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1.
Chemical compositions of precipitation samples collected from a remote and high elevation site (Nam Co Station, 30°46.44??N, 90°59.31??E, 4730?m?a.s.l.) in central Tibetan Plateau (TP, hereafter) from August 2005 to August 2009 are investigated. During the study period, Ca2+ and HCO 3 - have the highest concentrations among ions and are the dominant cation and anion in precipitation, taking 27.46?% and 30.84?% to the total ions respectively. Empirical Orthogonal Functions (EOFs) analyses reveal that crustal aerosol inputs significantly contributed to the loading of Ca2+, Mg2+, SO 4 2- and HCO 3 - in precipitation, while lake salt plays a major source of K+ and Cl-. Seasonal variations of ionic wet deposition fluxes show high values during monsoon seasons due to large precipitation amount. Among the cations, annual Ca2+ flux is the largest (86.26?eq hm?2), Na+ and NH 4 + fluxes are following. Among anions, HCO 3 - has the highest flux (98.66?eq hm?2) while that of NO 3 - is the lowest. Annual wet deposition of nitrogen has varied considerably with the average value of 0.70?kg?ha?1 a?1 at Nam Co Station. About 80?% of total nitrogen flux occurs during the monsoon seasons when precipitation is concentrated, in which NH 4 + and NO 3 - contributed to 61?% and 39?% of the total nitrogen deposition. Thus, our ionic concentrations and wet deposition fluxes in precipitation can provide a useful dataset to assess atmospheric environment and its impacts on ecosystem in the inland TP.  相似文献   

2.
Our long-term study provides an unequivocal evidence for near-quantitative (80–100%) depletion of chloride from sea-salts in the marine atmospheric boundary layer (MABL) of tropical Bay of Bengal. During the late NE-monsoon (Jan-Mar), continental outflow from south and south-east Asia dominate the wide-spread dispersal of pollutants over the Bay of Bengal. Among anthropogenic constituents, SO 4 2? (range: 0.6–35 μg m?3) is the most dominant. The non-sea-salt SO 4 2? (nss-SO 4 2? ) constitutes a major fraction (55–65%) of the aerosol water-soluble ionic composition (WSIC), whereas contribution of NO 3 ? is relatively minor. The magnitude of Cl-deficit (with respect to its sea-salt proportion) exhibits linear increase with the excess-nss-SO 4 2? (excess over NH 4 + ). We propose that displacement of HCl from sea-salt aerosols by H2SO4 is a dominant reaction mechanism for the chloride-depletion. These results also suggest that sea-salts could serve as a potential sink for anthropogenic SO2 in the downwind polluted marine environment. Furthermore, loss of hydrogen chloride, representing a large source of reactive chlorine, has implications to the oxidant chemistry in the MABL (oxidation of hydrocarbons and dimethyl sulphide).  相似文献   

3.
For the first time, simultaneous study on physical and chemical characteristics of PM10, PM2.5, and rainwater chemistry was attempted over the Bay of Bengal in monsoon season of 2009. The aerosols and rainwater samples were collected onboard ship ‘SK-261, ORV Sagar Kanya’ during Oceanographic Observations in the Northern Bay of Bengal under the Continental Tropical Convergence Zone (CTCZ) program conducted during 16 July to 19 Aug 2009. Aerosol samples collected by PM10 and PM2.5 were analyzed for various water soluble (Na+, K+, Ca2+, Mg2+, NH 4 + , Cl?, SO 4 2? and NO 3 ? and acid soluble (Fe2+, Al3+, Zn2+, Mn3+ and Ni2+) ionic constituents. The pH of rainwater varied from 5.10 to 7.04. Chloride ions contributed most to the total ion concentration in aerosol and rainwater, followed by Na+. Significant contributions of SO 4 2? , NO 3 ? and NH 4 + found in PM2.5, PM10 and high concentrations of TSP and non sea-salt SO 4 2? over the mid-ocean is attributed to the long range transport of anthropogenic pollution from the Indian continent. The scavenging ratio was maximum for coarse particles such as Ca2+ and minimum for fine particles like NH 4 + .  相似文献   

4.
This study elucidates the characteristics of ambient PM2.5 (fine) and PM1 (submicron) samples collected between July 2009 and June 2010 in Raipur, India, in terms of water soluble ions, i.e. Na+, NH 4 + , K+, Mg2+, Ca2+, Cl?, NO 3 ? and SO 4 2? . The total number of PM2.5 and PM1 samples collected with eight stage cascade impactor was 120. Annual mean concentrations of PM2.5 and PM1 were 150.9?±?78.6 μg/m3 and 72.5?±?39.0 μg/m3, respectively. The higher particulate matter (PM) mass concentrations during the winter season are essentially due to the increase of biomass burning and temperature inversion. Out of above 8 ions, the most abundant ions were SO 4 2? , NO 3 ? and NH 4 + for both PM2.5 and PM1 aerosols; their average concentrations were 7.86?±?5.86 μg/m3, 3.12?±?2.63 μg/m3 and 1.94?±?1.28 μg/m3 for PM2.5, and 5.61?±?3.79 μg/m3, 1.81?±?1.21 μg/m3 and 1.26?±?0.88 μg/m3 for PM1, respectively. The major secondary species SO 4 2? , NO 3 ? and NH 4 + accounted for 5.81%, 1.88% and 1.40% of the total mass of PM2.5 and 11.10%, 2.68%, and 2.48% of the total mass of PM1, respectively. The source identification was conducted for the ionic species in PM2.5 and PM1 aerosols. The results are discussed by the way of correlations and principal component analysis. Spearman correlation indicated that Cl? and K+ in PM2.5 and PM1 can be originated from similar type of sources. Principal component analysis reveals that there are two major sources (anthropogenic and natural such as soil derived particles) for PM2.5 and PM1 fractions.  相似文献   

5.
The temporal variation in concentrations of major water soluble ionic species has been studied from several rain events occurred over Gadanki (13.5 °N, 79.2 °E), located in tropical semi arid region in southern India. The contribution from rain-out (in cloud) and wash-out (below cloud) processes to the total removal of ionic species by rain events is also estimated using the pattern of variations of ionic species within an individual event. A number of rain samples were collected from each rain event during June–November in 2006, 2007 and 2008. On average, nearly 20% of the total NH 4 + and non-sea SO 4 2? is removed by in-cloud scavenging, suggesting that their removal by “below cloud” washout is relatively dominant. In contrast Na+, Ca2+, Mg2+, NO 3 ? and sea-SO 4 2? are mainly removed by below-cloud scavenging or wash-out process. A significant variation in the acidity was observed within rain events with successive precipitation showing higher acidity at the final stage of the precipitation due to partial neutralization of non-sea SO 4 2? . Overall, greater influence of both terrestrial and anthropogenic sources is recorded in the rain events compared to that from marine sources.  相似文献   

6.
Beryllium-7 Deposition and Its Relation to Sulfate Deposition   总被引：2，自引：0，他引：2  
Deposition of 7Be, a cosmogenic radionuclide, was observed at the Meteorological Research Institute in Tsukuba, Japan from 1986 to 1993 and compared with those of several chemical species observed in Tsukuba over the same period. We found a correlation between the monthly depositions of 7 Be and SO 4 2 -, a major acidic species. The correlation was especially strong for late spring and fall, when both species had high depositional fluxes. This correlation was also observed in precipitation samples collected daily in 1992 at the same site. The cause of this correlation is discussed in connection with the fact that the stratospheric aerosol is composed largely of SO 4 2 -. 7 Be is produced in the upper atmosphere, and detection of 7Be, especially in spring and fall in Japan, can be regarded as detection of stratospheric aerosol. However, we conclude that the bulk of the SO 4 2 - observed did not have a stratospheric or an upper tropospheric origin. The correlation, therefore, may present a new question regarding acidic deposition: Why does the deposition of stratospheric aerosol in Japan coincide with that of nss-SO 4 2 - originally from anthropogenic sources on the Earth's surface?  相似文献   

7.
This paper reports aerosol chemical properties for the first time over a Korean Global Atmosphere Watch (GAW) supersite, Anmyeon (36°32′N; 126° 19′E), during 2003–2004 period. Total suspended Particulates (TSP) showed significant seasonal variation with consistent higher mass concentrations during spring season (average of up to 230?±?190 μg/m3). PM10 also followed similar trend with higher concentrations during spring (average of up to 170?±?130 μg/m3) and showed reduced concentrations during summer. PM2.5 showed a significant increase during summer (average of up to 60?±?25 μg/m3), which could be due to the influx of fine mode sea salt aerosols associated with the Changma front (summer monsoon). Chemical composition analysis showed enhanced presence of acidic fractions, majorly contributed by sulphates (SO 4 2- ) and nitrates (NO 3 - ) in TSP, PM10 and PM2.5 during different seasons. Enhanced presence of Calcium (Ca2+) was observed during sand storm days during spring. The high correlation obtained on matrix analysis between crustal ions and acidic ions suggests that the ionic compositions over the site are mainly contributed by terrestrial sources of similar origin. The neutralization factors has been estimated to find the extend of neutralization of acidicity by main basic components, and found to have higher value for Ammonium (up to 1.1) in different seasons, indicating significant neutralization of acidic components over the region by NH 4 + . Back trajectory analysis has been performed during different seasons to constrain the possible sources of aerosol origin and the results are discussed in detail.  相似文献   

8.
Near real-time measurements of PM2.5 ionic compositions were performed at the summit of the highest mountain in the central-eastern plains in the spring and summer of 2007 in order to characterize aerosol composition and its interaction with clouds. The average concentrations of total water soluble ions were 27.5 and 36.7 μg?m?3, accounting for 44% and 62% of the PM2.5 mass concentration in the spring and summer, respectively. A diurnal pattern of SO 4 2- , NH 4 + and NO 3 - was observed in both campaigns and attributed to the upslope/downslope transport of air mass and the development of the planetary boundary layer (PBL). The average SO2 oxidation ratio (SOR) in summer was 57% (±27%), more than twice that in spring 24% (±16%); the fine nitrate oxidation ratio (NOR) was comparable in the two seasons (9?±?6% and 11?±?10% in summer and spring, respectively). This result indicates strong summertime production of sulfate aerosol. A principal component analysis shows that short-range and long-range transport of pollution, cloud processing, and crustal source were the main factors affecting the variability of the measured ions (and other trace gases and aerosols) at Mt. Tai. Strong indications of biomass burning were observed in summer. Cloud scavenging rates showed larger variations for different ions and in different cloud events. The elevated concentrations of the water soluble ions at Mt. Tai indicate serious aerosol pollution over the North China plain of eastern China.  相似文献   

9.
A regional atmospheric climate model with multi-layer snow module (RACMO2) is forced at the lateral boundaries by global climate model (GCM) data to assess the future climate and surface mass balance (SMB) of the Antarctic ice sheet (AIS). Two different GCMs (ECHAM5 until 2100 and HadCM3 until 2200) and two different emission scenarios (A1B and E1) are used as forcing to capture a realistic range in future climate states. Simulated ice sheet averaged 2 m air temperature (T2m) increases (1.8–3.0 K in 2100 and 2.4–5.3 K in 2200), simultaneously and with the same magnitude as GCM simulated T2m. The SMB and its components increase in magnitude, as they are directly influenced by the temperature increase. Changes in atmospheric circulation around Antarctica play a minor role in future SMB changes. During the next two centuries, the projected increase in liquid water flux from rainfall and snowmelt, together 60–200 Gt year?1, will mostly refreeze in the snow pack, so runoff remains small (10–40 Gt year?1). Sublimation increases by 25–50 %, but remains an order of magnitude smaller than snowfall. The increase in snowfall mainly determines future changes in SMB on the AIS: 6–16 % in 2100 and 8–25 % in 2200. Without any ice dynamical response, this would result in an eustatic sea level drop of 20–43 mm in 2100 and 73–163 mm in 2200, compared to the twentieth century. Averaged over the AIS, a strong relation between $\Updelta$ SMB and $\Updelta\hbox{T}_{2{\rm m}}$ of 98 ± 5 Gt w.e. year?1 K?1 is found.  相似文献   

10.
Doppler sodar derived values of the temperature structure parameter C infT sup2 , the vertical velocity variance ¯′w 2, and the rate of dissipation of turbulent energy ?, were measured during unstable conditions above the Lannemezan heterogeneous site. The vertical profiles of these turbulent parameters, normalized by the classical convective scales are compared with those obtained using the same acoustic sounder above an homogeneous site during convective conditions. The typical decrease of C infT sup2 as Z -4/3 is partially verified on the heterogeneous site: for the lower levels, C infT sup2 exhibits an increase with Z whereas for the intermediate levels C infT sup2 . decreases as Z -4/3. For the upper levels, C infT sup2 increases with Z due to a signal-to-noise ratio lower than 1. The vertical profiles of ¯′w 2 above the two sites are rather similar. However, near the base of the convective inversion Z i , the values measured on the heterogeneous site are more scattered. The same scattering is also observed with the ? values; moreover, for the lower levels (Z<0.17Z i ) the increase of ? as Z decreases is more important at the homogeneous site than at the heterogeneous one. It is suggested that these particular features observed at lower levels above the heterogeneous site are mainly related to a complex local boundary layer induced by the near environment of the sodar (vegetation and relief).  相似文献   

11.
Heat flux density at the soil surface (G 0) was evaluated hourly on a vegetal cover 0.08 m high, with a leaf area index of 1.07 m2 m?2, during daylight hours, using Choudhury et al. (Agric For Meteorol 39:283–297, 1987) ( $ G_0^{\text{rn}} $ ), Santanello and Friedl (J Appl Meteorol 42:851–862, 2003) ( $ G_0^{\text{s}} $ ), and force-restore ( $ G_0^{\text{fr}} $ ) models and the plate calorimetry methodology ( $ G_0^{\text{pco}} $ ), where the gradient calorimetry methodology (G 0R ) served as a reference for determining G 0. It was found that the peak of G 0R was at 1 p.m., with values that ranged between 60 and 100 W m?2 and that the G 0/Rn relation varied during the day with values close to zero in the early hours of the morning and close to 0.25 in the last hours of daylight. The $ G_0^{\text{s}} $ model presented the best performance, followed by the $ G_0^{\text{rn}} $ and $ G_0^{\text{fr}} $ models. The plate calorimetry methodology showed a similar behavior to that of the gradient calorimetry referential methodology.  相似文献   

12.
Climate and atmospheric CO2 concentration are intimately coupled in the Earth system: CO2 influences climate through the greenhouse effect, but climate also affects CO2 through its impact on the amount of carbon stored on land and in the ocean. The change in atmospheric CO2 as a response to a change in temperature ( $\varDelta CO_{2}/\varDelta T$ ) is a useful measure to quantify the feedback between the carbon cycle and climate. Using an ensemble of experiments with an Earth system model of intermediate complexity we show a pronounced time-scale dependence of $\varDelta CO_{2}/\varDelta T$ . A maximum is found on centennial scales with $\varDelta CO_{2}/\varDelta T$ values for the model ensemble in the range 5–12 ppm °C?1, while lower values are found on shorter and longer time scales. These results are consistent with estimates derived from past observations. Up to centennial scales, the land carbon response to climate dominates the CO2 signal in the atmosphere, while on longer time scales the ocean becomes important and eventually dominates on multi-millennial scales. In addition to the time-scale dependence, modeled $\varDelta CO_{2}/\varDelta T$ show a distinct dependence on the initial state of the system. In particular, on centennial time-scales, high $\varDelta CO_{2}/\varDelta T$ values are correlated with high initial land carbon content. A similar relation holds also for the CMIP5 models, although for $\varDelta CO_{2}/\varDelta T$ computed from a very different experimental setup. The emergence of common patterns like this could prove to usefully constrain the climate–carbon cycle feedback.  相似文献   

13.
The scalar flux–gradient relationships of temperature ( $\phi _{T}$ ? T ) and specific humidity ( $\phi _{q}$ ? q ) under unstable conditions are investigated using eddy-covariance measurements of air–sea turbulent fluxes and vertical profiles of temperature and specific humidity collected from a marine meteorological platform. The gradients of temperature and specific humidity are obtained from measurements at five heights above the sea surface using the log-square fitting method and the simpler first-order approximation method. The two methods yield similar results. The proposed flux–gradient relationships $\phi _{T}$ ? T and $\phi _{q}$ ? q covers a wide range of instability: the stability parameter $\zeta $ ζ ranges from $-$ ? 0.1 to $-$ ? 50. The functional form of the proposed flux–gradient relationships is an interpolation between the Businger–Dyer relation and the free convection relation, which includes the “ $-$ ? 1/2” and “ $-$ ? 1/3” scaling laws at two different stability regimes. The widely used COARE 3.0 algorithm, which is an interpolation between the integrals of the Businger–Dyer and the free convection relations, is also evaluated and compared. The analysis and comparisons show that both schemes generate reasonable values of $\phi _{q}$ ? q in the whole unstable regime. The COARE 3.0 algorithm, however, overestimates $\phi _{T}$ ? T values under very unstable conditions. The errors in the flux–gradient relationships induced by the random errors in the turbulence measurements are assessed. When the random errors are taken into account, the observations agree with predictions of various schemes fairly well, implying that the dominant transport mechanism is adequately captured by the Monin–Obukhov similarity theory. The study also shows that $\phi _{q}$ ? q is significantly ${>}\phi _{T}$ > ? T under unstable conditions and that the ratio $\phi _{q}/\phi _{T}$ ? q / ? T increases with $-\zeta $ ? ζ . The ratio of $\phi _{q}$ ? q to $\phi _{T}$ ? T and the ratio of turbulent transport efficiencies of heat and water vapour ( $R_{wT}/R_{wq}$ R wT / R wq ) suggest that heat is transported more efficiently than water vapour under unstable conditions.  相似文献   

14.
The data on deposition density of Ag, Al, As, B, Ba, Be, Bi, Br, Ca, Cd, Co, Cr, Cs, Cu, Fe, I, K, Li, Mg, Mn, Mo, Na, Ni, P, Pb, Rb, S, Sb, Se, Si, Sn, Sr, Th, Tl, U, V, Zn, Cl?, F?, NO 3 ? , and SO 4 2? in atmospheric precipitation were derived at six stations in the Republic of Karelia. The structure and space-time distribution of five sets (factors) of chemical components of the first order and two factors of the second order are revealed with the help of hierarchical factor analysis. Factor analysis of the second order demonstrated that atmospheric precipitation chemistry at all stations considered differs greatly in the winter and summer, forming two independent sets of components. The first-order factors revealed chemical indicators characterizing specific features of the atmospheric precipitation chemistry in the Karelian regions studied.  相似文献   

15.
Alkyl nitrate yields from the NO x photooxidations of neopentane, 2-methylbutane and 3-methylpentane have been determined over the temperature and pressure ranges 281–323 K and 54–740 torr, respectively. The formation of the alkyl nitrates is attributed to the reaction pathway (1b) $${\text{RO}}_{\text{2}} + {\text{NO}}^{{\text{ }}\underrightarrow {\text{M}}} {\text{ RONO}}_{\text{2}}$$ and rate constant ratios k 1b/(k 1a+k 1b) are estimated, where (1a) is the reaction pathway (1a) $${\text{RO}}_{\text{2}} + {\text{NO}} \to {\text{RONO}}_{\text{2}} .$$ A method for estimating this rate constant ratio for primary, secondary and tertiary alkyl peroxy radicals is presented.  相似文献   

16.
In studies of lake–atmosphere interactions, the fluxes of momentum, water vapour and sensible heat are often parametrized as being proportional to the differences in wind, humidity and air temperature between the water surface and a reference height above the surface. Here, the proportionality via transfer coefficients in these relationships was investigated with the eddy-covariance method at three sites within an eddy-covariance mesonet across Lake Taihu, China. The results indicate that the transfer coefficients decreased with increasing wind speed for weak winds and approached constant values for strong winds. The presence of submerged macrophytes reduced the momentum transfer (drag) coefficient significantly. At the two sites free of submerged macrophytes, the 10-m drag coefficients under neutral stability were 1.8 $(\pm \,0.4) \times \,10^{-3}$ ( ± 0.4 ) × 10 ? 3 and $1.7\,(\pm \,0.3) \times \,10^{-3 }$ 1.7 ( ± 0.3 ) × 10 ? 3 at the wind speed of $9\,\text{ m } \text{ s }^{-1}$ 9 m s ? 1 , which are 38 and 34 % greater than the prediction by the Garratt model for the marine environment.  相似文献   

17.
In October 2012 Hurricane Sandy devastated New York City and its vicinity caused mainly by the storm surge, which is the water height above normal astronomical tide level. The meteorological conditions were as follows: minimum central pressure, 962 hPa, highest sustained wind speed 27.1 m s $^{-1}$ ? 1 and maximum gust 37.8 m s $^{-1}$ ? 1 . The peak storm surge was at 3.9 m and the peak storm tide at 4.4 m (which is referenced above mean lower low water). The wind-stress tide relation shows that $S=K\,V^{2}$ S = K V 2 , where $S$ S is the storm surge, $V$ V is the wind speed and $K$ K is the coefficient. It is found that with $S$ S in units of m, and $V$ V in  m s $^{-1}$ ? 1 , $K = 0.0051$ K = 0.0051 with $R^{2}= 0.91$ R 2 = 0.91 ( $R$ R is the correlation coefficient) indicating that 91 % of the total variation of the storm surge can be explained by variations in the wind stress, which is proportional to $V^{2}$ V 2 . Similar results were obtained during Hurricane Irene in 2011, which also affected the New York area. Therefore, this simple wind stress-tide relation should be useful in coastal engineering, urban planning, and emergency management.  相似文献   

18.
Precipitation samples collected during 2005–2009 from a rural forest station of Bhubaneswar were analyzed for their chemical composition. The samples were collected through a wet-only (WO) collector and two bulk (B1 and B2) collectors. The ions were evenly balanced indicating good data quality. The overall pH of rainwater was slightly acidic and ~47% of all rain events during the period were acidic (pH?<?5.6). Multilinear regression analysis showed relation between the free acidity (H+) and other components in rainwater. Enrichment factors (EF) of the major components with respect to their sources such as marine and crustal were calculated. Maximum EF was observed for NO 3 ? for both marine and crustal sources for all the three collectors. Source apportionments were also carried for the ions. Trend analysis showed continuous increase in most of the ions over years during the study period driven by anthropogenic emissions. Statistical/factorial analysis established correlation among different ions.  相似文献   

19.
To investigate ocean variability during the last millennium in the Western Gulf of Maine (GOM), we collected a 142-year-old living bivalve (Arctica islandica L.) in 2004, and three fossil A. islandica shells (calibrated 14CAMS = 1030 ± 78 ad; 1320 ± 45 ad; 1357 ± 40 ad) for stable isotope and growth increment analysis. A statistically significant relationship exists between modern GOM temperature records [shell isotope-derived (30 m) (r = ?0.79; P < 0.007), Prince 5 (50 m) (r = ?0.72; P < 0.019), Boothbay Harbor SST (r = ?0.76; P < 0.011)], and Labrador Current (LC) transport data from the Eastern Newfoundland Slope during 1993–2003. In all cases, as LC transport increased, GOM water temperatures decreased the following year. Decadal trends in the North Atlantic Oscillation (NAO) and the Atlantic Multidecadal Oscillation (AMO) influence GOM water temperatures in the most recent period, with water temperatures decreasing during NAO and AMO negative modes most likely linked to LC transport and Gulf Stream interaction. Mean shell-derived isotopic changes (δ18Oc) during the last 1,000 years were +0.47‰ and likely reflect a 1–2°C cooling from 1000 ad to present. Based on these results, we suggest that observed cooling in the GOM during the last millennium was due to increased transport and/or cooling of the LC, and decreased Gulf Stream influence on the GOM.  相似文献   

20.
This paper addresses the relation between the net-radiation (Q *) and the ground heat flux (Q G), the energy stored in the soil ( $\Updelta Q_{\rm S}$ ), and the residual of the energy partition (R = Q * ? Q H  ? Q E ) of urban and suburban areas of Oklahoma City, USA. These three forms of energy were observed or estimated from observations taken during Joint Urban 2003 Campaign. The database includes net-radiation, soil temperature, ground heat flux, and turbulent fluxes. In most cases the estimates of the energy stored in the soil were obtained by assuming roughly a certain type of soil and an effective soil depth. From the residuals it seems to be possible to distinguish the urban boundary layer from the suburban boundary layer when plotted as a function of net-radiation. Hysteresis coefficients were computed for fits of net-radiation against R, $\Updelta Q_{\rm S}$ and Q G. In particular, the hysteresis patterns show that Q * vs. R represents clearer urban areas or suburban areas under the influence of an urban “plume”. On the other hand, hysteresis curves obtained from $\Updelta Q_{\rm S}$ or Q G account for better the ground composition. A possible consequence is that the land use of urban areas could be roughly inferred from curve shapes such as Q * vs. R, or Q * versus another input variable representing the storage term. The objective is to show the variability of the subsurface-related energy fluxes across an urban area using these three different quantities and also to show that $\Updelta Q_{\rm S}, \,Q_{\rm G}$ , or R (and their corresponding hysteresis curves) are likely to be quantitatively different, which have not been clearly stated in the literature.  相似文献   

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