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1.
Hydrometric and isotopic (oxygen-18) observations were used to delineate the runoff processes operating in several headwater catchments on the Precambrian Shield of Canada. The catchments comprise patches of conifer forest situated on thin soils among areas of lichen-covered granitic bedrock. Horton overland flow occurred from the lichen-bedrock areas in all precipitation events that exceeded 4–6 mm. Runoff from the forest stands occurred mainly as subsurface stormflow, but in some instances saturation overland flow was observed. The occurrence of saturation overland flow was controlled by the topography of the bedrock beneath the forest soils. The area contributing runoff and the pathway by which water was conveyed to the catchment outflow switched from the open lichen-bedrock areas producing overland flow on the rising limb of the storm hydrograph to the forest stands contributing subsurface stormflow on the recession limb of the hydrograph. The areal extent and position of the landscape units in the basin were important to the rate and magnitude of stormflow production. Runoff was generated from the catchments only during and immediately after snowmelt and/or rainfall events. The catchments were dry and/or frozen for about 70% of the year.  相似文献   

2.
Despite considerable research performed on forested catchments in the Ouachita Mountains of Oklahoma and Arkansas, little information on hydrological processes in operation is available. Based on catchment physical characteristics, subsurface flow was thought to be an important hydrological process in the region. Therefore, this study was undertaken to determine the occurrence, rates, timing and volumes of subsurface flow, and to estimate the importance of subsurface flow as a streamflow generating process. Subsurface flow was collected from three hillslope sites on a 7.7 ha forested catchment. Hillslope sites drained through natural seepage faces located near stream channels. Subsurface flow was collected from three depths at each hillslope site, below the litter layer, below the a horizon, and within the B horizon (Bt21). Subsurface flow occurred and was measured during 11 of 31 rainfall events. Subsurface flow responded rapidly to the initiation of and to changes in intensity of rainfall at all depths. the rapid response was indicative of flow through soil macropores. B horizon subsurface flow commenced within 10 to 180 min of the initiation of rainfall. Multiple linear regression showed that the volume of subsurface flow generated during a given storm was directly related to rainfall depth and a 7-day antecedent precipitation index used to represent antecedent water content. About 67 per cent of the total subsurface flow collected during the study was produced in one large storm under wet antecedent conditions. the storm was equal to the 2-year, 24-hour storm for the region. Measured subsurface flow volumes were extended to the watershed scale to provide estimates of catchment-wide contributions to streamflow. It was estimated that subsurface flow contributed from 1 to 48 per cent of total quickflow measured at the catchment outlet. Based on the timing of subsurface flow, it was estimated that subsurface flow May, contribute up to 70 per cent of quickflow before and soon after peak flow.  相似文献   

3.
Abstract

A physically-based hillslope hydrological model with shallow overland flow and rapid subsurface stormflow components was developed and calibrated using field experiments conducted on a preferential path nested hillslope in northeast India. Virtual experiments were carried out to perform sensitivity analysis of the model using the automated parameter estimation (PEST) algorithm. Different physical parameters of the model were varied to study the resulting effects on overland flow and subsurface stormflow responses from the theoretical hillslopes. It was observed that topographical shapes had significant effects on overland flow hydrographs. The slope profiles, surface storage, relief, rainfall intensity and infiltration rates primarily controlled the overland flow response of the hillslopes. Prompt subsurface stormflow responses were mainly dominated by lateral preferential flow, as soil matrix flow rates were very slow. Rainfall intensity and soil macropore structures were the most influential parameters on subsurface stormflow. The number of connected soil macropores was a more sensitive parameter than the size of macropores. In hillslopes with highly active vertical and lateral preferential pathways, saturation excess overland flow was not evident. However, saturation excess overland flow was generated if the lateral macropores were disconnected. Under such conditions, rainfall intensity, duration and preferential flow rate governed the process of saturation excess overland flow generation from hillslopes.
Editor D. Koutsoyiannis; Associate editor C. Perrin  相似文献   

4.
Urban development significantly alters the landscape by introducing widespread impervious surfaces, which quickly convey surface run‐off to streams via stormwater sewer networks, resulting in “flashy” hydrological responses. Here, we present the inadequacies of using raster‐based digital elevation models and flow‐direction algorithms to delineate large and highly urbanized watersheds and propose an alternative approach that accounts for the influence of anthropogenically modified land cover. We use a semi‐automated approach that incorporates conventional drainage networks into overland flow paths and define the maximal run‐off contributing area. In this approach, stormwater pipes are clustered according to their slope attributes, which define flow direction. Land areas drained by each cluster and contributing (or exporting) flow to a topographically delineated catchment were determined. These land masses were subsequently added or removed from the catchment, modifying both the shape and the size. Our results in a highly urbanized Toronto, Canada, area watershed indicate a moderate net increase in the directly connected watershed area by 3% relative to a topographically forced method; however, differences across three smaller scale subcatchments are greater. Compared to topographic delineation, the directly connected watershed areas of both the upper and middle subcatchments decrease by 5% and 8%, respectively, whereas the lower subcatchment area increases by 15%. This is directly related to subsurface storm sewer pipes that cross topographic boundaries. When directly connected subcatchment area is plotted against total streamflow and flashiness indices using this method, the coefficients of variation are greater (0.93 to 0.97) compared to the use of digital elevation model‐derived subcatchment areas (0.78 to 0.85). The accurate identification of watershed and subcatchment boundaries should incorporate ancillary data such as stormwater sewer networks and retention basin drainage areas to reduce water budget errors in urban systems.  相似文献   

5.
Linking quickflow response to subsurface state can improve our understanding of runoff processes that drive emergent catchment behaviour. We investigated the formation of non-linear quickflows in three forested headwater catchments and also explored unsaturated and saturated storage dynamics, and likely runoff generation mechanisms that contributed to threshold formation. Our analyses focused on two reference watersheds at the Coweeta Hydrologic Laboratory (CHL) in western North Carolina, USA, and one reference watershed at the Susquehanna Shale Hills Critical Zone Observatory (SHW) in Central Pennsylvania, USA, with available hourly soil moisture, groundwater, streamflow, and precipitation time series over several years. Our study objectives were to characterise (a) non-linear runoff response as a function of storm characteristics and antecedent conditions, (b) the critical levels of shallow unsaturated and saturated storage that lead to hourly flow response, and (c) runoff mechanisms contributing to rapidly increasing quickflow using measurements of soil moisture and groundwater. We found that maximum hourly rainfall did not significantly contribute to quickflow production in our sites, in contrast to prior studies, due to highly conductive forest soils. Soil moisture and groundwater dynamics measured in hydrologically representative areas of the hillslope showed that variable subsurface states could contribute to non-linear runoff behaviour. Quickflow generation in watersheds at CHL were dominated by both saturated and unsaturated pathways, but the relative contributions of each pathway varied between catchments. In contrast, quickflow was almost entirely related to groundwater fluctuations at SHW. We showed that co-located measurements of soil moisture and groundwater supplement threshold analyses providing stronger prediction and understanding of quickflow generation and indicate dominant runoff processes.  相似文献   

6.
Current conceptual runoff models hypothesize that stormflow generation on the Canadian Shield is a combination of subsurface stormflow and saturation overland flow. This concept was tested during spring runoff in a small (3.3 ha) headwater basin using: (1) isotopic and chemical hydrograph separation and (2) field mapping and direct tracing of saturated areas. Isotopic and chemical hydrograph separation indicated three runoff components: (1) pre-melt subsurface flow; (2) subsurface flow of new (event) water; and (3) direct precipitation on to saturated areas (DPS). During early thaw-freeze cycles, their relative contributions to total flow remained constant (65 per cent, 30 per cent, and 5 per cent respectively). It is hypothesized that lateral flow along the bedrock/mineral soil interface, possibly through macropores, supplied large volumes of subsurface flow (of both old and new water) rapidly to the stream channel. Much higher contributions of DPS were observed during an intensive rain-on-snow event (15 per cent of total flow). Mapping and direct tracing of saturated areas using lithium bromide, suggested that saturated area size was positively correlated to stream discharge but its response lagged behind that of discharge. These observations suggest that the runoff mechanisms, and hence the sources of stream flow, will vary depending on storm characteristics.  相似文献   

7.
The processes of stormflow generation were studied in a hill pasture catchment near Hamilton, New Zealand. Although rainfall was relatively evenly distributed throughout the year, stormflow was highly seasonal and over 65 per cent occurred during the winter. Three main processes contributing to stormflow were identified which could be related to soil type and physiographic position. On gleyed soils derived from rhyolitic colluvium, saturation overland flow was the dominant process. Hydrographs from ‘Whipkey’ throughflow troughs also indicated that there was a subsurface response (saturated wedge) from this soil type. On steeper convex slopes, more permeable soils were derived from weathered greywacke. The presence of ephemeral springs on the hillslopes and direct observation during storm events indicated that storm runoff was generated as return flow from this soil. It was noted that nitrate concentrations from subsurface sources were 5–10 times higher than surface runoff. This difference in concentration was utilized in a chemical mixing equation which partitioned stormflow sources. This was compared with the stormflow predicted from rain falling on to saturated areas. There was good agreement between the two models for winter-spring events with respect to the volumes of surface runoff predicted, however the saturated areas model underestimated total stormflow. The results of the study are briefly discussed in terms of the potential for water quality management.  相似文献   

8.
Rainfall retention and runoff detention are likely the most important ecosystem services provided by extensive green roofs (EGRs) that contribute to urban stormwater mitigation and management. However, the hydrological performance and runoff generation mechanisms of mature, well-established EGRs in tropical regions remain poorly understood. This study evaluated the rainfall retention, discharge detention times and processes of runoff generation in two neighbouring 20-year-old EGRs with different slopes (2° and 14° for EGRns and EGRws, respectively) and management practices in Mexico City; results were compared with those obtained in a conventional roof (CR, 2° slope). Precipitation, substrate moisture and storm runoff were continuously measured during the 2017 and 2018 rainy seasons (May–November). Results showed spatial differences in substrate properties and moisture within and between green roofs. In general, higher bulk densities and a wide range of variation in water content characterized the bare substrate areas compared to those below vegetation. Greatest increases in substrate moisture and storm runoff were observed in the steeper green roof. Subsurface flow was the dominant process controlling the amount and timing of stormflow in the EGRs. The occurrence of saturation excess overland flow was small and detected when large rain events were preceded by high wetness conditions. The main factors influencing the hydrological responses of the green roofs were their substrate hydrophysical properties, related mostly to vegetation cover, management and age, and to much lesser extent to slope and substrate depth. On average, rainfall retention was ~60% in the EGRs with significantly longer delays and prolonged runoff times (100 and 340 min, respectively) compared to CR (3%, 20 min, and 258 min, respectively). Overall, these findings highlight the potential of EGRs in reducing stormflow and peak discharges for most rainfall in Mexico City, and thus mitigating the risk of saturation and overflow of urban drainages.  相似文献   

9.
The Amazon basin covers an area of roughly 7 × 106 km2 and encompasses diverse soil – landscape types with potentially differing hydrological behaviour. This study was conducted in the Ultisol landscape of the western Amazon basin in Peru. Processes of stormflow generation were investigated on an event basis in a first‐order rainforest catchment to establish a causal link between soil physical and precipitation characteristics, hillslope flowpaths and stormflow hydrograph attributes. A sharp decrease in soil hydraulic conductivity with depth and high rainfall intensity and frequency favour rapid near‐surface flowpaths, mainly in the form of saturation‐excess overland flow and return flow. The latter results in an almost random occurrence of overland flow, with no obvious topographic control. Hillslope flowpaths do not vary much with respect to the hydrograph attributes time of rise, response time, lag time and centroid lag time. They have the same response time as streamflow, but a somewhat lower time of rise and significantly shorter lag times. The recession constant for hillslope hydrographs is about 10 min, in contrast to the streamflow recession constants of 28, 75 and 149 min. Stormflow generation in this Ultisol rainforest catchment differs strongly from that reported for Oxisol rainforest catchments. These two soilscapes may define a spectrum of possible catchment hydrological behaviour in the Amazon basin. Copyright © 2000 John Wiley & Sons, Ltd.  相似文献   

10.
Low‐elevation areas within a sandy barrier island are subject to flooding via saturation overland flow following moderate storm surges and rainfall events. Using a high resolution topographic survey and simple hydrology models, we estimate the discharge and velocities from storm surge return flow and saturation overland flow. Results show that return flow velocities are of the same magnitude as the critical velocity necessary to mobilize sand when a hydraulic connection between the watershed and back‐barrier bay is present. Storms of moderate strength and rainfall intensity may be sufficient to keep the return channels open within the back‐barrier, thus providing natural conduits for water exchange from overwash events during extreme storm surges triggered by hurricanes. Copyright © 2011 John Wiley & Sons, Ltd.  相似文献   

11.
Stormflow generation in headwater catchments dominated by subsurface flow has been studied extensively, yet catchments dominated by surface flow have received less attention. We addressed this by testing whether stormflow chemistry is controlled by either (a) the event‐water signature of overland flow, or (b) the pre‐event water signature of return flow. We used a high‐resolution hydrochemical data set of stormflow and end‐members of multiple storms in an end‐member mixing analysis to determine the number of end‐members needed to explain stormflow, characterize and identify potential end‐members, calculate their contributions to stormflow, and develop a conceptual model of stormflow. The arrangement and relative positioning of end‐members in stormflow mixing space suggest that saturation excess overland flow (26–48%) and return flow from two different subsurface storage pools (17–53%) are both similarly important for stormflow. These results suggest that pipes and fractures are important flow paths to rapidly release stored water and highlight the value of within‐event resolution hydrochemical data to assess the full range and dynamics of flow paths.  相似文献   

12.
Heavy winter rainfall produces double‐peak hydrographs at the Slapton Wood catchment, Devon, UK. The first peak is saturation‐excess overland flow in the hillslope hollows and the second (i.e. the delayed peak) is subsurface stormflow. The physically‐based spatially‐distributed model SHETRAN is used to try to improve the understanding of the processes that cause the double peaks. A three‐stage (multi‐scale) approach to calibration is used: (1) water balance validation for vertical one‐dimensional flow at arable, grassland and woodland plots; (2) two‐dimensional flow for cross‐sections cutting across the stream valley; and (3) three‐dimensional flow in the full catchment. The main data are for rainfall, stream discharge, evaporation, soil water potential and phreatic surface level. At each scale there was successful comparison with measured responses, using as far as possible parameter values from measurements. There was some calibration but all calibrated values at one scale were used at a larger scale. A large proportion of the subsurface runoff enters the stream from three dry valleys (hillslope hollows), and previous studies have suggested convergence of the water in the three large hollows as being the major mechanism for the production of the delayed peaks. The SHETRAN modelling suggests that the hillslopes that drain directly into the stream are also involved in producing the delayed discharges. The model shows how in the summer most of the catchment is hydraulically disconnected from the stream. In the autumn the catchment eventually ‘wets up’ and shallow subsurface flows are produced, with water deflected laterally along the soil‐bedrock interface producing the delayed peak in the stream hydrograph. Copyright © 2007 John Wiley & Sons, Ltd.  相似文献   

13.
In the semi‐arid Mediterranean environment, the rainfall–runoff relationships are complex because of the markedly irregular patterns in rainfall, the seasonal mismatch between evaporation and rainfall, and the spatial heterogeneity in landscape properties. Watersheds often display considerable non‐linear threshold behavior, which still make runoff generation an open research question. Our objectives in this context were: to identify the primary processes of runoff generation in a small natural catchment; to test whether a physically based model, which takes into consideration only the primary processes, is able to predict spatially distributed water‐table and stream discharge dynamics; and to use the hydrological model to increase our understanding of runoff generation mechanisms. The observed seasonal dynamics of soil moisture, water‐table depth, and stream discharge indicated that Hortonian overland‐flow was negligible and the main mechanism of runoff generation was saturated subsurface‐flow. This gives rise to base‐flow, controls the formation of the saturated areas, and contributes to storm‐flow together with saturation overland‐flow. The distributed model, with a 1D scheme for the kinematic surface‐flow, a 2D sub‐horizontal scheme for the saturated subsurface‐flow, and ignoring the unsaturated flow, performed efficiently in years when runoff volume was high and medium, although there was a smoothing effect on the observed water‐table. In dry years, small errors greatly reduced the efficiency of the model. The hydrological model has allowed to relate the runoff generation mechanisms with the land‐use. The forested hillslopes, where the calibrated soil conductivity was high, were never saturated, except at the foot of the slopes, where exfiltration of saturated subsurface‐flow contributed to storm‐flow. Saturation overland‐flow was only found near the streams, except when there were storm‐flow peaks, when it also occurred on hillslopes used for pasture, where soil conductivity was low. The bedrock–soil percolation, simulated by a threshold mechanism, further increased the non‐linearity of the rainfall–runoff processes. Copyright © 2013 John Wiley & Sons, Ltd.  相似文献   

14.
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15.
The hydrological behaviour of the cultivated Féfé catchment (17·8 ha) on the tropical volcanic island of Guadeloupe was studied to identify flow paths, to quantify water fluxes, and finally, to build a lumped model to simulate discharge and piezometer levels. The approach combined two steps, an experimental step and a modelling step, which covered two time scales, the annual and the storm event scale. The hydrological measurements were conducted over 2 years. The Féfé catchment is characterized by heavy rainfall (4229 mm year?1) on permeable Andosols; the results showed that underground flow paths involved two overlapping aquifers, and that the annual water balance in 2003 was shared among outflows of the deep aquifer (42%), evapotranspiration (31%), and streamflow (27%). On the event scale, the surface runoff coefficient ranges between 6·2% and 24·4% depending on antecedent dry or wet moisture conditions. Hortonian overland flow predominated over subsurface and saturation overland flow processes. Recharge of the shallow aquifer is mainly governed by a constant infiltration capacity of the Andosols with depth in the vadose zone. Outflows of this shallow aquifer were the baseflow of the main stream and the recharge of the deep aquifer. Volcanic deposits at Féfé promoted the underground flow path, and cultivated areas seemed to explain the high stormflow values relative to other tropical small catchments under rain forest. A conceptual lumped model integrating runoff, infiltration, evapotranspiration, and fluctuations of the two overlapping aquifers was developed. The model has six parameters and was calibrated and validated on the hydrograph at the outlet and on the two piezometers of the shallow and the deep aquifers. The results show fair to good agreement between measured and simulated variables, and consequently, the model was consistent with the main hydrological processes observed from experimental results in wet conditions. Copyright © 2008 John Wiley & Sons, Ltd.  相似文献   

16.
Hydrological budgets and flow pathways have been quantified for a small upland catchment (1.76 km2) in the northeast of Scotland. Water balance calculations for four subcatchments identified spatial variability within the catchment, with an estimated runoff enhancement of up to 25% for the upper western area, compared with the rest of the catchment. Data from spatial hydrochemical sampling, over a range of flow conditions, were used to identify the principal hillslope runoff mechanisms within the catchment. A hydrochemical mixing analysis revealed that runoff emerging from springs in various locations of the hillslope accounted for a significant proportion of flow in the streams, even during storm events. A hydrological model of the catchment was calibrated using the calculated stream flows for four locations, together with results from the mixing analysis for different time points. The calibrated model was used to predict the temporal variability in contributions to stream flow from the hillslope springs and soil water flows. The overall split ranged from 57%:43% spring water:soil water in the upper eastern subcatchment, to 76%:24% in the upper western subcatchment. Copyright © 2006 John Wiley & Sons, Ltd.  相似文献   

17.
The devastating impacts of the widespread flooding and landsliding in Puerto Rico following the September 2017 landfall of Hurricane Maria highlight the increasingly extreme atmospheric disturbances and enhanced hazard potential in mountainous humid-tropical climate zones. Long-standing conceptual models for hydrologically driven hazards in Puerto Rico posit that hillslope soils remain wet throughout the year, and therefore, that antecedent soil wetness imposes a negligible effect on hazard potential. Our post-Maria in situ hillslope hydrologic observations, however, indicate that while some slopes remain wet throughout the year, others exhibit appreciable seasonal and intra-storm subsurface drainage. Therefore, we evaluated the performance of hydro-meteorological (soil wetness and rainfall) versus intensity-duration (rainfall only) hillslope hydrologic response thresholds that identify the onset of positive pore-water pressure, a predisposing factor for widespread slope instability in this region. Our analyses also consider the role of soil-water storage and infiltration rates on runoff generation, which are relevant factors for flooding hazards. We found that the hydro-meteorological thresholds outperformed intensity-duration thresholds for a seasonally wet, coarse-grained soil, although they did not outperform intensity-duration thresholds for a perennially wet, fine-grained soil. These end-member soils types may also produce radically different stormflow responses, with subsurface flow being more common for the coarse-grained soils underlain by intrusive rocks versus infiltration excess and/or saturation excess for the fine-grained soils underlain by volcaniclastic rocks. We conclude that variability in soil-hydraulic properties, as opposed to climate zone, is the dominant factor that controls runoff generation mechanisms and modulates the relative importance of antecedent soil wetness for our hillslope hydrologic response thresholds.  相似文献   

18.
The impact of road‐generated runoff on the hydrological response of a zero‐order basin was monitored for a sequence of 24 storm events. The study was conducted in a zero‐order basin (C1; 0·5ha) with an unpaved mountain road; an adjacent unroaded zero‐order basin (C2; 0·2 ha) with similar topography and lithology was used to evaluate the hydrological behaviour of the affected zero‐order basin prior to construction of the road. The impact of the road at the zero‐order basin scale was highly dependent on the antecedent soil‐moisture conditions, total storm precipitation, and to some extent rainfall intensity. At the beginning of the monitoring period, during dry antecedent conditions, road runoff contributed 50% of the total runoff and 70% of the peak flow from the affected catchment (C1). The response from the unroaded catchment was almost insignificant during dry antecedent conditions. As soil moisture increased, the road exerted less influence on the total runoff from the roaded catchment. For very wet conditions, the influence of road‐generated runoff on total outflow from the roaded catchment diminished to only 5·4%. Both catchments, roaded and unroaded, produced equivalent amount of outflow during very wet antecedent conditions on a unit area basis. The lag time between the rainfall and runoff peaks observed in the unroaded catchment during the monitoring period ranged from 0 to 4 h depending on the amount of precipitation and antecedent conditions, owing mainly to much slower subsurface flow pathways in the unroaded zero‐order basin. In contrast, the lag time in the roaded zero‐order basin was virtually nil during all storms. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

19.
The suitability of the physically based model SHETRAN for simulating sediment generation and delivery with a high degree of spatial (20 m) and temporal (sub‐hourly) resolution was assessed through application of the model to a 167‐km2 catchment leading to an estuary in New Zealand. By subdividing the catchment and conducting calculations on a computer cluster for a 6‐month hydrology initialisation period, it was possible to simulate a large rainfall event and its antecedent conditions in 24 h of computation time. The model was calibrated satisfactorily to catchment outlet flow and sediment flux for a large rainfall event in two subcatchments (~2 km2). Validation for a separate subcatchment was successful for flow (Nash–Sutcliff efficiency of 0.84) with a factor 2.1 over‐prediction for sediment load. Validation for sediment at full catchment scale using parameters from the subcatchment scale was good for flow but poor for sediment, with gross under‐estimation of the dominant stream sources of sediment. After recalibration at catchment scale, validation for a separate event gave good results for flow (Nash–Sutcliff efficiency of 0.93) and sediment load within a factor of two of measurements. An exploratory spatially explicit landslide model was added to SHETRAN, but it was not possible to test this fully because no landslides were observed in the study period. Application to climate change highlighted the non‐linear response to extreme rainfall. However, full exploration of land use and climate change and the evaluation of uncertainty were severely constrained by computational limitations. Subdivision of the catchment with separate stream routing is suggested as a way forward to overcome these limitations. Copyright © 2011 John Wiley & Sons, Ltd.  相似文献   

20.
The aim of this study is to identify, in a small catchment area located within a tropical forest, the pedological compartments in which the export of nutrients and chemical erosion of solutes occur during a stormflow event. The catchment area displays two types of lateral flow: (i) overland flow at the surface of the soil in the litter and root mat and (ii) groundwater flow in a macroporous subsurface horizon. We interpret the variations of stream‐water chemistry during a storm‐flow event using the separation of storm‐flow hydrograph data between overland and groundwater flow, and (Cl?) as a chemical parameter characterizing the residence time of water in the soil. It appears that K+ especially was released into the throughfall, whereas Ca++, Mg++ and Na+ were clearly released from the litter. K+ disappeared rapidly from soil solution, whereas Ca++ and Mg++ were more progressively absorbed by the vegetation. The Ca++ and Mg++ contents in groundwater increased with increasing residence time owing to the transpiration of trees. The export of H4SiO4 in the overland flow was moderate, i.e. 24% of total H4SiO4 export in the stream flow, as overland flow represented 39% of total runoff. The subsurface horizon—where active groundwater flow occurs—was successively affected by chemical erosion during the storm‐flow peak, and then by neoformation of kaolinite favoured by increasing water residence time. Copyright © 2003 John Wiley & Sons, Ltd.  相似文献   

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