gqG) distribution with intermittency exponent,q, equal to 0.3 and 3/4, respectively. These results highlight the strong intermittency effect (patchiness) of the small-scale concentration eddy structures in the plume. The distribution of time intervals between successive high peaks in the squared derivative process, x2, is found to be well approximated by a power-law distribution, implying that occurrences of these high peaks are much more clustered than would be predicted by a Poisson or shot-noise process. The results are used to improve models for the joint pdf of and , and for the expected number of upcrossings per unit time interval of a fixed concentration level that have been proposed by Kristensenet al. (1989). The predictions of the improved models are in accord with observations, and suggest that the intercorrelation between and must be explicitly incorporated if good estimates of the upcrossing intensity are to be obtained.  相似文献   

6.
Summary A classification scheme for cold surges occurring along the Front Range of the Rocky Mountains has been developed using NMC surface and upper air data. A separation is seen in the data between cases with parent anticyclones that moved from Canada south into the United States (Northern type) and those which moved from the Eastern Pacific Ocean east into the central US (Western type). The Northern surges are further broken down into three types, A, B and B, when the degree of southward motion of the anticyclone and the leading edge of the cold air is considered. An anticyclone movement south of 40°N distinguishes type A, while anticyclone tracks remaining north of 40°N characterize types B and B. The leading edge of the surge (the surge line) associated with the type A anticyclone travels south of 25N, while the type B anticyclones produce two distinct surge line movements, one remaining north of 25°N and the other moving south of 25°N. It is not possible to break down the Western surges into distinct types. As a rule, the anticyclones associated with Western surges remain between 50°N and 30°N, with the surge line moving south to 18°N on average.Though the classification scheme is developed in a relatively subjective manner, the statistical robustness of the scheme is verified through application of the nonparametric Mann-Whitney test. Results of the test clearly provide support for the division of the surges that was obtained.With 16 Figures  相似文献   

7.
Summary A time series and extreme value analysis of maximum precipitation for distinct time intervals from 10 minutes to 1 day have been deduced for the observatory Zagreb-Gri ( = 45°49 and = 15°59,H s = 157 m) for the period between 1908 and 1985. The Spearman rank correlation test revealed that the short-term precipitation maxima series for the time intervals of 10 to 30 minutes and 8 to 24 hours indicate no significant trend for the 95 percent probability level. The 40-minute to 4-hour precipitation maxima exhibited an increaese in recent time. Annual maximumt-minute precipitation was estimated using the Gumbel distribution for sets of data gradually prolonged with 10-year steps towards the past. The ratios (q) of maximum precipitation estimates for the shorter periods and of estimates for the reference period (1908–1985) have been calculated. Their positions according to the confidence interval on the reference estimates were determined. Confident extreme value estimates could be obtained using at least the 50–60 year data series.With 3 Figures  相似文献   

8.
The total ozone content in the atmosphere was determined from the multichannel photometer observations of direct solar radiation made in the urban environment at Pune (18° 32 N, 73° 51E, 559 m ASL) and Sinhagad hill station (18° 22N, 73° 45E, 1305 m ASL) during March 1980-February 1982. The total ozone content of the atmosphere was computed making use of the differential absorption of solar radiation due to ozone at 0.4 and 0.6 m wavelengths in the Chappuis band. The values of the ozone data obtained from the photometer observations at Pune and Sinhagad were compared with the corresponding ozone data obtained from the Dobson spectrophotometer located at Pune. Values of ozone obtained by the photometric method were found to be smaller by 8–18% than the Dobson values when Vigroux's absorption coefficients were used. Similarly, when the absorption coefficients of Inn and Tanaka (1953) were used, the ozone values obtained by the photometric method were smaller by 4–14% than the Dobson values. The ozone values at the hill station obtained from the photometric method were in better agreement (5%) with the Dobson values.  相似文献   

9.
This paper presents a new reconstruction of the mean annual temperature obtained from a high altitude pollen sequence in equatorial Africa (3°28S, 29°34E, 2240 m). It has been achieved with an extended modern African reference data set by adding spectra from 228 new sites and using another selection for pollen taxa. The purpose of this paper is to test how the obtained temperature value depends upon the availability of modern analogues. The results are in good agreement with those previously published, reinforcing the validity of the method. The mean standard error is reduced by 0.3°C. The mean temperature for the Holocene appears + 1.4°C warmer than the present and the last glacial maximum (25-18 kyrs BP) cooling is better specified at – 3 ± 1.9° C, a conservative value, more consistent with reconstructed sea surface temperature in the equatorial ocean.Contribution to Clima Locarno - Past and Present Climate Dynamics; Conference September 1990, Swiss Academy of Sciences — National Climate Program  相似文献   

10.
Surfaces fluxes, turbulent kinetic energy and Flux Richardson number are calculated for three typical sea breeze days characterizing three types of sea breeze onset at an inland station Kharagpur (22°21 N, 87°19 E), 80 km inland, one of the sites for MONTBLEX (MONsoon Trough Boundary Layer EXperiment), in India. The sea breeze onset is associated with a decrease in momentum and heat fluxes and an increase in moisture flux. The turbulent kinetic energy shows quite a significant value even in the late afternoon. The surface layer becomes nearly stable even before sunset, due to the passage of the sea breeze.  相似文献   

11.
Observations of tidal currents in lat. 71° 01 S, long. 10° 55 W indicate that a semi-diurnal tidal wave progresses towards the WSW, that is, parallel to the main direction of the barrier. ForM 2 the cotidal hour appears to be about 7h, in good agreement with the value 6.7h, that is derived from observations of the atmospheric pressure. Furthermore, the current measurements indicate that the ratio(K 1+O1)/(M2+S2) is large, perhaps as large as 2.5.
Zusammenfassung Beobachtungen der Gezeitenströmungen in 71° 01 S und 10° 55 W lassen erkennen, daß eine halbtägige Gezeitenwelle gegen WSW, also parallel zur Hauptrichtung der Eisbarriere, wandert. FürM 2 scheint das Flutstundenintervall etwa 7 Stunden zu betragen und damit gut zu dem Wert von 6,7 Stunden zu stimmen, der aus Beobachtungen des Luftdrucks abgeleitet wird. Ferner lassen Strömungsmessungen erkennen, daß der Quotient(K 1+O1)/(M2+S2) mit etwa 2,5 groß ist.
Résumé Des observations des courants de marée, faites à 71° 01 S et 10° 55 W, montrent qu'une vague de marée semi-diurne progresse en direction WSW, ce qui est parallèle à la direction principale de la limite de la banquise. PourM 2 l'heure cotidale paraît être de 7h environ, ce qui correspond assez bien avec la valeur de 6.7h déduite des observations de la pression atmosphérique. En outre les mesures du courant indiquent que le quotient(K 1+O1)/(M2+S2) est assez grand et comporte environ 2.5.

With 1 Figure.  相似文献   

12.
Free tropospheric measurements of ozone, peroxyacetylnitrate andprecursors (CO, NMHC) that were made within the framework of the EUROTRACsub-project TOR (Tropospheric Ozone Research) between 1990 and 1995 at theGAW station Izana, Tenerife (28°18N, 16°30W) arediscussed. The average annual cycles reveal the importance of transport fromnorthern mid-latitudes and the role of photo-chemistry. According toair-mass trajectories, which were supplied to us from AEROCE(Atmosphere/Ocean Chemistry Experiment), transport from northernmid-latitudes is associated with high precursor concentrations in winter,whereas ozone concentrations in winter are not much influenced by transportpatterns, suggesting a rather uniform distribution over the northern part ofthe Northern Hemisphere around mean value of 43 ± 5 ppb. In summer,high ozone concentrations of up to 90 ppb are often encountered duringtransport from north, while the levels of precursors are much lower than inwinter, because of photochemical destruction. Trajectories from southerlylatitudes and the Sahara usually have the lowest ozone concentrationsassociated with them.  相似文献   

13.
Observations made with a monostatic sodar and from a 120 m instrumented tower have been used to study the variations in the atmospheric boundary layer at Tarapur (19° 50 N, 72° 41 E) during the solar eclipse of February 16, 1980. Atmospheric instability was reduced below normal values during the eclipse but the atmosphere at no time became stable.  相似文献   

14.
Wind characteristics in the lowest 340 m (agl) of the atmospheric boundary layer at Pune (18°32N, 73°51E, 559 m ASL) have been investigated using the pilot balloon wind observations obtained during the summer monsoon seasons of 1976, 1979 and 1980. Variations in the zonal and meridional components of wind at the surface, 40, 150 and 340 m (agl) have been described. Frequency distribution of the zonal component showed an unimodal character at the surface, which gradually approached a multimodal character at 340 m. The distribution pattern of the wind components was, by and large, normal. Spectral analysis of the wind components showed that the spectral energy was predominantly shared by 5–7 and 2–3 day periods.  相似文献   

15.
In early 1982 a station capable of sampling atmospheric trace gas constituents on a continuous basis was established at Palmer Station, Anvers Island, adjacent to the Antarctic Peninsula (64° 46S 64° 04W). Sampling operations began about 1 February 1982. This is an initial report on this station, its location, equipment and general research objectives along with some initial sampling results. The constituents being measured and recorded were: ozone, methane, carbon dioxide, carbon monoxide, CCl3F (fluorocarbon-11), CCl2F2 (fluorocarbon-12), carbontetrachloride, methylchloroform, nitrous oxide, and Aitken nuclei (CN). Data storage, data processing, and sampling system control is handled by a Hewlett-Packard 85 system. Preliminary analyses of about the first 20–22 months of data are presented and show not only the expected long-term trends but also shorter period concentration cycles that seem to be related to synoptic meteorology.  相似文献   

16.
Flow distortion by supporting structures   总被引：3，自引：0，他引：3  
During the 1976 International Turbulence Comparison Experiment, a number of participants found significant values of upflow over the horizontal support arm of the sensor used. For example, the Japanese sonic anemometer reported an average upflow of 2.4 °. By means of model experiments and fitting to a potential flow solution, it is predicted that the horizontal support would introduce an upflow of 0.5 °. Further model experiments with a full sonic anemometer model plus associated structures predicted an upflow of 2.2 °, in reasonable agreement with the observed result. The need for extreme care in the exposure of turbulence sensors is emphasized. The theory is capable of predicting the error incurred in the various turbulence parameters, such as uw, and these error equations bear a close similarity to those normally used in applying a tilt correction.  相似文献   

17.
Wind velocities within a plant canopy are much more strongly skewed than those of the air flow above. We have examined the governing Eulerian equations for the velocity products u i, u j uk using data from a wind tunnel study with an artificial canopy consisting of an array of 5 cm lengths of monofilament fishing line, and from measurements in corn (Zea mays L).Simple parameterizations for pressure-velocity correlations, and for the quadruple velocity products allowed reasonably accurate calculations of the third moments using measured profiles of the mean velocity, variance and covariance fields. Comparisons of individual terms in the rate equations for ovu i, u j u krevealed that diffusion (from above) and mean shear were most important in creating large skewness in the canopy. A drag term also contributed but was of lesser importance. These terms were balanced by return-to-isotropy and a turbulence interaction term. A quasi-Gaussian approximation considerably underestimated the magnitude of the fourth moments within the canopy.  相似文献   

18.
Vertical columns of HF, HCl, HNO3, ClONO2, N2O, ClO and COF2 were measured at Harestua, Norway (60.22° N, 10.75° E, Elevation 600 a.s.l.) beginning on 24 November 1994 and concluding on 1 May 1995 during Phase-III of the SESAME (Second European Stratospheric Arctic and Mid-latitude Experiment) measurement campaign. The vertical columns of HCl, HNO3 and ClONO2 measured on 81 days were compared with columns calculated by the 3-D Cambridge model SLIMCAT. In addition the results were also interpreted by comparison with a photochemical trajectory model. Good agreement was seen for HCl while the nitrogen compounds showed larger discrepancies, especially for ClONO2. Evidence for chlorine activation was seen with 65% reduction of the chlorine reservoirs (HCl + ClONO2) while the levels of ClO were greatly enhanced. Interpretation of the loss with the trajectory model indicated condensation of chlorine on PSCs. The vertical column ratio of COF2 and HF was measured to 0.21 outside the vortex and a factor of two lower inside. The recovery of ClONO2 was seen to be much faster than that of HCl in the early spring.  相似文献   

19.
Measurements of the concentrations of carbonyl sulfide (COS) in the marine atmosphere were made over a period of two years in the southern Indian Ocean (Amsterdam Island, 37°50 S–77°31 E; March 1987–February 1988 and April 1989–February 1990). The mean atmospheric COS concentration for the whole period was 475±48 pptv (n=544). Atmospheric COS concentrations show no significant seasonal variation with a summer to winter ratio of 1.05. Taking into account the observed variability of the atmospheric COS concentration (10%), a value of 1.4 yr is estimated as a lower limit for the atmospheric COS lifetime. A comparison of the COS data at Amsterdam Island with those obtained in the Southern Hemisphere in the past 12 yr does not reveal any significant trend in the tropospheric background COS mixing ratio.  相似文献   

20.
Summary Spectral measurements were made of solar ultraviolet-B (UVB) irradiance at Sutton Bonington (52° 50N, 1° 15W) under cloudless skies using a Licor LI 1800 scanning spectroradiometer. The finite bandpass of the instrument and the steep shape of the UVB spectra caused overestimation of irradiance at short wavelengths. Spectra were corrected mathematically for these effects.The corrected spectra were compared to estimates of global UVB irradiance as a function of zenith angle and amount of ozone. Comparisons were made at 300 nm, 310 nm and 320 nm. Estimates were significantly greater (p = 0.05) than the measurements except at 320 nm where differences were not significant. The differences may have been the result of overestimation of UVB at short wavelengths, since some of the assumptions on which the estimates were based may not be valid for Sutton Bonington conditions.
Zusammenfassung Unter wolkenlosem Himmel wurden in Sutton Bonington (52° 50N, 1° 15W) mittels eines Licor LI 1800 Spektroradiometer-Scanners Spektralmessungen von Ultraviolett-B (UVB)-Strahlung durchgeführt. Die endliche Bandbreite des Instruments und der steile Anstieg der UVB-Spektren führten zu einer Überschätzung der Strahlung im kurzwelligen Bereich. Die Spektren wurden in dieser Hinsicht mathematisch korrigiert.Die korrigierten Spektren wurden mit den Schätzwerten der globalen UVB-Strahlung — als Funktion von Zenithwinkel und Ozonmenge — bei 300nm, 310nm und 320nm verglichen. Hiebei erwiesen sich die Schätzwerte wesentlich höher (p = 0,05) als die Meßwerte, nur bei 320nm waren die Unterschiede nicht signifikant. Die Unterschiede könnten aus der Überschätzung von UVB im kurzwelligen Bereich resultieren, da einige der Schätzungsvoraussetzungen auf die Bedingungen in Sutton Bonington nicht zutreffen dürften.

On leave from Department of Agronomy and Soils, Washington State University, Pullman, WA, U.S.A.

With 4 Figures  相似文献   

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