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1.
The results of studying hydrocarbons during the flood in May 2005 are discussed. The concentration of aliphatic and polycyclic aromatic hydrocarbons are shown to match their concentrations in water areas with steady input of pollutants. Weathered oil and pyrogenic compounds dominated in their composition. The geochemical barrier the Northern Dvina River-Dvina Gulf is shown to become a filter during floods and prevents pollutants from penetrating into the White Sea.  相似文献   

2.
The White Sea is a natural analogue of arctic seas. The pollution of the sea by petroleum hydrocarbons is not high now. However, the load on sea ecosystem can increase in the nearest future because of the anticipated industrial development in its watershed, including an increase in oil, coal, and diamond production. The specific features of the nature of arctic marine systems (hydrological, ice, hydrobiological, hydrochemical, and radiation regimes), and the poor knowledge of the conditions of dispersion, transformation, and utilization of petroleum hydrocarbons in such seas make their ecological studies especially important. Petroleum hydrocarbon concentrations in the waters of tributaries and water areas of the White Sea (for 1980–2006 and 1989–2006, respectively) were evaluated using literary and authors’ data. Analysis of the collected materials shows that the majority of petroleum hydrocarbons enter the sea’s water areas with river runoff. Petroleum hydrocarbon concentrations were evaluated in major tributaries of the sea, including the rivers of Northern Dvina, Onega, Mezen, Niva, Kem, and Keret, delivering petroleum hydrocarbons into the bays of Dvina, Onega, Mezen, and Kandalaksha, water area near the Solovetskie Islands, and Chupa Bay, respectively (Bay — Gulf). Model calculations should yield within-year variations in petroleum hydrocarbon concentrations in different part of the sea (under a correctly specified load) and the conditions of their biotransformation and horizontal transport through the boundaries between areas within the sea.  相似文献   

3.
Water Resources - Water quality dynamics along the Northern Dvina River is analyzed under the conditions of anthropogenic impact. Overall, river water is classified as very polluted. The cases of...  相似文献   

4.
The available observational data on variations of oil hydrocarbon concentrations in White Sea tributaries and in individual parts of the sea are analyzed, and the contributions of different external sources to marine environment pollution are evaluated. The results of calculations are used to determine the possible total input of hydrocarbons from additional potential sources—internal natural (production by microorganisms) and external anthropogenic (navigation and sea shipping), which are most active in the summer and autumn. The hydroecological CNPSi-model is used to reproduce the processes of pollution of nine areas in the White Sea by oil hydrocarbons and their subsequent biodegradation in the marine environment. The annual dynamics of hydrocarbon concentrations was calculated using the long-term annual observations of monthly variations of the temperature, light intensity, and transparency of water, data on the morphometry of sea areas (the squares, mean depths, and water volumes) and water exchange between the chosen areas, calculated by a hydrodynamic model. For large bays (Dvina, Kandalaksha), the calculated concentrations of oil hydrocarbons are shown to be in agreement with the available estimates (the mean and maximal concentrations). The annual variations of oil hydrocarbon concentrations; the biomasses, oxidation activity and bioproduction characteristics of oil hydrocarbon-oxidizing bacteria are characterized. The calculated internal fluxes of oil hydrocarbons (the inputs from different sources, horizontal transport, and biotransformation) were used to calculate their annual balances for individual areas and the sea as a whole, showing the balanced character of their fluxes with the total balance discrepancies for individual areas varying within 0.3–4.1%.  相似文献   

5.
Nutrient Transport into the White Sea with River Runoff   总被引：1，自引：0，他引：1  
Leonov  A. V.  Chicherina  O. V. 《Water Resources》2004,31(2):152-173
Averaged data from long-term observations of concentrations of mineral-nutrient fractions along with fragmentary data and indirect estimates of organic-component concentrations in the tributaries of the sea (the Niva, the Onega, the Northern Dvina, the Mezen, and the Kem rivers) are analyzed. Monthly variations in the concentrations of the major nutrients in the river water flowing into the sea are characterized, and relationships between them in different seasons are determined. Annual nutrient transport into the White Sea by river water is assessed based on characteristics of river runoff and nutrient concentrations using a mathematical model. Wide variations are established in the ratios of organic and mineral fractions of nutrients delivered into the sea. The shares of mineral components in the total runoff of Ntot and Ptot into the sea are found to be equal to 18.1 and 18.8%, respectively.  相似文献   

6.
Water Resources - Aliphatic and polycyclic aromatic hydrocarbons have been studied in suspended matter and bottom sediments at the geochemical barrier the Northern Dvina–Dvina Bay during...  相似文献   

7.
The presented results have been obtained in a study of the concentrations and composition of aliphatic and polycyclic hydrocarbons in bottom sediments of Volga delta branches and in its shallow zone (2009–2010), as well as the Caspian Sea proper (2010–2013). Oil hydrocarbon pollution has been found to manifest itself mostly in Volga delta branches, which, despite the low concentrations (up to 54.5 μg/g), showed higher hydrocarbons share in Corg (up to 33.8%), while the composition of alkanes suggested their oil genesis. The geochemical barrier the Volga–the Caspian Sea prevents anthropogenic hydrocarbons from entering the open parts of the Caspian. Bottom sediments in the shallow zone of the Northern Caspian, represented by coarse-grained material, are now polluted by oil hydrocarbons to a lesser extent compared with other areas. The highest concentrations of aliphatic hydrocarbons (up to 178 μg/g) were recorded in the deepsea bottom sediments of Derbent Depression and in depressions of the Middle and Southern Caspian. These areas show a higher concentration of Corg (up to 9.884%) and a low concentration of hydrocarbons in Corg (up to 0.16%), while odd high-molecular homologues (n-C25–C31) dominate in the composition of alkanes.  相似文献   

8.
The distribution of reduced sulfuric compounds in the surface layer of bottom deposits in the Northern Dvina mouth was examined. The natural biogeochemical processes and anthropogenic pollution are found to cause the formation and accumulation of reduced sulfuric compounds (mostly pyrite and organic forms) in bottom deposits. The concentration of individual forms of sulfur and its total concentration are found to vary widely from year to year. The most intense accumulation of the total reduced sulfur is recorded near the wastewater discharge sites of pulp and paper mills.  相似文献   

9.
Literary data have been used to assess the inflow of petroleum hydrocarbons (with river runoff, precipitation, wastewaters, sea transport, and at ice thawing) into different regions of the White Sea. The hydroecological CNPSi-model was used as an instrument to reproduce the annual dynamics of hydrocarbon concentrations at their parallel inflow and subsequent transformation in the waters of the nine White Sea regions (the bays of Kandalaksha, Onega, Dvina, and Mezen; the Solovetskie Islands; the deep-water part: Bassein, Gorlo, Voronka, and Chupa Bay). The calculations were based on normal annual values of monthly variations of water temperature, light intensity, and transparency, the morphometric parameters of the regions (water areas, mean depths, and water volumes) and water exchange between the regions and with the Barents Sea (calculated by a hydrodynamic model). The calculated concentrations of hydrocarbons, the biomasses and activity characteristics of hydrocarbon-oxidizing bacteria have been analyzed (their values were estimated for the 2-m surface water layer). The results of calculations were used to evaluate hydrocarbon balances for regions and the sea as a whole. The calculations demonstrate the balanced character of hydrocarbon fluxes, the balance discrepancy for the regions being <0.1–16.1%.  相似文献   

10.
Water Resources - Data on river water quality and pollution level have been analyzed to show that the Northern Dvina basin water is characterized by class 3 quality (categories 3А and 3B,...  相似文献   

11.
The seasonal variability of the distribution of dissolved forms of mineral phosphorus and silicon and water alkalinity is studied in the Northern Dvina River mouth. The non-conservative behavior of mineral phosphorus and silicon (presumably caused by the biological consumption of these elements) and the conservative distribution of alkalinity are established. The conservative distribution of alkalinity makes it possible to use the relationship between the values of this parameter and the concentrations of chlorides for the analysis of the genetic structure of water in the desalinized part of the Baltic Sea.__________Translated from Vodnye Resursy, Vol. 32, No. 4, 2005, pp. 459–463.Original Russian Text Copyright © 2005 by Savenko, Shevchenko.  相似文献   

12.
A method is developed for scenario prediction of changes in water balance components in northern river basins in the context of possible climate changes. The method uses the land surface model SWAP, describing the heat and mass exchange between the land surface and the atmosphere. Four IPCC climate scenarios, corresponding to specified scenarios of economic, technological, political, and demographic development of the human civilization, were used to forecast different variants of the dynamics of meteorological characteristics in the Northern Dvina River basin in the XXI century, which served as a basis for evaluating possible changes in precipitation, evaporation, and runoff from the Northern Dvina basin until the year of 2063.  相似文献   

13.
Parameter estimates of the process of passage into water of 234U and 238U isotopes with inequilibrium ratios during 238U decay in rock are given. The Northern Dvina Depression is used as an example to show that data on the fractionation of natural U isotopes can be used to assess the duration of the contact of fresh infiltration water of atmospheric origin with rocks, as well as the presence in rocks of areas with higher U concentrations, with which groundwater with higher radioactivity is associated.  相似文献   

14.
The conditions and mechanisms of the formation of parallel-branch braidings—the least studied and most complex variety of braided channels are analyzed. They are proved to be related with the appearance of a vertical interface between water masses in rivers with weakly stable, wide, spread channel; large runoff of channel-forming (tractable) sediments. Channels of this type in the Northern Dvina and the Upper Ob are described in detail.  相似文献   

15.
Volkov  I. I.  Kokryatskaya  N. M. 《Water Resources》2004,31(4):423-430
The occurrence and distribution of reduced inorganic sulfur compounds in the waters of the White Sea and the Northern Dvina mouth are studied. Universal occurrence of micro-quantities of the above compounds in the oxic marine and fluvial waters is established. The White Sea water is found to be depleted of reduced sulfur, judging by the sum of reduced S forms (<0.5 mol), as compared with that in the water of the Black and Baltic seas.  相似文献   

16.
The results of studies of spatial and seasonal variations in hydrocarbon concentrations in hypertrophic Lake Nero are used to discuss the problem of division of hydrocarbons into anthropogenic and natural components. It is shown that the use of bitumoids as a component of oil pollution instead of total organic matter can introduce errors in the results. Seasonal variations in the activity of hydrobionts in an undisturbed area are shown to have a notable effect on the assessment of the proportion of anthropogenic hydrocarbons in their total concentration, that is, on the assessment of the extent of pollution of water bodies. The natural component is found to dominate over the anthropogenic component only in the periods of algae blooming. In spring and autumn, the total concentration of hydrocarbons was found to exceed the MAC and to be due mostly to natural hydrobiological factors.  相似文献   

17.
Variations in the characteristics of ice regime of rivers in the Northern Dvina basin over the last 125 years are analyzed. For the Northern Dvina lower course, potential changes in the dates of the appearance of floating ice and the breakup due to expected changes in the air temperature and the rate of streamflow in rivers are assessed. Special attention is paid to the factors that affect the formation of ice jams and their spatial and temporal variability. The prognostic relationship for the maximum ice-jam stage in the Sukhona River near the town of Velikii Ustyug is presented as an example.  相似文献   

18.
The study aimed to determine the spatial distribution of n-alkanes and polycyclic aromatic hydrocarbons (PAHs) in surface sediments of the Segara Anakan nature reserve and their potential origins using gas chromatography–mass spectrometry. Total alkane concentrations ranged from 3755 to 129,027 μg kg−1, and the concentrations of 16 PAHs ranged from 375 to 29,517 μg kg−1. The ratios of specific n-alkanes (e.g., CPI24–34, WaxCn, and Paq), including a new proposed index, terrestrial–marine discriminant (TMD), as well as the ratios of selected PAHs (e.g., Ant/∑178, Fl/∑202, BaAnt/∑228, and IPyr/∑276), showed that the sources of hydrocarbons in the sediments were generally biogenic, including both terrigenous and marine, with an anthropogenic pyrolytic contribution (petrogenic and biogenic combustion). For the environmental risk assessment, a sediment quality guideline (SQGs) comparison indicated that the station risk levels ranged from low to medium-low, except for R6, which has a greater impact on the ecological risk for marine organisms.  相似文献   

19.
In this study, mineral magnetic properties and petroleum hydrocarbons were statistically analysed in four sediment cores (C1, A1, T1 and K1) from the north east coast of Tamilnadu, India to examine the feasibility of PHC concentrations assessment using magnetic susceptibility. The C1 and A1 cores reveal a clear horizon of increase in PHC above 35 and 50 cm respectively suggesting the excess anthropogenic loading occurred in the recent past. Magnetic properties which were enhanced in the upper part of the sediment cores were the result of ferrimagnetic minerals from anthropogenic sources. Factor analysis confirmed that the input of magnetic minerals and petroleum hydrocarbons in Chennai coastal sediments are derived from the same sources. The present study shows that instead of expensive and destructive PHC chemical methods, magnetic susceptibility is found to be a suitable, cheap and rapid method for detailed study of petroleum hydrocarbon contamination in marine sediments.  相似文献   

20.
Sedimentary aliphatic (AH) and polycyclic aromatic hydrocarbons (PAHs) were studied in the Changjiang Estuary and the adjacent East China Sea. Total AH ranged from 2.20 to 11.82 μg g−1 and consisted of n-alkanes and a dominant petroleum-related unresolved complex mixture (UCM). Within the n-alkanes, terrestrial plant wax compounds prevailed at nearly all stations. Of the PAHs, biogenic perylene dominated at stations receiving riverine inputs. Anthropogenic PAHs originating from combustion/pyrolysis processes varied from 17 to 157 ng g−1, while fossil PAH concentrations ranged from 42 to 187 ng g−1. Both biogenic and anthropogenic hydrocarbons are primarily derived from riverine discharges and accumulate at shallow-water stations. Distinct phase associations lead, nevertheless, to different sedimentation patterns. Fossil PAHs are enhanced at offshore stations where they are introduced directly by shipping activities. Biomarker fingerprints ascribe their source to Chinese crude oils. The overall levels of anthropogenic hydrocarbons are low compared to relevant areas worldwide and reveal a low/moderate level of hydrocarbon pollution.  相似文献   

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