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1.
Fluvial processes, especially rates of floodplain accretion, are less well understood in the wet tropics than in other environments. In this study, the caesium-137 (137Cs) method was used to examine the recent historical sedimentation rate on the floodplain of the Wainimala River, in the basin of the Rewa River, the largest fluvial system in Fiji and the tropical South Pacific Islands. 137Cs activity in the floodplain stratigraphy showed a well-defined profile, with a clear peak at 115 cm depth. Our measured accretion rate of 3.2 cm year−1 over the last ca. 45 years exceeds rates recorded in humid regions elsewhere. This is explained by the high frequency of tropical cyclones near Fiji (40 since 1970) which can produce extreme rainfalls and large magnitude floods. Since the beginning of hydrological records, large overbank floods have occurred every 2 years on average at the study site. The biggest floods attained peak flows over 7000 m3 s−1, or six times the bankfull discharge. Concentrations of suspended sediments are very high (max. 200–500 g l−1), delivered mainly by channel bank erosion. In the future, climatic change in the tropical South Pacific region may be associated with greater tropical cyclone intensities, which will probably increase the size of floods in the Rewa Basin and rates of floodplain sedimentation.  相似文献   

2.
The Portil lagoon is a natural freshwater reservoir located at the southwest of Spain, near the coast. In its surroundings an important tourist complex has been developed since the earlier 1970s. This has resulted in increased loads of nutrients, specially during summer months. In order to evaluate the impact from humans on the lagoon caused by anthropogenic activities, we have determined vertical profiles of excess 210Pb and 137Cs in a sediment core taken from its bottom. Vertical profile of excess 210Pb seems to indicate that the sediment core was affected by large-scale mixing processes. Nevertheless this possibility was ruled out based on the shape of the 137Cs vertical distribution after modelling the 137Cs profile considering large-scale mixing. The chronology developed from 210Pb and 137Cs has allowed us to calculate the temporal evolution of the mass sedimentation rate during the last century. This mass sedimentation rate increased in 1973: from 0.08(2) g cm-2 a-1 in the period 1900-1973 to 0.17(5) g cm-2 a-1 in the period 1973-1995. This increase could be related to land-movements in the drainage area and to permitted sewage inputs into the lagoon, both with its origin in the growing/running of the surrounding tourist complex.  相似文献   

3.
Seven cores were collected from different sediment zones of tidal flats at Xinyanggang in north Jiangsu province in August 2007. Sediment grain-size distribution and radioisotopes of 137Cs and 210Pb analysis were carried out for these cores. Sediment rates of the cores and radioisotopes distribution in surface sediment in different zones of the tidal flat were calculated from the 137Cs and 210Pb activities in sediments cores. The results indicated that each tidal zone had experienced different evolution phases, hydrological dynamics in the tidal flats made the grain-size of the surface sediment change gradually. 137Cs and 210Pb activities on the superficial layer of the cores varied spatially and the reason was discussed. On tidal flats, the fluctuation of 137Cs and 210Pb activities in the cores reflected the special sedimentary characteristics. Vegetation affects the grain-size distribution and the vertical profiles of 137Cs and 210Pb in the upper depths. 137Cs and 210Pb chronology got the comparable average sediment rates on the tidal flat. The characteristics of 137Cs and 210Pb in the cores reflected various depositional dynamical environments in different tidal zones and gave information on the different evolvement phases of the tidal zones. Based on the information of grain-size distribution, texture of the cores, sediment rates and topography, the evolution lines of the tidal flat were reconstructed.  相似文献   

4.
210Pb geochronologies should be validated with independent tracers such as 137Cs. In the cases with constant 210Pb activity in the topmost sediments, the presence of a distinct 137Cs peak within the 210Pb plateau has been used as a definitive demonstration of acceleration (increase in the sedimentation rate in recent years) versus fast mixing. Nevertheless, some limitations can be identified in the use of semiquantitative arguments, and a global understanding of the whole 137Cs activity profile is then required. Particularly, the incomplete mixing within the top sediment zone (described through the Incomplete Mixing Zone model) can explain quantitatively and simultaneously the 137Cs peak and the flattening in the 210Pb activity profile. This is demonstrated using selected examples from literature data. Thus, measured constant 210Pb activities in the top 6 cm of a sediment core from Lake Zürich. Nevertheless, they found 7Be only in the uppermost layer, the distinct 137Cs maximum at 6 cm depth, and undisturbed varves. The fast mixing seemed then opposed to common sense. The constant rate of supply model shows acceleration and it adequately matches the position of the 1963 137Cs peak. Nevertheless it fails to explain the whole 137Cs profile when handling time series of 137Cs atmospheric deposition. Finally, it is shown how the incomplete mixing of the activity (through the pore water) over a certain mass depth at the top sediment, with a finite value of the mixing coefficient, can quantitatively explain the whole activity versus mass depth profiles of 137Cs and 210Pb, and the presence of 7Be only in the uppermost sediment layer. A further validation of these ideas is presented from other literature data.  相似文献   

5.
Most mathematical models for radiometric dating of recent sediments are particular solutions of a unique physical problem: the advective?Cdiffusive transport of a particle-bound radiotracer within a sediment profile that undergoes accretion. Regardless of the particular assumptions about fluxes, sedimentation rates and the diffusion term, all models assume ideal deposition as a boundary condition at the sediment water interface, i.e. new radioactive input will be deposited above the previously existing material. In sediments with very high porosities, this assumption may be unrealistic, because a fraction of the incoming flux may penetrate rapidly through the connected pore spaces. This process will be referred to as non-ideal deposition. This paper reviews evidence from literature data, discusses the basic processes involved, and establishes the mathematical basis to incorporate non-ideal deposition into one-phase radiometric dating models, as depth-distributed local sources. Through analytical and numerical solutions, this work demonstrates that such penetration patterns can explain excess 210Pb subsurface maxima, often observed in sediment cores, as well as penetration of 137Cs to depths greater than expected from sedimentation rates and diffusion. These ideas are illustrated using examples from the literature in which sediment porosities were >90?%. Implications for radiometric dating include: (1) spurious accelerations in sedimentation rate inferred when applying the constant rate of supply model, and (2) erroneous chronologies, developed when using the maximum depth at which 137Cs can be measured as a chronostratigraphic marker.  相似文献   

6.
Global fallout is the main source of anthropogenic radionuclides in the Mediterranean Sea. This work presents 137Cs, 239+240Pu and 241Am concentrations in the water column in the southwest Alboran Sea, which was sampled in December 1999. A sediment core was taken at 800 m depth in the area (35°47′ N, 04°48′ W). 210Pb, 226Ra, 137Cs and 239+240Pu specific activities were measured at multiple depths in the core for dating purposes. 137Cs and 239+240Pu profiles did not show defined peaks that could be used as time markers, and they extended up to depths for which the 210Pb-based constant rate of supply (CRS) dating model provided inconsistent dates. These profiles can be useful to test dating models, understood as particular solutions of a general advection–diffusion problem, if the time series of radionuclide inputs into the sediment is provided. Thus, historical records of depth-averaged 137Cs and 239+240Pu concentrations in water, and their corresponding fluxes into the sediment, were reconstructed. A simple water-column model was used for this purpose, involving atmospheric fallout, measured distribution coefficient (k d) values, and a first-estimate of sedimentation rates. A dating model of constant mixing with constant sedimentation rate was applied successfully to three independent records (unsupported 210Pb, 137Cs and 239+240Pu), and provided the objective determination of mixing parameters and mass sedimentation rate. These results provide some insight into the fate of atmospheric inputs to this marine environment and, particularly, into the contribution from the Chernobyl accident.  相似文献   

7.
Sediment cores collected from eight lakes along the western coast of Svalbard as part of a project investigating atmospheric pollution and environmental change in Arctic regions were dated radiometrically using natural (210Pb) and artificial (137Cs and 241Am) fallout radionuclides. At four sites the sedimentation rates were relatively uniform, and in consequence the 210Pb dates were relatively unambiguous. At the remaining sites there were irregularities in the 210Pb activity versus depth profiles, indicating significant variations in the net sediment accumulation rate during the past 120 years. At these sites, there were significant differences between 210Pb dates calculated using the two standard simple dating models, constant rate of supply (CRS) and constant initial concentration (CIC). In most cases, stratigraphic dates based on the 137Cs and 241Am records supported use of the CRS model, though at one site (Ossian Sarsfjellet) the CIC model appeared more appropriate. The irregularities in the 210Pb records were mainly caused by episodes of accelerated sedimentation due, for example, to inwash or slump events, though at some sites there appears to have been a systematic increase in sediment accumulation rates in recent decades. Sediment accumulation rates were generally lower at the northern sites, and higher at the more southerly locations. Mean sediment accumulation rates varied by an order of magnitude, ranging from 0.002 to 0.050 g cm−2 y−1 (0.02–0.10 cm y−1). 210Pb fluxes measured from the core inventories were mostly in the range 34–80 Bq m−2 y−1 typical of Arctic sites. Much higher values, recorded at two sites (Birgervatnet and Daltjørna), may be due to significant inputs from the catchments during spring thaw.  相似文献   

8.
We examine sediment distribution patterns in seven Florida lakes and discuss implications for paleolimnological studies of shallow, subtropical lakes. The study lakes are highly productive and should exhibit thick organic sediment deposits, but organic sediments are often grossly lacking because basins are shallow, and frequent mixing, lack of stratification, and warm temperatures lead to breakdown of organic material.Organic sediment distribution patterns are highly variable. We observe three types of distribution patterns. When organic sediments are abundant, there may be (1) uniform sediment distribution. In lakes lacking organic sediments, there are (2) distribution to deeper areas if present, or (3) distribution to peripheral areas and embayments when deep waters are absent. We advocate the use of systematic mapping surveys to locate optimal coring sites for paleolimnological studies of shallow, wind-stressed lakes. Because numerous factors affect diagenesis and sediment redistribution, sediment abundance and location are not predictable. Sediment chronologies may be discontinuous and disturbed even in accumulation zones. The extent to which sedimentary records are discontinuous or disturbed is not quantifiable in any practical manner. 210Pb and 137Cs radioisotopic profiles provide qualitative evidence of the degree of stratigraphic disturbance. Total excess 210Pb inventories show that sediments are focused into depositional zones when sediment distribution is uneven. Excess 210Pb inventories are not informative about the completeness of sedimentary profiles unless small inventories suggest discontinuous sedimentation or erosional events. We present examples of disturbed and undisturbed profiles, and discuss how we use radioisotopic and geochemical evidence, and multiple cores to assess stratigraphic continuity.Journal Series No. R-04815 of the Florida Agricultural Experiment Station.  相似文献   

9.
Reconstructing recent limnological history often relies on lead-210 dating to accurately ascribe a chronology to a sediment profile. In Lake Okeechobee, Florida, a large, shallow subtropical lake that may experience severe mixing, multiple dating methods are required to confirm that conformable sedimentation has been preserved and that the assumptions of the 210Pb method are satisfied. This study uses stratigraphic profiles of heavy metals, 137Cs, PCBs and pollen as independent dating markers to validate the sediment chronology as determined by 210Pb for three cores from the central mud zone of the lake. Unsupported 210Pb and most dating markers show distinct concentration/depth profiles, suggesting that the sediments have not been severely mixed for at least the last 75 years. Onset and maximum activity of the radioisotope 137Cs in the cores coincides with the 210Pb-dated interval of 1945–1970. This agrees well with the known timing of atmospheric deposition of 137Cs that resulted from above-ground nuclear testing during late 1940s until 1963. Sediment core profiles of atmospherically deposited metals such as Zn and Pb, which reflect regional increases during industrialization and decreases after regulation in the 1970s, exhibit expected concentration increases and peaks coinciding within 5–15 years of the predicted 210Pb dates. Uranium, a contaminant in some phosphate fertilizers, shows large concentration increases at core depths dated to be about 1950 by 210Pb, matching the intensification of agriculture after WWII. PCBs, which are expected to peak in the early 1970s, were measured in one core, and the observed peak corresponds to a 210Pb date of about 1960. Pollen makers were unable to verify specific events, but increases in disturbance taxa and declines in native types correspond generally with the expected dates assigned by 210Pb dating. Conformity between the 210Pb defined dates and independent markers of < ±15 years confirm that Lake Okeechobee sediments do preserve a sequential and reliable stratigraphic history of the lake, useful for reconstructing past limnological conditions.  相似文献   

10.
A combination of tephrochronology and 14C, 210Pb, and 137Cs measurements provides a robust chronology for sedimentation in Upper Klamath Lake during the last 45 000 years. Mixing of surficial sediments and possible mobility of the radio-isotopes limit the usefulness of the 137Cs and 210Pb data, but 210Pb profiles provide reasonable average sediment accumulation rates for the last 100–150 years. Radiocarbon ages near the top of the core are somewhat erratic and are too old, probably as a result of detrital organic carbon, which may have become a more common component in recent times as surrounding marshes were drained. Below the tops of the cores, radiocarbon ages in the center of the basin appear to be about 400 years too old, while those on the margin appear to be accurate, based on comparisons with tephra layers of known age.Taken together, the data can be combined into reasonable age models for each site. Sediments have accumulated at site K1, near the center of the basin, about 2 times faster than at site CM2, on the margin of the lake. The rates are about 0.10 and 0.05 cm/yr, respectively. The chronological data also indicate that accumulation rates were slower during the early to middle Holocene than during the late Holocene, consistent with increasing wetness in the late Holocene.  相似文献   

11.
Sediment cores collected from six sites in Lake Baikal as part of an extensive investigation of sediment records of recent environmental change were dated radiometrically by 210Pb. Although the results obtained were in some respects comparable to those obtained by previous 210Pb studies, there were some significant differences. Most notably, a core from abyssal depths in the centre of the middle basin appeared to record at least wo major episodes of rapid sedimentation, possibly caused by turbidity currents. All cores, including those from the North Basin, contained significant records of weapons test fallout 137Cs, though these were of little chronological value due to the long residence time of 137Cs in the water column. Models and budgets for sediment and radionuclide transport through Baikal are presented and used to help validate the 210Pb results.  相似文献   

12.
Seven cores were collected from different sediment zones of tidal flats at Xinyanggang in north Jiangsu province in August 2007. Sediment grain-size distribution and radioisotopes of 137Cs and 210Pb analysis were carried out for these cores. Sediment rates of the cores and radioisotopes distribution in surface sediment in different zones of the tidal flat were calculated from the 137Cs and 210Pb activities in sediments cores. The results indicated that each tidal zone had experienced different evolution phases, hydrological dynamics in the tidal flats made the grain-size of the surface sediment change gradually. 137Cs and 210Pb activities on the superficial layer of the cores varied spatially and the reason was discussed. On tidal flats, the fluctuation of 137Cs and 210Pb activities in the cores reflected the special sedimentary characteristics. Vegetation affects the grain-size distribution and the vertical profiles of 137Cs and 210Pb in the upper depths. 137Cs and 210Pb chronology got the comparable average sediment rates on the tidal flat. The characteristics of 137Cs and 210Pb in the cores reflected various depositional dynamical environments in different tidal zones and gave information on the different evolvement phases of the tidal zones. Based on the information of grain-size distribution, texture of the cores, sediment rates and topography, the evolution lines of the tidal flat were reconstructed.  相似文献   

13.
江苏北部潮滩沉积物中~(137)Cs和~(210)pb的分布特征(英文)   总被引：1，自引：0，他引：1  
Seven cores were collected from different sediment zones of tidal flats at Xin-yanggang in north Jiangsu province in August 2007. Sediment grain-size distribution and radioisotopes of ~(137)Cs and ~(210)Pb analysis were carried out for these cores. Sediment rates of the cores and radioisotopes distribution in surface sediment in different zones of the tidal flat were calculated from the ~(137)Cs and ~(210)Pb activities in sediments cores. The results indicated that each tidal zone had experienced different evolution phases, hydrological dynamics in the tidal flats made the grain-size of the surface sediment change gradually. ~(137)Cs and ~(210)Pb activities on the superficial layer of the cores varied spatially and the reason was discussed. On tidal flats, the fluctuation of ~(137)Cs and ~(210)Pb activities in the cores reflected the special sedimentary characteristics. Vegetation affects the grain-size distribution and the vertical profiles of ~(137)Cs and ~(210)Pb in the upper depths. ~(137)Cs and ~(210)Pb chronology got the comparable average sediment rates on the tidal flat. The characteristics of ~(137)Cs and ~(210)Pb in the cores reflected various depositional dynamical environments in different tidal zones and gave information on the different evolvement phases of the tidal zones. Based on the information of grain-size distribution, texture of the cores, sediment rates and topography, the evolution lines of the tidal flat were reconstructed.  相似文献   

14.
Traditional techniques used to assemble information on rates of erosion and soil redistribution possess many important limitations. As a result, the use of environmental radionuclides, and more particularly 137Cs measurements, has attracted increasing attention in recent years as a means of obtaining spatially distributed information on rates of erosion and deposition. The application of the 137Cs approach is, however, hampered in some areas of the world where 137Cs inventories are low and the low concentrations of 137Cs found in soils and sediments cause problems for laboratory analysis. These problems will increase as time progresses due to the radioactive decay of the existing inventory, most of which was deposited as fallout ca. 40 years ago. This contribution explores the potential for using another fallout radionuclide, namely unsupported 210Pb, as an alternative to 137Cs, in the small (63 km2) Upper Kaleya catchment in southern Zambia where 137Cs inventories are already very low. The approach employed with unsupported 210Pb is similar to that used for 137Cs, although the essentially constant fallout of unsupported 210Pb through time means that the resulting estimates of erosion and soil redistribution rates reflect a longer period of time (ca. 100 years rather than ca. 40 years). The estimates of erosion and deposition rates derived from the unsupported 210Pb measurements are used to construct typical sediment budgets for the three main land-use types in the Upper Kaleya catchment, namely, commercial cultivation, communal cultivation and bush grazing. The results obtained from the unsupported 210Pb are compared with equivalent results based on 137Cs measurements provided by a previous investigation undertaken in the study catchment. The two sets of results are highly consistent. The study reported confirms the viability of using unsupported 210Pb as an alternative to 137Cs in this environment and demonstrates that conjunctive use of both radionuclides can provide additional information on the erosional history of a study area.  相似文献   

15.
Sediment focusing in six small lake basins is inferred from sedimentary radionuclide profiles. The activities of137Cs and9+240Pu do not decrease to zero above the sub-surface maximum but tail off gradually. Similar behavior is observed in the sediments of three lakes for134Cs and60Co, which were added only to the lake. This upward tailing is not caused by bioturbation or erosion from the watershed. Sediment focusing is the likely cause, further substantiated by inventories in deep sediments of9+240Pu and210Pb that are twice as high as expected from atmospheric fallout. Inventories in deep sediments of137Cs are in several cases lower than expected from atmospheric fallout, and cannot be explained by hydraulic flushing from the lakes, as this would require unreasonable flushing rates. The low137Cs inventories and the sedimentary profiles of the137Cs/9+240Pu ratio are consistent with137Cs removal from the water column by boundary scavenging to shallow sediments. The profiles and inventories of all three nuclides could be reproduced with a simple three box model, assuming focusing of shallow sediments (50–60% of total sediment area) to deep sediments with a rate constant of 5–10% yr–1.This is the seventh of a series of papers to be published by this journal following the 20 th anniversary of the first application of210Pb dating of lake sediment. Dr P. G. Appleby is guest editing this series.  相似文献   

16.
We present 137Cs profiles for three low lying coastal lagoons in Southwest England that show a decline in activity with sediment depth. 137Cs inventories are lower than expected by comparison with local reference inventories despite the fact that sampling was undertaken in the deep-water zone of each lake where sediment and 137Cs focusing would be expected. At all three locations, lake sediment 7Be and unsupported 210Pb (210Pbun) inventories are not significantly lower than the local reference inventory. 137Cs inventories in the study cores range from 38 to 95% of local reference inventories. The standing water level and mud: water interface at two sites are below maximum tide level and, at all three sites, salinity increases significantly in the water columns between low and high tide and in the pore waters of the underlying sediments. We suggest that the difference in hydrostatic pressure between sea level and standing water levels in the lagoons forces salt water up through the sediment column and that monovalent cations (especially Na+ and K+) replace 137Cs on exchange sites leading to the upward migration and loss of 137Cs. Rising sea levels may therefore contribute to remobilisation and release of 137Cs to the aquatic environment from the sediments of coastal lagoons.  相似文献   

17.
Post-depositional mobility of137Cs,239+240Pu and210Pb was assessed in six small lake basins by comparing sedimentary nuclide profiles with their known fallout history. Laminae couplets, when present, were determined to be varves because the137Cs and239+240Pu 1963 fallout peaks are present in laminae couplets corresponding to years 1962–1964. There is no evidence of mobility of210Pb, because 1) mass accumulation rates based on210Pb agree with those based on137Cs and239+240Pu peak depths and with those based on varve counts, and 2)210Pb ages agree with varve ages. Significant mobility of137Cs is evident from the penetration of137Cs to depths 15–20 cm deeper than239+240Pu. Deep penetration of137Cs in spite of a sharp gradient below the peak is interpreted by a numerical model to suggest that137Cs is present in two distinct forms in these sediments, 67–82% as an immobile form and 18–33% reversibly adsorbed with a K d of approximately 5000. The profiles can be interpreted equally well assuming a small portionof the total137Cs was present as an extremely mobile phase (K d 5000) in the months to years following peak fallout, slowly becoming more strongly adsorbed. High NH 4 + concentrations in porewaters may enhance diffusion of the mobile form of137Cs, but not of the immobile form of137Cs that defines the sharp gradient. Mobility of137Cs is likely also enhanced by the low clay content and the high porosity of these sediments. Thus the first detection of137Cs in the sediments cannot automatically be assumed to correspond to a date of 1952 (initial testing of thermonuclear weapons), although the depth of the peak can be assumed to correspond to 1963 (the year of maximum fallout from testing of thermonuclear weapons).239+240Pu is a more reliable sediment chronometer than137Cs because it is significantly less mobile.This is the sixth of a series of papers to be published by this journal following the 20 th anniversary of the first application of210Pb dating of lake sediments. Dr P.G. Appleby is guest editing this series.  相似文献   

18.
Tectonically active coastal regions of the world recently have been suggested to supply the bulk of sediment from land to the oceans. Seabed sampling on the continental shelf and in coastal embayments of the north-east Gulf of Alaska (Alsek River to Prince William Sound) was performed to examine the temporal and spatial variability of sediment accumulation in a mountainous coastal setting. Cores of varying lengths (30–300 cm) were collected at 84 stations to provide information on sedimentary processes using radiochemical (210Pb and 137Cs) techniques. Four types of 210Pb activity profiles were observed, dominantly reflecting steady-state sediment accumulation. However, nonsteady-state profiles also were measured, resulting in part from episodic deposition near glacier-fed rivers and on the Copper River Delta. Sediment accumulation rates in the eastern half of the study area are highest at midshelf depths (≈100 m) (≥10 mm yr?1) and near rivers draining the Bering Glacier (≈20 mm yr?1). On the Copper River Delta, sediment accumulation rates are highest for the delta front (> 20 mm yr?1) and decrease westward along the sediment dispersal route. Total annual sediment accumulation is 90–140×106 tons yr?1 on the shelf in the study area. Annual sediment accumulation for the total marine environment in the study area (including Icy and Yakutat Bays) exceeds 250×106 tons yr?1, potentially making this region the largest sink for sediment in North America. Spatial patterns in sediment accumulation on the shelf are similar between centennial and Holocene time-scales, reflecting the dominance of the Copper River and Bering and Malaspina glaciers as sediment sources. Temporal variability in accumulation rates between centennial and Holocene time-scales exists for portions of the study area near fiords and demonstrates the considerable changes that occur in sediment supply during glacial advances and retreats.  相似文献   

19.
In this study, we combined grain size and geochemical analyses with radioisotope analysis of lead-210 (210Pb), caesium-137 (137Cs) and radiocarbon (14C) ages to reconstruct the sedimentation history of two urbanised coastal lagoons in south-east Australia. Towradgi and Fairy Lagoons were both found to exhibit slow initial sedimentation of less than 1 mm year−1 prior to anthropogenic influences. Land clearing in the catchments increased runoff and erosion in the creeks feeding into the estuaries, and has resulted in progradation of fluvial material into the estuarine systems with a marked increase in sedimentation to between 2 and 7 mm year−1. The upper 20–50 cm of the sediment column in both lagoons contained elevated concentrations of heavy metals such as Pb, Cu, Ni and Zn. This pollution trend was found to be consistent with the history of industrialisation and urbanisation in the region, which expanded rapidly post World War 2. The total metal concentrations were consistent with other urbanised/industrialised estuaries around the world. Despite the fairly disturbed nature of these coastal lagoons, the use of 210Pb, 137Cs and 14C dating in combination with bulk geochemical analyses allowed detailed reconstruction of sedimentation history.  相似文献   

20.
Low-background gamma counting: applications for210Pb dating of sediments   总被引：1，自引：0，他引：1  
Sediment cores from three lakes were dated with210Pb using a constant rate of supply (CRS) model. We used low-background gamma counting to measure naturally occurring levels of210Pb,226Ra, and137Cs in sediment samples because sample preparation is simple and non-destructive,226Ra activity provides a direct measure of supported210Pb activity for each sample analyzed, and137Cs activity may provide an independent age marker for the 1962–1963 peak in atmospheric fallout of this radionuclide. In one core supported210Pb activity was estimated equally well from226Ra activity of each sampling interval or from the mean total210Pb activity of constant activity samples at depth. Supported210Pb activity was constant with depth in this core. In a short freeze core, determining226Ra activity of every sample proved advantageous in estimating supported210Pb activity because supported210Pb activity could be estimated from210Pb measurements only at the deepest sampling interval. Supported210Pb activity estimated from226Ra activity also yielded more precise estimates of highly variable sedimentation rates. In the third core226Ra activity exceeded210Pb activity at the top of the core and varied 20 fold with depth. This high input of226Ra in disequilibrium with210Pb is attributed to recent erosion of radium-bearing materials in the drainage basin. These data invalidate the assumption that supported210Pb activity is constant in sediment cores and can be estimated from the mean total210Pb activity at depths where210Pb activity is constant. We recommend using gamma counting or another independent assay of226Ra to validate the assumption of constant supported210Pb activity in sediment cores if there is reason to expect that226Ra activity varies with depth.This is the fourth of a series of papers to be published by this journal following the 20 th anniversary of the first application of210Pb dating of lake sediments. Dr. P.G. Appleby is guest editing this series.  相似文献   

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