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1.
A growing body of research suggests that the marine environments of south Florida provide a critical link between the tropical and high-latitude Atlantic. Changes in the characteristics of water masses off south Florida may therefore have important implications for our understanding of climatic and oceanographic variability over a broad spatial scale; however, the sources of variability within this oceanic corridor remain poorly understood. Measurements of ΔR, the local offset of the radiocarbon reservoir age, from shallow-water marine environments can serve as a powerful tracer of water-mass sources that can be used to reconstruct variability in local-to regional-scale oceanography and hydrology. We combined radiocarbon and U-series measurements of Holocene-aged corals from the shallow-water environments of the Florida Keys reef tract (FKRT) with robust statistical modeling to quantify the millennial-scale variability in ΔR at locations with (“nearshore”) and without (“open ocean”) substantial terrestrial influence. Our reconstructions demonstrate that there was significant spatial and temporal variability in ΔR on the FKRT during the Holocene. Whereas ΔR was similar throughout the region after ∼4000 years ago, nearshore ΔR was significantly higher than in the open ocean during the middle Holocene. We suggest that the elevated nearshore ΔR from ∼8000 to 5000 years ago was most likely the result of greater groundwater influence associated with lower sea level at this time. In the open ocean, which would have been isolated from the influence of groundwater, ΔR was lowest ∼7000 years ago, and was highest ∼3000 years ago. We evaluated our open-ocean model of ΔR variability against records of local-to regional-scale oceanography and conclude that local upwelling was not a significant driver of open-ocean radiocarbon variability in this region. Instead, the millennial-scale trends in open-ocean ΔR were more likely a result of broader-scale changes in western Atlantic circulation associated with an increase in the supply of equatorial South Atlantic water to the Caribbean and shifts in the character of South Atlantic waters resulting from variation in the intensity of upwelling off the southwest coast of Africa. Because accurate estimates of ΔR are critical to precise calibrations of radiocarbon dates from marine samples, we also developed models of nearshore and open-ocean ΔR versus conventional 14C ages that can be used for regional radiocarbon calibrations for the Holocene. Our study provides new insights into the patterns and drivers of oceanographic and hydrologic variability in the Straits of Florida and highlights the value of the paleoceanographic records from south Florida to our understanding of Holocene changes in climate and ocean circulation throughout the Atlantic.  相似文献   

2.
From the last deglaciation to the Holocene, the Greenland Ice Core (GISP2) δ 18O records as well as the records of ice-rafted debris on the surface of the North Atlantic have revealed a succession of sudden cooling events on the centennial to millennial scales. However, the temperature proxy records are rarely studied systematically and directly to ensure that this air temperature cooling pattern simultaneously existed in the East Asian Region, in addition to the repeated pattern occurring in the Greater Atlantic Region. A peat cellulose δ 18O temperature proxy record proximately existing for 14000 years was picked up from the Hani peat in Jilin Province, China. It suggests by comparison that the sudden cooling events, such as the Older Dryas, Inter-Allerød, Younger Dryas, and nine ice-rafted debris events of the North Atlantic, are almost entirely reiterated in the temperature signals of Hani peat cellulose δ 18O. These cooling events show that the repeatedly occurring temperature cooling pattern not only appeared in the North Atlantic Region in the high latitudes, but also in the Northwest Pacific Region in the middle latitudes. The climate change events marking the start of the Holocene Epoch, the Holocene Megathermal, the “8.2 kyr” event, the “4.2 kyr” event, the Medieval Warm Period, and the Little Ice Age are further discussed. The sensitivity response of Hani peat cellulose δ 18O to the land surface temperature and the reason for the age accuracy of peat cellulose 14C are also discussed based on the characteristics of the peat bog environment.  相似文献   

3.
High resolution benthic foraminiferal stable isotopes (δ18O, δ13C) and molecular biomarkers in the sediments are used here to infer rapid climatic changes for the last 8200 years in the Ría de Muros (NW Iberian Margin). Benthic foraminiferal δ18O and δ13C potentially register migrations in the position of the hydrographic front formed between two different intermediate water masses: Eastern North Atlantic Central Water of subpolar origin (ENACWsp) and subtropical origin (ENACWst). The molecular biomarkers in the sediment show a strong coupling between continental organic matter inputs and negative δ13C values in benthic foraminifera. The rapid centennial and millennial events registered in these records have been compared with two well known North Atlantic Holocene records from the subtropical Atlantic sea surface temperatures (SST) anomalies off Cape Blanc, NW Africa and the subpolar Atlantic (Hematite Stained Grains percentage, subpolar North Atlantic). Comparison supports a strong link between high- and low-latitude climatic perturbations at centennial–millennial time scales during the Holocene. Spectral analyses also points to a pole-to-equator propagation of the so-called 1500 yr cycles. Our results demonstrate that during the Holocene, the NW Iberian Margin has undergone a series of rapid events which are likely triggered at high latitudes in the North Atlantic and are rapidly propagated towards lower latitudes. Conceivably, the propagation of these rapid climatic changes involves a shift in atmospheric and oceanic circulatory systems.  相似文献   

4.
The behavior of electric- and magnetic-field variations over the British Isles region is studied using a scaled laboratory analogue model. The model source frequencies used simulate periods of 20 min to 2 h in the geophysical scale. The results indicate that conductive channelling of induced electric current by the English Channel is important for both E- and H-polarization, while channelling through the North Channel, the Irish Sea, and the North Sea is particularly important for the E-polarization. The funnel shape of the North Sea, leading to the relatively narrow English Channel, results in diffusion of current into the continent and the east coast of the British Isles, contributing to highly frequency-dependent horizontal electric- and vertical magnetic-field coastal anomalies. The model results also give ample evidence of current deflection at the complex coastlines.The model results for simulated 12 h period variations indicate vertical magnetic-field values changing by as much as a factor of five or six between certain coastal locations, and at least by a factor of two or three between interior locations. The horizontal electric- and magnetic-field components also show almost equally large changes, with particularly large enhancements near narrow ocean channels and irregular coastlines, responding to channelled and deflected current. With the relatively close proximity of the coasts for essentially all locations on the British Isles, the coast effects associated with the very complex coastlines can be expected to play a major role in the behavior of the electromagnetic fields over the British Isles.  相似文献   

5.
The calibration of marine 14C dates requires the incorporation of regionally specific marine reservoir offsets known as ΔR, essential for accurate and meaningful inter-archive comparisons. Revised, regional ΔR (‘ΔRR’) values for the Barents Sea are presented for molluscs and cetaceans for the two latest iterations of the marine calibration curve, based on previously published pre-bomb live-collected and radiocarbon-dated samples (‘ΔRL’; molluscs: n = 16; cetaceans: n = 18). Molluscan ΔRR, determined for four broad regional oceanographic settings, are: western Svalbard (including Bjørnøya), −61 ± 37 14C yrs (Marine20), 94 ± 38 14C yrs (Marine13); Franz Josef Land, −277 ± 57 14C yrs (Marine20), −122 ± 38 14C yrs (Marine13); Novaya Zemlya, −156 ± 73 14C yrs (Marine20), 0 ± 76 14C yrs (Marine13); northern Norway, −86 ± 39 14C yrs (Marine20), 74 ± 24 14C yrs (Marine13). Molluscan ΔRR values are considered applicable to other marine carbonate materials (e.g., foraminifera, ostracods). Cetacean ΔRR are determined for toothed (n = 10) and baleen (n = 8) whales, and a combined toothed-baleen group (n = 18): toothed, −161 ± 41 14C yrs (Marine20), 1 ± 41 14C yrs (Marine13); baleen, −158 ± 43 14C yrs (Marine20), 8 ± 41 14C yrs (Marine13); combined baleen-toothed whales, −160 ± 41 14C yrs (Marine20), 4 ± 49 14C yrs (Marine13). Where identification and separation of baleen and toothed whales is impossible the combined ΔRR term may be used. However, we explicitly discourage the application of existing cetacean ΔRR terms to other marine mammals. Our new ΔRR values are applicable for as long as those broad oceanographic conditions (circulation and ventilation) have persisted, i.e., through the Holocene. We recommend using the latest iteration of the marine calibration curve, Marine20, which seems to better capture the time-variant nature of R compared to Marine13. More ΔRL datapoints for both molluscs and cetaceans would improve the accuracy and precision of ΔRR. In the meantime, our new ΔR terms facilitate the calibration of marine 14C dates across the region, paving the way for meaningful and accurate late Quaternary histories and inter-regional comparisons.  相似文献   

6.
Data on the content of the 14C cosmogenic isotope in tree rings, which were obtained as a result of laboratory measurements, are often used when solar activity (SA) is reconstructed for previous epochs, in which direct observations are absent. However, these data contain information not only about SA variations but also about changes in the Earth climatic parameters, such as the global temperature and the CO2 content in the Earth’s atmosphere. The effect of these variations on the 14C isotope content in different natural reservoirs after the last glacial termination to the middle of the Holocene is considered. The global temperature and the CO2 content increased on this time interval. In this case the 14C absolute content in the atmosphere increased on this time interval, even though the 14С to 12С isotope concentration ratio (as described by the Δ14С parameter) decreased. These variations in the radiocarbon absolute content can be caused by its redistribution between natural reservoirs. It has been indicated that such a redistribution is possible only when the rate of carbon exchange between the ocean and atmosphere depends on temperature. The values of the corresponding temperature coefficient for the 17–10 ka BC time interval, which make it possible to describe the carbon redistribution between the ocean and atmosphere, have been obtained.  相似文献   

7.
An algorithm based on simulated satellite signal calculated by the 6S radiative transfer model has been developed in order to retrieve the aerosol optical thickness of dust over the Atlantic ocean. The algorithm is applied to the visible channel of Geostationary Operational Environmental Satellite (GOES 8) images. The inversion uses a look-up table giving the satellite signal intensity as a function of surface albedo, viewing geometry, solar illumination and the optical properties of the aerosols. The study consists of assessing the feasibility of monitoring and mapping the transport of suspended particles across the Atlantic from the Sahara to the Caribbean. The study area is between 10 and 25 N and 30 and 65 W. The optical thickness of aerosols has been calculated over a period of 11 days between 10th and 20th of June 1997 for the 14:15 UT GOES image acquisition. The calculated aerosol optical thickness ranges from 0.0 to 0.81 with an important event of dust presence occurring between 13th and 16th of June. The retrieved aerosol optical thickness is in good agreement with the values obtained between 14h UT and 15h UT from ground based sun photometer measurements on the island of Guadeloupe, and a coefficient correlation (R2) of 0.88 has been found between the data sets.  相似文献   

8.
13C and ΣCO2 data from the North and South Atlantic, the Antarctic, and the North and South Pacific are given. The δ13C of the ΣCO2 in the deep water (～3000m) decreases from 1.7‰ in the North Atlantic to ?0.10‰ in the North Pacific. This change is attributed to the addition of about 158 μmoles of CO2 per kg of seawater. The in-situ oxidation of organic matter accounts for 83% of this increase in ΣCO2, while the remainder is attributed to dissolution of calcium carbonate.The δ13C of the dissolved CO2 in mid-latitude surface water samples is controlled by a quasi-steady-state equilibrium with atmospheric CO2 at a mean temperature of 16°C. The δ13C and ΣCO2 values of Antarctic surface water samples suggest that these waters are derived from a mixture of North Atlantic deep water and equilibrated surface water.  相似文献   

9.
New data for the direct measurement of the isotopic composition of neodymium in Atlantic Ocean seawater are compared with previous measurements of Pacific Ocean seawater and ferromanganese sediments from major ocean basins. Data for Atlantic seawater are in excellent agreement with Nd isotopic measurements made on Atlantic ferromanganese sediments and are distinctly different from the observed compositions of Pacific samples. These results clearly demonstrate the existence of distinctive differences in the isotopic composition of Nd in the waters of the major ocean basins and are characteristic of the ocean basin sampled. The average εNd(0) values for the major oceans as determined by data from seawater and ferromanganese sediments are as follows: Atlantic Ocean,εNd(0) ? ?12 ± 2; Indian Ocean,εNd(0) ? ?8 ± 2; Pacific Ocean,εNd(0) ? ?3 ± 2. These values are considerably less than εNd(0) value sources with oceanic mantle affinities indicating that the REE in the oceans are dominated by continental sources. The difference in the absolute abundance of143Nd between the Pacific and Atlantic Oceans corresponds to ～106 atoms143Nd per gram of seawater. The correspondence between the143Nd/144Nd in seawater and in the associated sediments suggests the possible application of this approach to paleo-oceanography.Distinctive differences in εNd(0) values are observed in the Atlantic Ocean between deep-ocean water associated with North Atlantic Deep Water and near-surface water. This suggests that North Atlantic Deep Water may be relatively well mixed with respect to Nd isotopic composition whereas near-surface water may be quite heterogeneous, reflecting different sources for surface waters relative to deep water. This suggests that it may be possible to distinguish the sources of water masses within an ocean basin on the basis of Nd isotopic composition.The Nd isotopic variations in seawater are used to relate the residence time of Nd and mixing rates between the oceans.  相似文献   

10.
A two-? ocean reservoir model is employed to examine the combined effects of vertical ocean circulation, organic matter extraction and cosmic ray production on the14C/12C in the atmosphere, ocean and sediment. In this model, dissolution of deep-sea calcium carbonate sediment is assumed to respond to the supply of particulate carbonate from the surface ocean and to the dissolved carbonate-ion concentration of the deep-sea.If the vertical ocean circulation decreased by 50% during the maximum rate of deglaciation, the atmospheric14C/12C would have increased concurrently by 10% relative to the pre-bomb present. Further, if cosmic ray production of14C was 50% greater than present at about 7800 years B.P. as suggested by archeomagnetic measurements, a double maximum of 10% occurs. The first is at about 10.5 ka and the second at 6.5 ka. This result is similar to the variation of14C/12C over the last 10,000 years calculated from the14C dates measured by Stuiver on the varved Lake of the Clouds. The result is not sensibly altered if 1017 moles of organic carbon is extracted from the ocean during sea-level rise.Reduction of the thermohaline ocean circulation by 50% over a one- to two-thousand-year interval would not be sensibly detected in the dating of deep-sea sediment. If Broecker's organic nutrient extraction occurs in conjunction with reduction of vertical circulation, a decrease in the atmospheric PCO2 will precede the eventual rise.  相似文献   

11.
Benthic foraminiferal oxygen and carbon isotopic records from Southern Ocean sediment cores show that during the last glacial period, the South Atlantic sector of the deep Southern Ocean filled to roughly 2500 m with water uniformly low in δ13C, resulting in the appearance of a strong mid-depth nutricline similar to those observed in glacial northern oceans. Concomitantly, deep water isotopic gradients developed between the Pacific and Atlantic sectors of the Southern Ocean; the δ13C of benthic foraminifera in Pacific sediments remained significantly higher than those in the Atlantic during the glacial episode. These two observations help to define the extent of what has become known as the ‘Southern Ocean low δ13C problem’. One explanation for this glacial distribution of δ13C calls upon surface productivity overprints or changes in the microhabitat of benthic foraminifera to lower glacial age δ13C values. We show here, however, that glacial-interglacial δ13C shifts are similarly large everywhere in the deep South Atlantic, regardless of productivity regime or sedimentary environment. Furthermore, the degree of isotopic decoupling between the Atlantic and Pacific basins is proportional to the magnitude of δ13C change in the Atlantic on all time scales. Thus, we conclude that the profoundly altered distribution of δ13C in the glacial Southern Ocean is most likely the result of deep ocean circulation changes. While the characteristics of the Southern Ocean δ13C records clearly point to reduced North Atlantic Deep Water input during glacial periods, the basinal differences suggest that the mode of Southern Ocean deep water formation must have been altered as well.  相似文献   

12.
Radiocarbon data for 11 stations and tritium data for 16 stations in the North Atlantic Ocean from 74°N to 3°N are presented. For radiocarbon, normal errors inΔ14C are± 4‰, and in tritium,± 0.09TU or± 3%, whichever is larger. There is a remarkable, but not simply linear, correlation between oceanic bomb transients in14C and3H. The deep convective mixing in the Greenland Sea is reflected in substantial bomb tracer penetration to all depths, with residence time for the deep, cold core water that seems to be 20 to 30 years. The outflow in the bottom layer southward over the sills of the Denmark Strait and Faroe Passage carries significant tritium concentration, at least to 40°N. Complicated, but coherent, profile structures in the subtropical Atlantic suggest effects of large-scale lateral advection. In particular, a pronounced minimum in both14C and3H might be associated with the Antarctic intermediate water.  相似文献   

13.
《水文科学杂志》2013,58(3):602-617
Abstract

The main areas of net moisture uptake are examined in air masses over the Orinoco River basin, located in equatorial South America, north of the Amazon basin. Although the Orinoco River has the third largest average annual discharge in the world (with 5.4 × 1011 m3 year?1 draining into the Atlantic Ocean), the sources of moisture that feed it have not previously been studied in any detail. The results are presented from analyses of back-tracking of all the air masses over the Orinoco basin over a period of five years (2000–2004) using the diagnostic Lagrangian tool FLEXPART. The input data for the model were obtained from the European Centre for Medium-range Weather Forecasts (ECMWF). Air transported into the Orinoco basin experiences a large uptake of water over the tropical North Atlantic within the three days prior to its arrival over the basin. The Tropical South Atlantic and the eastern coast of the Pacific become significant moisture sources for about 5–10 days before arriving over the Orinoco basin. Contrary to what might be expected, large areas of the Amazon basin, along with the Gulf of Mexico, do not provide significant moisture to the study area. Interestingly, over these zones the air experiences net moisture loss. Preliminary analysis of the processes that occur leads to the conclusion that most of the water observed over the Orinoco basin derives from advective fluxes into the area, while recycling of moisture is negligible.  相似文献   

14.
Coastal and oceanic SST variability along the western Iberian Peninsula   总被引：1，自引：0，他引：1  
The inter-annual variability of the sea surface temperature (SST) was analyzed along the western Iberian Peninsula in the region ranging from 9.5 °W to 21.5 °W and from 37.5 °N to 42.5 °N with a spatial resolution of 1°×1° from 1900 to 2008. Both coastal and oceanic SST showed an overall increase with warming and cooling cycles similar to those observed in the North Atlantic region and in previous regional studies. In addition, the evolution of coastal and ocean water has been observed to be different. In general, ocean water is more affected by the different warming–cooling cycles than coastal water. In spite of coast and ocean are highly influenced by global changes affecting the whole North Atlantic region, near shore SST has been observed to be correlated with local wind regime, which is itself a manifestation of the Eastern Atlantic (EA) teleconnection pattern.  相似文献   

15.
The Milankovi theory stresses that the summer insolation in the high northern latitudes that is dominated by the precession cycle controls the glacial/interglacial cycles in global climate change.If the climate system responds linearly to the external insolation forcing,the precession cycle of 23 or 19 ka should dominate the variations in the climatic proxy records.I performed spectral and evolutive cross spectral analyses on the high resolution benthic 18O and 13C records from the South China Sea and the North Atlantic,the proxies of global ice volume and ocean carbon reservoir respectively.I found that the obliquity instead of the eccentricity or the precession is the most marked cycle in the global ice volume and ocean carbon reservoir variations over the past 5 Ma.The analysis further reveals that only at the obliquity band instead of the eccentricity or the precession band does the global ice volume and ocean carbon reservoir display consistently high coherency and stable phase relationship over the past 5 Ma.The consistently positive or near-zero phases of the benthic 18O relative to the benthic13C at the obliquity band suggest that the global carbon cycle is involved in the polar ice sheet growth as an important internal feedback,not a determinative driving factor.The obliquity instead of the precession or the eccentricity takes the dominant role of driving the global climate change during the Pliocene and Pleistocene.  相似文献   

16.
This study utilizes a combined stable isotope and 14C dating approach to determine the radiocarbon reservoir age correction, ΔR, for the James River, Virginia estuary from 17th century Crassostrea virginica shells of known collection dates. ΔR, which can vary spatially and temporally, is a locality-specific adjustment applied to the global ocean reservoir, R, to further account for the offset between the atmospheric and marine 14C calibration curves. To assess the temporal variability in ΔR, continuous δ18O sampling along the oyster shell hinge provides a seasonal record throughout the oyster's life. This is then used to identify sampling locations for 14C measurements based on calcite precipitated during the Summer (>19 °C) and Fall through Spring (F-Sp, <15 °C) months. The resulting seasonal ΔR values range from −151 ± 46 to +109 ± 55 14C years (260 years) due to changes in the contribution and age of dissolved inorganic carbon (DIC) from marine and freshwater sources in the James River estuary. The F-Sp samples display a larger ΔR range than the Summer samples, as do the shells precipitated during drought conditions (1606–1612) when compared to shells from the remainder of the 17th century. The largest intrashell ΔR variability, 195 14C years, is similarly found in a drought shell and is attributed to variability caused by the extreme regional 1606–1612 drought. Early land use changes related to European development and farming practices also altered the age of DIC in the James River estuary. We estimate that the soil inorganic carbon (SIC) contributing to freshwater DIC ranged from 0 to ∼1800 years old and reflected both the drought and land use changes that occurred during the 17th century. Using only the Summer samples, which represent the majority of shell calcite, we obtain a mean ΔR = −32 ± 11 14C years (1σ) for 17th century James River estuary ΔR at the very onset of European colonization. Employing a seasonally resolved sampling method will provide the greatest constraint on 14C measurements in an estuarine environment where multiple carbon sources can fluctuate on seasonal timescales and as a result of large scale environmental change.  相似文献   

17.
A flight of Holocene marine terraces on the southwestern coast of Cape Omaezaki of central Japan provides evidence of recurrent millennium‐scale uplift events. We reconstructed the uplift history of these terraces by using facies analysis of drill core and geoslicer samples, environmental analysis of trace fossils, and 14C age determinations. Coastal uplift can be identified by the displacement of beach deposits such as foreshore deposits, which represent the intertidal swash zone of a wave‐dominated sandy coast. Three levels of former beach deposits facing the Nankai Trough were identified near the coast in the Omaezaki area. The highest of these, dated at about 3020–2880 BC, records a maximum of 2.2–2.7 m of emergence. The middle beach surface, of minimum age 370–190 BC, shows 1.6–2.8 m of emergence. The lowest beach surface, which is older than 1300–1370 AD, records 0.4–1.6 m of emergence. Our analysis of vertical crustal deformation data during the Holocene in this region suggests that rapid and strong uplift was restricted to the southwestern coast of the Omaezaki area and was probably caused by high‐angle thrusting on subsidiary faults branching from the underlying plate boundary megathrust.  相似文献   

18.
We present a new speleothem record of atmospheric Δ14C between 28 and 44 ka that offers considerable promise for resolving some of the uncertainty associated with existing radiocarbon calibration curves for this time period. The record is based on a comprehensive suite of AMS 14C ages, using new low-blank protocols, and U–Th ages using high precision MC-ICPMS procedures. Atmospheric Δ14C was calculated by correcting 14C ages with a constant dead carbon fraction (DCF) of 22.7 ± 5.9%, based on a comparison of stalagmite 14C ages with the IntCal04 (Reimer et al., 2004) calibration curve between 15 and 11 ka. The new Δ14C speleothem record shows similar structure and amplitude to that derived from Cariaco Basin foraminifera (Hughen et al., 2004, 2006), and the match is further improved if the latter is tied to the most recent Greenland ice core chronology (Svensson et al., 2008). These data are however in conflict with a previously published 14C data set for a stalagmite record from the Bahamas — GB-89-24-1 (Beck et al., 2001), which likely suffered from 14C analytical blank subtraction issues in the older part of the record. The new Bahamas speleothem ?14C data do not show the extreme shifts between 44 and 40 ka reported in the previous study (Beck et al., 2001). Causes for the observed structure in derived atmospheric Δ14C variation based on the new speleothem data are investigated with a suite of simulations using an earth system model of intermediate complexity. Data-model comparison indicates that major fluctuations in atmospheric ?14C during marine isotope stage 3 is primarily a function of changes in geomagnetic field intensity, although ocean–atmosphere system reorganisation also played a supporting role.  相似文献   

19.
Concentrations of lead were measured in a surface transect and at two vertical profile stations (15°N and 20°S) in the Central Pacific. These measurements complement similar measurements made earlier in the North Pacific at 33°N and in the Northwest Atlantic at 34°N [1,2], as well as recent measurements of eolian lead input fluxes near each of these locations [3]. The new transect of surface water concentrations of lead corroborates previous measurements, which decrease from 13 ng/kg at 30°N to 4 ng/kg at 17°S in the Central Pacific [4]. This transect gradient is shown to overlie a similar geographic gradient of subsurface maximum concentrations of lead in the three Pacific vertical profile stations, decreasing from 14 ng/kg at 33°N to 11 ng/kg at 14°N to 2.5 ng/kg at 20°S. Lead concentrations at each of those locations exhibit maxima at 400 m, decreasing concentrations to 2500 m and approximately concentrations of 0.8–1.1 ng/kg below that depth. The subsurface maximum at the northwest Atlantic profile station (36 ng/kg at 34°N) is also congruent with surface water lead concentrations which decrease from 806 ng/kg to 32 ng/kg in an offshore transect from Rhode Island to 34°N, 66°W [5], and the shape of the Atlantic profile is congruent with those in the Pacific. There is a positive correlation between the magnitudes of eolian lead input fluxes and the magnitudes of the upper water maxima in lead concentration profiles at corresponding locations as follows: South Pacific easterlies 3 ng/cm2 yr vs. 2.5 ng/kg; North Pacific easterlies 6 ng/cm2 yr vs. 11 ng/kg; North Pacific westerlies 50 ng/cm2 yr vs. 14 ng/kg; and North Atlantic westerlies 170 ng/cm2 yr vs. 36 ng/kg.This relationship enables one to view the anthropogenic perturbations of the marine lead cycle on a global scale, since the industrial origin of eolian and seawater lead has been established by correlations between geographic patterns of industrial lead emissions to the atmosphere and isotopic ratios of industrial leads [3] and by geographic patterns of Pb/silicate-dust ratios and lead isotopic ratios in ocean surface waters [3–5]. These new data coupled with earlier biogeochemical data indicate that surface water concentrations of lead in the North Pacific and North Atlantic are now conservatively estimated to be 8 to 20-fold greater and those in the South Pacific are 2-fold greater than natural concentrations because of industrial emissions of lead to the atmosphere.  相似文献   

20.
A sediment core from the western tropical Atlantic covering the last 21,000 yr has been analysed for centennial scale reconstruction of sea surface temperature (SST) and ice volume-corrected oxygen isotopic composition of sea water (δ18Oivc-sw) using Mg / Ca and δ18O of the shallow dwelling planktonic foraminifer Globigerinoides ruber (white). At a period between 15.5 and 17.5 kyr BP, the Mg / Ca SST and δ18Oivc-sw, a proxy for sea surface salinity (SSS), reveals a warming of around 2.5 °C along with an increase in salinity. A second period of pronounced warming and SSS increase occurred between 11.6 and 13.5 kyr BP. Within age model uncertainties, both warming intervals were synchronous with air temperature increase over Antarctica and ice retreat in the southern South Atlantic and terminated with abrupt centennial scale SSS decrease and slight SST cooling in conjunction with interglacial reactivation of the meridional overturning circulation (MOC). We suggest that during these warm intervals, production of saline and warm water of the North Brazil Current resulted in pronounced heat and salt accumulation, and was associated with warming in the southern Atlantic, southward displacement of the intertropical convergence zone and weakened MOC. At the termination of the Younger Dryas and Heinrich event 1, intensification of cross-equatorial heat and salt transport caused centennial scale cooling and freshening of the western tropical Atlantic surface water. This study shows that the western tropical Atlantic served as a heat and salt reservoir during deglaciation. The sudden release of accumulated heat and salt at the end of Younger Drays and Heinrich event 1 may have contributed to the rapid reinvigoration of the Atlantic MOC.  相似文献   

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